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At least 523 records · Page 29
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Engineered chirality of one-dimensional nanowires

The origin and function of chirality in DNA, proteins, and other building blocks of life represent a central question in biology. Observations of spin polarization and magnetization associated with electron transport through chiral molecules, known collectively as the chiral induced spin selectivity effect, suggest that chirality improves electron transfer. Using reconfigurable nanoscale control over conductivity at the LaAlO 3 /SrTiO 3 interface, we create chiral electron potentials that explicitly lack mirror symmetry. Quantum transport measurements on these chiral nanowires reveal enhanced electron pairing persisting to high magnetic fields (up to 18 tesla) and oscillatory transmission resonances as functions of both magnetic field and chemical potential. We interpret these resonances as arising from an engineered axial spin-orbit interaction within the chiral region. The ability to create one-dimensional electron waveguides with this specificity creates opportunities to test, via analog quantum simulation, theories about chirality and spin-polarized electron transport in one-dimensional geometries.

Science & Technology - Other Topics↗
DOE OSTI2023

Constraining light thermal inelastic dark matter with NA64

A vector portal between the Standard Model and the dark sector is a predictive and compelling framework for thermal dark matter. Through co-annihilations, models of inelastic dark matter (iDM) and inelastic Dirac dark matter (i2DM) can reproduce the observed relic density in the MeV to GeV mass range without violating cosmological limits. In these scenarios, the vector mediator behaves like a semi-visible particle, evading traditional bounds on visible or invisible resonances, and uncovering new parameter space to explain the muon (g–2) anomaly. By means of a more inclusive signal definition at the NA64 experiment, we place new constraints on iDM and i2DM using a missing energy technique. With a recast-based analysis, we contextualize the NA64 exclusion limits in parameter space and estimate the reach of the newly collected and expected future NA64 data. Our results motivate the development of an optimized search program for semi-visible particles, in which fixed-target experiments like NA64 provide a powerful probe in the sub-GeV mass range.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2025

Coupling between collective modes in the deformed 98 Zr nucleus: Insights from consistent HFB+QRPA calculations with the Gogny interaction

The Zirconium isotopes exhibit structural properties that present multiple challenges to nuclear theory. Investigations of the coupling present within isoscalar modes and within isovector modes are scarce but important for advancing our understanding of the microscopic picture of nuclei. To explore some of these underlying coupling features, and to test the predictive power of a state-of the-art nuclear structure approach, we provide a detailed analysis of the properties of 90,96,98Zr. This region includes a benchmarking case and offers insights into nuclear deformation phenomena. To investigate the coupling between collective modes in deformed nuclei, we focused our analysis on the ground and excited-state properties of these isotopes, employing a consistent approach with the axially-symmetric deformed Hartree-Fock-Bogoliubov (HFB) and the Quasiparticle Random Phase Approximation (QRPA) framework, both using the Gogny D1M force. This approach effectively describes both low-lying and giant-resonance states. We devoted special attention to the deformed 98Zr nucleus, where we confirm the existence of coupling between monopole and quadrupole excitations through the K π = 0 + QRPA components and demonstrate an analogous dipole-octupole coupling through the K π = 0 − and K π = 1 − components. Intrinsic transition densities and associ ated radial projections illustrate the coupling. Our work complements and extends earlier studies carried out using density-functional-based methods and notably, we included the complete Coulomb interaction also in the pairing fields, i.e. we treat terms exactly that are approximated in typical calculations that use the Gogny D1 and D2 interaction families.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
NASA NTRS1998

The Dynamics of Disorder-Order Transition in Hard Sphere Colloidal Dispersions

The Physics of Hard Spheres Experiment (PHaSE) seeks a complete understanding of the entropically driven disorder-order transition in hard sphere colloidal dispersions. The light scattering instrument designed for flight collects Bragg and low angle light scattering in the forward direction via a CCD camera and performs conventional static and dynamic light scattering at 10-160 deg. through fiber optic cables. Here we report on the kinetics of nucleation and growth extracted from time-resolved Bragg images and measurements of the elastic modulus of crystalline phases obtained by monitoring resonant responses to sinusoidal forcing through dynamic light scattering. Preliminary analysis of the former indicates a significant difference from measurements on the ground, while the latter confirms nicely laboratory experiments with the same instrument and predictions from computer simulations.

