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At least 55 records · Page 3

Exploring New Diamond Surfaces with Precision Chemistry and Quantum Spectroscopy

Point defects in diamond known as color centers are a promising platform for quantum sensing. As atom-like systems, they can exhibit excellent spin coherence and can be manipulated with light. As solid-state defects, they can be produced at high densities and be incorporated into scalable devices. Diamond is a uniquely excellent host; it has a large band gap, can be synthesized with sub-ppb impurity concentrations, and can be isotopically purified to eliminate magnetic noise from nuclear spins. Specifically, the nitrogen vacancy (NV) center has been demonstrated to be a highly sensitive, non-invasive magnetic probe capable of resolving the magnetic field of a single electron spin with nanometer spatial resolution. However, the development of NV centers and other color centers in diamond as a quantum platform crucially relies on developing methods to functionalize and process diamond surfaces. Diamond is the hardest material, making polishing and processing challenging, and diamond surfaces are inert and sterically hindered, making them notoriously difficult to chemically terminate and functionalize. Our approach is to discover new surface chemistries for diamond by combining multimodal surface spectroscopy with NV-based quantum spectroscopy to carefully characterize the diamond surface. We have developed a suite of techniques for characterizing the diamond surface using rapid tools for reaction screening and detailed surface spectroscopy tools for definitive identification of the surface bonding.

36 MATERIALS SCIENCE↗

Asymptotic optimality of twist-untwist protocols for Heisenberg scaling in atom-based sensing

Twist-untwist protocols for quantum metrology consist of a serial application of (1) unitary nonlinear dynamics (e.g., spin squeezing or Kerr nonlinearity), (2) parameterized dynamics U ( φ ) (e.g., a collective rotation or phase space displacement), and (3) time reversed application of step 1. Such protocols are known to produce states that allow Heisenberg scaling for experimentally accessible estimators of φ even when the nonlinearities are applied for times much shorter than required to produce Schrödinger cat states. In this work, we prove that, asymptotically in the number of particles, twist-untwist protocols provide the lowest estimation error among quantum metrology protocols that utilize two calls to a weakly nonlinear evolution and a readout involving only first and second moments of a total spin operator n → · J → . We consider the following physical settings: all-to-all interactions generated by one-axis twisting J z 2 (e.g., interacting Bose gases), constant finite range spin-spin interactions of distinguishable or bosonic atoms (e.g., trapped ions or Rydberg atoms, or lattice bosons). In these settings, we further show that the optimal twist-untwist protocols asymptotically achieve 85% and 92% of the respective quantum Cramér-Rao bounds. We show that the error of a twist-untwist protocol can be decreased by a factor of L without an increase in the noise of the spin measurement if the twist-untwist protocol can be noiselessly iterated as an L layer quantum alternating operator ansatz.

74 ATOMIC AND MOLECULAR PHYSICS↗

Extracting free-energy landscapes of AgMn spin glass thin films with 1/$f$ resistance fluctuations

The temperature-dependent 1/f noise is reported for AgMn (12 at. %) thin films with multiple thicknesses ranging from 15 to 80 nm. A significant increase in the noise magnitude occurs in the spin-glass state. Analysis of the temperature-dependent exponent provides information on the energy barrier distribution and height, which in turn are related to the spin-glass coherence length. Here, we compare our results with those obtained previously on CuMn (13.5 at. %) thin films with similar thicknesses. We observe a similar trend of the increase of the barrier height with respect to thickness, but with relatively lower values for the AgMn barriers as compared to CuMn.

36 MATERIALS SCIENCE↗

Spin-lattice relaxation and the calculation of gain, pump power, and noise temperature in ruby

The use of a quantitative analysis of the dominant source of relaxation in ruby spin systems to make predictions of key maser amplifier parameters is described. The spin-lattice Hamiltonian which describes the interaction of the electron spins with the thermal vibrations of the surrounding lattice is obtained from the literature. Taking into account the vibrational anisotropy of ruby, Fermi's rule is used to calculate the spin transition rates between the maser energy levels. The spin population rate equations are solved for the spin transition relaxation times, and a comparison with previous calculations is made. Predictions of ruby gain, inversion ratio, and noise temperature as a function of physical temperature are made for 8.4-GHz and 32-GHz maser pumping schemes. The theory predicts that ruby oriented at 90 deg will have approximately 50 percent higher gain in dB and slightly lower noise temperature than a 54.7-deg ruby at 32 GHz (assuming pump saturation). A specific calculation relating pump power to inversion ratio is given for a single channel of the 32-GHz reflected wave maser.

