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At least 55 records · Page 3
All sourcesNASA NTRSDOE OSTI
NASA NTRS1995

Measurements of Band Intensities, Herman-Wallis Parameters, and Self-Broadening Line-Widths of the 30011 - 00001 and 30014 - 00001 Bands of CO2 at 6503 cm(exp -1) and 6076 cm(exp -1)

Rotationless band intensities and Herman-Wallis parameters are listed in HITRAN tabulations for several hundred CO2 overtone-combination bands. These parameters are based on laboratory measurements when available, and on DND calculations for the unmeasured bands. The DND calculations for the Fermi interacting nv(sub 1) + v(sub 3) polyads show the a(sub 2) Herman-Wallis parameter varying smoothly from a negative value for the first member of the polyad to a positive value for the final member. Measurements of the v(sub 1) + v(sub 3) dyad are consistent with the DND calculations for the a(sub 2) parameter, as are our recent measurements of the 4v(sub 1) + v(sub 3) pentad. However, the measurement-based values in the HITRAN tables for the 2v(sub 1) + v(sub 3) triad and the 3v(sub 1) + v(sub 3) tetrad do not support the DND calculated values for the a(sub 2) parameters. We therefore decided to make new measurements to improve some of these intensity parameters. With the McMath FTS at Kitt Peak National Observatory/National Solar Observatory we recorded several spectra of the. 4000 to 8000 cm(exp -1) region of pure CO2 at 0.011 cm(exp -1) resolution using the 6 meter White absorption cell. The signal/noise and absorbance of the first and fourth bands of the 3v(sub 1) + v(sub 3) tetrad of C-12O-16 were ideal on these spectra for measuring line intensities and broadening widths. Our selfbroadening results agree with the HITRAN parameterization, while our measurements of the rotationless band intensities are about 15% less than the HITRAN values. We find a negative value of a(sub 2) for the 30011-00001 band and a positive value for the 30014-00001 band, whereas the HITRAN values of a(sub 2) are positive for all four tetrad bands. Our a(sub 1) and a(sub 2) Herman-Wallis parameters are closer to DND calculated values than the 1992 HITRAN values for both the 30011-00001 and the 30014-00001 band.

Giver, L. P.↗
NASA NTRS1988

A very high resolution study of emission line widths in Galactic and extragalactic H II regions

Very high spectral resolution spectroscopy was performed using the 5007-A forbidden O III line on two Galactic H II regions (NGC 6611 and NGC 7000) and three giant extragalactic H II regions (NGC 588, NGC 604, and IC 133) in M33. Use of the thermally narrow forbidden O III line also aided in the determination of the broadening due to mass motion, although the results are in agreement with the average values obtained in earlier studies primarily done with H-alpha. Evidence is confirmed and found for multiple velocity components in each of the extragalactic systems.

O'Dell, C. R.↗
NASA NTRS2006

Temperature-Dependence of Air-Broadened Line Widths and Shifts in the nu3 Band of Ozone

The 9.6-micron bands of O3 are used by many remote-sensing experiments for retrievals of terrestrial atmospheric ozone concentration profiles. Line parameter errors can contribute significantly to the total errors in these retrievals, particularly for nadir-viewing. The McMath-Pierce Fourier transform spectrometer at the National Solar Observatory on Kitt Peak was used to record numerous high-resolution infrared absorption spectra of O3 broadened by various gases at temperatures between 160 and 300 K. Over 30 spectra were analyzed simultaneously using a multispectrum nonlinear least squares fitting technique to determine Lorentz air-broadening and pressure-induced shift coefficients along with their temperature dependences for selected transitions in the 3 fundamental band of (16)O3. We compare the present results with other measurements reported in the literature and with the ozone parameters on the 2000 and 2004 editions of the HITRAN database.

Smith, Mary A. H.↗
NASA NTRS1983

Sensitivity of ozone retrievals in limb-viewing experiments to errors in line-width parameters

The variance of atmospheric ozone concentration profiles retrieved in i.r. limb-viewing experiments is examined over the range of published ozone halfwidth values. Simulated retrievals are performed for a typical satellite-based high-resolution absorption experiment and a broad-band emission experiment. The results indicate that, for limb-viewing experiments, inaccurate collision-broadened linewidth values can lead to significant errors in retrieved profiles for broad-band radiometric data or for isolated strong lines in high-resolution spectra.

Smith, M. A. H.↗
NASA NTRS1991

Characteristics of intermediate-degree solar p-mode line widths

Measurements of the p-mode linewidths over the frequency range v = 1.87-4.93 mHz and degree range 1 = 1-150 are presented. The linewidth is observed to vary with mode frequency and degree. The variation with frequency is consistent with the observations of Libbrecht although the measurements are systematically narrower. The frequency variation has been explained in terms of radiative and convective damping of the modes. The observed variation with degree resolves previous contradictory results and is shown to exceed the 1/S variation that is expected in theoretical grounds. Here S is the travel time of a mode from its lower turning point in the solar interior, to its reflection at the solar surface. The deviations from a 1/S variation suggest that there are two possible damping mechanisms, in addition to radiative and convective damping, that affect the modes.

Jefferies, S. M.↗
NASA NTRS1991

Methane spectral line widths and shifts, and dependences on physical parameters

A detailed report of the recent high-resolution spectroscopic research on widths and shifts measured for a strong infrared-active fundamental of methane is presented. They were measured in collision with several rare gases and diatomic molecules, in the vibrational-rotational fundamental near 3000/cm. These measurements were made at an ambient temperature of 294 K over a range of pressures from 100 to 700 torr. The measurements are discussed in a preliminary but detailed and quantitative manner with reference to masses, polarizabilities, and quadrupole moments. Some functional dependences on these physical parameters are considered. The present data are useful for studies of corresponding planetary spectra.

Fox, K.↗
NASA NTRS1992

Line-width temperature dependence of selected R-branch transitions in the nu-3 fundamental of (N-14)2O-16 between 135 and 295 K

Tunable diode laser spectroscopy has been used to measure the temperature dependence of N2 foreign gas broadening coefficients for eight R-branch transitions in the nu-3 fundamental of (N-14)2O-16 at 135, 176, 210, and 295 K. The exponent n of the relation for quadrupole-quadrupole collisional interactions is found to range from 0.66 to 0.71, in approximate agreement with the theoretically predicted value of 0.75.

Loewenstein, Max↗
NASA NTRS1994

The Stokes line width and uncertainty relations

For a function given by contour integral the two types (conventions) of asymptotic representations are considered: the usual representation by asymptotic series in inverse powers of large parameters and the special division of contour integral in contributions of high and low saddle points. It is shown that the width of the recessive term formation zone (Stokes strip) in the second convention is determined by uncertainty relation and is much less than the zone width in the first convention. The reasons of such a difference is clarified. The results of the work are useful for understanding of formation region of the exponentially small process arising on the background of the strong one.

Nikishov, A. I.↗
NASA NTRS1999

Semiconductor Laser Line-width Measurements for Space Interferometry Applications

This work discusses results using the self-heterodyne delay atechnique to measure 1.3 um InP based DFB lasers. We will also address practical issues concerning detection and elimination of back reflections, choice of fiber length and resolution, and measurement of laser 1/f and current supply noise.

DFB laser delayed self-heterodyne interferometer l↗