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Extended spin relaxation times of optically addressed vanadium defects in silicon carbide at telecommunication frequencies

Optically interfaced solid-state defects are promising candidates for quantum communication technologies. The ideal defect system would feature bright telecom emission, long-lived spin states, and a scalable material platform, simultaneously. Here, in this study, we use one such system, vanadium (V 4+ ) in silicon carbide, to establish a potential telecom spin-photon interface within a mature semiconductor host. This demonstration of efficient optical spin polarization and readout facilitates all-optical measurements of temperature-dependent spin relaxation times (T 1 ). By using this technique, and lowering the temperature from approximately 2 K to approximately 100 mK, we observe a remarkable 4-orders-of-magnitude increase in spin T 1 across all measured sites, with site-specific values ranging from 57.1 ms to 27.9 s. Furthermore, we identify the underlying relaxation mechanisms, which involve a two-phonon Orbach process, indicating the opportunity for strain tuning to enable qubit operation at higher temperatures. These results position V 4+ in SiC as a prime candidate for scalable quantum nodes in future quantum networks.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC

Measurements of the methane relaxation times for application to the infrared emission models of the upper atmospheres of outer planets and Titan

The 7.8 micrometer emission from the nu(sub 4) band of methane (CH4) is a regularly observed feature in the stratosphere of all the giant planets and Titan. On Jupiter, enhancements in this emission are associated with the infrared hot spots in the auroral zone. Attempts to model this phenomenon in particular, and to understand the role of methane in general, have been hampered in part by a lack of adequate laboratory measurements of the collisional relaxation times for the nu(sub 3) and nu(sub 4) levels over the appropriate temperature range. To provide this needed data, a series of laboratory experiments were initiated. In the experimental arrangement the nu(sub3) band of methane is pumped at 3.3 micrometers using a pulsed infrared source (Nd:YAG/dye laser system equipped with a wave-length extender). The radiative lifetime of the nu(sub 3) level (approximately 37 ms) is much shorter than the nu(sub 4) lifetime (approximately 390 ms); however, a rapid V-V energy transfer rate ensures that the nu(sub 4) level is substantially populated. The photoacoustic technique is used to acquire relaxation rate information. The experiments are performed using a low-temperature, low-pressure cell. Experimental apparatus and technique are described. In addition some of the experimental difficulties associated with making these measurements are discussed and some preliminary results are presented.

Halthore, Rangasayi N.

Magnetic field dependence of plasma relaxation times

A previously derived Fokker-Planck collision integral for an electron plasma in a dc magnetic field is examined in the limit in which the Debye length is greater than the thermal gyroradius, which is in turn greater than the mean distance of closest approach. It is demonstrated that the collision integral can be satisfactorily approximated by the classical Landau value (which ignores the presence of a dc magnetic field) if the following replacement is made: In the Coulomb logarithm, the Debye length is replaced by the gyroradius. This induces a fundamental logarithmic dependence on magnetic field in the relaxation times. Numerical comparison of the asymptotic approximations with the previously derived exact results is made, and good agreement is found. The simplification this introduces into the description of collision processes in magnetized plasma is considerable.

Montgomery, D.

Picosecond excite-and-probe absorption measurement of the intra-2E(g)E(3/2)-state vibrational relaxation time in Ti(3+):Al2O3

The Ti(3+)-doped Al2O3 has been recently demonstrated to be a tunable solid-state laser system with Ti(3+) as the laser-active ion. In this paper, the kinetics of vibrational transitions in the 2E(g)E(3/2) electronic state of Ti(3+):Al2O3a (crucial for characterizing new host materials for the Ti ion) was investigated. A 527-nm 5-ps pulse was used to excite a band of higher vibrational levels of the 2E(g)E(3/2) state, and the subsequent growth of population in the zero vibrational level and lower vibrational levels was monitored by a 3.9-micron picosecond probe pulse. The time evolution curve in the excited 2E(g)E(3/2) state at room temperature was found to be characterized by a sharp rise followed by a long decay, the long lifetime decay reflecting the depopulation of the zero and the lower vibrational levels of the 2E(g)E(3/2) state via radiative transitions. An upper limit of 3.5 ps was estimated for intra-2E(g)E(3/2)-state vibrational relaxation time.

Gayen, S. K.

Relaxation time measurements by an electronic method.

Description of a simple electronic system that permits the direct measurement of time constants of decaying signals. The system was used in connection with relaxation experiments on hydrogen and rubidium masers and was found to operate well. The use of a computing counter in the systems gives the possibility of making averages on several experiments and obtaining the standard deviation of the results from the mean. The program for the computing counter is given.

Brousseau, R.

