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At least 523 records · Page 29

Bias Between ENDF/B-VIII and ENDF/B-VII.1 for LEU Pin Array Systems

Extensive testing of new cross section data is performed in SCALE prior to its release. The release of ENDF/B-VIII.0 requires the generation and testing of new data libraries which are planned to be included in the release of SCALE 6.3 in 2019 or 2020. KENO benchmark results have been published previously for beta and final releases of ENDF/B-VIII.0 using the entire Verified, Archived Library of Inputs and Data (VALID). This work presents an energy-dependent change in the results for low-enriched uranium (LEU) pin array systems. The process of identifying the difference is highlighted as a case study to determine how data testing and benchmarking can be performed to provide more detailed feedback to the data community on potential data deficiencies.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Adding ($\mathcal{α}$,n) Emission to an Existing Subcritical Benchmark Statistical Uncertainty Method

Subcritical measurements often use radiation detectors to infer parameters related to the physics of a measured system. One type of subcritical measurements typically performed are called neutron noise measurements. These types of measurements utilize the fact that prompt neutrons are produced from fission immediately after a fission event and are therefore correlated in time. Subcritical benchmarks require evaluation of the statistical and systematic uncertainties of a measurement. Previous work established methods for determining statistical and systematic uncertainties in subcritical benchmarks. The data were analyzed using the Hage-Cifarelli formalism of the Feynman Variance-to-Mean method. The previous work made an assumption that the ($\mathcal{α}$,n) emission rate was negligible. This assumption was used because the previous work focused on systems with metal Plutonium. This work extends the existing statistical uncertainty method to include ($\mathcal{α}$,n) emissions.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Verification of MCNP6.2 for Nuclear Criticality Safety Applications

Several suites of verification/validation benchmark problems were run in early 2017 to verify that the new production release of MCNP6.2 performs correctly for nuclear criticality safety applications (NCS). MCNP6.2 results for several NCS validation suites were compared to the results from MCNP6.1 [1] and MCNP6.1.1 [2]. MCNP6.1 is the production version of MCNP® released in 2013, and MCNP6.1.1 is the update released in 2014. MCNP6.2 includes all of the standard features for NCS calculations that have been available for the past 15 years, along with new features for sensitivity-uncertainty based methods for NCS validation [3]. Results from the benchmark suites were compared with results from previous verification testing [4-8]. Criticality safety analysts should consider testing MCNP6.2 on their particular problems and validation suites. No further development of MCNP5 is planned. MCNP6.1 is now 4 years old, and MCNP6.1.1 is now 3 years old. In general, released versions of MCNP are supported only for about 5 years, due to resource limitations. All future MCNP improvements, bug fixes, user support, and new capabilities are targeted only to MCNP6.2 and beyond.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

Critical Configuration for Beryllium Reflected Assemblies of U(93.15)O 2 Fuel Rods (1.506-CM Pitch and 7-Tube Clusters)

A series of critical experiments were completed in 1962-1965 at Oak Ridge National Laboratory’s Critical Experiments Facility in support of the Medium-Power Reactor Experiments (MPRE) program. In the late 1950’s efforts were made to study “power plants for the production of electrical power in space vehicles”. The MPRE program was a part of those efforts and studied the feasibility of a stainless steel system, boiling potassium 1 MW(t), or about 140 kW(e), reactor. The program was carried out in [fiscal years] 1964, 1965, and 1966. A summary of the program’s effort was compiled in 1967. The delayed critical experiments were a mockup of a small, potassium-cooled space power reactor for validation of reactor calculations and reactor physics methods.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Impact of Increased Latent Generations on Sensitivity Calculations with SCALE

