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At least 55 records · Page 3

Identifying Entangled Physics Relationships Through Sparse Matrix Decomposition to Inform Plasma Fusion Design

We report a sustainable burn platform through inertial confinement fusion (ICF) has been an ongoing challenge for over 50 years. Mitigating engineering limitations and improving the current design involves an understanding of the complex coupling of physical processes. While sophisticated simulation codes are used to model ICF implosions, these tools contain necessary numerical approximation but miss physical processes that limit predictive capability. Identification of relationships between controllable design inputs to ICF experiments and measurable outcomes (e.g., neutron yield, neutron velocity, areal density) from performed experiments can help guide the future design of experiments and development of simulation codes, to potentially improve the accuracy of the computational models used to simulate ICF experiments. We use sparse matrix decomposition methods to identify clusters of a few related design variables. Sparse principal component analysis (SPCA) identifies groupings that are related to the physical origin of the variables (laser, hohlraum, and capsule). A variable importance analysis finds that in addition to variables highly correlated with neutron yield, such as picket power and laser energy, variables that represent a dramatic change of the ICF design, such as number of pulse steps, are also very important. The obtained sparse components are then used to train a random forest (RF) regression surrogate for predicting total yield. The RF performance on the training and testing data compares with the performance of the RF trained using all the design variables considered. This work is intended to inform design changes in future ICF experiments by augmenting the expert intuition and simulation results.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

High-yield magnetic recoil neutron spectrometer on the National Ignition Facility for operation up to 60 MJ

We report that recent progress at the National Ignition Facility (NIF), with neutron yields of order 1 x 10 17 , places new constraints on diagnostics used to characterize implosion performance. The Magnetic Recoil neutron Spectrometer (MRS), which is routinely used to measure yield, ion temperature (T ion ), and down-scatter ratio (dsr), has been adapted to allow measurements of dsr up to 5 x 10 17 , and yield and T ion up to 2 x 10 18 in the near term with new data processing techniques and conversion foil solutions. This paper presents a solution for extending MRS operation up to a yield of 2 x 10 19 (60 MJ) by moving the spectrometer outside of the NIF shield wall. This will not only enhance the upper yield limit by 10x but also improve signal-to-background by 5x.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Neutron Radiation Characteristics of Plutonium Dioxide Fuel

The major sources of neutrons from plutonium dioxide nuclear fuel are considered in detail. These sources include spontaneous fission of several of the Pu isotopes, reactions with low Z impurities in the fuel, and reactions with O-18. For spontaneous fission neutrons a value of (1.95 plus or minus 0.07) X 1,000 n/s/q PuO2 is obtained. The neutron yield from (alpha, neutron) reactions with oxygen is calculated by integrating the reaction rate equation over all alpha particle energies and all center-of-mass angles. The results indicate a neutron emission rate of (1.42 plus or minus 0.32) X 10,000 n/s/q PuO2. The neutron yield from (alpha, neutron) reactions with low Z impurities in the fuel is presented in tabular form for one part per million of each impurity. The total neutron flux emitted from a particular fuel geometry is estimated by adding the neutron yield due to the induced fission to the other neutron sources.

Taherzadeh, M.↗

Experimental validation of an integrated modelling approach to neutron emission studies at JET

An integrated modelling methodology for the calculation of realistic plasma neutron sources for the JET tokamak has been developed. The computational chain comprises TRANSP plasma transport and DRESS neutron spectrum calculations, and their coupling to the MCNP neutron transport code, bridging plasma physics and neutronics. Here, we apply the developed methodology to the analysis of neutron emission properties of deuterium and helium plasmas at JET, and validate individual modelling steps against neutron diagnostic measurements. Two types of JET discharges are modelled—baseline-like and three-ion radio-frequency scenarios—due to their diversity in plasma heating, characteristics of the induced fast ion population, and the imprint of these on neutron emission properties. The neutron emission modelling results are quantitatively compared to the total neutron yield from fission chambers, neutron emissivity profiles from the neutron camera, neutron spectra from the time-of-flight spectrometer, and neutron activation measurements. The agreement between measured and calculated quantities is found to be satisfactory for all four diagnostic systems within the estimated experimental and computational uncertainties. Additionally, the effect of neutrons not originating from the dominating D(D, n) 3 He reactions is studied through modelling of triton burnup DT neutrons, and, in mixed D- 3 He plasmas, neutrons produced in the 9 Be(D, nγ) 10 B reaction on impurities. It is found that these reactions can contribute up to several percent to the total neutron yield and dominate the neutron activation of samples. Finally, the effect of MeV-range fast ions on the neutron activation of 115 In and 27 Al samples is measured and computationally validated.

