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At least 523 records · Page 29
All sourcesNASA NTRSDOE OSTI
DOE OSTI2022

Thermal Neutron Scattering Cross Sections for Graphitic Amorphous Carbon

Carbon materials are commonly found in both nuclear reactors and experimental systems. Various carbon structures occur in nuclear applications ranging from crystalline and nuclear graphite to the amorphous carbon seen in next-generation advanced reactor designs. Amorphous carbon is based on a randomized graphite-like structure and offers the unique ability to disperse impurities throughout the bulk composition. A graphite-like amorphous carbon system was modeled using the classical molecular dynamics (MD) code LAMMPS (Large-scale Atomic/Molecular Massively Parallel Simulator). An improved version of the temperature-dependent Adaptive Intermolecular Reactive Empirical Bond Order (AIREBO) potential was used to model the carbon-carbon atomic interactions for the temperature at 300 K along with densities 1.60, 1.70, 1.85, and 2.23 g/cm 3 . From the normalized velocity autocorrelation function (VACF), the phonon density of state (DOS) was then calculated as the Fourier transform of the normalized VACF. This DOS was then used as the primary input for the evaluation of the thermal scattering law (TSL, i.e. S(α,β)) and associated neutron thermal scattering cross sections. The TSL was analyzed using the Full Law Analysis Scattering System Hub (FLASSH). The amorphous structure results in shifts of the phonon DOS to lower energy modes than typically displayed for ideal crystalline graphite. This impact on the DOS is directly reflected in the TSL. Furthermore, the typical features and the optical graphitic peak at 0.25 eV for the ideal graphite DOS disappear for graphite-like amorphous carbon, which shows good agreement with the expected structure.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2023

Searching for resonance states in Ne 22 ( p , γ ) Na 23

Globular clusters show strong correlations between different elements, such as the well-known sodium-oxygen anticorrelation. One of the main sources of uncertainty in this anticorrelation is the 22 Ne(p,γ) 23 Na reaction rate, due to the possible influence of an unobserved resonance state at E x = 8862 keV (E r,c.m. =68 keV). The influence of two higher-lying resonance states at E x = 8894 and 9000 keV has already been ruled out by direct 22 Ne(p,γ) 23 Na measurements. To study excited states in 23 Na above the proton threshold to determine if the unconfirmed resonance states in 23 Na exist. The non-selective proton inelastic scattering reaction at low energies was used to search for excited states in 23 Na above the proton threshold. Protons scattered from various targets were momentum-analysed in the Q3D magnetic spectrograph at the Maier-Leibnitz Laboratorium, Munich, Germany. The resonance states previously reported at E x = 8862, 8894 and 9000 keV in other experiments were not observed in the present experiment at any angle. This result, combined with other non-observations of these resonance states in most other experiments, results in a strong presumption against the existence of these resonance states. Here, the previously reported resonance states at E x = 8862, 8894 and 9000 keV are unlikely to exist and should be omitted from future evaluations of the 22 Ne(p,γ) 23 Na reaction rates. Indirect studies using low-energy proton inelastic scattering are a simple and yet exceptionally powerful tool in helping to constrain astrophysical reaction rates by providing non-selective information of the excited states of nuclei.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Re-evaluation of the TSL for Yttrium Hydride

