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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 55 records · Page 3
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Relevant capture cross sections for intentional nuclear forensics, table summary

This summary provides a brief list of capture cross section metrics for naturally occurring isotopes for review by the Intentional Forensics Venture. This introduction is a companion to the column tabulated data, available in pdf and spreadsheet form. Cross section values for this summary list are taken from ENDF/B-VIII.0 and the development library for ENDF/B-VIII.1, with abundances taken from Nuclear Wallet Cards abundance tables. The cross section metrics are thermal cross section, resonance integral (RI), Maxwellian averaged cross section at 30 keV, and 252 Cf spontaneous fission spectrum averaged cross section. The isotopes are listed in order of Z, then A, with the elemental symbol also reported. This memo gives a brief introduction and overview of the data presented.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
NASA NTRS1986

Nuclear tracks, Sm isotopes and neutron capture effects in the Elephant Morraine shergottite

Nuclear track studies, uranium concentration measurements and Sm-isotope studies have been performed on both lithologies A and B of the Elephant Morraine shergottite, EETA 79001. Track studies show that EETA 79001 was a rather small object in space with a preatmospheric radius of 12 + or - 2 cm, corresponding to a preatmospheric mass of 28 + or - 13 kg. Phosphates have U concentrations ranging from 0.3 to 1.3 ppm. There are occasional phosphates with excess fission tracks, possibly produced from neutron-induced fission of U and Th, during the regolith exposure in the shergottite parent body (SPB). Sm-isotope studies, while not showing any clear-cut excess in Sm-150, make it possible to derive meaningful upper limits to thermal neutron fluences of 2 to 3 x 10 to the 15th n/sq cm, during a possible regolith irradiation. These limits are consistent with the track data and also make it possible to derive an upper limit to the neutron exposure age of EETA 79001 of 55 Myr in the SPB regolith.

Rajan, R. S.↗
DOE OSTI2021

MuSun - Muon Capture on the Deuteron

The MuSun experiment is a precision measurement of the rate for nuclear muon capture on the deuteron, designed to resolve a long-standing disagreement between experiment and theory, and to determine an important low-energy constant relevant for a variety of weak and strong dynamics. The experiment is based on a novel active target method employing a pure deuterium cryogenic time-projection chamber. The data taking was completed in two main campaigns and the analysis is well advanced. The unique challenges and corresponding strategy of the experiment as well as the status of the analysis are presented.

Kammel, Peter↗
DOE OSTI2025

Signal processing and spectral modeling for the BeEST experiment

The Beryllium Electron capture in Superconducting Tunnel junctions (BeEST) experiment searches for evidence of heavy neutrino mass eigenstates in the nuclear electron capture decay of 7 Be by precisely measuring the recoil energy of the 7 Li daughter. In Phase III, the BeEST experiment has been scaled from a singl superconducting tunnel junction (STJ) sensor to a 36-pixel array to increase sensitivity and mitigate gamma-induced backgrounds. Phase III also uses a new continuous data acquisition system that greatly increases the flexibility for signal processing and data cleaning. Here, we have developed procedures for signal processing and spectral fitting that are sufficiently robust to be automated for large datasets. Furthermore, this article presents the optimized procedures before unblinding the majority of the Phase III dataset to search for physics beyond the standard model.

6 ≤ A ≤ 19↗
DOE OSTI2021

Random sub-diffusion and capture of genes by the nuclear pore reduces dynamics and coordinates inter-chromosomal movement

Hundreds of genes interact with the yeast nuclear pore complex (NPC), localizing at the nuclear periphery and clustering with co-regulated genes. Dynamic tracking of peripheral genes shows that they cycle on and off the NPC and that interaction with the NPC slows their sub-diffusive movement. Furthermore, NPC-dependent inter-chromosomal clustering leads to coordinated movement of pairs of loci separated by hundreds of nanometers. We developed fractional Brownian motion simulations for chromosomal loci in the nucleoplasm and interacting with NPCs. These simulations predict the rate and nature of random sub-diffusion during repositioning from nucleoplasm to periphery and match measurements from two different experimental models, arguing that recruitment to the nuclear periphery is due to random sub-diffusion and transient capture by NPCs. Finally, the simulations do not lead to inter-chromosomal clustering or coordinated movement, suggesting that interaction with the NPC is necessary, but not sufficient, to cause clustering.

