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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 523 records · Page 29
All sourcesNASA NTRSDOE OSTI
NASA NTRS1980

Velocity servo for continuous scan Fourier interference spectrometer

A velocity servo for continuous scan Fourier interference spectrometer of the double pass retroreflector type having two cat's eye retroreflectors is described. The servo uses an open loop, lead screw drive system for one retroreflector with compensation for any variations in speed of drive of the lead screw provided by sensing any variation in the rate of reference laser fringes, and producing an error signal from such variation used to compensate by energizing a moving coil actuator for the other retroreflector optical path, and energizing (through a highpass filter) piezoelectric actuators for the secondary mirrors of the retroreflectors.

Schindler, R. A.↗
NASA NTRS1991

Instrument design and test results of the new all-reflection spatial heterodyne spectrometer

An all-reflection spatial heterodyne spectrometer (SHS) has been recently developed. The advantages over conventional high-resolution grating spectrometers are that the SHS requires no mechanical scanning, a self-compensating optical design permits easy alignment, and it is much smaller than other spectrometers of comparable resolution. Since all beam-splits and recombinations occur by reflection off of a diffraction grating, the interferometer is capable of operating well into the extreme ultraviolet (EUV) and possibly into the soft X-ray region. A description of the design and the characteristics of the instrument is presented. Also, test results, including sample interferograms as well as their Fourier-transformed spectra, at both visible and UV wavelengths are shown. Finally, we report on future developments and possible applications.

Bush, Brett C.↗
DOE OSTI2025

Frequency-Selectable Laser Source for Cosmic Microwave Background Experiments

Cosmic Microwave Background (CMB) experiments measure remnant radiation from the early universe and use that data to determine fundamental properties of the universe. We can constrain key parameters, such as \textit{r}, the cosmic tensor-to-scalar ratio, and $N_\text{eff}$, the effective number of relativistic species, by analyzing the CMB power spectra. Improving our measurements of the CMB requires improving our instrument systematics, one of the most important of which is detector bandpass. Current experiments use a Fourier Transform Spectrometer (FTS) to measure bandpass. However, the FTS is systematics limited, and cannot achieve the accuracy needed to make improved CMB measurements. For this reason, we are developing a new instrument, the Frequency-Selectable Laser Source (FLS) to decrease the uncertainty in bandpass by an order of magnitude. In this paper, we describe work completed to support the version 2 upgrade to the FLS. Using ray-tracing software, we modeled the FLS optics to set physical tolerances for the new design. We also discuss the laser calibration, and future work to be completed in further development of the FLS upgrade.

Rosen-Turits, Gabriel M. [Fermilab]↗
NASA NTRS1971

An interim report on remote sensing of environmental pollutants with a Fourier interference spectrometer.

A small Fourier interference spectrometer for sensing environmental pollutants from spacecraft has been developed at the Jet Propulsion Laboratory. The instrument is intended for obtaining high spectral resolution infrared absorption spectra in the 1.2 to 5.5 micron region at speeds sufficiently high for medium altitude orbital satellite surveys. The paper reviews basic details of the instrument servo and infrared detection systems, previously described, as well as recent developments. In particular, the data-handling system, data reduction techniques and optical tolerance problems are discussed. Preliminary results are included.

Schindler, R. A.↗
NASA NTRS1988

Cryogenic Fourier spectrometer for measuring trace species in the lower stratosphere

A cryogenic Fourier transform spectrometer has been built to measure thermal emission of the earth's limb from a balloon-borne platform. Liquid nitrogen cooling of the spectrometer and liquid helium cooling of the detectors has provided sufficient sensitivity to detect, at 5-15 microns, fifteen molecular species relevant to stratospheric ozone chemistry. The spectral resolution achieved, 0.022/cm, is the best yet attained for emission mode data at these wavelengths. The philosophy behind the design of the optical and electronic systems is presented, followed by an analysis of the performance achieved during balloon flight.

Brasunas, John C.↗
NASA NTRS1980

Optical phase distortion due to compressible flow over laser turrets

Analytical models for optical phase distortion due to compressible flow over a laser turret are developed. Phase distortion is calculated for both blunt and small perturbation turrets. For the blunt turret, the Janzen-Rayleigh technique is used to determine the flow field. Phase distortions of 2.2 wavelengths at 3.8 microns are calculated for the blunt turret. For small perturbation turrets, a versatile analytical model is developed for a turret on a fuselage with circular cross section. With a two dimensional Fourier series representation of the turret, any shape can be considered. Both subsonic and supersonic flows can be calculated. Phase distortions of 1.2 wavelengths at 3.8 microns are calculated for one turret at high subsonic Mach number. In addition to being of value for laser turrets, the methods are applicable to reconnaissance aircraft using photographic equipment and cruise missiles using celestial navigation.

