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At least 523 records · Page 29

LEOMAC: A Future 'Global Atmospheric Composition Mission' (CACM) Concept

Resolution of important outstanding questions in air quality, climate change and ozone layer stability demands global observations of multiple chemical species with high horizontal and vertical resolution from the boundary layer to the stratopause. We present a mission concept that delivers the needed atmospheric composition observations, along with cloud ice and water vapor data needed for improvements in climate and weather forecasting models. The mission comprises ultraviolet and infrared nadir and microwave limb viewing instruments observing wide swaths each orbit. We review the scientific goals of the mission and the measurement capabilities this concept will deliver. We describe how precessing orbits offer significant improvements in temporal resolution and diurnal coverage compared to sun-synchronous orbits. Such improvements are needed to quantify the impact of critical 'fast processes' such as deep convection on the composition and radiative properties of the upper troposphere, a region where water vapor and ozone are strong but poorly understood greenhouse gases. This concept can serve as the 'Global Atmospheric Composition Mission' (GACM) recently recommended by the National Academy of Sciences decadal survey as one of 17 priority earth science missions for the coming decade.

chemistry↗

Land and Atmosphere Near-Real-Time Capability for Earth Observing System

The past decade has seen a rapid increase in availability and usage of near-real-time data from satellite sensors. The EOSDIS (Earth Observing System Data and Information System) was not originally designed to provide data with sufficiently low latency to satisfy the requirements for near-real-time users. The EOS (Earth Observing System) instruments aboard the Terra, Aqua and Aura satellites make global measurements daily, which are processed into higher-level 'standard' products within 8-40 hours of observation and then made available to users, primarily earth science researchers. However, applications users, operational agencies, and even researchers desire EOS products in near-real-time to support research and applications, including numerical weather and climate prediction and forecasting, monitoring of natural hazards, ecological/invasive species, agriculture, air quality, disaster relief and homeland security. These users often need data much sooner than routine science processing allows, usually within 3 hours, and are willing to trade science product quality for timely access. While Direct Broadcast provides more timely access to data, it does not provide global coverage. In 2002, a joint initiative between NASA (National Aeronautics and Space Administration), NOAA (National Oceanic and Atmospheric Administration), and the DOD (Department of Defense) was undertaken to provide data from EOS instruments in near-real-time. The NRTPE (Near Real Time Processing Effort) provided products within 3 hours of observation on a best-effort basis. As the popularity of these near-real-time products and applications grew, multiple near-real-time systems began to spring up such as the Rapid Response System. In recognizing the dependence of customers on this data and the need for highly reliable and timely data access, NASA's Earth Science Division sponsored the Earth Science Data and Information System Project (ESDIS)-led development of a new near-real-time system called LANCE (Land, Atmosphere Near-Real-Time Capability for EOS) in 2009. LANCE consists of special processing elements, co-located with selected EOSDIS data centers and processing facilities. A primary goal of LANCE is to bring multiple near-real-time systems under one umbrella, offering commonality in data access, quality control, and latency. LANCE now processes and distributes data from the Moderate Resolution Imaging Spectroradiometer (MODIS), Atmospheric Infrared Sounder (AIRS), Advanced Microwave Scanning Radiometer Earth Observing System (AMSR-E), Microwave Limb Sounder (MLS) and Ozone Monitoring Instrument (OMI) instruments within 3 hours of satellite observation. The Rapid Response System and the Fire Information for Resource Management System (FIRMS) capabilities will be incorporated into LANCE in 2011. LANCE maintains a central website to facilitate easy access to data and user services. LANCE products are extensively tested and compared with science products before being made available to users. Each element also plans to implement redundant network, power and server infrastructure to ensure high availability of data and services. Through the user registration system, users are informed of any data outages and when new products or services will be available for access. Building on a significant investment by NASA in developing science algorithms and products, LANCE creates products that have a demonstrated utility for applications requiring near-real-time data. From lower level data products such as calibrated geolocated radiances to higher-level products such as sea ice extent, snow cover, and cloud cover, users have integrated LANCE data into forecast models and decision support systems. The table above shows the current near-real-time product categories by instrument. The ESDIS Project continues to improve the LANCE system and use the experience gained through practice to seek adjustments to improve the quality and performance of the system. For example, anGC-compliant Web Map Service (WMS) will be added shortly that will allow users to download geo-referenced MODIS images for arbitrary bounding boxes. Further, an OGC-compliant Web Coverage Service (WCS) will be added later this year that will expedite user access to arbitrary data subsets or re-formatted products. AIRS images are now served through WMS and available in multiple formats (PNG, GeoTIFF, KMZ). NASA has established a LANCE User Working Group to steer the development of the system and create a forum for sharing ideas and experiences that are expected to further improve the LANCE capabilities. The LANCE system has proved a success by satisfying the growing needs of the applications and operational communities for land and atmosphere data in near-real-time. NASA's Earth Sciences Division was able to leverage existing science research capabilities to provide the near-real-time community with products and imagery that support monitoring of disasters in a timely manner.

