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At least 523 records · Page 29

Uncertainty Quantification of Global Net Methane Emissions From Terrestrial Ecosystems Using a Mechanistically Based Biogeochemistry Model

Quantification of methane (CH4) emissions from wetlands and its sinks from uplands is still fraught with large uncertainties. Here, a methane biogeochemistry model was revised, parameterized, and verified for various wetland ecosystems across the globe. The model was then extrapolated to the global scale to quantify the uncertainty induced from four different types of uncertainty sources including parameterization, wetland type distribution, wetland area distribution, and meteorological input. We found that global wetland emissions are 212 ± 62 and 212 ± 32 Tg CH4 year -1 (1Tg = 10 12 g) due to uncertain parameters and wetland type distribution, respectively, during 2000–2012. Using two wetland distribution data sets and three sets of climate data, the model simulations indicated that the global wetland emissions range from 186 to 212 CH 4 year -1 for the same period. The parameters were the most significant uncertainty source. After combining the global methane consumption in the range of -34 to -46 Tg CH 4 year -1 , we estimated that the global net land methane emissions are 149–176 Tg CH 4 year -1 due to uncertain wetland distribution and meteorological input. Spatially, the northeast United States and Amazon were two hotspots of methane emission, while consumption hotspots were in the Eastern United States and eastern China. During 1950–2016, both wetland emissions and upland consumption increased during El Niño events and decreased during La Niña events. This study highlights the need for more in situ methane flux data, more accurate wetland type, and area distribution information to better constrain the model uncertainty.

58 GEOSCIENCES↗

Improving a Multilevel Turbulence Closure Model for a Shallow Lake in Comparison With Other 1-D Models

Lakes differ from lands in water availability, heat capacity, albedo, and roughness, which affect local surface-atmospheric interactions. This study modified a multilevel upper ocean model (UOM) for lake applications and evaluated its performance in Lake Taihu (China) with comprehensive measurements against three popular one-dimensional (1-D) lake models. These models were based on different concepts, including the self-similarity (FLake), the wind-driven eddy diffusion (LISSS), the k-ε turbulence closure (SIMSTRAT), and a simplified turbulence closure (UOM). The surface flux scheme in these models was unified to exclude the discrepancies in representing air-lake exchanges. All models in their default formulations presented obvious cold water temperature biases and largely underestimated the lake surface temperature (LST) diurnal range. For each model, these deficiencies were significantly reduced by incorporating new physics schemes or calibrated tunable parameters based on systematic sensitivity tests. The primary modifications for UOM included (1) a new scheme of decreased surface roughness lengths to better characterize the shallow lake, (2) a solar radiation penetration scheme with increased light extinction coefficient and surface absorption fraction to account for the high water turbidity, and (3) turbulent Prandtl number increased by a factor of 20 to reduce the turbulent vertical mixing. All other models were improved in these three aspects (roughness, extinction, and mixing) within their original formulations. Given these improvements, UOM showed superior performance to other models in capturing LST diurnal cycle and daily to seasonal variations, as well as summer-autumn vertical stratification changes. The new UOM is well suited for application in shallow lakes.

54 ENVIRONMENTAL SCIENCES↗

Regional MJO Modulation of Northwest Pacific Tropical Cyclones Driven by Multiple Transient Controls

The Madden–Julian Oscillation (MJO) is widely acknowledged for its ability to modulate Northwest Pacific tropical cyclones (TCs), but a complete understanding of the underlying mechanisms remains uncertain. Beyond established effects of the MJO's relative humidity envelope, other dynamical factors have recently been invoked via new genesis potential indices and high-resolution modeling studies. Here we revisit the ability of the MJO to modulate West Pacific TCs through a quasi-explicit cyclone downscaling strategy driven by composited observations, paired later with a genesis index to investigate regional drivers of modulation. In this work, we reveal two distinct spatial modes of TC modulation in which the MJO's dynamic and thermodynamic effects act in tandem to increase TCs. In the South China Sea, for instance, shear reductions associated with the MJO's circulation lead to increasing potential intensity ahead of the arrival of a positive humidity anomaly, all of which combine for an extended period of cyclogenesis favorability.