Yttrium hydride (YH x ) is of interest as a high-temperature moderator material in advanced nuclear reactor systems because of its superior ability to retain hydrogen at elevated temperatures. Thermal neutron scattering laws (TSL) for hydrogen bound in yttrium hydride (H-YH 2 ) and yttrium bound in yttrium hydride (Y-YH 2 ) were previously evaluated by Naval Nuclear Laboratory using the ab initio approach and released in ENDF/B-VIII.0. In that work, density functional theory, incorporating the generalized gradient approximation (GGA) for the exchange-correlation energy, was used to simulate the face-centered cubic structure of YH 2 and calculate the interatomic Hellmann-Feynman forces for a 2×2×2 supercell containing 96 atoms. Lattice dynamics calculations using PHONON were used to determine the phonon density of states. The calculated phonon density of states for H and Y in YH 2 were then used to prepare H-YH 2 and Y-YH 2 TSL evaluations, in the incoherent approximation, using the LEAPR module of NJOY. In addition, elastic scattering was assumed to be incoherent for both H and Y. While the incoherent elastic scattering approximation is appropriate for H-YH 2 , it introduces an undesirable approximation for Y-YH 2 . In this work, we re-evaluate the TSL for Y-YH 2 using FLASSH (Full Law Analysis Scattering System Hub). Y-YH 2 is evaluated using the FLASSH generalized coherent elastic scattering capability in order to capture the Bragg peaks associated with the YH 2 crystal structure which were neglected in the prior NJOY-based evaluation due to limitations in LEAPR. An experimental approach to validate the Y-YH 2 TSL using neutron transmission measurements is discussed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Absorption of fermionic dark matter by nuclear targets

Absorption of fermionic dark matter leads to a range of distinct and novel signatures at dark matter direct detection and neutrino experiments. We study the possible signals from fermionic absorption by nuclear targets, which we divide into two classes of four Fermi operators: neutral and charged current. In the neutral current signal, dark matter is absorbed by a target nucleus and a neutrino is emitted. This results in a characteristically different nuclear recoil energy spectrum from that of elastic scattering. The charged current channel leads to induced $\beta$ decays in isotopes which are stable in vacuum as well as shifts of the kinematic endpoint of $ \beta$ spectra in unstable isotopes. To confirm the possibility of observing these signals in light of other constraints, we introduce UV completions of example higher dimensional operators that lead to fermionic absorption signals and study their phenomenology. Most prominently, dark matter which exhibits fermionic absorption signals is necessarily unstable leading to stringent bounds from indirect detection searches. Nevertheless, we find a large viable parameter space in which dark matter is sufficiently long lived and detectable in current and future experiments.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2022

Depth-resolved thermal conductivity and damage in swift heavy ion irradiated metal oxides

We investigated thermal transport in swift heavy ion (SHI) irradiated insulating single crystalline oxide materials: yttrium aluminum garnet- Y 3 Al 5 O 12 (YAG), sapphire (Al 2 O 3 ), zinc oxide (ZnO) and magnesium oxide (MgO) irradiated by 167 MeV Xe ions at 10 12 – 10 14 ions/cm 2 fluences. Depth profiling of the thermal transport on nano- and micro- meter scales was assessed by time-domain thermoreflectance (TDTR) and modulated thermoreflectance (MTR) methods, respectively. This combination allowed us to isolate the conductivities of different sub-surface damage-regions characterized by their distinct microstructure evolution regimes. Thermal conductivity degradation in SHI irradiated YAG and Al 2 O 3 is attributed to formation of ion tracks and subsequent amorphization, while in ZnO and MgO it is mostly due to point defects. Additionally, notably lower conductivity when probed by very low penetrating thermal waves is consistent with surface hillock formation. An analytical model based on Klemens-Callaway method for thermal conductivity coupled with a simplified microstructure evolution capturing saturation in defect concentration was used to obtain depth dependent damage across the ion impacted region. The studies showed that YAG has the highest damage profile resulting in the less dependence of thermal conductivity with the depth, while MgO on the contrary has the strongest dependence. The presented work sheds new light on how SHI induced defects affect thermal transport degradation and recovery of oxide ceramics as promising candidates for next generation nuclear reactor applications.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Reconstruction of fast neutron direction in segmented organic detectors using deep learning

A method for reconstructing the direction of a fast neutron source using a segmented organic scintillator-based detector and deep learning model is proposed and analyzed. Here, the model is based on recurrent neural network, which can be trained by a sequence of data obtained from an event recorded in the detector and suitably pre-processed. The performance of deep learning-based model is compared with the conventional double-scatter detection algorithm in reconstructing the direction of a fast neutron source. With the deep learning model, the uncertainty in source direction of 0.301 rad is achieved with 100 neutron detection events in a segmented cubic organic scintillator detector with a side length of 46 mm. To reconstruct the source direction with the same angular resolution as the double-scatter algorithm, the deep learning method requires 75% fewer events. Application of this method could augment the operation of segmented detectors operated in the neutron scatter camera configuration for applications such as special nuclear material detection.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2022

