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At least 523 records · Page 29

Optimizing conformance control for gas injection EOR in unconventional reservoirs

Field observations have shown that interference between wells caused by connected fractures commonly exists in unconventional reservoirs. The well interference effect and conformance issues could lead to minimal enhanced oil recovery response (EOR) in actual operations if they are not properly controlled. A series of data analysis, modeling, and experimental activities were performed in this study to investigate the gas EOR strategies in the Bakken Formation. Employing the embedded discrete fracture modeling technology, a multiple-well, multiple-fracture model was developed to capture the well interference and conformance issues in the Bakken. The model made it possible to investigate the complex flow behavior between wells in the EOR (huff ‘n’ puff) processes. Alternative EOR and conformance control strategies using water and surfactant injections were studied to improve oil production performance based on experimental observations. Results showed that water injection could be used for conformance control in the Bakken because of its relatively low mobility compared to gas; however, water could also block oil flow around the conformance control wells because of the high interfacial tension between oil and water. Adding surfactant to the injection water is more effective for improving gas EOR performance since surfactant reduces the oil–water interfacial tension and contact angle effectively. Up to 9.4% more oil could be produced from the huff ‘n’ puff wells in 2 years of EOR operations when rich gas was injected at only 3 MMscf/d with 6000 psi of surfactant injection in the offset wells for conformance control.

42 ENGINEERING↗

Dynamic simulation of CO 2 -injection-induced fault rupture with slip-rate dependent friction coefficient

It is known that poro-elastic stress and effective stress reduction associated with deep underground fluid injection can potentially trigger shear rupture along pre-existing faults. We modeled an idealized CO 2 injection scenario, to assess the effects on faults in the first phase of a generic CO 2 aquifer storage operation. We used coupled multiphase fluid flow and geomechanical numerical modeling to evaluate the stress and pressure perturbations induced by fluid injection and the response of a nearby normal fault. Slip-rate dependent friction and inertial effects have been taken into account during rupture. Contact elements have been used to take into account the frictional behavior of the rupture plane. We investigated different scenarios of injection rate to induce rupture on the fault, employing various fault rheologies. Published laboratory data on CO 2 -saturated intact and crushed rock samples, representative of a potential target aquifer, sealing formation and fault gouge, have been used to define a scenario where different fault rheologies apply at different depths. Nucleation of fault rupture takes place at the bottom of the reservoir, in agreement with analytical poro-elastic stress calculations, depending on injection-induced reservoir inflation and the tectonic stress scenario. For the stress state considered here, the first triggered rupture always produces the largest rupture length and slip magnitude, both of which correlate with the fault rheology. Velocity weakening produces larger ruptures and generates larger magnitude seismic events. Heterogeneous faults have been considered including velocity-weakening or velocity strengthening sections inside and below the aquifer, with the upper sections being velocity-neutral. Nucleation of rupture in a velocity-strengthening section results in a limited rupture extension, both in terms of maximum slip and rupture length. For a heterogeneous fault with nucleation in a velocity-weakening section, the rupture may propagate into the overlying velocity-neutral section, if the extent of velocity-weakening and associated friction drop are large enough.

58 GEOSCIENCES↗

Fines migration during CO 2 injection: Experimental results interpreted using surface forces

The South West Hub project is one of the Australian Flagship Carbon Capture and Storage projects located in the south-west of Western Australia. To evaluate the injectivity potential during the forthcoming full-scale CO 2 injection, we conducted three core-flooding experiments using reservoir core plugs from the well Harvey-1. We aimed to investigate in this paper whether the injection of CO 2 leads to fines migration and permeability reduction due to the relatively high kaolinite content (up to 13%) in the injection interval of the target formation (i.e. the Wonnerup Member of the Lesueur Formation). We imaged the core samples before flooding to verify the presence of kaolinite at the pore-scale using scanning electron microscopy (SEM). We also examined the pore network of the core plugs before and after the core-flooding experiments using Nuclear Magnetic Resonance (NMR). Moreover, to gain a better understanding of any kaolinite fines migration, we delineated surface force using two models based on Derjaguin-Landau-Verwey-Overbeek (denoted by DLVO) theory coupled hydrodynamic force: (1) sphere/flat model representing interaction between kaolinite/quartz, and (2) flat/flat model representing interaction between kaolinite/kaolinite. Our core-flooding experimental results showed that CO 2 /brine injection triggered moderate to significant reduction in the permeability of the core samples with a negligible porosity change. NMR measurements supported the core-flooding results, suggesting that the relatively large pores disappeared in favour of a higher proportion of the medium to small pores after flooding. The DLVO calculations showed that some kaolinite particles probably lifted off and detached from neighbouring kaolinite particles rather than quartz grains. Moreover, the modelling results showed that the kaolinite fines migration would not occur under normal reservoir multiphase flow conditions. This is not because of the low hydrodynamic force. It is rather because the geometries of the particles dominate their interplay. Finally and overall, both of the experimental and analytical modelling results point to the fines migration to be the most likely cause of the permeability impairment observed during core-flooding experiments.

