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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 523 records · Page 29
All sourcesNASA NTRSDOE OSTI
DOE OSTI2013

Selective excitation of spin resonance in orthoferrite PrFeO{sub 3} with impulsive polarized terahertz radiation

Single cycle terahertz (THz) pulses were employed to excite coherent spin waves in (110)-oriented PrFeO{sub 3} single crystal. The free induction decay radiations at frequency of 0.34 THz (quasi-ferromagnetic mode, FM mode) and 0.41 THz (quasi-antiferromagnetic mode, AFM mode) were observed arising from the coupling of magnetic moment with the impulsive magnetic field of polarized terahertz radiation. These two spin modes in PrFeO{sub 3} can be excited and modulated by the magnetic field of THz pulse with a specific polarization with respect to the crystal axis. The extracted complex dielectric permittivity and magnetic permeability dispersion in THz range suggest a higher efficiency of energy transfer from the impulsive THz pulse into the AFM than the FM spin system.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2015

Skyrmion stability in nanocontact spin-transfer oscillators

We investigate the conditions for nanocontact spin-transfer oscillators (NC-STOs) that allow for stabilization of a skyrmion. Emphasis is made on the breathing mode, which can be regarded as a source of microwave generation. Micromagnetic simulations of NC-STOs with varying parameters have been performed, with the resulting magnetization plotted in the form of phase diagrams. It is found that control of spin wave mode in conventional STOs can be applied to skyrmion-based STOs.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2026

A personal spin on spin currents

This article contains my personal account on how I got interested in spin transport phenomena, which ultimately resulted in investigating multiple facets of spin–orbit torques, as well as magnetization dynamics. Originally this research focused on questions that seemed rather academic with little relevance to applications. But over time it developed into one of the key research areas for modern spintronic devices. This journey started off with investigating spin polarized charge currents, later focused on pure spin currents, and ultimately explored spin waves (magnons) as the potential carriers of spin information. Most of this work was performed in the Magnetic Films group of the Argonne National Laboratory, which for more than three decades used to be one of the world-leading places for magnetism research.

36 MATERIALS SCIENCE↗
DOE OSTI2026

Phase diagram and spectroscopic signatures of a supersolid in the quantum ising magnet K 2 Co(SeO 3 ) 2

Supersolid phases are quantum-entangled states of matter exhibiting the dual characteristics of superfluidity and solidity. Theory predicts that hard-core bosons on a triangular lattice can form such phases at half filling and near complete filling. Leveraging an exact mapping between bosons and spin-$\frac{1}{2}$ degrees of freedom, here we show that these phases are realized in the triangular-lattice antiferromagnet K 2 Co(SeO 3 ) 2 . At zero field, neutron diffraction reveals the development of quasi-two-dimensional $\sqrt3$ x $\sqrt3$ magnetic order with Z 3 translational symmetry breaking (solidity), though with reduced amplitude indicating strong quantum fluctuations. These fluctuations manifest as equidistant bands of continuum neutron scattering, where the lowest-energy mode is gapless at K ($\frac{1}{3}$ $\frac{1}{3}$), consistent with broken U(1) spin rotational symmetry (superfluidity). For c-axis-oriented magnetic fields near saturation, we find a second phase consistent with a high-field supersolid. These two supersolids are separated by a pronounced 1/3 magnetization plateau phase that supports coherent spin waves, from which we determine the underlying spin Hamiltonian.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2025

Spin dynamics in linear magnetoelectric material Mn 3 Ta 2 O 8

We performed inelastic neutron scattering experiments on single crystal samples of a linear magnetoelectric material Mn 3 Ta 2 O 8 , which exhibits a collinear antiferromagnetic order, to reveal the spin dynamics. Numerous modes observed in the neutron spectra were reasonably reproduced by linear spin-wave theory on the basis of the spin Hamiltonian including eight Heisenberg interactions and an easy-plane type single-ion anisotropy. In conclusion, the presence of strong frustration was found in the identified spin Hamiltonian.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2023

