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DOE OSTI2023

Prospects for annihilating dark matter from M31 and M33 observations with the Cherenkov Telescope Array

M31 and M33 are the closest spiral galaxies and the largest members (together with the Milky Way) of the Local group, which makes them interesting targets for indirect dark matter searches. In this paper we present studies of the expected sensitivity of the Cherenkov Telescope Array (CTA) to an annihilation signal from weakly interacting massive particles from M31 and M33. Here, we show that a 100 h long observation campaign will allow CTA to probe annihilation cross-sections up to <συ> ≈ 5•10 -25 cm 3 s -1 for the τ + τ - annihilation channel (for M31, at a DM mass of 0.3 TeV), improving the current limits derived by HAWC by up to an order of magnitude. We present an estimate of the expected CTA sensitivity, by also taking into account the contributions of the astrophysical background and other possible sources of systematic uncertainty. We also show that CTA might be able to detect the extended emission from the bulge of M31, detected at lower energies by the Fermi /LAT.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2020

Antideuterons and antihelium nuclei from annihilating dark matter

Recent studies of the cosmic-ray antiproton-to-proton ratio have identified an excess of ~10–20 GeV antiprotons relative to the predictions of standard astrophysical models. Intriguingly, the properties of this excess are consistent with the same range of dark matter models that can account for the long-standing excess of γ-rays observed from the Galactic Center. Such dark matter candidates can also produce significant fluxes of antideuterium and antihelium nuclei. In this work we study the production and transport of such particles, both from astrophysical processes as well as from dark matter annihilation. Importantly, in the case of AMS-02, we find that Alfvénic reacceleration (i.e., diffusion in momentum space) can boost the expected number of $\bar {\text d}$ and $^ {\text 3} \overline {\text {He}}$ events from annihilating dark matter by an order of magnitude or more. For relatively large values of the Alfvén speed, and for dark matter candidates that are capable of producing the antiproton and γ-ray excesses, we expect annihilations to produce a few antideuteron events and about one antihelium event in 6 yr of AMS-02 data. This is particularly interesting in light of recent reports from the AMS-02 Collaboration describing the detection of a number of antihelium candidate events.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2022

Search for GeV-scale dark matter annihilation in the Sun with IceCube DeepCore

The Sun provides an excellent target for studying spin-dependent dark matter-proton scattering due to its high matter density and abundant hydrogen content. Dark matter particles from the Galactic halo can elastically interact with Solar nuclei, resulting in their capture and thermalization in the Sun. The captured dark matter can annihilate into Standard Model particles including an observable flux of neutrinos. Here, we present the results of a search for low-energy (<500 GeV) neutrinos correlated with the direction of the Sun using 7 years of IceCube data. This work utilizes, for the first time, new optimized cuts to extend IceCube's sensitivity to dark matter mass down to 5 GeV. We find no significant detection of neutrinos from the Sun. Our observations exclude capture by spin-dependent dark matter-proton scattering with cross section down to a few times 10 -41 cm 2 , assuming there is equilibrium with annihilation into neutrinos/antineutrinos for dark matter masses between 5 GeV and 100 GeV. These are the strongest constraints at GeV energies for dark matter annihilation directly to neutrinos.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2025

First observation of antiproton annihilation at rest on argon in the LArIAT experiment

We report the first observation and measurement of antiproton annihilation at rest on argon track and shower multiplicities and particle identification conducted with the LArIAT experiment. Stopping antiprotons from the Fermilab Test Beam Facility’s charged particle test beam are identified using beamline instrumentation and LArIAT’s liquid argon time projection chamber (LArTPC). The charged particle multiplicity from the annihilation vertex is manually evaluated via hand scanning, yielding a mean of 3.2 ± 0.4 tracks and a standard deviation of 1.3 tracks, consistent with a semiautomated reconstruction resulting in 2.8 ± 0.4 tracks and a standard deviation of 1.2 tracks. Both methods are consistent with Monte Carlo simulations within statistical uncertainty. The shower multiplicities and particle identification for outgoing tracks are also consistent with eant4 model predictions. These results, obtained from a low-statistics sample, provide a foundation for higher-statistics studies in larger LArTPCs, which could refine modeling of intranuclear annihilation on argon and inform scenarios such as neutron-antineutron oscillations. Published by the American Physical Society 2025

