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At least 55 records · Page 3

Neutronics Analysis for ITER Diagnostic Generic Upper Port Plug

This paper presents new results of neutronics analysis performed for the updated design of the ITER Diagnostic Generic Upper Port Plug (DGUPP). Such analysis is performed regularly during the development of the ITER Ports design. Neutronics analysis is an important step in support of the development of ITER components irradiated by 14 MeV neutrons generated in D-T fusion thermonuclear reactions. The neutrons are born in the ITER tokamak plasma chamber and then impinge on the surrounding blanket and port plugs, after that they diffuse through shielding material of vacuum vessel components or could stream through the diagnostic channels and assembly gaps far away from plasma up to the bio-shield and in a small amount beyond it. While ITER machine is in operation it is inaccessible, after the shut-down it is planned to provide personnel access to the Upper Port Inter-Space Structure (UP ISS) behind the Port Plug via the corridors. Neutrons activate the ITER materials and those radioactive materials emit decay gammas during the shut-down causing a Shut-Down Dose Rate (SDDR) field distributed all around the activated materials. Decay gammas could also stream through the void channels. That emphasizes the need for calculation of decay gamma transport in evaluations of SDDR, which is reflected in the use of transport - activation interface code described in Section of Computational Modelling. The assessment of radiation environment (fluxes and SDDR) at DGUPP was focused on the port back-side area of UP ISS, where personnel access is planned along the ISS maintenance corridors. Minimization of SDDR at the front part of the ISS maintenance corridors was the target value for optimization of the DGUPP shielding and analysis of related neutronics effects. Following the dose ALARA (As Low As Reasonably Achievable) principle, every possibility to reduce SDDR should be investigated, emphasizing the importance of this analysis. The challenges of such analysis are inextricably connected with the engineering complexity of the ITER machine, with integration of many diagnostics systems having channels and gaps inside the ITER ports. Those gaps result in radiation streaming and negatively affect the shielding performance of the port plugs. The computational complication is caused by the need to model precisely the ITER geometry and then to run deep penetrating radiation transport in the substantially heterogenic toroidal geometry of ITER large-size tokamak, with 30 m height and diameter of its bio-shield. The whole mass of Upper Port Plug (UPP) could be up to 25 tons and it must be very precisely positioned inside the port opening in blanket and Vacuum Vessel. Facing the engineering challenges for the assembly of DGUPP, there were proposed two Project Change Requests (PCRs) No. 439 and 709 concerning the design updates of UPP/blanket interface and its remote handling.

61 RADIATION PROTECTION AND DOSIMETRY↗

Titanium Material Comparison for Second Target Station Moderators

Two titanium alloys, Ti 15-3-3-3 and Grade 5 Ti, have been analyzed for their neutronic differences after being exposed to neutron fluxes from a 5-year operational period in the Second Target Station (STS)moderators. There are several differences in the original composition of the two alloys where Ti 15-3-3-3contains Cr and Sn and Grade 5 Ti does not. The differences in original composition propagate through the analysis to yield discrepancies in decay power density and decay gamma intensity density of more than a factor of 3.5 at some times during operation. Immediately after the 5-year operational period, Ti 15-3-3-3has a factor of 3.59 higher intensity of high-energy decay gammas than Grade 5 Ti, and Ti 15-3-3-3 also has a factor of 3.53 higher decay power than Grade 5 Ti. After 1 year of shutdown, Ti 15-3-3-3 has a 48% higher intensity of high-energy decay gammas and a 86% greater decay power density when compared with Grade 5 Ti. The quantities-of-interest in this report are per unit volume and the overall volume of titanium should be considered when making engineering judgment on final titanium alloy selection.

36 MATERIALS SCIENCE↗

Possible Detection of Pi(exp 0)-Decay Gamma-Ray Emission from Cyg OB2 by EGRET

We report possible detection of pi (exp 0) decay radiation from Cyg OB2, a nearby (1.7 kpc) massive OB star association. The EGRET flux (greater than 100 MeV) maps clearly indicate a point source whose error circle includes both Cyg OB2 and Cyg X-3. We show that Cyg X-3 is unlikely to be the counterpart for the EGRET source, because of the marginal spatial consistency and the lack of the 4.8 hour modulation seen in other high energy emissions from Cyg X-3. If confirmed, this will be the first detection by EGRET of massive stars.