58 GEOSCIENCES↗

Inference of Rock Flow and Mechanical Properties from Injection-Induced Microseismic Events During Geologic CO 2 Storage

Monitoring microseismic activities during CO 2 injection into geologic formations is important for ensuring the safety of the storage operations. The resulting data provide insight into the response of the storage formation to CO 2 injection and can be used to infer the underlying rock flow and mechanical properties. In this paper, assimilation of microseismic data is performed for dynamic characterization of the storage formation by using a stochastic simulation model to forecast the microseismic response of a geologic formation during CO 2 injection. Two modeling approaches are adopted to predict the space-time distribution of the injection-induced microseismicity. The first model is based on pore pressure relaxation assumption, while the second model uses coupled flow and geomechanics simulation to establish the complex physical relation between the storage formation properties and the corresponding microseismic responses during CO 2 injection. The stochastic predictive models in each case are used in ensemble data assimilation frameworks to estimate rock properties from the observed microseismic data. Two data assimilation methods are considered: (i) a new ensemble-based stochastic point process filter (EnPPF) that can directly integrate discrete microseismic events, and (ii) a variant of ensemble smoother, known as the ensemble smoother with multiple data assimilation (ES-MDA), which requires continuous representation of microseismic events for assimilation. The two methods are successfully applied to a geologically realistic model of the Farnsworth Field in Texas, with complex geologic flow units and interacting fault systems.

42 ENGINEERING↗

Seismic monitoring of a small CO 2 injection using a multi-well DAS array: Operations and initial results of Stage 3 of the CO 2 CRC Otway project

Active time-lapse seismic is widely employed for monitoring CO 2 geosequestration due to its ability to track the distribution of fluids in space and time. However, standard 4D seismic monitoring suffers from several challenges, including high cost, disruption to other land uses, and, consequently, relatively large intervals between monitor surveys. Some of these challenges can be mitigated using permanently installed sources and receivers. Such an approach was tested at the CO 2 CRC Otway site by continuous offset VSP monitoring of 15,000 t of supercritical CO 2 injected into an aquifer 1,500 m deep with nine permanent seismic sources (surface orbital vibrators or SOVs) and five downhole fibre-optic receivers. This continuous monitoring is complemented by multi-well 4D VSP using a mobile vibroseis source and the same DAS receivers, which included one baseline and two monitor surveys after injection of 4,000 and 12,000 t of CO 2 . The continuous DAS-SOV monitoring detected an abrupt increase of travel times below the injection interval on the second day of injection (after injection of 300 t of CO 2 ) and tracked the growth of the areal CO 2 plume by mapping changes of reflection amplitudes. The plume is also detected by time-lapse changes of reflection amplitudes in multi-well 4D VSPs. The plume images obtained from continuous offset VSP and 4D VSP are broadly consistent with each other but with some differences due to differences in illumination, lateral variations of velocities and seismic anisotropy. Furthermore, these differences also serve as a measure of uncertainty of 4D VSP images.

4D VSP↗

Prostate Hypofractionated Radiation Therapy: Injection of Hyaluronic Acid to Better Preserve The Rectal Wall