Chaikin, Paul M.↗
NASA NTRS2008

Behavior of Spinning Space Vehicles with Onboard Liquids, 2nd Edition, Technical Report B8030

Although the fundamental principles of spin stabilization are well established, uncertainty regarding the potential for rapid nutation growth caused by onboard liquids is a continuing concern. NASA and other organizations regularly encounter the issue of rapid nutation growth due to energy dissipation by liquids on spinning vehicles. Of concern is the stability of spinning upper stages and of spacecraft that spin for part or all of their missions. Several missions have required last-minute hardware or operational changes to deal with rapid nutation divergences that were identified late in the program. In some instances, major schedule slips were barely averted. In at least two cases, it was determined that a spinning upper stage was not a viable option. Historically, the "slosh" issue has been addressed by each space vehicle project individually, if it has been addressed at all. Due to budgetary and programmatic constraints, individual projects are unable to address the problem globally. Hence, there has been little effort to collect available test and flight data and use that data to make a coherent, unified picture of the "slosh" effect and how to deal with it. To some extent, each project has had to "reinvent the wheel", which can be both costly and risky. This study is a step toward correcting the situation. Specifically, the goal was to identify and collect available flight and test data for spinning vehicles with onboard liquid propellants. A total of 149 flight data points and 1,692 test points were collected as part of this study. This data was analyzed, correlated, and is presented here in a normalized form. In most cases, the normalization involves a dimensionless nutation time constant that can be used to predict performance of other vehicles with the same type of tank. For some configurations, it was also possible to identify conditions that can lead to resonance between nutational motion and liquid modes. Gaps in the knowledge base are identified and approaches to filling those gaps are outlined. The data presented here has two different but related uses. First, it can be applied directly to current and future spacecraft programs. Second, it can provide truth models for testing analytical techniques. Experience has shown that purely analytical models of the liquid "slosh" effect on spinning vehicles are unreliable unless they are validated against flight or test data. To the author's knowledge, this report contains the most extensive and varied data set available. As such, it should be a good resource for anyone seeking to develop and validate improved analytical techniques. All of the original digital data sets have been archived on disk, with copies provided to NASA/KSC. With some restrictions, many of these data sets can be made available to researchers within the United States. Whenever possible, spacecraft are identified by name in this report. However, several organizations provided access to data with the explicit proviso that their programs not be identified and that parameters be presented only in normalized form. These constraints have been respected.

Hubert, Carl↗
DOE OSTI2025

Studying 𝜋 + ⁢𝜋 − photoproduction beyond Pomeron exchange

Forward photoproduction of 𝜋 + ⁢𝜋 − pairs with invariant mass of the order of 𝑚 𝜌 ∼770 MeV is traditionally attributed to Pomeron exchange. Based on a detailed analysis of the CEBAF Large Acceptance Spectrometer photoproduction data collected at photon energies below 4 GeV, it is shown from a study of the angular moments that the dynamics of two-pion photoproduction for |𝑡| ≳ 0.5 GeV 2 cannot be explained by Pomeron exchange alone. This motivates the development of a new theoretical model of two-pion photoproduction which incorporates both two-pion and pion-nucleon resonant contributions. After fitting free parameters, the model provides an excellent description of the low moments of the angular distribution measured at CLAS and enables an assessment of the relative contributions of particular production mechanisms and an interpretation of the various features of the data in terms of these mechanisms.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Charge Correlations in Cuprate Superconductors

High-temperature superconductivity, with transition temperatures up to ≈134 K at ambient pressure, occurs in layered cuprate compounds. The conducting CuO 2 planes, which are universally present, are responsible for the superconductivity but also show a disposition to other competing states including spin and charge order. Charge-density-wave (CDW) order appears to be a universal property of cuprate superconductors. It has been studied via a multitude of probes including X-ray and neutron scattering, nuclear magnetic resonance, scanning probe techniques, electronic transport, and quantum oscillations. Here, we review the microscopic properties of the CDW order. We discuss the nature of the ordered state, that is, its symmetry and microscopic structure. Furthermore, we show how the CDW order is related to quenched disorder, host structure, symmetry breaking perturbations, and magnetic fields. Here, we also describe measurements of dynamic collective charge excitations that are closely related to the quasi-static CDW order. Finally, we highlight some of the debated issues in the field, including the origin of the CDW order, the relationship to spin order, and the nature of the spatial CDW correlations.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
NASA NTRS2010