integrated modelling↗

PANDA-FES: Portable and Adaptable Neutron Diagnostics for Advancing Fusion Energy Science

Nuclear fusion is a potential source of carbon-free electricity with many concepts in development. The Portable and Adaptable Neutron Diagnostics for Advancing Fusion Energy Science (PANDA-FES) suite has been deployed since 2021 to measure neutron yield, energy, and spatiotemporal source location at two different Z-pinch fusion devices. This diagnostic can be used at a variety of facilities pursuing fusion in the magnetic, inertial, and magneto-inertial regimes. These different regimes have a wide range of time scales from less than 100 ns to a few μ s, neutron yields from 10 6 to 10 11 , and noise environments. Neutron yield is measured through activation of 79 Br and 89 Y with calibrated detectors. Temporal, spatial, and energy dependence of neutrons is measured with scintillators coupled to photomultiplier tubes (PMTs). Experimental setups and data analysis methods have been developed for these conditions. Finally, neutron yield, neutron energy anisotropy, and spatiotemporal evolution of the source have been measured.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Characterizing secondary neutrons at BLIP for isotope production applications

Fast secondary neutrons created at the Brookhaven Linac Isotope Producer (BLIP) facility following proton irradiation were characterized by the foil activation technique and compared with FLUKA Monte Carlo simulations. The FLUKA-simulated neutron flux was spectrally adjusted following the maximum entropy formalism using the International Reactor Dosimetry and Fusion File (IRDFF-II), with predictions agreeing with experimental measurements to within 9 % following the adjustment procedure. Here, a multitude of degrader configurations were simulated to assess the feasibility of improving the fast (E n > 20 MeV) secondary neutron yield at the proposed neutron target position (“N-slot”). A configuration where the N-slot is closest to the proton degrader produced the highest fast neutron yield, with tungsten degraders achieving the best performance. Assuming the optimized target-degrader configuration proposed in this work, we discuss potential isotope production opportunities with secondary neutrons. In most cases the yields are in the order of several mCi.

07 ISOTOPE AND RADIATION SOURCES↗

High yield polar direct drive fusion neutron sources at the National Ignition Facility

Polar direct drive neutron source experiments were performed at the National Ignition Facility showing substantial improvement in total neutron yield and efficiency of conversion of laser energy to fusion output. Plastic capsules 3–4 mm in diameter were filled with 1.5 mg/cc of deuterium–tritium (DT) fuel and imploded with laser beam pointing and defocus designed to compensate for polar asymmetry introduced by the facility beam entrance angles. Radiation-hydrodynamics simulations were employed to optimize the multi-dimensional laser and target parameter space, within facility and target fabrication constraints. Ensembles of 1D simulations tuned to match the outputs of early shots in the series were used to design subsequent shots in the series. This allowed the later shots to be designed based on empirically motivated sensitivities to laser and target input parameters, while eliminating the need to explicitly model phenomena such as hydrodynamic instabilities and nonlinear laser–plasma interactions. Additionally, one experiment with a 3.0 mm diameter CH capsule produced 13.6 kJ (4.81 × 10 15 DT neutrons) from a laser input below the NIF optics damage threshold at 585 kJ, 328 TW. Two experiments with 4.0 mm capsules produced 31.3 and 33.6 kJ of fusion output (1.11 × 10 16 and 1.19 × 10 16 DT neutrons) with 1.10 MJ, 390 TW and 1.26 MJ, 425 TW of laser input, respectively.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

(α,n) nuclear data scoping study

Neutrons from the (α,n) reaction are an important component of nondestructive assay techniques to determine enriched uranium and other actinide inventories in a variety of critical points in the nuclear fuel cycle. However, uncertainties in the cross section, total neutron yield and neutron spectrum, and gamma emissions from these reactions, such as 19 F(α,n) and 17,18 O(α,n), introduce large uncertainties in the determination of mass of actinides of interest and can represent several significant quantities in unaccounted material in certain facility processes. Calculations and measurements depend on accurate nuclear data; however, much of the relevant data in use today was measured in the 1980s and earlier and has not been updated. Thus, the current uncertainties in the cross sections and neutron emission spectra are unacceptably large. This report documents the results of a scoping study of (α,n) reaction data that considered the current state of the data and recommends areas of improvement. It also addresses the codes use to calculate the (α,n) neutron and gamma source terms and recommends code improvements to support required analysis.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Neutron radiation characteristics of plutonium dioxide fuel

