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At least 55 records · Page 3

Beam Energy Dependence of the Linear and Mode-Coupled Flow Harmonics Using the a Multi-Phase Transport Model

In the framework of the A Multi-Phase Transport (AMPT) model, the multi-particle azimuthal cumulant method is used to calculate the linear and mode-coupled contributions to the quadrangular flow harmonic (v4) and the mode-coupled response coefficient as functions of centrality in Au+Au collisions at sNN = 200, 39, 27 and 19.6 GeV. This study indicates that the linear and mode-coupled contributions to v4 are sensitive to beam energy change. Nevertheless, the correlations between different-order flow symmetry planes and the mode-coupled response coefficients show weak beam energy dependence. In addition, the presented results suggest that the experimental measurements that span a broad range of beam energies can be an additional constraint for the theoretical model calculations.

79 ASTRONOMY AND ASTROPHYSICS↗

Collision-energy dependence of deuteron cumulants and proton-deuteron correlations in Au+Au collisions at RHIC

We report the first measurements of cumulants, up to 4th order, of deuteron number distributions and proton-deuteron correlations in Au+Au collisions recorded by the STAR experiment in phase-I of Beam Energy Scan (BES) program at the Relativistic Heavy Ion Collider. Deuteron cumulants, their ratios, and proton-deuteron mixed cumulants are presented for different collision centralities covering a range of center-of-mass energy per nucleon pair $\sqrt{s_{NN}} = 7.7$ to 200 GeV. It is found that the cumulant ratios at lower collision energies favor a canonical ensemble over a grand canonical ensemble in thermal models. An anti-correlation between proton and deuteron multiplicity is observed across all collision energies and centralities, consistent with the expectation from global baryon number conservation. The UrQMD model coupled with a phase-space coalescence mechanism qualitatively reproduces the collision-energy dependence of cumulant ratios and proton-deuteron correlations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Beam energy dependence of the linear and mode-coupled flow harmonics in Au+Au collisions

The linear and mode-coupled contributions to higher-order anisotropic flow are presented for Au+Au collisions at √ S NN = 27, 39, 54.4, and 200 GeV and compared to similar measurements for Pb+Pb collisions at the Large Hadron Collider (LHC). The coefficients and the flow harmonics' correlations, which characterize the linear and mode-coupled response to the lower-order anisotropies, indicate a beam energy dependence consistent with an influence from the specific shear viscosity (η/s). In contrast, the dimensionless coefficients, mode-coupled response coefficients, and normalized symmetric cumulants are approximately beam-energy independent, consistent with a significant role from initial-state effects. These measurements could provide unique supplemental constraints to (i) distinguish between different initial-state models and (ii) delineate the temperature (T) and baryon chemical potential (μ B ) dependence of the specific shear viscosity η/s(T, μ B ).

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Energy Dependent Fission Product Yields (2nd year Milestone and Deliverables)

Introduction to the project: One of the Laboratory missions is to provide consistent, high-precision fission product; yield data critical for testing fission models and maintaining the safety and security of the nation’s nuclear weapons stockpile. However, high-quality, energy-differential fission product yield data is missing for certain actinides and neutron energies important to constrain the new U.S. Nuclear Data Program evaluation effort; It has been shown that the reactor antineutrino anomaly may be at least partially caused by roughly 20 fission products. The fission product yield data is missing or incomplete for many of these isotopes, thus it is necessary to accurately determine these values to better constrain the anomaly; Aitor Bracho is measuring very short-lived (seconds to minutes) fission product yields of 235 U and 239 Pu using monoenergetic neutron beams at E n = 60 and 560 keV; Aitor Bracho is using a direct approach utilizing a state-of-the-art rabbit transfer system, superior HPGe detector, and digital acquisition systems for fission decay measurements. The goals of this project: lop experimental capabilities and data analysis techniques to carry out the gamma-ray spectra analysis necessary for fission product yield calculation; Provide high-precision and energy-dependent fission product data supporting fission theory, neutrino physics, and applied physics.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Energy dependence of polarized 𝛾⁢𝛾 → 𝑒 + ⁢ 𝑒− in peripheral Au+Au collisions at $\sqrt{s_{NN}}$ = 54.4 and 200 GeV with the STAR experiment at RHIC