Fuhs, A. E.↗
DOE OSTI2023

Making and breaking terahertz waves with fluid plasmas

Vigorous research efforts during the past several decades have successfully closed the “terahertz gap” between microwaves and infrared light, offering new and increasingly efficient ways to produce, detect, and manipulate radiation fields in the terahertz (THz) frequency range. In our laboratory, THz time-domain spectroscopy (THz-TDS) and optical-pump THz-probe (OPTP) experiments have been routinely utilized as ultrafast spectroscopy tools to investigate a variety of emerging quantum materials and metamaterials. The ultrafast THz pulses are produced by femtosecond laser excitation of photoconductive antennas, semiconductor surfaces (InAs), and nonlinear crystals (ZnTe, GaSe, and LiNbO 3 ). Photoconductive antennas and nonlinear crystals also allow for the coherent detection of these pulses in the time domain, with amplitude and phase spectra obtained in the frequency domain via fast Fourier transform. Although such solid-state schemes are highly desirable in many aspects and thus also commonly utilized in many research laboratories and industrial applications, they typically suffer from limited bandwidths due to the absorption and frequency dispersion induced primarily by phonon resonances, limiting THz applications such as spectroscopy of emerging materials, imaging and detection, and biomedical characterization.

77 NANOSCIENCE AND NANOTECHNOLOGY↗
DOE OSTI2025

Using Ultrafast Entangled Photon Correlations to Measure the Temporal Evolution of Optically Excited Molecular Entanglement (Final Technical Report)

The goal of this project is to build an ultrafast entangled photon spectrometer and use it to measure theoretical predictions that photoexcited states are enhanced by spin-photon interactions. Entanglement of two states describes a specific type of quantum superposition in which measuring one state gives information about a second state. While entanglement is well explored for quantum information and computing systems, its effects on photoexcited states are less understood, especially in the ultrafast domains of molecular vibronic coupling. The grant designs a frequency and temporally resolved entangled photon spectrometer and uses it to test theoretical predictions like enhanced two photon absorption, non-reciprocal Fourier relations, and coupling of photons to spin systems. The end goal of the project is an understanding of how, when, and where entanglement is useful for spectroscopy.

47 OTHER INSTRUMENTATION↗
NASA NTRS1990

Maximum likelihood estimates of polar motion parameters

Two estimators developed by Jeffreys (1940, 1968) are described and used in conjunction with polar-motion data to determine the frequency (Fc) and quality factor (Qc) of the Chandler wobble. Data are taken from a monthly polar-motion series, satellite laser-ranging results, and optical astrometry and intercompared for use via interpolation techniques. Maximum likelihood arguments were employed to develop the estimators, and the assumption that polar motion relates to a Gaussian random process is assessed in terms of the accuracies of the estimators. The present results agree with those from Jeffreys' earlier study but are inconsistent with the later estimator; a Monte Carlo evaluation of the estimators confirms that the 1968 method is more accurate. The later estimator method shows good performance because the Fourier coefficients derived from the data have signal/noise levels that are superior to those for an individual datum. The method is shown to be valuable for general spectral-analysis problems in which isolated peaks must be analyzed from noisy data.

Wilson, Clark R.↗
DOE OSTI2022

Thermal neutron scattering cross sections for amorphous carbon

Carbon materials are commonly found in both nuclear reactors and experimental systems. Various carbon structures occur in nuclear applications ranging from crystalline and nuclear graphite to the amorphous carbon seen in next-generation advanced reactor designs. Amorphous carbon is based on a randomized graphite-like structure and offers the unique ability to disperse impurities throughout the bulk composition. A graphite-like amorphous carbon system was modeled using the classical molecular dynamics (MD) code LAMMPS (Large-scale Atomic/Molecular Massively Parallel Simulator). An improved version of the temperature-dependent Adaptive Intermolecular Reactive Empirical Bond Order (AIREBO) potential was used to model the carbon-carbon atomic interactions for the temperature at 300 K along with densities 1.60, 1.70, 1.85, and 2.23 g/cm{sup 3}. From the normalized velocity autocorrelation function (VACF), the phonon density of state (DOS) was then calculated as the Fourier transform of the normalized VACF. This DOS was then used as the primary input for the evaluation of the thermal scattering law (TSL, i.e. S(α,β)) and associated neutron thermal scattering cross sections. The TSL was analyzed using the Full Law Analysis Scattering System Hub (FLASSH). The amorphous structure results in shifts of the phonon DOS to lower energy modes than typically displayed for ideal crystalline graphite. This impact on the DOS is directly reflected in the TSL. Furthermore, the typical optical peak at 0.25 eV for the ideal graphite disappears for amorphous carbon, in good agreement with the expected structure. (authors)