Lyons, J. R.↗

Development and Demonstration of Active Noise Control Concepts

This report details design methods for and feasibility of an Active Noise Control (ANC) system using flush-wall-mounted sensors and actuators to reduce turbofan engine rotor-stator interaction noise. ANC concepts capable of suppressing discrete-tone spinning modes containing several cut-on radial mode were identified, developed analytically, and evaluated. Separate ANC systems that suppressed at least three radial modes in a cylindrical inlet duct and three radial modes in an exhaust annulus were developed. These designs resulted in inlet duct and exhaust duct tests that were performed at NASA on the 4-ft ANC Fan in the NASA Glenn AAPL facility. Effective suppression of 2-BPF spinning mode m = 2 tone noise was achieved over a range of fan speeds 1800 to 2450 rpm, where up to 4 radials were present. In the inlet duct, up to 12 dB reduction was obtained for 3 radial modes, and up to 4 dB was obtained with 4 radial modes. In the exhaust duct, up to 15 dB PWL reduction was obtained with either two or three radial modes present. Thus, the ability to suppress multiple radial modes for tones in both the inlet and exhaust ducts has been successfully demonstrated. Implications of ANC system design requirements on installation and system integration issues for ANC systems capable of suppressing higher order radial mode content when applied to a 767 using twin CF6 engines were evaluated analytically. The analytical results indicated an ANC system must be part of an integrated design to be effective.

Kraft, R.↗

Observations of LHR noise with banded structure by the sounding rocket S29 barium-GEOS

The measurement of electrostatic noise near the lower hybrid frequency made by the sounding rocket S29 barium-GEOS is reported. The noise is related to the spin of the rocket and reaches well below the local lower hybrid resonance frequency. Above the altitude of 300 km the noise shows banded structure roughly organized by the hydrogen cyclotron frequency. Simultaneously with the banded structure a signal near the hydrogen cyclotron frequency is detected. This signal is also spin modulated. The character of the noise strongly suggests that it is locally generated by the rocket payload disturbing the plasma. If this interpretation is correct, plasma wave experiments on other spacecrafts are expected to observe similar phenomena.

Koskinen, H. E. J.↗

Baseline acoustic levels of the NASA Active Noise Control Fan rig

Extensive measurements of the spinning acoustic mode structure in the NASA 48 inch Active Noise Control Fan (ANCF) test rig have been taken. A continuously rotating microphone rake system with a least-squares data reduction technique was employed to measure these modes in the inlet and exhaust. Farfield directivity patterns in an anechoic environment were also measured at matched corrected rotor speeds. Several vane counts and spacings were tested over a range of rotor speeds. The Eversman finite element radiation code was run with the measured in-duct modes as input and the computed farfield results were compared to the experimentally measured directivity pattern. The experimental data show that inlet spinning mode measurements can be made very accurately. Exhaust mode measurements may have wake interference, but the least-squares reduction does a good job of rejecting the non-acoustic pressure. The Eversman radiation code accurately extrapolates the farfield levels and directivity pattern when all in-duct modes are included.

Sutliff, Daniel L.↗

Tone excited jets. IV - Acoustic measurements

Attention is given to acoustic results from an experiment designed to deepen insight into the noise generated by a tone-excited jet, with emphasis on the mechanism of broadband jet noise amplification. Results are presented for both heated and unheated jets, with and without the effect of forward flight simulation over a range of excitation frequencies and levels, and for zero-order and first-order spinning modes. Broadband jet noise amplifications of up to 5 dB have been observed in this study. Relative velocity effects are the same for both excited and unexcited jets. It is concluded that small scale turbulence generates the additional broadband noise upon excitation of the jet by an upstream-injected discrete tone acoustic wave.

Ahuja, K. K.↗

An observation of LHR noise with banded structure by the sounding rocket S29 Barium-GEOS

The measurement of electrostatic and obviously locally produced noise near the lower hybrid frequency made by the sounding rocket S29 Barium-GEOS is reported. The noise is strongly related to the spin of the rocket and reaches well below the local lower hybrid resonance frequency. Above the altitude of 300 km the noise shows banded structure roughly organized by the hydrogen cyclotron frequency. Simultaneously with the banded structure, a signal near the hydrogen cyclotron frequency is detected. This signal is also spin related. The characteristics of the noise suggest that it is locally generated by the rocket payload disturbing the plasma. If this interpretation is correct we expect plasma wave experiments on other spacecrafts, e.g., the space shuttle to observe similar phenomena.