58 GEOSCIENCES↗

Parameterizing Subgrid Variations of Land Surface Heat Fluxes to the Atmosphere Improves Boreal Summer Land Precipitation Simulation With the NCAR CESM1.2

Subgrid horizontal variations of land surface heat fluxes to the atmosphere resulting from subgrid land cover heterogeneity are important in land-atmosphere interaction in global climate models (GCMs). To incorporate it, a parameterization using stochastic sampling based on truncated normal distributions diagnosed from the land model and internal ensemble mean of multiple calls to the planetary boundary layer and deep convection schemes is developed. After its implementation in the National Center for Atmospheric Research (NCAR) Community Earth System Model version 1.2 (CESM1.2), large changes of simulated land precipitation are found to occur in regions where large subgrid variations of surface heat fluxes exist. The simulated precipitation is improved in boreal summer, especially over eastern China and the coastal areas of the Bay of Bengal. The improved precipitation is mainly a result of improved large-scale moisture convergence and advection by altered vertical diffusion and convection.

58 GEOSCIENCES↗

A Global High‐Resolution Mesoscale Convective System Database Using Satellite‐Derived Cloud Tops, Surface Precipitation, and Tracking

Abstract A new methodology is developed to construct a global (60°S–60°N) long‐term (2000–2019) high‐resolution (∼10‐km h) mesoscale convective system (MCS) database by tracking MCS jointly using geostationary satellite infrared brightness temperature ( T b ) and precipitation feature (PF) characteristics from the Integrated Multi‐satellitE Retrievals for GPM precipitation data sets. Independent validation shows that the satellite‐based MCS data set is able to reproduce important MCS statistics derived from ground‐based radar network observations in the United States and China. We show that by carefully considering key PF characteristics in addition to T b signatures, the new method significantly improves upon previous T b ‐only methods in detecting MCSs in the midlatitudes for all seasons. Results show that MCSs account for over 50% of annual total rainfall across most of the tropical belt and in selected regions of the midlatitudes, with a strong seasonality over many regions of the globe. The tracking database allows Lagrangian aspects such as MCS lifetime and translational speed and direction to be analyzed. The longest‐lived MCSs preferentially occur over the subtropical oceans. The land MCSs have higher cloud‐tops associated with more intense convection, and oceanic MCSs have much higher rainfall production. While MCSs are observed in many regions of the globe, there are fundamental differences in their dynamic and thermodynamic structures that warrant a better understanding of processes that control their evolution. This global database provides significant opportunities for observational and modeling studies of MCSs, their characteristics, and roles in regional and global water and energy cycles, as well as their hydrologic and other impacts.

54 ENVIRONMENTAL SCIENCES↗

Assimilation of X-band Phased-Array Radar Data with EnKF for the Analysis and Warning Forecast of a Tornadic storm

The impact of assimilating China's operational X-band Phased-Array radar's (X-PAR) data on the analysis and warning forecast of the vortex structure and intensity of the June 8, 2018 Foshan, Guangdong province, tornadic storm was investigated for the first time using an Ensemble Kalman Filter (EnKF) data assimilation system. Both radar radial velocity (Vr) and reflectivity (Z) from two S-band operational radars and one X-PAR were assimilated. Deterministic forecasts were launched every 6 min from 05:42 UTC (20 min before the tornado touched down) to 06:00 UTC from the EnKF mean analysis field. Five experiments were conducted to examine the added capability of Z assimilation of the EnKF system, and to investigate the impact of assimilating X-PAR data on the analysis and prediction of the tornadic storm. Compared to the experiment without Z assimilation, the assimilation of Z reduced the analysis error and greatly reduced the forecast error of Z. Furthermore, the assimilation of X-PAR data greatly improved the vortex structure of the tornadic storm at low levels, and improved the intensity of the rear inflow of the tornadic storm, especially with a higher assimilation frequency. Compared to the experiments without X-PAR data assimilation, assimilating X-PAR data improved the predictability of tornadic storm.