Murphy, Kevin J.↗

Microphysical modeling of cirrus. 1: Comparison with 1986 FIRE IFO measurements

We have used a one-dimensional model of cirrus formation to study the development of cirrus clouds during the 1986 First ISCCP (International Satellite Cloud Climatology Project) Regional Experiment (FIRE) intensive field observations (IFO). The cirrus model includes microphysical, dynamical, and radiative processes. Sulfate aerosols, solution drops, ice crystals, and water vapor are all treated as interactive elements in the model. Ice crystal size distributions are fully resolved based on calculations of homogeneous freezing nucleation, growth by water vapor deposition, evaporation, coagulation, and vertical transport. We have focused on the cirrus observed on November 1, 1986. Vertical wind speed for the one-dimensional simulation is taken from a mesoscale model simulation for the appropriate time period. The mesoscale model simulation suggested that strong upward motions over Wyoming and subsequent horizontal transport of upper level moisture were responsible for the cirrus observed over Wisconsin on this date. We assumed that our one-dimensional model could be used to represent a vertical column moving from Wyoming to Wisconsin over a period of several hours. Ice crystal nucleation occurs in our model in the 8 to 10-km region as a result of the strong updrafts (and cooling) early in the simulation. Growth, coagulation, and sedimentation of these ice crystals result in a broad cloud region (5-10 km thick) with an optical depth of 1-2 after a few hours, in agreement with the FIRE measurements. Comparison with aircraft microphysical measurements made over Wisconsin indicates that the simulation generated reasonable ice water content, but the predicted ice number densities are too low, especially for radii less than about 50 microns. Sensitivity tests suggest that better agreement between simulated and observed microphysical properties is achieved if the nucleation rate is higher or stronger vertical mixing (perhaps associated with multidimensional motions) is present.

Jensen, Eric J.↗

Three dimensional modeling of cirrus during the 1991 FIRE IFO 2: Detailed process study

A three-dimensional model of cirrus cloud formation and evolution, including microphysical, dynamical, and radiative processes, was used to simulate cirrus observed in the FIRE Phase 2 Cirrus field program (13 Nov. - 7 Dec. 1991). Sulfate aerosols, solution drops, ice crystals, and water vapor are all treated as interactive elements in the model. Ice crystal size distributions are fully resolved based on calculations of homogeneous freezing of solution drops, growth by water vapor deposition, evaporation, aggregation, and vertical transport. Visible and infrared radiative fluxes, and radiative heating rates are calculated using the two-stream algorithm described by Toon et al. Wind velocities, diffusion coefficients, and temperatures were taken from the MAPS analyses and the MM4 mesoscale model simulations. Within the model, moisture is transported and converted to liquid or vapor by the microphysical processes. The simulated cloud bulk and microphysical properties are shown in detail for the Nov. 26 and Dec. 5 case studies. Comparisons with lidar, radar, and in situ data are used to determine how well the simulations reproduced the observed cirrus. The roles played by various processes in the model are described in detail. The potential modes of nucleation are evaluated, and the importance of small-scale variations in temperature and humidity are discussed. The importance of competing ice crystal growth mechanisms (water vapor deposition and aggregation) are evaluated based on model simulations. Finally, the importance of ice crystal shape for crystal growth and vertical transport of ice are discussed.