We report the differential yields at mid-rapidity of the Breit-Wheeler process (𝛾⁢𝛾 → 𝑒 + ⁢𝑒 − ) in peripheral Au+Aucollisions at $\sqrt{s_{NN}}$ = 54.4 and 200 GeV with the STAR experiment at the Relativistic Heavy Ion Collider (RHIC), as a function of energy $\sqrt{s_{NN}}$, 𝑒 + ⁢𝑒 − transverse momentum 𝑝 T , 𝑝$^{2}_{T}$, invariant mass 𝑀 𝑒⁢𝑒 , and azimuthal angle. In the invariant mass range of 0.4 < 𝑀 𝑒⁢𝑒 < 2.6GeV/𝑐 2 at low transverse momentum (𝑝 T < 0.15GeV/𝑐), the yields increase while the pair √⟨𝑝$^{2}_{T}$⟩ decreases with increasing $\sqrt{s_{NN}}$, a feature that is correctly predicted by the QED calculation. Here, the energy dependencies of the measured quantities are sensitive to the nuclear form factor, infrared divergence and photon polarization. The data are compiled and used to extract the charge radius of the Au nucleus.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Energy-dependent implementation of secondary electron emission models in continuum kinetic sheath simulations

The plasma-material interactions present in multiple fusion and propulsion concepts between the flow of plasma through a channel and a material wall drive the emission of secondary electrons. This emission is capable of altering the fundamental structure of the sheath region, significantly changing the expected particle fluxes to the wall. The emission spectrum is separated into two major energy regimes, a peak of elastically backscattered primary electrons at the incoming energy, and cold secondary electrons inelastically emitted directly from the material. The ability of continuum kinetic simulations to accurately represent the secondary electron emission is limited by relevant models being formulated in terms of monoenergetic particle interactions which cannot be applied directly to the discrete distribution function. As a result, rigorous implementation of energy-dependent physics is often neglected in favor of simplified, constant models. We present here a novel implementation of semi-empirical models in the boundary of continuum kinetic simulations which allows the full range of this emission to be accurately captured in physically-relevant regimes.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Energy-dependent optimization of the prompt fission neutron spectrum with CGMF

Throughout the course of FY21, significant effort was put into investigating models within the LANL developed Hauser-Feshbach fission fragment decay code, CGMF, to understand and potentially solve the long-standing challenge of a too-soft prompt fission neutron spectrum, PFNS. Several inputs and models to CGMF were investigated, including the discrete nuclear levels, the optical model potential, level densities, and the fission fragment initial conditions. Some of the global models within CGMF led to a slight hardening of the neutron spectrum—particularly the likely incomplete discrete levels in through which γ-rays decay—but none of the changes where large enough for the tail of the PFNS to reproduce experimental data. A significant hardening of the spectrum tail was observed when the fission fragment initial conditions were optimized based on their sensitivities to the PFNS data for thermal incident neutrons. In this way, the parameters for the CGMF mass and total kinetic energy distributions, along with the spin cutoff factor were adjusted to better reproduce the experimental PFNS measurements. This optimization hardened the tail of the PFNS slightly but led to unphysical mass distributions for the fission fragments before neutron emission. It was clear from the above that we do not expect to be able to produce an evaluation-quality PFNS with CGMF in the near future. Challenges at thermal will persist–and possibly worsen–with increasing incident energy, where more models are needed to completely describe the fission. Basic-science research funding exceeding the amount available and scope of our NCSP funds would be needed to tackle this decade-long challenge impacting many fission-fragment event generator. And, in fact, Amy Lovell won LDRD ECR funding to do so over the next few years. Therefore, we focused in FY22 on extending evaluation capabilities beyond thermal incident neutrons, to take into account the incident energy dependence of the PFNS and fission fragment initial condition distributions in CGMF. We chose to set up the evaluation methodology to perform PFNS evaluations with CGMF across incident-neutron energies, in order to have it readily available for future NCSP evaluations when the PFNS from CGMF has improved. In this report, we outline the evaluation methodology, along with the results of the optimization, including full model calculations with CGMF using the evaluated parameters.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Energy dependence of intermittency for charged hadrons in Au+Au collisions at RHIC

