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NASA NTRS1999

J6 Himalia: New Compositional Evidence and Interpretations for the Origin of Jupiter's Small Satellites

New narrowband spectrophotometric data of J6 Himalia, some of which are spatially resolved, support its C-type classification. The new spectra confirm the presence of a weak absorption feature centered near 0.7 micron attributed to oxidized iron in phyllosilicates, products of aqueous alteration, which varies in depth on opposite sides of the satellite. Evaluation of older UBV photometry of J6 and J7 Elara compared to UBV photometry of C-class (and subclass) asteroids showing spectral evidence of the 0.7-microns absorption feature suggests that J6 Himalia is an F-class asteroid. We propose that the parent body of the prograde Jovian satellites originated as part of the Nysa asteroid family. Evolutionary models of the Jovian system are used to address the capture and dispersal of the irregular satellites.

Vilas, Faith↗

NASA NTRSDate not supplied

Reanalysis Activities at the NASA Global Modeling and Assimilation Office

This talk presents an overview of recent reanalysis activities at the NASA Global Modeling and Assimilation Office (GMAO) as part of a multi-faceted strategy towards an Integrated Earth System retrospective analysis, coupling components of the atmosphere, ocean, chemistry, land, and ice. While elements of the atmosphere-ocean coupled Goddard Earth Observing System (GEOS) model and data assimilation are being actively developed, a suite of reanalysis products is designed to provide further understanding of key aspects of Earth system coupling in a reanalysis context: The baseline atmospheric reanalysis, the GEOS Retrospective analysis for the early 21st Century (GEOS-R21C), features recent advances in the GEOS model and data assimilation, and targets the NASA’s Earth Observing System EOS and post-EOS satellite observations; GEOS-IT, a user-tailored low-resolution atmospheric reanalysis, serves as a second baseline to the NASA Instrument Teams for validation and calibration and drives a one-way coupled ocean reanalysis, GEOSIT-Ocean; PolarMERRA, a high-resolution downscaled product for the polar regions, focuses on improving the representation of polar atmospheric processes with an assessment of current cryospheric biases, and targeted improvements to surface sea ice and glacier conditions; Finally, R21C-Chem, an off-line atmospheric chemistry and composition reanalysis, includes both tropospheric and stratospheric trace gases. The diversity of these reanalysis activities presents unique opportunities for collaborations cross-teams/institutions, with new commercial data partners, and with end-user groups. This talk will discuss these opportunities and explore leveraging the lessons learned along the way on key drivers in Earth system interactions as we converge towards the next generation of the Modern-Era Retrospective analysis for Research and Applications (MERRA) suite.

Amal El Akkraoui↗

NASA NTRS2010

Lunar Crustal History from Isotopic Studies of Lunar Anorthosites

Anorthosites occur ubiquitously within the lunar crust at depths of approx.3-30 km in apparent confirmation of the Lunar Magma Ocean (LMO) hypothesis. [1]. We will present recent chronological studies of anorthosites [2] that are relevant both to the LMO hypothesis and also to the lunar cataclysm hypothesis. Old (approx.4.4 Ga) Sm-Nd ages have been determined for some Apollo 16 anorthosites, and primitive initial Sr-87/Sr-86 ratios have been measured for several, but well-defined Rb-Sr ages concordant with the Sm-Nd ages have not been determined until now. Lunar anorthosite 67075, a Feldspathic Fragmental Breccia (FFB) collected near the rim of North Ray Crater, has concordant Sm-Nd and Rb-Sr ages of 4.47+/-0.07 Ga and 4.49+/-0.07 Ga, respectively. Initial Nd-143/Nd-144 determined from the Sm-Nd isochron corresponds to E(sub Nd,CHUR) = 0.3+/-0.5 compared to a Chondritic Uniform Reservoir, or E(sub Nd,HEDPB) = -0.6+/-0.5 compared to the initial Nd-143/Nd-144 of the HED Parent Body [3]. Lunar anorthosites tend to have E(sub Nd) > 0 when compared to CHUR, apparently inconsistent with derivation from a single lunar magma ocean. Although E(sub Nd) < 0 for some anorthosites, if lunar initial Nd-143/Nd-144 is taken equal to HEDR for the HED parent body [3], enough variability remains among the anorthosite data alone to suggest that lunar anorthosites do not derive from a single source, i.e., they are not all products of the LMO. An anorthositic clast from desert meteorite Dhofar 908 has an Ar-39-Ar-40 age of 4.42+/-0.04 Ga, the same as the 4.36-4.41+/-0.035 Ga Ar-39-Ar-40 age of anorthositic clast Y-86032,116 in Antarctic meteorite Yamato- 86032 [3,4]. Conclusions: (i) Lunar anorthosites come from diverse sources. Orbital geochemical studies confirm variability in lunar crustal composition [1, 5]. We suggest that the variability extends to anorthosites alone as shown by the Sm-Nd data (Fig. 2) and the existence of magnesian anorthosites (MAN, [6]) and "An93 anorthosites" [3,4]. (ii) Anorthositic clasts in lunar meteorites retain "high" Ar-Ar ages compared to Apollo anorthosites. This is perhaps a hint that "cataclysmic" impacts were on average less energetic in the mostly farside source regions of these meteorites than on the lunar nearside.

