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At least 523 records · Page 29

FY27 Annual LDRD Call for Proposals - external release

Proposals are now being accepted for the fiscal year 2027 (FY-27) Laboratory Directed Research and Development (LDRD) call, the FY-27 Annual LDRD Call for Proposals. Idaho National Laboratory (INL) has renewed its research and development (R&D) portfolio to align with its strategy, and this call seeks high-quality proposals that address these renewed research priorities. The LDRD Office encourages proposals that offer the potential to achieve breakthroughs in the three science and technology (S&T) strategic initiatives: • Unleashing America’s Energy Abundance: Enabling the Quadrupling of Nuclear Power by 2050; • Securing America’s Future by Developing Domestic Supply Chains for Critical and Strategic Minerals and Materials (CSMM); and • Delivering Critical National Security Technology. Proposals that support INL’s four strategic thrust areas are also encouraged: • Enabling Future Fusion Energy Systems; • Delivering Small Nuclear Reactor Technology for Space Exploration and Defense Missions; • Accelerating Technologies for Hybrid Energy and Nuclear Applications; and • Securing America’s Energy Future Through Artificial Intelligence (AI).

99 - GENERAL AND MISCELLANEOUS↗

Deuterium permeation and retention in 316L Stainless Steel Manufactured by Laser Powder Bed Fusion

Deployment of additively manufactured materials into nuclear energy systems requires investigation of the full range of the unique environmental effects on these materials. Hydrogen isotopes are common gaseous species in nuclear reactors and exhibit ample high mobility in most materials. While hydrogen isotopes mobility in wrought stainless steel is well understood, this property is not thoroughly studied for its additively manufactured variants. In this study, we investigated the deuterium permeation and retention in 316L stainless steel manufactured by laser powder bed fusion. The results showed that the deuterium permeability in the as-built additively manufactured 316L stainless steel (AM SS316L) is greater than that of the reference wrought 316L stainless steel by a factor of 2.8. However, the stress-relieved and solution-annealed AM SS316L samples exhibit lower deuterium permeability in comparison with the as-built condition. Following the solution annealing, the deuterium permeability of AM SS316L is comparable with that of the reference wrought SS316L. Deuterium retention in the as-built AM SS316L is 45% higher than that of the wrought 316L stainless steel and slightly higher than that of the two thermally annealed AM SS316L materials. Finally, transmission electron microscopy and positron annihilation lifetime spectroscopy were used to obtain microstructural information used to determine deuterium permeation and retention behavior in the studied materials.

36 MATERIALS SCIENCE↗

Single particle trace element analysis of uranium oxide standards with laser-induced breakdown spectroscopy

Femtosecond Laser-Induced Breakdown Spectroscopy (LIBS) was used to analyze over 1000 individual particles of uranium oxide trace element standard CRM124. Intra-granular analysis showed elemental concentrations were consistent across different surface locations on each uranium grain. However, inter-granular comparison revealed large heterogeneity between different grains of the same sample. By comparing the distribution of elemental concentrations across the particle populations, we were able to correctly identify a manufacturing process involving wet chemistry, rather than a dry mixing of two powders to give an overall chemical average. In conclusion, this demonstrates the utility of LIBS as a large-scale single particle analysis tool for nuclear forensics.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Frontiers in the Application of RF Vacuum Electronics

The application of radio frequency (RF) vacuum electronics for the betterment of the human condition began soon after the invention of the first vacuum tubes in the 1920s and has not stopped since. Today, microwave vacuum devices are powering important applications in health treatment, material and biological science, wireless communication-terrestrial and space, Earth environment remote sensing, and the promise of safe, reliable, and inexhaustible energy. This article highlights some of the exciting application frontiers of vacuum electronics.