59 BASIC BIOLOGICAL SCIENCES↗
DOE OSTI2021

H 2 production in the 10 B(n,α) 7 Li reaction in water

Herein we demonstrate a method for measuring the H2 produced in water from the 10 B(n,α) 7 Li fission reaction. Low energy neutrons from the NIST Center for Neutron Research interact with borate-containing water in a temperature-controlled high pressure cell made from titanium. After exposure for one to several hours, the water is extracted and sparged with argon. H 2 entrained in the sparging gas is sampled with a small mass spectrometer. To determine the neutron exposure, a small amount of sodium is included in the borate solution. The water is collected and 24 Na activation is measured in a counting apparatus on the following day. The G-value for H 2 at room temperature is found to be (1.18 ± 0.10) molecules H 2 /100eV, in good agreement with previous estimates and recent modeling calculations.

10B↗
DOE OSTI2021

Thermal Energy Transport in Oxide Nuclear Fuel

To efficiently capture the energy of the nuclear bond, advanced nuclear reactor concepts seek solid fuels that must withstand unprecedented temperature and radiation extremes. In these advanced fuels, thermal energy transport under irradiation is directly related to reactor performance as well as reactor safety. The science of thermal transport in nuclear fuel is a grand challenge as a result of both computational and experimental complexities. Here we provide a comprehensive review of thermal transport research on two actinide oxides: one currently in use in commercial nuclear reactors, uranium dioxide (UO 2 ), and one advanced fuel candidate material, thorium dioxide (ThO 2 ). In both materials, heat is carried by lattice waves or phonons. Crystalline defects caused by fission events effectively scatter phonons and lead to a degradation in fuel performance over time. Bolstered by new computational and experimental tools, researchers are now developing the foundational work necessary to accurately model and ultimately control thermal transport in advanced nuclear fuels. We begin by reviewing research aimed at understanding thermal transport in perfect single crystals. The absence of defects enables studies that focus on the fundamental aspects of phonon transport. Next, we review research that targets defect generation and evolution. Here the focus is on ion irradiation studies used as surrogates for damage caused by fission products. We end this review with a discussion of modeling and experimental efforts directed at predicting and validating mesoscale thermal transport in the presence of irradiation defects. While efforts in these research areas have been robust, challenging work remains in developing holistic tools to capture and predict thermal energy transport across widely varying environmental conditions.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2025

Techno-Economic Performance of Nuclear Reactors to Power Direct Air Capture Technologies

This research contributes to the expanding body of work by academia and industry on the synergy between nuclear energy and DAC systems. It provides an independent and transparent assessment of the cost associated with capturing CO2 from the atmosphere when powering DAC with various nuclear technologies, and by comparing these findings with non-nuclear alternatives. This study utilizes the latest models and cost estimates for both nuclear and DAC technologies.

direct air capture (DAC)↗
DOE OSTI2023

Updated evaluation of potential ultralow Q -value β -decay candidates

“Ultralow” Q-value β decays are referred to as such due to their low decay energies of less than ≈1 keV. Such a low energy decay is possible when the parent nucleus decays to an excited state in the daughter, with an energy close to that of the Q value. These decays are of interest as potential new candidates for neutrino mass determination experiments and as a testing ground for studies of atomic interference effects in the nuclear decay process. In this paper, we provide an updated evaluation of atomic mass data and nuclear energy-level data to identify potential ultralow Q-value β decay candidates. For many of these candidates, more precise and accurate atomic mass data is needed to determine if the Q value of the potential ultralow decay branch is energetically allowed and in fact ultralow. Furthermore, the relevant precise atomic mass measurements can be achieved via Penning trap mass spectrometry.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

Description of di-hadron saturation signals within a universal nuclear parton distribution function approach

Di-hadron and di-jet correlation measurements in proton-nucleus (𝑝+𝐴) and electron-nucleus collisions are widely motivated as sensitive probes of novel, nonlinear quantum chromodynamices saturation dynamics in hadrons, which are particularly accessible in the dense nuclear environment at low values of Bjorken-𝑥 (𝑥 A ). Current measurements at the BNL Relativistic Heavy Ion Collider (RHIC) and the CERN Large Hadron Collider (LHC) observe a significant suppression in the per-trigger yield at forward rapidities compared to that in proton-proton collisions, nominally consistent with the “mono-jet” production expected in a saturation scenario. However, the width of the azimuthal correlation remains unmodified, in contradiction to the qualitative expectations from this physics picture. I investigate whether the construction of these observables leaves them sensitive to effects from simple nuclear shadowing as captured by, for example, universal nuclear parton distribution function (nPDF) analyses. I find that modern nPDF sets, informed by recent precision measurements sensitive to the shadowing of low-𝑥 A gluon densities in LHC and other data, can describe all or the majority of the di-hadron/jet suppression effects in 𝑝+𝐴 data at both RHIC and the LHC, while giving a natural explanation for why the azimuthal correlation width is unmodified. Notably, this is achieved via a (𝑥 A ,𝑄 2 )-differential suppression of overall cross sections only, without requiring additional physics dynamics which alter the interevent correlations.