54 ENVIRONMENTAL SCIENCES↗

Contrasting Responses of Soil Inorganic Carbon to Afforestation in Acidic Versus Alkaline Soils

Afforestation is recommended as an effective approach for carbon sequestration and environmental benefits. However, it remains less clear, and sometimes controversial, regarding how afforestation may impact soil inorganic carbon (SIC), a crucial component of the ecosystem carbon pool. Here, using field data from 619 afforested plots and 163 control plots across northern China, we investigated the relative and absolute differences in SIC between afforested and corresponding control plots. Our results suggested that afforestation increased SIC in acidic soils, while decreased SIC in alkaline soils. Fitting a linear mixed model and further a structure equation model, we found that afforestation-induced soil pH change was the most significant factor regulating SIC responses. In particular, SIC was more sensitive to pH change in more arid areas, where both soil pH and SIC stocks were high. Other factors could indirectly affect SIC responses to afforestation through modulating soil pH and soil organic carbon (SOC) dynamics. Moreover, afforestation-induced SIC changes also varied considerably among different species of tree plantations and across different soil depths. Importantly, in plantations of Pinus sylvestris var. mongholica, Pinus tabuliformis, and Populus spp., changes in SIC caused by afforestation were even comparable to that in SOC. Overall, our findings provide a data-based understanding on the comprehensive soil carbon dynamics following afforestation and its underlying mechanisms. With the increased use of afforestation and reforestation as nature-based solutions to climate change, their associated impacts on SIC need to be taken into account, especially in SIC-rich areas.

54 ENVIRONMENTAL SCIENCES↗

New Insights Into Error Decomposition for Precipitation Products

Abstract It is very important to quantify errors of precipitation estimation products. However, the existing methods do not describe all error components and are therefore not comprehensive enough. In this study, we propose a four‐component error decomposition method (4CED) that decomposes the total errors of precipitation products into four independent parts: hit positive bias, hit negative bias, false bias, and missed bias. And we use it to evaluate the performance of the three latest satellite precipitation products in the eastern monsoon region of China. Our study reveals 4CED has apparent improvements compared with the previous method. Results also provide new insights for tracking error sources and quantifying the error magnitudes of precipitation products. Moreover, the proposed 4CED can be extended to different spatial and temporal scales. Our new method will not only contribute to product upgrades, but also provide guidance for potential applications.

58 GEOSCIENCES↗

Impacts of Suppressing Excessive Light Rain on Aerosol Radiative Effects and Health Risks

Global climate models (GCMs) have been used widely to study radiative forcing and health risks of aerosols. A recent study using two GCMs found that light rain plays a dominant role in controlling aerosol loading. However, “too much light rain and too little heavy rain” is a longstanding bias in GCMs. It is unclear how much light rain affects aerosol-cloud-radiation interactions and health risks from air pollution. Here, in this work, we show that, with the correction of the rainfall intensity spectrum in the National Center for Atmospheric Research Community Atmosphere Model version 5.3 by introducing a stochastic deep convection scheme, the reduced frequency of light rain (1–20 mm d -1 ) results in changes of aerosol direct radiative effects (DRE) of up to -0.5 ± 0.03 W/m 2 and aerosol cloud radiative effects (CRE) of up to -0.9 ± 0.03 W/m 2 . The total (CRE + DRE) radiative effects of light rain-mediated aerosol changes exceed the present-day anthropogenic forcing of aerosols relative to preindustrial levels from the Coupled Model Intercomparison Project (CMIP5&6) models. However, the correction of the rainfall intensity spectrum has little effect on anthropogenic aerosol forcing (defined as the radiative perturbation due to changes in aerosol concentrations between the industrial era and preindustrial levels). Due to increased exposure to fine particulates (PM 2.5 ), the estimated global total premature mortality is much higher than previously estimated, by 300,000 ± 60,000 deaths per year, and is more severe in populous regions such as India and China. The findings in this study highlight the need to understand uncertainties in radiative effects and health risks of aerosols due to simulation biases of precipitation in GCMs.