Continuous Spin Excitations in the Three-Dimensional Frustrated Magnet K 2 Ni 2 ⁢(SO 4 ) 3

Continuous spin excitations are widely recognized as one of the hallmarks of novel spin states in quantum magnets, such as quantum spin liquids (QSLs). Here, we report the observation of such kind of excitations in K 2 Ni 2 (SO 4 ) 3 , which consists of two sets of intersected spin-1 (Ni 2+ ) trillium lattices. Our inelastic neutron scattering measurement on single crystals clearly shows a dominant excitation continuum, which exhibits a distinct temperature-dependent behavior from that of spin waves and is rooted in strong quantum spin fluctuations. Further using the self-consistent-Gaussian-approximation method, we determine that the fourth- and fifth nearest-neighbor exchange interactions are dominant. These two bonds together form a unique three-dimensional network of corner-sharing tetrahedra, which we name as a “hypertrillium” lattice. In conclusion, our results provide direct evidence for the existence of QSL features in K 2 Ni 2 (SO 4 ) 3 and highlight the potential for the hypertrillium lattice to host frustrated quantum magnetism.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2016

Surface spin-electron acoustic waves in magnetically ordered metals

Degenerate plasmas with motionless ions show existence of three surface waves: the Langmuir wave, the electromagnetic wave, and the zeroth sound. Applying the separated spin evolution quantum hydrodynamics to half-space plasma, we demonstrate the existence of the surface spin-electron acoustic wave (SSEAW). We study dispersion of the SSEAW. We show that there is hybridization between the surface Langmuir wave and the SSEAW at rather small spin polarization. In the hybridization area, the dispersion branches are located close to each other. In this area, there is a strong interaction between these waves leading to the energy exchange. Consequently, generating the Langmuir waves with the frequencies close to hybridization area we can generate the SSEAWs. Thus, we report a method of creation of the spin-electron acoustic waves.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2015

Spectral shape deformation in inverse spin Hall voltage in Y{sub 3}Fe{sub 5}O{sub 12}|Pt bilayers at high microwave power levels

We report on the deformation of microwave absorption spectra and of the inverse spin Hall voltage signals in thin film bilayers of yttrium iron garnet (YIG) and platinum at high microwave power levels in a 9.45-GHz TE{sub 011} cavity. As the microwave power increases from 0.15 to 200 mW, the resonance field shifts to higher values, and the initially Lorentzian spectra of the microwave absorption intensity as well as the inverse spin Hall voltage signals become asymmetric. The contributions from opening of the magnetization precession cone and heating of YIG cannot well reproduce the data. Control measurements of inverse spin Hall voltages on thin-film YIG|Pt systems with a range of line widths underscore the role of spin-wave excitations in spectral deformation.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2015

Non-local detection of spin dynamics via spin rectification effect in yttrium iron garnet/SiO{sub 2}/NiFe trilayers near simultaneous ferromagnetic resonance

The spin rectification effect (SRE), a phenomenon that generates dc voltages from ac microwave fields incident onto a conducting ferromagnet, has attracted widespread attention due to its high sensitivity to ferromagnetic resonance (FMR) as well as its relevance to spintronics. Here, we report the non-local detection of yttrium iron garnet (YIG) spin dynamics by measuring SRE voltages from an adjacent conducting NiFe layer up to 200 nm thick. In particular, we detect, within the NiFe layer, SRE voltages stemming from magnetostatic surface spin waves (MSSWs) of the adjacent bulk YIG which are excited by a shorted coaxial probe. These non-local SRE voltages within the NiFe layer that originates from YIG MSSWs are present even in 200 nm-thick NiFe films with a 50 nm thick SiO{sub 2} spacer between NiFe and YIG, thus strongly ruling out the mechanism of spin-pumping induced inverse spin Hall effect in NiFe as the source of these voltages. This long-range influence of YIG dynamics is suggested to be mediated by dynamic fields generated from YIG spin precession near YIG/NiFe interface, which interacts with NiFe spins near the simultaneous resonance of both spins, to generate a non-local SRE voltage within the NiFe layer.

