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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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All sourcesNASA NTRSDOE OSTI
DOE OSTI2014

Impact of velocity correlation and distribution on transport in fractured media: Field evidence and theoretical model

Flow and transport through fractured geologic media often leads to anomalous (non-Fickian) transport behavior, the origin of which remains a matter of debate: whether it arises from variability in fracture permeability (velocity distribution), connectedness in the flow paths through fractures (velocity correlation), or interaction between fractures and matrix. Here we show that this uncertainty of distribution- versus correlation-controlled transport can be resolved by combining convergent and push-pull tracer tests because flow reversibility is strongly dependent on velocity correlation, whereas late-time scaling of breakthrough curves is mainly controlled by velocity distribution. We build on this insight, and propose a Lagrangian statistical model that takes the form of a continuous time random walk (CTRW) with correlated particle velocities. In this framework, velocity distribution and velocity correlation are quantified by a Markov process of particle transition times that is characterized by a distribution function and a transition probability. Our transport model accurately captures the anomalous behavior in the breakthrough curves for both push-pull and convergent flow geometries, with the same set of parameters. Thus, the proposed correlated CTRW modeling approach provides a simple yet powerful framework for characterizing the impact of velocity distribution and correlation on transport in fractured media.

58 GEOSCIENCES↗
DOE OSTI2022

On the differential representation and color-kinematics duality of AdS boundary correlators

The AdS boundary correlators and their dual correlation functions of boundary operators have been the main dynamic observables of the holographic duality relating a bulk AdS theory and a boundary conformal field theory. We show that tree-level AdS boundary correlators for generic states can be expressed as nonlocal differential operators of a certain structure acting on contact Witten diagrams. We further write the boundary correlators in a form that is very similar to flat space amplitudes, with Mandelstam variables replaced by certain combinations of single-state conformal generators, prove that all tree-level AdS boundary correlators have a differential representation, and detail the conversion of such differential expressions to position space. We illustrate the construction through the computation of the boundary correlators of scalars coupled to gluons and gravitons; when converted to position space, they reproduce known results. Color-kinematics duality and BCJ relations can be defined in analogy with their flat space counterparts, and are respected by the scalar correlators with a gluon exchange. We also discuss potential approaches to the double copy and find that its direct generalization may require nontrivial extensions.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2018

CP symmetry and thermal effects on Dirac bi-spinor spin–parity local correlations

Intrinsic quantum correlations supported by the SU(2)ⓍSU(2) structure of the Dirac equation used to describe particle/antiparticle states, optical ion traps and bilayer graphene are investigated and connected to the description of local properties of Dirac bi-spinors. For quantum states driven by Dirac-like Hamiltonians, quantum entanglement and geometric discord between spin and parity degrees of freedom – sometimes mapped into equivalent low energy internal degrees of freedom – are obtained. Such spin–parity quantum correlations and the corresponding nonlocal intrinsic structures of bi-spinor fermionic states can be classified in order to relate quantum observables to the (non)local behavior of these correlations. It is shown that free particle mixed states do not violate the Clauser–Horne–Shimony–Holt inequality: the correlations in such mixed bi-spinors, although quantum, can be reproduced by a suitable local hidden variable model. Additionally, the effects due to a non-minimal coupling to a homogeneous magnetic field, and to the inclusion of thermal effects are evaluated, and quantum correlations of associated quantum mixtures and of the thermal states are all quantified. The above-mentioned correlation quantifiers are then used to measure the influence of CP transformations on spin–parity quantum correlations, and our results show that quantum entanglement is invariant under CP transformations, although the geometric discord is highly sensitive to the CP symmetry.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2019

Assessing Correlations of Perovskite Catalytic Performance with Electronic Structure Descriptors

Electronic structure descriptors are computationally efficient quantities used to construct qualitative correlations for a variety of properties. In particular, the oxygen p-band center has been used to guide material discovery and fundamental understanding of an array of perovskite compounds for use in catalyzing the oxygen reduction and evolution reactions. Yet, an assessment of the effectiveness of the oxygen p-band center at predicting key measures of perovskite catalytic activity has not been made and would be highly beneficial to guide future predictions and codify best practices. In this work, we have used density functional theory at the Perdew–Burke–Ernzerhof (PBE), PBEsol, PBE + U, strongly constrained and appropriately normed functional, and Heyd–Scuseria–Ernzerhof (HSE06) levels to assess the correlations of numerous measures of catalytic performance for a series of technologically relevant perovskite oxides, using the bulk oxygen p-band center as an electronic structure descriptor. We have analyzed correlations of the calculated oxygen p-band center for all considered functionals with the experimentally measured X-ray emission spectroscopy oxygen p-band center and multiple measures of catalytic activity, including high-temperature oxygen reduction surface exchange rates, aqueous oxygen evolution current densities, and binding energies of oxygen evolution intermediate species. Our findings show that the best correlations for all measures of catalytic activity considered here are made with PBE-level calculations, with strong observed linear correlations with the bulk oxygen p-band center (R 2 = 0.81–0.87). This study illustrates that strong linear correlations between numerous important measures of catalytic activity and the oxygen p-band bulk descriptor can be obtained under a consistent computational framework, and these correlations can serve as a guide for future experiments and simulations for development of perovskite and related oxide catalysts.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2021