Purpose: The aim of this study was to evaluate the contribution of an injection of hyaluronic acid (HA) between the rectum and the prostate for reducing the dose to the rectal wall in a hypofractionated irradiation for prostate cancer. Methods and Materials: In a phase 2 study, 10 cc of HA was injected between the rectum and prostate. For 16 patients, the same intensity modulated radiation therapy plan (62 Gy in 20 fractions) was optimized on 2 computed tomography scans: CT1 (before injection) and CT2 (after injection). Rectal parameters were compared: dose to 2.5 cc (D2.5), 5 cc (D5), 10 cc (D10), 15 cc (D15), and 20 cc (D20) of rectal wall and volume of rectum covered by the 90% isodose line (V90), 80% (V80), 70% (V70), 60% (V60), and 50% (V50). Results: The mean V90, V80, V70, V60, and V50 values were reduced by 73.8% (P<.0001), 55.7% (P=.0003), 43.0% (P=.007), 34% (P=.002), and 25% (P=.036), respectively. The average values of D2.5, D5, D10, D15, and D20 were reduced by 8.5 Gy (P<.0001), 12.3 Gy (P<.0001), 8.4 Gy (P=.005), 3.7 Gy (P=.026), and 1.2 Gy (P=.25), respectively. Conclusions: The injection of HA significantly limited radiation doses to the rectal wall.

62 RADIOLOGY AND NUCLEAR MEDICINE↗

Fully coupled wellbore-reservoir simulation of supercritical CO 2 injection from fossil fuel power plant for heat mining from geothermal reservoirs

The concept of injecting supercritical CO 2 (sCO 2 ) into a geothermal reservoir was computationally investigated to assess its performance in terms of the benefit of using CO 2 captured from fossil power plants for geothermal heat mining. A coupled wellbore-reservoir system was simulated considering the flow of pure sCO 2 in an injection well, the interaction of sCO 2 and water in a permeable reservoir, and the flow of the two-phase mixture of sCO 2 and water in a production well. Results of simulations indicate that this CO 2 application is capable of providing a good source of renewable energy. It was found that for a reservoir with a 0.08 km 3 volume, about 8-9 MW th could be extracted in a steady state fashion for a 30-year lifetime operation. This is approximately equivalent to 100 MW th /km 3 . A sensitivity analysis provided information on the impact of certain parameters on the performance of the integrated system. The injection flowrate, the distance between the production and injection wellbores and the penetrating depth of the production wellbore into the reservoir have a first order impact on the pressure management of the reservoir. Additionally, CO 2 injection temperature has a large effect on the thermosiphon characteristics of the system.

20 FOSSIL-FUELED POWER PLANTS↗

Dosimetric comparison of rectal-sparing capabilities of rectal balloon vs injectable spacer gel in stereotactic body radiation therapy for prostate cancer: lessons learned from prospective trials

This study aimed to compare the rectal-sparing capabilities of rectal balloons vs absorbable injectable spacer gel in stereotactic body radiation therapy (SBRT) for prostate cancer. Patient samples included in this analysis were obtained from 2 multi-institutional prospective trials of SBRT for prostate cancer using a rectal balloon (n = 36 patients) and injectable spacer gel (n = 36). Treatment prescription dose was 45 Gy in 5 fractions in 42 patients; for equal comparison, the remaining 30 patients were rescaled to 45 Gy from 47.5 Gy prescription (n = 6) and 50 Gy prescription (n = 24). The median prostate volumes and body mass index in the 2 patient samples were not statistically significantly different (p = 0.67 and 0.45, respectively), supporting anatomic similarity between cohorts. The injectable spacer gel achieved dosimetric superiority over the rectal balloon with respect to the maximum dose to the rectum (42.3 vs 46.2 Gy, p vs 35.1 Gy, p Gy ), V40{sub Gy}, and V30{sub Gy} (0.3 vs 1.7 cc, 1 vs 5.4 cc, and 4.1 vs 9.6 cc, respectively; p Gy of the rectum or the dose to 50% of the rectal circumference (p = 0.29 and 0.06, respectively). The V18.3{sub Gy} of the bladder was significantly larger with the rectal balloon (19.9 vs 14.5 cc, p = 0.003). In this analysis of patients enrolled on 2 consecutive multi-institutional prospective trials of SBRT for prostate cancer, the injectable spacer gel outperformed the rectal balloon in the majority of the examined and relevant dosimetric rectal-sparing parameters. The rectal balloon did not outperform the injectable spacer gel in any measured rectal dose parameter.

