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At least 523 records · Page 29

Temperature-dependent characterization of large-area superconducting microwire array with single-photon sensitivity in the near-infrared

Superconducting nanowire single photon detectors (SNSPDs) are a leading detector technology for time-resolved single-photon counting from the ultraviolet to the near-infrared regime. The recent advancement in single-photon sensitivity in micrometer-scale superconducting wires opens up promising opportunities to develop large area SNSPDs with applications in low background dark matter detection experiments. Here, we present the first detailed temperature-dependent study of a 4-channel 1×1 mm 2 WSi superconducting microwire single photon detector (SMSPD) array, including the internal detection efficiency, dark count rate, and importantly the coincident dark counts across pixels. The detector shows saturated internal detection efficiency for photon wavelengths ranging from 635 nm to 1650 nm, time jitter of about 160 ps for 1060 nm photons, and a low dark count rate of about 10 -2 Hz. Additionally, the coincidences of dark count rate across pixels are studied for the first time in detail, where we observed an excess of correlated dark counts, which has important implications for low background dark matter experiments. The results presented is the first step towards characterizing and developing SMSPD array systems and associated background for low background dark matter detection experiments.

47 OTHER INSTRUMENTATION↗

Revealing Possible Coherence Limiting Sources in Superconducting Qubit with Advanced Electron Microscopy

Superconducting materials hold great potential for solid-state quantum computing. Their fabrication relies on established semiconductor fabrication techniques, such as thin film deposition and lithography, but the complex processing steps can result in defects at the qubits' interfaces and surfaces that can negatively impact coherence time. To improve superconducting qubit performance, it is essential to understand the structural features, at the atomic scale, that may act as sources of decoherence limiting factor in both the Josephson junction (JJ) and resonators, which are key components of superconducting qubit. This talk will present our recent studies on the microstructures in a 2D-transmon, with an emphasis on the JJ. For this research, a combination of advanced microscopy techniques, including high-resolution (S)TEM imaging, and spectroscopy (EDS and EELS) are used to identify possible coherence-limiting defects or structural features.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

The Frequency Shift and $Q$ of Disordered Superconducting RF Cavities

Niobium superconducting radio-frequency (SRF) cavities for high-energy accelerator applications have been greatly improved in terms of the quality factor $Q$ by techniques such as Nitrogen doping. However, the mechanisms leading to improvement in $Q$ are still not fully understood. Quite recently the SRF group at Fermilab measured anomalies in the frequency shift of N-doped SRF Niobium cavities near the transition temperature. Here we report our theoretical analysis of these results based on the microscopic theory of superconductivity that incorporates anisotropy of the superconducting gap and inhomogeneous disorder in the screening region of the SRF cavities. We are able to account for frequency shift anomalies very close to $T_c$ on the order of fractions of 1 kHz. Our results for the frequency shift and Q are in good agreement with the experimental data reported for all four N-doped Nb SRF cavities by Bafia et al. We also compare our theory with an earlier report on a Nb sample measured at 60 GHz. In addition, we show that the quality factor calculated theoretically has a peak of upper convexity with the largest $Q$ at intermediate levels of disorder. For strong disorder, i.e. the dirty limit, pair breaking in the presence of disorder and screening currents limits the $Q$.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Unified Picture of Superconductivity and Magnetism in CeRh 2 ⁢As 2

Here, we propose a theory for the microscopic origin of the multiple superconducting and magnetic phases observed in CeRh 2 ⁢As 2 based on the existence of Van Hove singularities near the Fermi energy. The nonsymmorphic symmetry of this material implies that these singularities are located away from high-symmetry momenta; i.e., they have so-called type-II character. This allows us to include the significant Rashba spin-orbit coupling in CeRh 2 ⁢As 2 in a parquet renormalization group approach. When Fermi-surface nesting is strong, our analysis reveals two closely competing superconducting states with opposite parities, as well as an instability toward spin-density wave states that support both of them, consistent with the phase diagram of CeRh 2 ⁢As 2 . Type-II Van Hove singularities are generic to nonsymmorphic space groups, and so our theory implies that many other compounds may support closely competing even- and odd-parity superconductivity.

