Engineering Papers⌕ Search

SEARCH · Engineering Papers

Results for “Nuclear Reactions”

Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

Quote a phrase for an exact phrase match. Source license links do not imply unrestricted reuse.

At least 505 records · Page 28
All sourcesNASA NTRSDOE OSTI
DOE OSTI2023

Measurement of the 25 Al(𝑑,𝑛)⁢ 26 Si reaction and impact on the 25 Al⁢(𝑝,𝛾)⁢ 26 Si reaction rate

The 25 Al(p,γ) 26 Si reaction plays a key role in nucleosynthesis pathways that influence the galactic abundance of 26 Al. A more precise determination of the proton strength of the lowest ℓ = 0 proton resonance in 26 Si is needed to improve reaction-rate calculations. This work measures the 25 Al(d,n) 26 Si proton-transfer reaction in inverse kinematics using a radioactive ion beam at RESOLUT, determining excitation energies and cross sections for the lowest ℓ = 0 resonance associated with the 3 + 3 state at 5.92(2) MeV. Coupled-reaction-channels calculations (FRESCO) are used to extract the ℓ = 0 spectroscopic factor and the corresponding proton width, yielding Γₚ = 2.19(45) eV and a (p,γ) resonance strength of 26(10) meV. This resonance is found to dominate the 25 Al(p,γ) 26 Si reaction rate above 0.2 GK.

20 ≤ A ≤ 38↗
DOE OSTI2025

Elastic scattering in the 12 N + 197 Au system at 𝐸 lab = 70 MeV

Halo structure is an interesting exotic configuration developed in some light weakly bound nuclei, where a valence particle orbits a nuclear core. Signatures of halo structure can be observed in the angular distributions of the elastic scattering induced by these nuclei at energies around the Coulomb barrier. There are some well-studied reactions with neutron-rich halo nuclei, such as 6 He and 11 Li . However, the information is scarce on the proton-rich side. Recent works confirm the halo structure in the 8B nuclei but still lack more experimental studies for other proton-halo candidates, such as 12 N and 17 F. In this work, we report experimental data for the elastic scattering of 12 N on 197 Au target at 𝐸 lab = 70 MeV. The 12 N is a proton-rich nucleus with proton separation energy 𝑆 𝑝 = 600 keV, which is higher than the 8 B (𝑆 𝑝 = 137 keV) and almost the same as the 17 F (𝑆 𝑝 = 601 keV). Data were obtained at the Cyclotron Institute of Texas A&M University where the 12 N radioactive beam was produced by the momentum achromatic recoil spectrometer. The calculation of the optical model was used to fit the measured angular distribution for the elastic scattering and to obtain the reaction cross section 𝜎 𝑅 . We also performed continuum discretized coupled-channel calculations to compare with the experimental data. The angular distribution of the elastic cross sections exhibits a suppression of the Fresnel peak. From the fitting of the optical model, we obtain the total reaction cross section, 𝜎 𝑅 = 1269 ± 41 mb. The agreement between the CDCC calculation and the experimental elastic scattering data is limited and the breakdown does not exhaust the measured 𝜎 𝑅 . The resulting reduced reaction cross section 𝜎 Red for 12 N + 197 Au is large and comparable to the one obtained for the 8 B + 208 Pb system. This suggests a strong decoupling of the valence proton from the core because of the low binding energy and a dynamic polarization effect. Here, more research is required to estimate the contribution of core excitation.

Elastic scattering reactions↗
DOE OSTI2023

g 9/2 neutron strength in the N = 29 isotones and the 52 Cr(d,p)⁢ 53 Cr reaction

We performed a measurement of the 52 Cr(d,p)⁢⁢ 53 Cr reaction at 16 MeV using the Florida State University Super-Enge Split-Pole Spectrograph (SE-SPS) and observed 26 states. While all of the states observed here had been seen in previous (d,p) experiments, we changed five L assignments from those reported previously and determined L values for nine states that had not had such assignments made previously. The g 9/2 neutron strength observed in 53 Cr in the present work and in the N = 29 isotones 49 Ca, 51 Ti, and 55 Fe via (d,p) reactions is much smaller than the sum rule for this strength. Most of the observed L = 4 strength in these nuclei is located in states near 4 MeV excitation energy. The remaining g 9/2 strength may be located in the continuum or may be fragmented among many bound states. A covariant density-functional theory calculation provides support for the hypothesis that the g 9/2 neutron orbit is unbound in 53 Cr. The (α, 3 He) reaction may provide a more sensitive probe for the missing g 9/2 neutron strength. Additionally, particle-γ coincidence experiments may help resolve some remaining questions in this nucleus.