Jets & heavy flavor physics↗
DOE OSTI2020

Bulk Viscous Damping of Density Oscillations in Neutron Star Mergers

In this paper, we discuss the damping of density oscillations in dense nuclear matter in the temperature range relevant to neutron star mergers. This damping is due to bulk viscosity arising from the weak interaction “Urca” processes of neutron decay and electron capture. The nuclear matter is modelled in the relativistic density functional approach. The bulk viscosity reaches a resonant maximum close to the neutrino trapping temperature, then drops rapidly as temperature rises into the range where neutrinos are trapped in neutron stars. We investigate the bulk viscous dissipation timescales in a post-merger object and identify regimes where these timescales are as short as the characteristic timescale ~10 ms, and, therefore, might affect the evolution of the post-merger object. Our analysis indicates that bulk viscous damping would be important at not too high temperatures of the order of a few MeV and densities up to a few times saturation density.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

Integrated Operations for Nuclear: Work Reduction Opportunity Demonstration

Integrated Operations for Nuclear: Work Reduction Opportunity Demonstration The DI BCA document also identifies specific, digitally enabled WRO categories for further study. These were selected as most relevant by Reference Plant personnel from a larger list of WRO areas identified across the nuclear industry as captured INL/RPT-21-64134, “Process for Significant Nuclear Work Function Innovation Based on Integrated Operations Concepts.” This ION WRO demonstration report was developed to provide illustrative, specific, and actionable direction for intertwined PTPG changes associated with digital modernization efforts. The coordinated changes in these areas are intended to maximize safe plant operational and economic performance. This includes enabling WROs associated with detailed configuration, implementation, and use of digital systems and how they are supported over their lifecycle. Illustrating this direction through a minimum set of advanced technology examples establishes a model PTPG framework that can be leveraged across the spectrum of nuclear plant digital modernization efforts going forward. This document addresses many related concepts. To promote an integrated understanding of the topics that make up this work, this document contains an extensive set of internal hyperlinks. This set includes hyperlinks to page numbers in the table of contents, section numbers, items in lists, figures, tables, and references to other documents within the report. When hovering the cursor above hyperlinked text in Adobe, the cursor will change from “ ” to “ .” When the “ ” appears, a left mouse click will take the reader to the referenced location in the document. To return to the original location in the document, the reader need only press and hold the “alt” button on the keyboard and then simultaneously press the “<” directional key on the keyboard.

42 ENGINEERING↗
DOE OSTI2026

Enhanced antineutrino emission from 𝛽 decay in core-collapse supernovae with self-consistent weak decay rates

Nuclear weak-interaction rates are known to exert a prominent effect in the late stages of stellar collapse. Despite their importance, most studies to date on core-collapse supernovae (CCSNe) have focused primarily on the effects of electron captures, neglecting 𝛽 decay contributions. In this work, we present the first CCSNe simulation incorporating global 𝛽 decay rates from a microscopic theory. These are enabled by a large-scale evaluation of both electron capture and 𝛽 decay rates, obtained self-consistently utilizing the relativistic energy density functional theory and finite-temperature quasiparticle random-phase approximation. Including 𝛽 decay leads to a dramatic enhancement of the pre-bounce antineutrino signal as the antineutrino emissivity increases by more than two orders of magnitude and the luminosity by a factor of 50 relative to thermal emission alone, while the average antineutrino energy increases by over 1 MeV. Furthermore, it is expected that these new rates could help us constrain the model uncertainties related to weak-interaction processes, improving the prediction of antineutrino signal during the final stages of stellar death.

Beta decay↗
DOE OSTI2021

Ultrafast Imaging of Molecules with Electron Diffraction

Photoexcited molecules convert light into chemical and mechanical energy through changes in electronic and nuclear structure that take place on femtosecond timescales. Gas phase ultrafast electron diffraction (GUED) is an ideal tool to probe the nuclear geometry evolution of the molecules and complements spectroscopic methods that are mostly sensitive to the electronic state. GUED is a passive probing tool that does not alter the molecular properties during the probing process and is sensitive to the spatial distribution of charge in the molecule, including both electrons and nuclei. Improvements in temporal resolution have enabled GUED to capture coherent nuclear motions in molecules in the excited and ground electronic states with femtosecond and subangstrom resolution. Here we present the basic theory of GUED and explain what information is encoded in the diffraction signal, review how GUED has been used to observe coherent structural dynamics in recent experiments, and discuss the advantages and limitations of the method.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2021