Analyses of cross section sensitivity data from systems with fissile material allow analysts to associate an importance for each material, nuclide, reaction, and neutron energy by simulating real world criticality scenarios. Although criticality safety validation efforts can be guided by the cross-section sensitivity and uncertainty data generated for a particular system, these calculations can often be computationally expensive and sometimes cumbersome without proper guidance. The TSUNAMI suite within the SCALE code package has several methods for generating sensitivity data, including multigroup and continuous energy (CE) capabilities. The release of SCALE 6.3 has three different CE methods for generating cross section sensitivity data: (1) the Iterated Fission Probability (IFP) method with the KENO Monte Carlo transport solver, (2) the IFP method with the Shift Monte Carlo transport solver, and (3) the Contributon-Linked eigenvalue sensitivity/Uncertainty estimation via Tracklength importance CHaracterization (CLUTCH) method with the KENO Monte Carlo transport solver. Although the CLUTCH method has additional parameters for generating sensitivity data files relative to the IFP method, all three methods use latent generations, which are the generations between an event (i.e., fission) and the assessment of importance based on the asymptotic population of progeny neutrons. Increasing the number of latent generations in a calculation leads to increased discrimination of the sensitivity coefficients but at the cost of the increased uncertainty associated with those generated values. Analysts must balance the accuracy of the sensitivity calculations and its uncertainty with the associated computational cost involved in generating the values. This paper discusses the impact of adjusting the latent generation parameter for a range of sensitivity values and how these changes compare with the direct perturbation values obtained from a change of ±0.5% Δ k in both benchmark and safety application models. Two benchmarks from the International Handbook of Evaluated Criticality Safety Benchmark Experiments and the MPC-32 dual purpose canister for spent nuclear fuel are used for analysis.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Update on the Benchmark Analysis of the Jupiter Experiments: Plutonium Moderated by Lead

The Jupiter experiment was a series of measurements in the summer of 2017 to analyze the effects of voids in lead moderated plutonium assemblies. This experiment was part of a larger campaign that took place at the National Criticality Experiments Research Center (NCERC) in collaboration with the Japan Atomic Energy Agency (JAEA) that also investigated assemblies with differing uranium enrichments. The purpose for this campaign was to provide data useful for a potential lead-bismuth cooled accelerator driven system. This data is needed due to the low number of benchmarks involving lead. Given the wide use of lead for shielding in addition to new reactor designs, there is a need for further benchmarking that this experiment could help fulfill. In addition, adding more benchmarks to the International Criticality Safety Benchmark Evaluation Project (ICSBEP) is helpful for further validation of simulation methods used for criticality safety. This summary is an update on the current progress of this analysis, and all results shown are preliminary.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Benchmark Testing of a new {sup 56}Fe evaluation for criticality safety applications - 14451

The SAMMY code was used to evaluate resonance parameters of the {sup 56}Fe cross section in the resolved resonance energy range of 0-2 MeV using transmission data, capture, elastic, inelastic, and double differential elastic cross sections. The resonance analysis was performed with the code SAMMY that fits R-matrix resonance parameters using the generalized least-squares technique (Bayes' theory). The evaluation yielded a set of resonance parameters that reproduced the experimental data very well, along with a resonance parameter covariance matrix for data uncertainty calculations. Benchmark tests were conducted to assess the evaluation performance in benchmark calculations. (authors)

42 ENGINEERING↗

Preliminary Results on Bayesian Inverse UQ for OECD/NEA WPNCS Subgroup 14 Benchmark Exercise for Error Recovery and Experimental Coverage

The Organization for Economic Cooperation and Development (OECD) Working Party on Nucelar Criticality Safety (WPNCS) has proposed a benchmark exercise representative of neutronic behavior in criticality experiments. Here, the goal is to develop confidence in data assimilation techniques used to adjust nuclear data. Participants are given synthetic experimental models with associated measured data and asked to estimate the model parameters given the model and measurements as well as provide predictions for separate application models. In this work, we performed data assimilation using Bayesian inverse Uncertainty Quantification (UQ) with machine learning surrogate models to produce posterior parameter distributions for the requested parameters and posterior predictive distributions for the requested responses. Several experimental models are shown to insufficiently inform the posterior parameter distributions for the applications involved. However, given sufficient experimental data, posterior parameter estimates yielded reduced uncertainty in the response predictions of interest while covering the experimental data.