36 MATERIALS SCIENCE↗
DOE OSTI2015

Magnonic crystal as a delay line for low-noise auto-oscillators

It is demonstrated that a delay line based on a one-dimensional magnonic crystal used in a feedback loop of a microwave auto-oscillator can substantially reduce the phase noise figure and improve other vital performance characteristics of the auto-oscillator. The advantage is achieved due to the increase of the effective delay time in the magnonic crystal, compared to the case of an un-patterned yttrium iron garnet (YIG) film, and improvement of the power-handling characteristics due to the now possible increase of the YIG film thickness. The internal modes of a magnonic crystal caused by the periodic energy exchange between the incident and reflected spin waves play the dominant role in the described effect.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2014

Collective modes in cold paramagnetic gases

We have obtained a condition for the emergence of spin waves in paramagnetic gases Re >> ImÂ, which is fulfilled only at temperatures of the order of 1 μK. (laser applications and other topics in quantum electronics)

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2018

Condensation of Pseudomagnons in a Two-Dimensional Anisotropic S = 1 Pseudospin System

Abstract—A 2D anisotropic system of S = 1 centers of the charge triplet type in systems with variable valence or “semi-hard-core” boson systems with a limitation for the occupation of lattice sites n = 0, 1, 2 is studied in the framework of the pseudospin formalism. Assuming that the ground state is a quantum paramagnet, the pseudo-spin wave spectrum and also the conditions of the condensation of pseudomagnons with a phase transition to a superconducting state have been found using the Schwinger boson method.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2014

Observations of thermally excited ferromagnetic resonance on spin torque oscillators having a perpendicularly magnetized free layer

Measurements of thermally excited ferromagnetic resonance were performed on spin torque oscillators having a perpendicularly magnetized free layer and in-plane magnetized reference layer (abbreviated as PMF-STO in the following) for the purpose of obtaining magnetic properties in the PMF-STO structure. The measured spectra clearly showed a large main peak and multiple smaller peaks on the high frequency side. A Lorentzian fit on the main peak yielded Gilbert damping factor of 0.0041. The observed peaks moved in proportion to the out-of-plane bias field. From the slope of the main peak frequency as a function of the bias field, Lande g factor was estimated to be about 2.13. The mode intervals showed a clear dependence on the diameter of the PMF-STOs, i.e., intervals are larger for a smaller diameter. These results suggest that the observed peaks should correspond to eigenmodes of lateral spin wave resonance in the perpendicularly magnetized free layer.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2019

Simulation of the Interaction of a Magnetic Resonance Force Microscope Probe with a Ferromagnetic Sample

We propose an algorithm and present results of micromagnetic simulation of the resonant response of a probe pickup (cantilever) of a magnetic resonance force microscope. Simulation of induced oscillations of sample magnetization makes it possible to calculate the varying component of the force exerted on the probe by the sample and to construct spectra in the form of dependences of the amplitude of oscillations of the cantilever on the external magnetic field strength. Simulation of time dependences of all magnetization field components makes it possible to analyze the spatial distributions of spin-wave resonances of samples. For test objects in the form of rectangular permalloy microstrips, good agreement between model and experimental spectra is achieved.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2015

Angular dependent study on ferromagnetic resonance and spin excitations by spin rectification

We report angular dependent spin rectification spectra which are applied to studying spin excitations in single permalloy stripe. Based on planar Hall effect, those spin excitations generate special resonant dc Hall voltages, which have been characterized as functions of the amplitude and direction of applied magnetic field. Through high angular resolution 2D mappings, the evolutions of different spin excitation can be directly presented, and the dynamic magnetic parameters such as the gyromagnetic ratio, effective exchange field, as well as the quantized numbers of standing spin waves can be accurately determined through fitting the angular evolution of each resonance.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2018