Singular value decomposition and similarity renormalization group evolution of nuclear interactions

One of the main challenges for ab initio nuclear many-body theory is the growth of computational and storage costs as calculations are extended to heavy, exotic, and structurally complex nuclei. Here, we investigate the factorization of nuclear interactions as a means to address this issue. We perform Singular Value Decompositions of nucleon-nucleon interactions in partial wave representation and study the dependence of the singular value spectrum on interaction characteristics like regularization scheme and resolution scales. We develop and implement the Similarity Renormalization Group (SRG) evolution of the factorized interaction, and demonstrate that this SVD-SRG approach accurately preserves two-nucleon observables. We find that low-resolution interactions allow the truncation of the SVD at low rank, and that a small number of relevant components is sufficient to capture the nuclear interaction and perform an accurate SRG evolution, while the Coulomb interaction requires special consideration. The rank is uniform across all partial waves, and almost independent of the basis choice in the tested cases. This suggests an interpretation of the relevant singular components as mere representations of a small set of abstract operators that can describe the interaction and its SRG flow. Following the traditional workflow for nuclear interactions, we discuss how the transformation between the center-of-mass and laboratory frames creates redundant copies of the partial wave components when implemented in matrix representation, and we discuss strategies for mitigation. Lastly, we test the low-rank approximation to the SRG-evolved interactions in many-body calculations using the In-Medium SRG. By including nuclear radii in our analysis, we verify that the implementation of the SRG using the singular vectors of the interaction does not spoil the evolution of other observables.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Review of capture cross sections relevant for intentional nuclear forensics

The NA-22 Intentional Forensics Venture is developing a system for tagging nuclear fuel using various methods of information encoding. One of the main methods under development is the insertion of isotopically enriched tracers into the fuel. In order to aid in the understanding of the neutronic performance of these taggants, we assess the quality of the nuclear data underpinning simulations, which are driven by the neutron-capture cross sections. We present these cross sections of naturally occurring isotopes of the elements provided in the neutron sublibrary of the planned ENDF/B-VIII.1 Feb. 2023 library release. We make this assessment using a rubric designed for this effort, which quantifies orthogonal features related to the overall quality. The quality metric highlights 6 aspects: experimental data, resonance evaluations, integral metrics, covariances, fission products, and documentation. We focus on energy ranges relevant for reactor applications. We also discuss additional sources for new, high-quality cross-section data that may be utilized on the time scale of the venture, including existing global data, new experiments, and computational methods. Finally, overall outlook is presented with conclusions.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

Water–Hydrocarbon Interactions in Anionic Pyrene Monohydrate

Interactions between water and polycyclic aromatic hydrocarbons are essential in many aspects of chemistry, from interstellar and atmospheric processes to interfacial hydrophobicity and wetting phenomena. Despite their growing importance, the intermolecular potentials of the water-hydrocarbon interactions are underdeveloped compared to water-water potentials, and there are similarly few experimental probes that are sensitive to the details of the water-hydrocarbon potential. We present a combined experimental and computational study of anionic pyrene monohydrate, one of the simplest water/hydrocarbon clusters. The action spectrum in the OH region of the mass-selected cluster ion provides a rigorous benchmark for intermolecular potentials and computational methodologies. We identify missing intermolecular interactions and shortcomings in conventional dynamics calculations by comparing experimental data to density functional theory and classical molecular dynamics calculations. Kinetic trapping is prevalent, even for one water molecule and one pyrene molecule, leading to slow equilibration in conventional molecular dynamics calculations, even on nanosecond timescales and at low temperatures (50 K). At constant energy, temperature fluctuations for the pair of molecules are substantial. Immersing the system in a bath of soft spheres and employing parallel tempering alleviates kinetic trapping and dampens temperature fluctuations, bringing the system closer to the thermodynamic limit. With such augmented sampling, a simple, flexible water model reproduces the linewidth and the asymmetric broadening of the symmetric OH stretching mode, which we assign to spectral diffusion. In the OH stretching region, dynamics calculations predict a more intense antisymmetric peak than experiments observe but do not predict the bimodal split symmetric peak that the experiments show. Furthermore, our work suggests that electronic polarization, missing in the empirical force field, is responsible for the first discrepancy and that quantum nuclear effects, captured neither in density functional theory nor in classical dynamics, may be responsible for the second.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