A Transportable Gravity Gradiometer Based on Atom Interferometry

A transportable atom interferometer-based gravity gradiometer has been developed at JPL to carry out measurements of Earth's gravity field at ever finer spatial resolutions, and to facilitate high-resolution monitoring of temporal variations in the gravity field from ground- and flight-based platforms. Existing satellite-based gravity missions such as CHAMP and GRACE measure the gravity field via precise monitoring of the motion of the satellites; i.e. the satellites themselves function as test masses. JPL's quantum gravity gradiometer employs a quantum phase measurement technique, similar to that employed in atomic clocks, made possible by recent advances in laser cooling and manipulation of atoms. This measurement technique is based on atomwave interferometry, and individual laser-cooled atoms are used as drag-free test masses. The quantum gravity gradiometer employs two identical atom interferometers as precision accelerometers to measure the difference in gravitational acceleration between two points (Figure 1). By using the same lasers for the manipulation of atoms in both interferometers, the accelerometers have a common reference frame and non-inertial accelerations are effectively rejected as common mode noise in the differential measurement of the gravity gradient. As a result, the dual atom interferometer-based gravity gradiometer allows gravity measurements on a moving platform, while achieving the same long-term stability of the best atomic clocks. In the laboratory-based prototype (Figure 2), the cesium atoms used in each atom interferometer are initially collected and cooled in two separate magneto-optic traps (MOTs). Each MOT, consisting of three orthogonal pairs of counter-propagating laser beams centered on a quadrupole magnetic field, collects up to 10(exp 9) atoms. These atoms are then launched vertically as in an atom fountain by switching off the magnetic field and introducing a slight frequency shift between pairs of lasers to create a moving rest frame for the trapped atoms. While still in this moving-frame molasses, the laser frequencies are further detuned from the atomic resonance (while maintaining this relative frequency shift) to cool the atom cloud's temperature to 2 K or below, corresponding to an rms velocity of less than 2 cm/s. After launch, the cold atoms undergo further state and velocity selection to prepare for atom interferometry. The atom interferometers are then realized using laser-induced stimulated Raman transitions to perform the necessary manipulations of each atom, and the resulting interferometer phase is measured using laser-induced fluorescence for state-normalized detection. More than 20 laser beams with independent controls of frequency, phase, and intensity are required for this measurement sequence. This instrument can facilitate the study of Earth's gravitational field from surface and air vehicles, as well as from space by allowing gravity mapping from a low-cost, single spacecraft mission. In addition, the operation of atom interferometer-based instruments in space offers greater sensitivity than is possible in terrestrial instruments due to the much longer interrogation times available in the microgravity environment. A space-based quantum gravity gradiometer has the potential to achieve sensitivities similar to the GRACE mission at long spatial wavelengths, and will also have resolution similar to GOCE for measurement at shorter length scales.

Yu, Nan↗
NASA NTRS2011

Enhancement of Otolith Specific Ocular Responses Using Vestibular Stochastic Resonance

Introduction: Astronauts experience disturbances in sensorimotor function after spaceflight during the initial introduction to a gravitational environment, especially after long-duration missions. Our goal is to develop a countermeasure based on vestibular stochastic resonance (SR) that could improve central interpretation of vestibular input and mitigate these risks. SR is a mechanism by which noise can assist and enhance the response of neural systems to relevant, imperceptible sensory signals. We have previously shown that imperceptible electrical stimulation of the vestibular system enhances balance performance while standing on an unstable surface. Methods: Eye movement data were collected from 10 subjects during variable radius centrifugation (VRC). Subjects performed 11 trials of VRC that provided equivalent tilt stimuli from otolith and other graviceptor input without the normal concordant canal cues. Bipolar stochastic electrical stimulation, in the range of 0-1500 microamperes, was applied to the vestibular system using a constant current stimulator through electrodes placed over the mastoid process behind the ears. In the VRC paradigm, subjects were accelerated to 216 deg./s. After the subjects no longer sensed rotation, the chair oscillated along a track at 0.1 Hz to provide tilt stimuli of 10 deg. Eye movements were recorded for 6 cycles while subjects fixated on a target in darkness. Ocular counter roll (OCR) movement was calculated from the eye movement data during periods of chair oscillations. Results: Preliminary analysis of the data revealed that 9 of 10 subjects showed an average increase of 28% in the magnitude of OCR responses to the equivalent tilt stimuli while experiencing vestibular SR. The signal amplitude at which performance was maximized was in the range of 100-900 microamperes. Discussion: These results indicate that stochastic electrical stimulation of the vestibular system can improve otolith specific responses. This will have a significant impact on development of vestibular SR delivery systems to aid recovery of function in astronauts after long-duration spaceflight or in people with balance disorders.