39 ≤ A ≤ 58↗
DOE OSTI2021

Measurement of deeply virtual Compton scattering off 4 He with the CEBAF Large Acceptance Spectrometer at Jefferson Lab

We report on the measurement of the beam spin asymmetry in the deeply virtual Compton scattering off $^4$He using the CEBAF Large Acceptance Spectrometer (CLAS) at Jefferson Lab using a 6 GeV longitudinally polarized electron beam incident on a pressurized $^4$He gaseous target. We detail the method used to ensure the exclusivity of the measured reactions, in particular the upgrade of CLAS with a radial time projection chamber to detect the low-energy recoiling $^4$He nuclei and an inner calorimeter to extend the photon detection acceptance at forward angles. Our results confirm the theoretically predicted enhancement of the coherent ($e^4$He$~\to~e'$$^4$He$'\gamma'$) beam spin asymmetries compared to those observed on the free proton, while the incoherent ($e^4$He$~\to~e'$p$'\gamma'$X$'$) asymmetries exhibit a 30$\%$ suppression. From the coherent data, we were able to extract, in a model-independent way, the real and imaginary parts of the only $^4$He Compton form factor, $\cal H_A$, leading the way toward 3D imaging of the partonic structure of nuclei.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Measuring the cross section of the N 15 ( α , γ ) 19 F reaction using a single-fluid bubble chamber

15 N(α, γ) 19 F is believed to be the primary means of stellar nucleosynthesis of fluorine. Here we present the use of a single-fluid bubble chamber to measure the cross section of the time-inverse photo-dissociation reaction. The method benefits from a luminosity increase of several orders of magnitude due to the use of a thicker liquid target - compared to thin films or gas targets - and from the reciprocity theorem. We discuss the results of experiments at the Thomas Jefferson National Accelerator Facility, where the cross section of the photodisintegration process 19 F(γ, α) 15 N was measured by bombarding a superheated fluid of C 3 F 8 with bremsstrahlung γ rays produced by impinging a 4 - 5.5 MeV electron beam on a Cu radiator. From the photodissociation yield the cross section was extracted by performing a convolution with a Monte Carlo–generated γ-ray beam spectrum. The measurement produced a cross section that was then time inverted using the reciprocity theorem. The cross section for the 15 N(α, γ) 19 F reaction was determined down to a value in the range of hundreds of picobarns. We report that with further improvements of the experimental setup the technique could potentially push cross section measurements down to the single picobarn range.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Nuclear recoil response of liquid xenon and its impact on solar 8B neutrino and dark matter searches

Knowledge of the ionization and scintillation responses of liquid xenon (LXe) to nuclear recoils is crucial for LXe-based dark matter experiments. Current calibrations carry large uncertainties in the low-energy region below ∼3 keV nr where signals from dark matter particles of <10 GeV/c 2 masses are expected. The coherent elastic neutrino-nucleus scattering (CE ν NS) by solar 8 B neutrinos also results in a continuum of nuclear recoil events below 3.0 keV nr (99% of events), which further complicates low-mass dark matter searches in LXe experiments. In this paper, we describe a method to quantify the uncertainties of low-energy LXe responses using published calibration data, followed by case studies to evaluate the impact of yield uncertainties on 8 B searches and low-mass dark matter sensitivity in a typical ton-scale LXe experiment. We conclude that naively omitting yield uncertainties leads to overly optimistic limits by factor ∼2 for a 6 GeV WIMP mass. Future nuclear recoil light yield calibrations could allow experiments to recover this sensitivity and also improve the accuracy of solar 8 B flux measurements.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2025