Koskinen, H. E. J.↗

Squeezed spin states: Squeezing the spin uncertainty relations

The notion of squeezing in spin systems is clarified, and the principle for spin squeezing is shown. Two twisting schemes are proposed as building blocks for spin squeezing and are shown to reduce the standard quantum noise, s/2, of the coherent S-spin state down to the order of S(sup 1/3) and 1/2. Applications to partition noise suppression are briefly discussed.

Kitagawa, Masahiro↗

Anomalous magnetic noise in an imperfectly flat landscape in the topological magnet Dy 2 Ti 2 O 7

Noise generated by motion of charge and spin provides a unique window into materials at the atomic scale. From temperature of resistors to electrons breaking into fractional quasiparticles, “listening” to the noise spectrum is a powerful way to decode underlying dynamics. Here, we use ultrasensitive superconducting quantum interference device (SQUIDs) to probe the puzzling noise in a frustrated magnet, the spin-ice compound Dy 2 Ti 2 O 7 (DTO), revealing cooperative and memory effects. DTO is a topological magnet in three dimensions—characterized by emergent magnetostatics and telltale fractionalized magnetic monopole quasiparticles—whose real-time dynamical properties have been an enigma from the very beginning. We show that DTO exhibits highly anomalous noise spectra, differing significantly from the expected Brownian noise of monopole random walks, in three qualitatively different regimes: equilibrium spin ice, a “frozen” regime extending to ultralow temperatures, and a high-temperature “anomalous” paramagnet. We present several distinct mechanisms that give rise to varied colored noise spectra. In addition, we identify the structure of the local spin-flip dynamics as a crucial ingredient for any modeling. Thus, the dynamics of spin ice reflects the interplay of local dynamics with emergent topological degrees of freedom and a frustration-generated imperfectly flat energy landscape, and as such, it points to intriguing cooperative and memory effects for a broad class of magnetic materials.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Radiation of cylindrical duct acoustic modes with flow mismatch

Motivated by the problem of Mach number and temperature discontinuity mismatch between the tailpipe and the surrounding medium, and the effect of this flow mismatch on aircraft engine noise, the radiation of spinning turbo-acoustic modes from a round duct is investigated. The model, based on a plug flow exhaust jet, solves the convected wave equations using Fourier transforms, inversion being accomplished via a coupled Wiener-Hopf and Carrier-Koiter technique. It is concluded that the Mach number discontinuity results in a conflict between convection and refraction effects, while the temperature mismatch results in a sharp beaming of sound off to the side.

Savkar, S. D.↗

Limitations of Phased Array Beamforming in Open Rotor Noise Source Imaging

Phased array beamforming results of the F31/A31 historical baseline counter-rotating open rotor blade set were investigated for measurement data taken on the NASA Counter-Rotating Open Rotor Propulsion Rig in the 9- by 15-Foot Low-Speed Wind Tunnel of NASA Glenn Research Center as well as data produced using the LINPROP open rotor tone noise code. The planar microphone array was positioned broadside and parallel to the axis of the open rotor, roughly 2.3 rotor diameters away. The results provide insight as to why the apparent noise sources of the blade passing frequency tones and interaction tones appear at their nominal Mach radii instead of at the actual noise sources, even if those locations are not on the blades. Contour maps corresponding to the sound fields produced by the radiating sound waves, taken from the simulations, are used to illustrate how the interaction patterns of circumferential spinning modes of rotating coherent noise sources interact with the phased array, often giving misleading results, as the apparent sources do not always show where the actual noise sources are located. This suggests that a more sophisticated source model would be required to accurately locate the sources of each tone. The results of this study also have implications with regard to the shielding of open rotor sources by airframe empennages.

Horvath, Csaba↗

Quantum Simulations of Fermionic Hamiltonians with Efficient Encoding and Ansatz Schemes

Here, we propose a computational protocol for quantum simulations of fermionic Hamiltonians on a quantum computer, enabling calculations on spin defect systems which were previously not feasible using conventional encodings and a unitary coupled-cluster ansatz of variational quantum eigensolvers. We combine a qubit-efficient encoding scheme mapping Slater determinants onto qubits with a modified qubitcoupled cluster ansatz and noise-mitigation techniques. Our strategy leads to a substantial improvement in the scaling of circuit gate counts and in the number of required qubits, and to a decrease in the number of required variational parameters, thus increasing the resilience to noise. We present results for spin defects of interest for quantum technologies, going beyond minimum models for the negatively charged nitrogen vacancy center in diamonds and the double vacancy in 4H silicon carbide (4H-SiC) and tackling a defect as complex as negatively charged silicon vacancy in 4H-SiC for the first time.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Electron-nuclear decoupling at a spin clock transition