Relaxation times for disoriented isospin condensates in high energy heavy ion collisions

Fluctuations between charged and neutral kaons measured by the ALICE Collaboration in Pb-Pb collisions at the CERN Large Hadron Collider (LHC) exceed conventional explanations. Previously it was shown that if the scalar condensate is accompanied by an electrically neutral isospin-1 field then the combination can produce large equilibrium fluctuations where ⟨$\overline{𝑢}$ ⁢𝑢⟩≠⟨ $\overline{𝑑}$𝑑⟩. Hadronizing strange and antistrange quarks might then strongly fluctuate between charged ($\overline{𝑢}$⁢𝑠 or $\overline{𝑠}$⁢𝑢) and neutral (𝑑⁢$\overline{𝑠}$⁢ or 𝑠⁢$\overline{𝑑}$) kaons. Here, we estimate the times for the condensates to achieve their equilibrium probability distributions within causal volumes in high energy heavy ion collisions. This is achieved by modeling the temperature dependence of the condensates, mesonic collective excitations, decay rates of the associated fields, and employing the Langevin and Fokker-Planck equations. Within this model, we find that the equilibration times are short compared with the expansion time, making disoriented isospin condensates a viable explanation for the anomalous fluctuations observed at the LHC.

Quark-gluon plasma

Effective masses, relaxation times, and carrier mobilities in some chloride intercalants of graphite

The effective masses, carrier scattering times and carrier mobilities have been measured in selected graphite intercalation compounds using the Shubnikov-de Haas effect at a series of temperatures between 4 and 50 K. Effective masses are less than or equal to 0.1 of the free-electron mass, scattering times are about 10 to the -13th/s and carrier mobilities are on the order of 10,000 sq cm/V s.

Woollam, J. A.

Vibrational relaxation in expanding N2 and air

New N2 vibrational temperature data, obtained in expanding N2 and air using the electron beam technique, are analyzed permitting the vibrational relaxation times to be determined as a function of temperature. In addition, the effects on N2 vibrational relaxation times of direct vibrational energy transfer between N2 and H2O, between N2 and O2, and between N2 and free electrons introduced from arc contaminants are analyzed. The vibrational relaxation times determined from the present measurements agree with those measured in the expanding flows of shock tunnels and impact tubes. These expanding data also agree with relaxation times observed in acoustical resonant cavities where alternating compressions and expansions take place. The relaxation times in expanding flows (vib-tran exchange process) are found to be approximately 50 times faster than those measured in the compressing flow of shock tubes (tran-vib exchange process). This evidence strongly supports the concept that one relaxation time distribution cannot be applied to both exchange processes.

Sebacher, D. I.

Indications for common origin and gravitational interaction in three binary LMC clusters

Three close pair clusters of the LMC, NGC 2006/SL 538, NGC 2011 a/b, and NGC 2042 a/b, have been studied in order to establish their binarity. The stellar content in the outer region of each cluster has been investigated by means of low resolution objective UK Schmidt prism spectra, the cores of the clusters have been examined using low resolution integrated IUE spectra, whereas their density profiles and their observed dynamical parameters have been derived by means of star counts. The integrated spectra of their cores and the stellar content of their outer cluster regions have shown a common origin and a very young age (less than 2 x 10 exp 7 yr) for each member of the pairs, whereas their dynamical study has shown that they are gravitationally interacting. Comparing the age of their stellar content with their dynamical and relaxation times, it has been found that these clusters are physically associated and had no time to relax by stellar encounters, no time to merge, and no time to be destroyed by dynamical friction.

Kontizas, E.

Evaluation of muscle injury using magnetic resonance imaging

The objective of this study was to investigate spin echo T2 relaxation time changes in thigh muscles after intense eccentric exercise in healthy men. Spin echo and calculated T2 relaxation time images of the thighs were obtained on several occasions after exercise of one limb; the contralateral limb served as control. Muscle damage was verified by elevated levels of serum creatine kinase (CK). Thirty percent of the time no exercise effect was discernible on the magnetic resonance (MR) images. In all positive MR images (70%) the semitendinosus muscle was positive, while the biceps femoris, short head, and gracilis muscles were also positive in 50% and 25% of the total cases, respectively. The peak T2 relaxation time and serum CK were correlated (r = 0.94, p<0.01); temporal changes in muscle T2 relaxation time and serum CK were similar, although T2 relaxation time remained positive after serum CK returned to background levels. We conclude that magnetic resonance imaging can serve as a useful tool in the evaluation of eccentric exercise muscle damage by providing a quantitative indicator of damage and its resolution as well as the specific areas and muscles.

NASA Discipline Number 26-10

Time-domain approach for the transient responses in stratified viscoelastic Earth models

We have developed the numerical algorithm for the computation of transient viscoelastic responses in the time domain for a radially stratified Earth model. Stratifications in both the elastic parameters and the viscosity profile have been considered. The particular viscosity profile employed has a viscosity maximum with a constrast of O(100) in the mid lower mantle. The distribution of relaxation times reveals the presence of a continuous spectrum situated between O(100) and O(exp 4) years. The principal mode is embedded within this continuous spectrum. From this initial-value approach we have found that for the low degree harmonics the non-modal contributions are comparable to the modal contributions. For this viscosity model the differences between the time-domain and normal-mode results are found to decrease strongly with increasing angular order. These calculations also show that a time-dependent effective relaxation time can be defined, which can be bounded by the relaxation times of the principal modes.

Hanyk, L.