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47 records · Page 3

Report on Inventory of Samples from Six Capsules from BOR-60

As part of the University of Michigan Grand Challenge Integrated Research Project, Oak Ridge National Laboratory (ORNL) received a drum containing six capsules from Pacific Northwest National Laboratory in August 2025. Each capsule originated at the University of Michigan and contained approximately 44 disks of various iron-based alloys (T91, HT9, T92, 800H, and others). These capsules were irradiated at several temperatures in the BOR-60 fast reactor for multiple cycles to accumulate high levels of damage. The drum was sent to the Irradiated Materials Examination and Testing (IMET) hot cell facility, a Class III nuclear facility, located in Building 3025E at ORNL. The IMET hot cell facility at ORNL is designed to receive irradiation capsules from the High Flux Isotope Reactor and perform capsule opening, basic optical examination, and mechanical testing on neutron-irradiated materials. Capsules were unloaded from the drum and placed in cell 6 for disassembly in February 2026. A low-speed saw opened each capsule, and a manipulator moved the disks to a dual microscope setup for disk identification, as shown in Figure 1.

36 MATERIALS SCIENCE↗

Degradation and Failure Phenomena of Advanced Reactor Fuel Concepts: Sodium-Cooled Fast Reactor Metallic Fuel

The U.S. Nuclear Regulatory Commission (NRC) is anticipating licensing applications and commercial use of new fuel types in advanced nuclear power reactors that would be designed and built in the United States. Pacific Northwest National Laboratory (PNNL) is providing technical assistance to the NRC related to the newly proposed nuclear fuel and cladding designs that would be deployed in these reactors. This report focuses specifically on the metallic fuel that is being considered for sodium-cooled fast reactors and specifically on mechanisms that would cause damage or failure to the fuel under reactor operating conditions and design basis accident conditions. There is historic experience with both metallic and oxide fuels in experimental sodium-cooled fast reactors, but this report will focus solely on metallic fuel. Currently two U.S.-based reactor designers are engaged with the NRC in the application or pre-application review and considering a sodium-cooled fast reactor. TerraPower is engaged with NRC in pre-application review of its Natrium reactor. The current design for this fuel uses a sodium-bonded uranium-10wt% zirconium (U10Zr) fuel clad in HT9 stainless steel. ARC Clean Technology is engaged with NRC in pre-application review of its ARC-100 reactor. The current design for this fuel uses a sodium-bonded uranium-10wt% zirconium (U10Zr) fuel with steel cladding. This report will focus on this fuel system specifically, with broader information given regarding other metallic fuel systems with other stainless steel alloy claddings. To support the NRC’s readiness efforts, this report will identify and discuss degradation and failure modes of metallic fuel concepts for sodium-cooled fast reactors, including fuel performance characteristics that may not be addressed within existing regulatory documents.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Mechanical Property Measurements of HFIR-irradiated FM and ODS Alloys

This report provides a summary of the post-irradiation examination of the tensile properties of three ODS ferritic alloys, 14YWT-SM13, 9YWTV-PM2 and OFRAC, and two HT9 ferritic/martensitic steels, one with low N content and the other with high N content. The neutron irradiations were conducted in the flux trap of the High Flux Isotope Reactor as part of the Additive Manufacturing, Oxide Dispersion Strengthened Alloys and Wrought Steels (AMOW) irradiation campaign. Sub-sized tensile specimens fabricated from each material were exposed to nominal target temperatures and neutron doses of 300°C, 385°C, and 525°C and 8 dpa, 16 dpa, and 50 dpa, respectively.

36 MATERIALS SCIENCE↗

Material Characterization Report of EBR II Mark IV Fuel Element

The focus of this report is the characterization of an unirradiated as-built fuel element from the Experimental Breeder Reactor II (EBR-II) Mark IV driver fuel design. The fuel in this element is a metallic uranium-zirconium alloy, and the cladding material is HT9 stainless steel. Both the metallic fuel and cladding materials are characterized, including chemical composition, grain size, morphology, phase composition, precipitate composition, crystallography, density, and hardness.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Non-Destructive Postirradiation Examination of the AFC-4C Capsule/Rodlet 5 Experiment

The AFC-4C irradiation test was irradiated at the Idaho National Laboratory Advanced Test Reactor to investigate several different fast reactor fuels that could be used to facilitate ultra-high burnup applications in sodium fast reactors. Several different alloys, fuel geometries, bonding materials, and coating/barrier were tested in ferritic-martensitic HT-9 cladding. The AFC-4C capsule 5 was removed from the reactor at around 8.7 at %HM burnup to begin postirradiation examination. This report presents and discusses the non-destructive PIE results of the AFC-4C-capsule / rodlet 5, a U-10Zr solid fuel, sodium bonded with HT9 with internal Cr-coating, and its performance is evaluated against the historical fuel performance of previously irradiated fuel from literature.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Comparison of FAST Experiments to BISON Simulations

The Fission Accelerated Steady-State Test (FAST) experiments utilize the effects of scaling to accelerate the burnup experienced by the fuel. This experimental technique offers a unique opportunity to evaluate the effects of scaling on fuel and cladding material modelling. Currently, models used in the BISON fuel performance code for metallic fuel performance are calibrated for EBR-II conditions and geometries. Comparing BISON simulations to FAST experimental data will allow for the identification of shortcomings in the models for conditions outside the EBR-II paradigm. FAST experiments have been performed on U-Zr and U-10Mo fuel types with HT9 cladding. Initial comparisons of simulated cladding strains to experimental results show that the BISON simulations consistently overpredict cladding strain in the fuel region but underpredict the cladding strain in the plenum region. This indicates potential issues with the simulation of swelling and gas pressure at smaller geometries. Further comparison with fission gas release measurements is planned as data becomes available.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

