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All sourcesNASA NTRSDOE OSTI
DOE OSTI2015

Of the final end state for decommissioning of reactors at SRS: collaboration between stakeholders, regulators, and the Federal Government - 15279

The Savannah River Site (SRS) is an 802 square-kilometer (310 square-miles) United States Department of Energy (US DOE) nuclear facility located along the Savannah River near Aiken, South Carolina. Nuclear weapons material production began in the early 1950's, utilizing five (5) production reactors. In the early 1990's all SRS production reactor operations were terminated. The first reactor closure end-state declaration was documented in a Comprehensive Environmental Response and Compensation and Liability Act (CERCLA) Early Action Record of Decision. The decision for the final closure of the 29,543 square-meter (318,000 square-feet) 105-P Reactor was determined to be in situ decommissioning (ISD). ISD is an acceptable and cost-effective alternative to off-site disposal for the reactor building, which will allow for consolidation of remedial action wastes generated from other cleanup activities within the P Area. ISD is considered protective by the regulators, U.S. Environmental Protection Agency (USEPA) and the South Carolina Department of Health and Environmental Control (SCDHEC), public and stakeholders as waste materials are stabilized / immobilized, and radioactivity is allowed to naturally decay, thus preventing future exposure to the environment. Stakeholder buy-in was critical in the up-front planning in order to achieve this monumental final decision. Numerous public meetings and workshops were held in two different states (covering a 321 kilometer (200-mile) radius) with stakeholder and SRS Citizens Advisory Board (CAB) participation. These meetings were conducted over an eight- month period as the end-state decision making progressed. Information provided to the public evolved from workshop to workshop as data became available and public input from the public meetings were gathered. ISD is being considered for the balance of the four (4) SRS reactors and other hardened facilities such as the chemical Separation Facilities (canyons). Closure of the SRS P Reactor Area was precedent setting and sets the stage for closure of other reactors and hardened facilities. The DOE, USEPA, and SCDHEC engaged in active, up-front, and timely involvement with the SRS. The SRS CAB, elected officials, and citizens of South Carolina and Georgia met to discuss the P reactor area closure and associated risks. Early public involvement gave SRS and the regulators assurance that the selected decision was valid and would not be overturned. Public input improved the process and ensured that the important decision on the final end-state of the reactor facilities was not made in isolation. ISD of P Reactor will provide adequate protection of human health and the environment and the lowest cost since short-term risk is minimized to remedial workers from exposure to contaminated equipment and facilities by leaving the reactor vessel in place allowing for radiological decay over time. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗
DOE OSTI2017

Coupled CFD-DEM Analysis of Molten Salt-Cooled Pebble-Bed Reactor Experiment

The development of new nuclear reactor designs is an area of ongoing investigation, and a focus of dedicated work for various laboratories around the world. Despite the steadfast and reliable service of Light Water Reactors (LWR), the ideal power reactor, with a combination of high operational temperature, passive safety, proliferation resistance, economic build and waste minimization remains elusive. One promising design that might address these diverse, and at times contradictory requirements, is the Molten Salt Reactor (MSR). In its most radical form, a liquid fueled (LF) MSR has the nuclear fuel dissolved in the molten-salt primary coolant itself, as demonstrated by Oak Ridge National Lab (ORNL) in 1965 to 1969. An alternative fuel arrangement is to retain conventional, solid fuel elements. A proposed method is to implement pebble fuel elements, as have been used in previous gas-cooled reactors, with the gas coolant being replaced with a molten salt. This is referred to as pebble-bed, molten-salt reactor (PB-MSR). The spherical fuel pebbles used within PB-MSRs contain TRISO particles dispersed throughout the pebble's graphite matrix. Many pebbles are constrained to form a porous bed within the core region of a reactor. Coolant molten-salt passes through the pebble bed to remove heat produced due to the nuclear fission taking place within the fuel pebbles' TRISO particles. Various benefits are apparent with the PB-MSR design. When considering the choice of fuel elements, they are a geometry that has been produced and utilized in a similar way in the past, within gas-cooled reactors. The fuel pebbles are also able to be added to, and removed from, the core during operation, enabling on-line refueling. When considering the coolant choice, molten-salts have much higher boiling points (1703 K at 1 atm. for FLiBe) than conventional coolants such as water (630 K at 150 atm.), and are capable of reaching these temperatures at atmospheric pressure. This in turn removes the need for high pressure containment that is present in light water reactors and gas-cooled reactors. The future implementation of new reactors, and the search for improvements in efficiency and safety in current designs, require the advancement of simulation tools, which this work ultimately aims to address.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2024

