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At least 55 records · Page 3

Event-by-event correlations between Λ ( Λ ¯ ) hyperon global polarization and handedness with charged hadron azimuthal separation in Au + Au collisions at s N N = 27 GeV from STAR

Global polarizations (P) of Λ (Λ¯) hyperons have been observed in non-central heavy-ion collisions. The strong magnetic field primarily created by the spectator protons in such collisions would split the Λ and Λ¯ global polarizations (ΔP=P Λ –P Λ ¯<0). Additionally, quantum chromodynamics (QCD) predicts topological charge fluctuations in vacuum, resulting in a chirality imbalance or parity violation in a local domain. This would give rise to an imbalance (Δn = N L –N R /< N L +N R > ≠0) between left- and right-handed Λ (Λ¯) as well as a charge separation along the magnetic field, referred to as the chiral magnetic effect (CME). This charge separation can be characterized by the parity-even azimuthal correlator (Δγ) and parity-odd azimuthal harmonic observable (Δa 1 ). Measurements of ΔP, Δγ, and Δa 1 have not led to definitive conclusions concerning the CME or the magnetic field, and Δn has not been measured previously. Correlations among these observables may reveal new insights. Furthermore, this paper reports measurements of correlation between Δn and Δa 1 , which is sensitive to chirality fluctuations, and correlation between ΔP and Δγ sensitive to magnetic field in Au+Au collisions at 27 GeV. For both measurements, no correlations have been observed beyond statistical fluctuations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Charge-dependent flow induced by electromagnetic fields in heavy ion collisions

The colliding heavy ions create extremely strong magnetic and electric fields that significantly affect the evolution of the produced quark-gluon plasma (QGP). The knowledge of these fields is essential for establishing the role of topological fluctuations in the QGP through the chiral magnetic effect and related anomaly-induced phenomena. In this talk, we describe our work on the evolution of the QGP in electric and magnetic fields in the framework of hydrodynamics supplemented, in a perturbative fashion, by the dynamical electromagnetism. The evolution of the QGP fluid is described within the iEBE-VISHNU framework. We find that the electromagnetically induced currents result in a charge-odd directed flow Δv 1 and a charge-odd Δv 3 flow both of which are odd in rapidity. Furthermore, while the predicted magnitude of these charge-odd flows agrees with the data from RHIC and LHC, the sign of the predicted asymmetry between the flows of positive and negative hadrons is opposite to the data.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Spectral theorems for generalized Weyl nodes with impurities in a magnetic field

Here, we prove a few spectral theorems for the density of states of a Weyl node with arbitrary topology. We show that the density of extended states of a Weyl node with random impurity potentials remains gapless in the presence of a magnetic field. Therefore, a magnetic field precludes Anderson localization in Weyl semimetals, when internode transitions are suppressed for smooth enough potentials. We also provide a rigorous quantum mechanical proof of the chiral magnetic effect for arbitrary topology of a Weyl node.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Insights into the Mechanism of Chiral‐Induced Spin Selectivity: The Effect of Magnetic Field Direction and Temperature

Chiral oligopeptide monolayers are adsorbed on a ferromagnetic surface and their magnetoresistance is measured as a function of the angle between the magnetization of the ferromagnet and the surface normal. These measurements are conducted as a function of temperature for both enantiomers. The angle dependence is found to follow a changing trend with a period of 360°. Quantum simulations reveal that the angular distribution can be obtained only if the monolayer has significant effective spin orbit coupling (SOC), that includes contribution from the vibrations. The model shows that SOC only in the leads cannot reproduce the observed angular dependence. The simulation can reproduce the experiments if it included electron–phonon interactions and dissipation.

