5g to 4f pionic transition in Th 232 and U 238
Th 232 and U 238 pionic X ray energies and widths, suggesting anomalous effect for interaction between high-Z nuclei and pion
SEARCH · Engineering Papers
Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.
Quote a phrase for an exact phrase match. Source license links do not imply unrestricted reuse.
Th 232 and U 238 pionic X ray energies and widths, suggesting anomalous effect for interaction between high-Z nuclei and pion
Apollo 11 lunar samples composition for Na 22, Al 26, Th and U, investigating positron activities
Lunar surface material age and post- crystallization from isotopic investigation of Apollo 11 samples of U-Th-Pb systematics
X ray energy measurements in 5g yields 4f pionic transitions of Th-232 and U-238
Apollo 12 lunar rock 12013 origin, determining age by U, Th and Pb isotopic study
Primordial radionuclides K, Th and U concentrations in Apollo 12 lunar rocks, breccias and fines, using gamma ray spectrometry
Age determination of Apollo 12 rocks by U-Th-Pb method
The following boulder samples are analyzed for U, Th, and Pb concentrations and for Pb isotopic compositions: 72275,53/matrix; 72275,73/matrix; 72275,81/dark rind, clast #1; 72275,117/white interior, clast #1; 72255,49/Civet Cat clast; 72255,54/light gray matrix; and 72255,67/dark gray matrix.
U, Th, and Pb concentrations and lead isotopic compositions of Apollo 16 samples are interpreted as follows: (1) an early period of lunar differentiation of either global or regional scale occurred about 4.47 b.y. ago; (2) the Imbrian impact event affected many Apollo 16 samples about 3.99 b.y. ago; (3) some Apollo 16 metaclastic rocks and breccias contain a large amount of KREEP-like material; (4) lead produced in the early history of the moon has been concentrated in lunar highland soils yielding high Pb-207/Pb-206 ratios corresponding to apparent ages of more than 4.8 b.y.; and (5) South Ray Crater soils reflect the approximately 2-b.y.-old event previously proposed for the Apollo 12 and 14 samples.
Portions of highland breccia boulder 7 collected during the Apollo 17 mission were studied using U-Th-Pb and Rb-Sr systematics. A Rb-Sr internal isochron age of 3.89 plus or minus 0.08 b.y. with an initial Sr-87/Sr-86 of 0.69926 plus or minus 0.00008 was obtained for clast 1 (77135,57) (a troctolitic microbreccia). A troctolitic portion of microbreccia clast 77215,37 yielded a U-Pb internal isochron of 3.8 plus or minus 0.2 b.y. and an initial Pb-206/Pb-207 of 0.69. These internal isochron ages are interpreted as reflecting metamorphic events, probably related to impacts, which reset Rb-Sr and U-Pb mineral systems of older rocks.
A Pb-Pb internal isochron for the Barwell L5-6 chondrite yields an age of 4.530 plus or minus 0.005 billion years, using the measured U-238/U-235 ratio of 135.24 plus or minus .17. If the terrestrial U isotope composition is used, an age of 4.559 billion years is obtained. The Pb isotopic composition is distinctly different from that of a terrestrial contaminant found in the fusion crust of the Barwell stone. When the U-Th-Pb data are plotted on the concordia diagram, the data define a line that intersects the concordia curve at approximately 4.53 and 0 billion years, and nearly all of the data plot above the concordia curve, regardless of the initial Pb correction. This discordancy and the Pb isotopic composition of the triolite are attributed to a recent reequilibration of Pb and not to terrestrial contamination.
Spectra of very highly charged ions of Au, Pb, Bi, Th, and U have been observed in laser-produced plasmas generated by the OMEGA laser. Line identifications in the region 9-110 A were made for ions in the Fe, Co, Cu, and Zn isoelectronic sequences. Comparison of the measured wavelengths of the Cu-like ions with values calculated with and without QED corrections shows that the inclusion of QED corrections greatly improves the accuracy of the calculated 4s-4p wavelengths. However, significant differences between the observed and calculated values remain.
The advantage of studying returned planetary samples cannot be overstated. A wider range of analytical techniques with higher sensitivities and accuracies can be applied to returned samples. Measurement of U-Th-Pb, Sm-Nd, Rb-Sr, and Lu-Hf isotopic systematics for chronology and isotopic tracer studies of planetary specimens cannot be done in situ with desirable precision. Returned Mars samples will be examined using all the physical, chemical, and geologic methods necessary to gain information on the origin and evolution of Mars. A returned Martian sample would provide ample information regarding the accretionary and evolutionary history of the Martian planetary body and possibly other planets of our solar system.