Rashba coupling↗

Parameter extraction for a SPICE model of an hTron superconducting thermal switch

Efficiently simulating large circuits is crucial to the development of superconducting nanowire-based electronics. However, current simulation tools for this technology are not adapted to the scaling of circuit size and complexity. We focus on the multilayered heater-nanocryotron (hTron), a promising superconducting nanowire-based switch used in applications such as superconducting nanowire single-photon detector readout. Previously, the hTron was modeled using traditional finite-element methods, which fall short in simulating systems at a larger scale. An empirical-based method would be better adapted to this task, enhancing both simulation speed and agreement with experimental data. In this work, we perform switching current and activation delay measurements on 17 hTron devices. We then develop a method for extracting physical fitting parameters used to characterize the devices. We build a SPICE behavioral model that reproduces the static and transient device behavior using these parameters, and validate it by comparing its performance to a model developed in prior work, showing an improvement in simulation time by several orders of magnitude. Furthermore, our model provides circuit designers with a tool to help understand the hTron’s behavior during all design stages, thus enabling broader use of the hTron across various new areas of application.

Caloritronics↗

Light-induced microwave noise in superconducting microwave-optical transducers

Microwave-to-optical transducers are integral to the future of superconducting quantum computing, as they would enable scaling and long-distance communication of superconducting quantum processors through optical-fiber links. However, optically induced microwave noise poses a significant challenge in achieving quantum transduction between microwave and optical frequencies. In this work, we study light-induced microwave noise in an integrated electro-optical transducer harnessing the Pockels effect of thin-film lithium niobate. We reveal three sources of added noise with distinctive time constants ranging from sub-100 ns to milliseconds. Furthermore, our results provide insights into the mechanisms and corresponding mitigation strategies for light-induced microwave noise in superconducting microwave-optical transducers and pave the way toward realizing the ultimate goal of quantum transduction.

42 ENGINEERING↗

Signatures of enhanced superconducting properties in niobium cavities

Superconducting radio-frequency (SRF) niobium cavities are critical for modern particle accelerators, as well as for advancing superconducting quantum systems and enabling ultrasensitive searches for new physics. In this work, we report a systematic observation of an anomalous frequency dip in Nb cavities, which occurs at temperatures just below the critical temperature (𝑇𝑐 ), indicative of enhanced superconducting properties at 𝑇 ≪ 𝑇 𝑐 . The magnitude of this dip is strongly correlated with the rf surface resistance, impurity distribution near the surface, and 𝑇𝑐 . Additionally, we report measurements of the coherence peak in the ac conductivity of two Nb SRF cavities processed using distinct methods. By comparing recent theories developed to model this experimental data, we show that the frequency-dip feature, larger coherence peak height, and reduction in the temperature-dependent surface resistance with rf current occur at minimal but finite levels of disorder.

43 PARTICLE ACCELERATORS↗

Robust d x 2 - y 2 -wave superconductivity of infinite-layer nickelates

Motivated by the recent observation of superconductivity in strontium-doped NdNiO 2 , we study the superconducting instabilities in this system from various vantage points. Starting with first-principles calculations, we construct two distinct tight-binding models, a simpler single-orbital as well as a three-orbital model, both of which capture the key low-energy degrees of freedom to varying degrees of accuracy. We study superconductivity in both models using the random phase approximation. We then analyze the problem at stronger coupling, and study the dominant pairing instability in the associated t-J model limit. Finally, in all instances, the dominant pairing tendency is in the d x 2 -y 2 channel, analogous to the cuprate superconductors.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Lifetime renormalization of weakly anharmonic superconducting qubits. I. Role of number nonconserving terms