Particle-based high-temperature thermochemical energy storage reactors

Solar and other renewable energy driven gas-solid thermochemical energy storage (TCES) technology is a promising solution for the next generation energy storage systems due to its high operating temperature, efficient energy conversion, ultra-long storage duration, and potential high energy density. Experimental and theoretical studies suggest that the respective gravimetric and volumetric TCES energy storage densities vary from 200 to 3000 kJ kg –1 and 1–3 GJ m –3 . Solar radiation or heat generated from electric furnaces powered by renewable electricity can be stored in the form of chemical energy through endothermic reactions, while the stored chemical energy can be converted to thermal energy via an exothermic reaction when needed. The design of highly effective reactors requires a deep understanding of materials, thermodynamics, chemical kinetics, and transport phenomena. At time of writing, TCES reactors are yet to be deployed at commercially relevant scales, leaving a substantial gap between development efforts and commercial feasibility. Therefore, this review aims to examine the state-of-the-art design and performance of particle-based TCES reactors with different reactive materials. Fundamentals related to TCES reactive materials, reaction conditions, thermodynamics and kinetics, and transport phenomena are reviewed in detail to provide a comprehensive understanding of the reactor design and operation. Five major types of TCES reactors have been comprehensively reviewed and compared, including fixed, moving, rotary, fluidized, and entrained bed reactors. Most reported prototype reactors in the literature operate at lab scale with thermal inputs below 40 kW, and scaled TCES reactors (e.g., at megawatt level) are yet to be demonstrated. The nominal reactor operating temperatures range from 300 to 1500 °C, depending on the selected chemistry, reactive material, and heat sources. To evaluate their designs, the reactors are assessed in aspects of performance, cost, and durability. Discrepancies in performance indicators of energy storage density, extent of reaction, and various energy efficiencies are highlighted. The scale-up of reactors and power block integration, which hold the key to the successful commercialization of TCES systems, are critically analyzed. Furthermore, advanced materials (both reactive materials and ceramic reactor housing materials), effective particle flow control, advanced modeling tools, and novel system design may bring significant improvement to the energy efficiency, storage density and cost competitiveness of particle-based TCES reactors.

25 ENERGY STORAGE↗
DOE OSTI2019

Cardinal: A Lower Length-scale Simulator for Fluoride Cooled High Temperature Reactors

The new DOE-NE “Center of Excellence for Thermal-fluids applications in Nuclear Energy” inaugurated in April 2018 considers and researches novel new solution strategies for historically challenging flow issues that still plague the current fleet of deployed Light Water Reactor (LWR) nuclear reactors as well as predicting various fluid flow and fluid related issues with advanced reactor technologies. Our advanced thermal-fluids research and development approach synergistically combines three natural, though overlapping, length and time scales in a hierarchal multi-scale approach to avoid the temptation and pitfalls of attempting to develop a single “solve all” algorithm for physical fluid flow problems that will span 109 in spatial and temporal scales. The demonstrate the multi-scale philosophy of the center we focus first on Fluoride Cooled High Temperature Reactors (FHRs), and in particular on the Berkeley’s PB-FHR design Mark-I design. The Fluoride salt cooled High temperature Reactor (FHR) is a class of advanced nuclear reactors that combine the robust coated particle fuel form from high temperature gas cooled reactors, direct reactor auxiliary cooling system (DRACS) passive decay removal of liquid metal fast reactors, and the transparent, high volumetric heat capacitance liquid fluoride salt working fluids - Flibe - from molten salt reactors. This combination of fuel and coolant enables FHRs to operate in a high-temperature low-pressure design space that has beneficial safety and economic implications. The PB-FHR reactor relies on a pebble bed approach and pebble bed reactors are in a sense the poster child for multiscale analysis. The lower length-scale simulator for pebble reactor cores comprises three physics: neutronics (OpenMC), thermal-fluids (Nek5000) and fuel performance (BISON). As part of center of excellence ongoing research efforts we have developed “Cardinal”, a new tool platform for lower length-scale simulation. Cardinal tightly couples all three physics and leverages advances in MOOSE such as the MultiApp system and the concept of MOOSE-wrapped Apps. Moreover it is designed from the ground-up to scale on massively parallel architectures and perform well on world-class super-computing architectures. In this report we describe the design of Cardinal and present a demo of the application of Cardinal to an FHR.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗
DOE OSTI2022