Nyquist, Laurence E.↗

NASA NTRS1996

Assessment of Rainfall Estimates Using a Standard Z-R Relationship and the Probability Matching Method Applied to Composite Radar Data in Central Florida

Precipitation estimates from radar systems are a crucial component of many hydrometeorological applications, from flash flood forecasting to regional water budget studies. For analyses on large spatial scales and long timescales, it is frequently necessary to use composite reflectivities from a network of radar systems. Such composite products are useful for regional or national studies, but introduce a set of difficulties not encountered when using single radars. For instance, each contributing radar has its own calibration and scanning characteristics, but radar identification may not be retained in the compositing procedure. As a result, range effects on signal return cannot be taken into account. This paper assesses the accuracy with which composite radar imagery can be used to estimate precipitation in the convective environment of Florida during the summer of 1991. Results using Z = 30OR(sup 1.4) (WSR-88D default Z-R relationship) are compared with those obtained using the probability matching method (PMM). Rainfall derived from the power law Z-R was found to he highly biased (+90%-l10%) compared to rain gauge measurements for various temporal and spatial integrations. Application of a 36.5-dBZ reflectivity threshold (determined via the PMM) was found to improve the performance of the power law Z-R, reducing the biases substantially to 20%-33%. Correlations between precipitation estimates obtained with either Z-R relationship and mean gauge values are much higher for areal averages than for point locations. Precipitation estimates from the PMM are an improvement over those obtained using the power law in that biases and root-mean-square errors are much lower. The minimum timescale for application of the PMM with the composite radar dataset was found to be several days for area-average precipitation. The minimum spatial scale is harder to quantify, although it is concluded that it is less than 350 sq km. Implications relevant to the WSR-88D system are discussed.

Crosson, William L.↗

DOE OSTI2021

Convergence of micro-geochemistry and micro-geomechanics towards understanding proppant shale rock interaction: A Caney shale case study in southern Oklahoma, USA

As a direct outcome of economic development coupled with an increase in population, global energy demand will continue to rise in the coming decades. Although renewable energy sources are increasingly investigated for optimal production, the immediate needs require focus on energy sources that are currently available and reliable, with a minimal environmental impact; the efficient exploration and production of unconventional hydrocarbon resources is bridging the energy needs and energy aspirations, during the current energy transition period. The main challenges are related to the accurate quantification of the critical rock properties that influence production, their heterogeneity and the multiscale driven physico-chemical nature of rock–fluid interactions. A key feature of shale reservoirs is their low permeability due to dominating nanoporosity of the clay-rich matrix. As a means of producing these reservoirs in a cost-effective manner, a prerequisite is creation of hydraulic fracture networks capable of the highest level of continued conductivity. Fracturing fluid chemical design, formation brine geochemical composition, and rock mineralogy all contribute to swelling-induced conductivity damage. The Caney Shale is an organic-rich, often calcareous mudrock. Many studies have examined the impact that clay has on different kinds of shale productivity but there is currently no data reported on the Caney Shale in relation to horizontal drilling; all reported data on the Caney Shale is on vertical wells which are shallow, compared to an emerging play that is at double the depth. Here, in this work we develop geochemical–geomechanical integration of rock properties at micro-and nanoscales that can provide insights into the potential proppant embedment and its mitigation. The novel methodology amalgamates the following: computed X-ray tomography, scanning electron microscopy, energy dispersive spectroscopy, micro-indentation, and Raman spectroscopy techniques. Here, our results show that due to the multiscale heterogeneity in the Caney Shale, these geochemical and structural properties translate into a variation in mechanical properties that will impact interaction between the proppant and the host shale rock.

