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At least 55 records · Page 3
All sourcesNASA NTRSDOE OSTI
NASA NTRS1989

Isotopic abundances of stratospheric ozone from balloon-borne high-resolution infrared solar spectra

IR solar absorption spectra at 0.002-0.0003/cm resolution in the 10-micron region obtained during two balloon flights near 32 deg N latitude are examined to determine the isotopic ratios of (O-16)(O-16)(O-18) and (O-16)(O-18)(O-16) relative to normal ozone in the stratosphere. For November 18, 1987, the results show column-averaged isotopic enhancement ratios of 1.20 + or - 0.14 and 1.40 + or - 0.18 for (O-16)(O-18)(O-16)/(O-16)(O-16)(O-16) and (O-16)(O-16)(O-18)/(O-16)(O-16)(O-16), respectively. The corresponding values for June 6, 1988, show ratios of 1.16 + or - 0.08 and 1.25 + or - 0.12. The results are compared with heavy-to-normal O3 ratios obtained using other techniques.

Goldman, A.↗
NASA NTRS1980

Some isotopic abundances in the cosmic radiation

Cosmic ray nuclei with Z not less than 10 have been observed in a detector which measures charge with a double scintillator-Cherenkov array and mass by combining the Cherenkov signal with residual range measured in nuclear emulsions. Results are presented for the isotopic analyses of Al, Ca, Sc, Mn, Fe, Co, Ni and Cu in the energy range 300-800 MeV/amu.

Young, J. S.↗
NASA NTRS1979

Cosmic ray isotope abundances from chromium to nickel

IRIS, a telescope consisting of a large-area precision Cerenkov detector, scintillators, spark chambers, and a passive stack of Lexan polycarbonate track detectors, was exposed to the primary cosmic radiation for 6.6 sq m sr hr in a balloon flight in 1976. This measurement has yielded the isotopic composition of the iron-group elements Cr, Mn, Fe, and Ni with an average mass resolution of 0.65 amu for the energies 320-500 MeV per amu at the detector. This experiment places the most severe constraints to date on deviation from solar-system composition of the source of the cosmic radiation. Upper limits of 10 percent are placed on the ratios Fe-54/Fe-56 and Fe-58/Fe-56, which are inconsistent with large departures from solar system source composition reported by other workers. The isotopic measurements of Fe and Ni preclude the possibility that these cosmic rays were produced in a single e-process zone. The mean mass of Mn is less than 55, indicating the presence of electron-capture species produced by spallation.

Tarle, G.↗
NASA NTRS1979

Upper limits on argon isotope abundances in the Venus thermosphere

On December 9, 1978 the neutral gas mass spectrometer aboard the NASA Pioneer Venus multiprobe bus has measured density, composition, and temperature of the Venus dayside thermosphere. There was no positive identification of argon down to the lowest measuring altitude of 130 km. For the altitude level of 135 km the following upper limits for the number densities of argon isotopes were derived: n(Ar-36) less than 1.3 times 10 to the 6th power per cu cm and n(Ar-40) less than 2.8 times 10 to the 6th power per cu cm. From our upper atmosphere observations we infer for the troposphere of Venus the following upper limits for the mixing ratios: n(Ar-36)/total number density less than 9 times 10 to the minus 6th power and n(Ar-40)/total number density less than 20 times 10 to the minus 6th power.

Mauersberger, K.↗
NASA NTRS1974

Isotopic abundances and line formation in the Orion Nebula

Measurements of the spatial variation of HC-12N-14 and HC-13N-14 line emission from the molecular cloud associated with the Orion Nebula indicate that HC-12N-14 has a high central opacity. This result seems to contradict a recent suggestion that the observed hyperfine structure of the line indicates a low opacity, which in turn would yield a C-13/C-12 abundance significantly different from other determinations. The observed hyperfine structure can be understood in the high-opacity case if radiative trapping in the lines is considered.

Wannier, P. G.↗
NASA NTRS1979

The elemental and isotopic abundances of H, C, N, O in comets

The elemental abundances of light elements in comets is discussed by considering gas and dust separately. It is noted that the icy conglomerate model of the nucleus (Whipple, 1957) has been confirmed, and that the dust-to-gas mass ratio has been estimated within a factor of two for two recent comets. It is found that the total amount of oxygen available is also nominally in solar abundance; this implies that the oxygen of the solar nebula has probably been quantitatively bound in compounds that have been completely condensed and accreted in cometary nuclei. In addition, the amount of hydrogen is clearly depleted by a factor of 2,000, suggesting that the only hydrogen present is that linked in molecular compounds of H, C, N and O.

