Development of Shielding Benchmarks Using the Godiva IV Assembly
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IER 555: Godiva Benchmark Update CED-2 (Final Design Report)
The International Criticality Safety Benchmark Evaluation Project (ICSBEP) evaluation of the Godiva IV critical assembly, HEU-MET-FAST-086: GODIVA-IV DELAYED-CRITICAL EXPERIMENTS (HMF-086), was completed by Russ Mosteller. Five critical experiment configurations performed at the Los Alamos National Laboratory (LANL) Technical Area (TA)-18 were evaluated as acceptable benchmark cases. The five cases consist of four delayed critical configurations which differ in control rod positions and one prompt critical configuration. All cases calculated a lower $k_{eff}$ than measured by experiment. This data is referred to as the TA-18 Godiva IV benchmark in this report. In 2005, Godiva IV was disassembled for relocation to the Nevada Test Site (NTS), now Nevada National Security Site (NNSS), at the National Criticality Experiments Research Center (NCERC). Following the disassembly and subsequent reassembly and startup of Godiva IV at NCERC, additional information about the Godiva IV components was obtained. An errata note was added to the HMF-086 evaluation in the ICSBEP handbook to provide this new information until a revision to the benchmark evaluation could be performed. In addition to those corrections, there are differences between the Godiva IV assembly at TA-18 and the Godiva IV assembly at NCERC. These differences include both assembly-specific differences (differences in the safety block gap, differences in the control rod positions, a new NCERC Top Hat and contamination shield) as well as environmental differences, such as the size and shape of the experimental building where the assembly is located. An additional model with similar cases, referred to as the NCERC Godiva IV benchmark in this report, will be added to the revised HMF-086 to capture these additional differences. This will provide the best benchmark model of Godiva for use by those performing experiments at NCERC. The IER 555 CED-2 report documents the information that will be updated in the HMF-086 revision, both the corrections to the TA-18 Godiva IV benchmark and the subsequent changes to create a NCERC Godiva IV benchmark. It describes the measurements that will be performed for cases similar to those performed at TA-18. It also describes measurements that will be included in the evaluation as additional data.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
National Criticality Experiments Research Center (NCERC) - capabilities and recent measurements
The National Criticality Experiments Research Center (NCERC) located at the Device Assembly Facility (DAF) at the Nevada National Security Site (NNSS) and operated by Los Alamos National Laboratory (LANL) is home to four critical assemblies which are used to support of range of missions, including nuclear criticality safety and nuclear nonproliferation. Additionally, subcritical systems can also be assembled at NCERC. NCERC is providing critical and subcritical experiments valuable to the nuclear data community and experiments performed at NCERC are often published as benchmarks in the International Criticality Safety Benchmark Evaluation Project (ICSBEP) Handbook. This manuscript will give a broad overview of recent experiments performed at NCERC, upcoming experiments, and why integral measurements are important and useful to the nuclear data community. The four critical assemblies are GODIVA IV, FLATTOP, COMET, and PLANET. GODIVA IV is a cylindrical metal fast burst reactor, the fourth in the GODIVA series that dates back to the 1950’s. FLATTOP is an highly enriched uranium (HEU) or Pu core reflected by natural uranium. COMET and PLANET are vertical lift assemblies, where one half of the reactor can be lifted to the upper half of the reactor to create a critical system. Some recent experiments include various critical intermediate energy assemblies with lead, and subcritical measurements of plutonium reflected by copper, tungsten, and nickel. Work is also underway to make a better measurement of the critical mass of neptunium, using a neptunium sphere surrounded by nickel shells. Additionally, measurements will be performed next year with HEU shells from Rocky Flats. These HEU shells will be stacked together to make larger systems, allowing for a large range of criticality (from subcritical to delayed critical). Other upcoming measurements include an HEU critical assembly sensitive to intermediate energy neutrons.
