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At least 55 records · Page 3

Conceptual design of inverted core lead bismuth eutectic fast reactor for marine applications

The development of an inverted core fast reactor aims to generate 60 MWth for about 30 Effective Full Power Years without refueling. The reactor design is a transportable reactor using UO{sub 2} fuel and lead-bismuth-eutectic cooled designed for marine applications and is intended to improve the reactor performances compared to the normal core design: better condition for passive cooling system capability by lower core pressure drop, taking advantage of potential power uprate from the lower maximum fuel temperature. Systematic design processes are presented in this work: fuel pin geometry selection, fuel assembly (FA) design, and core design. A relationship between pressure drops, coolant velocity, maximum fuel temperature, coolant channel diameter, and fuel volume fraction was introduced in a single graph used as a tool to select fuel pin geometry. Fuel fabrication capability also took place in consideration of FA design which led to 7 holes per FA, and two-dimensional temperature distribution studies were also carried out. Core design processes including radial zoning, axial zoning, and core optimization were conducted using Monte Carlo code MCS, which is UNIST CORE laboratory in-house code. The current core design uses 3 fuel enrichment levels and 3 FA types to control the local power distribution and power shift during its lifetime. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Dynamic Response Testing in an Electrically Heated Reactor Test Facility

Non-nuclear testing can be a valuable tool in development of a space nuclear power or propulsion system. In a non-nuclear test bed, electric heaters are used to simulate the heat from nuclear fuel. Standard testing allows one to fully assess thermal, heat transfer, and stress related attributes of a given system, but fails to demonstrate the dynamic response that would be present in an integrated, fueled reactor system. The integration of thermal hydraulic hardware tests with simulated neutronic response provides a bridge between electrically heated testing and full nuclear testing. By implementing a neutronic response model to simulate the dynamic response that would be expected in a fueled reactor system, one can better understand system integration issues, characterize integrated system response times and response characteristics, and assess potential design improvements at a relatively small fiscal investment. Initial system dynamic response testing was demonstrated on the integrated SAFE-100a heat pipe cooled, electrically heated reactor and heat exchanger hardware, utilizing a one-group solution to the point kinetics equations to simulate the expected neutronic response of the system (Bragg-Sitton, 2005). The current paper applies the same testing methodology to a direct drive gas cooled reactor system, demonstrating the applicability of the testing methodology to any reactor type and demonstrating the variation in system response characteristics in different reactor concepts. In each testing application, core power transients were controlled by a point kinetics model with reactivity feedback based on core average temperature; the neutron generation time and the temperature feedback coefficient are provided as model inputs. Although both system designs utilize a fast spectrum reactor, the method of cooling the reactor differs significantly, leading to a variable system response that can be demonstrated and assessed in a non-nuclear test facility.

Bragg-Sitton, Shannon M.↗

Computational Design of Improved Fast Reactor Cladding

HT9 ferritic-martensitic (FM) steel has served as a leading candidate for sodium-cooled fast reactor (SFR) cladding due to its favorable resistance to irradiation-induced swelling and good thermal and chemical properties. However, its limited creep strength at temperatures above 600 °C and susceptibility to α′ phase embrittlement under specific conditions could limit its application in next-generation SFRs.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Assessing the Impact of Effective Thermal Conductivity on Gas-cooled Reactor Transients in RELAP5-3D

In block-type high-temperature gas-cooled reactors (HTGRs), coolant holes in blocks lead to a reduction in heat transfer through conduction. In systems codes like RELAP5-3D, we must account for this degradation by using an effective thermal conductivity (ETC). This presentation discusses a few ETC relationships and demonstrates the impact of ETC for the modular High-Temperature Gas-Cooled Reactor 350 MW -- a computational benchmark for HTGR modeling -- and for the High Temperature Test Facility (HTTF) -- an HTGR thermal hydraulics test facility. We demonstrate that the use of ETC leads to temperatures that are higher than the bulk thermal conductivity of the block material would yield, but these differences have no meaningful impact on the transient performance of the reactors. The ETC also reduces the cooldown rate, leading to more time at elevated temperatures. Overall, while accounting for ETC is important in capturing the physics of the reactor, it is not expected to have a meaningful impact on transient performance.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Effects of Internal and External Heat Sources on Cladding Microstructure and Rupture Performance