36 MATERIALS SCIENCE↗

Auxiliary field diffusion Monte Carlo calculations of magnetic moments of light nuclei with chiral effective field theory interactions

We calculate the magnetic moments of light nuclei $( A < 20 )$ using the auxiliary field diffusion Monte Carlo method and local two- and three-nucleon forces with electromagnetic currents from chiral effective field theory. For all nuclei under consideration, we also calculate the ground-state energies and charge radii. We generally find a good agreement with experimental values for all of these observables. For the electromagnetic currents, we explore the impact of employing two different power counting schemes, and study theoretical uncertainties stemming from the truncation of the chiral expansion order by order for select nuclei within these two approaches. In conclusion, we find that it is crucial to employ consistent power counting schemes for interactions and currents to achieve a systematic order-by-order convergence.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Photoredox Catalysis with Spin Magnetic Field Effects: A Scheme for Chiral Resolution

Quantities that break both mirror symmetry and time-reversal symmetry, such as the orbital angular momentum, are known to connect molecular chirality with an applied magnetic field. This concept has led to observations such as magneto-chiral dichroism and chirality-induced spin selectivity (CISS). However, being small, these effects often require additional amplification procedures such as flow chemistry to achieve bulk enantioseparation. In this work, we demonstrate how the magnetic field effect on photogenerated radical pairs, which also breaks time-reversal symmetry, can be harnessed for enantiopurification. Fundamental to this process is the collective decay of the singlet and triplet radical-pair states made possible by an applied magnetic field. Because opposite enantiomers exhibit spin-orbit coupling matrix elements of opposite signs, the singlet and triplet decay channels interfere constructively in one enantiomer. Meanwhile, molecules of the other enantiomer are funnelled into the first enantiomer through excited-state chirality inversion, achieving (dynamic kinetic) chiral resolution. Using an axially chiral binaphthyl derivative and a borane photosensitizer as prototype, we predict an appreciable enantiomeric excess (e.e.) of 90% to be possible at steady state, attained within hundreds of milliseconds when irradiated by a laser. Importantly, our analytical results showcase regimes of perfect enantioselectivity (100% e.e.), accessible by further chemical optimization of the photosensitizer for which general strategies are discussed. Altogether, this work illustrates a so-far untapped but powerful control knob for photoredox catalysis based on spin chemistry principles.

Magnetic properties↗

Vortical effects in chiral band structures

The chiral vortical effect is a chiral anomaly-induced transport phenomenon characterized by an axial current in a uniformly rotating chiral fluid. It is well understood for Weyl fermions in high energy physics, but its realization in condensed matter band structures, including those of Weyl semimetals, has been controversial. In this work, we develop the Kubo response theory for electrons in a general band structure subject to space- and time-dependent rotation or vorticity relative to the background lattice. For continuum Hamiltonians, we recover the chiral vortical effect in the static limit and the transport or uniform limit when the fluid, strictly, is not a Fermi liquid. In the transport limit of a Fermi liquid, we describe an effect that we dub the gyrotropic vortical effect. The latter is governed by Berry curvature of the occupied bands while the former contains an additional contribution from the magnetic moment of electrons on the Fermi surface. The two vortical effects can be understood as kinematic analogs of the well-known chiral and gyrotropic magnetic effects in chiral band structures. As a result, we address recent controversies in the field and conclude by describing device geometries that exploit Ohmic or Seebeck transport to drive the vortical effects.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Deconvolution of X-ray natural and magnetic circular dichroism in chiral Dy-ferroborate

Structural chirality and magnetism, when intertwined, can have profound implications on materials properties. Using X-ray imaging and spectroscopic measurements that leverage the natural and magnetic circular dichroic effects present in magnetized chiral crystal structures, we probe the interplay between chirality and magnetism across the field-induced spin-flop transition of Dy ferroborate, DyFe 3 (BO 3 ) 4 . Deconvolution of natural and magnetic circular dichroic signals at the Fe K and Dy L 2,3 absorption edges of the non-centrosymmetric structure was enabled by use of tunable temperature and magnetic field, providing access to element-specific magnetic information across the spin-flop transition. The magnetic response of Fe and Dy sublattices was found to be independent of domain chirality. The chiral domains were robust against both the (chirality preserving) R32 to P3 1 21/P3 2 21 structural phase transition at 280 K, and application of magnetic field up to 4 Tesla. A third flavor of X-ray dichroism, magneto-chiral dichroism, was not detected within the accuracy of our measurements. The absence of significant Fe magnetization along the screw, c-axis for the magnetic field strength used in this study, together with non-linear coupling of magnetic field to electric polarization across the spin-flop transition, may hinder observation of magneto-chiral dichroic effects in this system.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Chiral Magnetic Josephson Junction as a Base for Low-Noise Superconducting Qubits