Measurement of beam-recoil observables 𝐶 𝑥 and 𝐶 𝑧 for 𝐾 + ⁢Λ photoproduction

Exclusive photoproduction of 𝐾 + ⁢Λ final states off a proton target has been an important component in the search for missing nucleon resonances and our understanding of the production of final states containing strange quarks. Polarization observables have been instrumental in this effort. The current work is an extension of previously published CLAS results on the beam-recoil transferred polarization observables 𝐶 𝑥 and 𝐶 𝑧 . Here, we extend the kinematic range up to invariant mass 𝑊 = 3.33 GeV from the previous limit of 𝑊 = 2.5 GeV with significantly improved statistical precision in the region of overlap. These data will provide for tighter constraints on the reaction models used to unravel the spectrum of nucleon resonances and their properties by not only improving the statistical precision of the data within the resonance region, but also constraining 𝑡-channel processes that dominate at higher 𝑊 but extend into the resonance region.

Electrons↗
DOE OSTI2022

Sensitivity of time-dependent density functional theory to initial conditions

Time-dependent density-functional theory is mathematically formulated through nonlinear coupled time-dependent three-dimensional partial differential equations, and it is natural to expect a strong sensitivity of its solutions to variations of the initial conditions, akin to the butterfly effect ubiquitous in classical dynamics. Since the Schrödinger equation for an interacting many-body system is, however, linear and mathematically the exact equations of the density-functional theory reproduce the corresponding one-body properties, it would follow that the Lyapunov exponents are also vanishing within a density-functional theory framework. Whether for realistic implementations of the time-dependent density-functional theory the question of the absence of the butterfly effect and whether the dynamics provided is indeed a predictable theory was never discussed. At the same time, since the time-dependent density-functional theory is a unique tool allowing us to study the nonequilibrium dynamics of strongly interacting many-fermion systems, the question of predictability of this theoretical framework is of paramount importance. Here our analysis, for a number of quantum superfluid many-body systems (unitary Fermi gas, nuclear fission, and heavy-ion collisions) with a classical equivalent number of degrees of freedom O(10 10 ) and larger, suggests that its maximum Lyapunov exponents are negligible for all practical purposes.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Coriolis coupling effects in proton-pickup spectroscopic factors from 12 B

Spectroscopic factors to low-lying negative-parity states in Be 11 extracted from the B 12 ( d , He 3 ) Be 11 proton-removal reaction are interpreted within the rotational model. Earlier predictions of the p -wave proton-removal strengths in the strong-coupling limit of the Nilsson model underestimated the spectroscopic factors to the 3 / 2 1 - and 5 / 2 1 - states and suggested that deviations in the 1 + ground state of the odd-odd B 12 due to Coriolis coupling should be further explored. Furthermore, in this work we use the particle rotor model to take into account these effects and obtain a good description of the level scheme in B 11 , with a moderate K mixing of the proton Nilsson levels [110]1/2 and [101]3/2. This mixing, present in the 1 + bandhead of B 12 , is key to explaining the proton-pickup data.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2026

Investigation of the 244 Pu ⁢( 48 Ca,𝑥⁢𝑛) 292−𝑥 Fl reaction with the LBNL SHREC detector: Investigation of decay chains of isotopes of flerovium (𝑍=114)

The 244 Pu ⁢( 48 Ca,𝑥⁢𝑛)⁢ 292−𝑥 Fl reaction was investigated at Lawrence Berkeley National Laboratory’s 88 Inch Cyclotron using the Berkeley Gas-filled Separator (BGS), the newly installed Superheavy Recoil detector, along with an upgraded digital electronics and data acquisition system. Seven decay chains were observed starting with an evaporation residue, followed by a single 𝛼 decay and a spontaneous fission. The decay characteristics of these seven decay chains led to an assignment to 288 Fl , the product of the 4⁢𝑛 reaction channel. Two additional chains were (tentatively) assigned to the decay of the 3⁢𝑛 exit channel, 289 Fl . Cross sections for the 4⁢𝑛 and 3⁢𝑛 exit channels were 𝜎 prod =6.7⁢($^{36}_{25}$) pb and 𝜎 prod =1.6⁢($^{22}_{11}$) pb, respectively. Another decay chain, tentatively assigned to the 5⁢𝑛 exit channel through the 48 Ca + 244 Pu reaction or the 3⁢𝑛 exit channel of the 48 Ca + 242 Pu reaction, was also detected. Detailed information regarding the observed decay chains and their nuclear structure aspects is discussed, along with the performance of the BGS and the new detection system.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