Correlation between Spin and Orbital Dynamics during Laser-Induced Femtosecond Demagnetization

Spin and orbital angular momenta are two intrinsic properties of an electron and are responsible for the physics of a solid. How the spin and orbital evolve with respect to each other on several hundred femtoseconds is largely unknown, but it is at the center of laser-induced ultrafast demagnetization. In this paper, we introduce a concept of the spin–orbital correlation diagram, where spin angular momentum is plotted against orbital angular momentum, much like the position-velocity phase diagram in classical mechanics. We use four sets of highly accurate time-resolved X-ray magnetic circular dichroism data to construct four correlation diagrams for iron and cobalt. To our surprise, a pattern emerges. The trace on the correlation diagram for iron is an arc, and at the end of demagnetization, it has a pronounced cusp. The correlation diagram for cobalt is different and appears more linear but with kinks. We carry out first-principles calculations with two different methods: time-dependent density functional theory (TDDFT) and time-dependent Liouville density functional theory. These two methods agree that the experimental findings for both Fe and Co are not due to experimental errors. It is the spin–orbit coupling that correlates the spin dynamics to the orbital dynamics. Microscopically, Fe and Co have different orbital occupations, which leads to distinctive correlation diagrams. We believe that this correlation diagram presents a useful tool to better understand spin and orbital dynamics on an ultrafast time scale. A brief discussion on the magnetic anisotropy energy is also provided.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2021

Correlation polarimeter-interferometer in the DIII-D tokamak

A correlation polarimeter-interferometer system has been developed for the DIII-D tokamak to detect small amplitude magnetic and density fluctuations. Two collinear, frequency-offset (5–15 MHz), orthogonally polarized (right- and left-handed, circularly polarized) electromagnetic waves at 650 GHz probing the plasma are used to detect the Faraday effect. A third, linearly polarized, electromagnetic wave serves as the local-oscillator to provide a measure of the line-averaged density. Correlation polarimetric measurement is accomplished by correlating the Faraday effect measured along the same line of sight using two independent detectors, whereas simultaneous correlation interferometric measurement is realized by correlating the line-averaged density measured at two different intermediate frequencies. The noise floor of the correlation polarimeter-interferometer has been demonstrated to be more than one order of magnitude lower than that of a standard polarimeter-interferometer measurement. Line-averaged correlation polarimetric-interferometric measurements in DIII-D H-mode plasmas show broadband (up to 750 kHz) magnetic and density fluctuations with amplitudes as low as 0.03 $Gauss$/$\sqrt{kHz}$ and 4 × 10 13 m –3 /$\sqrt{kHz}$, respectively.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2015

Radio–far-infrared correlation in “blue cloud” galaxies with 0 < z < 1.2

We study the radio–far-infrared (FIR) correlation in “blue cloud” galaxies chosen from the PRism MUltiobject Survey up to redshift (z) of 1.2 in the XMM-LSS field. We use rest-frame emission at 1.4 GHz in the radio and both monochromatic (at 70 μm) and bolometric (between 8 and 1000 μm) emission in the FIR. To probe the nature of the correlation up to z ∼1.2, where direct detection of blue star-forming galaxies is impossible with current technology, we employ the technique of image stacking at 0.325 and 1.4 GHz in the radio and in six infrared bands, 24, 70, 160, 250, 350, and 500 μm. For comparison, we also study the correlation for more luminous galaxies that are directly detected. The stacking analysis allows us to probe the radio–FIR correlation for galaxies that are up to two orders of magnitude fainter than the ones detected directly. The k correction in the infrared wavebands is obtained by fitting the observed spectral energy distribution with a composite mid-IR power law and a single temperature graybody model. We find that the radio luminosity at 1.4 GHz (L{sub 1.4 GHz}) is strongly correlated with monochromatic FIR luminosity at 70 μm (L{sub 70 μm}) having slope 1.09 ± 0.05 and with bolometric luminosity (L{sub TIR}) having slope 1.11 ± 0.04. The quantity q{sub TIR}(=log{sub 10}[L{sub TIR}/(3.75×10{sup 12}L{sub 1.4 GHz})]) is observed to decrease with redshift as q{sub TIR}∝(1+z){sup −0.16±0.03} probably caused due to the nonlinear slope of the radio–FIR correlation. Within the uncertainties of our measurement and the limitations of our flux-limited and color-selected sample, we do not find any evolution of the radio–FIR correlation with redshift.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2015