Fiedler, Matthew↗
DOE OSTI2021

Intra-Molecular Isotope Study of Light Hydrocarbons

Light hydrocarbons (C 1 -C 10 ) are the largest fraction of petroleum hydrocarbons and some of the most ubiquitous and mobile fluids within sedimentary basins. It has been increasingly recognized that hydrocarbons of varying chain-lengths can be stable even under mantle conditions and that their fluxes may play a key role in the carbon dynamics of the Earth. Major formation mechanisms of these light hydrocarbons include microbial, thermogenic, and abiogenic origins. Despite their proven utility, conventional approaches using the bulk or global stable isotopes of light hydrocarbons are often not sufficient to distinguish their sources (particularly, biogenic vs. abiogenic), maturation stages/temperatures, and migration-degradation processes. Most natural compounds, including light hydrocarbons, are composed of a set of diverse isotopic molecules that differ in the number of isotopic substitutions and/or positions of isotopic substitution within a given molecules. Many of light hydrocarbon molecules contain hydrogen and carbon in energetically non-equivalent positions: isotopomers or position-specific (intra-molecular) isotope fractionation. Position-specific isotopic compositions can differ due either to equilibrium or to path-dependent kinetic or biological processes. Thus, the position-specific isotopic fractionation between different carbon and hydrogen positions within a single molecular compound could be used regardless of their reactants and other products. We hypothesize that the formation, transport and degradation processes of light hydrocarbons in the subsurface induce and control significant, perhaps unique position-specific 13 C/ 12 C and 2 H/ 1 H isotope fractionation. In this proposal, we propose to develop a new dimension in stable isotope geochemistry of light hydrocarbons: intra-molecular isotope study of light hydrocarbons. The specific objectives of our proposal include: (a) develop robust and routine quantitative nuclear magnetic resonance (NMR) methods for high-precision/high-accuracy isotopomer analysis of propane and other light hydrocarbons (C 3 -C 10 ), (b) gain a first clear picture on position-specific δ 2 H and δ 13 C values of select light hydrocarbons of both natural and industrial sources, including samples of natural gases (C 3 and possibly C 4 -C 5 ) collected from select sedimentary basins with conventional and unconventional reservoirs, (c) acquire information on position-specific 13 C/ 12 C and 2 H/ 1 H isotope fractionation of light hydrocarbons in key natural processes (thermogenic formation and oxidative degradation) based on well-controlled laboratory experiments, and (d) establish a general framework for interpreting/modeling position-specific 13 C/ 12 C and 2 H/ 1 H isotope compositions of light hydrocarbons. Intra-molecular isotope study of light hydrocarbons is expected to open up great potentials that the bulk and position-specific isotope fractionation of light hydrocarbons, in combination with mathematical/theoretical kinetic models, could provide unprecedented wealth of information on the sources, transport, and sinks of light hydrocarbons in sedimentary basins and deep Earth.

03 NATURAL GAS↗
DOE OSTI2023

Study of e+e- → γΦJ/ψ from $\sqrt{s}$ = 4.600 to 4.951 GeV

Using data samples with an integrated luminosity of 6.4 fb -1 collected by the BESIII detector operating at the BEPCII storage ring, the process of e+e- → γΦJ/ψ is studied. The processes of e + e - → Φχc1,c2, χc1,c2 → γJ/ψ are observed with a significance of more than 10σ. The √s-dependent cross section of e + e - → Φχc1,c2 is measured between 4.600 and 4.951 GeV, and evidence of a resonance structure is found for the first time in the Φχc2 process. We also search for the processes of e + e - → γX(4140), γX(4274) and γX(4500) via the γΦJ/ψ final state, but no obvious structures are found. The upper limits on the production cross section times the branching fraction for these processes at the 90% confidence level are reported.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2020

Development of FRET clusters for CBRN Detection

Advanced sensor capabilities for the simultaneous on-site detection of specific chemical, biological, and radiological/nuclear (CBRN) threats is important to significantly limit the risk of exposure to personnel and allow the rapid collection of essential scientific data and critical evidence. Commercially available sensor capabilities are generally complex, and/or require highly specific and ultra-sensitive methods that are often power demanding or require offsite post-analysis for positive detection, leaving personnel vulnerable. The goal of this project is to develop a portable sensor capable of simultaneously detecting CBRN signatures using a multiplexed Förster Resonance Energy Transfer (FRET) based sensor. FRET sensors are tailorable, specific, and highly dependent on the donor-acceptor distance. In this project, nanoparticles were functionalized with aptamers that were designed for the detection of methylphosphonate, a sarin metabolite. FRET was measured between quantum dot donors and dye and metal nanoparticle acceptors using optical spectroscopy.