First measurement of 𝑎$^{0}_{2}$⁡(1320) polarized photoproduction cross section

We measure for the first time the differential photoproduction cross section dσ/dt of the a 2 (1320) meson at an average photon beam energy of 8.5 GeV, using data with an integrated luminosity of 104 pb −1 collected by the GlueX experiment. We fully reconstruct the γp → ηπ 0 p reaction and perform a partial-wave analysis in the a 2 (1320) mass region with amplitudes that incorporate the linear polarization of the beam. This allows us to separate for the first time the contributions of natural- and unnatural-parity exchanges. Furthermore, these measurements provide novel information about the photoproduction mechanism, which is critical for the search for spin-exotic states.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Intensity of a weak 519-keV γ ray following β decay of the superallowed emitter 34 Ar determined via the 33 S(p,γ) 34 Cl reaction

The predominant branch in the β decay of 34 Ar is the superallowed 0 + → 0 + transition to the ground state of 34 Cl. To determine its important branching ratio one must first establish the ratios for the competing Gamow-Teller branches based on the measured intensities of γ rays subsequently emitted from the excited states they populate in 34 Cl. The strongest of these branches populates the 1 + state at 666 keV in 34 Cl, which has three possible γ-decay paths. Here, we report here a measurement of the decay of this state, which we populated via resonant proton capture in the reaction 33 S(p,γ) 34 Cl. We find that the intensity of the 519-keV γ-ray path is 1.46(19)% relative to that of the 666-keV path. This result is critical to new precise measurements of the superallowed decay of 34 Ar.

20 ≤ A ≤ 38↗
DOE OSTI2020

Sensitivity of the 13 C(α,n) 16 O S factor to the uncertainty in the level parameters of the near-threshold state

The 13 C(α,n) 16 O reaction is the main source of neutrons for the s and i processes in asymptotic giant branch stars and carbon-enhanced metal-poor stars, respectively. The reaction rate over the relevant temperature range from 0.1 to 0.3 GK translates into a center-of-mass energy range of 150 to 540 keV. Current measurements extend down to 300 keV, still requiring an extrapolation of the cross section. At these low energies, the high-energy tail of a 1/2 + state near the reaction threshold makes a significant contribution to the cross section, but its amplitude is still highly uncertain. In this work the uncertainties associated with the low-energy cross-section extrapolation are investigated, in particular the sensitivity to the energy, width, and Coulomb renormalized asymptotic normalization coefficient of the near-threshold resonance. Furthermore, recently it has been suggested that the energy of the near-threshold level may have a large impact on the extrapolation, but this is not found to be the case compared with the other sources of uncertainty.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Ab initio single-neutron spectroscopic overlaps in lithium isotopes

We calculate single-neutron spectroscopic overlaps for lithium isotopes in the framework of the ab initio symmetry-adapted no-core shell model. We report the associated neutron-nucleus asymptotic normalization coefficients (ANCs) and spectroscopic factors (SFs) that are important ingredients in many reaction cross-section calculations. While spectroscopic factors have been traditionally extracted from experimental cross sections, their sensitivity on the type of reactions, the energy, and the underlying models point to the need for determining SFs from first-principle structure considerations. As illustrative examples, we present 6 Li + n, 7 Li ⁢+ n, and 8 Li ⁢+ n, and we show that the results are in a good agreement with those of other ab initio methods, where available, including the quantum Monte Carlo approach. Here, we compare ANCs and SFs to available experimentally deduced values, with a view toward expanding this study to heavier nuclei and to extracting intercluster effective interactions for input into analyses of existing and future experimental data.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

First experiment at the Super Heavy Element Factory: High cross section of Mc 288 in the Am 243 + Ca 48 reaction and identification of the new isotope Lr 264