Measurement of fluid rotation, dilation, and displacement in particle image velocimetry using a Fourier–Mellin cross-correlation

Traditional particle image velocimetry (PIV) uses discrete Cartesian cross correlations (CCs) to estimate the displacements of groups of tracer particles within small subregions of sequentially captured images. However, these CCs fail in regions with large velocity gradients or high rates of rotation. In this paper, we propose a new PIV correlation method based on the Fourier–Mellin transformation (FMT) that enables direct measurement of the rotation and dilation of particle image patterns. In previously unresolvable regions of large rotation, our algorithm significantly improves the velocity estimates compared to traditional correlations by aligning the rotated and stretched particle patterns prior to performing Cartesian correlations to estimate their displacements. Furthermore, our algorithm, which we term Fourier–Mellin correlation (FMC), reliably measures particle pattern displacement between pairs of interrogation regions with up to ±180° of angular misalignment, compared to 6–8° for traditional correlations, and dilation/compression factors of 0.5–2.0, compared to 0.9–1.1 for a single iteration of traditional correlations.

42 ENGINEERING↗
DOE OSTI2017

Interferometric constraints on quantum geometrical shear noise correlations

Final measurements and analysis are reported from the first-generation Holometer, the first instrument capable of measuring correlated variations in space-time position at strain noise power spectral densities smaller than a Planck time. The apparatus consists of two co-located, but independent and isolated, 40 m power-recycled Michelson interferometers, whose outputs are cross-correlated to 25 MHz. The data are sensitive to correlations of differential position across the apparatus over a broad band of frequencies up to and exceeding the inverse light crossing time, 7.6 MHz. By measuring with Planck precision the correlation of position variations at spacelike separations, the Holometer searches for faint, irreducible correlated position noise backgrounds predicted by some models of quantum space-time geometry. The first-generation optical layout is sensitive to quantum geometrical noise correlations with shear symmetry---those that can be interpreted as a fundamental noncommutativity of space-time position in orthogonal directions. General experimental constraints are placed on parameters of a set of models of spatial shear noise correlations, with a sensitivity that exceeds the Planck-scale holographic information bound on position states by a large factor. Furthermore, this result significantly extends the upper limits placed on models of directional noncommutativity by currently operating gravitational wave observatories.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2025

Characterization of contaminants in the Lyman-alpha forest auto-correlation with DESI

Baryon Acoustic Oscillations can be measured with sub-percent precision above redshift two with the Lyman-α (Lyα) forest auto-correlation and its cross-correlation with quasar positions. This is one of the key goals of the Dark Energy Spectroscopic Instrument (DESI) which started its main survey in May 2021. We present in this paper a study of the contaminants to the Lyα forest which are mainly caused by correlated signals introduced by the spectroscopic data processing pipeline as well as astrophysical contaminants due to foreground absorption in the intergalactic medium. Notably, an excess signal caused by the sky background subtraction noise is present in the Lyα auto-correlation in the first line-of-sight separation bin. We use synthetic data to isolate this contribution, we also characterize the effect of spectro-photometric calibration noise, and propose a simple model to account for both effects in the analysis of the Lyα forest. We then measure the auto-correlation of the quasar flux transmission fraction of low redshift quasars, where there is no Lyα forest absorption but only its contaminants. We demonstrate that we can interpret the data with a two-component model: data processing noise and triply ionized Silicon and Carbon auto-correlations. This result can be used to improve the modeling of the Lyα auto-correlation function measured with DESI.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2017

Nano-engineering of electron correlation in oxide superlattices

Oxide heterostructures and superlattices (SLs) have attracted a great deal of attention in recent years owing to the rich exotic properties encountered at their interfaces. We focus on the potential of tunable correlated oxides by investigating the spectral function of the prototypical correlated metal SrVO3 , using soft x-ray absorption spectroscopy and resonant inelastic soft x-ray scattering to access both unoccupied and occupied electronic states, respectively. We demonstrate a remarkable level of tunability in the spectral function of SrVO 3 by varying its thickness within the SrVO 3 /SrTiO 3 SL, showing that the effects of electron correlation can be tuned from dominating the energy spectrum in a strongly correlated Mott–Hubbard insulator, towards a correlated metal. We show that the effects of dimensionality on the correlated properties of SrVO 3 are augmented by interlayer coupling, yielding a highly flexible correlated oxide that may be readily married with other oxide systems.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2021