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

Observation of Antiproton Annihilation at Rest in LArIAT

Antiproton annihilation at-rest can provide a unique probe into the intra-nuclear structure of nuclei. This process was first observed in the 1950’s using photographic emulsion and has since been observed and studied on a variety of nuclei. We present here the first observation and reconstruction of antiproton annihilation at-rest interactions on argon nuclei using data from the LArIAT experiment, a liquid argon time projection chamber (LArTPC). LArIAT was exposed to a charged particle test-beam at Fermilab from 2015-2017. Antiprotons tagged using LArIAT’s beamline instrumentation were reconstructed in the LArTPC, and the multiplicities of final-state particles emerging from the identified annihilation at-rest vertex were measured. These results will inform searches for neutron-antineutron oscillation events in the future LArTPCs like DUNE due to their similar topological signature.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2025

Evaluating the Potential to Constrain Dark Matter Annihilation with Fermi-LAT Observations of Ultrafaint Compact Stellar Systems

Recent results from numerical simulations and models of galaxy formation suggest that recently discovered ultrafaint compact stellar systems (UFCSs) in the halo of the Milky Way (MW) may be some of the smallest and faintest galaxies. If this is the case, these systems would be attractive targets for indirect searches of weakly interacting massive particle dark matter (DM) annihilation due to their relative proximity and high expected DM content. In this study, we analyze 14.3 yr of γ-ray data collected by the Fermi-Large Area Telescope coincident with 26 UFCSs. No significant excess γ-ray emission is detected, and we present γ-ray flux upper limits for these systems. Assuming that the UFCSs are DM-dominated galaxies consistent with being among the faintest and least massive MW dwarf spheroidal (dSph) satellite galaxies, we derive the projected sensitivity for a DM annihilation signal. We find that observations of UFCSs have the potential to yield some of the most powerful constraints on DM annihilation, with sensitivity comparable to observations of known dSphs and the Galactic center. This result emphasizes the importance of precise kinematic studies of UFCSs to empirically determine their DM content.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2020

Positron annihilation lifetime spectroscopy study of polyvinylpyrrolidone‐added polyvinylidene fluoride membranes: Investigation of free volume and permeation relationships

ABSTRACT Polyvinylidene fluoride (PVDF) membranes were prepared via the phase inversion method from casting solutions containing PVDF, dimethylformamide (DMF), and polyvinylpyrrolidone (PVP) as pore former. PVP was used in the casting solution in a range of 0–5 wt % and extracted. The effect on membranes of using PVP in the casting process was analyzed by X‐ray diffraction, differential scanning calorimetry, scanning electron microscopy, viscosity, and water permeability techniques. With an increase of PVP from 0 to 5 wt %, the PVDF casting solution viscosities increased from 858 to 1148 cP; the resulting PVDF membrane thickness increased; and the crystallinity of PVDF membranes decreased from 40.0 to 33.3%, which indicates that the addition of PVP inhibits the degree of crystallization in the PVDF membranes. SEM results revealed the shape and size of macropores in the membranes; these macropores changed after PVP addition to the casting solutions. The impact of structural changes on free‐volume properties was evaluated using positron annihilation lifetime spectroscopy (PALS) studies. PALS analysis indicated no effect on the average radius (~3.4 Å) of membrane free‐volume holes from the addition of PVP to the casting solution. However, the percentage of o ‐Ps pick‐off annihilation intensity, I 3 , increased from 1.7 to 5.1% with increased PVP content. Further, increasing the PVP content from 0.5 to 5% resulted in an increased final pure water permeability flux. For instance, the 210 min flux for a 14% PVDF + 0.5% PVP membrane was found to be 3.3 times greater than a control membrane having the same PVDF concentration. © 2020 Wiley Periodicals, Inc. J. Polym. Sci. 2020 , 58 , 589–598

Eren, Bilge↗
DOE OSTI2021

Defect Characterization Using Positron Annihilation Spectroscopy on Laser-Ablated Surfaces