61 RADIATION PROTECTION AND DOSIMETRY↗
DOE OSTI2021

Proton Nuclear Magnetic Resonance (H NMR) of Glycolate in Real Waste: Developing and Testing Analytical Methods for the Savannah River Site Liquid Waste System

In preparation for implementing the NG acid flowsheet for the SRS LWS, analytical methods for determining glycolate at low concentration are desired to support system management and safety. Previous work documented that the IC method performed well for samples with low to moderate ionic strength. That work also included a scoping effort to determine if an alternate analytical strategy using H NMR would complement and extend the capabilities of the IC method. The H NMR scoping results indicated that the method had the potential to expand glycolate analysis in LWS samples to higher ionic strength tanks/solutions. The scope of this work is to develop innovative proton NMR techniques, including demonstrating ion exchange decontamination protocols needed for application of the technique to real waste samples. Part of radioactive waste processing at SRS uses formic acid to reduce oxidized (Hg 2+ ) to more volatile elemental Hg for steam striping, collecting, and disposal. Under acidic conditions found in the Chemical Processing Cell (CPC) at the Defense Waste Processing Facility (DWPF), formic acid has a much higher hydrogen generation rate than an alternative reductant, glycolic acid. Thus, an NG acid flowsheet has been developed utilizing glycolic acid with the benefit of easing the need for headspace monitoring requirements for hydrogen and ammonia at DWPF. Low concentrations of glycolate are conservatively assumed to be in the recycle stream, which will collect in the Recycle Collection Tank (RCT). The DWPF recycle stream collected in the RCT has a distinct pathway to the LWS waste tanks that feed the 2H and 3H Evaporator. This route involves transfer of the DWPF recycle to Tank 22 in the Concentration, Storage, and Transfer Facilities (CSTF) followed by transfer to the LWS tank farm/evaporators.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
DOE OSTI2020

Large Polarons as Key Quasiparticles in SrTiO 3 and SrTiO 3 -Based Heterostructures

Despite its simple structure and low degree of electronic correlation, SrTiO 3 (STO) features collective phenomena linked to charge transport and, ultimately, superconductivity, that are not yet fully explained. Thus, a better insight into the nature of the quasiparticles shaping the electronic and conduction properties of STO is needed. We studied the low-energy excitations of bulk STO and of the LaAlO 3 / SrTiO 3 two-dimensional electron gas (2DEG) by Ti L 3 edge resonant inelastic x-ray scattering. In all samples, we find the hallmark of polarons in the form of intense d d + phonon excitations, and a decrease of the LO3-mode electron-phonon coupling when going from insulating to highly conducting STO single crystals and heterostructures. Overall, both results are attributed to the dynamic screening of the large polaron self-induced polarization, showing that the low-temperature physics of STO and STO-based 2DEGs is dominated by large polaron quasiparticles.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2023

Fermilab’s Muon Campus: Status, Experiments, and Future

The Fermilab Muon Campus, repurposed Tevatron-era Antiproton Source facilities, is currently the home to the g-2 and Mu2e muon experiments. Collecting data since 2017, the g-2 experiment is wrapping up a final run before the Muon Campus transitions to Mu2e operation. Currently in the commissioning process, the Mu2e experiment is expected to begin calibration and data collection in fiscal year 2024. A majority of the Muon Campus is shared between the two experiments, however the modes of operation for each are significantly different. An 8 GeV primary proton beam strikes a target to produce a 3.1 GeV/c secondary muon beam for g-2, while the Mu2e experiment uses the Delivery Ring, formerly the Antiproton Accumulator Ring, for a pulsed, resonantly extracted, 8 kW, 8 GeV proton beam incident on a target in the experiment's target hall to produce a muon beam for the experiment. The design and current state of the Muon Campus and the current and future plans of the g-2 and Mu2e experiments, including the transition between operating modes, will be presented.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2020