54 ENVIRONMENTAL SCIENCES↗

Occurrence of Warm Freezing Rain: Observation and Modeling Study

Freezing rain has been normally considered to be composed of supercooled raindrops when the 2 m air temperature (hereafter T as ) is below freezing. However, according to a statistical survey of freezing rain observations in China from 2000 to 2019, we find that there were 656 events that occurred at T as greater than 0°C (hereafter warm freezing rain and denoted by WFR), which account for 7% of the total freezing rain observations. Additionally, nearly 3% (266 observations) of freezing rain events occurred when the near-surface wet-bulb temperature was greater than 0°C. The modeling and sensitivity experiments on the nonequilibrium raindrop temperature (hereafter T r ) how that the temperature difference between raindrops and the atmosphere is the main cause of WFR. The magnitudes of the Δ T ar (difference between raindrop temperature T r and air temperature T a ) and Δ T ur (difference between T r and wet-bulb temperature T w ) are determined by the raindrop diameter D, temperature lapse rate $\Gamma$, and relative humidity RH. Increases of D and $\Gamma$, and a decrease of RH enhance Δ T ar and Δ T ur and thus the occurrence of WFR. Further simulations of 4 idealized and 370 real sounding profiles reveal that either the T a or the T w cannot properly distinguish the WFR events. When considering the temperature difference between raindrops and the atmosphere, the WFR can form by the “melting of solid hydrometeors” or “supercooled warm rain process.” This study can also deepen our understanding of the conditions of WFR and freezing rain formation at different altitudes.

54 ENVIRONMENTAL SCIENCES↗

Multiscale Simulation of Precipitation Over East Asia by Variable Resolution CAM-MPAS

This study evaluates the precipitation over East Asia simulated by the variable resolution CAM-MPAS featuring the Model for Prediction Across Scales (MPAS) atmospheric dynamical core coupled with the physics parameterizations of the Community Atmosphere Model (CAM) version 5.4. Two CAM-MPAS experiments, one with a global quasi-uniform resolution mesh of 120 km (MPAS-UR) and the other with a variable resolution mesh of 30 to 120 km refined over East Asia (MPAS-VR), are conducted from 1989 to 2005 following the Atmospheric Model Intercomparison Project protocol. Two regional climate model simulations at ~25 km resolution from the Coordinated Regional Downscaling Experiment East Asia second plan are also analyzed for comparison. Results show that CAM-MPAS performs better than the selected regional models in simulating the precipitation climatology over East Asia. Compared with MPAS-UR, MPAS-VR with refinement over East Asia better simulates the precipitation over and around the Tibetan Plateau (TP), the frequency distribution of light, moderate, and heavy precipitation in various regions of China, and the interannual precipitation pattern associated with the East Asian summer monsoon. The improvements in MPAS-VR relative to MPAS-UR largely come from the decreased grid spacing rather than the use of finer-scale terrain information. Particularly, decreased grid spacing is more essential for simulating the precipitation magnitude over TP and the location of peak precipitation south of TP, likely due to the better resolved physical and dynamical processes associated with orographic precipitation. The 30-120 km CAM-MPAS model is shown to be a promising tool for precipitation simulation over East Asia.

54 ENVIRONMENTAL SCIENCES↗

Response of Extreme Rainfall to Atmospheric Warming and Wetting: Implications for Hydrologic Designs Under a Changing Climate

Understanding the processes of rainfall extremes and their response to anthropogenic climate change is pivotal for improved adaptation of unprecedented flood hazards around the world. Here we take the record-breaking 20 July 2021 storm over central China as an example. We investigate the response of this particular storm to atmospheric warming (i.e., increase in air temperature) and wetting (i.e., increase in atmospheric moisture content) based on a series of convection-permitting model simulations. Our results show non-monotonic changes of the space-time rainfall variability to either increased temperature or atmospheric moisture content. The most extreme rain rate is produced when relative humidity is increased by 20~40 % or temperature is increased by less than 2°C. The non-monotonic rainfall response is more clearly revealed at fine spatial (100-1000 km 2 ) and temporal scales (less than 6 hours) rather than over the entire domain (~10 4 km 2 ) and aggregated over the storm duration (around two days). This is mainly attributable to the distinct feedbacks from atmospheric dynamics (i.e., moisture convergence and interaction with regional topography) rather than regulated by thermodynamic changes alone. Furthermore, atmospheric warming poses notable changes in the vertical structure of storm cells, contributing to reduced areal reduction factors at small spatial scales and short durations, while atmospheric wetting additionally modifies storm evolution properties. Our modeling analyses challenge the existing practices for hydrologic designs under a changing climate, highlighting particular vulnerability for cities or small basins to short-duration rainfall extremes and the resultant flash flood hazards.