61 RADIATION PROTECTION AND DOSIMETRY↗

Integrated simulation of vertical fracture propagation induced by water injection and its borehole electromagnetic responses in shale gas systems

We analyze fracture propagation induced by hydraulic fracturing with water injection and examine their detectability with crosswell electromagnetic (EM) geophysical methods. For rigorous 3D coupled flow-geomechanical modeling, we employ a numerical method that can model failure by tensile and shear stresses, dynamic nonlinear permeability, dual continuum approach, and thermo-poro-mechanical effects. From numerical simulation, we find that the fracture propagation is not the same as propagation of the water front, because fracturing is governed by geomechanics whereas water saturation is determined by multiphase flow. At early times, the water front is almost identical to the fracture tip, suggesting that the fracture is mostly filled with the injected water. However, at late times, movement of the water front is retarded compared to fracture propagation, yielding a significant gap between the water front and the fracture top, filled with reservoir gas. During fracture propagation, the coupled flow-geomechanical models are transformed via a rock-physics model into electrical conductivity models. We employ a full 3D finite-element EM geophysical simulator to evaluate the sensitivity of the crosswell EM method to fracture propagation. It is shown that anomalous distribution of electrical conductivity is closely related to the injected water saturation, but not closely related to newly created unsaturated fractures. Our numerical modeling experiments demonstrate that the crosswell EM method can be highly sensitive to electrical conductivity changes that directly indicate the migration pathways of the injected fluid. Accordingly, the EM method can serve as an effective monitoring tool for monitoring the injected fluids during hydraulic fracturing operations.

58 GEOSCIENCES↗

Reducing ultrafine particle emissions using air injection in wood-burning cookstoves

In order to address the health risks and climate impacts associated with pollution from cooking on biomass fires, researchers have focused on designing new cookstoves that improve cooking performance and reduce harmful emissions, specifically particulate matter (PM). One method for improving cooking performance and reducing emissions is using air injection to increase turbulence of unburned gases in the combustion zone. Although air injection reduces total PM mass emissions, the effect on PM size-distribution and number concentration has not been thoroughly investigated. Using two new wood-burning cookstove designs from Lawrence Berkeley National Laboratory, this research explores the effect of air injection on cooking performance, PM and gaseous emissions, and PM size distribution and number concentration. Both cookstoves were created using the Berkeley-Darfur Stove as the base platform to isolate the effects of air injection. The thermal performance, gaseous emissions, PM mass emissions, and particle concentrations (ranging from 5 nm to 10 μm in diameter) of the cookstoves were measured during multiple high-power cooking tests. Finally, the results indicate that air injection improves cookstove performance and reduces total PM mass but increases total ultrafine (less than 100 nm in diameter) PM concentration over the course of high-power cooking.

54 ENVIRONMENTAL SCIENCES↗

Coupled Flow and Deformation Modeling of Carbon Dioxide Migration in the Presence of a Caprock Fracture during Injection

Understanding the transport of carbon dioxide (CO{sub 2}) during long-term CO{sub 2} injection into a typical geologic reservoir, such as a saline aquifer, could be complicated because of changes in geochemical, hydrogeological, and hydromechanical behavior. While the caprock layer overlying the target aquifer is intended to provide a tight, impermeable seal in securing injected CO{sub 2}, the presence of geologic uncertainties, such as a caprock fracture or fault, may provide a channel for CO{sub 2} leakage. There could also be a possibility of the activation of a new or existing dormant fault or fracture, which could act as a leakage pathway. Such a leakage event during CO{sub 2} injection may lead to a different pressure and ground response over a period of time. In the present study, multiphase fluid flow simulations in porous media coupled with geomechanics were used to investigate the overburden geologic response and plume behavior during CO{sub 2} injection in the presence of a hypothetical permeable fractured zone in a caprock, existing or activated. Both single-phase and multiphase fluid flow simulations were performed. The CO{sub 2} migration through an existing fractured zone leads to changes in the fluid pressure in the overburden geologic layers and could have a significant impact on ground deformation behavior. Results of the study show that pressure signatures and displacement patterns are significantly different in the presence of a fractured zone in the caprock layer. The variation in pressure and displacement signatures because of the presence of a fractured zone in the caprock at different locations may be useful in identifying the presence of a fault/fractured zone in the caprock. The pressure signatures can also serve as a mechanism to identify the activation of leakage pathways through the caprock during CO{sub 2} injection. Pressure response and ground deformation behavior from sequestration modeling could be useful in the development of smart technologies to monitor safe CO{sub 2} storage and understand CO{sub 2} transport, with limited field instrumentation.