The dynamics of a weakly anharmonic superconducting qubit in a complex electromagnetic environment is generally well described by an effective multimode Kerr Hamiltonian at sufficiently weak excitation. This Hamiltonian can be embedded in a master equation with losses determined by the details of the electromagnetic environment. Recent experiments indicate, however, that when a superconducting circuit is driven with microwave signals populating the system with sufficiently high excitations, the observed relaxation rates appear to be substantially different from expectations based on the electromagnetic environment of the qubit alone. This issue is a limiting factor in the optimization of superconducting qubit readout schemes. We claim here that an effective master equation with drive-power-dependent parameters is an efficient approach to model such quantum dynamics. In this sequence of papers, we derive effective master equations, whose parameters exhibit nonlinear dependence on the excitation level of the circuit as well as the electromagnetic environment of the qubit. Further, we show that the number nonconserving terms in the qubit nonlinearity generally lead to a renormalization of dissipative parameters of the effective master equation, while the number conserving terms give rise to a renormalization of the system frequencies. Here, in Paper I, we consider the excitation-relaxation dynamics of a transmon qubit that is prepared in a certain initial state, but is not driven otherwise. A unitary transformation technique is introduced to study the renormalization of (i) qubit relaxation due to coupling to a generic bath and (ii) Purcell decay. Analytic expressions are provided for the dependence of the nonlinear dissipative terms on the details of the electromagnetic environment of the qubit. The perturbation technique based on unitary transformations developed here is generalized to the continuously driven case in Paper II.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

$\testit{d}$-wave superconductivity and Bogoliubov-Fermi surfaces in Rarita-Schwinger-Weyl semimetals

In this work, we uncover the properties of complex tensor ($\textit{d}$-wave) superconducting order in three-dimensional Rarita-Schwinger-Weyl semimetals that host pseudospin-$\frac{3}{2}$ fermions at a fourfold linear band-crossing point. Although the general theory of $\textit{d}$-wave order was originally developed for materials displaying quadratic band touching, it directly applies to the case of semimetals with linear dispersion, several candidate compounds of which have been discovered experimentally very recently. The spin-$\frac{3}{2}$ nature of the fermions allows for the formation of spin-2 Cooper pairs which may be described by a complex second-rank tensor order parameter. In the case of linear dispersion, for the chemical potential at the Fermi point and at strong coupling, the energetically preferred superconducting state is the uniaxial nematic state, which preserves time-reversal symmetry and provides a full (anisotropic) gap for quasiparticle excitations. In contrast, at a finite chemical potential, we find that the usual weak-coupling instability is toward the “cyclic state,” well known from the studies of multicomponent Bose-Einstein condensates, which breaks time-reversal symmetry maximally, has vanishing average value of angular momentum, and features 16 small Bogoliubov-Fermi surfaces. The Rarita-Schwinger-Weyl semimetals provide therefore the first example of weakly coupled, three-dimensional, isotropic $\textit{d}$-wave superconductors where the $\textit{d}$-wave superconducting phase is uniquely selected by the quartic expansion of the mean-field free energy, and is not afflicted by the accidental degeneracy first noticed by Mermin over 40 years ago. We discuss the appearance and stability of the Bogoliubov-Fermi surfaces in absence of inversion symmetry in the electronic Hamiltonian, as in the case at hand.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Theoretical investigation of superconductivity in trilayer square-planar nickelates

The discovery of superconductivity in Sr-doped NdNiO 2 is a crucial breakthrough in the long pursuit for nickel oxide materials with electronic and magnetic properties similar to those of the cuprates. NdNiO 2 is the infinite-layer member of a family of square-planar nickelates with general chemical formula R n +1 Ni n O 2 n +2 (R = La, Pr, Nd, n = 2, 3,...∞). In this Rapid Communication, we investigate superconductivity in the trilayer member of this series (R4Ni 3 O 8 ) using a combination of first-principles and $\textit{t–J}$ model calculations. R 4 Ni 3 O 8 compounds resemble cuprates more than RNiO 2 materials in that only Ni-d n 2 – y 2 bands cross the Fermi level, they exhibit a largely reduced charge transfer energy, and as a consequence superexchange interactions are significantly enhanced. In this work, we find that the superconducting instability in doped R 4 Ni 3 O 8 compounds is considerably stronger with a maximum gap about four times larger than that in Sr 0.2 Nd 0.8 NiO 2 .