Integration of Control Methods and Digital Twins for Advanced Nuclear Reactors

Advanced nuclear reactors offer a new set of features to energy generation, due to their ability to adapt to variable energy demand, operate autonomously, be deployed in rural locations and monitored remotely, afford compact size and lower power ratings, and rely on novel technologies to achieve safer operations. Thus, a requirement for the success of these reactors is the use of intelligent forms of control to track changing power demands, make autonomous decisions, and reduce the need for human involvement. Regulatory requirements pertaining to control of nuclear reactors could be met via historical means of control; however, these are not expected to enable the level of highly autonomous operations desired in advanced nuclear reactors. Historical control methods rely on both logical and high-performance (HP) control. These two types of control are usually used separately, with a human element being introduced whenever decisions are cascaded from one science to another. AI/ML control, on the other hand, can replace the human element in the current U.S. fleet of nuclear power plants (NPPs) by acting as a supervisory optimizer that understands the plant internal/external variables in order to make control decisions, and can easily handle non-linear and multi-input/multi out (MIMO) decisions—another requirement for advanced nuclear reactors that could be difficult to handle via logical and HP control. Because of the harsh operating environments produced in advanced reactors, resulting in the frequent failure of sensors and other types of equipment, and considering the lack of operating history for advanced nuclear reactors, control of advanced nuclear reactors would necessitate relying on a model that can track and adapt to the actual process (i.e., a digital twin). This digital twin can make approximations when knowledge and data are unavailable and would evolve as more knowledge is gained. The reactor control must also be risk-informed to account for the high-consequence nature of advanced reactors. This report introduces a high-level (i.e., not method- or process-specific) integration of the three different control and digital twinning methods able to meet the requirements for advanced nuclear reactors. These methods could be applied during both the operational and design stages of these reactors. The aim is to demonstrate how each method interfaces with and highlights enabling solutions necessitated by the unique features of advanced nuclear reactors.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2026

Radiological Releases from Novel Fuel Forms in Advanced Reactors During Severe Accidents for Consequence Analyses

Various advanced reactor developers are exploring the potential for reductions in the size of physical security forces and emergency planning zones. These reductions are based on robust fuel forms and inherently safe reactor designs. However, such reductions in physical protection measures could increase the risk of sabotage. To assess the possibility of reducing these measures, sabotage-induced radiological consequence analyses were carried out. These analyses considered accident scenarios that were beyond design basis accidents and overly conservative (Shah, 2025a; Shah, 2025b; Shah and Hartanto, 2026), yielding very large release fractions. These fractions, which can be used to evaluate physical protection and emergency planning requirements, have been crudely determined and applied as demonstrations for a sodium-cooled fast reactor (SFR) (Shah and Hartanto, 2025a), a high-temperature gas-cooled reactor (HTGR) (Shah and Hartanto, 2025b), a heat pipe–cooled reactor (HPR) (Shah and Hartanto, 2025c), and a molten salt–cooled reactor (MSR) (Shah et al., 2026). A Sandia National Laboratories (SNL) team used MELCOR—a fully integrated severe accident analysis code—to demonstrate the code’s capability to analyze advanced (i.e., not light water–cooled) reactors (including a fluoride salt–cooled high-temperature reactor [FHR]) and calculate radiological releases to the environment during severe accidents (Wagner et al., 2022a, 2022b, 2022c, 2023a, and 2023b). Although the analyses were carried out to demonstrate MELCOR’s growing capability, the release source terms were estimated for advanced reactors, providing valuable insights into the accident progression and radiological releases. These findings from prior SNL studies, including estimated source terms and related sensitivity studies, were leveraged to derive source terms for postulated sabotage-induced accidents. Insights from these sensitivity studies informed the scaling of SNL’s estimated source terms for the defined accident scenarios. The derived release fractions for the severe accident scenarios for the respective reactor designs can be used to perform more nuanced dose consequence analyses to evaluate the reactors’ physical protection and emergency planning zone requirements. These analyses are in accordance with the risk-informed, performance-based approach proposed under 10 CFR Part 53. This study builds on the prior source term analyses and associated sensitivity studies by SNL to derive time-dependent and design-informed release fractions. Section 2 describes the diverse advanced reactor designs analyzed by the SNL team. Section 3 discusses the severe accident analyses, the release fractions calculated, and the limitations and assumptions of the demonstration project. Section 4 presents the release percentages derived for the hypothetical sabotage-induced severe accidents at the advanced reactors. Section 5 summarizes the study’s findings and conclusions.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗
DOE OSTI2012