Chen, W.↗

Structure for Storing Properties of Particles (PoP)

Evaluated nuclear databases are critical for applications such as nuclear energy, nuclear medicine, homeland security, and stockpile stewardship. Particle masses, nuclear excitation levels, and other “Properties of Particles” are essential for making evaluated nuclear databases. Currently, these properties are obtained from various databases that are stored in outdated formats. A “Properties of Particles” (PoP) structure is being designed that will allow storing all information for one or more particles in a single place, so that each evaluation, simulation, model calculation, etc. can link to the same data. Information provided in PoP will include properties of nuclei, gammas and electrons (along with other particles such as pions, as evaluations extend to higher energies). Presently, PoP includes masses from the Atomic Mass Evaluation version 2003 (AME2003), and level schemes and gamma decays from the Reference Input Parameter Library (RIPL-3). The data are stored in a hierarchical structure. An example of how PoP stores nuclear masses and energy levels will be presented here.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Photon strength and the low-energy enhancement

Several measurements in medium mass nuclei have reported a low-energy enhancement in the photon strength function. Although, much effort has been invested in unraveling the mysteries of this effect, its physical origin is still not conclusively understood. Here, a completely model-independent experimental approach to investigate the existence of this enhancement is presented. The experiment was designed to study statistical feeding from the quasi-continuum (below the neutron separation energy) to individual low-lying discrete levels in {sup 95}Mo produced in the (d, p) reaction. A key aspect to successfully study gamma decay from the region of high-level density is the detection and extraction of correlated particle-gamma-gamma events which was accomplished using an array of Clover HPGe detectors and large area annular silicon detectors. The entrance channel excitation energy into the residual nucleus produced in the reaction was inferred from the detected proton energies in the silicon detectors. Gating on gamma-transitions originating from low-lying discrete levels specifies the state fed by statistical gamma-rays. Any particle-gamma-gamma event in combination with specific energy sum requirements ensures a clean and unambiguous determination of the initial and final state of the observed gamma rays. With these requirements the statistical feeding to individual discrete levels is extracted on an event-by-event basis. The results are presented and compared to {sup 95}Mo photon strength function data measured at the University of Oslo.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Development of the Advanced D1S for Shutdown Dose Rate Calculations in Fusion Reactors

The assessment of the shutdown dose rate due to neutron activation is fundamental for shielding design, materials selection, licensing and planning of maintenance operations in high performances fusion devices. The shutdown dose rate calculations require the combined use of radiation transports and inventory codes. The typical approach consists in a two steps procedure. A pure neutron transport simulation is performed in a first step to calculate the spatial distribution of neutron spectra. The results are used as input for an activation calculation that provides the decay gamma source used in a second step for a pure gamma transport simulation (rigorous-two step, R2S). The Direct 1-Step (D1S) approach has been developed more than ten years ago by ENEA and the ITER team: this technique relies on a coupled neutron-decay gamma transport in a single simulation. It is based on the use of a modified version of the MCNP5 Monte Carlo code with specially tailored nuclear cross-section data for transport and FISPACT inventory code for temporal behaviour. The 'Advanced-D1S' is an improved version of D1S in which additional computational features have been introduced, such as the mesh tally capability and continuous time evolution assessment of the dose rate in single run dose. It has been validated through measurements at JET tokamak and comparison with R2S codes and a future benchmark experiment during next high performance deuterium-tritium campaign is in preparation at JET. It has also been extensively used for ITER calculations and recently applied to DEMO assessment. Present limitations and in progress code improvement strategy are described and discussed in this paper.

61 RADIATION PROTECTION AND DOSIMETRY↗

Study of extreme nuclear shapes in extreme conditions

Studies of extreme nuclear shapes have always fascinated scientists and are being pursued quite strongly over the years. Nuclei present themselves with interesting shapes and structures at different conditions of spin, excitation and also with the number of neutrons and/or protons in them. Gamma decays from the Giant dipole Resonances in nuclei can probe directly their shapes at different extreme conditions by looking at their resonant line-shapes, e.g., Jacobi shapes and shape-transitions, super/hyper-deformation etc. Similar such studies, done for the first time, using the LAMBDA high energy gamma spectrometer developed at VECC, is discussed here.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Analysis of Second Target Station Target Removal Dose Rates

The Second Target Station (STS) project at Oak Ridge National Laboratory’s spallation neutron source is a crucial initiative for maintaining U.S. leadership in neutron sciences. The STS aims to create the world’s brightest pulsed cold neutron source, enabling cutting-edge research across various scientific disciplines. To ensure safe and efficient maintenance operations, understanding the effects of shutdown dose rates from activated components within the STS target systems is essential. This study establishes a computational framework for calculating decay gamma sources and subsequent shutdown dose rates utilizing advanced methods to account for all activation channels, including high-energy interactions down to thermal neutron capture. This study describes a novel integration of multiple tools and provides an effective means of analyzing activation and shutdown dose rates at spallation neutron facilities. A custom-developed script automates the decay gamma source generation process, ensuring proper sampling during the variance reduction phase, which is critical for accurate predictions of shutdown dose rates.

Transmutation↗

The Shell-Model Code NuShellX@MSU

Use of the code NuShellX@MSU is outlined. It connects to the ENSDF data files for automatic comparisons to energy level data. Operator overlaps provide predictions for spectroscopic factors, two-nucleon transfer amplitudes, nuclear moments, gamma decay and beta decay.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Neutron and proton activation measurements from Skylab

Radioactivity induced by high-energy protons and secondary neutrons (from nuclear interactions) in various samples returned from different locations in Skylab was measured directly by gamma-ray spectroscopy measurements of decay gamma rays from the samples. Incident fluxes were derived from the activation measurements, using known nuclear cross-section. Neutron and proton flux values were found to range from 0.2 to 5 particles/sq cm-sec, depending on the energy range and location in Skylab. The thermal neutron flux was less than 0.07 neutrons/sq cm-sec. The results are useful for data analysis and planning of future high-energy astronomy experiments.