The lack of space inversion symmetry endows non-centrosymmetric superconducting materials with various interesting parity-breaking phenomena, including the anomalous Josephson effect. Our paper considers a Josephson junction of two non-centrosymmetric superconductors connected by a uniaxial ferromagnet. We show that this “Chiral Magnetic Josephson junction” (CMJ junction) exhibits a direct analog of the Chiral Magnetic Effect, which has already been observed in Weyl and Dirac semimetals. We suggest that the CMJ can serve as an element of a qubit with a Hamiltonian tunable by the ferromagnet’s magnetization. The CMJ junction avoids using an offset magnetic flux in inductively shunted qubits, thus enabling a simpler and more robust architecture. Furthermore, when the uniaxial ferromagnet’s easy axis is directed across the junction, the resulting “chiral magnetic qubit” provides robust protection from the noise caused by magnetization fluctuations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Magnetic moments of A = 3 nuclei obtained from chiral effective field theory operators

Chiral effective field theory (χEFT) provides a framework for obtaining internucleon interactions in a systematically improvable fashion from first principles, while also providing for the derivation of consistent electroweak current operators. In this study, we apply consistently derived interactions and currents towards calculating the magnetic dipole moments of the A = 3 systems 3 H and 3 He. We focus here on LENPIC interactions obtained using semilocal coordinate-space (SCS) regularization. Starting from the momentum-space representation of the LENPIC χEFT vector current, we derive the SCS-regularized magnetic dipole operator up through next-to-next-to-leading order (N 2 LO). We then carry out no-core shell-model calculations for 3 H and 3 He systems using the SCS LENPIC interaction at N 2 LO in χEFT and evaluate the magnetic dipole moments obtained using the consistently derived one-nucleon and two-nucleon electromagnetic currents. As anticipated by prior results with χEFT currents, the current corrections through N 2 LO provide improved, but not yet complete, agreement with experiment for the 3 H and 3 He magnetic dipole moments.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Path integral approach to quantum anomalies in interacting models

The prediction and subsequent discovery of topological semimetal phases of matter in solid state systems has instigated a surge of activity investigating the exotic properties of these unusual materials. Among these are transport signatures which can be attributed to the chiral anomaly; the breaking of classical chiral symmetry in a quantum theory. This remarkable quantum phenomenon, first discovered in the context of particle physics has now found new life in condensed-matter physics, connecting topological quantum matter and band theory with effective field theoretic models. In this paper we investigate the interplay between interactions and the chiral anomaly in field theories inspired by semimetals using Fujikawa's path integral method. Starting from models in one spatial dimension we discuss how the presence of interactions can affect the consequences of the chiral anomaly leading to renormalization of excitations and their transport properties. This is then generalized to the three-dimensional case where we show that the anomalous response of the system, namely, the chiral magnetic and quantum Hall effects, are modified by the presence of interactions. These properties are investigated further through the identification of anomalous modes which exist within interacting Weyl semimetals. These massive excitations are nonperturbative in nature and are a direct consequence of the chiral anomaly. The effects of interactions on mixed axial-gravitational anomalies are then investigated and the conditions required for interaction effects to be observed are discussed.