Jensen, Eric J.↗

Radiative effects of polar stratospheric clouds during the Airborne Antarctic Ozone Experiment and the Airborne Arctic Stratospheric Expedition

Results are presented of a study of the radiative effects of polar stratospheric clouds during the Airborne Antarctic Ozone Experiment (AAOE) and the Airborne Arctic Stratospheric Expedition (AASE) in which daily 3D Type I nitric acid trihydrate (NAT) and Type II water ice polar stratospheric clouds (PSCs) were generated in the polar regions during AAOE and the AASE aircraft missions. Mission data on particular composition and size, together with NMC-analyzed temperatures, are used. For AAOE, both Type I and Type II clouds were formed for the time period August 23 to September 17, after which only Type I clouds formed. During AASE, while Type I clouds were formed for each day between January 3 and February 10, Type II clouds formed on only two days, January 24 and 31. Mie theory and a radiative transfer model are used to compute the radiative heating rates during the mission periods, for clear and cloudy lower sky cases. Only the Type II water ice clouds have a significant radiative effect, with the Type I NATO PSCs generating a net heating or cooling of 0.1 K/d or less.

Rosenfield, Joan E.↗

A numerical study of thunderstorm electrification - Model development and case study

A numerical model was developed for examining the thunderstorm electrification process in which it is assumed that the electrification is entirely due to noninductive charge transfer between colliding ice crystals and hail. Since this ice-hail charge mechanism is very dependent on particle sizes and distributions, an explicit microphysical framework is used. To maintain simplicity, the electrification model is kinematic; thus the temperature and velocity fields are input into the electrification model. The cloud model of Taylor (1989) was used to generate the temperature and velocity fields to examine the July 19, 1981, Cooperative Convective Precipitation Experiment thundercloud. Using these fields, the electrification model produced time-dependent ice particle concentrations, radar reflectivities, charge, and vertical electric field distributions in good general agreement with those observed. The model produced a maximum electric field strength of 1.27 kV/cm, which is on the order of that needed for lightning initiation, and this maximum occurred very close to the time of the observed discharge. Thus, the ice-hail charge mechanism appears to have played an important role in the electrical development of the July 19 cloud.

Norville, K.↗

Radiometric Model and Inter-Comparison Results of the SGLI-VNR On-Board Calibration

The Second Generation Global Imager (SGLI) on Global Change Observation Mission– Climate (GCOM-C) satellite empowers surface and atmospheric measurements related to the carbon cycle and radiation budget, with two radiometers of Visible and Near Infrared Radiometer (SGLI-VNR) and Infrared Scanning Radiometer (SGLI-IRS) that perform a wide-band (380 nm–12 µm) optical observation not only with as wide as a 1150–1400 km field of view (FOV), but also with as high as 0.25–0.5 km resolution. Additionally, polarization and along-track slant view observations are quite characteristic of SGLI. It is important to calibrate radiometers to provide the sensor data records for more than 28 standard products and 23 research products including clouds, aerosols, ocean color, vegetation, snow and ice, and other applications. In this paper, the radiometric model and the first results of on-board calibrations on the SGLI-VNR, which include weekly solar and light-emitting diode (LED) calibration and monthly lunar calibration, will be described. Each calibration data was obtained with corrections, where beta angle correction and avoidance of reflection from multilayer insulation (MLI) were applied for solar calibration; LED temperature correction was performed for LED calibration; and the GIRO (GSICS (Global Space-based Inter-Calibration System) Implementation of the ROLO (RObotic Lunar Observatory) model) model was used for lunar calibration. Results show that the inter-comparison of the relative degradation amount between these three calibrations agreed to within 1% or less.

Urabe, Tomoyuki↗

Assimilation of satellite microwave observations over the rainbands of tropical cyclones

A novel Bayesian Monte Carlo integration (BMCI) technique was developed to retrieve geophysical variables from satellite microwave radiometer data in the presence of tropical cyclones. The BMCI technique includes three steps: generating a stochastic database, simulating satellite brightness temperatures using a radiative transfer model, and retrieving geophysical variables such as profiles of temperature, relative humidity, and cloud liquid and ice water content from real observations. The technique also provides uncertainty estimates for each retrieval and can output the error covariance matrix of selected parameters. The measurements from the Advanced Technology Microwave Sounder (ATMS) on board Suomi National Polar-Orbiting Partnership (Suomi NPP) and the Global Precipitation Measurement (GPM) Microwave Imager (GMI) were used as input. A new technique was developed to correct the ATMS and GMI observations for the beam-filling effect, which is due to small-scale variability of precipitation and clouds when compared with the instrument footprint and also the nonlinear relation between the brightness temperature and precipitation. In addition, the assimilation of the BMCI retrievals into the NASA GEOS model is discussed for Hurricane Maria. The results show that assimilating the BMCI retrievals can influence the dynamical features of the cyclone, including a stronger warm core, a symmetric eye, and vertically aligned wind columns. Two possible factors that may limit the impact of the BMCI retrievals include 1) the resolution of the model (about 25 km), which was too coarse to show the potential of the BMCI data in improving the representation of tropical storms in the model forecast, and 2) the data assimilation system not being able to consider vertically correlated observation errors.