Density fluctuations near the QCD critical point can be probed via an intermittency analysis in relativistic heavy-ion collisions. We report the first measurement of intermittency in Au+Au collisions at $\sqrt{s{NN}}$ = 7.7-200 GeV measured by the STAR experiment at the Relativistic Heavy Ion Collider (RHIC). The scaled factorial moments of identified charged hadrons are analyzed at mid-rapidity and within the transverse momentum phase space. We observe a power-law behavior of scaled factorial moments in Au+Au collisions and a decrease in the extracted scaling exponent (ν) from peripheral to central collisions. The ν is consistent with a constant for different collisions energies in the mid-central (10-40%) collisions. Moreover, the ν in the 0-5% most central Au+Au collisions exhibits a non-monotonic energy dependence that reaches a minimum around $\sqrt{s{NN}}$ = 27 GeV. The physics implications on the QCD phase structure are discussed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Symmetry-Energy Dependence of the Bulk Viscosity of Nuclear Matter

We clarify how the weak-interaction-driven bulk viscosity ζ and the bulk relaxation time τ Π of neutrino-transparent n p e matter depend on the nuclear symmetry energy. We show that, at saturation density, the equation-of-state dependence of these transport quantities is fully determined by the experimentally constrained nuclear symmetry energy S and its slope L . Variations of L can change the bulk viscosity by orders of magnitude, which can affect both the dissipative and the conservative tidal response of neutron stars. Furthermore, this suggests that both conservative and dissipative effects encoded in the gravitational-wave signatures of binary neutron star inspirals may help constrain nuclear symmetry-energy properties.

Neutron stars & pulsars↗

Collision-System and Beam-Energy Dependence of Anisotropic Flow Fluctuations

Here, elliptic flow measurements from two-, four- and six-particle correlations are used to investigate flow fluctuations in collisions of U+U at $\sqrt{s_{NN}}$ = 193 GeV, Cu+Au at $\sqrt{s_{NN}}$ = 200 GeV and Au+Au spanning the range $\sqrt{s_{NN}}$ = 11.5 - 200 GeV. The measurements show a strong dependence of the flow fluctuations on collision centrality, a modest dependence on system size, and very little if any, dependence on particle species and beam energy. The results, when compared to similar LHC measurements, viscous hydrodynamic calculations, and Glauber model eccentricities, indicate that initial-state-driven fluctuations predominate the flow fluctuations generated in the collisions studied.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Excitation Laser Energy Dependence of the Gap-Mode TERS Spectra of WS 2 and MoS 2 on Silver

In this work we present a systematic study of the dependence of the gap mode tip-enhanced Raman scattering (TERS) response of the mono- and bi-layer WS 2 and MoS 2 on silver as a function of the excitation laser energy in a broad spectral range from 473nm to 830 nm. For this purpose, we collected consecutive TERS maps of the same area in the sample containing mono-and bi-layer regions with the same TERS probe with 6 different excitation lasers. To decrease the number of collected TERS maps, we used for the first time to the best of our knowledge, concurrent excitation and collection with two lasers simultaneously. We found that the E 2g /A 1g peak intensity ratio for the bilayer WS 2 @Ag and the ratio of the A’/A 1g peak intensity of the out-of-plane mode for the mono- and the bilayer, change in a significantly non-monotonous way as the excitation laser energy is swept from 1.58 eV to 2.62 eV. The former ratio increases at energies corresponding to A and B excitons (~2.0 eV and 2.4 eV correspondingly) in bilayer WS 2 . The absolute intensity of the A’ peak in the monolayer, and correspondingly the A’/A 1g ratio, is surprisingly high at lower excitation energies, but dips dramatically at the energy corresponding to the A exciton, being restored partially in between A and B excitons, but still showing the descending trend as the excitation laser energy increases. A somewhat similar picture was observed in mono- and bi-layers of MoS 2 @Ag, though the existing set of excitation lasers did not match the excitonic profile of this material as nicely as for the case of WS 2 . We attribute the observed behavior to the presence of intermediate (Fano resonance) or strong (Rabi splitting) coupling between the excitons in transition metal dichalcogenides (TMDs) and the plasmons in the tip-substrate nanocavity. This is akin to the so-called Fano (Rabi) transparency experimentally observed in far field scattering from transition metal dichalcogenides between two plasmonic metals. The possibility of the formation of intermediate/strong coupling between the excitonic resonances in TMDs and the nanocavity re-evaluates the role of various resonances in the gap-mode TERS and should become an important factor to be considered by TERS practitioners during planning the experiments. Lastly, based on observed phenomena and its explanation, we propose the “ideal” substrate for efficient TERS and tip enhanced photoluminescence (TEPL) measurements.