Enhancing VHTR Passive Safety and Economy with Thermal Radiation Based Direct Reactor Auxiliary Cooling System

One of the most important requirements for Gen. IV Very High Temperature Reactor (VHTR) is passive safety. Currently all the gas cooled version of VHTR designs use Reactor Vessel Auxiliary Cooling System (RVACS) for passive decay heat removal. The decay heat first is transferred to the core barrel by conduction and radiation, and then to the reactor vessel by thermal radiation and convection; finally the decay heat is transferred to natural circulated air or water systems. RVACS can be characterized as a surface based decay heat removal system. The RVACS is especially suitable for smaller power reactors since small systems have relatively larger surface area to volume ratio. However, RVACS limits the maximum achievable power level for modular VHTRs due to the mismatch between the reactor power (proportional to volume) and decay heat removal capability (proportional to surface area). When the relative decay heat removal capability decreases, the peak fuel temperature increases, even close to the design limit. Annular core designs with inner graphite reflector can mitigate this effect; therefore can further increase the reactor power. Another way to increase the reactor power is to increase power density. However, the reactor power is also limited by the decay heat removal capability. Besides the safety considerations, VHTRs also need to be economical in order to compete with other reactor concepts and other types of energy sources. The limit of decay heat removal capability set by using RVACS has affected the economy of VHTRs. A potential alternative solution is to use a volume-based passive decay heat removal system, called Direct Reactor Auxiliary Cooling Systems (DRACS), to remove or mitigate the limitation on decay heat removal capability. DRACS composes of natural circulation loops with two sets of heat exchangers, one on the reactor side and another on the environment side. For the reactor side, cooling pipes will be inserted into holes made in the outer or inner graphite reflector blocks. There will be gaps between these cooling pipes and their corresponding surrounding graphite surfaces. Graphite has an excellent heat conduction property. By taking advantage of this feature, we can have a volume-based method to remove decay heat. The scalability can be achieved, if needed, by employing more rows of cooling pipes to accommodate higher decay heat rates. Since heat can easily conduct through the graphite regions between the holes made for the cooling pipes, those cooling pipes located further away from the active core region can still be very effective in removing decay heat. By removing the limit on the decay heat removal capability due to the limited available surface area as in a RVACS, the reactor power and power density can be significantly increased, without losing the passive heat removal feature. This paper will introduce the concept of using DRACS to enhance VHTR passive safety and economics. Three design options will be discussed, depending on the cooling pipe locations. Analysis results from a lumped volume based model and CFD simulations will be presented.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗
DOE OSTI2020

Assessment of Survey Results from Advanced Reactor Industry Domain Experts on Nonlinear Soil-Structure Interaction Analysis Software Verification and Validation

The seismic load case has a significant impact on the design and cost of nuclear power plants. Given the need to substantially reduce cost, advanced reactor designers are looking to leverage numerical tools that enable seismic analysis of an integrated vessel/support/structure/soil system. Modern nonlinear analysis tools provide a solution, capturing dynamic coupling between components (including soil-structure interaction (SSI)) concurrent with nonlinear behavior in one or more parts of the system. Although these methods have a rich history of technical development and implementation, software quality assurance (SQA) following nuclear industry standards remains a significant burden for those wishing to adopt such methods for advanced reactor design and licensing. To reduce the SQA burden, this project will develop the guidance for SQA verification and validation (V&V) of coupled nonlinear SSI analysis tools, to include a test matrix of software features and test problems to support commercial grade dedication (CGD). The guidance is intended to be technology-neutral: supporting designers of all advanced reactors. To maximize the value of the project to reactor designers, the project team performed focused surveys of and interviews with advanced reactor designers. Additionally, the project surveyed members of the broader industry involved in reactor design and licensing. The aggregated industry feedback consists of written survey responses, live polling responses, focused interviews, and informal feedback provided after outreach presentations, collectively referred to as “survey results”. Herein, the survey results are reported, reviewed, and assessed to inform follow-on project activities. The survey results confirmed the familiarity of the industry with the coupled nonlinear SSI analysis. They also affirm the project need based upon the expressed intent to (1) incorporate nonlinear features and (2) pursue the coupled nonlinear SSI analysis to reduce seismic demands and construction costs. All reactor designers indicated their intent to incorporate two or more nonlinear features, and all reactor designer respondents opined that the coupled nonlinear SSI analysis would allow for the optimization of the reactor design and construction. However, the programmatic challenges, whether real or perceived, present a significant barrier to reactor designers. The barrier most commonly identified by the reactor designer population was regulatory risk, with 70% citing this as a reason not to pursue the approach. The perceived regulatory risk identified by the reactor designers underscores the importance of regulator engagement and dialogue in this project. Additionally, half of the reactor designers identified cost and lack of guidance as a deterrent. The survey results also provide insights to tailor specific aspects of the guidance document and test matrix. The project plans to prepare both a formal referenceable guidance document and a collaborative, web-based test matrix and problem set. The project will focus on more complete test problem definitions for the prioritized nonlinear features over shallower problem descriptions for a larger set of features. The nonlinearities prioritized as high based upon survey feedback include fluid-structure interaction and seismic isolation and energy dissipation devices. The nonlinearities prioritized as intermediate include nonlinear geomaterials, nonlinear concrete, nonlinear steel, and interface/contact nonlinearity. Deep embedment and the associated nonlinear phenomena are assigned the lowest priority based upon survey feedback.