Isaac Moradi↗

Absorption and scattering properties of the Martian dust in the solar wavelengths

A new wavelength-dependent model of the single-scattering properties of the Martian dust is presented. The model encompasses the solar wavelengths (0.3 to 4.3 micrometers at 0.02 micrometer resolution) and does not assume a particular mineralogical composition of the particles. We use the particle size distribution, shape, and single-scattering properties at Viking Lander wavelengths presented by Pollack et al. [1995]. We expand the wavelength range of the aerosol model by assuming that the atmospheric dust complex index of refraction is the same as that of dust particles in the bright surface geologic units. The new wavelength-dependent model is compared to observations taken by the Viking Orbiter Infrared Thermal Mapper solar channel instrument during two dust storms. The model accurately matches afternoon observations and some morning observations. Some of the early morning observations are much brighter than the model results. The increased reflectance can be ascribed to the formation of a water ice shell around the dust particles, thus creating the water ice clouds which Colburn et al. [1989], among others, have predicted.

Atmosphere/analysis↗

Microphysical fundamentals governing cirrus cloud growth: Modeling studies

For application to Global Climate Models, large scale numerical models of cirrus cloud formation and maintenance need to be refined to more reliably simulate the effects and feedbacks of high level clouds. A key aspect is how ice crystal growth is initiated in cirrus, which has started a cloud microphysical controversy between camps either believing that heterogeneous or homogeneous drop freezing is predominantly responsible for cold cirrus ice crystal nucleation. In view of convincing evidence for the existence of highly supercooled cloud droplets in the middle and upper troposphere, however, it is concluded that active ice nuclei are rather scarce at cirrus cloud altitudes, and so a new understanding of cirrus cloud formation is needed. This understanding is sought through an examination of cirrus cloud growth models.

Sassen, Kenneth↗

Ice Sheet and Ice Shelf Freshwater Forcing of the NASA GISS ModelE GCM

Recent mass loss from ice sheets and ice shelves is now persistent and prolonged enough that it impacts downstream oceanographic conditions. To demonstrate this, we use an ensemble of coupled GISS-E2.1-G (a CMIP6 model) simulations forced with historical estimates of anomalous freshwater, in addition to other climate forcings, from 1990 through 2019. In this ensemble there are detectable differences in zonal-mean sea surface temperatures (SST) and sea ice in the Southern Ocean, and in regional sea level around Antarctica and in the western North Atlantic. These impacts mostly improve the model's representation of historical changes, including reversing the forced trends in Southern Ocean surface temperature and Antarctic sea ice. The changes in SST may have implications for estimates of the SST pattern effect on climate sensitivity and for cloud feedbacks. We conclude that the changes are sufficiently large that model groups should strive to include more accurate estimates of these drivers in all-forcing historical simulations in future coupled model intercomparisons.

Ice sheet↗

Investigation on the Practicality of Developing Reduced Thermal Models

Throughout the spacecraft design and development process, detailed instrument thermal models are created to simulate their on-orbit behavior and to ensure that they do not exceed any thermal limits. These detailed models, while generating highly accurate predictions, can sometimes lead to long simulation run times, especially when integrated with a spacecraft observatory model. Therefore, reduced models containing less detail are typically produced in tandem with the detailed models so that results may be more readily available, albeit less accurate. In the current study, both reduced and detailed instrument models are integrated with their associated spacecraft bus models to examine the impact of instrument model reduction on run time and accuracy. Preexisting instrument bus thermal model pairs from several projects were used to determine trends between detailed and reduced thermal models; namely, the Mirror Optical Bench (MOB) on the Gravity and Extreme Magnetism Small Explorer (GEMS) spacecraft, Advanced Topography Laser Altimeter System (ATLAS) on the Ice, Cloud, and Elevation Satellite 2 (ICESat-2), and the Neutral Mass Spectrometer (NMS) on the Lunar Atmosphere and Dust Environment Explorer (LADEE). Hot and cold cases were run for each model to capture the behavior of the models at both thermal extremes. It was found that, though decreasing the number of nodes from a detailed to reduced model brought about a reduction in the run-time, a large time savings was not observed, nor was it a linear relationship between the percentage of nodes reduced and time saved. However, significant losses in accuracy were observed with greater model reduction. It was found that while reduced models are useful in decreasing run time, there exists a threshold of reduction where, once exceeded, the loss in accuracy outweighs the benefit from reduced model runtime.