In the event of a Loss of Coolant Accident (LOCA), the primary supply of cooling water for a nuclear reactor is lost, leading to a significant pressure differential across the cladding wall. Without adequate cooling, the fuel rods continue to heat as a result of fission reactions. Research at Oak Ridge National Laboratory’s (ORNL’s) Severe Accident Test Station (SATS) is currently focused on evaluating fuel cladding performance using an external infrared lamp as a heat source, whereas legacy testing primarily utilized an internal heating approach. While external heating may better simulate the effect of neighboring fuel rods heating a central rod, it may not accurately represent the internal heat absorption from the fuel during accident transients. The heating dynamics depend greatly on the fuel rod's position within the bundle and the reactor. To fully understand the implications of a LOCA event and assess the influence of internal heating on cladding performance, combined internal heating and pressurization capability was developed at ORNL. Tests were conducted to compare cladding segments heated internally (representing heat from the fuel within the rod) and externally (representing heat from adjacent fuel rods). The findings indicate that both internal and external heating result in comparable rupture temperatures during 5°C/s laboratory LOCA tests and also agree with legacy test data. Axial temperature gradients and internal heat source dispersal were found to significantly impact cladding deformation and rupture geometry. Clear modifications were outlined to further improve the capability with heating rates above 5°C/s.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Effects of Internal and External Heat Sources on Cladding Microstructure and Rupture Performance

In the event of a Loss of Coolant Accident (LOCA), the primary supply of cooling water for a nuclear reactor is lost, leading to a significant pressure differential across the cladding wall. Without adequate cooling, the fuel rods continue to heat as a result of fission reactions. Research at Oak Ridge National Laboratory’s (ORNL’s) Severe Accident Test Station (SATS) is currently focused on evaluating fuel cladding performance using an external infrared lamp as a heat source, whereas legacy testing primarily utilized an internal heating approach. While external heating may better simulate the effect of neighboring fuel rods heating a central rod, it may not accurately represent the internal heat absorption from the fuel during accident transients. The heating dynamics depend greatly on the fuel rod's position within the bundle and the reactor. To fully understand the implications of a LOCA event and assess the influence of internal heating on cladding performance, combined internal heating and pressurization capability was developed at ORNL. Tests were conducted to compare cladding segments heated internally (representing heat from the fuel within the rod) and externally (representing heat from adjacent fuel rods). The findings indicate that both internal and external heating result in comparable rupture temperatures during 5°C/s laboratory LOCA tests and also agree with legacy test data. Axial temperature gradients and internal heat source dispersal were found to significantly impact cladding deformation and rupture geometry. Clear modifications were outlined to further improve the capability with heating rates above 5°C/s.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Understanding Fission Gas Bubble Distribution and Zirconium Redistribution in Neutron-irradiated U-Zr Metallic Fuel Using Machine Learning

U-10wt.% Zr (U-10Zr) based metallic fuel is the leading candidate for next-generation sodium cooled fast reactor in United States. Currently, Idaho National Laboratory (INL) has been the leading national laboratory for research, development, and demonstration (RD&D) on metallic fuel. Advanced post-irradiation characterization will help to understand fuel microstructure and property change during irradiation, benefiting fuel qualification for commercial application. Characterization capabilities ranging from sub-nanometer to micrometer, such as scanning electron microscopy (SEM), focused ion beam (FIB) sampling, transmission electron microscopy (TEM) characterization, and local thermal conductivity microscopy (TCM), have been utilized recently on irradiated U-10Zr fuel samples to gain a better understanding of nuclear fuel microstructure and property evolution inside a reactor. The FIB/SEM coupled with energy dispersive X-ray spectroscopy (EDS) can capture the essential information to achieve better understanding of fuel behaviors. Inside a nuclear reactor, the phase and microstructure of U-10Zr is constantly changing under neutron bombardment. For example, the gaseous fission product atoms have a limited solubility inside fuel matrix and tend to precipitate out in bubble form, which not only contribute to fuel thermal conductivity degradation but also provide a shortcut for movement of fission products, i.e. lanthanides. The resultant deposition of lanthanides at the cladding inner surface will potentially trigger a chemical reaction/interaction between nuclear fuel and cladding at reactor operational conditions, threatening fuel integrity and safety. FIB/SEM coupled with EDS can provide the fission bubble information as well as probe into phase separation or Zr redistribution, which is fundamental to predict the fuel performance. With high velocity image data generating method, such as FIB/SEM, an automatic way to extract the microstructural information quantitively can better serve the needs from post irradiation characterization. A trained machine learning model, named Decision Tree, is employed to generate a bubble classifier and to categorize bubbles into three categories: isolated bubble, connected without lanthanides, and connected with lanthanides bubbles[3]. This work presents a showcase of this approach on six regions of a fuel cross-section along the radial temperature gradient. We obtained distributions of bubble categories and porosity rates along the six regions. Moreover, a secondary phase U-Zr2 was determined and found on regions 5 and 6. The secondary phase fraction was increasing from 15.61% in region 5 to 34.79% in region 6 based on this approach . This quantitative data offers insights into the lanthanide migration and potentially thermal conductivity degradation. This information from machine learning will be fed into fuel design code for better prediction of fuel performance.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Simulation of Isotopic Concentrations and Gamma Spectra from Dynamic Fission Sources

