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At least 505 records · Page 28

A Grassroots Network and Community Roadmap for Interconnected Autonomous Science Laboratories for Accelerated Discovery

Scientific discovery is being revolutionized by AI and autonomous systems, yet current autonomous laboratories remain isolated islands unable to collaborate across institutions. We present the Autonomous Interconnected Science Lab Ecosystem (AISLE), a grassroots network transforming fragmented capabilities into a unified system that shorten the path from ideation to innovation to impact and accelerates discovery from decades to months. AISLE addresses five critical dimensions: (1) cross-institutional equipment orchestration, (2) intelligent data management with FAIR compliance, (3) AI-agent driven orchestration grounded in scientific principles, (4) interoperable agent communication interfaces, and (5) AI/ML-integrated scientific education. By connecting autonomous agents across institutional boundaries, autonomous science can unlock research spaces inaccessible to traditional approaches while democratizing cutting-edge technologies. This paradigm shift toward collaborative autonomous science promises breakthroughs in sustainable energy, materials development, and public health.

Ferreira da Silva, Rafael [Oak Ridge National Labo↗

Co-sputter deposition of Nb₃Sn layer into SRF cavity using Nb-Sn composite target

Nb₃Sn, with its superior superconducting critical temperature (Tc ~18.3 K) and superheating field (Hsh ~400 mT), is considered a promising material for superconducting radiofrequency (SRF) cavities, offering enhanced cryogenic performance compared to bulk niobium cavities. A Nb₃Sn coating technique has been developed for Nb SRF cavities using co-sputtering of Nb-Sn composite target in a DC cylindrical magnetron sputtering system. The composite target configuration and discharge conditions for co-sputtering were optimized to deposit Nb-Sn films on flat Nb substrates, followed by annealing to form Nb₃Sn. Multiple strategies have been explored to improve the surface homogeneity of the Nb₃Sn coating, including optimizing a two-step annealing process, annealing in Sn vapor, and a light Sn recoating process. A 1.5 µm Nb-Sn co-sputtered film was deposited on the interior of a 2.6 GHz Nb SRF cavity and annealed at 600 °C for 6 h, followed by 950 °C for 1 h. Cryogenic RF testing of the annealed cavity demonstrated a Tc of 17.8 K, confirming the formation of Nb₃Sn. Then, the annealed cavity underwent a light recoating treatment and attained a quality factor (Q0) of 8.5E+08 at 2.0 K.

Accelerator Physics↗

BEAM ACCELERATION WITH A Nb3Sn CRYOMODULE AT JLAB

We report on the electron beam acceleration experiment with a Nb3Sn cryomodule at Thomas Jefferson National Laboratory (JLAB). Two CEBAF-style 5-cell 1.5 GHz Nb3Sn cavities operated at 4 K, accelerating a 100 nA continuous-wave (CW) electron beam from 200 keV to 4 MeV at JLAB’s Upgraded Injector Test Facility (UITF). The acceleration gradients in each cavity reached 11 MV/m and 7 MV/m, respectively. No field emission was observed. The unloaded quality factors reached 2¿109 at low fields at 4 K.

Geng, R. [Thomas Jefferson National Accelerator Fa↗

Sputter coating of Nb₃Sn into SRF cavity using stoichiometric target

Nb₃Sn has emerged as a leading alternative material due to its higher superconducting critical temperature (Tc) and superheating field (Hsh), promising a viable solution to the intrinsic performance limit currently faced by Nb superconducting radiofrequency (SRF) cavities. We sputter-coated Nb₃Sn inside Nb SRF cavity using a stoichiometric Nb₃Sn tube target in a DC cylindrical magnetron sputter coater. The target was fabricated by growing an estimated >20 μm thick Nb₃Sn layer on a Nb tube via Sn vapor diffusion using Jefferson Lab’s coating system. Approximately 150 nm thick Nb-Sn films were sputter-deposited onto flat Nb samples at positions representing the beam tubes and equator of a 2.6 GHz Nb cavity. Post-deposition annealing at 950 °C for 3 h resulted in the formation of Nb₃Sn. Microstructural analysis of the annealed films was carried out to investigate the morphology and structure of the Nb₃Sn films. Later, a 2.6 GHz Nb SRF cavity was coated with a ~1.2 μm thick sputtered Nb-Sn film using a stoichiometric Nb₃Sn target, followed by annealing. Cryogenic RF testing of the annealed cavity demonstrated a Tc of 17.8 K, indicating the formation of Nb₃Sn. After a light Sn recoating treatment, the cavity achieved a quality factor (Q0) of 6.7E+08 at lower field at 2.0 K.