0000↗

Contrasting aerosol effects on longwave cloud forcing in South East Asia and Amazon simulated with Community Atmosphere Model version 5.3

Aerosols modify cloud microphysical and radiative properties and thus impact the shortwave (SW) and longwave cloud forcing (LWCF). This study first reports the finding of contrasting aerosol effects on LWCF in South East Asia and Amazon in the Community Atmosphere Model version 5.3 (CAM5.3), which corresponds to the sum of LW indirect and semi-direct effects investigated in Ghan et al., (2012). A series of numerical experiments is conducted to decompose the complex aerosol effects on LWCF. Our analysis indicates that the cooling (negative aerosol effects on LWCF) in Amazon is due mainly to the aerosol effects on warm clouds and the inhibition of vertical motion by the aerosol-induced radiative cooling. In contrast, the warming (positive aerosol effects on LWCF) in South East Asia is due mainly to the aerosol effect on homogeneous freezing, thus reducing the ice particle size and prolonging the existence of ice cloud. Our results emphasize that a comprehensive analysis of integrated aerosol effects on both warm and ice clouds is necessary for better understanding the aerosol effects on LWCF.

54 ENVIRONMENTAL SCIENCES↗

Ice Cloud Formation and Dehydration in the Tropical Tropopause Layer

Stratospheric water vapor is important not only for its greenhouse forcing, but also because it plays a significant role in stratospheric chemistry. Several recent studies have focused on the potential for dehydration due to ice cloud formation in air rising slowly through the tropical tropopause layer (TTL). Holton and Gettelman showed that temperature variations associated with horizontal transport of air in the TTL can drive ice cloud formation and dehydration, and Gettelman et al. recently examined the cloud formation and dehydration along kinematic trajectories using simple assumptions about the cloud properties. In this study, a Lagrangian, one-dimensional cloud model has been used to further investigate cloud formation and dehydration as air is transported horizontally and vertically through the TTL. Time-height curtains of temperature are extracted from meteorological analyses. The model tracks the growth, advection, and sedimentation of individual cloud particles. The regional distribution of clouds simulated in the model is comparable to the subvisible cirrus distribution indicated by SAGE II. The simulated cloud properties and cloud frequencies depend strongly on the assumed supersaturation threshold for ice nucleation. The clouds typically do not dehydrate the air along trajectories down to the temperature minimum saturation mixing ratio. Rather the water vapor mixing ratio crossing the tropopause along trajectories is 10-50% larger than the saturation mixing ratio. I will also discuss the impacts of Kelvin waves and gravity waves on cloud properties and dehydration efficiency. These simulations can be used to determine whether observed lower stratospheric water vapor mixing ratios can be explained by dehydration associated with in situ TTL cloud formation alone.

Jensen, Eric↗

Can High-resolution WRF Simulations Be Used for Short-term Forecasting of Lightning?

A number of research teams have begun to make quasi-operational forecast simulations at high resolution with models such as the Weather Research and Forecast (WRF) model. These model runs have used horizontal meshes of 2-4 km grid spacing, and thus resolved convective storms explicitly. In the light of recent global satellite-based observational studies that reveal robust relationships between total lightning flash rates and integrated amounts of precipitation-size ice hydrometeors in storms, it is natural to inquire about the capabilities of these convection-resolving models in representing the ice hydrometeor fields faithfully. If they do, this might make operational short-term forecasts of lightning activity feasible. We examine high-resolution WRF simulations from several Southeastern cases for which either NLDN or LMA lightning data were available. All the WRF runs use a standard microphysics package that depicts only three ice species, cloud ice, snow and graupel. The realism of the WRF simulations is examined by comparisons with both lightning and radar observations and with additional even higher-resolution cloud-resolving model runs. Preliminary findings are encouraging in that they suggest that WRF often makes convective storms of the proper size in approximately the right location, but they also indicate that higher resolution and better hydrometeor microphysics would be helpful in improving the realism of the updraft strengths, reflectivity and ice hydrometeor fields.