42 ENGINEERING↗

𝐵⁡(𝐸⁢2) measurements in the yrast band of 28 Mg: Implications for the 𝑁 = 20 island of inversion

High-precision lifetime measurements in 28 Mg were performed to study neutron shell evolution in Mg isotopes and the onset of the N = 20 island of inversion. Here, using both the recoil distance and Doppler shift attenuation methods, five lifetimes were measured in addition to six upper limits. The observation of two long-lived, negative-parity states demonstrate the importance of studying Mg isotopes for the contribution of intruder configurations to sd-shell nuclei. Lifetimes of the $2^+_1$ and $4^+_1$ states of 1.81(5) ps and 172⁢($^{+11}_{–10}$) stat.⁢ (4) stop. ⁢(8) feed.⁢ (4) targ. fs, respectively, demonstrate a loss of collectivity with increasing spin in the yrast band, permitting for distinguishing between current theoretical models. These measurements also highlight the progression of yrast structure across the Mg isotopic chain from rotational at N = 12 to large shape mixing at N = 16 and back to collective behavior at N = 20 but with dominating intruder configurations.

20 ≤ A ≤ 38↗

Impact of Pycnonuclear Fusion Uncertainties on the Cooling of Accreting Neutron Star Crusts

Abstract The observation of X-rays during quiescence from transiently accreting neutron stars provides unique clues about the nature of dense matter. This, however, requires extensive modeling of the crusts and matching the results to observations. The pycnonuclear fusion reaction rates implemented in these models are theoretically calculated by extending phenomenological expressions and have large uncertainties spanning many orders of magnitude. We present the first sensitivity studies of these pycnonuclear fusion reactions in realistic network calculations. We also couple the reaction network with the thermal evolution code dStar to further study their impact on the neutron star cooling curves in quiescence. Varying the pycnonuclear fusion reaction rates alters the depth at which nuclear heat is deposited although the total heating remains constant. The enhancement of the pycnonuclear fusion reaction rates leads to an overall shallower deposition of nuclear heat. The impurity factors are also altered depending on the type of ashes deposited on the crust. These total changes correspond to a variation of up to 9 eV in the modeled cooling curves. While this is not sufficient to explain the shallow heat source, it is comparable to the observational uncertainties and can still be important for modeling the neutron star crust.

79 ASTRONOMY AND ASTROPHYSICS↗

Many-body Nuclear Dynamics

The principal goal of this work was to better understand the fusion of neutron-rich nuclei a topic relevant to the fields of both nuclear physics and nuclear astrophysics. The work provides insight into the structure and reactions of neutron-rich nuclei namely the extent of their neutron density distribution and its polarizability. By comparing the fusion excitation functions for a chain of isotopes with a common target nucleus changes in the attractive nuclear potential are assessed. This change in the attractive potential is related to changes in the neutron density distribution with increasing number of neutrons or changes in fusion dynamics with increasing neutron number. The impact of the pairing of valence neutrons and protons on the fusion cross-section is also examined. Measurement of an isotopic chain is a powerful tool to address this topic. The experimental program made use of several different accelerator facilities. The core of the experimental work involved experiments at the ReA3 accelerator and the Facility for Rare Isotope Beams (FRIB) situated at Michigan State University, at GANIL, the French national nuclear physics laboratory, and the University of Notre Dame. At ReA3 the degree to which α-clusters associated with fusion of 28,30,32 Si + 28 Si result from the collision dynamics or reflect an initial α-cluster structure was explored. Alpha clusters observed in fusion reactions exceed the predictions of the standard statistical model. This experiment provides a measure of how clusterization is impacted by the increasing neutron-richess of the system. In the experiment at GANIL we investigated fusion in 19 O + 12 C and 20 O + 12 C. This experiment utilized the recently developed active-target detector MuSIC@Indiana. Using this proven, highly efficient, active-target detector we measured the fusion excitation function for these neutron-rich systems. Grounded by these experimental measurements, theoretical models were used to examine the role of unpaired valence neutrons on the fusion cross-section at energies just above the fusion barrier.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