54 ENVIRONMENTAL SCIENCES↗

Incorporating the Effect of Large‐Scale Vertical Motion on Convection Through Convective Mass Flux Adjustment in E3SMv2

Abstract Recent observational studies suggest that the large‐scale dynamical forcing (vertical motion) plays important roles in deep convection development. In this study we propose a convective mass flux adjustment (MAdj) approach to represent the dynamical effects of large‐scale vertical motion on convection in the Department of Energy's Energy Exascale Earth System Model version 2 (E3SMv2). With MAdj, convection is enhanced (suppressed) when there is large‐scale ascending (descending) motion at the planetary boundary layer top. The coupling of convection with large‐scale circulation significantly improves the simulation of climate variability in E3SMv2 across multiple scales from the diurnal cycle, convectively coupled equatorial waves, to the Madden‐Julian Oscillation (MJO). The standard E3SMv2 tends to simulate overly weak diurnal amplitude of precipitation and overly weak variance of convectively coupled equatorial Kelvin and westward inertio‐gravity (WIG) waves. It also fails to simulate the essential characteristics of the MJO: continuous eastward propagation. With MAdj, the amplitude of diurnal cycle of precipitation is systematically increased and its probability density distribution is much closer to observations. The MAdj can also simulate more realistic eastward propagation of the MJO and much stronger convectively coupled Kelvin and WIG waves. Moreover, the MAdj approach slightly improves the climatology simulations in precipitation, cloud, radiation, circulation, temperature, and moisture fields, with overall root‐mean‐square error (RMSE) of major climatological fields reduced by about 2%. The MAdj approach suppresses excessive grid‐scale precipitation, reducing precipitation wet biases over South China Sea, Philippine Sea, Himalayas, and South Pacific Convergence Zone in western Pacific in summer.

54 ENVIRONMENTAL SCIENCES↗

Isopycnal Submesoscale Stirring Crucially Sustaining Subsurface Chlorophyll Maximum in Ocean Cyclonic Eddies

Abstract Mesoscale and submesoscale processes have crucial impacts on ocean biogeochemistry, importantly enhancing the primary production in nutrient‐deficient ocean regions. Yet, the intricate biophysical interplay still holds mysteries. Using targeted high‐resolution in situ observations in the South China Sea, we reveal that isopycnal submesoscale stirring serves as the primary driver of vertical nutrient transport to sustain the dome‐shaped subsurface chlorophyll maximum (SCM) within a long‐lived cyclonic mesoscale eddy. Density surface doming at the eddy core increased light exposure for phytoplankton production, while along‐isopycnal submesoscale stirring disrupted the mesoscale coherence and drove significant vertical exchange of tracers. These physical processes play a crucial role in maintaining the elevated phytoplankton biomass in the eddy core. Our findings shed light on the universal mechanism of how mesoscale and submesoscale coupling enhances primary production in ocean cyclonic eddies, highlighting the pivotal role of submesoscale stirring in structuring marine ecosystems.

Cao, Haijin↗

Impact of Anthropogenic Aerosol Transport on Cloud Condensation Nuclei Activity During Summertime in Qilian Mountain, in the Northern Tibetan Plateau

Here in this study, we conducted field campaigns at two mountain-top observatories on the Qilian Mountains (QLM) in the northeastern Tibetan Plateau of China, which plays a vital role in sustaining water resources for the downstream arid and semi-arid regions. The two observatories, Waliguan Baseline Observatory (WLG) and Laohugou station (LHG), are situated on the eastern and western edge of the QLM, respectively. The objectives of this study were to examine the properties of atmospheric aerosols, CCN concentrations (NCCN) at varying supersaturation levels (SS = 0.2%–1.0%), and the hygroscopic nature of aerosols in the QLM, especially during the formation of orographic cloud. Notably, the average aerosol concentration and N CCN was approximately 2–3 factors higher at WLG compared to LHG. The chemical compositions of aerosols were primarily dominated by sulfate and organic aerosol (OA) at these two sites. A very high hygroscopicity parameter of aerosol calculated using chemical composition was observed at these two sites (0.37 ± 0.03 at LHG vs. 0.30 ± 0.04 at WLG). Enhanced aerosol loading episodes impacted by anthropogenic emission were observed at these two sites. Exploration on high-loading cases at each site, we found that the CCN activity was dominated by aerosol size, but the chemical processes of aerosol during the formation of orographic cloud could also be important in CCN activity, especially for low SS conditions. These findings collectively underscore the significant impact of anthropogenic air plumes on CCN concentrations in the QLM and their potential influence on precipitation patterns.