In recent years, short, pulsed laser ablation has been gaining popularity for machining small-scale test geometries from bulk samples and for efficient serial sectioning. These laser-based techniques are being added to the toolbox in material science, which makes it necessary to understand the changes in the material that occur from the laser–material interaction. Positron annihilation spectroscopy is a unique, nondestructive technique to investigate small defects in materials difficult to investigate by other tools. In this work, Doppler broadening and positron lifetime annihilation spectroscopy are utilized to help quantify the damage in materials treated with short, pulsed lasers. Using a femtosecond laser on single crystal silicon, this manuscript shows that clusters of vacancy-like defects and small voids increase systematically with laser power. Lastly, the damage induced by the laser can also reach to micrometer depths.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Search for invisible decays of a dark photon using e + e – annihilation data at BESIII

We report a search for a dark photon using 14.9 fb –1 of e + e – annihilation data taken at center-of-mass energies from 4.13 to 4.60 GeV with the BESIII detector operated at the BEPCII storage ring. The dark photon is assumed to be produced in the radiative annihilation process of e + e – and to predominantly decay into light dark matter particles, which escape from the detector undetected. The mass range from 1.5 to 2.9 GeV is scanned for the dark photon candidate, and no significant signal is observed. The mass dependent upper limits at the 90% confidence level on the coupling strength parameter ϵ for a dark photon coupling with an ordinary photon vary between 1.6 x 10 –3 and 5.7 x 10 –3 .

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2024

Homomolecular Triplet–Triplet Annihilation in Metalloporphyrin Photosensitizers

Metalloporphyrins are ubiquitous in their applications as triplet photosensitizers, particularly for promoting sensitized photochemical upconversion processes. In this study, bimolecular excited state triplet–triplet quenching kinetics, termed homomolecular triplet–triplet annihilation (HTTA), exhibited by the traditional triplet photosensitizers–zinc(II) tetraphenylporphyrin (ZnTPP), palladium(II) octaethylporphyrin (PdOEP), platinum(II) octaethylporphyrin (PtOEP), and platinum(II) tetraphenyltetrabenzoporphyrin (PtTPBP)–were revealed using conventional transient absorption spectroscopy. Nickel(II) tetraphenylporphyrin was used as a control sample as it is known to be rapidly quenched intramolecularly through ligand-field state deactivation and, therefore, cannot result in triplet–triplet annihilation (TTA). The single wavelength transients associated with the metalloporphyrin triplet excited state decay–measured as a function of incident laser pulse energy in toluene–were well modeled using parallel first- and second-order kinetics, consistent with HTTA being operable. The combined transient kinetic data enabled the determination of the first-order rate constants (k T ) for excited triplet decay in ZnTPP (4.0 × 10 3 s –1 ), PdOEP (3.6 × 10 3 s –1 ), PtOEP (1.2 × 10 4 s –1 ), and PtTPBP (2.1 × 10 4 s –1 ) as well as the second-order rate constant (k TT ) for HTTA in ZnTPP (5.5 × 10 9 M –1 s –1 ), PdOEP (1.1 × 10 10 M –1 s –1 ), PtOEP (7.1 × 10 9 M –1 s –1 ), and PtTPBP (1.6 × 10 10 M –1 s –1 ). In most instances, triplet excited state extinction coefficients are either reported for the first time or have been revised using ultrafast transient absorption spectroscopy and singlet depletion: ZnTPP (78,000 M –1 cm –1 ) at 470 nm, PdOEP (67,000 M –1 cm –1 ) at 430 nm, PtOEP (51,000 M –1 cm –1 ) at 418 nm, and PtTPBP (100,000 M –1 cm –1 ) at 460 nm. Furthermore, the combined experimental results establish competitive time scales for homo- and heteromolecular TTA rate constants, implying the significance of considering HTTA processes in future research endeavors harnessing TTA photochemistry using common metalloporphyrin photosensitizers.