The advanced tokamak path to a compact net electric fusion pilot plant

Abstract Physics-based simulations project a compact net electric fusion pilot plant with a nuclear testing mission is possible at modest scale based on the advanced tokamak concept, and identify key parameters for its optimization. These utilize a new integrated 1.5D core-edge approach for whole device modeling to predict performance by self-consistently applying transport, pedestal and current drive models to converge fully non-inductive stationary solutions, predicting profiles and energy confinement for a given density. This physics-based approach leads to new insights and understanding of reactor optimization. In particular, the levering role of high plasma density is identified, which raises fusion performance and self-driven ‘bootstrap currents’, to reduce current drive demands and enable high pressure with net electricity at a compact scale. Solutions at 6–7 T, ∼4 m radius and 200 MW net electricity are identified with margins and trade-offs possible between parameters. Current drive comes from neutral beam and ultra-high harmonic (helicon) fast wave, though other advanced approaches are not ruled out. The resulting low recirculating power in a double null configuration leads to a divertor heat flux challenge that is comparable to ITER, though reactor solutions may require more dissipation. Strong H-mode access (x2 margin over L–H transition scalings) and ITER-like heat fluxes are maintained with ∼20%–60% core radiation, though effects on confinement need further analysis. Neutron wall loadings appear tolerable. The approach would benefit from high temperature superconductors, as higher fields would increase performance margins while potential for demountability may facilitate nuclear testing. However, solutions are possible with conventional superconductors. An advanced load sharing and reactive bucking approach in the device centerpost region provides improved mechanical stress handling. The prospect of an affordable test device which could close the loop on net-electric production and conduct essential nuclear materials and breeding research is compelling, motivating research to validate the techniques and models employed here.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Observation of kinetic mix enhancement in thin-shell OMEGA implosions

Recent separated reactant experiments for thin-shell (6 µ⁢m) shock-driven implosions on OMEGA have demonstrated significant mix from a buried deuterated layer of the shell into the hot spot. Time resolved D 3 He-p reaction history data demonstrate a (50 ± 20)⁢ ps shift earlier in peak nuclear emission for separated reactant experiments relative to control, in contrast to past experimental data for thicker, 20 µ⁢m shells with no laser burn through that show a 75 ps delay due to the time required for hydrodynamic instabilities to develop. This contrast suggests that the mix mechanism was not hydrodynamic. Ion kinetic simulations utilizing fall line analyses show much closer agreement with mix yield and temperature than diffusion models, predicting a D 3 He-p mix yield of 1.7 × 10 9 as compared to the experimental value of 9.3⁢ (±2.1) × 10 8 . This is three orders of magnitude closer than the fall line analysis from a hydrodynamic simulation with an inline diffusive mix model, which suggests minimal mix and D 3 He-p yields of 5×10 5 . This makes kinetic mechanisms the only feasible explanation for the mix seen, demonstrating impact of a non-standard mix mechanism. An analytical model of this kinetic mix mechanism suggests that it can remain significant in situations when the shell expands significantly to low densities, and diffusive models predict negligible mix. Finally, kinetic mix will impact multiple types of high energy density, laser-driven fusion experiments including high-adiabat direct drive cryoexperiments, nuclear cross section experiments, and thin-shell polar direct drive experiments used to tune heat conduction models.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

IRDFF-II: A New Neutron Metrology Library

High quality nuclear data is the most fundamental underpinning for all neutron metrology applications. This paper describes the release of version II of the International Reactor Dosimetry and Fusion File (IRDFF-II) that contains a consistent set of nuclear data for fission and fusion neutron metrology applications up to 60 MeV neutron energy. The library is intended to support: a) applications in research reactors; b) safety and regulatory applications in the nuclear power generation in commercial fission reactors; and c) material damage studies in support of the research and development of advanced fusion concepts. The paper describes the contents of the library, documents the thorough verification process used in its preparation, and provides an extensive set of validation data gathered from a wide range of neutron benchmark fields. The new IRDFF-II library includes 119 metrology reactions, four cover material reactions to support self-shielding corrections, five metrology metrics used by the dosimetry community, and cumulative fission products yields for seven fission products in three different neutron energy regions. In support of characterizing the measurement of the residual nuclei from the dosimetry reactions and the fission product decay modes, the present document lists the recommended decay data, particle emission energies and probabilities for 68 activation products. It also includes neutron spectral characterization data for 29 neutron benchmark fields for the validation of the library contents. Additional six reference fields were assessed (four from plutonium critical assemblies, two measured fields for thermal-neutron induced fission on 233U and 239Pu targets) but not used for validation due to systematic discrepancies in C/E reaction rate values or lack of reaction-rate experimental data. Another ten analytical functions are included that can be useful for calculating average cross sections, average energy, thermal spectrum average cross sections and resonance integrals. The IRDFF-II library and comprehensive documentation is available online at www-nds.iaea.org/IRDFF/. Evaluated cross sections can be compared with experimental data and other evaluations at www-nds.iaea.org/exfor/endf.htm. The new library is expected to become the international reference in neutron metrology for multiple applications.