Raman spectroscopy↗

Search for the chiral magnetic effect through beam energy dependence of charge separation using event shape selection

High-energy, heavy-ion collisions can create local domains of chirality-imbalanced quarks, reflecting the topological features of quantum chromodynamics. The chiral magnetic effect (CME) predicts an electric charge separation of quarks in such topological domains along the magnetic field ($\vec{B}$) generated by the passing of two high-Z nuclei. Here, we use a correlation observable Δ⁢𝛾$^{112}$ between charged meson pairs to detect the CME-induced charge separation and a novel event shape selection (ESS) method to mitigate the background effects related to elliptic flow (𝑣 2 ). The ESS method classifies events based on the emission pattern of final-state particles and determines Δ⁢𝛾$^{112}_{ESS}$ from the zero-flow limit. We reconstruct the $\vec{B}$ field direction from the spectator nucleons, which minimizes backgrounds unrelated to the collective motion of the system. In this work, we report the measurements of Δ⁢𝛾$^{112}$ and a background indicator Δ⁢𝛾$^{132}$ in Au+Au collisions from the Brookhaven National Laboratory Relativistic Heavy Ion Collider (RHIC) Beam Energy Scan phase II and at the top RHIC energy. After background suppression, Δ⁢𝛾$^{132}_{ESS}$ aligns with zero, and Δ⁢𝛾$^{112}_{ESS}$ is reduced to no more than 20% of Δ⁢𝛾$^{112}$. We observe a finite residual charge separation with 2.5⁢𝜎, 3⁢𝜎, and 3.2⁢𝜎 significance in the 20–50% centrality range of Au + Au collisions at 11.5, 14.6, and 19.6 GeV. The results at 17.3 and 27 GeV also show positive values but with a lower significance of 1.3⁢𝜎 and 1.1⁢𝜎, respectively. The corresponding Δ⁢𝛾$^{112}_{ESS}$ values at 7.7, 9.2, and 200 GeV are consistent with zero within uncertainties.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Experimental study of energy-dependent angular broadening of MeV electron beams for high-resolution imaging in thick samples

In scanning transmission electron microscopy (STEM), spatial resolution is primarily influenced by the projected size of the electron probe within the specimen. In thin samples, a large semi-convergence angle enables a tightly focused beam and sub-nanometer resolution. However, in thick specimens, resolution is fundamentally limited by transverse beam broadening from multiple large-angle scattering events—for example, a probe with 10 mrad angular divergence can broaden by ∼100 nm over a 10 μm path. Since this broadening scales inversely with beam energy, MeV-STEM offers a promising route for high-resolution imaging in thick materials. To quantitatively assess this effect, we performed high-precision measurements at UCLA’s PEGASUS beamline, characterizing beam divergence and intensity profiles for 3–8 MeV electrons transmitted through a wedged-silicon sample of varying thickness. Our results reconcile discrepancies among analytical models and validate Monte Carlo simulations. Here, we find that increasing beam energy from 3.0 to 5.8 MeV reduces angular broadening by a factor of 2.6, with diminishing returns observed at 7.6 MeV. These findings provide a quantitative framework for optimizing MeV-STEM parameters in high-resolution imaging of thick biological and microelectronic specimens, and for guiding beam energy selection in other advanced imaging modes beyond STEM.