42 ENGINEERING↗
DOE OSTI2017

Versatile Irradiation Test Reactor User Needs Assessment

An assessment of potential test reactor industry user needs has been completed. The needs of DOE R&D programs have also been assessed and included in this document. A process of discussions with industry representatives under non-disclosure agreements (NDAs) was undertaken during the last half of the calendar year. This activity was performed by staff members of the Idaho National Laboratory (INL), Argonne National Laboratory (ANL) and Oak Ridge National Laboratory (ORNL). Contributors to this assessment were selected from a list of representative organizations. As the duration for completion was short, all reactor vendors were not included and some chose not to participate. However, the contributors represent well-established reactor vendors and reactor developers working to bring new designs to the reactor market. Equally important was the breadth of the reactor technologies that are included: sodium cooled fast reactors, lead cooled fast reactors, high-temperature gas-cooled reactors, light water reactors and molten salt reactors. Throughout this report the term Molten Salt Reactors is used to represent all of the variants of molten-salt cooled reactors with either dissolved or solid fuel: fast, thermal, dissolved and prismatic fueled.

99 GENERAL AND MISCELLANEOUS↗
DOE OSTI2015

Delayed Gamma Measurements in Different Nuclear Research Reactors Bringing Out the Importance of the Delayed Contribution in Gamma Flux Calculations

Neutron and gamma flux levels are key parameters in nuclear research reactors. In Material Testing Reactors, such as the future Jules Horowitz Reactor, under construction at the French Alternative Energies and Atomic Energy Commission (CEA Cadarache, France), the expected gamma flux levels are very high (nuclear heating is of the order of 20 W/g at 100 MWth). As gamma rays deposit their energy in the reactor structures and structural materials it is important to take them into account when designing irradiation devices. There are only a few sensors which allow measurements of the nuclear heating ; a recent development at the CEA Cadarache allows measurements of the gamma flux using a miniature ionization chamber (MIC). The measured MIC response is often compared with calculation using modern Monte Carlo (MC) neutron and photon transport codes, such as TRIPOLI-4 and MCNP6. In these calculations only the production of prompt gamma rays in the reactor is usually modelled thus neglecting the delayed gamma rays. Hence calculations and measurements are usually in better accordance for the neutron flux than for the gamma flux. In this paper we study the contribution of delayed gamma rays to the total MIC signal in order to estimate the systematic error in gamma flux MC calculations. In order to experimentally determine the delayed gamma flux contributions to the MIC response, we performed gamma flux measurements with CEA developed MIC at three different research reactors: the OSIRIS reactor (MTR - 70 MWth at CEA Saclay, France), the TRIGA MARK II reactor (TRIGA - 250 kWth at the Jozef Stefan Institute, Slovenia) and the MARIA reactor (MTR - 30 MWth at the National Center for Nuclear Research, Poland). In order to experimentally assess the delayed gamma flux contribution to the total gamma flux, several reactor shut down (scram) experiments were performed specifically for the purpose of the measurements. Results show that on average about 30 % of the MIC signal is due to the delayed gamma rays. In this paper we describe experiments in each of the three reactors and how we estimate delayed gamma rays with MIC measurements. The results and perspectives are discussed. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗
DOE OSTI2016