Anomalies↗

Multimodal Approach Reveals the Symmetry-Breaking Pathway to the Broken Helix in EuIn 2 ⁢As 2

Understanding and manipulating emergent phases, which are themes at the forefront of quantum-materials research, rely on identifying their underlying symmetries. This general principle has been particularly prominent in materials with coupled electronic and magnetic degrees of freedom, in which magnetic order influences the electronic band structure and can lead to exotic topological effects. However, identifying symmetry of a magnetically ordered phase can pose a challenge, particularly in the presence of small domains. Here we introduce a multimodal approach for determining magnetic structures, which combines symmetry-sensitive optical probes, scattering, and group-theoretical analysis. We apply it to EuIn 2 ⁢As 2 , a material that has received attention as a candidate axion insulator. While first-principles calculations predict this state on the assumption of a simple collinear antiferromagnetic structure, subsequent neutron-scattering measurements reveal a much more intricate magnetic ground state characterized by two coexisting magnetic wave vectors reached by successive thermal phase transitions. The proposed high- and low-temperature phases are a spin helix and a state with interpenetrating helical and Néel antiferromagnetic order termed a “broken helix,” respectively. Employing a multimodal approach, we identify the magnetic structure associated with these two phases of EuIn 2 ⁢As 2 . We find that the higher-temperature phase is characterized by a variation of the magnetic moment amplitude from layer to layer, with the moment vanishing entirely in every third Eu layer. The lower-temperature structure is similar to the broken helix, with one important difference: Because of local strain, the relative orientation of the magnetic structure and the lattice is not fixed. Consequently, the symmetry required to protect the axion phase is not generically protected in EuIn 2 ⁢As 2 , but we show that it can be restored if the magnetic structure is tuned with uniaxial strain. Finally, we present a spin Hamiltonian that identifies the spin interactions that account for the complex magnetic order in EuIn 2 ⁢As 2 . Our work highlights the importance of a multimodal approach in determining the symmetry of complex order parameters.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Magnetic structure of few-nucleon systems at high momentum transfers in a chiral effective field theory approach

The five low-energy constants (LECs) in the electromagnetic current derived in chiral effective field theory ( χ EFT ) up to one loop are determined by a simultaneous fit to the A = 2 – 3 nuclei magnetic moments and to the deuteron magnetic form factor and threshold electrodisintegration at backward angles over a wide range of momentum transfers. The resulting parametrization then yields predictions for the 3 He/ 3 H magnetic form factors in excellent accord with the experimental values for momentum transfers ranging up to ≈0.8 GeV/c, beyond the expected regime of validity of the χEFT approach. The calculations are based on last-generation two-nucleon interactions including high orders in the chiral expansion and derived by Entem, Machleidt, and Nosyk [Phys. Rev. C 96, 024004 (2017)] and by Piarulli et al. [Phys. Rev. C 94, 054007 (2016)], using different χEFT formulations. In the A = 3 calculations, (chiral) three-nucleon interactions are also accounted for. The model dependence resulting from these different formulations of the interactions is found to be mild for momentum transfer below ≈0.8 GeV/c . Further, an analysis of the convergence of the chiral expansion is also provided.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Multiple ferroic orders and toroidal magnetoelectricity in the chiral magnet BaCoSiO 4

Discovering ferroic phase transitions and their consequential physical properties is at the core of condensed matter science due to rich physics and tremendous technological promises. BaCoSiO 4 , a chiral antiferromagnet, belongs to the tetrahedron-based chiral system, and exhibits diverse ferroic orders with coexisting chirality, polarity, trimerization, ferrorotational distortions, and magnetism. However, their mutual couplings remain to be explored. Here in this work, we used a comprehensive combination of several experimental tools—in situ x-ray, transmission electron microscopy, magnetization, and magnetoelectric measurements of single-crystalline BaCoSiO 4 —to investigate hierarchical phase transitions, their microscopic domain structures, and the resulting magnetoelectricity. We found that two different structural chiralities develop through distinct processes: global homochirality and local heterochirality induced by the ferrorotational distortions on top of existing polarization. In addition, magnetic chirality, with the simultaneous presence of net magnetic moment and magnetic toroidal moment, develops below 3.2 K due to the global chirality, which leads to magnetic field tunable toroidal magnetoelectricity. Thus, BaCoSiO 4 exhibits uniquely all four types of ferroic orders and provides an avenue to explore, for example, tunable or dynamic coupling of multiple ferroic degrees of freedom.

36 MATERIALS SCIENCE↗