The major sources of neutrons from plutonium dioxide nuclear fuel are considered in detail. These sources include spontaneous fission of several of the Pu isotopes, (alpha, n) reactions with low Z impurities in the fuel, and (alpha, n) reactions with O-18. For spontaneous fission neutrons a value of (1.95 + or - 0.07) X 1,000 n/s/g PuO2 is obtained. The neutron yield from (alpha, n) reactions with oxygen is calculated by integrating the reaction rate equation over all alpha-particle energies and all center-of-mass angles. The results indicate a neutron emission rate of (1.14 + or - 0.26) X 10,000 n/s/g PuO2. The neutron yield from (alpha, n) reactions with low Z impurities in the fuel is presented in tabular form for one part part per million of each impurity. The total neutron yield due to the combined effects of all the impurities depends upon the fractional weight concentration of each impurity. The total neutron flux emitted from a particular fuel geometry is estimated by adding the neutron yield due to the induced fission to the other neutron sources.

Taherzadeh, M.↗

Prediction of neutron production and energy spectrum by the inverse kinematic reaction between an incident 7 Li 3+ beam and a proton target in PHITS

A neutron source using the inverse kinematic reaction between lithium and proton, p( 7 Li, n) 7 Be, achieves forward-directed neutrons, potentially enhancing neutron yield in the forward direction. Despite the advantage, no evaluated-cross-section data for this reaction can be used in Monte Carlo simulation codes, such as PHITS. To solve this problem, this study aims to evaluate the applicability of the user-defined cross-section data, Frag data, for p ( 7 Li, n) 7 Be in PHITS. The simulations reproduced collisions between 7 Li 3+ ions and polypropylene targets. The Frag data was edited based on the JENDL-5 by utilizing the two-body collision kinematics. The neutron yield and angular distribution were investigated in the simulation. As a result, the forward neutron convergence with a reasonable neutron yield and energy spectrum was observed. The expected neutron yield in the forward 1-steradian area is 2.46 × 10 10 n/s when lithium-ion energy and current are 16.45 MeV and 0.1 mA.

43 PARTICLE ACCELERATORS↗

Overview of interpretive modelling of fusion performance in JET DTE2 discharges with TRANSP

In the paper we present an overview of interpretive modelling of a database of JET-ILW 2021 D-T discharges using the TRANSP code. The main aim is to assess our capability of computationally reproducing the fusion performance of various D-T plasma scenarios using different external heating and D-T mixtures, and to understand the performance driving mechanisms. We find that interpretive simulations confirm a general power-law relationship between increasing external heating power and fusion output, which is supported by absolutely calibrated neutron yield measurements. A comparison of measured and computed D-T neutron rates shows that the calculations' discrepancy depends on the absolute neutron yield. The calculations are found to agree well with measurements for higher performing discharges with external heating power above ~20 MW, while low-neutron shots display an average discrepancy of around +40% compared to measured neutron yields. A similar trend is found for the ratio between thermal and beam-target fusion, where larger discrepancies are seen in shots with dominant beam-driven performance. We compare the observations to studies of JET-ILW D discharges, to find that on average the fusion performance is well modelled over a range of heating power, although an increased unsystematic deviation for lower-performing shots is observed. The ratio between thermal and beam-induced D-T fusion is found to be increasing weakly with growing external heating power, with a maximum value of ≳1 achieved in a baseline scenario experiment. An evaluation of the fusion power computational uncertainty shows a strong dependence on the plasma scenario type and fusion drive characteristics, varying between ±25% and 35%. D-T fusion alpha simulations show that the ratio between volume-integrated electron and ion heating from alphas is ≲10 for the majority of analysed discharges. Alphas are computed to contribute between ~15% and 40% to the total electron heating in the core of highest performing D-T discharges. An alternative workflow to TRANSP was employed to model JET D-T plasmas with the highest fusion yield and dominant non-thermal fusion component because of the use of fundamental radio-frequency heating of a large minority in the scenario, which is calculated to have provided ~10% to the total fusion power.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Neutron-producing gas puff Z-pinch experiments on a fast, low-impedance, 0.5 MA linear transformer driver