54 ENVIRONMENTAL SCIENCES↗

Holistic Assessment of SO 2 Injections Using CESM1(WACCM): Introduction to the Special Issue

We introduce a special issue on a holistic assessment of geoengineering via stratospheric SO 2 injection in the state-of-the-art climate model, Community Earth System Model, version 1 with the Whole Atmosphere Community Climate Model as its atmospheric component (CESM1(WACCM)). This model has numerous complexities that allow it to represent some of the most important nonlinearities associated with stratospheric SO 2 injection, including aerosol microphysical growth and stratospheric chemistry. The studies described herein represent the steps towards and first attempt in a state-of-the-art climate model to use geoengineering to meet multiple simultaneous objectives via SO 2 injection at multiple locations. First, a “matrix” of simulations was carried out to better understand the response of geoengineering to variations in latitude, altitude, and amount of sulfur dioxide injections. Subsequently, in a century long simulation, a feedback algorithm was employed to meet specific objectives and manage uncertainty, wherein the injection amount at each location was adjusted every model year. Most of the analyses contained in this special issue focus on surface climate and stratospheric changes in the matrix and century long simulations. In addition, 20 ensemble members of the feedback simulation have been carried out and provided to the community to expand the scope of analyses to low signal-to-noise ratio fields, including regional effects, impacts assessment, and extreme events. The demonstration provided by these simulations is a step toward understanding the space of achievable climate objectives via geoengineering, or, phrased differently, determining what geoengineering can do and what it cannot do.

54 ENVIRONMENTAL SCIENCES↗

Comparing surface and stratospheric impacts of geoengineering with different SO2 injection strategies

Geoengineering with stratospheric sulfate aerosols can, to some extent, be designed to achieve different climate objectives. Here we use the the state-of-the-art Community Earth System Model, version 1, with the Whole Atmosphere Community Climate Model as its atmospheric component (CESM1(WACCM)), to compare surface climate and stratospheric effects of two geoengineering strategies. In one, SO2 is injected into the tropical lower stratosphere at the equator to keep global mean temperature nearly constant under an RCP8.5 scenario, as has been commonly simulated in previous studies. In another, the Geoengineering Large Ensemble (GLENS), SO2 is injected into the lower stratosphere at four different locations (30°N/S and 15°N/S) to keep global mean temperature, the interhemispheric temperature gradient, and the equator-to-pole temperature gradient nearly unchanged. Both simulations are effective at offsetting changes in global mean temperature and the interhemispheric temperature gradient that result from increased greenhouse gases, but only GLENS offsets changes in the equator-to-pole temperature gradient. GLENS results in a more even aerosol distribution, whereas equatorial injection tends to result in an aerosol peak in the tropics. Many other aspects of surface climate changes, including precipitation and sea ice coverage, also show reduced changes in GLENS as compared to equatorial injection. Stratospheric changes, including heating, circulation, and effects on the quasi-biennial oscillation are greatly reduced in GLENS as compared to equatorial injection.

Kravitz, Benjamin S.↗

Injection Parameters That Promote Branching of Hydraulic Cracks

Fluid injection into rock formations can either produce complex branched hydraulic fractures, create simple planar fractures, or be dominated by porous diffusion. Currently, the optimum injection parameters to create branched fractures are unknown. We conducted repeatable hydraulic fracturing experiments using analog-rock samples with controlled heterogeneity to quantify the fluid parameters that promote fracture branching. A large range of injection rates and fluid viscosities were used to investigate their effects on induced fracture patterns. Paired with a simple analytical model, our results identify the threshold at which fracture transitions from an isolated planar crack to branched cracks when closed natural fractures exist. These results demonstrate that this transition can be controlled by injection rate and fluid viscosity. In relation to the field practices, the present model predicts slickwater and lower viscosity fluid injections promote fracture branching, with the Marcellus shale used as an example.

58 GEOSCIENCES↗

Coupled Hydromechanical Modeling of Induced Seismicity From CO 2 Injection in the Illinois Basin

Injection of CO 2 for geologic carbon sequestration into deep sedimentary formations involves fluid pressure increases that engage hydromechanical processes that can cause seismicity by activation of existing faults. In this work, we use a coupled multiphase fluid flow and geomechanical simulator to model spatiotemporal fluid pressure and stress changes in order to study the poroelastic effect of CO 2 injection on faults in crystalline basement rock below the injection zone. The seismicity rate along features interpreted to be basement faults is modeled using Dieterich's rate-and-state earthquake nucleation model. The methodology is applied to microseismicity detected during CO 2 injection into the Mount Simon formation during the Illinois Basin—Decatur Project. The modeling accurately captures an observed reduction in seismicity rate when the injection in the second well was into a slightly shallower zone above the base of the Mount Simon formation. Moreover, the modeling shows that it is important to consider poroelastic stress changes, in addition to fluid pressure changes for accurately modeling of the observed seismicity rate.