A tool was developed to rapidly generate synthetic gamma-ray spectra to evaluate safeguards material control and accounting methods for liquid-fueled molten salt reactors. Molten salt reactor operations pose unique challenges to nuclear safeguards methods and protocols compared to deployed reactors designs (e.g., light water reactors). This research evaluates the use of gamma-ray spectroscopy to monitor fission product isotopic flow through a reactor model to understand expected operations and investigate changes to the spectra with material diversion scenarios. The large design space of molten salt reactors (e.g., liquid-fueled, liquid-cooled, online separations) could potentially lead to many measurement points within the reactor system. The developed analytical tool generates and evaluates synthetic gamma-ray spectra from dynamic reactor simulations by extracting isotopic inventory to generate source terms. An implementation in the Gamma Detector Response and Analysis Software (GADRAS) Application Program Interface (API) uses the source terms, a model of the reactor component, a detector response function, and measurement plan to quickly generate and analyze spectra. Prospective measurements are then evaluated in the more accurate but slower Geant4 simulations. Utilization of the developed modeling tool and analysis of the subsequent spectra enables optimization of collimation, shielding requirements, and expected count rates that are used to determine key measurement points in the modeled reactor design.

O'Brien, Sean↗

A MOOSE-Based Model for Fission Product Transport and Source Term Estimation for High-Temperature Gas-Cooled Reactors

Thanks to fuel elements containing tristructural isotropic (TRISO) particles combined with a low core power density and passive feedback mechanisms leading to modest temperature rises in the event of accidental events, high-temperature gas-cooled reactors (HTGRs) offer a high degree of reliability in terms of fission product retention. While the anticipated source term for HTGRs is expected to be very low, it is important to provide a quantitative estimate of radiological releases during nominal and accidental conditions. Here, we propose a computationally efficient mechanistic source term methodology relying on the Multiphysics Object Oriented Simulation Environment (MOOSE) for tracking fission product transport from TRISO particles up to the coolant pressure boundary, as well as modeling the transport and potential deposition of these nuclides inside the reactor coolant loop. The proposed computational scheme is applied to estimate source term inventories for a representative 10-MW(thermal) prismatic high-temperature microreactor and is qualitatively compared against known release fractions. In addition to providing an alternate analysis tool, this MOOSE model can help reactor designers quantify the influence of key design parameters relevant for studies of radiological dose consequences.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Modeling of transient heat pipe operation

The use of heat pipes is being considered as a means of reducing the peak temperature and large thermal gradients at the leading edges of reentry vehicles and hypersonic aircraft and in nuclear reactors. In the basic cooling concept, the heat pipe covers the leading edge, a portion of the lower wing surface, and a portion of the upper wing surface. Aerodynamic heat is mainly absorbed at the leading edge and transported through the heat pipe to the upper and lower wing surface, where it is rejected by thermal radiation and convection. Basic governing equations are written to determine the startup, transient, and steady state performance of a haet pipe which has initially frozen alkali-metal as the working fluid.