98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗
Criticality Accident Alarm System Shielding Benchmark: Integral Experiment Request 498, Critical Engineering Decision 1 Report
This report supports Critical/Subcritical Experiment Decision 1 (CED-1) for Integral Experiment Request (IER) 498, a shielding benchmark produced using the Godiva IV critical assembly at the National Critical Experiments Research Center (NCERC). Shielding benchmarks are datasets collected to provide a comparison for computer models that simulate the effect of shielding on radiation transmission from a source to a detector. The purpose of a CED-1 report is to produce a conceptual design for an integral experiment and to identify the long lead-time items. The design presented in this report favors certain detailed design options such as material selections. However, alternative options can be selected as the project evolves. Dimensions are specified only as needed to evaluate feasibility and performance. Development of Criticality Accident Alarm System (CAAS) shielding benchmarks supports two main programmatic needs. The first need is to improve confidence in models of facilities that house nuclear material handling operations. Better models can support effective CAAS detector placement when criticality may result in dose, and it enables more accurate analysis of criticality accident impacts at various locations in a facility. A key quantity that can be verified is the secondary gamma production caused by neutron interactions with various materials. The second programmatic need supported by shielding benchmarks is the ongoing development of methods being integrated into nuclear simulation codes such as the Monte Carlo N-Particle (MCNP) transport code and the SCALE code system used in efforts funded by the Nuclear Criticality Safety Program (NCSP). Previous work performed under the International Criticality Safety Benchmark Experimental Program (ICSBEP) to produce shielding benchmark data is primarily limited to a set of measurements at the SILENE critical assembly at the Valduc facility in France. The experiment used an open configuration and a burst mode operation, which limited detector options to thermoluminescent dosimeters (TLDs) and activation foils. Because TLDs do not record gamma spectra, it was difficult to verify the gamma energy spectrum from the experiment. In this work, the Godiva IV assembly will be used because it is a fast system capable of producing a wide range of source strengths, including super-prompt critical bursts. The room return for the facility is expected to be substantial and challenging to characterize, so a more closed, shielded experimental configuration is considered. Furthermore, because the physics of radiation transport outside the assembly does not change between the burst mode and the delayed critical mode, it is anticipated that most measurements will be made with the Godiva IV assembly in delayed critical mode, operating within a range that will allow electronic counters to collect accurate data. Scoping calculations concluded that a workable room return shield is comprised of 40 cm of 5% borated polyethylene backed by 7 cm of lead. This configuration was shown to produce a ratio of signal–to–room return of over 100 for up to 2 mean free paths of shield sample material, and over 10 for up to 4 mean free paths of shield sample material, ensuring that useful results can be obtained. With no shielding sample in the room return shield, it was shown that the neutron and gamma spectra do not appreciably change with a change in room size. This scoping calculation does not preclude the use of tungsten powder in a binder, some other effective gamma shielding material, or a hybrid design. Dose rates for various source intensities at an unshielded detector are listed herein to inform detector selection during CED-2, and calibration chains are identified. Preliminary estimates of costs and schedules are outlined but remain to be verified. Values could double or triple as estimates become more accurate and are principally included here to demonstrate feasibility. Preliminary estimates indicate that the apparatus can be installed within a feasible schedule and budget. Two measurements per day are assumed. Producing a shielding benchmark at NCERC using the Godiva IV assembly has been shown to be feasible, with manageable uncertainties and risks. A clear, continuing need for shielding benchmark data remains present, and this report identifies and evaluates a method for creating integrated shielding benchmark datasets.