Bayesian Inference↗

Critical configuration and physics measurements for graphite reflected assemblies of U(93.15)O 2 fuel rods (1.506-CM pitch)

A series of critical experiments were completed in 1962-1965 at Oak Ridge National Laboratory’s Critical Experiments Facility in support of the Medium-Power Reactor Experiments (MPRE) program. In the late 1950’s efforts were made to study “power plants for the production of electrical power in space vehicles”. The MPRE program was a part of those efforts and studied the feasibility of a stainless steel system, boiling potassium 1 MW(t), or about 140 kW(e), reactor. The program was carried out in [fiscal years] 1964, 1965, and 1966. A summary of the program’s effort was compiled in 1967. The delayed critical experiments were a mockup of a small, potassium-cooled space power reactor for validation of reactor calculations and reactor physics methods.

1.506-cm pitch UO2 Assembly↗

Critical Configuration and Physics Measurements for Assemblies of U(93.15)O 2 Fuel Rods (1.506-cm Pitch)

A series of critical experiments were completed from 1962–1965 at Oak Ridge National Laboratory’s (ORNL’s) Critical Experiments Facility (CEF) in support of the Medium-Power Reactor Experiments (MPRE) program. In the late 1950s, efforts were made to study “power plants for the production of electrical power in space vehicles.”(a) The MPRE program was a part of those efforts and studied the feasibility of a stainless-steel system, boiling potassium 1 MW(t), or about 140 kW(e), reactor. The program was carried out in [fiscal years] 1964, 1965, and 1966. A summary of the program’s effort was compiled in 1967.a The delayed critical experiments were a mockup of a small, potassium-cooled space power reactor for validation of reactor calculations and reactor physics methods. Initial experiments, performed in November and December of 1962, consisted of a core of unmoderated stainless-steel tubes, each containing 26 UO 2 fuel pellets, surrounded by a graphite reflector. Measurements were performed to determine critical reflector arrangements, relative fission-rate distributions, and cadmium ratio distributions. Subsequent experiments used beryllium reflectors and also measured the reactivity for various materials placed in the core. “The [assemblies were built] on [a] vertical assembly machine so that the movable part was the core and bottom reflector” (see Reference 1). The experiment studied in this evaluation was the second of the series and had the fuel rods in a 1.506-cm-triangular pitch. One critical configuration was found (see Reference 3). Once the critical configuration had been achieved, various measurements of reactivity, relative axial and radial activation rates of 235U,bc and cadmium ratios were performed. The cadmium ratio, reactivity, and activation rate measurements performed on the critical configuration are described in Sections 1.3, 1.4, and 1.7, respectively.

1.506-cm pitch↗

Critical Configuration and Physics Measurements for Beryllium Reflected Assemblies of U(93.15)O 2 Fuel Rods (1.506-cm Pitch)

Cadmium ratios were measured with enriched uranium metal foils at various locations in the assembly with the fuel tube at the 1.506-cm spacing. They are described in the following subsections. The experiment configuration was the same as the first critical configuration described in HEU-COMP-FAST-004 (Case 1). The experimenter placed 0.75-cm-diameter × 0.010-cm-thick 93.15%-235U-enriched uranium metal foils with and without 0.051-cm-thick cadmium covers at various locations in the core and top reflector. One part of the cadmium cover was cupshape and contained the uranium foil. The other part was a lid that fit over the exposed side of the foil when it was in the cup shaped section of the cover. As can be seen in the logbook, two runs were required to obtain all the measurements necessary for the cadmium ratio. The bare foil measurements within the top reflector were run first as part of the axial foil activation measurements. The results of this run are used for both the axial activation results and the cadmium ratios. Cadmium covered foils were then placed at the same location through the top reflector in a different run. Three pairs of bare and cadmium covered foils were also placed through the core tank. One pair was placed at the axial center of a fuel tube 11.35 cm from the center of the core. Two pairs of foils were placed on top of fuel tubes 3.02 and 12.06 cm from the center of the core. The activation of the uranium metal foils was measured after removal from the assembly using two lead shielded NaI scintillation detectors as follows. The NaI scintillators were carefully matched and had detection efficiencies for counting delayed-fission-product gamma rays with energies above 250 KeV within 5%. In all foil activation measurements, one foil at a specific location was used as a normalizing foil to remove the effects of the decay of fission products during the counting measurements with the NaI detectors. The normalization foil was placed on one NaI scintillator and the other foil on the other NaI detector and the activities measured simultaneously. The activation of a particular foil was compared to that of the normalization foil by dividing the count rate for each foil by that of the normalization foil. To correct for the differing efficiencies of the two NaI detectors, the normalization foil was counted in Detector 1 simultaneously with the foil at position x in Detector 2, and then the normalization foil was counted simultaneously in Detector 2 with the foil from position x in Counter 1. The activity of the foil from position x was divided by the activity of the normalization foil counted simultaneously. This resulted in obtaining two values of the ratio that were then averaged. This procedure essentially removed the effect of the differing efficiencies of the two NaI detectors. Differing efficiencies of 10% resulted in errors in the ratios measured to less than 1%. The background counting rates obatined with the foils used for the measurements on the NaI detectors before their irradiation measurement were subtracted from all count rates. The results of the cadmium ratio measurements are given in Table 1.3-1 and Figure 1.3-1. “No correction has been made for self shielding in the foils” (Reference 3).