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Magnetism and its coexistence with superconductivity in CaK(Fe 0.949 Ni 0.051 ) 4 As 4 : Muon spin rotation/relaxation studies

Here, the magnetic response of Ca K ( Fe 0.949 Ni 0.051 ) 4 As 4 was investigated by means of the muon spin rotation/relaxation. The long-range commensurate magnetic order sets in below the Néel temperature T N = 50.0 ( 5 ) K. The density-functional theory calculations have identified three possible muon stopping sites. The experimental data were found to be consistent with only one type of magnetic structure, namely, the long-range magnetic spin-vortex-crystal order with the hedgehog motif within the a b plane and the antiferromagnetic stacking along the c direction. The value of the ordered magnetic moment at T ≈ 3 K was estimated to be m Fe = 0.38 ( 11 ) μ B ( μ B is the Bohr magneton). A microscopic coexistence of magnetic and superconducting phases accompanied by a reduction of the magnetic order parameter below the superconducting transition temperature T c ≃ 9 K is observed. Comparison with 11, 122, and 1144 families of Fe-based pnictides points to existence of correlation between the reduction of the magnetic order parameter at T → 0 and the ratio of the transition temperatures T c / T N . Such correlations were found to be described by Machida's model for coexistence of itinerant spin-density-wave magnetism and superconductivity [K. Machida, J. Phys. Soc. Jpn. 50 , 2195 (1981) ; S. L. Bud'ko et al. , Phys. Rev. B 98 , 144520 (2018) ].

36 MATERIALS SCIENCE↗

Spin magnetometry as a probe of stripe superconductivity in twisted bilayer graphene

The discovery of alternating superconducting and insulating ground states in magic angle graphene has suggested an intriguing analogy with cuprate high-T c materials. In this paper we argue that the network states of small angle twisted bilayer graphene (TBG) afford a further perspective on the cuprates by emulating their stripe-ordered phases, as in La 1.875 Ba 0.125 CuO 4 . We show that the spin and valley quantum numbers of stripes in TBG graphene fractionalize, developing characteristic signatures in the tunneling density of states and the magnetic noise spectrum of impurity spins. By examining the coupling between the charge rivers we determine the superconducting transition temperature. Our study suggests that twisted bilayer graphene can be used for a controlled emulation of stripe superconductivity and quantum sensing experiments of emergent anyonic excitations.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Topological and nematic superconductivity mediated by ferro-SU(4) fluctuations in twisted bilayer graphene

We propose an SU(4) spin-valley-fermion model to investigate the superconducting instabilities of twisted bilayer graphene (TBG). In this approach, bosonic fluctuations associated with an emergent SU(4) symmetry, corresponding to combined rotations in valley and spin spaces, couple to the low-energy fermions that comprise the flat bands. These fluctuations are peaked at zero wave vector, reflecting the “ferromagnetic-like” SU(4) ground state recently found in strong-coupling solutions of microscopic models for TBG. Focusing on electronic states related to symmetry-imposed points of the Fermi surface, dubbed here “valley hot-spots” and “van Hove hot-spots,” we find that the coupling to the itinerant electrons partially lifts the huge degeneracy of the ferro-SU(4) ground state manifold, favoring intervalley order, spin-valley coupled order, ferromagnetic order, spin-current order, and valley-polarized order, depending on details of the band structure. Here, these fluctuations, in turn, promote attractive pairing interactions in a variety of closely competing channels, including a nodeless f-wave state, a nodal i-wave state, and topological d+id and p+ip states with unusual Chern numbers 2 and 4, respectively. Nematic superconductivity, although not realized as a primary instability of the system, appears as a consequence of the near-degeneracy of superconducting order parameters that transform as one-dimensional and two-dimensional irreducible representations of the point group D 6 .