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
NASA NTRS1973

Optical data processing using paraboloidal mirror segments

An optical data processing system using paraboloidal reflecting surfaces is disclosed. In the preferred embodiment the paraboloidal reflecting surfaces are segments of a paraboloidal mirror. A source of coherent light is in the focal plane of the first paraboloidal mirror segment which collimates the beam and reflects it toward a second paraboloidal mirror surface. The information to be analyzed, on a transparency for example, is placed in the collimated beam. The beam is reflected from the second paraboloidal mirror segment and focused on a Fourier transform plane. A photon detector could be placed in the Fourier transform plane or suitable spatial filters, with the filtered beam then being reflected from a third paraboloidal mirror segment to be focused on a reconstruction plane.

Husain-Abidi, A. S.↗
NASA NTRS1983

A study of a space-station-associated multiple spacecraft Michelson spatial interferometer

One approach to Michelson spatial interferometry at optical wavelengths involves use of an array of spacecraft in which two widely-separated telescopes collect light from a star and direct it to a third, centrally-located, device which combines the beams in order to detect and measure interference fringes. The original version of a spacecraft array for Michelson spatial interferometry (SAMSI) was modified so that the system uses the fuel resupply capability of a space station. The combination of this fuel resupply capability with a method of obtaining image Fourier transform phase information, necessary for full image reconstruction, permits SAMSI to be used to synthesize images equivalent to those produced by huge apertures in space. Synthesis of apertures in the 100 to 500 meter range is discussed. Reconstruction can be performed to a visual magnitude of at least 8 for a 100 A passband in 9 hours. Data are simultaneously collected for image generation from 0.1 micron to 18 microns. In the one-dimensional mode, measurements can be made every 90 minutes (including acquisition and repointing time) for objects as faint as 19th magnitude in the visible.

Stachnik, R. V.↗
DOE OSTI2020

Spectral Radiative Properties of Ceramic Particles for Concentrated Solar Thermal Energy Storage Applications

This work investigates the spectral radiative properties of ceramic particles using a monochromator and a Fourier-transform infrared spectrometer (FTIR) with integrating spheres at wavelengths from 0.38 μm to 15 μm. Particles are encased between two transparent windows to obtain the directional-hemispherical reflectance of the particle bed. Two types of commercially available particles with three different sizes are examined. Integration over the solar spectrum reveals that the solar absorptance of the particle beds is between 0.940 and 0.957. The total emittance at 1000 K is also estimated by assuming the spectral emittance is independent of temperature. The optical constants of particles are modeled with effective medium approaches, considering the optical properties of individual constituent materials. The absorptance of the particle is estimated using the effective optical constants and compared with that of the particle bed from the measurement. Finally, this work facilitates the characterization of radiative properties of particles with a windowed method and provides a modeling scheme for approximating the radiative properties of composite ceramic materials.

14 SOLAR ENERGY↗
DOE OSTI2025

Organic Matter Composition in June 2023 and September 2023 Across the McKenzie Sub-Basin Impacted by the 2020 Holiday Farm Fire

This dataset represents results from a field study aiming to understand the variability in post-fire responses of dissolved organic matter and determine drivers of post-fire responses. Samples were collected at 58 sites within the McKenzie River Watershed (Oregon, USA) that were upstream, within, and downstream of the Holiday Farm Fire burn perimeter. The samples were collected in June 2023 and September 2023 during storm events, approximately 3 years post-fire. Samples were characterized for benezenepolycarboxylic acids (BPCA) and ultra-high resolution mass spectrometry. Dissolved organic carbon and optics (absorbance and fluorescence) data can be found in a separate data packages (https://ir.library.oregonstate.edu/concern/datasets/zc77sz60m, https://ir.library.oregonstate.edu/concern/datasets/mc87q034m). Related data from a subset of sites from 2020-2022 can be found at https://data.ess-dive.lbl.gov/datasets/doi:10.15485/1869708 and https://data.ess-dive.lbl.gov/datasets/doi:10.15485/2478546. For details on how to navigate data packages generated by this project, see https://data.ess-dive.lbl.gov/portals/PNNLRiverCorridorSFA/About. This dataset contains (1) file-level metadata; (2) data dictionary; (3) data package readme; (4) metadata; (5) methods information; (6) benzene polycarboxylic acid (BPCA) concentration data; (7) Fourier transform ion cyclotron resonance mass spectrometry (FTICR-MS) methods; (8) folder of high resolution characterization of organic matter via 12 Tesla FTICR-MS data generated through the Environmental Molecular Sciences Laboratory (EMSL; https://www.pnnl.gov/environmental-molecular-sciences-laboratory). This package contains the following file types: csv, xml, pdf.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS2001