The ability to design quantum systems that decouple from environmental noise sources is highly desirable for development of quantum technologies with optimal coherence. The chemical tunability of electronic states in magnetic molecules combined with advanced electron spin resonance techniques provides excellent opportunities to address this problem. Indeed, so-called clock transitions have been shown to protect molecular spin qubits from magnetic noise, giving rise to significantly enhanced coherence. Here we conduct a spectroscopic and computational investigation of this physics, focusing on the role of the nuclear bath. Away from the clock transition, linear coupling to the nuclear degrees of freedom causes a modulation and decay of electronic coherence, as quantified via electron spin echo signals generated experimentally and in silico. Meanwhile, the effective hyperfine interaction vanishes at the clock transition, resulting in electron-nuclear decoupling and an absence of quantum information leakage to the nuclear bath, providing opportunities to characterize other decoherence sources.

74 ATOMIC AND MOLECULAR PHYSICS↗

Observations of interplanetary plasma waves, spacecraft noise, and sheath phenomena on Imp 7

The Imp 7 plasma wave instrument measures electric and magnetic wave components of plasma oscillations over the frequency range from 10 Hz to 100 kHz. The instrumentation and relevant external characteristics of the spacecraft that appear to be responsible for some in-flight disturbance effects are briefly described. It is shown that as each one of the 16 solar panel flats rotates into shadow or sunlight, the array transients produce fluctuating magnetic fields that are detected on the magnetic loop mounted 3.4 m from the spacecraft. These transients occur 16 times per spin period, and the corresponding magnetic noise has a high frequency on the rapidly spinning Imp 7 spacecraft. The analysis suggests that some Imp magnetic threshold levels measured 3-4 m from the spacecraft are determined by the solar array current transient effects associated with the discrete 16-sided geometry of the spacecraft. The geometry also influences the response of the electric dipole antenna by modulating the sheath.

Scarf, F. L.↗

First Test of Fan Active Noise Control (ANC) Completed

With the advent of ultrahigh-bypass engines, the space available for passive acoustic treatment is becoming more limited, whereas noise regulations are becoming more stringent. Active noise control (ANC) holds promise as a solution to this problem. It uses secondary (added) noise sources to reduce or eliminate the offending noise radiation. The first active noise control test on the low-speed fan test bed was a General Electric Company system designed to control either the exhaust or inlet fan tone. This system consists of a "ring source," an induct array of error microphones, and a control computer. Fan tone noise propagates in a duct in the form of spinning waves. These waves are detected by the microphone array, and the computer identifies their spinning structure. The computer then controls the "ring source" to generate waves that have the same spinning structure and amplitude, but 180 out of phase with the fan noise. This computer generated tone cancels the fan tone before it radiates from the duct and is heard in the far field. The "ring source" used in these tests is a cylindrical array of 16 flat-plate acoustic radiators that are driven by thin piezoceramic sheets bonded to their back surfaces. The resulting source can produce spinning waves up to mode 7 at levels high enough to cancel the fan tone. The control software is flexible enough to work on spinning mode orders from -6 to 6. In this test, the fan was configured to produce a tone of order 6. The complete modal (spinning and radial) structure of the tones was measured with two builtin sets of rotating microphone rakes. These rakes provide a measurement of the system performance independent from the control system error microphones. In addition, the far-field noise was measured with a semicircular array of 28 microphones. This test represents the first in a series of tests that demonstrate different active noise control concepts, each on a progressively more complicated modal structure. The tests are in preparation for a demonstration on a flight-type engine.

Source record↗

A beamline for ultrafast extreme ultraviolet magneto-optical spectroscopy in reflection near the shot noise limit

High harmonic generation (HHG) makes it possible to measure spin and charge dynamics in materials on femtosecond to attosecond timescales. However, the extreme nonlinear nature of the high harmonic process means that intensity fluctuations can limit measurement sensitivity. Here we present a noise-canceled, tabletop high harmonic beamline for time-resolved reflection mode spectroscopy of magnetic materials. We use a reference spectrometer to independently normalize the intensity fluctuations of each harmonic order and eliminate long term drift, allowing us to make spectroscopic measurements near the shot noise limit. Here, these improvements allow us to significantly reduce the integration time required for high signal-to-noise (SNR) measurements of element-specific spin dynamics. Looking forward, improvements in the HHG flux, optical coatings, and grating design can further reduce the acquisition time for high SNR measurements by 1–2 orders of magnitude, enabling dramatically improved sensitivity to spin, charge, and phonon dynamics in magnetic materials.

47 OTHER INSTRUMENTATION↗