Colwell, Gene T.↗

Grain growth kinetics of the gamma phase metallic uranium

We report metallic uranium is a leading fuel form for sodium cooled fast reactors as an enabling technology of future nuclear energy systems. Mechanistic understanding of fuel behaviors and kinetics under thermodynamic equilibrium and highly non-equilibrium conditions are essential for evaluating fuel performance. It is important to understand and predict the grain and pore evolutions of metallic fuels under thermal and irradiation conditions. However, very limited data are available on the grain growth kinetics and mechanisms of pure gamma phase uranium. In this paper, the pure gamma uranium pellets with different grain structures were fabricated by combining high-energy ball milling and spark plasma sintering. Isothermal annealing tests were performed to investigate the grain growth behavior of the pure gamma phase uranium with different initial grain sizes. A parabolic relationship in grain growth with time was identified for the submicron-sized (374 nm) sample. In contrast, for the nano-sized (137 nm) sample, the grain growth shows a linear relationship with time. The activation energies of grain growth were determined as 199.5 KJ/mol and 80.6 KJ/mol for nano-sized and submicron-sized grain structures, respectively. For the nano-sized sample, the rate-control step of grain growth is dominated by the triple-junction migration, in which the grain boundary triple junction drags the grain growth, leading to a higher activation energy than the bulk diffusion. The dominating mechanism for the submicron-sized sample is grain boundary diffusion. The mechanistic understanding and critical data obtained on the kinetics of pure uranium phases will be useful to evaluate fuel behavior under thermodynamic equilibrium conditions and develop a high fidelity model to predict fuel performance.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Informing and Engaging the Future Workforce on Generation IV International Forum Reactor Systems

Generation IV reactors are six nuclear reactor designs, Sodium Fast reactor (SFR), Very High Temperature Reactor (VHTR), Gas cooled Fast Reactor (GFR), Molten Salt Reactor (MSR), Lead Fast Reactor (LFR), and Supercritical Water Reactor (SCWR), that are considered to be the most promising in light of various criteria based on the following objectives: • continuation of the progress made by Generation III water reactors in terms of competitiveness and safety; • more effective use of uranium resources; • less radioactive waste, especially high-level, long-lived waste; • greater protection against malicious acts and the diversion or theft of nuclear materials. The GIF Education and Training Working Group (ETWG) launched two major initiatives in 2016 and in 2021 to not only inform and educate but also to engage the future workforce in support of these reactor systems. This paper will present an overview of the GIF EWTG webinar series as well as the 2021 Pitch your Gen IV Research Competition which is followed by the 2023 Pitch your Gen IV Research. Competition

Paviet, Patricia D.↗

Qualification of System-Level Advanced Reactor Safety Analysis Software for Lead Systems: Final CRADA Report

SAS4A/SASSYS-1 is a simulation tool used to perform deterministic analysis of anticipated events as well as design basis and beyond design basis accidents for advanced liquid-metal-cooled nuclear reactors. With its origin as SAS1A in the late 1960s, the SAS series of codes has been under continuous use and development for over forty-five years and represents a critical investment in safety analysis capabilities for the U.S. Department of Energy. Although SAS4A/SASSYS-1 was developed to support the analysis of any liquid-metal-cooled nuclear reactor, it has primarily been utilized to design and analyze Sodium Fast Reactors (SFRs). As a result, most of the qualification basis for SAS4A/SASSYS-1 has utilized sodium as a coolant and geometry descriptions that are prototypic of SFR configurations. In this project, which partnered with Westinghouse Electric Company, LLC, the initial foundation for a qualification basis centered on prototypic pool-type lead-cooled systems has been established, where the end goal is to extend support for utilization of SAS4A/SASSYS-1 in Lead Fast Reactor (LFR) licensing or authorization. This project included three fundamental technical tasks: LFR V&V test suite development (Task 1); qualification support for LFRs (Task 2); and LFR modeling capabilities evaluation and improvement (Task 3)

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Capability Enhancements for System-level thermal Hydraulic Modeling of Lead Fast Reactors

This project has focused on the use, assessment, and development of the SAS4A/SASSYS-1 (SAS) safety analysis software. Although SAS was originally intended as a safety analysis tool for Liquid Metal cooled Fast Reactors (LMFRs), which includes both Sodium Fast Reactors (SFRs) and Lead Fast Reactors (LFRs), the vast majority of its recent development and customization has been tailored to SFRs. In general, enhancements that are made to the software for SFRs are applicable to LFRs, however, the fuel composition and corrosive nature of lead requires careful consideration when performing safety analysis of an LFR. In this project an emphasis was placed on closing gaps that are associated with modeling LFRs using SAS. The principal objective of the project was to enhance the ability of SAS as a licensing tool for LFRs. This objective was to be accomplished through three tasks: 1) Enhance the ability of SAS to couple with external software; 2) Improve the underlying physics models in SAS, with priority given to models that are highly relevant to LFRs; 3) Extend the Verification and Validation (V&V) basis of the software

