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At least 505 records · Page 28

Fast estimation of dense gas dispersion from multiple continuous CO 2 surface leakage sources for risk assessment

Surface leakage of CO 2 , and associated potential impacts on health, safety, and the environment (HSE) are considered hazards of geologic carbon sequestration (GCS). There are two challenges associated with impact assessment of CO 2 surface dispersion. First, the fact that CO 2 is a dense gas makes its dispersion in air a complex process. Rigorous numerical solutions for modeling concentration distributions are relatively time-consuming. Second, impact assessment requires consideration of uncertainty, e.g., quantification of how much uncertainty is propagated through input parameters to model outputs by carrying out large numbers of model runs. In order to assess the potential consequences of surface leakage of CO 2 , it is useful to have a model that executes very quickly for repeated model calculations (e.g., in Monte Carlo mode) of the atmospheric dispersion of CO 2 (concentrations as a function of space and time). In addition, the model should be able to handle multiple surface leakage sources. In this work, we have extended the nomograph approach of Britter and McQuaid (1988) for estimating dense gas plume length from single leakage source to multiple leakage sources. The method is very fast and therefore amenable to general system-level GCS risk assessment including uncertainty quantification within the framework of the National Risk Assessment Partnership (NRAP) Integrated Assessment Model (IAM). The method is conservative in that it assumes the wind could be from any direction, and it handles multiple sources by a simple superposition approach. The method produces results in reasonable agreement with a sophisticated computational fluid dynamics (CFD) code, but runs in a small fraction of the time.

58 GEOSCIENCES↗

Characterizations of double pulsing in neutron multiplicity and coincidence counting systems

Passive neutron coincidence/multiplicity counters are subject to non-ideal behavior, such as double pulsing and dead time. It has been shown in the past that double-pulsing exhibits a distinct signature in a Rossi-alpha distribution, which is not readily noticed using traditional Multiplicity Shift Register analysis. But, it has been assumed that the use of a pre-delay in shift register analysis removes any effects of double pulsing. Here, we use high-fidelity simulations accompanied by experimental measurements to study the effects of double pulsing on multiplicity rates. By exploiting the information from the double pulsing signature peak observable in the Rossi-alpha distribution, the double pulsing fraction can be determined. Algebraic correction factors for the multiplicity rates in terms of the double pulsing fraction have been developed. We also discuss the role of these corrections across a range of scenarios.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Estimating the mass variance in neutron multiplicity counting $-$ A comparison of approaches

In the standard practice of neutron multiplicity counting, the first three sampled factorial moments of the event triggered neutron count distribution are used to quantify the three main neutron source terms: the spontaneous fissile material effective mass, the relative (α,n) production and the induced fission source responsible for multiplication. This study compares three methods to quantify the statistical uncertainty of the estimated mass: the bootstrap method, propagation of variance through moments, and statistical analysis of cycle data method. Each of the three methods was implemented on a set of four different NMC measurements, held at the JRC-laboratory in Ispra, Italy, sampling four different Pu samples in a standard Plutonium Scrap Multiplicity Counter (PSMC) well counter.

74 ATOMIC AND MOLECULAR PHYSICS↗

Experimental evaluation of the extended Dytlewski-style dead time correction formalism for neutron multiplicity counting

Over the past few decades, neutron multiplicity counting has played an integral role in Special Nuclear Material (SNM) characterization pertaining to nuclear safeguards. Current neutron multiplicity analysis techniques use singles, doubles, and triples count rates because a methodology to extract and dead time correct higher order count rates (i.e. quads and pents) was not fully developed. This limitation is overcome by the recent extension of a popular dead time correction method developed by Dytlewski. This extended dead time correction algorithm, named Dytlewski-Croft-Favalli (DCF), is detailed in reference Croft and Favalli (2017), which gives an extensive explanation of the theory and implications of this new development. Dead time corrected results can then be used to assay SNM by inverting a set of extended point model equations which as well have only recently been formulated. Here, we discuss and present the experimental evaluation of practical feasibility of the DCF dead time correction algorithm to demonstrate its performance and applicability in nuclear safeguards applications. In order to test the validity and effectiveness of the dead time correction for quads and pents, 252 Cf and SNM sources were measured in high efficiency neutron multiplicity counters at the Los Alamos National Laboratory (LANL) and the count rates were extracted up to the fifth order and corrected for dead time. To assess the DCF dead time correction, the corrected data is compared to traditional dead time correction treatment within INCC. In conclusion, the DCF dead time correction is found to provide adequate dead time treatment for broad range of count rates available in practical applications.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Event-by-event neutron–photon multiplicity correlations in 252Cf(sf)