Results are presented on a detailed U-Th-Pb systematics of the Estherville mososiderite, which was performed in a study involving stepwise leaching experiments. The Pb-Pb internal 'isochrons' for Estherville yielded ages of 4556 + or - 35 Ma, 4506 + or - 75 Ma, and 4422 + or - 50 Ma, indicating that the silicate fraction of the Estherville mesosiderite is very heterogeneous and was formed early in the solar system history. Results clearly identifies the Pb-Pb isochron as a mixing line. The U-Pb lower-intercept ages could be divided into two groups: (1) around 3 Ga, and likely related to the 3.6 Ga heating event, and (2) close to 0 Ma and to 62 Ma.
The U-Th-Pb, Rb-Sr, and Sm-Nd isotopic systematics of four lightly leached residues of pristine, high-Mg, troctolitic cumulate 76535 were analyzed in order to determine their ages and magma sources. The data indicate that the cumulate was in isotopic equilibrium with a fluid or magma characterized by a high U-238/Pb-204 (mu) value of 600 at 4.236 Ga. Two and three stage Pb evolution calculations define even greater source mu values of about 1000, assuming low lunar initial mu values between 5 and 40 prior to about 4.43 Ga. These results are similar to mu values for KREEP sources and are also consistent with values from 78235, suggesting that at least some high-Mg suite rocks were derived from magma sources with high-mu values similar to KREEP, and support that idea that these rocks postdate primary lunar differentiation and formation of ferroan anorthosites.
U-Th disequilibrium analyses of the Naivasha basalts show a very small (U-238/Th-230) ratios which are lower than any previously analyzed basalts. The broadly positive internal isochron trend from one sample indicates that the basalts may have source heterogeneities, this is supported by earlier work. The Naivasha complex comprises a bimodal suite of basalts and rhyolites. The basalts are divided into two stratigraphic groups each of a transitional nature. The early basalt series (EBS) which were erupted prior to the Group 1 comendites and, the late basalt series (LBS) which erupted temporally between the Broad Acres and the Ololbutot centers. The basalts represent a very small percentage of the overall eruptive volume of material at Naivasha (less than 2 percent). The analyzed samples come from four stratigraphic units in close proximity around Ndabibi, Hell's Gate and Akira areas. The earliest units occur as vesicular flows from the Ndabibi plain. These basalts are olivine-plagioclase phyric with the associated hawaiites being sparsely plagioclase phyric. An absolute age of 0.5Ma was estimated for these basalts. The next youngest basalts flows occur as younger tuft cones in the Ndabibi area and are mainly olivine-plagioclase-clinopyroxcene phyric with one purely plagioclase phyric sample. The final phase of activity at Ndabibi resulted in much younger tuft cones consisting of air fall ashes and lapilli tufts. Many of these contain resorbed plagioclase phenocrysts with sample number 120c also being clinopyroxene phyric. The isotopic evidence for the basalt formation is summarized.
Positive correlations of (U-238/Th-230) versus Th show the rhyolites to be products of partial melting. Positive correlations of U and Cl and U and F show that the U enrichment in the rhyolites is associated with the halogen contents which may be related to the minor phenocryst phase fractionation. Instantaneous Th/U ratios exceed time integrated Th/U ratios providing further evidence of the hydrous nature of the Olkaria rhyolite source. Excess (U-238/Th-230) in the subduction related rocks has been associated to the preferential incorporation of uranium in slab derived fluids, but no evaluation of the size of this flux has been made. The majority of the Naivasha samples show a (U-238/Th-230) less than 1 and plot close to the subduction related samples indicating the Naivasha rhyolites may also have been influenced by fluids during their formation. In general samples with high (U-238/Th-230) ratios reflecting recent enrichment of uranium relative to thorium have high thorium contents, thereby the high (U-238/Th-230) ratios are restricted to the most incompatible element enriched magmas and, hence, are a good indication that the rhyolites were formed by partial melting. If a fluid phase had some influence on the formation of the rhyolites then the uranium and thorium may have some correlation with F and Cl contents which can be mirrored by the peralkalinity. Plots of uranium against F and Cl contents are shown. The positive correlation indicates that the uranium enrichments are associated with the halogen contents. There seems to be a greater correlation for U against Cl than F indicating that the U may be transported preferentially as Cl complexes.
Previously we have reported carbonate liq./silicate liq. partition coefficients (D) for a standard suite of trace elements (Nb, Mo, Ba, Ce, Pb, Th, and U) and Ra and Pa as well. In brief, we have found that immiscible liquid partitioning is a strong function of temperature. As the critical temperature of the carbonate-silicate solvus is approached, all partition coefficients approach unity. Additionally, for the overwhelming majority of the partitioning elements, InD is a linear function of 'ionic field strength,' z/r, where z is the charge of the partitioned cation and r is its ionic radius.