Study of Reactor BN-350 Wastewater Impact on the Environment

The fast neutron reactor BN-350 had a dual purpose: steam production and plutonium accumulation. The steam produced in the reactor was used to generate electricity (up to 150 MW) and desalination of seawater (up to 120,000 tons/day). The BN-350 reactor became operational in July 1973; its design operation lifetime was 20 years. After expiration of the reactor design lifetime in July 1993, its subsequent operation was continued according to the annual decisions on extension of the reactor operation, by one year. The reactor has been idle since December 1998. On April 22, 1999 Resolution No. 456 'About decommissioning of the BN-350 reactor in Aktau, Mangistau region' was adopted by the RK Government. Thus, the total operation period of the reactor was more than 25 years. One of the important issues related to the long-term operation of a radiation-hazardous facility, such as the BN-350 reactor, is to assess its impact on the environment. The necessity and urgency of detailed studies of the radiation situation is explained by the location of the Caspian Sea and Aktau city in the area of the BN-350 reactor's potential impact. This paper describes the preliminary results of the evaluation of the BN-350 reactor's effect on the level of radionuclide contamination of surface water, including the Caspian Sea via the mechanism of radionuclide discharge in wastewater. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
DOE OSTI2015

Optimization of tritium breeding and shielding analysis to plasma in ITER fusion reactor

The development of fusion energy is one of the important International energy strategies with the important milestone is ITER (International Thermonuclear Experimental Reactor) project, initiated by many countries, such as: America, Europe, and Japan who agreed to set up TOKAMAK type fusion reactor in France. In ideal fusion reactor the fuel is purely deuterium, but it need higher temperature of reactor. In ITER project the fuels are deuterium and tritium which need lower temperature of the reactor. In this study tritium for fusion reactor can be produced by using reaction of lithium with neutron in the blanket region. With the tritium breeding blanket which react between Li-6 in the blanket with neutron resulted from the plasma region. In this research the material used in each layer surrounding the plasma in the reactor is optimized. Moreover, achieving self-sufficiency condition in the reactor in order tritium has enough availability to be consumed for a long time. In order to optimize Tritium Breeding Ratio (TBR) value in the fusion reactor, there are several strategies considered here. The first requirement is making variation in Li-6 enrichment to be 60%, 70%, and 90%. But, the result of that condition can not reach TBR value better than with no enrichment. Because there is reduction of Li-7 percent when increasing Li-6 percent. The other way is converting neutron multiplier material with Pb. From this, we get TBR value better with the Be as neutron multiplier. Beside of TBR value, fusion reactor can analyze the distribution of neutron flux and dose rate of neutron to know the change of neutron concentration for each layer in reactor. From the simulation in this study, 97% neutron concentration can be absorbed by material in reactor, so it is good enough. In addition, it is required to analyze spectrum neutron energy in many layers in the fusion reactor such as in blanket, coolant, and divertor. Actually material in that layer can resist in high temperature and high pressure condition for more than ten years.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2021

Comparison of Irradiated TRISO Fuel Radioactivity from Multiple Advanced Reactor Designs

The SCALE code system was used to model, deplete, and compare several different TRISO-fueled reactor designs: a helium-cooled prismatic reactor, a helium-cooled pebble-bed reactor (PBR), and a Fluoride-Lithium-Beryllium (FLIBE) molten-salt-cooled PBR. The purpose of this comparison was to understand how differences in the reactor designs affect the radioactivity of the fuel after discharge and whether those differences are significant. First, the various reactor designs were build and depleted in the TRITON module for each design and fuel enrichment. Then, the TRITON outputs were used to create burn-up dependent reactor libraries. These libraries were then used by ORIGEN to determine the activities of discharged fuel for each reactor, which were compared to generic Westinghouse 17x17 fuel. Overall, the results showed that short term decays are dominated by reactors with higher operating powers, and the reactor type, initial fuel enrichment, and maximum burn-up are of only secondary importance. Although this analysis only focuses on activities in becquerels, these dependencies are consistent with the expected behavior of decay heat. However, analysis of long- term time periods post-irradiation shows that the reactor type and maximum burn-up have strong impacts on the activities; initial fuel enrichment has a secondary impact while operating power is inconsequential. These results would be useful for analyses, such as dose assessment and modeling in post- release scenarios; normal fuel handling operations; and spent fuel transport, storage and disposal. Of particular interest, the results in this report show that analyses that focus on spent nuclear fuel of advanced reactors need to consider each parameter carefully. Unsurprisingly, if the correct operating power is not used in short term analyses, the results will not be correct. Perhaps unexpectedly, however, if the correct reactor type is not used, then the long term results will also be incorrect, especially for areas such as permanent disposal. Even though this report focuses on the total activity of nuclear fuel, it provides initial results on the effects of various input parameters and also provides a framework to extend the work into other analyses of spent fuel from advanced reactors, especially those employing TRISO fuel.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2013