IAEA IRDFF↗

Quantifying Uncertainties of Microscopic Nuclear Theories

The goal of this project was to produce modernized nuclear data libraries of light ion fusion reactions and actinide fission product yields. Such libraries are essential input in both stockpile science but also fundamental science (nucleosynthesis, superheavy nuclei). When such libraries are used to model complex processes involving exotic, very short-lived nuclei that have not been measured experimentally, the underlying nuclear data come from theoretical models, the predictive power of which needs to be quantified, together with its uncertainties. By teaming up nuclear theorists and statisticians, we built comprehensive theoretical frameworks based on the most fundamental theories of fusion and fission that we coupled for the first time with a Bayesian framework with machine learning techniques for uncertainty quantification. Our results include: (1) statistical emulators for neutron-alpha scattering, and the fission product mass yields of neutron-induced fission of 239 Pu, which will enable developers to generate random realizations of the corresponding data for uncertainty quantification (UQ) in applications; (2) the first complete and most accurate ab initio prediction of the S-factor for proton capture on 7 Be, which – combined with UQ – may become the recommended value at solar energies in the next review of solar fusion cross sections; (3) statistical emulators for fission mass yields in the neutron-induced fission of 239 Pu; (4) the first quantification of how uncertainties in nuclear forces impact fission properties that are relevant in nucleosynthesis simulations to explain how heavy elements are formed in the Cosmos.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Physics Flash Spring 2020

Published by the Physical Sciences Directorate at LANL, the Spring 2020 issue of this newsletter contains an update from the division leader, Tanja Pietraß, Physics Division news roundaup, welcome to new hires, snapshots of Physics managers' work-from-home offices, and service celebrations.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

MST e-News Winter 2020

Articles in this issue include: From Ellen's desk; Advances in aerial payload vessels: Spherical aerogel shells hold vacuum; New materials deformation details emerge through combination of neutron and high-energy x-ray diffraction measurements; and Hans Herrmann named 2019 APS Fellow.

36 MATERIALS SCIENCE↗

Radiation effects in Mn+1AXn phases

M n+1 AX n phases exhibit unique laminated atomic structures that result in properties typical of both ceramics and metals. Due to their unusual characteristics, these materials have been proposed for use in a wide variety of industrial applications, including in nuclear reactors—both fission and fusion systems—where they will be exposed to extreme irradiation conditions and high temperatures. Recently, numerous studies have investigated radiation effects on the M n+1 AX n phases, revealing complex behavior—phase transformations, surface modification, and mechanical property changes—induced by ion or neutron irradiation over a range of temperatures. This review summarizes recent experimental and theoretical work on the response of the M n+1 AX n phases to irradiation and discusses the intrinsic controls on the radiation tolerance of these materials. Based on the review of the present body of work, a comprehensive understanding of the mechanisms of irradiation-induced structural modification and defect evolution in M n+1 AX n phases is developed, as well as proposed strategies for designing novel M n+1 AX n phases with enhanced performance under extreme irradiation conditions.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Fuel–shell mix and yield degradation in kinetic shock-driven inertial confinement fusion implosions

Fuel–shell mix in kinetic plasma conditions is probed using nuclear and x-ray self-emission in shock-driven, D 3 He-gas-filled inertial confinement fusion implosions. As initial gas fill density decreases, measured nuclear yields and ion temperatures are lower than expected as compared to radiation-hydrodynamic simulations. Spatially and temporally resolved x-ray emissions indicate significant mixing at the fuel–shell interface in implosions with low initial gas fill density. In conclusion, this observed fuel–shell mix introduces a substantial amount of shell ions into the center of the implosion prior to and during shock flash and is the key mechanism needed in the kinetic-ion simulations to match experimental nuclear yields.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