Excited nuclear fragments are emitted during nuclear fission. The de-excitation of these fission fragments takes place as sequential emission of neutrons followed by photons. A correlation between neutron and photon multiplicities accompanying fission is thus expected. Fission event generators based on established statistical nuclear physics models predict a negative event-by-event correlation in neutron-photon multiplicity. A survey of published experimental results of an event-by-event covariance between the neutron - photon multiplicities emitted following the spontaneous fission of 252 Cf is presented. Analytic unfolding expressions are developed in this work to determine the bias introduced by background sources, particle misclassification, pulse pileup, and inelastic photon production. The published experimental data are re-analyzed using these unfolding techniques and are found to be in qualitative agreement with the predictions of model-based calculations. Finally, in particular, we have concluded that there exists a significant event-by-event neutron-photon emission competition following the spontaneous fission of 252 Cf.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

At-power subcritical multiplication in the advanced test reactor

The degree to which a given physical subdivision of a critical reactor acts as a neutron source for other lobes is not analytically characterized for general application. ATR and ATRC both operate at power, and individual power-producing lobes rely on each other as neutron sources in order to maintain constant power, which in general requires either exactly critical multiplication within a reactor or an external neutron source. Here, this work shows that lobe powers in ATR or ATRC can be related with subcritical multiplication theory, demonstrating that the lobes are not individually critical. This explanation is significant for ATR due to the desire to irradiate a large variety of experiments simultaneously, each having its impact on the core neutron population. This work also establishes the lack of relationship between experiment reactivity worth and cross-sections calculated from fundamental nuclear data. For any physical subdivision of any other critical reactor, it is likewise true that the subdivision undergoes only subcritical multiplication.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Unified framework for heavy flavor and quarkonium production in high multiplicity p+p and p+A collisions at RHIC and LHC

We discuss the production of $D$-mesons and $J/\psi$ in high multiplicity proton-proton and proton-nucleus collisions within the Color-Glass-Condensate (CGC) framework. We demonstrate that the modification of the LHC data on $D$ and $J/\psi$ yields in high multiplicity events relative to minimum bias events arise from a significant enhancement of the gluon saturation scales of the corresponding rare parton configurations in the colliding protons and nuclei. For a given event multiplicity, we predict these relative yields to be energy independent from $\sqrt{s}=200$ GeV at RHIC to the highest LHC energies.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Multithreaded sparse matrix-matrix multiplication for many-core and GPU architectures

Sparse matrix-matrix multiplication is a key kernel that has applications in several domains such as scientific computing and graph analysis. Several algorithms have been studied in the past for this foundational kernel. In this work, we develop parallel algorithms for sparse matrix-matrix multiplication with a focus on performance portability across different high performance computing architectures. The performance of these algorithms depend on the data structures used in them. We compare different types of accumulators in these algorithms and demonstrate the performance difference between these data structures. Furthermore, we develop a meta-algorithm, kkSpGEMM, to choose the right algorithm and data structure based on the characteristics of the problem. We show performance comparisons on three architectures and demonstrate the need for the community to develop two phase sparse matrix-matrix multiplication implementations for efficient reuse of the data structures involved.

97 MATHEMATICS AND COMPUTING↗

Theoretical limits of multiple exciton generation and singlet fission tandem devices for solar water splitting