Burnup Concept for a Long-Life Fast Reactor Core using MCNPX

This report describes a reactor design with a burnup concept for a long-life fast reactor core that was evaluated using Monte Carlo N-Particle eXtended (MCNPX). The current trend in advanced reactor design is the concept of a small modular reactor (SMR). However, very few of the SMR designs attempt to substantially increase the lifetime of a reactor core, especially without zone loading, fuel reshuffling, or other artificial mechanisms in the core that “flatten” the power profile, including non-uniform cooling, non-uniform moderation, or strategic poison placement. Historically, the limitations of computing capabilities have prevented acceptable margins in the temporal component of the spatial excess reactivity in a reactor design, due primarily to the error in burnup calculations. This research was performed as an initial scoping analysis into the concept of a long-life fast reactor. It can be shown that a long-life fast reactor concept can be modeled using MCNPX to predict burnup and neutronics behavior. The inherent characteristic of this conceptual design is to minimize the change in reactivity over the lifetime of the reactor. This allows the reactor to operate substantially longer at full power than traditional Light Water Reactors (LWRs) or other SMR designs. For the purpose of this study, a single core design was investigated: a relatively small reactor core, yielding a medium amount of power (~200 to 400 MW th ). The results of this scoping analysis were successful in providing a preliminary reactor design involving metal U-235/U-238 fuel with HT-9 fuel cladding and sodium coolant at a 20% volume fraction.

Holschuh, Thomas Vernon↗
DOE OSTI2021

Nuclear Data to Reduce Uncertainties in Reactor Antineutrino Measurements

The large quantities of antineutrinos produced through the decay of fission fragments in nuclear reactors provide an opportunity to study the properties of these particles and investigate their use in reactor monitoring. The reactor antineutrino spectra are measured using specialized, large area detectors that detect antineutrinos through inverse beta decay, electron elastic scattering, or coherent elastic neutrino nucleus scattering; although, inverse beta decay is the only demonstrated method so far. Reactor monitoring takes advantage of the differences in the antineutrino yield and spectra resulting from uranium and plutonium fission providing an opportunity to estimate the fissile material composition in the reactor. Recent experiments reveal a deviation between the measured and calculated antineutrino flux and spectra (the reactor anomaly) indicating either the existence of yet undiscovered neutrino physics, uncertainties in the reactor source term calculation, incorrect nuclear data, or a combination of all three. To address the nuclear data that impact the antineutrino spectrum calculations and measurements, an international group of over 180 experts in antineutrino physics, reactor analysis, detector development, and nuclear data came together during the Workshop on Nuclear Data for Reactor Antineutrino Measurements (WoNDRAM) to discuss nuclear data needs and achieve concordance on a set of recommended priorities for nuclear data improvements. Three topical sessions focused on the reactor source term, the antineutrino spectrum, and the detector response, provided a forum to gain consensus amongst the participants on the most important data improvements to address two goals: 1) understand the reactor anomaly and 2) improve the ability to monitor reactors using antineutrinos. This report summarizes the outcomes of the workshop discussions and the recommendations for nuclear data efforts that reduce reactor antineutrino measurement uncertainties.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2013

Predicting Reactor Antineutrino Emissions Using New Precision Beta Spectroscopy

Neutrino experiments at nuclear reactors are currently vital to the study of neutrino oscillations. The observed antineutrino rates at reactors are typically lower than model expectations. This observed deficit is called the “reactor neutrino anomaly”. A new understanding of neutrino physics may be required to explain this deficit, though model estimation uncertainties may also play a role in the apparent discrepancy. PNNL is currently investigating an experimental technique that promises reduced uncertainties for measured data to support these hypotheses and interpret reactor antineutrino measurements. The experimental approach is to 1) direct a proton accelerator beam on a metal target to produce a source of neutrons, 2) use spectral tailoring to modify the neutron spectrum to closely simulate the energy distribution of a power reactor neutron spectrum, 3) irradiate isotopic fission foils (235U, 238U, 239Pu, 241Pu) in this neutron spectrum so that fissions occur at energies representative of a reactor, 4) transport the beta particles released by the fission products in the foils to a beta spectrometer, 5) measure the beta energy spectrum, and 6) invert the measured beta energy spectrum to an antineutrino energy spectrum. A similar technique using a beta spectrometer and isotopic fission foils was pioneered in the 1980’s at the ILL thermal reactor. Those measurements have been the basis for interpreting all subsequent antineutrino measurements at reactors. A basic constraint in efforts to reduce uncertainties in predicting the antineutrino emission from reactor cores is any underlying limitation of the original measurements. This may include beta spectrum energy resolution, the absolute normalization of beta emission to number of fission, statistical counting uncertainties, lack of 238U data, the purely thermal nature of the IIL reactor neutrons used, etc. An accelerator-based neutron source that can be tailored to match various reactor neutron spectra provides an advantage for control in studying how changes in the neutron spectra (i.e. "in the reactor core") affects the resulting fission product beta spectrum. Furthermore, the 238U antineutrino spectrum, which has not been measured, can be studied directly because of the enhanced 1 MeV fast neutron flux available at the accelerator source. A facility such as the Project X Injector Experiment (PXIE) 30 MeV proton linear accelerator at Fermilab is being considered for this experiment. The hypothesis is that a new approach utilizing the flexibility of an accelerator neutron source with spectral tailoring coupled with a careful design of an isotopic fission target and beta spectrometer and the inversion of the beta spectrum to the neutrino spectrum will allow further reduction in the uncertainties associated with prediction of the reactor antineutrino spectrum.