46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
PNNL Measurement Results for the 2018 FlatTop Criticality Nuclear Accident Dosimetry Exercise at the Nevada National Security Site (IER-253)
The Pacific Northwest National Laboratory (PNNL) participated in the FlatTop exercise IER-253 at the National Nuclear Security Site (NNSS) during the week of May 21, 2018. This report summarizes the measurements of the personal nuclear accident dosimeters (PNAD). Additionally, portable survey instrument readings and measurements of the simulated biological samples are included. The FlatTop exercise (IER-253) tested only PNADs and did not include fixed nuclear accident dosimeters (FNAD). Previous PNAD results obtained in 2016 at the Godiva-IV exercise IER-148 were summarized in PNNL Measurement Results for the 2016 Criticality Accident Dosimetry Exercise at the Nevada National Security Site IER-148 (PNNL-26497). The results clearly indicated that the previous dose conversions were a historical legacy of the Hanford Site and corresponded closer to kerma dose (or first collision dose, and not to Hp(10) dose). The technical basis for PNAD dose was based on the Godiva-IV exercise and documented in A New Dose Calculation Methodology for New PNAD and FNAD Designs at PNNL (PNNL-27023). The configuration of the PNAD was described in these two documents. The FlatTop exercise was the first time PNNL tested this new dose calculation methodology. Results were generally favorable with some results conservatively over reported that fell above the performance criteria. The reported gamma dose results fell non-conservatively low because only the default parameters obtained from the Godiva-IV exercise were used, and because the OSL gamma dosimeter has an energy dependency. The results from the simulated biological samples were also favorable, and in several cases conservatively over reported.
61 RADIATION PROTECTION AND DOSIMETRY↗
IER 268 CED-3b Report
The goal of IER 268 was to collect information from the operation of the Godiva IV super-prompt critical assembly to support multi-physics modeling efforts. There were two types of systems deployed. One was a Photo-Doppler Velocimetry (PDV) system which used the reflection of laser light on the surface of the Godiva IV core. The other consisted of an MHD 240 detector with two other detectors (an MHD-241 and an Eljen EJ-325A) used for reference as the MHD-240 detector was moved. The collection is referred to as the MHD Detector in the narrative log. There were two types of Godiva operations performed to gather data. A series of super-prompt critical bursts were performed and data collected on both systems, tied to a common trigger. Separately, a series of delayed critical operations at various power levels was performed for a combination of MHD detector distances from Godiva and the presence and absence of a shield in the line of sight between Godiva and the MHD detector. This data was collected to determine the contribution of room return during the burst measurements.
46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
UPF and Y-12 Criticality Accident Alarm System (CAAS) Radiation Testing Report
This report documents the experimental conditions and results for the testing of the Mirion Technologies CAAS-3S Criticality Accident Alarm System (CAAS) for the Y-12 National Security Complex (Y-12) and Uranium Processing Facility (UPF). The testing was conducted at the Godiva IV Burst Reactor at the National Criticality Experiments Research Center (NCERC) at the Nevada National Security Site (NNSS) during the week of January 11, 2021. The testing was conducted in accordance with 25774-QL-POA-JR00-00002-VDE-27.0, CAAS-3S Radiation Testing of Cabinet Components Test Plan. The tests subjected the CAAS-3S system to intense and short duration mixed neutron and gamma radiation fields and to high integrated radiation doses. The purpose of the test was to environmentally qualify various CAAS-3S components in a radiation environment. Successful completion of the tests was predicated on the collaborative efforts of several organizations. Sandia National Laboratory (SNL) and Lawrence Livermore National Laboratory (LLNL) provided dosimetry to estimate photon and neutron dose. Los Alamos National Laboratory (LANL) manages the NCERC facility, operated the Godiva IV reactor, and provided field support for CAAS-3S placement and communications interface for data acquisition systems supplied by Mirion Technologies. Throughout the test campaign, Y-12 and UPF personnel provided technical support in determining changes to the test schedule, as needed, interpretation of the results, and comparison between the measured dosimetry data and predicted results. Throughout the test campaign, Mirion personnel provided technical support in the operation of the CAAS-3S system itself.