36 MATERIALS SCIENCE↗

Nonmonotonic Energy Dependence of Net-Proton Number Fluctuations

Nonmonotonic variation with collision energy (√ s NN) of the moments of the net-baryon number distribution in heavy-ion collisions, related to the correlation length and the susceptibilities of the system, is suggested as a signature for the quantum chromodynamics critical point. Here, we report the first evidence of a nonmonotonic variation in the kurtosis times variance of the net-proton number (proxy for net-baryon number) distribution as a function of √ s NN with 3.1 σ significance for head-on (central) gold-on-gold (Au+Au) collisions measured solenoidal tracker at Relativistic Heavy Ion Collider. Data in noncentral Au+Au collisions and models of heavy-ion collisions without a critical point show a monotonic variation as a function of √ s NN.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Probing Gluon Fluctuations in Nuclei with the First Energy-Dependent Measurement of Incoherent 𝐽/𝜓 Photoproduction in Ultraperipheral PbPb Collisions

Incoherent 𝐽/𝜓 photoproduction in heavy ion ultraperipheral collisions (UPCs) provides a sensitive probe of localized, fluctuating gluonic structures within heavy nuclei. This Letter reports the first measurement of the photon-nucleon center-of-mass energy (𝑊 𝛾⁢N ) dependence of this process in PbPb UPCs at a nucleon-nucleon center-of-mass energy of 5.02 TeV, using 1.52 nb −1 of data recorded by the CMS experiment. The measurement covers a wide 𝑊 𝛾⁢N range of ≈40–400 GeV, probing gluons carrying a fraction 𝑥 of nucleon momentum down to an unexplored regime of 6.5 ×10 −5 . Compared to baseline predictions neglecting nuclear effects, the measured cross sections exhibit significantly greater suppression at lower 𝑥. Additionally, the ratio of incoherent to coherent photoproduction is found to be constant across the probed 𝑊 𝛾⁢N and 𝑥 range, disfavoring the establishment of the black disk limit. This Letter provides critical insights into the 𝑥-dependent evolution of fluctuating gluonic structures within nuclei and calls for further advancements in theoretical models incorporating nuclear shadowing and gluon saturation.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Beam Energy Dependence of Fifth- and Sixth-Order Net-Proton Number Fluctuations in Au + Au Collisions at RHIC

We report the beam energy and collision centrality dependence of fifth and sixth order cumulants (C 5 , C 6 ) and factorial cumulants (κ 5 , κ 6 ) of net-proton and proton distributions, from $\sqrt{s_{NN}}$=3-200 GeV Au+Au collisions at RHIC. The net-proton cumulant ratios generally follow the hierarchy expected from QCD thermodynamics, except for the case of collisions at $\sqrt{s_{NN}}$ = 3 GeV. C 6 /C 2 for 0-40\% centrality collisions is increasingly negative with decreasing $\sqrt{s_{NN}}$, while it is positive for the lowest $\sqrt{s_{NN}}$ studied. These observed negative signs are consistent with QCD calculations (at baryon chemical potential, μ B ≤ 110 MeV) that include a crossover quark-hadron transition. In addition, for $\sqrt{s_{NN}}$≥ 11.5 GeV, the measured proton κ n , within uncertainties, does not support the two-component shape of proton distributions that would be expected from a first-order phase transition. Taken in combination, the hyper-order proton number fluctuations suggest that the structure of QCD matter at high baryon density, μ B ~750 MeV ($\sqrt{s_{NN}}$ = 3 GeV) is starkly different from those at vanishing μ B ~20MeV ($\sqrt{s_{NN}}$ = 200 GeV and higher).

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Inefficient intramolecular vibrational energy redistribution for the H + HO2 reaction and negative internal energy dependence for its rate constant

Quasiclassical trajectories (QCT) and newly constructed global potential energy surfaces are used to compute thermal and nonthermal rate constants for the H + HO 2 reaction. The thermal QCTs rate constants are up to 50% smaller than transition state theory (TST) rate constants based on the same level of electronic structure theory. This reduction is demonstrated to result from inefficient intramolecular vibrational energy redistribution (IVR) in the transient H 2 O 2 well, with a significant fraction of trajectories that reach the H 2 O 2 well promptly dissociating back to reactants instead of via the heavily statistically favored 2OH channel. The nonstatistical reduction factor, κ IVR , that quantifies this effect is shown to increase in importance with temperature, with κ IVR = 0.81 at 300 K and 0.47 at 2500 K. Finally, we show that inefficient IVR causes H + HO 2 rate constants mediated by H 2 O 2 to depend inversely on the initial vibrational excitation of HO 2 .

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