Here, we present results of the first experiment aimed at the synthesis of Mc isotopes in the 243 Am+ 48 Ca reaction performed at the new gas-filled separator DGFRS-2 online to the new cyclotron DC280 at the Super Heavy Element Factory at JINR. Fifty-five new decay chains of 288 Mc and six chains assigned to 289 Mc were detected. The α decay of 268 Db with an energy of 7.6–8.0 MeV, half-life of 16$^{+6}_{-4}$h, and a branch of 55$^{+20}_{-15}$% was registered for the first time, and a new spontaneously fissioning isotope 264 Lr with a half-life of 4.9$^{+2.1}_{-1.3}$h was identified. The cross section for the 243 Am( 48 Ca,3n) 288 Mc reaction was measured to be 17.1$^{+6.3}_{-4.7}$ pb, which is the largest value for the known superheavy nuclei at the island of stability.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

New 13 C(α,n) 16 O Cross Section with Implications for Neutrino Mixing and Geoneutrino Measurements

Precise antineutrino measurements are very sensitive to proper background characterization. Here, we present an improved measurement of the 13 C(α,n) 16 O reaction cross section which constitutes significant background for large v¯ detectors. We greatly improve the precision and accuracy by utilizing a setup that is sensitive to the neutron energies while making measurements of the excited state transitions via secondary γ-ray detection. Our results shows a 54% reduction in the background contributions from the 16 O(3–, 6.13 MeV) state used in the KamLAND analysis.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

γ -ray spectroscopy of astrophysically important states in Ca 39

Background: Nova explosions synthesize elements up to A ≃ 40 , and discrepancies exist between calculated and observed abundances of Ar and Ca created in the explosion. The K 38 ( p , γ ) Ca 39 reaction rate has been illustrated to be influential on these isotopic abundances at the endpoint of nova nucleosynthesis. The energies of the three most important resonances, corresponding to J π = 5 / 2 + excited states in the Ca 39 nucleus above the proton separation threshold, are uncertain and one has been measured with conflicting values [ E r = 679 ( 2 ) versus E r = 701 ( 2 ) keV] in previous experiments. Purpose: Reducing the uncertainties on the resonance energies would allow for a better understanding of the reaction rate. To improve these uncertainties, we searched for γ rays from the depopulation of the corresponding excited states in Ca 39 . Methods: We report a new measurement of these resonance energies via the observation of previously unobserved γ -ray transitions. These transitions were observed by studying the Ca 40 ( 3 He , α γ ) Ca 39 reaction with Gammasphere ORRUBA Dual Detectors for Experimental Structure Studies (GODDESS). The updated resonance energies were then used to calculate the K 38 ( p , γ ) Ca 39 reaction rate and assess its uncertainties. Results: In total, 23 new transitions were found, including three γ -ray transitions corresponding to the three J π = 5 / 2 + states of astrophysical interest at energies of 6156.2(16), 6268.8(22), and 6470.8(19) keV. These correspond to resonance energies in the K 38 ( p , γ ) Ca 39 reaction of 386(2), 498(2), and 701(2) keV. Conclusions: Updated K 38 ( p , γ ) Ca 39 reaction rate calculations reflect a reduced upper limit at nova temperatures. However, the lower-than-previously-measured energy of the 498-keV resonance and uncertainty in its resonance strength increases the upper limit of the rate close to previous estimates at 0.4 GK.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

Alpha-decay width of a near proton-threshold resonance in the 7 Li( α, α ) channel

We investigate the alpha-decay width of a near proton-threshold resonance in 11 B by the excitation functions of 7 Li(α, α) and 7 Li(α, α’) reactions. This resonance is an example of loosely bound atomic nuclei, understood as small open quantum systems, that exhibit properties significantly influenced by their coupling to the continuum. The present experiment focuses on the formation of a specific state in 11 B at excitation energy in the region near 11.4 MeV by bombarding a 7 Li target with a 4 He beam at energies ranging from 3.92 to 4.56 MeV in the laboratory frame. The study provides data complementary to previous observations of the proton emission in the β-decay of the neutron-rich halo nucleus 11 Be. An R-matrix fit to the data provides resonance energy and partial widths consistent with J π =1/2 + for a narrow near-threshold state in 11 B at 11.400(20) MeV, that is 171(20) keV above the proton emission threshold, with partial α-decay width Γ α =2.5$^{+3.5}_{–1.5}$ keV in elastic scattering and Γ α' =15.8$^{+1.9}_{–0.4}$ keV in inelastic scattering. These findings contribute to the understanding of the structure of this open quantum system resonance.

11B↗