Direct Observation of Ammonia Storage in UiO-66 Incorporating Cu(II) Binding Sites

The presence of active sites in metal–organic framework (MOF) materials can control and affect their performance significantly in adsorption and catalysis. However, revealing the interactions between the substrate and active sites in MOFs at atomic precision remains a challenging task. Here, we report the direct observation of binding of NH 3 in a series of UiO-66 materials containing atomically dispersed defects and open Cu(I) and Cu(II) sites. While all MOFs in this series exhibit similar surface areas (1111–1135 m 2 g –1 ), decoration of the -OH site in UiO-66-defect with Cu(II) results in a 43% enhancement of the isothermal uptake of NH 3 at 273 K and 1.0 bar from 11.8 in UiO-66-defect to 16.9 mmol g –1 in UiO-66-Cu II . A 100% enhancement of dynamic adsorption of NH 3 at a concentration level of 630 ppm from 2.07 mmol g –1 in UiO-66-defect to 4.15 mmol g –1 in UiO-66-Cu II at 298 K is observed. In situ neutron powder diffraction, inelastic neutron scattering, and electron paramagnetic resonance, solid-state nuclear magnetic resonance, and infrared spectroscopies, coupled with modeling reveal that the enhanced NH 3 uptake in UiO-66-Cu II originates from a {Cu(II)···NH 3 } interaction, with a reversible change in geometry at Cu(II) from near-linear to trigonal coordination. This work represents the first example of structural elucidation of NH 3 binding in MOFs containing open metal sites and will inform the design of new efficient MOF sorbents by targeted control of active sites for NH 3 capture and storage.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2020

Carbon ablator areal density at fusion burn: Observations and trends at the National Ignition Facility

For inertial confinement fusion experiments, the pusher is composed of a high-density deuterium tritium cyrogenic fuel layer and an ablator, often made of carbon. In an ideal, no-mix implosion, increasing the areal density of the pusher transfers more pressure to the hot spot and increases the hot spot confinement time. There has been a lack of knowledge about the final compressed state of the ablator for implosions at the National Ignition Facility. 14 MeV fusion neutrons inelastically scattering on the remaining carbon ablator excites a nuclear metastable state that emits a prompt 4.4 MeV gamma ray. The gamma reaction history diagnostic data, when reduced by a new data analysis technique, can isolate and measure the carbon gamma rays, which are proportional to the areal density of the ablator during fusion burn. The trends over many National Ignition Facility campaigns show that the ablator areal density is weakly sensitive to the maximum shell velocity, the cold fuel radius, the ablator mass remaining, or the laser picket intensity. Controlled parameter scans reveal that, for specific campaigns, ablator compression has a strong dependence on laser coast time, high Z dopants, and the laser drive foot duration. Using a model of the compressed ablator density profile reveals that the greatest variation of the ablator areal density comes from its thickness, with highly compressed, thin layers having high areal density values. The compression and thickness of the ablator are other metrics that designers should understand to differentiate the types of capsule degradation and maximize the inertial confinement fusion performance.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2025

Five-point functions and the permutation group 𝑆 5

Five-point functions and five-body wave functions play an important role in many areas of nuclear and particle physics, e.g., in 2 →3 scattering processes, in the five-gluon vertex, or in the study of pentaquarks. In this work we consider the permutation group 𝑆 5 to facilitate the description of such objects. We work out the multiplets transforming under irreducible representations of 𝑆 5 and provide compact formulas allowing one to cast the permutations of an object 𝑓 12345 into combinations with definite permutation symmetry. We also give the explicit expressions for the irreducible multiplet products. We consider several practical applications as examples: We arrange the four-momenta and Lorentz invariants of a five-point function into the multiplet structure, we work out the color tensors of the five-gluon vertex in the multiplet notation, and we discuss applications for five-body wave functions like those of pentaquarks.

