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At least 55 records · Page 3
All sourcesNASA NTRSDOE OSTI
DOE OSTI2026

Signal-to-background estimates for the inverse-kinematics 78 Kr(n,γ) experiment at LANSCE

The idea of a neutron target enables the measurement of neutron-induced reactions in inverse kinematics. This idea is part of the LANSCE strategy to stay a worldwide leader for neutron-induced research. The proof-of-principle experiment outlined in is the core of the LDRD project 20240004DR. The current approach is to use an ion source capable of accelerating single-charged ions up to about 60 keV. A beam of 78 Kr + ions will be created to interact with a neutron target and implanted. During the passage of the target, neutrons can be captured and the freshly produced 79 Kr + ions will be implanted along with the main beam.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
NASA NTRS1971

Xe and Kr analyses of silicate inclusions from iron meteorites.

Measurements have been conducted of the amounts and isotopic composition of Xe and Kr in silicate inclusions of several iron meteorites. It is shown that the Xe and Kr contents are comparable to chondritic values. The isotopic compositions show trapped gas of both chondritic and atmospheric composition. Large spallation effects occur in some of the meteorites; the spallation spectra in some instances differ from those reported for stone meteorites. In several meteorites, very large neutron capture effects on Br and I occur. All samples have pronounced Xe129 excesses which apparently indicate differences in the formation times from chondrites of less than about 100 million years; however, the presence of trapped Xe132 in silicates which were enclosed in molten Fe-Ni and cooled slowly proves that they were not entirely outgassed, so that some of the Xe129 excess may also be trapped.

Bogard, D. D.↗
NASA NTRS1981

Assignment of the /Li-7/2 optically pumped laser transitions pumped by Ar/+/ and Kr/+/ laser lines

Welling and Wellegehausen (1977) have reported a list of Na2 and Li2 lines (belonging to B-X and A-X systems) which lase when vapors of these dimers are pumped with an Ar(+) or Kr(+) laser. A description is presented of a fluorescence study of the A-X system of the (Li-7)2 molecule excited by a Kr(+) laser (6471 A). The optically pumped laser lines are identified as P and R doublets in two different fluorescence series. The conditions which favor lasing action of these lines are pointed out. All but one of the known optically pumped laser lines of (Li-7)2 along with their assignments are presented in a table. For each pumping line, several additional wavelengths are listed which satisfy the condition for laser oscillations and which might well lase well under slightly improved conditions.

Verma, K. K.↗
NASA NTRS1983

Short wavelength laser calculations for electron pumping in neon-like krypton (Kr XXVII)

Calculations of electron impact collision strengths and spontaneous radiative decay rates are made for neon-like krypton (Kr XXVII) for the 2s2 2p6, 2s2 2p5 3s, 2s2 2p5 3p, and 2s2 2p5 3d configurations. From these atomic data, the level populations as a function of the electron density are calculated at two temperatures, 1 x 10 to the 7th K and 3 x 10 to the 7th K. An analysis of level populations reveals that a volume of krypton in which a significant number of the ions are in the Kr XXVII degree of ionization can produce a significant gain in transition between the 2s2 2p5 3s and 2s2 2p5 3p configurations. At an electron density of 1 x 10 to the 19th/cu cm the plasma length has to be of the order of 1 m; at a density of 1 x 10 to the 21st/cu cm the length is reduced to approximately 0.5 cm; and at an electron density of 1 x 10 to the 22nd/cu cm the length of the plasma is further reduced to approximately 1 mm.

Feldman, U.↗
NASA NTRS1987

Isotopic fractionation of Kr and Xe implanted in solids at very low energies

Results on the implantation of Kr and Xe in W under closed system conditions at very low energies (50-500 eV) are reported. Investigation of the fraction of gas trapped as a function of time reveals the existence of competing trapping and release mechanisms, and analysis of recovered trapped gas and residual gas phases shows that both elemental and isotropic fractionation result from these mechanisms. It is determined that the mass dependence for the overall implantation process is at or near m exp 1, with heavier isotopes enriched in the implanted gas. This mass dependence is inferred to result from implantation and a combination of diffusive and gas sputtering release mechanisms. These results reaffirm the conclusion of Bernatowicz and Fahey (1986) that previously observed isotopic fractionation of Kr and Xe in carbonaceous material synthesized in electrical discharges owes its origin to low-energy ion implantation, and also suggest that this process may be relevant to incorporation of noble gases in early solar system materials. The implication of these results for noble gas mass spectrometry are discussed.