Observing correlations between dark matter accretion and galaxy growth: II. testing the impact of galaxy mass, star formation indicator, and neighbour colours

A crucial question in galaxy formation is what role new accretion has in star formation. Theoretical models have predicted a wide range of correlation strengths between halo accretion and galaxy star formation. Previously, we presented a technique to observationally constrain this correlation strength for isolated Milky Way mass galaxies at z ~ 0.12, based on the correlation between halo accretion and the density profile of neighbouring galaxies. By applying this technique to both observational data from the Sloan Digital Sky Survey and simulation data from the UNIVERSEMACHINE , where we can test different correlation strengths, we ruled out positive correlations between dark matter accretion and recent star formation activity. In this work, we expand our analysis by (1) applying our technique separately to red and blue neighbouring galaxies, which trace different infall populations, (2) correlating dark matter accretion rates with D n 4000 measurements as a longer-term quiescence indicator than instantaneous star-formation rates, and (3) analysing higher-mass isolated central galaxies with 10 11.0 < M * /M ⊙ < 10 11.5 out to z ~ 0.18. Finally, in all cases, our results are consistent with non-positive correlation strengths with ≳ 85 percent confidence, which is most consistent with models where processes such as gas recycling dominate star formation in massive z = 0 galaxies.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2020

Curvature-slope correlation of nuclear symmetry energy and its imprints on the crust-core transition, radius, and tidal deformability of canonical neutron stars

Background: The nuclear symmetry energy E sym (ρ) encodes information about the energy necessary to make nuclear systems more neutron-rich. While its slope parameter L at the saturation density ρ 0 of nuclear matter has been relatively well constrained by recent astrophysical observations and terrestrial nuclear experiments, its curvature K sym characterizing the E sym (ρ) around 2ρ 0 remains largely unconstrained. Over 520 calculations for E sym (ρ) using various nuclear theories and interactions in the literature have predicted several significantly different K sym –L correlations. Purpose: If a unique K sym –L correlation of E sym (ρ) can be firmly established, it will enable us to progressively better constrain the high-density behavior of E sym (ρ) using the available constraints on its slope parameter L. Here, we investigate if and by how much the different K sym –L correlations may affect neutron star observables. Method: A meta-model of nuclear Equation of States (EOSs) with three representative K sym –L correlation functions is used to generate multiple EOSs for neutron stars. We then examine effects of the K sym –L correlation on the crust-core transition density and pressure as well as the radius and tidal deformation of canonical neutron stars. Results: The K sym –L correlation affects significantly both the crust-core transition density and pressure. It also has strong imprints on the radius and tidal deformability of canonical neutron stars especially at small L values. The available data from LIGO/VIRGO and NICER set some useful limits for the slope L but can not distinguish the three representative K sym –L correlations considered.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Structure in the event-by-event energy-dependent neutron-$γ$ multiplicity correlations in 252 Cf(sf)

The emission of neutrons and γ rays by fission fragments reveal important information about the properties of fragments immediately following scission. The initial fragment properties, correlations between fragments, and emission competition give rise to correlations in neutron-γ emission. Recent theoretical and experimental advances have been proposed to explain the mechanism of angular momentum generation in fission, which would result in observable signature in neutron-γ emission correlations. In this paper, we present a novel analysis method of neutrons and γ rays emitted by fission fragments that allows us to discern structure in the observed correlations. We have analyzed data collected on 252 Cf (sf) at the Chi-Nu array at the Los Alamos Neutron Science Center. Through our analysis of the energy-differential neutron-γ multiplicity covariance, we have observed enhanced neutron-γ correlations, corresponding to rotational band γ-ray transitions, at γ-ray energies of 0.7 and 1.2 MeV. To shed light on the origin of this structure, we compare the experimental data with the predictions of three model calculations. The origin of the observed correlation structure is understood in terms of a positive spin-energy correlation in the generation of angular momentum in fission.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

Correlations of conserved quantities at finite baryon density

Correlations involving the seven conserved quantities, namely energy, baryon number, electric charge, strangeness, and the three components of momentum, give rise to correlations in heavy-ion collisions. Through the utilization of a simple one-dimensional hydrodynamic model, we calculate the evolution of the entire 7×7 matrix of correlations as a function of relative spatial rapidity. This comprehensive analysis accounts for finite baryon density, which results in off-diagonal correlations between the charge-related quantities and the energy-momentum quantities. These correlations in coordinate space are subsequently transformed into correlations in momentum space using statistical weighting. As a result, the entire matrix of correlations is revealed to be highly sensitive to the equation of state, viscosity, and diffusivity.