58 GEOSCIENCES↗

Association Between Injection and Microseismicity in Geothermal Fields With Multiple Wells: Data-Driven Modeling of Rotokawa, New Zealand, and Húsmúli, Iceland

Understanding injection-induced microseismicity in geothermal systems can provide insight into reservoir connectedness. However, fault and reservoir complexity are difficult to represent in simple analytical models, which makes it difficult to discern clear relationships from incidental associations. Here, we have used data-driven models to study how fluid injection and microseismicity are related in the Rotokawa (New Zealand) and Hellisheiði (Iceland) geothermal fields. We tested two classes of model: (a) lagged linear regression of seismicity rate as a function of well injection rates; and (b) systematic extraction of injection time series features that are then evaluated for associations with the seismicity. These models allowed us to determine which wells had the greatest correlation with microseismicity and to explain this association in a reservoir context. Finally, exploring different data types and transformations, we were unable to establish a link between rapid changes in injection rate and seismicity spikes, as suggested by some theoretical models.

15 GEOTHERMAL ENERGY↗

Leakage From Coexisting Geologic Forcing and Injection‐Induced Pressurization: A Semi‐Analytical Solution for Multilayered Aquifers With Multiple Wells

Abstract Abnormal fluid pressures (above or below hydrostatic pressure) can develop and persist in sedimentary basins. The common occurrence of abnormal pressures may cause challenges for project permitting of geological carbon sequestration (GCS), particularly in reservoirs with pre‐injection overpressure. The leaky wells that may exist in some sedimentary basins can provide flow paths between deep brine aquifers and shallower freshwater aquifers. Pre‐injection relative overpressures can cause brine leakage through leaky wells even before any injection occurs. The tendency for flow through leaky wells is coupled with the process of pressure dissipation that occurs through aquitards. Specifically, with non‐zero permeability, aquitards can dissipate pressure over large areal extents and thereby reduce leakage rates through leaky wells. This study presents development of a semi‐analytical solution for hydraulic head and brine leakage in multilayered aquifer–aquitard systems with geologic pressure forcing. The geologic forcing that causes abnormal pressures in the multilayered system can coexist with any number of injection, extraction, and leaky wells that also affect fluid pressure. The semi‐analytical model is applied to explore how leakage through leaky wells varies as functions of pressurization rate, along with aquitard and leaky well properties in an overpressured multilayered system. The results show that although injection‐induced pressures can dissipate rapidly through suitably permeable aquitards, coexisting geologic forcing may create sustained rates of brine leakage into freshwater aquifers through leaky wells. In GCS, a very low‐permeability aquitard with high capillary entry pressure to free‐phase CO 2 is desired to serve as the caprock to prevent leakage of CO 2 from the storage reservoir. Nevertheless, the results from this study show that the brine leakage impact to shallow freshwater aquifers through leaky wells might substantially decrease with increasing aquitard permeability values, as long as small aquitard permeability and high capillary entry pressure serve to prevent CO 2 leakage.

Cihan, A.↗

Radiative Forcing From the 2014–2022 Volcanic and Wildfire Injections

Abstract Volcanic and wildfire events between 2014 and 2022 injected ∼3.2 Tg of sulfur dioxide and 0.8 Tg of smoke aerosols into the stratosphere. With injections at higher altitudes and lower latitudes, the simulated stratospheric lifetime of the 2014–2022 injections is about 50% longer than the volcanic 2005–2013 injections. The simulated global mean effective radiative forcing (ERF) of 2014–2022 is −0.18 W m −2 , ∼40% of the ERF of the period of 1991–1999 with a large‐magnitude volcanic eruption (Pinatubo). Our climate model suggests that the stratospheric smoke aerosols generate ∼60% more negative ERF than volcanic sulfate per unit aerosol optical depth. Studies that fail to account for the different radiative properties of wildfire smoke relative to volcanic sulfate will likely underestimate the negative stratospheric forcings. Our analysis suggests that stratospheric injections offset 20% of the increase in global mean surface temperature between 2014–2022 and 1999–2002.

54 ENVIRONMENTAL SCIENCES↗