14 SOLAR ENERGY↗
DOE OSTI2025

Amplifying Magnetic Field Effects on Upconversion Emission via Molecular Qubit-Driven Triplet–Triplet Annihilation

Triplet-triplet annihilation (TTA) enables photon upconversion by combining two lower-energy triplet excitons to produce a higher-energy singlet exciton. This mechanism enhances light-harvesting efficiency for solar energy conversion and enables the use of lower-energy photons in bioimaging and photoredox catalysis applications. The magnetic modulation of such high-energy excitons presents an exciting opportunity to develop molecular quantum information technologies. While the spin dynamics of triplet exciton pairs are sensitive to external magnetic fields, the magnetic field effects (MFEs) associated with these pairs are generally limited by spin statistics to at most 10% at low fields (<1 Tesla), making them challenging to apply in technological advancements. In contrast, MFEs on spin-correlated radical pairs (SCRPs) can be significantly greater, surpassing those on triplet pairs. By using SCRPs-based molecular qubits as triplet sensitizers in the sensitized TTA scheme, we can magnetically modulate TTA and consequently, the delayed fluorescence of annihilators. In our current system, we have achieved more than 70% magnetic modulation of delayed fluorescence, effectively harnessing and even amplifying magnetic modulation within SCRPs to influence high-energy excitons. In conclusion, this work opens new opportunities for advancing spin-controlled chemical reactions and molecular quantum information technologies.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2021

Velocity-dependent J-factors for annihilation radiation from cosmological simulations

Abstract We determine the dark matter pair-wise relative velocity distribution in a set of Milky Way-like halos in the Auriga and APOSTLE simulations. Focusing on the smooth halo component, the relative velocity distribution is well-described by a Maxwell-Boltzmann distribution over nearly all radii in the halo. We explore the implications for velocity-dependent dark matter annihilation, focusing on four models which scale as different powers of the relative velocity: Sommerfeld, s-wave, p-wave, and d-wave models. We show that the J-factors scale as the moments of the relative velocity distribution, and that the halo-to-halo scatter is largest for d-wave, and smallest for Sommerfeld models. The J-factor is strongly correlated with the dark matter density in the halo, and is very weakly correlated with the velocity dispersion. This implies that if the dark matter density in the Milky Way can be robustly determined, one can accurately predict the dark matter annihilation signal, without the need to identify the dark matter velocity distribution in the Galaxy.

Astronomy & Astrophysics↗
DOE OSTI2025

Neutrino and gamma-ray signatures of inelastic dark matter annihilating outside neutron stars

We present a new inelastic dark matter search: neutron stars in dark matter-rich environments capture inelastic dark matter which, for interstate mass splittings between about 45 - 285 MeV, will annihilate away before becoming fully trapped inside the object. This means a sizable fraction of the dark matter particles can annihilate while being outsidethe neutron star, producing neutron star-focused gamma-rays and neutrinos. We analyze this effect for the first time and target the neutron star population in the Galactic Center, where the large dark matter and neutron star content makes this signal most significant. Depending on the assumed neutron star and dark matter distributions, we set constraints on the dark matter-nucleon inelastic cross-section using existing H.E.S.S. observations. We also forecast the sensitivity of upcoming gamma-ray and neutrino telescopes to this signal, which can reach inelastic cross-sections as low as ∼ 2 × 10 -47 cm 2 .

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2026

Energy-energy correlators in 𝑒 + ⁢𝑒 − annihilation and deep inelastic scattering

We study energy-energy correlators (EECs) in 𝑒 + ⁢𝑒 − annihilation and deep inelastic lepton-hadron scattering (DIS), focusing on aspects of nonperturbative physics in these observables. We introduce the EEC jet functions and investigate the infrared behavior of both small-angle EECs and angle-integrated EECs by performing explicit one-loop calculations. The factorization and universality of the EECs in these processes are demonstrated. A matching scheme is proposed to smoothly connect kinematic regions where different scaling behaviors with jet energy are observed. In combination with the next-to-leading order correction, this matching provides a good description of the EEC data and pythia simulations in high-energy 𝑒 + ⁢𝑒 − annihilation. Predictions for DIS processes for future electron-ion collider kinematics are also presented.

Guo, Yuxun [Lawrence Berkeley National Laboratory ↗
DOE OSTI2020

Role of weak interlayer coupling in ultrafast exciton-exciton annihilation in two-dimensional rhenium dichalcogenides