Asner, David M.↗
DOE OSTI2017

Assessment of Sensor Technologies for Advanced Reactors

This paper provides an assessment of sensor technologies and a determination of measurement needs for advanced reactors (AdvRx). It is a summary of a study performed to provide the technical basis for identifying and prioritizing research targets within the instrumentation and control (I&C) Technology Area under the Department of Energy’s (DOE’s) Advanced Reactor Technology (ART) program. The study covered two broad reactor technology categories: High Temperature Reactors and Fast Reactors. The scope of “High temperature reactors” included Gen IV reactors whose coolant exit temperatures exceed ≈650 °C and are moderated (as opposed to fast reactors). To bound the scope for fast reactors, this report reviewed relevant operating experience from US-operated Sodium Fast Reactor (SFR) and relevant test experience from the Fast Flux Test Facility (FFTF). For high temperature reactors the study showed that in many cases instrumentation have performed reasonably well in research and demonstration reactors. However, even in cases where the technology is “mature” (such as thermocouples), HTGRs can benefit from improved technologies. Current HTGR instrumentation is generally based on decades-old technology and adapting newer technologies could provide significant advantages. For sodium fast reactors, the study found that several key research needs arise around (1) radiation-tolerant sensor design for in-vessel or in-core applications, where possible non-invasive sensing approaches for key parameters that minimize the need to deploy sensors in-vessel, (2) approaches to exfiltrating data from in-vessel sensors while minimizing penetrations, (3) calibration of sensors in-situ, and (4) optimizing sensor placements to maximize the information content while minimizing the number of sensors needed.

Korsah, Kofi↗
DOE OSTI2019

Enhancing Research Reactor Safeguards Through the Use of Mailbox Declarations

There are historic examples in several States of research reactors being misused to produce undeclared nuclear material. However, misuse of a State’s research reactor has typically only been discovered after further investigation into the State’s non-compliance related to other undeclared activities. Light water research reactors are typically designed with sample irradiation ports, where the introduction of fertile material can illicitly produce fissile material. Additionally, some light water reactors continue to be fueled by highly enriched uranium, which is a more significant safeguards concern by the International Atomic Energy Agency (IAEA). Heavy water and graphite reactors can be used for illicit plutonium production, which is of particular proliferation concern. Because research reactors are designed for flexible operations and small research reactors are less frequently inspected by the IAEA than other nuclear facilities (depending on power and fuel type, it could several years between inspections), the likelihood of timely detection by the IAEA of misuse of the research reactor is low. During a 2013 workshop on safeguarding research reactors, the United States, France, and the United Kingdom made recommendations to the IAEA on how safeguards could be strengthened for such facilities. One of the recommendations was to assess the use of “mailbox” declarations coupled with short notice random inspections or unannounced inspections by the IAEA at research reactors. An electronic mailbox declaration refers to the use of a secure information repository into which an operator submits operating reports. The near real time submittal of information enables the IAEA to better implement randomized short notice inspections. These mailboxes are not used for collecting and submitting State reports to the IAEA, but for collecting and transmitting operator data. The use of mailboxes, in conjunction with short notice random inspections, is in routine use for some other facility types. This paper assesses the potential for the practical application of mailbox declarations for various research reactor types and how the approach could be effectively used. Potential diversion scenarios are described and operator data records are discussed in connection to mailbox declarations, including discussion of how the data could indicate research reactor misuse.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