A study on the neutron production from single and double gas puff Z-pinches on the CESZAR linear transformer driver with ~0.45 MA current and 170 ns rise time is presented. Total neutron yield measurements made with a LaBr activation detector are compared for three configurations, using a double nozzle setup. When a single, hollow, deuterium gas shell was used, reliable implosions could only be attained at higher load mass than the optimal value to match implosion time with the driver rise time, with neutron yields of ~10 6 per pulse. The use of a double gas puff configuration with a deuterium center jet allowed a reduction in the shell density and operation closer to machine-matched conditions, recording up to (4.1 ± 0.3) × 10 7 neutrons/pulse when either Kr or D 2 was used in the shell. For a comparable mass and implosion time, using a higher atomic-number gas in the outer shell results in more unstable plasma surface and smaller plasma radius at the location of instability bubbles, which, however, do not seem to consistently correlate with a higher neutron yield. Comparing implosion dynamics with models and neutron yields with literature scaling suggests that the machine current is not well coupled to the plasma during the final stages of compression. Optimizing current and energy coupling to the pinched plasma is critical to improving performance, particularly in low-impedance drivers.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Investigating boosted decision trees as a guide for inertial confinement fusion design

Inertial confined fusion experiments at the National Ignition Facility have recently entered a new regime approaching ignition. Improved modeling and exploration of the experimental parameter space were essential to deepening our understanding of the mechanisms that degrade and amplify the neutron yield. The growing prevalence of machine learning in fusion studies opens a new avenue for investigation. Here in this paper, we have applied the Gradient-Boosted Decision Tree machine-learning architecture to further explore the parameter space and find correlations with the neutron yield, a key performance indicator. We find reasonable agreement between the measured and predicted yield, with a mean absolute percentage error on a randomly assigned test set of 35.5%. This model finds the characteristics of the laser pulse to be the most influential in prediction, as well as the hohlraum laser entrance hole diameter and an enhanced capsule fabrication technique. We used the trained model to scan over the design space of experiments from three different campaigns to evaluate the potential of this technique to provide design changes that could improve the resulting neutron yield. While these data-driven model cannot predict ignition without examples of ignited shots in the training set, it can be used to indicate that an unseen shot design will at least be in the upper range of previously observed neutron yields.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Measurement of Neutron Multiplicity in Charged Current Neutrino Interactions on Oxygen

The Accelerator Neutrino Neutron Interaction Experiment (ANNIE) is a 26-ton gadolinium-doped water Cherenkov detector located 100~meters downstream in the Booster Neutrino Beam (BNB) at the Fermi National Accelerator Laboratory (Fermilab). Its primary goals are to (1) measure the neutron yield from $\nu_\mu$ interactions as a function of momentum transfer $Q^2$ so that neutrino-nucleus interaction models can be better constrained, and (2) demonstrate the power of novel, fast-timing detectors with the first deployment of Large Area Picosecond PhotoDetectors (LAPPDs). Current knowledge of neutrino-nucleus interactions fall short in modeling the topologies of such interactions, leading to inaccurate reconstruction of event kinematics such as particle energy, direction, and vertex. As a consequence, the accuracy of cross section measurements is impacted, which is necessary for precise physics measurements. Neutrons are an indication of inelasticity and affect the determination of the energy of the parent neutrino. Quantifying the neutron yield is a step towards reducing the associated uncertainties, and thus improving our understanding of these complex interactions and benefiting the next generation of long-baseline neutrino experiments. ANNIE will make use of LAPPDs to measure neutron multiplicity of CC-0$\pi$ $\nu_\mu$ interactions on oxygen, making it the first experiment to deploy an array of these photodetectors. Because the LAPPD is a novel photodetection technology, much customization is required to integrate it into existing electronics. The first half of this thesis covers the significant progress made towards the first deployment of the LAPPD system. From its test stand at Fermilab, the LAPPD system was systematically tested and put together until deployment readiness was achieved. I present my contributions to the design, fabrication, and testing of the waterproof housing and cables, and the commissioning of the LVHV board that powers the LAPPD and its readout electronics. These efforts brought the LAPPD system significantly closer to deployment, and eventually first data. The second half of this thesis presents the vertex and energy reconstruction algorithms developed to analysis the beam data with PMT-only information. While much progress has been made towards the deployment of LAPPDs, with several in the detector tank, efforts to integrate the LAPPD datastream are in progress. Thus, I developed a ring edge detection technique using PMT data to fit the muon vertex and determine its energy. The analysis in this thesis finds average neutron yields of $\Bar{n}_{data} = 0.452 \pm 0.039 (\text{stat}) \pm 0.27 (\text{sys})$ for a selection of muon neutrino candidates in the fiducial volume of ANNIE and corrected with an averaged neutron detection efficiency. An equivalent analysis for simulated beam data results in an average neutron yield of $\Bar{n}_{MC} = 0.582 \pm 0.018 (\text{stat}) \pm 0.25 (\text{sys})$. Future work includes application of efficiency corrections at a positional level, quantification of all systematic uncertainties, and neutron multiplicity measurements with other event topologies.