Equations of state of nuclear matter↗
DOE OSTI2018

Event plane dependence of the flow modulated background in dihadron and jet-hadron correlations in heavy ion collisions

Di-hadron and jet-hadron correlations are commonly used in relativistic heavy ion collisions to study the soft component of jets in a quark gluon plasma. There is a large correlated background which is described by the Fourier decomposition of the azimuthal anisotropy where vn is the nth order coefficient. The path length dependence of partonic energy loss can be studied by varying the angle of the high momentum trigger particle or jet relative to a reconstructed event plane. This modifies the shape of the background correlated with that event plane. The original derivation of the shape of this background only considered correlations relative to the second order event plane, which is correlated to the initial participant plane. We derive the shape of this background for an event plane at an arbitrary order. There is a phase shift in the case of jets restricted to asymmetric regions relative to the event plane. For realistic correlations between event planes, the correlation between the second and fourth order event planes leads to a much smaller effect than the finite event plane resolution at each order. Lastly, we assess the status of the rapidity even v1 term due to low, which has been measured to be comparable to v 2 and v 3 terms.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2019

Evolving charge correlations in a hybrid model with both hydrodynamics and hadronic Boltzmann descriptions

Background: Correlations from charge correlation, known as charge balance functions, provide critical tests of the chemical evolution of matter in a heavy-ion collision. Comparisons of experimental balance functions with calculations from parametric descriptions of the final state suggest that the charge production in the earliest stages of a heavy-ion collision are consistent with having generated an amount of light up, down, and strange quarks that are largely consistent with expectations for creating a chemically equilibrate quark-gluon plasma. Purpose: This work describes a full simulation of the evolving correlations superimposed on a state-of-the-art microscopic description of the collision. Methods: The creation and diffusion of balancing charges is modeled on the background of a hybrid description of the evolution based on hydrodynamics, for when the matter’s temperature is above 155 MeV, and a microscopic hadronic simulation, for the breakup stage. The translation of the charge-charge correlation function, indexed by the flavors up, down, and strange, into correlations between specific hadron species is built on the assumption that differential charges enhance differential yields according to statistical equilibrium. Monte Carlo methods are implemented when applicable. Results: The charge balance functions are predicted for pairs indexed by charge alone or by whether the particle pairs are any combination of pions, kaons, or protons. We report comparisons with experiment are remarkably successful except for the proton-kaon balance functions. Conclusions: This demonstrates first that two-particle correlations from charge conservation can be calculated for a state-of-the-art model of the evolution with moderate amounts of computation. Aside from the magnitude of the proton-kaon correlations, the calculations well describe preliminary experimental results from the STAR Collaboration at the Relativistic Heavy Ion Collider. Ignoring the one disagreement, this suggests that the matter in a heavy-ion collision comes close to maintaining chemical equilibrium during the superhadronic stage of a heavy-ion collision.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2015

Correlated two-particle diffusion in dense colloidal suspensions at early times: Theory and comparison to experiment

The spatially resolved diffusive dynamic cross correlations of a pair of colloids in dense quasi-two-dimensional monolayers of identical particles are studied experimentally and theoretically at early times where motion is Fickian. In very dense systems where strong oscillatory equilibrium packing correlations are present, we find an exponential decay of the dynamic cross correlations on small and intermediate length scales. At large separations where structure becomes random, an apparent power law decay with an exponent of approximately –2.2 is observed. For a moderately dense suspension where local structural correlations are essentially absent, this same apparent power law decay is observed over all probed interparticle separations. A microscopic nonhydrodynamic theory is constructed for the dynamic cross correlations which is based on interparticle frictional effects and effective structural forces. Hydrodynamics enters only via setting the very short-time single-particle self-diffusion constant. No-adjustable-parameter quantitative predictions of the theory for the dynamic cross correlations are in good agreement with experiment over all length scales. The origin of the long-range apparent power law is the influence of the constraint of fixed interparticle separation on the amplitude of the mean square force exerted on the two tagged particles by the surrounding fluid. The theory is extended to study high-packing-fraction 3D hard sphere fluids. Here, the same pattern of an oscillatory exponential form of the dynamic cross correlation function is predicted in the structural regime, but the long-range tail decays faster than in monolayers with an exponent of –3.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