Accelerator Physics↗

Physics Division Strategic Plan Fiscal Years 2020-2024

The vision of the Physics Division (PHY) at Argonne National Laboratory is to continue enhancing its role as a world-leading institution in basic nuclear physics research and its applications. Key to this vision is for PHY to continue to safely and effectively operate and evolve the capabilities of the Argonne Tandem Linac Accelerator System (ATLAS) facility to best serve its users. ATLAS is the Department of Energy (DOE) accelerator facility for low-energy nuclear physics research. The research carried out by PHY covers many themes in contemporary science but can be distilled into five areas of focus. These themes are interconnected, with continuously evolving synergies between the various groups and facilities in PHY and the broader Laboratory. This five-year strategic plan serves to illustrate our current capabilities and new directions related to these five areas of focus (ATLAS also develops an independent strategic plan): Accelerator research and design. The goal of this theme is to design, fabricate, test, and implement novel accelerator systems, with a focus on high-intensity ion and electron systems. These R&D activities have led to enhancements in the ATLAS accelerator system. Among others, the division’s accelerator systems are in use or planned for use at Fermilab, the Advanced Photon Source, and in a broad variety of applications at the Facility for Rare Isotope Beams (FRIB). Atom trapping and fundamental symmetries. The goal of this theme is to explore and exploit the uses of advanced laser cooling and trapping techniques to manipulate atoms. There are three main areas of focus. First is in the application of the atom trap trace analysis (ATTA) technique for age determination of groundwater and ice by using radio-krypton dating. The next two trapping-based programs involve tests of fundamental symmetries in nature: the cooling and trapping of radium-225 with the aim of determining limits on an observation of its electric dipole moment and precision measurements of the beta decay properties of helium-6 to set limits on the tensor coupling constant. This is complemented by measurements of similar properties in lithium-8 and boron-8. Nuclear astrophysics. The goal of this theme is to enhance our understanding of how elements are created in the universe via explosive nucleosynthesis and how stars evolve. To meet the challenges of this theme, many of the capabilities of ATLAS are being enhanced, including the development of new beams through a new in-flight separator (RAISOR) and the anticipated neutron-generator upgrade of the Californium Rare Isotope Breeder Upgrade facility (nuCARIBU). These are coupled to state-of-the-art instruments such as the Canadian Penning Trap, Helical Orbit Spectrometer, Gammasphere, GRETINA, Multi-Sampling Ionization Chamber, the Fragment Mass Analyzer, and Argonne Gas-filled Fragment Analyzer, and a new low-background experimental area for decay studies. Nuclear structure. The goal of this theme is to understand the structure of nuclei, both stable and radioactive, in terms of single-particle properties, their shapes, and the dynamics governing reactions between them. These include questions such as what are the limits of nuclear stability and what are the properties of super heavy nuclei. As with the nuclear astrophysics theme, the capabilities of ATLAS, guided by the ATLAS user community, are continuously being enhanced to this end. The Division has strategic initiatives to play a leading role in the development of instrumentation and research programs at the FRIB. Quantum chromodynamics (QCD) and hadron physics. The goal of this theme is to lead major research programs focused on revealing the quark and gluon structure of protons, neutrons, nuclei, and short-lived mesons and baryons. These involve major programs at Jefferson Lab, Fermilab, and smaller facilities. They are complemented by theoretical endeavors centered on the question of how hadrons and their properties emerge from QCD. Out of these activities arise strategic initiatives to play a major role in the forthcoming Electron-Ion Collider (EIC).

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

A hybrid CNN-LSTM surrogate model for hyper-resolution spatiotemporal flood forecasting in Norfolk, Virginia

Study region: Norfolk, Virginia, United States Study focus: Accurate and timely flood forecasting is essential for enhancing resilience in coastal urban areas in the context of increasing frequency and intensity of rainfall, sea level rise and urbanization. This study presents a hybrid deep learning-based surrogate model that integrates Convolutional Neural Networks (CNN) and Long Short-Term Memory (LSTM) networks to enable real-time spatiotemporal flood forecasting. The model leverages CNN to capture spatial features from inputs such as elevation and Topographic Wetness Index (TWI), while LSTM processes time-series inputs of rainfall and tide data to capture temporal features. New hydrologic insights for the region: The hybrid CNN-LSTM model was trained using the physics-based hydrodynamic model simulations obtained from the Two-dimensional Unsteady FLOW (TUFLOW) model for Norfolk, Virginia, and achieved high predictive accuracy across diverse flood-prone areas. The reduced computational time from four to six hours using TUFLOW to 3.2 min per event using CNN-LSTM enables rapid flood inundation mapping and early warning applications. The model effectively captured both spatial flood extents and their temporal evolution across different flooding scenarios, providing forecasts at a 2.5-m spatial resolution and 15-min temporal resolution and a one-hour-ahead prediction horizon. While challenges remain in terms of transferability to new regions and real-time data assimilation, this approach demonstrates strong potential for supporting operational flood risk management in coastal urban environments.