Strong interactions between excitons are a characteristic feature of two-dimensional (2D) semiconductors, determining important excitonic properties, such as exciton lifetime, coherence, and photon-emission efficiency. Rhenium disulfide (ReS 2 ), a member of the 2D transition-metal dichalcogenide (TMD) family, has recently attracted great attention due to its unique excitons that exhibit excellent polarization selectivity and coherence features. However, an in-depth understanding of exciton-exciton interactions in ReS 2 is still lacking. In this work, we used ultrafast pump-probe spectroscopy to study exciton-exciton interactions in monolayer (1L), bilayer (2L), and triple layer ReS 2 . Additionally, we directly measure the rate of exciton-exciton annihilation, a representative Auger-type interaction between excitons. It decreases with increasing layer number, as observed in other 2D TMDs. However, while other TMDs exhibit a sharp weakening of exciton-exciton annihilation between 1L and 2L, such behavior was not observed in ReS 2 . We attribute this distinct feature in ReS 2 to the relatively weak interlayer coupling, which prohibits a substantial change in the electronic structure when the thickness varies. This work not only highlights the unique excitonic properties of ReS 2 but also provides novel insight into the thickness dependence of exciton-exciton interactions in 2D systems.

36 MATERIALS SCIENCE↗
DOE OSTI2021

Study of the decay D s + → π + π + π - η and observation of the W -annihilation decay D s + → a 0 ( 980 ) + ρ 0

The decay $D^+_s$ → $π^+π^+π^-η$ is observed for the first time, using e + e - collision data corresponding to an integrated luminosity of 6.32 fb -1 collected by the BESIII detector at center-of-mass energies between 4.178 and 4.226 GeV. The absolute branching fraction for this decay is measured to be $\mathscr{B}$($D^+_s$ → $π^+π^+π^-η$) = (3.12 ± 0.13 stat ± 0.90 syst )%. The first amplitude analysis of this decay reveals the substructures in $D^+_s$ → $π^+π^+π^-η$ nd determines the relative fractions and the phases among these substructures. The dominant intermediate process is $D^+_s$ → $a_1$(1260) + $η,a_1$(1260) + → ρ(770) 0 $π^+$ with a branching fraction of (1.73 ± 0.14 stat ±0.08 syst )%. We also observe the W-annihilation process $D^+_s$ → $a_0$(980) + ρ(770) 0 , $a_0$(980) + → $π^+η$ with a branching fraction of (0.21 ± 0.08 stat ± 0.05 syst )%, which is larger than the branching fractions of other measured pure W-annihilation decays by 1 order of magnitude.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

CTA and SWGO can discover Higgsino dark matter annihilation

Thermal Higgsino dark matter (DM), with a mass near 1.1 TeV, is one of the most well-motivated and untested DM candidates. Leveraging recent hydrodynamic cosmological simulations that give DM density profiles in Milky Way analog galaxies we show that the linelike gamma-ray signal predicted from Higgsino annihilation in the Galactic Center could be detected at high significance with the upcoming Cherenkov Telescope Array (CTA) and Southern Wide-field Gamma-ray Observatory (SWGO) for all but the most pessimistic DM profiles. We perform the most sensitive search to-date for the linelike signal using 15 years of data from the Fermi Large Area Telescope, coming within an order one factor of the necessary sensitivity to detect the Higgsino for some Milky Way analog DM density profiles. We show that H.E.S.S. has subleading sensitivity relative to Fermi for the Higgsino at present. In contrast, we analyze H.E.S.S. inner Galaxy data for the thermal wino model with a mass near 2.8 TeV; we find no evidence for a DM signal and exclude the wino by over a factor of two in cross section for all DM profiles considered. In the process, we identify and attempt to correct what appears to be an inconsistency in previous H.E.S.S. inner Galaxy analyses for DM annihilation related to the analysis effective area, which may weaken the DM cross-section sensitivity claimed in those works by around an order of magnitude.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2024

High-energy neutrinos from millicharged dark matter annihilation in the Sun

Millicharged dark matter particles can be efficiently captured by the Sun, where they annihilate into tau leptons, leading to the production of high-energy neutrinos. In contrast to the Earth, the high temperature of the Sun suppresses the fraction of millicharged particles that are bound to nuclei, allowing for potentially high annihilation rates. We recast existing constraints from the IceCube Neutrino Observatory and use this information to place new limits on the fraction of the dark matter that is millicharged. This analysis excludes previously unexplored parameter space for masses of m χ ∼ ( 5 – 100 ) GeV , charges of q χ ∼ 10 − 3 – 10 − 2 , and fractional abundances as small as f DM ∼ 10 − 5 . Published by the American Physical Society 2024

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