43 PARTICLE ACCELERATORS↗

Effect of laser preheat in magnetized liner inertial fusion at OMEGA

Integrated magnetized liner inertial fusion (MagLIF) experiments on the OMEGA laser system are modeled to investigate the effects of laser preheat on implosion performance. In both simulations and experiments, preheating the fuel with a laser enhances the neutron yield, with the maximum yield occurring at an optimal preheat laser energy. Increasing the preheat energy past the optimal value reduces the neutron yield. In simulations, the rate of the drop in neutron yield depends on the inclusion of the Nernst effect. The Nernst effect advects the magnetic field away from the center of the fuel region during the preheat stage of MagLIF on OMEGA and weakens magnetic-flux compression. If the Nernst effect is not included, the simulated drop in yield past the optimal preheat laser energy is more gradual as opposed to the sharper drop seen in experiments. Simulations are able to model trend in measured ion temperatures seen in experiments. Here, a mix model is used to show that including mix from the wall in the simulated fuel region further degrades the yield and lowers the optimal preheat laser energy. Simulations with mix predict that increasing the initial axial magnetic field may still enhance yield performance in integrated implosions.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Nonlinear light-output calibration of the oxygenated xylene scintillators used in OMEGA neutron time-of-flight spectrometers

Neutron time-of-flight (nTOF) spectrometers are essential instruments for measuring and evaluating the performance of inertial confinement fusion implosions. The neutron spectrometers utilized for the OMEGA laser include two liquid-based scintillators, each consisting of a large volume filled with xylene that is coupled to four photomultiplier tubes. Analysis of the signal from these detectors requires detailed knowledge of the scintillator’s light output, which is needed to fit the nTOF spectrum, from which the neutron energy spectrum is informed. The light output is nonlinearly proportional to the neutron energy, which, in turn, affects the interpretation of the neutron energy spectrum from a TOF signal. A recent campaign on OMEGA was performed to calibrate the xylene detectors and infer the shape of the light-output curve. The campaign utilized materials with increasing Z placed in the OMEGA target chamber to initiate scattering events with the 14 MeV fusion neutrons. This process leads to the production of backscatter neutrons of varying energies that appear as peaks in the nTOF data. Simulations using a neutron transport code were combined with the measured deuterium–tritium neutron yields to calculate the expected backscattered neutron yields from the well-known scattering cross sections of each material. Furthermore, the neutron-energy dependent light output of the scintillator inferred from the experiment is compared to the light-output curve simulated with a neutron transport code for the following neutron energies: 1.5, 2.5, 6, and 14 MeV.

47 OTHER INSTRUMENTATION↗

First measurement of the 10B(α,n)13N reaction in an inertial confinement fusion implosion at the National Ignition Facility: Initial steps toward the development of a radiochemistry mix diagnostic

We report the first measurement of the 10B(α,n)13N reaction in a polar-direct-drive exploding pusher (PDXP) at the National Ignition Facility (NIF). This work is motivated by the need to develop alternative mix diagnostics, radiochemistry being the focus here. The target is composed of a 65/35 at. % deuterium–tritium (DT) fill surrounded by a roughly 30 μm thick beryllium ablator. The inner portion of the beryllium ablator is doped with 10 at. % of 10B. Radiation-hydrodynamics calculations were performed in 1D to optimize both the remaining boron rho-R and the DT neutron yield. A charged-particle transport post-processor has been developed to study α-induced reactions on the ablator material. Results indicate a large 13N production from α-induced reactions on 10B, measurable by the radiochemical analysis of a gaseous samples system at the NIF. The PDXP target N201115-001 was successfully fielded on the NIF, and nitrogen from the 10B(α,n)13N reaction was measured. The 13N production yield, as well as the DT neutron yield, was, however, lower than expected. Some of the reduced yields can be explained by the oblate shape, but the ratios of the various radiochemical signals are not commensurate with expectations based on a simple reduction of the 1D results. Preliminary 2D radiation-hydrodynamics computations are consistent with the experimental measurements, and work is ongoing to extend the radiochemistry analysis into higher dimensions.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