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

A fine pore-preserved deep neural network for porosity analytics of a high burnup U-10Zr metallic fuel

Abstract U-10 wt.% Zr (U-10Zr) metallic fuel is the leading candidate for next-generation sodium-cooled fast reactors. Porosity is one of the most important factors that impacts the performance of U-10Zr metallic fuel. The pores generated by the fission gas accumulation can lead to changes in thermal conductivity, fuel swelling, Fuel-Cladding Chemical Interaction (FCCI) and Fuel-Cladding Mechanical Interaction (FCMI). Therefore, it is crucial to accurately segment and analyze porosity to understand the U-10Zr fuel system to design future fast reactors. To address the above issues, we introduce a workflow to process and analyze multi-source Scanning Electron Microscope (SEM) image data. Moreover, an encoder-decoder-based, deep fully convolutional network is proposed to segment pores accurately by integrating the residual unit and the densely-connected units. Two SEM 250 × field of view image datasets with different formats are utilized to evaluate the new proposed model’s performance. Sufficient comparison results demonstrate that our method quantitatively outperforms two popular deep fully convolutional networks. Furthermore, we conducted experiments on the third SEM 2500 × field of view image dataset, and the transfer learning results show the potential capability to transfer the knowledge from low-magnification images to high-magnification images. Finally, we use a pre-trained network to predict the pores of SEM images in the whole cross-sectional image and obtain quantitative porosity analysis. Our findings will guide the SEM microscopy data collection efficiently, provide a mechanistic understanding of the U-10Zr fuel system and bridge the gap between advanced characterization to fuel system design.

36 MATERIALS SCIENCE↗

Quantitative Insight to Fission Gas Pores Distribution in Irradiated Annular U-10Zr Metallic Fuel Using Machine Learning

Metallic fuels, particularly U-10Zr and its performance in reactor irradiation conditions, have been thoroughly investigated and are a promising candidate for next-generation sodium-cooled fast spectrum nuclear reactors. Irradiation in reactors can lead to the formation of fission gas and increased pore formation which can significantly impact fuel performance. Due to the large number of pores and various phases formed in metallic fuel during irradiation, a quantitative description of fission gas pores as a function of irradiation conditions is not yet available, undermining the fidelity of fuel performance modeling to support fuel qualification. It has been difficult to clearly detect pore boundaries and distinguish matrix phases from fission gas pores using optical microscopy by using simple threshold methods working with low magnification images. The pre-trained deep learning model for fission gas pore detection was applied to ~10,260 high magnification scanning electron microscopy images. The model increased the accuracy of fission gas pore segmentation to obtain statistical features, which cannot be processed manually. A pre-trained decision tree model was used to classify pores as isolated or connected pores, providing new insight into the correlation between the movement of lanthanides, solid fission products, and the radial temperature gradient developed in fuel irradiation conditions. This paper emphasizes the potential that artificial intelligence-based machine learning models have to accelerate qualification and support nuclear fuel development.

36 MATERIALS SCIENCE↗

Segmentation and Classification of Fission as Pores in Reactor Irradiated Annular U–10Zr Metallic Fuel Using Machine Learning Models

Metallic fuels, particularly U—10Zr, are promising candidates for next-generation sodium-cooled fast reactors. Irradiation of nuclear fuels in reactors can lead to the formation of solid and gas fission product which subsequently forms microstructural pores, deteriorating fuel performance. Due to the massive amount of pores and complex phases formed, a quantitative description of fission gas pores is not yet available, preventing the development of microstructure-informed fuel performance modeling for fuel qualification. This paper applied a pre-trained deep learning model to ~10,260 high magnification scanning electron microscopy images. This method increased the accuracy of fission gas pore segmentation and allows statistical features to be extracted which cannot be achieved manually. A pre-trained decision tree model worked on the segemenation results and further classified the pores into different categories to produce a correlation between the pores, movement of lanthanides, and temperature gradient during irradiation. Finally, this paper emphasizes the potentials of machine learning models to accelerate fuel research, development, and qualification for advanced reactors.

36 MATERIALS SCIENCE↗