Photoelectrochemical (PEC) water splitting is one of the most important approaches being investigated for solar fuel generation. In this study, we determine the maximum thermodynamic power conversion efficiencies (PCEs) of PEC water splitting two-bandgap tandem devices that produce multiple carriers per photon absorbed via Multiple Exciton Generation (MEG) or Singlet Fission (SF) and in the presence of solar concentration. Here, we employ a detailed balance thermodynamic analysis to determine the effects of top cell thickness, solar concentration, carrier multiplication, electrode overvoltage (VO), and water absorption on PEC power conversion efficiency for water splitting cells. We have found a maximum PEC power conversion efficiency of 62.9% in cells using two ideal tandem MEG absorbers with bandgaps of 0.3 and 1.2 eV at 1000-suns solar concentration and 0 overvoltage; the maximum PCE for two tandem SF absorbers under the same conditions is nearly the same at 59% with the same values for the absorption thresholds. A very interesting and important result was that, upon thinning the top cell, the range of viable bandgaps for both the top and bottom cells is extended by as much as 0.5-1 eV while still maintaining high maximum conversion efficiency (60-63%). The effects of imposing different solar concentrations from 1X to 1000X and having different tandem configurations of SF and MEG layers were also studied.

14 SOLAR ENERGY↗

A Note on the Nomenclature in Neutron Multiplicity Mathematics

The purpose of this technical note is to consolidate the notations used for describing parameters that pertain to neutron multiplicity mathematics relevant to various applications including nonproliferation, international safeguards, and criticality safety among others. The nomenclatures used in these techniques vary widely depending on the origin of the work and their applications. We aim here to consolidate many of the previously used notations in a single document to enhance past, present, and future technical exchanges pertaining to neutron multiplicity. This will help avoid confusion in future publications and will facilitate wider application-independent advancements and utility of peer-reviewed findings. A brief introduction and history of neutron multiplicity counting is presented, followed by a summary of commonly used techniques in a variety of different applications. In each section, we present the notations used in previous publications for the reader’s reference.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

OBSERVATIONS OF HIERARCHICAL SOLAR-TYPE MULTIPLE STAR SYSTEMS

Twenty multiple stellar systems with solar-type primaries were observed at high angular resolution using the PALM-3000 adaptive optics system at the 5 m Hale telescope. The goal was to complement the knowledge of hierarchical multiplicity in the solar neighborhood by confirming recent discoveries by the visible Robo-AO system with new near-infrared observations with PALM-3000. The physical status of most, but not all, of the new pairs is confirmed by photometry in the Ks band and new positional measurements. In addition, we resolved for the first time five close sub-systems: the known astrometric binary in HIP 17129AB, companions to the primaries of HIP 33555, and HIP 118213, and the companions to the secondaries in HIP 25300 and HIP 101430. We place the components on a color–magnitude diagram and discuss each multiple system individually.

79 ASTRONOMY AND ASTROPHYSICS↗

SUB-STELLAR COMPANIONS AND STELLAR MULTIPLICITY IN THE TAURUS STAR-FORMING REGION

We present results from a large, high-spatial-resolution near-infrared imaging search for stellar and sub-stellar companions in the Taurus-Auriga star-forming region. The sample covers 64 stars with masses between those of the most massive Taurus members at ∼3 M {sub ☉} and low-mass stars at ∼0.2 M {sub ☉}. We detected 74 companion candidates, 34 of these reported for the first time. Twenty-five companions are likely physically bound, partly confirmed by follow-up observations. Four candidate companions are likely unrelated field stars. Assuming physical association with their host star, estimated companion masses are as low as ∼2 M {sub Jup}. The inferred multiplicity frequency within our sensitivity limits between ∼10-1500 AU is 26.3{sub −4.9}{sup +6.6}%. Applying a completeness correction, 62% ± 14% of all Taurus stars between 0.7 and 1.4 M {sub ☉} appear to be multiple. Higher order multiples were found in 1.8{sub −1.5}{sup +4.2}% of the cases, in agreement with previous observations of the field. We estimate a sub-stellar companion frequency of ∼3.5%-8.8% within our sensitivity limits from the discovery of two likely bound and three other tentative very low-mass companions. This frequency appears to be in agreement with what is expected from the tail of the stellar companion mass ratio distribution, suggesting that stellar and brown dwarf companions share the same dominant formation mechanism. Further, we find evidence for possible evolution of binary parameters between two identified sub-populations in Taurus with ages of ∼2 Myr and ∼20 Myr, respectively.