1.506-cm pitch↗

Application of the EPRI depletion reactivity benchmarks - 14423

The EPRI measured-based depletion reactivity benchmarks intend to facilitate the validation of burnup credit by validating the combined effect of changes in isotopic content and cross-sections. In the framework of burnup credit implementation for PWR fuels, this paper proposes to study the application of the EPRI benchmarks for a spent fuel pool criticality evaluation using the French tools: the DARWIN 2.2 depletion package and the CRISTAL V1 criticality safety package, both based on cross-section libraries from the JEF2.2 evaluation. For that purpose, the benchmarks are analyzed using the connection of DARWIN 2.2 with APOLLO2-MORET 4, allowing the determination of the bias for the reactivity decrement. Then, these results are used to define a bias to take into account in the criticality evaluation of a spent fuel pool. In addition, the benefit of the EPRI depletion reactivity benchmarks is assessed through a comparison with the validation approach adopted in France until now. The bias resulting from this latter approach is evaluated by 1) applying, to the calculated nuclides concentrations, isotopic penalizing factors derived from the comparison between calculated values of nuclide concentrations and experimental values obtained from used fuel chemical analyses from French reactors, 2) analyzing representative critical experiments. Additional analysis of the benchmarks using the connection of VESTA 2.1 with MORET 5 is performed as these codes allow calculations of complex 3D geometrical configurations and the use of various nuclear data libraries. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

ENDF/B-VIII.0: the 8. major release of the ENDF/B library containing CIELO-project evaluations, new standards and thermal scattering data - 25580

The ENDF/B-VIII.0 evaluated nuclear reaction data library was released on February 2, 2018. ENDF/B-VIII.0 incorporates many improvements including the new IAEA standards, a nearly completely new thermal neutron scattering sublibrary and the CIELO project evaluations for neutron reactions on {sup 16}O, {sup 56}Fe, {sup 235}U, {sup 238}U and {sup 239}Pu. These evaluations are a direct result of improvements in theory and simulation and benefit from recent experimental data obtained in the U.S. and Europe. Notable other advances include updated evaluated data for light nuclei, structural materials, actinides and charged-particle reactions, and specific updates to fission energy release, prompt fission neutron and γ-ray spectra. ENDF/B-VIII.0 has undergone substantial testing including a wide range of criticality, reaction rate, and shielding benchmarks. Our integral validation demonstrates that performance of the library is a noticeable improvement over the previous ENDF/B-VII.1 library. (authors)

61 RADIATION PROTECTION AND DOSIMETRY↗

Verification of the Uniformly-Ordered Binary Decision Algorithm in Correlated-Benchmark Whisper Calculations

Whisper is a nuclear criticality safety code package that aids analysts in validation exercises by computing upper subcritical limits (USL) for applications of interest. To obtain statistically meaningful, significant, and conservative USLs, the analyst must ensure that Whisper selects a sufficient number of benchmarks that are neutronically similar to the application. Many of the available benchmarks are correlated but are currently treated as independent, leading to an artificially small sample size, as their individual information contributions will be overestimated. To aid the analyst in obtaining a sufficient sample size, prior work [2] demonstrated application of the Uniformly-Ordered Binary Decision (UOBD) algorithm in adjusting benchmark weights to account for benchmark correlations. This work provides verification of the Whisper implementation and considers the impact of updated benchmark correlations compared to those available previously. We demonstrate that the UOBD algorithm performs as expected with an analytic example. With HEU-SOL-THERM-001 cases 1 through 10 as the applications, we compare the USLs computed with benchmark correlations available in the Whisper 1.1 release only to those computed with additional benchmark correlations from DICE 2023 and demonstrate substantive differences.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Investigation of Application Specific k eff Sensitivities to Existing and New Subcritical and Critical Experiments