21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗
IER 557: Godiva Pulse Repeatability and Characterization (CED-3A Report)
Godiva IV is a fast burst critical assembly constructed of approximately 65 kg of highly enriched uranium (HEU) fuel alloyed with 1.5% molybdenum for strength. Godiva IV is proposed as the radiation source for IER 498: Design a Shielding Benchmark with a Metal Critical Source. IER 498 proposes a two-burst method to determine the performance of shielding samples, comparing the transmission of the source radiation to detectors with and without a shielding sample present. This eliminates the need for an absolute calibration and allows many uncertainties to cancel. However, the source term variability must be low compared to other sources of experimental uncertainty to ensure the overall uncertainty meets acceptable levels to provide useful measurements. The primary goal of this experiment is to quantify the source term variability, or reproducibility, of Godiva bursts, focusing on the 70 °C bursts planned for IER 498 measurements. Discussions during IER 498 noted that a number of bursts (on the order of six to ten) as identical as possible would be performed and that a 5-7% standard deviation in source intensity would be acceptable.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
Godiva Experiments for the Nuclear Criticality Safety Program (NCSP)
Godiva IV is a fast burst critical assembly constructed of approximately 65 kg of highly enriched uranium (HEU) fuel alloyed with 1.5 percent molybdenum for strength. Godiva is one of the last such critical assemblies in the United States, and can be used for studies of super-prompt critical behavior as well as irradiations and demonstrations. A demonstration of a Godiva burst is usually performed as a highlight of the hands-on portion of the Criticality Safety Training Classes taught at the National Criticality Experiment Research Center (NCERC). The Godiva burst is used to demonstrate the concept of super-prompt critical and the time-scale of a criticality accident. In addition, several NCSP projects have been conducted on Godiva IV over the past two years. One experiment focused on collecting data to support multiphysics simulations using Photo-Doppler Velocimetry (PDV) to measure surface movement and gamma detectors to measure the burst output as the burst develops from background to peak over ten orders of magnitude. Another experiment was performed to demonstrate the functionality of the Criticality Accident Alarm System (CAAS) system developed for installation in the Y-12 Uranium Processing Facility (UPF). The system must not only respond to a criticality event and alarm, but must also be shown to operate in a high dose environment.
46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
Au-198 and TLD-600 results from IER-593 Godiva irradiations
This report summarizes the results from dosimetry packets deployed during a nominally 250 ◦C temperature rise Godiva IV burst. Dosimetry packets including Bare Au foils, Cd covered Au foils, and Thermoluminescent Dosimeters (TLDs) were deployed at five positions around Godiva at a height corresponding to the center height of the HEU fuel.
61 RADIATION PROTECTION AND DOSIMETRY↗
NCERC 2024 Highlights
The National Nuclear Security Administration (NNSA) is entrusted with ensuring the safety, security, and reliability of the nation’s nuclear weapons stockpile while advancing programs aimed at reducing global nuclear proliferation. These critical mission objectives are achieved through the expertise of a highly skilled team of professionals. The operations at the National Criticality Experiments Research Center (NCERC) play a vital role in developing and enhancing knowledge and expertise in advanced nuclear technologies. NCERC supports a wide range of mission areas, including nuclear criticality safety, nuclear emergency response, and nuclear nonproliferation, safeguards, and arms control. It also provides support to the Department of Homeland Security, advances stockpile stewardship science, and delivers scientific expertise to other government agencies, such as NASA and the Defense Threat Reduction Agency. NCERC conducts experiments utilizing diverse nuclear materials, from small neutron-emitting sources for testing radiation detection equipment to larger quantities of uranium and plutonium for criticality experiments. A cornerstone of NCERC's mission portfolio includes the operation of four critical mass assembly machines—Planet, Comet, Flattop, and Godiva-IV—which are instrumental in advancing nuclear science and ensuring the nation’s nuclear security objectives.