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Spectral properties and enhanced superconductivity in renormalized Migdal-Eliashberg theory

Migdal-Eliashberg theory describes the properties of the normal and superconducting states of electron-phonon-mediated superconductors based on a perturbative treatment of the electron-phonon interactions. It is necessary to include both electron and phonon self-energies self-consistently in Migdal-Eliashberg theory in order to match numerically exact results from determinantal quantum Monte Carlo in the adiabatic limit. Here in this work we provide a method to obtain the real-axis solutions of the Migdal-Eliashberg equations with electron and phonon self-energies calculated self-consistently. Our method avoids the typical challenge of computing cumbersome singular integrals on the real axis and is numerically stable and exhibits fast convergence. Analyzing the resulting real-frequency spectra and self-energies of the two-dimensional Holstein model, we find that self-consistently including the lowest-order correction to the phonon self-energy significantly affects the solution of the Migdal-Eliashberg equations. The calculation captures the broadness of the spectral function, renormalization of the phonon dispersion, enhanced effective electron-phonon coupling strength, minimal increase in the electron effective mass, and the enhancement of superconductivity which manifests as a superconducting ground state despite strong competition with charge-density-wave order. We discuss surprising differences in two common definitions of the electron-phonon coupling strength derived from the electron mass and the density of states, quantities which are accessible through experiments such as angle-resolved photoemission spectroscopy and electron tunneling. An approximate upper bound on 2Δ/T c for conventional superconductors mediated by retarded electron-phonon interactions is proposed.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Observation of topological Dirac fermions and surface states in superconducting BaSn3

The interplay between topological electronic structure and superconductivity has attracted tremendous research interests recently as they could induce topological superconductivity (TSCs) which may be used to realize topological qubits for quantum computation. Among various TSC candidates, superconducting BaSn 3 (T c ~ 4.4K) has been predicted to be a topological Dirac semimetal (TDS) hosting two pairs of Dirac points along the Γ-A direction. Here, by combining the use of angle-resolved photoemission spectroscopy and ab initio calculations, we identified the predicted topological Dirac fermions and confirmed the TDS nature of the compound. In addition, we observed surface states connecting the Dirac points. Our observations demonstrate BaSn 3 as a superconductor with nontrivial topological electronic structures.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

First-principles study of superconductivity in α and β gallium

Elemental gallium can exist in several phases under ambient pressure. The stable α phase has a superconducting transition temperature, T c , of 0.9 K. By contrast, the T c of the metastable β phase is around 6 K. To understand the significant improvement in T c in the β phase, we first calculate the electronic structure, phonon dispersion, and the electron-phonon coupling of gallium in the α and β phases. Next, we solve the Eliashberg equations to obtain the superconducting gaps and the transition temperatures. Additionally, using these results, we relate the increased T c in the β phase to structural differences between the phases that affect the electronic and phonon properties. The structure motif of the α phase is Ga 2 dimers, which form strong covalent bonds leading to bonding and antibonding states that reduce the density of states at the Fermi level. The β-Ga structure consists of arrays of Ga chains that favor strong coupling between the lattice vibrations and the electronic states near the Fermi level. The increased density of states and strong coupling to the phonons for the β-Ga chains compared to the αGa 2 dimers enhance superconductivity in the β-Ga phase.

36 MATERIALS SCIENCE↗

Superconductivity of incoherent electrons in the Yukawa Sachdev-Ye-Kitaev model

We study a model of N fermions in a quantum dot, coupled to M bosons by a disorder-induced complex Yukawa coupling [Yukawa Sachdev-Ye-Kitaev (SYK) model], in order to explore the interplay between non-Fermi liquid and superconductivity in a strongly coupled, (quantum-)critical environment. We analyze the phase diagram of the model for an arbitrary complex interaction and arbitrary ratio of N/M, with special focus on the two regimes of non-Fermi-liquid behavior: an SYK-like behavior with a power-law frequency dependence of the fermionic self-energy and an impuritylike behavior with frequency independent self-energy. We show that the crossover between the two can be reached by varying either the strength of the fermion-boson coupling or the ratio M/N. We next argue that in both regimes the system is unstable to superconductivity if the strength of time-reversal-symmetry-breaking disorder is below a certain threshold. We show how the corresponding onset temperatures vary between the two regimes. We argue that the superconducting state is highly unconventional with an infinite set of minima of the condensation energy at T = 0, corresponding to topologically different gap functions. We discuss in detail similarities and differences between this model and the model of dispersion-full fermions tuned to a metallic quantum-critical point, with an effective singular dynamical interaction V(Ω) ∝ 1/|Ω| γ (the γ model).

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