Bethe-Salpeter equation↗
DOE OSTI2025

On two nucleons near unitarity with perturbative pions

We explore the impact of perturbative pions on the Unitarity Expansion in the two-nucleon S-waves of Chiral Effective Field Theory at next-to-next-to leading order (N 2 LO). Pion exchange explicitly breaks the nontrivial fixed point’s universality, i.e. invariance of S waves under both conformal and Wigner’s combined SU(4) spin–isospin transformations. On the other hand, Unitarity explicitly breaks chiral symmetry. The two seem incompatible in their respective exact-symmetry limits. χEFT with Perturbative Pions in the Unitarity Expansion resolves the apparent conflict in the Unitarity Window (phase shifts 45° ≲ δ(k) ≲ 135°), i.e. around momenta most relevant for low-energy nuclear systems. Its only LO scale is the scattering momentum; NLO adds only scattering length, effective range and non-iterated one-pion exchange (OPE); and N 2 LO only once-iterated OPE. Agreement in the 1 S 0 channel is very good.

Chiral symmetry↗
DOE OSTI2022

Isotope-selective radiography and material assay using high-brilliance, quasi-monochromatic, high-energy photons

We demonstrate the possibility to directly detect microgram amounts of the isotope 7 Li using a quasi-monochromatic high-energy photon beam. The isotope selective detection is based on a witness scatterer absorbing and re-emitting photons via nuclear resonance fluorescence. This enables the detection of isotopes with microgram accuracy at long distances from the actual sample. Further, we demonstrate that the technique can deliver quantitative information without specific knowledge of the photon flux and no spectral capabilities or knowledge of the resonance fluorescence cross section. Detection of low-atomic-weight isotopes screened by heavy shielding is also shown. The techniques described are applicable to all next-generation, ultrahigh brilliance, laser-Compton light sources currently under construction.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Beryllium (Be) Handbook

Beryllium (Be), atomic number 4, is a silver gray metal of low density (1.85g/cm 3 ), moderately high melting point (1289°C), and quite good stability in the atmosphere. Favorable mechanical properties, particularly specific stiffness (elastic modulus/density), have resulted in a number of weight-critical structural applications. Other notable properties of beryllium include good dimensional stability, high specific heat and extremely high transparency to X-radiation. The nuclear properties of beryllium include a high neutron scattering cross section (6 barns for thermal neutrons) and a low neutron absorption cross section (0.009 barns for thermal neutrons) making it a good choice for a neutron reflector. The (n, 2n) reaction in beryllium also makes it suitable for a neutron multiplier.

36 MATERIALS SCIENCE↗
DOE OSTI2021

Preliminary Design of a New Pulsed-Neutron Die-Away Experimental Testbed for Thermal Scattering Law Benchmarks (PNDA) (IER-501 CED-1)

This report presents the preliminary design (CED-1) of IER-501, a new testbed for pulsed-neutron die-away (PNDA) experiments at Lawrence Livermore National Laboratory (LLNL). The PNDA experiments will be high-quality benchmarks that serve to optimize and validate thermal scattering laws (TSLs), which are high-priority nuclear data for the Department of Energy’s Criticality Safety Program (NCSP). PNDA experiments can be used to generate nuclear data validation benchmarks quickly and cheaply, as they do not require fissile material or a nuclear facility to conduct them.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗
DOE OSTI2022

Thermal Neutron Cross Section Measurements at the RPI LINAC [Slides]

Cold polyethylene shows adequate capacity for enhancing sub-thermal neutron flux. Cold moderator system produced high quality thermal cross section measurements. Measurements were performed for polyethylene, polystyrene, Plexiglas, yttrium hydride and beryllium and compared with ENDF/B-VIII.0 TSL evaluations. All data reduction for all measurements was finalized. Future work includes completion of necessary journal publications.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