79 ASTRONOMY AND ASTROPHYSICS↗

The Auger Radioisotope Microscope: an instrument for characterization of Auger electron multiplicities and energy distributions

We describe a new instrument, the Argonne Auger Radioisotope Microscope (ARM), capable of characterizing the Auger electron (AE) emission of radionuclides, including candidates relevant in nuclear medicine. Our approach relies on event-by-event ion–electron coincidence, time-of-flight, and spatial readout measurement to determine correlated electron multiplicity and energy distributions of Auger decays. We present a proof-of-principle measurement with the ARM using x-ray photoionization of stable krypton beyond the K-edge and identify a bifurcation in the electron multiplicity distribution depending on the emission of K-LX electrons. Extension of the ARM to the characterization of radioactive sources of AE emissions is enabled by the combination of two recent developments: (1) cryogenic buffer gas beam technology to introduce Auger emitters into the detection region with well-defined initial conditions, and (2) large-area micro-channel plate detectors with multi-hit detection capabilities to simultaneously detect multiple electrons emitted in a single decay.

Auger emitters↗

A polarization-switch effect of silicon crystals under multiple-beam diffraction geometry

On the basis of rigorous dynamical-theory calculations, a complete X-ray polarization-switch effect of silicon crystals at the exact multiple-beam diffraction condition is demonstrated in this paper. The underlying physical mechanism of this unique phenomenon can be revealed using a simple multiple-wave propagation and interference model. The constructive and destructive interference of the multiple detoured-diffraction beams along the direction of the primary diffracted beam directly leads to the complete polarization switch. This phenomenon can be realized using both synchrotron and laboratory X-ray sources at many discrete wavelengths, and used to design a novel crystal-based polarizer to achieve a 90° polarization rotation.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DXRD : a user-friendly suite of two- and multiple-beam dynamical X-ray diffraction programs

The DXRD program suite consisting of a series of dynamical theory programs is introduced for computing dynamical X-ray diffraction from single crystals. Its interactive graphical user interfaces (GUIs) allow general users to make complicated calculations with minimal effort. It can calculate plane-wave Darwin curves of single crystals (or multiple crystals) for both the Bragg and Laue cases, including grazing-incidence diffraction and backward diffraction (with Bragg angles approaching 90°). It is also capable of simulating rocking curves for divergent incident X-ray beams with finite bandwidths. A unique feature of DXRD is that it provides a convenient GUI-based multiple-beam diffraction program that can accurately compute arbitrary N-beam diffraction of any geometry using a universal 4N × 4N matrix method. DXRD also provides a mapping program for plotting all the multiple-beam diffraction lines (monochromator glitches) in the azimuth–energy coordinate system. All these functions make DXRD a convenient and powerful software tool for designing crystal-based synchrotron/X-ray optics (monochromators, analyzers, polarizers, phase plates etc.) and for crystal characterization, X-ray spectroscopy and X-ray diffraction teaching.

Bragg reflection↗

Sixteen multiple-amplifier sensing charge-coupled devices and characterization techniques targeting the next generation of astronomical instruments

We present a candidate sensor for future spectroscopic applications, such as a Stage-5 Spectroscopic Survey Experiment or the Habitable Worlds Observatory. This type of charge-coupled device (CCD) sensor features multiple in-line amplifiers at its output stage allowing multiple measurements of the same charge packet, either in each amplifier or in the different amplifiers. Recently, the operation of an eight-amplifier sensor has been experimentally demonstrated, and we present the operation of a 16-amplifier sensor. This new sensor enables a noise level of ∼1 erms− with a single sample per amplifier. In addition, it is shown that sub-electron noise can be achieved using multiple samples per amplifier. In addition to demonstrating the performance of the 16-amplifier sensor, we aim to create a framework for future analysis and performance optimization of this type of detectors. New models and techniques are presented to characterize specific parameters, which are absent in conventional CCDs and Skipper CCDs: charge transfer between amplifiers and independent and common noise in the amplifiers and their processing.

16 multiple-amplifer sensing CCD (MAS-CCD)↗

Neutron Multiplicity Counting Diagnosis of Uranium Assemblies Interrogated by Cf-252 [Poster]

Researchers concluded: First neutron multiplicity counting of tens of kilograms of 235 U with organic scintillators; leakage multiplication estimates to be improved by incorporating detector cross-talk; provides data comparison for “Multiplicity Theory Beyond the Point Model;" promotes continued use of organic scintillators for NCERC and elsewhere.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