A comparison of surrogate constitutive models for viscoplastic creep simulation of HT-9 steel

Mechanistic microstructure-informed constitutive models for the mechanical response of polycrystals are a cornerstone of computational materials science. However, as these models become increasingly more complex – often involving coupled differential equations describing the effect of specific deformation modes – their associated computational costs can become prohibitive, particularly in optimization or uncertainty quantification tasks that require numerous model evaluations. To address this challenge, surrogate constitutive models that balance accuracy and computational efficiency are highly desirable. Data-driven surrogate models, that learn the constitutive relation directly from data, have emerged as a promising solution. In this work, we develop two local surrogate models for the viscoplastic response of a steel: a piecewise response surface method and a mixture of experts model. These surrogates are designed to adapt to complex material behavior, which may vary with material parameters or operating conditions. The surrogate constitutive models are applied to creep simulations of HT-9 steel, an alloy of considerable interest to the nuclear energy sector due to its high tolerance to radiation damage, using training data generated from viscoplastic self-consistent (VPSC) simulations. In conclusion, we define a set of test metrics to numerically assess the accuracy of our surrogate models for predicting viscoplastic material behavior, and show that the mixture of experts model outperforms the piecewise response surface method in terms of accuracy.

36 MATERIALS SCIENCE↗

An integrated approach to examine fuel-cladding chemical interaction in HT9/U-10Zr metallic fast reactor fuels: Coupling machine learning with electron microscopy and local mechanical properties analysis

The metallic U-Zr nuclear fuel alloy has garnered renewed interest as a promising candidate for next-generation sodium-cooled fast reactors. Recent studies and technology assessments have identified several areas requiring improvements, enhanced knowledge, and reliable data to strengthen the U-Zr fuel design basis for qualification and commercial applications. One of the most challenging phenomena impacting this fuel system’s performance is fuel-cladding chemical interaction (FCCI). This work aimed to harvest FCCI data by examining selected HT9/U-10Zr (wt. %) fuel samples of prototypic full-length fuel pins through an integrated approach. This approach integrated scanning electron microscopy (SEM) microstructure characterization with localized mechanical properties examination to deepen understanding of FCCI phenomenon in HT9/U-10Zr fuel system. Particularly, this study focused on MFF fuel pins irradiated at Fast Flux Test Facility (FFTF), which aimed to qualify metallic fuel as a driver fuel for FFTF and to assess its viability for larger-scale fast reactors. Electron microscopy provided high confidence in detecting and distinguishing the different FCCI layers, while small-scale mechanical testing (SSMT) probed the mechanical properties of these layers. SEM examination of a MFF-2 pin 192167, with a time averaged inner cladding temperature (TICT) slightly over 500°C, revealed minimal cladding-side FCCI (cladding wastage). In contrast, significantly thicker cladding wastage comprising two distinct sublayers was observed in samples from the thermally hot MFF-3 pin 193045 and MFF-5 pin 195011 where the TICT ranged from 610-635°C. SSMT indicated complete embrittlement in the sublayer adjacent to the fuel and a tendency toward embrittlement in the other sublayer. Additionally, a new machine learning method was developed, validated, and used to quantify cladding wastage thickness. The machine learning method reliably predicted the wastage thickness across various fuel pins and sample cross-sections. Furthermore, the available cladding wastage data from HT9/U-10Zr fuel system demonstrated a strong temperature dependency. However, the dataset remains small, and ongoing research activities are essential to further understand the FCCI phenomenon and develop a reliable FCCI model for enhanced fuel performance simulation under various conditions.

36 - MATERIALS SCIENCE↗

VTR Fuel Design

VTR fuel design presentation for the May 25, 2021 VTR quarterly integration meeting

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Effective Lanthanide Diffusivity through U-Zr Metallic Fuel

Fuel-cladding chemical interaction (FCCI) is one of the main concerns for the performance of U-Zr metallic fuels. Although FCCI results in complex phase transformations and morphological changes in both the fuel and cladding sides of the interface, the formation of a brittle layer in the cladding side of the interface (sometimes referred to as wastage) has one of the most significant impacts on the cladding mechanical integrity. This brittle layer is associated with the formation of intermetallic compounds between the cladding constituents Fe, Cr and the lanthanide fission product species. The formation of this cladding wastage layer has been the focus of recent efforts to develop a mechanistic modeling framework, including production of lanthanides in the fuel, transport through the fuel to the fuel-cladding interface, and phase transformation to form intermetallic phases. To calculate the rate of transport of lanthanides through the fuel, a multi-scale computational approach has been used. Atomistic calculations have been performed to determine the diffusivities of Nd, the most prevalent lanthanide species, through the solid fuel matrix and along pore surfaces. These diffusivities have been used as input parameters for a mesoscale model to determine an effective diffusion coefficient that accounts for the formation of porosity, its interconnection, and infiltration with bond sodium from the fuel-cladding gap. The effective diffusivity has been used in engineering-scale simulations using the BISON fuel performance code, and BISON simulations have been compared to representative validation cases from the EBR-II reactor.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