Magnonic Floquet Hofstadter butterfly

We introduce the magnonic Floquet Hofstadter butterfly in the two-dimensional (2D) insulating honeycomb ferromagnet using a combination of spin wave theory and quantum field theory. We show that hopping magnetic dipole moment (i.e. magnon quasiparticles) in the 2D insulating honeycomb ferromagnet accumulates the Aharonov–Casher phase when irradiated by an oscillating space- and time-dependent electric field. We study two different cases. In the first case, we consider the effects of only space-dependent electric field. In this case, we realize the magnonic Hofstadter spectrum with similar fractal structure as graphene subject to a perpendicular magnetic field, but with no spin degeneracy due to broken time-reversal symmetry by the ferromagnetic order. In addition, the magnonic Dirac points and Landau levels occur at finite energy as expected in a bosonic system. Remarkably, this discrepancy does not affect the topological invariant of the system. Consequently, the magnonic Chern number assumes odd values and the magnon Hall conductance gets quantized by odd integers. In the second case, we study the effects of both space- and time-dependent electric field. In this case, the theoretical framework is studied by the Floquet formalism. We show that the magnonic Floquet Hofstadter spectrum emerges entirely from the oscillating space- and time-dependent electric field, which is in stark contrast to electronic Floquet Hofstadter spectrum, where irradiation by circularly polarized light and a perpendicular magnetic field are applied independently. We study the deformation of the fractal structure at different laser frequencies and amplitudes, and analyze the topological phase transitions associated with gap openings in the magnonic Floquet Hofstadter butterfly.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2015

Preparing magnetic yttrium iron garnet nanodot arrays by ultrathin anodic alumina template on silicon substrate

Ultrahigh density periodically ordered magnetic yttrium iron garnet (Y{sub 3}Fe{sub 5}O{sub 12}, YIG) nanodot arrays have been prepared by pulsed laser deposition through an ultrathin alumina mask (UTAM). UTAM having periodically ordered circularly shaped holes with 350 nm in diameter, 450 nm in inter-pore distance, and 700 nm in height has been prepared on silicon substrate. Furthermore, the microstructure and magnetic properties of YIG nanodot arrays have been characterized. Nanodot arrays with a sharp distribution in diameter centered at 340 nm with standard deviation of 10 nm have been fabricated. Moreover, typical hysteresis loops and ferromagnetic resonance spectra in in-plane and out-of-plane revealed that this unique structure greatly influences the magnetics properties of YIG. First, coercivity of YIG nanodot arrays in in-plane was increased about from 15 Oe of YIG films to 500 Oe. Then, the degree of uniformity about nanodot height decided that two or more resonance peaks in out-of-plane were detected in the spectra. The peak-to-peak linewidth values were about 94 Oe and 40 Oe in the parallel and perpendicular directions, respectively, which indicated that the values were larger by the two-magnon scattering. Consequently, this pattering method creates opportunities for studying physics in oxide nanomagnets and may be applied in spin-wave devices.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2024

Magnon interactions in the quantum paramagnetic phase of CoNb 2 O 6

In this work, we study effects of magnon interactions in the excitation spectrum of CoNb 2 O 6 in the quantum paramagnetic phase in transverse field, where the 1/S spin-wave theory exhibits unphysical divergences at the critical field. We propose a self-consistent Hartree-Fock approach that eliminates such unphysical singularities while preserving the integrity of the singular threshold phenomena of magnon decay and spectrum renormalization that are present in both theory and experiment. With the microscopic parameters adopted from previous studies, this method yields a close quantitative agreement with the available experimental data for CoNb 2 O 6 in the relevant regime. Furthermore, insights into the general structure of the spin-anisotropic model of CoNb 2 O 6 and related zigzag chain materials are also provided and a discussion of the effects of additional longitudinal field on the spectrum is given.

1-dimensional spin chains↗