Bernatowicz, Thomas J.↗
NASA NTRS1988

Trapping Ne, Ar, Kr, and Xe in Si2O3 smokes

Simple Si2O3 smokes have been condensed at both low (less than 750 K) and high (greater than 1000 K) temperature at 35 torr H2 pressure in the presence of 0, 10, 100, and 1000 microns of a noble gas mixture containing Ne, Ar, Kr, and Xe. In general, both Ne and Ar are quite loosely bound in the smokes (6.0 x 10 to the -8th and 2.6 x 10 to the -4th ccSTP/g, respectively), and are degassed at temperatures below 1200 K. Both Kr and Xe are somewhat more strongly bound at concentrations of 1.0 x 10 to the -7th and 8.2 x 10 to the -8th ccSTP/g, respectively, and in addition show a double release with a second component at a temperature of about 1875 K. With the exception that Si2O3 smokes appear to show a particular affinity for argon, possibly due to an anomalous absorption of atmospheric argon, none of the other noble gases are found in sufficient concentration to explain the gases observed in meteorites as primary circumstellar condensates. However, this data in conjunction with observations of Honda et al. (1979) do seem to show a degree of dependence between noble gas retention and chemical composition.

Nuth, Joseph A., III↗
NASA NTRS1993

Abundance and composition of solar KR in the H3-H6 chondrite ACFER111

He/Ne, Ne/Ar, and Ar/Kr abundance ratios of solar gases extracted by stepped heating, stepped oxidation, and stepped etching of lunar and meteoritic regoliths are significantly lower than ratios measured directly or predicted by model estimates. Of these, the differences in the He/Ne and Ne/Ar ratios are explained to be owing to diffusive fractionation losses from the host minerals. In contrast, it remains controversial if the Ar/Kr and Kr/Xe ratios were fractionated prior to or after the implantation of the gases into the minerals. In the H3-H6 chondritic regolith breccia ACFER 111, measured He/Ne and Ne/Ar ratios appear to be of nearly unfractionated solar composition. The Ar/Kr ratio of ACFER 111, might thus be also unfractionated. We examined by stepped etching a metal sample of ACFER 111 and obtained an average solar 36Ar/84Kr = 3150 plus or minus 300 which is in agreement with the model predictions. The isotopic composition of solar Kr was observed to change in the course of the etching in a way very similar to that report for lunar ilmenites by the Zurich group. This can be interpreted as a change of the mixing ratio of Solar Wind (SW) and Solar Energetic Particles (SEP). The isotopic composition of the SEP component obtained from our Kr data, however, is distinct from that reported by the Zurich group.

Pedroni, A.↗
NASA NTRS2001

Neutron-Capture Kr-80 and Ar-36 in the Martian Atmosphere and Regolith

We calculate that approximately 10% of martian atmospheric Kr-80 formed by neutron capture on Mars in approx. 0.5 Ga. The regolith contains even larger amounts of n-capture Kr-80 and Ar-36, which may provide clues to the evolution of the martian regolith and atmosphere. Additional information is contained in the original extended abstract.

Rao, M. N.↗
NASA NTRS2005

Rare Gases Inserted into Biological Building Blocks: A Theoretical Study of Glycine - Rg Compounds (Rg-Xe, Kr, Ar)

Compounds formed by insertion of rare-gas atoms (Xe, Kr, and Ar) into glycine molecule are investigated using accurate ab initio computational methods. Identification of such insertion compounds may open new frontiers in the field of rare-gas chemistry, such as possible existence of biological molecules that include chemically bound rare gas atoms. The most stable glycine-Rg configuration is found to correspond to insertion of Rg atoms into the 0-H bond of glycine. These NH2CH2COORgH compounds are metastable , but separated by sizable potential barriers from the Rg + glycine dissociation products. Preliminary calculations show that NH2CH2COOXeH compound is energetically stable with respect to another (3-body) dissociation channel (NH2CH2COO + Rg + H), while the corresponding Ar species is not stable in this respect. The compound with the inserted Kr is a borderline case, with the 3-body dissociation products being close in energy to the NH2CH2COOKrH minimum.