Demonstration of Imaging Fourier Transform Spectrometer (FTS) Performance for Planetary and Geostationary Earth Observing

The combination of massively parallel spatial sampling and accurate spectral radiometry offered by imaging FTS makes it extremely attractive for earth and planetary remote sensing. We constructed a breadboard instrument to help assess the potential for planetary applications of small imaging FTS instruments in the 1 - 5 micrometer range. The results also support definition of the NASA Geostationary Imaging FTS (GIFTS) instrument that will make key meteorological and climate observations from geostationary earth orbit. The Planetary Imaging FTS (PIFTS) breadboard is based on a custom miniaturized Bomen interferometer that uses corner cube reflectors, a wishbone pivoting voice-coil delay scan mechanism, and a laser diode metrology system. The interferometer optical output is measured by a commercial infrared camera procured from Santa Barbara Focalplane. It uses an InSb 128x128 detector array that covers the entire FOV of the instrument when coupled with a 25 mm focal length commercial camera lens. With appropriate lenses and cold filters the instrument can be used from the visible to 5 micrometers. The delay scan is continuous, but slow, covering the maximum range of +/- 0.4 cm in 37.56 sec at a rate of 500 image frames per second. Image exposures are timed to be centered around predicted zero crossings. The design allows for prediction algorithms that account for the most recent fringe rate so that timing jitter produced by scan speed variations can be minimized. Response to a fixed source is linear with exposure time nearly to the point of saturation. Linearity with respect to input variations was demonstrated to within 0.16% using a 3-point blackbody calibration. Imaging of external complex scenes was carried out at low and high spectral resolution. These require full complex calibration to remove background contributions that vary dramatically over the instrument FOV. Testing is continuing to demonstrate the precise radiometric accuracy and noise characteristics.

Revercomb, Henry E.↗
DOE OSTI2022

Thermal Neutron Scattering Cross Sections for Graphitic Amorphous Carbon

Carbon materials are commonly found in both nuclear reactors and experimental systems. Various carbon structures occur in nuclear applications ranging from crystalline and nuclear graphite to the amorphous carbon seen in next-generation advanced reactor designs. Amorphous carbon is based on a randomized graphite-like structure and offers the unique ability to disperse impurities throughout the bulk composition. A graphite-like amorphous carbon system was modeled using the classical molecular dynamics (MD) code LAMMPS (Large-scale Atomic/Molecular Massively Parallel Simulator). An improved version of the temperature-dependent Adaptive Intermolecular Reactive Empirical Bond Order (AIREBO) potential was used to model the carbon-carbon atomic interactions for the temperature at 300 K along with densities 1.60, 1.70, 1.85, and 2.23 g/cm 3 . From the normalized velocity autocorrelation function (VACF), the phonon density of state (DOS) was then calculated as the Fourier transform of the normalized VACF. This DOS was then used as the primary input for the evaluation of the thermal scattering law (TSL, i.e. S(α,β)) and associated neutron thermal scattering cross sections. The TSL was analyzed using the Full Law Analysis Scattering System Hub (FLASSH). The amorphous structure results in shifts of the phonon DOS to lower energy modes than typically displayed for ideal crystalline graphite. This impact on the DOS is directly reflected in the TSL. Furthermore, the typical features and the optical graphitic peak at 0.25 eV for the ideal graphite DOS disappear for graphite-like amorphous carbon, which shows good agreement with the expected structure.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
NASA NTRS1991

FTIR Spectroscopic Characterization Of II-VI Semiconductors

Combination of commercial Fourier-transform infrared (FTIR) spectrometer with computer and special-purpose software constitutes highly automated facility for acquisition and processing of infrared transmission or reflection spectral image data. Intended principally to acquire transmission spectra of some compounds of elements in groups II and VI of periodic table. System used to characterize specimens of II/VI alloy semiconductors grown by directional solidification and quenching. Transmission-edge maps helpful in studies of flows, gradients of temperature, and coefficients of diffusion in solidifying melts. Data acquired by system include optical characteristics, and they both verify and complement data obtained by such other techniques as measurements of density and x-ray-dispersion analysis.

Perry, G. L. E.↗