03 NATURAL GAS↗

DOE OSTI2025

Myco-CORPSE simulations assessing mycorrhizal carbon allocation across U.S. forests and global change scenarios

Plants allocate a substantial portion of their fixed carbon belowground to mycorrhizal fungi in exchange for nutrients and other benefits. However, most current ecosystem models omit mycorrhizal processes, limiting our ability to predict plant–soil carbon dynamics under environmental change. To address this gap, we used a mycorrhiza-explicit soil biogeochemical model, Myco-CORPSE (Mycorrhizal Carbon, Organisms, Rhizosphere, and Protection in the Soil Environment), to simulate tree carbon allocation to arbuscular mycorrhizal (AM) and ectomycorrhizal (ECM) fungi in temperate forests.The dataset includes outputs from two sets of model simulations:1. Perturbation experiments: Simulations across gradients of ECM dominance (0–100%), nitrogen deposition, soil temperature, and net primary productivity (NPP) to test how these factors affect mycorrhizal C allocation and nutrient cycling.2. FIA-based simulations: Model applications to over 1,800 U.S. forest sites using site-specific data from the U.S. Forest Inventory and Analysis (FIA) program, including vegetation composition, mycorrhizal type, climate, litter traits, soil properties, and N deposition.Model outputs include simulated mycorrhizal carbon allocation and related biogeochemical variables, such as soil and microbial carbon and nitrogen stocks. Data are provided in CSV format and organized by experiment type (in separate ZIP files). Python scripts for running simulations, plotting, and spatial mapping are also included and organized similarly. No proprietary software is required. These outputs support a peer-reviewed study and were used to generate figures and tables in the associated publication.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS1993

Process Analyzer

Under a NASA Small Business Innovation Research (SBIR) contract, Axiomatics Corporation developed a shunting Dielectric Sensor to determine the nutrient level and analyze plant nutrient solutions in the CELSS, NASA's space life support program. (CELSS is an experimental facility investigating closed-cycle plant growth and food processing for long duration manned missions.) The DiComp system incorporates a shunt electrode and is especially sensitive to changes in dielectric property changes in materials at measurements much lower than conventional sensors. The analyzer has exceptional capabilities for predicting composition of liquid streams or reactions. It measures concentrations and solids content up to 100 percent in applications like agricultural products, petrochemicals, food and beverages. The sensor is easily installed; maintenance is low, and it can be calibrated on line. The software automates data collection and analysis.

Source record↗

NASA NTRS1980

F region above Kauai - Measurement, model, modification

Results of the Lagopedo II experiment conducted from Kauai, Hawaii to investigate the ionospheric modification that occurs when rocket combustion products are introduced into the O(+)-rich F region are presented. The experiment involved the detonation of a chemical explosion in the F2 peak accompanied by rocket-borne measurements of ion composition and electron content in the vicinity of the explosion. The experimental data is found to be in good agreement with the predictions of a model of the nighttime ion densities in the midlatitude laminar ionosphere, with the exception of N2(+) densities before the explosion. H2O(+) and H3O(+) currents produced by considerable H2O outgassing from the rocket are used to determine a H3O(+)/H2O(+) dissociative recombination rate averaging 1.6 to 1.08, depending on model assumptions. At the time of the explosion, an ionic void 1 km in radius is observed, the boundary of which is characterized by a steep gradient in ionic densities. Evidence of variations in the concentrations of ambient ion species, new reactant species and ionic depletion by sweeping is also obtained.