Chaban, Galina M.↗
DOE OSTI2022

In-situ TEM study of Kr ion irradiation tolerance of SiFeOC nanocomposite

Here, in this work, ion irradiation of polymer derived SiFeOC nanocomposite was carried out using 1.2 MeV Kr ions at room temperature and 600°C. The starting composite was composed of Fe 3 Si, SiC, SiOC, SiO 2 , and graphitic C. In-situ TEM investigations show uniform distribution of nano-crystalline Fe 3 Si and SiC phases in the amorphous SiOC matrix. During ion irradiation, the SiOC bulk microstructure and interfaces between Fe 3 Si or SiC crystallites and the SiOC matrix remain defect-free and demonstrate outstanding ion irradiation resistance. At room temperature, the crystalline domains are stable up to 2 dpa. At 600°C, Fe 3 Si crystallites are more stable than SiC; SiC crystallites are stable up to 4 dpa while the Fe 3 Si crystallites are stable up to 10 dpa. These crystallites also coalescence and amorphize simultaneously during ion irradiation. The exceptional tolerance to defect formation and irradiation of the SiFeOC nanocomposite provides important guidance to developing irradiation resistant fuels for advanced gas cooled reactors.

36 MATERIALS SCIENCE↗
DOE OSTI2022

Observation and diagnostic application of Kr K-shell emission in magnetized liner inertial fusion experiments at Z

In a series of Magnetized Liner Inertial Fusion (MagLIF) experiments performed at the Z pulsed power accelerator of Sandia National Laboratories, beryllium liners filled with deuterium gas pressures in the 4–8 atm range and a tracer amount of krypton were imploded. At the collapse of the cylindrical implosion, temperatures in the 1–3 keV range and atom number densities of ∼1023 cm−3 were expected. The plasma was magnetized with a 10 T axial magnetic field. Krypton was added to the fuel for diagnosing implosion plasma conditions. Krypton K-shell line emission was recorded with the CRITR time-integrated transmission crystal x-ray spectrometer. The observation shows n = 2 to n = 1 line emissions in B-, Be-, Li-, and He-like Kr ions and is characteristic of the highest electron temperatures achieved in the thermonuclear plasma. Detailed modeling of the krypton atomic kinetics and radiation physics permits us to interpret the composite spectral feature, and it demonstrates that the spectrum is temperature sensitive. We discuss temperatures extracted from the krypton data analysis for experiments performed with several filling pressures.

Clapp, J. T. (ORCID:0000000219928146)↗
DOE OSTI2026

Project 8 apparatus for cyclotron radiation emission spectroscopy with 83m Kr and tritium

Cyclotron Radiation Emission Spectroscopy (CRES) is a novel technique for the precise measurement of relativistic electron energy. This technique is being employed by the Project 8 collaboration for measuring a high-precision tritium beta decay spectrum to perform a frequency-based measurement of the neutrino mass. In this work, we describe the Project 8 Phase II apparatus, used for the detection of the CRES signal from the conversion electrons of 83m Kr and the first CRES measurement of the beta-decay spectrum of molecular tritium.

Neutrino detectors↗
DOE OSTI2024

Cyclotron radiation emission spectroscopy of electrons from tritium $β$ decay and 83m Kr internal conversion

Project 8 has developed a novel technique, cyclotron radiation emission spectroscopy (CRES), for direct neutrino mass measurements. A CRES-based experiment on the beta spectrum of tritium has been carried out in a small-volume apparatus. Here, we provide a detailed account of the experiment, focusing on systematic effects and analysis techniques. In a Bayesian (frequentist) analysis, we measure the tritium endpoint as ${18}$ ${553}_{—19}^{+18}$ (${18}$ ${548}_{—19}^{+19}$) eV and set upper limits of 155 (152) eV (90% C.L.) on the neutrino mass. No background events are observed beyond the endpoint in 82 days of running. We also demonstrate an energy resolution of 1.66 ± 0.19 eV in a resolution-optimized magnetic trap configuration by measuring 83m Kr 17.8-keV internal-conversion electrons. These measurements establish CRES as a low-background, high-resolution technique with the potential to advance neutrino mass sensitivity

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2025

Measurement of the inhomogeneity of the KATRIN tritium source electric potential by high-resolution spectroscopy of conversion electrons from $\mathbf {^{83m}}$Kr

Precision spectroscopy of the electron spectrum of the tritium β-decay near the kinematic endpoint is a direct method to determine the effective electron antineutrino mass. The KArlsruhe TRItium Neutrino (KATRIN) experiment aims to determine this quantity with a sensitivity of better than 0.3 eV (90% C.L.). An inhomogeneous electric potential in the tritium source of KATRIN can lead to distortions of the β-spectrum, which directly impact the neutrino-mass observable. This effect can be quantified through precision spectroscopy of the conversion-electrons of co-circulated metastable 83m Kr. Therefore, dedicated, several-weeks long measurement campaigns have been performed within the KATRIN data taking schedule. In this work, we infer the tritium source potential observables from these measurements, and present their implications for the neutrino-mass determination.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