Integral subcritical and critical experiments are essential in providing validation of computational codes which improve confidence in the predicted k eff results of specific applications. This work discusses the relevance of existing integral subcritical and critical experiments to applications far reaching across the nuclear complex. These applications include Travelling Wave Reactors (TWR), Kilopower Reactor Using Stirling Technology (KRUSTY), and plutonium reflected by tantalum. The primary goal of this work is to improve knowledge of energy-dependent cross-section sensitivities for specific applications, identify nuclear data gaps in existing experiments, enable an optimized design of new experiments to address these gaps, and design practical new experiments that could be executed at the National Criticality Experiments Research Center (NCERC) that have a high-value to these applications.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Evaluation of isotopic measurements and burn-up value of samples GU3, GU3' and BM5, BM5' of Ariane project - 14481

Estimation of the burn-up value and the corresponding isotopic composition of the nuclear fuel are the most important subjects for criticality analysis and source term estimation in the framework of spent fuel management. The only practical way to estimate the fuel composition and burn-up value is the isotopic depletion calculation with well qualified codes and nuclear data. Such qualification requires the availability of well evaluated experimental measurements to be used as benchmarks. The purpose of this study is evaluation of the isotopic measurements of GU3 (GU3') and BM5 (BM5') samples of ARIANE project in order to judge their adequacy for qualification of the codes and libraries. Additionally the sensitivity analyses to manufacturing and operation parameters are performed in order to obtain the uncertainty due to both types of parameters. (authors)

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Benchmark of the Chlorine Worth Study Experiments in Support of Chlorine Nuclear Data Validation for Nuclear Criticality Safety

The Chlorine Worth Study (CWS) was a critical experiment to address an urgent need for thermal chlorine nuclear data validation in plutonium systems. This urgent need is tied directly to plutonium recycle and recovery operations in the plutonium facility at Los Alamos National Laboratory, where exceptionally conservative criticality safety limits are used because no credit is taken for the neutron capture by chlorine. The experiment used weapons-grade plutonium metal plates clad in stainless steel, known as the PANN (plutonium aluminum no nickel) ZPPR (zero power physics reactor) plates. The plutonium was reflected and moderated by high-density polyethylene and included combinations of polyvinyl chloride (PVC) and chlorinated polyvinyl chloride (CPVC) as absorbers. The experiment and benchmark included three configurations mimicking 30 g 239 Pu/L plutonium, 300 g 239 Pu/L plutonium, and 600 g 239 Pu/L plutonium in an aqueous chloride solution. Uncertainties in the benchmark included five broad categories: (1) criticality measurement, (2) mass and density, (3) dimensions, (4) material compositions, and (5) positioning. The largest contribution to the overall uncertainties for all three cases came from the material compositions, in particular the PVC and CPVC absorber compositions. A detailed model was created to be a near match (that is within expectations of transport code users) and a simplified model was created to minimize offset dimensions and expedite modeling for code validation. Sample calculations were completed in MCNP6.3 with ENDF/B-VIII.0 and ENDF/B-VII.1 nuclear data. For the detailed and simplified models, the average difference between the computed and experimental k eff was 951 pcm. CWS will serve as the key validation experiment for nuclear criticality safety in support of aqueous chloride operations. The sensitivity to the chlorine capture cross section is orders of magnitude greater than other existing benchmarks. The current limits, as defined by nuclear criticality safety, are 520 g Pu per batch, i.e. the minimum critical mass of the Pu solution infinitely reflected by water [Criticality Handbook: Volume II, (1969)]. This extremely conservative critical mass limit does not credit any neutron capture by chlorine (in particular neutron capture by 35 Cl) and greatly impedes the throughput required for current and future operations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