Johnson, C. Y.↗

NASA NTRS2011

Forecasting Lake-Effect Precipitation in the Great Lakes Region Using NASA Enhanced-Satellite Data

Lake-effect precipitation is common in the Great Lakes region, particularly during the late fall and winter. The synoptic processes of lake-effect precipitation are well understood by operational forecasters, but individual forecast events still present a challenge. Locally run, high resolution models can assist the forecaster in identifying the onset and duration of precipitation, but model results are sensitive to initial conditions, particularly the assumed surface temperature of the Great Lakes. The NASA Short-term Prediction Research and Transition (SPoRT) Center has created a Great Lakes Surface Temperature (GLST) composite, which uses infrared estimates of water temperatures obtained from the MODIS instrument aboard the Aqua and Terra satellites, other coarser resolution infrared data when MODIS is not available, and ice cover maps produced by the NOAA Great Lakes Environmental Research Lab (GLERL). This product has been implemented into the Weather Research and Forecast (WRF) model Environmental Modeling System (WRF-EMS), used within forecast offices to run local, high resolution forecasts. The sensitivity of the model forecast to the GLST product was analyzed with a case study of the Lake Effect Storm Echinacea, which produced 10 to 12 inches of snowfall downwind of Lake Erie, and 8 to 18 inches downwind of Lake Ontario from 27-29 January 2010. This research compares a forecast using the default Great Lakes surface temperatures from the Real Time Global sea surface temperature (RTG SST), in the WRF-EMS model to the enhanced NASA SPoRT GLST product to study forecast impacts. Results from this case study show that the SPoRT GLST contained less ice cover over Lake Erie and generally cooler water temperatures over Lakes Erie and Ontario. Latent and sensible heat fluxes over Lake Ontario were decreased in the GLST product. The GLST product decreased the quantitative precipitation forecast (QPF), which can be correlated to the decrease in temperatures and heat fluxes. A slight increase in precipitation coverage was noted over Lake Erie due to a decrease in ice cover. Both the RTG SST and the GLST products predicted the precipitation south of the actual location of precipitation. This single case study is the first part of an examination to determine how MODIS data can be applied to improve model forecasts in the Great Lakes region.

Cipullo, Michelle↗

NASA NTRS2014

Composite Overview and Composite Aerocover Overview

Materials Science Division within the Engineering Directorate tasked by the Ares Launch Vehicle Division (LX-V) and the Fluids Testing and Technology Development Branch (NE-F6) to design, fabricate and test an aerodynamic composite shield for potential Heavy Lift Launch Vehicle infusion and a composite strut that will serve as a pathfinder in evaluating calorimeter data for the CRYOSTAT (cryogenic on orbit storage and transfer) Project. ATP project is to carry the design and development of the aerodynamic composite cover or "bracket" from cradle to grave including materials research, purchasing, design, fabrication, testing, analysis and presentation of the final product. Effort consisted of support from the Materials Testing & Corrosion Control Branch (NE-L2) for mechanical testing, the Prototype Development Branch (NE-L3) for CAD drawing, design/analysis, and fabrication, Materials & Processes Engineering Branch (NE-L4) for project management and materials selection; the Applied Physics Branch (NE-LS) for NDE/NDI support; and the Chemical Analysis Branch (NE-L6) for developmental systems evaluation. Funded by the Ares Launch Vehicle Division and the Fluids Testing and Technology Development Branch will provide ODC

Caraccio, Anne↗

DOE OSTI2021

Data from Bioenergy Sorghum Maintains Photosynthetic Capacity in Elevated Ozone Concentrations

Elevated tropospheric ozone concentration (O3) significantly reduces photosynthesis and productivity in several C4 crops including maize, switchgrass and sugarcane. However, it is unknown how O3 affects plant growth, development and productivity in sorghum ( Sorghum bicolor L.), an emerging C4 bioenergy crop. Here, we investigated the effects of elevated O3 on photosynthesis, biomass and nutrient composition of a number of sorghum genotypes over two seasons in the field using free-air concentration enrichment (FACE), and in growth chambers. We also tested if elevated O3 altered the relationship between stomatal conductance and environmental conditions using two common stomatal conductance models. Sorghum genotypes showed significant variability in plant functional traits, including photosynthetic capacity, leaf N content and specific leaf area, but responded similarly to O3. At the FACE experiment, elevated O3 did not alter net CO2 assimilation (A), stomatal conductance (gs), stomatal sensitivity to the environment, chlorophyll fluorescence and plant biomass, but led to reductions in the maximum carboxylation capacity of phosphoenolpyruvate and increased stomatal limitation to A in both years. These findings suggest that bioenergy sorghum is tolerant to O3 and could be used to enhance biomass productivity in O3 polluted regions.