Goodman, S. J.↗

Tropical Oceanic Precipitation Processes Over Warm Pool: 2D and 3D Cloud Resolving Model Simulations

Rainfall is a key link in the hydrologic cycle as well as the primary heat source for the atmosphere. The vertical distribution of convective latent-heat release modulates the large-scale circulations of the topics. Furthermore, changes in the moisture distribution at middle and upper levels of the troposphere can affect cloud distributions and cloud liquid water and ice contents. How the incoming solar and outgoing longwave radiation respond to these changes in clouds is a major factor in assessing climate change. Present large-scale weather and climate model simulate processes only crudely, reducing confidence in their predictions on both global and regional scales. One of the most promising methods to test physical parameterizations used in General Circulation Models (GCMs) and climate models is to use field observations together with Cloud Resolving Models (CRMs). The CRMs use more sophisticated and physically realistic parameterizations of cloud microphysical processes, and allow for their complex interactions with solar and infrared radiative transfer processes. The CRMs can reasonably well resolve the evolution, structure, and life cycles of individual clouds and clouds systems. The major objective of this paper is to investigate the latent heating, moisture and momentum budgets associated with several convective systems developed during the TOGA COARE IFA - westerly wind burst event (late December, 1992). The tool for this study is the Goddard Cumulus Ensemble (GCE) model which includes a 3-class ice-phase microphysics scheme.

Tao, W.-K.↗

LGM Paleoclimate Constraints Inform Cloud Parameterizations and Equilibrium Climate Sensitivity in CESM2

The Community Earth System Model version 2 (CESM2) simulates a high equilibrium climate sensitivity (ECS > 5°C) and a Last Glacial Maximum (LGM) that is substantially colder than proxy temperatures. In this study, we examine the role of cloud parameterizations in simulating the LGM cooling in CESM2. Through substituting different versions of cloud schemes in the atmosphere model, we attribute the excessive LGM cooling to the new CESM2 schemes of cloud microphysics and ice nucleation. Further exploration suggests that removing an inappropriate limiter on cloud ice number (NoNimax) and decreasing the time-step size (substepping) in cloud microphysics largely eliminate the excessive LGM cooling. NoNimax produces a more physically consistent treatment of mixed-phase clouds, which leads to an increase in cloud ice content and a weaker shortwave cloud feedback over mid-to-high latitudes and the Southern Hemisphere subtropics. Microphysical substepping further weakens the shortwave cloud feedback. Based on NoNimax and microphysical substepping, we have developed a paleoclimate-calibrated CESM2 (PaleoCalibr), which simulates well the observed twentieth century warming and spatial characteristics of key cloud and climate variables. PaleoCalibr has a lower ECS (∼4°C) and a 20% weaker aerosol-cloud interaction than CESM2. PaleoCalibr represents a physically more consistent treatment of cloud microphysics than CESM2 and is a valuable tool in climate change studies, especially when a large climate forcing is involved. Our study highlights the unique value of paleoclimate constraints in informing the cloud parameterizations and ultimately the future climate projection.

equilibrium climate sensitivity↗

The Ice Particle and Aggregate Simulator (IPAS). Part II: Analysis of a Database of Theoretical Aggregates for Microphysical Parameterization

Abstract Bulk ice-microphysical models parameterize the dynamic evolution of ice particles from advection, collection, and sedimentation through a cloud layer to the surface. Frozen hydrometeors can grow to acquire a multitude of shapes and sizes, which influence the distribution of mass within cloud systems. Aggregates, defined herein as the collection of ice particles, have a variety of formations based on initial ice particle size, shape, falling orientation, and the number of particles that collect. This work focuses on using the Ice Particle and Aggregate Simulator (IPAS) as a statistical tool to repetitively collect ice crystals of identical properties to derive bulk aggregate characteristics. A database of 9 744 000 aggregates is generated with resulting properties analyzed. After 150 single ice crystals (monomers) collect, the most extreme aggregate aspect ratio calculations asymptote toward and ϕ ca ≈ 0.50 for aggregates composed of quasi-horizontally oriented and randomly oriented monomers, respectively. The results presented are largely consistent with both a previous theoretical study and estimates derived from ground-based observations from two different geographic locations. Particle falling orientation highly influences newly formed aggregate aspect ratios from the collection of particles with extreme aspect ratios; quasi-horizontally oriented particles can produce aggregate aspect ratios an order of magnitude more extreme than randomly oriented particles but can also produce near-spherical aggregates as the number of monomers comprising the aggregate reach approximately 100. Finally, a majority of collections result in aggregates that are closer to prolate than oblate spheroids.

54 ENVIRONMENTAL SCIENCES↗