Delsemme, A. H.↗
NASA NTRS1987

Radio observations of carbon monoxide toward Zeta Ophiuchi - Velocity structure, isotopic abundances, and physical properties

This paper presents a small-scale map of the molecular gas around the line of sight toward Zeta Oph made with measurements of the (C-12)O (1-0) emission obtained at high signal-to-noise ratio and high velocity resolution. In addition, a measurement of the (C-12)O (2-1) line emission and a detection of (C-13)O along the line of sight to the star are reported. The results show that the CO emission toward the star is composed from at least four components with peak velocities at -2.0, -0.7, 0.0, and +0.6 km/s. The radio observations yield a total CO column density of 1.4 x 10 to the 15th/sq cm, with about one-half of the total CO column density being in the main component at -0.7 km/s. The main cmponent is uniform over the map, but the other components are variable, suggesting that the cloud is clumpy. The data on the two CO transitions imply that the excitation temperature and the density of the main component are about 7 K and 800/cu cm, respectively.

Langer, William D.↗
NASA NTRS1978

Nitrogen abundances and isotopic compositions in stony meteorites

Nitrogen contents range from a few parts per million in ordinary chondrites and achondrites to several hundred parts per million in enstatite chondrites and carbonaceous chondrites. Four major isotopic groups are recognized: (1) C1 and C2 carbonaceous chondrites, (2) enstatite chondrites, (3) C3 chondrites, and (4) ordinary chondrites. The major variations are primary, representing isotopic abundances established at the time of condensation and accretion. Secondary processes, such as spallation reactions, solar wind implantation and metamorphic loss may cause small but observable isotopic variations in particular cases. The large isotopic difference between enstatite chondrites and carbonaceous chondrites cannot be accounted for by equilibrium condensation from a homogeneous nebular gas, and requires either unusually large kinetic effects, or a temporal or spatial variation of isotopic composition of the nebula. Nitrogen isotopic heterogeneity in the nebula due to nuclear processes has not been firmly established, but may be required to account for the large variations found within the Allende and Leoville meteorites. The unique carbonaceous chondrite, Renazzo, also requires a special source. It is not yet possible, from the meteoritic data, to establish the mode of accretion of nitrogen onto the primitive earth.

Kung, C.-C.↗
NASA NTRS1994

Search for important weak interaction nuclei in presupernova evolution

A search is made for the most important electron captures and beta-decays after core silicon burning in massive stars. A nuclear statistical equilibrium code is used to compute isotopic abundances. Electron capture and beta-decay rates are estimated for the 150 most abundant isotopes in a simplified fashion which generally includes the strongest transitions. These estimates are made for nuclei in the fp-shell and use techniques similar to Fuller, Fowler, & Newman (1982a), and are compared to them. The general behavior of the rate of change of Y(sub e) is examined. These methods are then used to follow a typical stellar trajectory, seeking the most important weak interactions during the formation of the iron core. Ranked lists of nuclei are given, to prioritize more detailed studies on individual nuclei. Beta-decays are found to ben an important modification to the evolution below the rate of change of Y(sub e) approx. = 0.46 as the core approaches a state of dynamic equilibrium between electron captures and beta-decays.

Aufderheide, Maurice B.↗
NASA NTRS1999

Comets after Hyakutake and Hale-Bopp

Being icy, cometary nuclei are the most easily modified bodies in the solar system - even modest heating is sufficient to induce significant weight loss. This sublimative loss and longterm storage far from the sun protect the nucleus against internal warming and ensure that cometary nuclei today contain the least processed material remaining from the early nebula - or perhaps from the natal cloud. The chemical compositions of ices, low temperature-refractory organics, and refractory minerals (and their physical states) provide sensitive probes of the origin and history of this material. The fortunate appearance of Hyakutake and Hale-Bopp has provided a wealth of information on these Oort cloud comets, obtained with a wide range of astronomical approaches. I will review certain key results for these comets, such as chemical abundances, isotopic abundance ratios, nuclear spin statistics, and nuclear vs extended production of "parent volatiles", and will illustrate how these test the origins of cometary material. A comparison with 1P/Halley--a third comet from the giant planet nebular region--will be discussed in the context of heterogeneity among these bodies.

Mumma, Michael J.↗
NASA NTRS2004

The Abundance and Isotopic Composition of Hg in Extraterrestrial Materials

During the past three year grant period we made excellent progress in our study of the abundances and isotopic compositions of Hg and other volatile trace elements in extraterrestrial materials. As part of my startup package I received funds to construct a state-of-the-art experimental facility to study gas-solid reaction kinetics. Much of our effort was spent developing the methodology to measure the abundance and isotopic composition of Hg at ultratrace levels in solid materials. In our first study, the abundance and isotopic composition of Hg was determined in bulk samples of the Murchison (CM) and Allende (CV) carbonaceous chondrites. We have continued our study of mercury in primitive meteorites and expanded the suite of meteorites to include other members of the CM and CV chondrite group as well as CI and CO chondrites. Samples of the CI chondrite Orgueil, the CM chondrites Murray, Nogoya, and Cold Bokkeveld, the CO chondrites Kainsaz, Omans, and Isna, and the CV chondrites Vigarano, Mokoia, and Grosnaja were tested. We have developed a thermal analysis ICP-MS technique and applied it to the study of a suite of thermally labile elements (Zn, As, Se, Cd, In, Sn, Sb, Te, Hg, Au, Tl, Pb, and Bi) in geologic materials as well.

Lauretta, D. S.↗