Feedstock Production↗

NASA NTRS2012

Standardization of the Definitions of Vertical Resolution and Uncertainty in the NDACC-archived Ozone and Temperature Lidar Measurements

The international Network for the Detection of Atmospheric Composition Change (NDACC) is a global network of high-quality, remote-sensing research stations for observing and understanding the physical and chemical state of the Earth atmosphere. As part of NDACC, over 20 ground-based lidar instruments are dedicated to the long-term monitoring of atmospheric composition and to the validation of space-borne measurements of the atmosphere from environmental satellites such as Aura and ENVISAT. One caveat of large networks such as NDACC is the difficulty to archive measurement and analysis information consistently from one research group (or instrument) to another [1][2][3]. Yet the need for consistent definitions has strengthened as datasets of various origin (e.g., satellite and ground-based) are increasingly used for intercomparisons, validation, and ingested together in global assimilation systems.In the framework of the 2010 Call for Proposals by the International Space Science Institute (ISSI) located in Bern, Switzerland, a Team of lidar experts was created to address existing issues in three critical aspects of the NDACC lidar ozone and temperature data retrievals: signal filtering and the vertical filtering of the retrieved profiles, the quantification and propagation of the uncertainties, and the consistent definition and reporting of filtering and uncertainties in the NDACC- archived products. Additional experts from the satellite and global data standards communities complement the team to help address issues specific to the latter aspect.

Detection of Atmospheric Composition Change (NDACC↗

DOE OSTI2020

Role of shell composition and morphology in achieving single-emitter photostability for green-emitting “giant” quantum dots

The use of the varied chemical reactivity of precursors to drive the production of a desired nanocrystal architecture has become a common method to grow thick-shell graded alloy quantum dots (QDs) with robust optical properties. Conclusions on their behavior assume the ideal chemical gradation and uniform particle composition. In this work, advanced analytical electron microscopy (high-resolution scanning transmission electron microscopy coupled with energy dispersive spectroscopy) is used to confirm the nature and extent of compositional gradation and these data are compared with performance behavior obtained from single-nanocrystal spectroscopy to elucidate structure, chemical-composition, and optical-property correlations. In particular, the evolution of the chemical structure and single-nanocrystal luminescence was determined for a time-series of graded-alloy “CdZnSSe/ZnS” core/shell QDs prepared in a single-pot reaction. In a separate step, thick (~6 monolayers) to giant (>14 monolayers) shells of ZnS were added to the alloyed QDs via a successive ionic layer adsorption and reaction (SILAR) process, and the impact of this shell on the optical performance was also assessed. By determining the degree of alloying for each component element on a per-particle basis, we observe that the actual product from the single-pot reaction is less “graded” in Cd and more so in Se than anticipated, with Se extending throughout the structure. The latter suggests much slower Se reaction kinetics than expected or an ability of Se to diffuse away from the initially nucleated core. It was also found that the subsequent growth of thick phase-pure ZnS shells by the SILAR method was required to significantly reduce blinking and photobleaching. However, correlated single-nanocrystal optical characterization and electron microscopy further revealed that these beneficial properties are only achieved if the thick ZnS shell is complete and without large lattice discontinuities. Thus, we identify the necessary structural design features that are required for ideal light emission properties in these green-visible emitting QDs.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2023

Dominant heterocyclic composition of dissolved organic nitrogen in the ocean: A new paradigm for cycling and persistence