54 ENVIRONMENTAL SCIENCES↗

More Heavy Precipitation in World Urban Regions Captured Through a Two‐Way Subgrid Land‐Atmosphere Coupling Framework in the NCAR CESM2

Abstract Current global climate models (GCMs), limited to grid‐scale land‐atmosphere coupling, cannot represent subgrid urban‐rural precipitation contrasts. This study develops an innovative two‐way subgrid land‐atmosphere coupling framework in the National Center for Atmospheric Research (NCAR) Community Earth System Model version 2 (CESM2) to explicitly resolve land‐atmosphere interaction over subgrid individual land units. Results show that urban heat island (UHI) leads to the urban rainfall effect (URE), which in turn alleviates overestimated UHI over China in CESM2. The URE manifests as a shift toward more heavy precipitation and less light precipitation in world urban areas than in surrounding rural counterparts. This feature is consistent with available observations. In heavy precipitation situations, the UHI promotes atmospheric instability and enhances atmospheric water vapor holding capacity, resulting in more heavy precipitation in urban areas. Conversely, in light precipitation situations, the UHI and decreased evaporation from urban impermeable surfaces diminish atmospheric relative humidity, suppressing light precipitation.

Geology↗

Photolytic Degradation of Water‐Soluble Organic Carbon in Snowmelts: Changes in Molecular Characteristics, Brown Carbon Chromophores, and Radiative Effects

Abstract Water‐soluble organic carbon (WSOC) deposited in ambient snowpack play key roles in regional carbon cycle and surface energy budget, but the impacts of photo‐induced processes on its optical and chemical properties are poorly understood yet. In this study, melted samples of the seasonal snow collected from northern Xinjiang, northwestern China, were exposed to ultraviolet (UV) radiation to investigate the photolytic transformations of WSOC. Molecular characteristics and chemical composition of WSOC and its brown carbon (BrC) constituents were investigated using high‐performance liquid chromatography interfaced with a photodiode array detector and a high‐resolution mass spectrometer. Upon illumination, formation of nitrogen‐ and sulfur‐containing species with high molecular weight was observed in snow samples influenced by soil‐ and plant‐derived organics. In contrast, the representative sample collected from remote region showed the lowest molecular diversity and photolytic reactivity among all samples, in which no identified BrC chromophores decomposed upon illumination. Approximately 65% of chromophores in urban samples endured UV irradiation. However, most of BrC composed of phenolic/lignin‐derived compounds and flavonoids disappeared in the illuminated samples containing WSOC from soil‐ and plant‐related sources. Effects of the photochemical degradation of WSOC on the potential modulation of snow albedo were estimated. Apparent half‐lives of WSOC estimated as albedo reduction in 300–400 nm indicated 0.1–0.4 atmospheric equivalent days, which are shorter than typical photolysis half‐lives of ambient biomass smoke aerosol. This study provides new insights into the roles of WSOC in snow photochemistry and snow surface energy balance.

Meteorology & Atmospheric Sciences↗

Impact of Orographic Drag Schemes on East Asia Rainfall

Current generation of climate models often has significant biases in mountainous regions where the gradient of elevation is steep, and the terrain is complex. Potential reasons for these biases include under‐representation of orographic drag process in climate models. In this study, we assess the impact of orographic drag on East Asia rainfall by comparing the impact of a new orographic drag scheme that considers 3D orographic anisotropy (3D‐oro) with a 2‐D scheme in a general circulation model. Two sets of simulations (medium‐range and seasonal forecast) are carried out for the comparison and validation against observation. It is shown that through local/remote forcing of the drag in the mountainous regions, the 3D‐oro alleviates part of the excessive rainfall in west Tibetan Plateau and parts of insufficient rainfall in Southeast China by about 25%∼50% in the January/winter forecasts; it alleviates about 25%∼50% of the rainfall bias in part of south Tibetan Plateau and of East Asia in the July/summer forecasts. The results suggest the importance of improved orographic drag process and its impact in climate modeling for those regions that are prone to significant impact of hydroclimate events.

orographic anisotropy↗