Measurement of the Photon Beam Asymmetry in yP -> K+S0 at Ey=8.5 GeV with GlueX

In this work the photon beam asymmetry Sigma for the reaction yp ? K+S0 (1193) is measured using the GlueX experiment in Hall D at Jefferson Lab. The analysis used data that were collected using a linearly polarized photon beam in the energy range (8.2 - 8.8) GeV incident on a liquid hydrogen target. The beam asymmetries are measured as a function of the Mandelstam variable t and as a single value for the low u region. These are the first exclusive measurements of the photon beam asymmetry Sigma in this reaction at energies above the baryon resonance region. For the t-channel, results are close to unity and show that the reaction is dominated by the natural-parity exchange of the K? (892) Regge trajectory as predicted by theoretical models. A value of Sigma = 0.410±0.090 is obtained for the u-channel and suggests the exchange of both Sigma(J = 1/2) and Y*(J = 3/2) trajectory contributions to the production of K+S0.

Wickramaarachchi, Nilanga↗
NASA NTRS2010

Miniature Low-Mass Drill Actuated by Flextensional Piezo Stack

Recent experiments with a flextensional piezoelectric actuator have led to the development of a sampler with a bit that is designed to produce and capture a full set of sample forms including volatiles, powdered cuttings, and core fragments. The flextensional piezoelectric actuator is a part of a series of devices used to amplify the generated strain from piezoelectric actuators. Other examples include stacks, bimorphs, benders, and cantilevers. These devices combine geometric and resonance amplifications to produce large stroke at high power density. The operation of this sampler/drill was demonstrated using a 3x2x1-cm actuator weighing 12 g using power of about 10-W and a preload of about 10 N. A limestone block was drilled to a depth of about 1 cm in five minutes to produce powdered cuttings. It is generally hard to collect volatiles from random surface profiles found in rocks and sediment, powdered cuttings, and core fragments. Toward the end of collecting volatiles, the actuator and the bit are covered with bellows-shaped shrouds to prevent fines and other debris from reaching the analyzer. A tube with a miniature bellows (to provide flexibility) is connected to the bit and directs the flow of the volatiles to the analyzer. Another modality was conceived where the hose is connected to the bellows wall directly to allow the capture of volatiles generated both inside and outside the bit. A wide variety of commercial bellows used in the vacuum and microwave industries can be used to design the volatiles capture mechanism. The piezoelectric drilling mechanism can potentially be operated in a broad temperature range from about-200 to less than 450 C. The actuators used here are similar to the actuators that are currently baselined to fly as part of the inlet funnel shaking mechanism design of MSL (Mars Science Laboratory). The space qualification of these parts gives this drill a higher potential for inclusion in a future mission, especially when considering its characteristics of low mass, small size, low power, and low axial loads for sampling.

Sherrit, Stewart↗
DOE OSTI2022

Thermal scattering law for structure-dependent-Doppler broadening in FLASSH

Traditional Doppler broadening methods assume that target nuclei velocities follow a Maxwell-Boltzmann distribution which inherently assumes that the atoms are a free gas or that their velocities are independent of each other. This approximation is reasonable at high target temperatures and high neutron energies. However, nuclei are not independent: the lattice temperature and chemical binding will define the atomic motion. The thermal scattering law (i.e., TSL or S(α,β)) is a material property which describes the chemical binding and temperature response in terms of available momentum and energy states. In the thermal energy range, this TSL will define the thermal scattering cross sections. In the resonance region, the TSL offers a first-principles description of the probability distribution function for the velocity of the target nuclei. Using the TSL in Doppler broadening captures the structure of the material consistently from the thermal range into the resonance cross sections. In this work, both traditional free-gas and precise TSL Doppler broadening methods for resonance cross section evaluation have been implemented within the Full Law Analysis Scattering System Hub (FLASSH). This framework provides a generalized formulation for evaluating low-lying resonance data and streamlines nuclear data processing methods. TSL data generated using ab initio lattice dynamics (AILD) can be used to broaden cross section libraries in ENDF format for high-fidelity input into reactor physics calculations. These capabilities are demonstrated for the lowest absorption resonances of {sup 238}U in UO{sub 2}, UC and UN. (authors)

22 GENERAL STUDIES OF NUCLEAR REACTORS↗