11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
Hands-On Experimental Training [Slides]
Training provided includes: Nuclear Criticality Safety Fundamentals, Sub-Critical "Hands On" Demonstration, Hand-Stacking and Remote Approach to Critical Using the Planet Assembly, Flattop Free-Run Demonstration, and Godiva-IV Critical Assembly Demonstration.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
Improved Cumulative Fission Yield Measurements with Fission Spectrum Neutrons on 238U
Two isotopically-characterized targets of high-purity (99.961±0.002%) 238U metal and a neutron dosimetry package were exposed to a pulsed neutron irradiation using the Godiva IV critical assembly at the National Criticality Experiments Research Center to measure the integral fission product yields produced in a Watt fission neutron-energy spectrum. Following irradiation, the fissioned targets were counted with two broad energy germanium detectors. Estimates of the total fissions for each target were made using measurements of well-known fission products. The total number of fissions in each target were then used to measure the fission yields of 33 fission products, 18 of which are published as new measurements. Twelve of the 18 isotopes were in agreement with ENDF/B- VIII.0 using the zeta test and treating ENDF/B-VIII.0 as the true mean: 84mBr, 93Y, 94Y, 104Tc, 134I, 135I, 138Xe, 141Ba, 142Ba, 142La, 146Ce, and 149Nd. The ENDF/B-VIII.0 fission yield for 139Ba was only slightly outside of 1-s relative to the uncertainty measured in this work. Uncertainties for 5 fission product yields were markedly improved over those reported in ENDF/B-VIII.0: 128Sn, 129Sb, 130gSb, 131mTe, and 133I. The fission yields measured for 128Sn, 131mTe, and 133I were in good agreement with the ENDF/B-VIII.0 predicted fission yields. However, fission yields measurements of the isotopes 129Sb, and 130gSb deviated from the ENDF/B-VIII.0 value. Both of these isotopes reside near the doubly magic nuclear shell closures of 50 protons and 82 neutrons. These fission yields may be suppressed because of the odd-odd nuclear structure of 130gSb and the odd-even structure of 129Sb and isomer splitting. Comparisons to other recent work and a brief review with citations are included to support this conclusion.
Fission Yields↗
A Review of Nuclear Reactor Transients
This paper explores the nuclear yield that is produced during nuclear transients in small reactors. Nuclear reactor transients can have a wide range of effects such as the reproducible power excursions as found in Godiva-IV to full reactor destruction as planned for in the Kiwi-TNT test. Criticality accidents are also included in this study as in essence a small nuclear reactor has been inadvertently created. The motivation for this paper is to educate the audience as to the likely fission energy release for a typical transient in a small nuclear reactor.
22 GENERAL STUDIES OF NUCLEAR REACTORS↗
NCERC Capabilities [Slides]
NCERC is our nation’s only generalpurpose critical experiments facility and is one of only a few that remain operational throughout the world. The mission of the National Criticality Experiments Research Center (NCERC) is to conduct experiments and training with critical assemblies and fissionable material at or near criticality in order to explore reactivity phenomena, and to operate the assemblies in the regions from subcritical through delayed critical. One critical assembly, Godiva-IV, is designed to operate above prompt critical.
61 RADIATION PROTECTION AND DOSIMETRY↗
Simulations of Gadolinium Oxide Gamma Converter System for the Godiva Critical Assembly [Slides]
Godiva IV is a fast burst critical assembly constructed of approximately 65 kg of highly enriched uranium (HEU) fuel alloyed with 1.5 percent molybdenum for strength. Can be used for studies of super-prompt-critical behavior as well as irradiations and demonstrations.
11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
Gamma Converter Box Preliminary Design [Slides]
Objective: Develop a test capability near Godiva IV fast burst reactor to maximize gamma dose to neutron dose ratio and gain increase in gamma dose over free field. Goal: Maximize gamma dose to neutron dose ratio and gain increase in gamma dose over free field.
22 GENERAL STUDIES OF NUCLEAR REACTORS↗
193 mIr/ 192 Ir ratio from irradiation with various NCERC critical assemblies
Eight irradiations of K 2 IrCl 6 pellets were carried out with three critical assemblies: Flattop-Oy, Flattop-Pu and Godiva IV. One of the irradiations was performed with three pellets at different locations of the critical assembly, while the other irradiations with pellets at the center, but operating the critical assembly at different power and, respectively, different neutron flux. Counting samples were prepared from the irradiated pellets and X-ray spectra measured with silicone drift detectors. The 193 mIr/ 192 Ir ratio is reported for each irradiation.
38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