Fishman, G. J.↗

Decay Curve Correction Analysis Report

The decay curve analysis that is done on the short-lived radionuclide gas samples is used to differentiate between gaseous radionuclides that have the same characteristic gamma decay energy, 511 kiloelectron-volts (keV). A sample of stack gas is isolated and the total counts in the 511 keV peak are counted repeatedly in 10-second intervals to evaluate the decay rate of the sample over time. Analysis of this decay data required a series of steps. First, a raw data report is generated by the gamma acquisition system, based on an analysis template within the acquisition software. The data report file was then loaded into Microsoft Word, and a macro was used to perform minor formatting (remove colons and insert tabs between data columns) to allow analysis within Excel. The file is then saved as a text file at this point. The text file is then uploaded into Excel and a series of macros are used to add labels, calculate radioactive decay constants, and analyze the gamma decay data using linear regression techniques. The analysis template has been used since 1998 for stack 53000303 (TA-53, building 0003, exhaust stack 03) and 2000 for stack 53000702. The overall process, including the gamma report format and the macros used in Word and Excel for processing the report, had remained unchanged until 2015. In October of 2015, staff made a change to the report template in the gamma acquisition software which resulted in an error in the calculations later performed by the Excel macro. This error was not caught until a more in-depth review of the analysis took place regarding 2020 data. This report covers a much more complete review of the issue that occurred regarding the decay curve analysis, a review of the calculations completed to correct the issue, a review of the updated decay curve analysis process, and recommendations for moving forward.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Effects of He Ion Irradiation in Simple Borosilicate Glasses for HLW Immobilisation - 20324

High-level radioactive waste (HLW) consists of fission products and minor actinides. Borosilicate glass is the host material of choice in most countries to safely immobilize HLW, followed by eventual geological disposal. HLW glasses will experience both self-heating and self-irradiation effects due to the decay of fission products and minor actinides present therein. During the first 500 years of geological disposal, beta-gamma decay will be the main source of radiation due to short half-lives of fission products, as compared to very long-lived actinides which will be responsible for irradiation over much longer timescales. High-energy alpha particles and alpha recoil nuclei can potentially have significant impact (stored energy, volume change, accumulated dose, chemical durability) on the performance of the wasteform over longer timescales. Thus, to ensure safe and economic disposal over geological periods (10{sup 4} - 10{sup 6} years), the assessment of performance and properties in terms of radiation effects becomes indispensable. This work aims to simulate the effects of alpha decay in radioactive waste glasses. Two international glasses, namely UK 'MW' lithium-sodium borosilicate and Indian sodium-barium borosilicate, which are being used as HLW immobilization matrices by the UK and India respectively, were prepared by a melt-quench method and annealed below their glass transition temperatures. Both glasses were irradiated with 650 KeV He{sup 2+} ions with doses ranging from 10{sup 15} to 10{sup 17} ions/cm{sup 2}. Structural analysis was carried out using electron paramagnetic resonance (EPR) and Raman spectroscopies. First derivative continuous wave EPR spectra were recorded for all pristine and irradiated glass monoliths at room temperature using an X-band (frequency 9.6 GHz) EPR Bruker spectrometer. Results from EPR analyses showed the formation of irradiation induced paramagnetic centers at g ∼ 2.00 in all irradiated glasses. Raman spectra of pristine and irradiated samples were acquired, and showed notable changes in glass structure post-irradiation, with the emergence of a broad Raman band at 1560 cm{sup -1} upon irradiation with high fluences. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Reconstruction of neutrino induced NC-1π{sup 0} using the T2K-ND280 tracker

Single π{sup 0} production is the one of the most important backgrounds in the υ{sub e} appearance measurement in T2K. Large uncertainties in this production make it difficult to predict. Measurement at the near detector (ND280) is required both to constrain the background prediction at the far detector (Super-K) and also at the near detector to improve knowledge of beam υ{sub e} contamination. We present an analysis based on Monte Carlo simulation of neutral current (NC) single π{sup 0} in the tracker region. NC-1π{sup 0} events are selected using a specific two-gamma signature in the tracker region. One decay gamma is reconstructed by selecting an e+/e− pair starting in the Fine-Grained target Detector (FGD) and extending into the TPC, where the leptons can be identified and their momentum measured accurately. The second gamma is then selected in-time in the Calorimeter modules surrounding the tracker. Selections cuts, efficiency and purity of the selection are presented and projection of the expected number of single π{sup 0} candidates for 3 × 10{sup 20} protons on target (PoT) exposure is made.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