Marine dissolved organic nitrogen (DON) is one of the planet’s largest reservoirs of fixed N, which persists even in the N-limited oligotrophic surface ocean. The vast majority of the ocean’s total DON reservoir is refractory (RDON), primarily composed of low molecular weight (LMW) compounds in the subsurface and deep sea. However, the composition of this major N pool, as well as the reasons for its accumulation and persistence, are not understood. Past characterization of the analytically more tractable, but quantitatively minor, high molecular weight (HMW) DON fraction revealed a functionally simple amide-dominated composition. While extensive work in the past two decades has revealed enormous complexity and structural diversity in LMW dissolved organic carbon, no efforts have specifically targeted LMW nitrogenous molecules. Here, we report the first coupled isotopic and solid-state NMR structural analysis of LMW DON isolated throughout the water column in two ocean basins. Together these results provide a first view into the composition, potential sources, and cycling of this dominant portion of marine DON. Our data indicate that RDON is dominated by 15N-depleted heterocyclic-N structures, entirely distinct from previously characterized HMW material. This fundamentally new view of marine DON composition suggests an important structural control for RDON accumulation and persistence in the ocean. The mechanisms of production, cycling, and removal of these heterocyclic-N-containing compounds now represents a central challenge in our understanding of the ocean’s DON reservoir.

58 GEOSCIENCES↗

NASA NTRS1974

An interdisciplinary study of the estaurine and coastal oceanography of Block Island Sound and adjacent New York coastal waters

ERTS-1 photographic data products have been analyzed using additive color viewing and electronic image analysis techniques. Satellite data were compared to water sample data collected simultaneously with the data of ERTS-1 coverage in New York Bight. Prediction of the absolute value of total suspended particles can be made using composites of positives of MSS bands 5 and 6 which have been precisely made using the step wedge supplied on the imagery. Predictions of the relative value of the extinction coefficient can be made using bands 4 and 5. Thematic charts of total suspended particles (particles per litre) and extinction coefficient provide scientists conducting state and federal water sampling programs in New York Bight with data which improves the performance of these programs.

Yost, E.↗

NASA NTRS1974

Crystallization behavior of anorthite

The growth rate of anorthite crystals from the melt is studied as a function of temperature with undercooling in the ranges 52-152 and 402-652 degrees C. The triclinic form is invariably observed as the crystallization product, growth is preferentially in the c direction, and the interface morphology is faceted. Significant growth rate anisotropy is indicated. The maximum growth rate of anorthite from the melt is higher than for anorthite-rich lunar compositions. Recent computer studies are combined with experimental data to estimate the heat of fusion of anorthite as 28000-45000 cal/mol; the corresponding range for entropy of fusion is (7.8-12)R (where R is the gas constant). The observations and kinetic data support Jackson's predictions concerning materials with large entropies of fusion and his suggestion that entropy of fusion is an important parameter for characterizing the crystal-liquid interface and the nature of the crystallization process.

Klein, L.↗

NASA NTRS1975

Ancient meteoritic component in Apollo 17 boulders

The reported investigation is concerned with the resolution of a number of questions related to the ancient meteoritic component in Apollo 17 boulders. Numerical taxonomic methods have been adopted to objectively group the components. Only the nonvolatile siderophile elements have been used for the classification. Efforts were made to obtain data on the metal composition of breccias analyzed for trace elements, to determine if metal homogeneity was reflected in siderophile ratios. Thirty-one samples were analyzed of which twenty-eight have significant siderophile contents. It is concluded that highland breccias are largely the product of large basin-forming impacts. Highland soils are then produced by comminution of the breccias by small local impacts and micrometeorite bombardment. The long-lived component of bulk soils considered by Baedecker et al. (1974) is thought to contain a substantial micrometeorite contribution, plus assorted debris.

Higuchi, H.↗

NASA NTRS1985

Crustal development in the terrestrial planets

The development of planetary crusts may be divided into primary, resulting from melting during accretion, and secondary crusts developed by partial melting from planetary mantles. The Mercurian crust is probably primary with no compelling evidence of later basaltic extrusions. Reflectance spectral evidence for the existence Fe2(+) is equivocal. The Viking Lander XRF data on Mars indicate basaltic material at both sites 4,000 km apart. Surface aeolian processes would be expected to provide a homogeneous average of the crust, but no evidence of more siliceous material is present. This conclusion is weakly supported by the Russian gamma ray data. No evidence for granite appears from the Russian Venera XRF data which indicates MORB-type and alkali basalt (4% K2O) surface compositions. The highlands of Ishtar Terra and Aphrodite probably owe their elevation to tectonic processes rather than compositional effects. Venus may thus resemble the early Archean Earth. The terrestrial granitic continental crust is a product of episodic multiple partial melting events, probably a consequence of the presence of surface water.

Taylor, S. R.↗