Coastal urban flooding↗

APOLLO: a facility-scale differentiable virtual accelerator for Fermilab

As the design complexity of modern accelerators grows, there is more interest in using advanced simulations that have fast execution time or yield additional insights like gradients. The FAST/IOTA facility has been working on implementing and experimentally validating an end-to-end digital twin that is both fast and gradient-aware, allowing for rapid prototyping of new software and experiments with minimal beam time costs. Our framework integrates physics and ML codes for linac and ring simulation through a set of generic interfaces between surrogate and physics-based sections. To reproduce device inputs and outputs, system state is exposed as a deterministic discrete event simulator. Because Fermilab is undergoing control system transition, both EPICS and ACNET frontends are supported. Recently, we have begun transitioning to a new community lattice standard, PALS, as well as developing standardized infrastructure for data ingest and normalization to prepare for model calibration during FAST proton injector commissioning. We discuss implementation details as well as challenges, and future plans to extend modelling to main complex proton accelerators like PIPII and Booster.

Kuklev, Nikita [Fermilab]↗

Novel Materials and Concepts for Next-Generation High Power Target Applications

Novel beam-intercepting materials and targetry concepts are essential to improve the performance, reliability and operation lifetimes of next generation multi-megawatt (multi-MW) accelerator target facilities. The beam-intercepting materials and components must sustain an order-of-magnitude increase in particle beam intensities and are beyond the current state-of-the-art. With conventional materials already limiting the scope of experiments, it is crucial to investigate novel target materials, technologies and concepts that will satisfy the requirements and maximize the physics benefits of future energy and intensity frontier experiments. This paper provides an overview of the related targetry R&D required over the next 10 years to support and enable future high-power accelerator target facilities.

43 PARTICLE ACCELERATORS↗

Business Plan for a Domestic Supply of Superconducting Radiofrequency Cavities

Superconducting radiofrequency (SRF) cavities are critical components of modern particle accelerators. The industrialization of SRF technology in the U.S. has a long history, with several companies becoming interested in the technology in the past 30 years. However, there is currently no U.S. manufacturer with the capability to produce fully assembled, ready-to-test SRF cavities. A majority of these companies have either left the field or shut their doors. As a result, government-sponsored SRF accelerator projects in the U.S. largely rely on European vendors for the cavity supply. This presents not only a supply chain risk for scientific use cases, but also severely limits the commercialization of accelerator-based technologies. SRF accelerators have a range of strategic applications, including environmental remediation, semiconductor lithography, medical isotope production, and irradiation/sterilization. The nurturing of a domestic SRF industry is critical to maintaining U.S. economic competitiveness.

43 PARTICLE ACCELERATORS↗

Effects of Grain Size and Interstitial Content on Recrystallization in Nb after Cold Rolling

A fully recrystallized microstructure with a fine grain size can improve the performance of superconducting radio-frequency (SRF) cavities produced from high-purity Nb (ASTM B393–18 Type 5 Nb) while providing mechanical strength. Recrystallization depends on impurity content, initial microstructure, deformation state, and annealing conditions. To better understand how fine-grained, fully recrystallized microstructures may be produced, the recrystallization behaviors of Type 5 and Type 2 Nb materials were studied. Type 5 Nb specimens were produced with both fine and coarse initial grain sizes. All were cold rolled and then annealed under vacuum for one hour to determine the rolling reductions and temperatures required for recrystallization. The recrystallized fraction exceeded 95% in fine-grained Type 5 Nb rolled to a 30% or greater thickness reduction and then annealed at 800 °C or higher. The coarse grained Type 5 Nb required greater rolling reductions to produce any recrystallized grains at 800 °C. The higher interstitial content of the Type 2 Nb required a temperature of 1000 °C or higher to reach a recrystallized fraction greater than 95% in specimens rolled to a 60% reduction. Recrystallization is more easily achieved during annealing at a given temperature for a set time by increasing rolling reduction, decreasing interstitial content, and decreasing initial grain size prior to cold rolling. In conclusion, to avoid grain growth following recrystallization, which increases grain size, the minimum time and temperature necessary for complete recrystallization should be applied.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Chromaticity compensation of a ghost collider

The GHOST collider final focus system is a pure quadrupole-drift beamline targeting ¿* = 2 mm at four serial interaction points, with peak ¿-functions reaching ~65 km in the final triplet. Beam tracking simulations reveal that a nominal bunch develops a pronounced C-shape in longitu- dinal phase space at IP1, with ¿¿ growing from 0.15 mm to ~2.3 mm — a factor of ~15× increase that directly re- duces luminosity. The mechanism is identified as chromat- ically amplified betatron path length: off-momentum par- ticles acquire enlarged betatron amplitudes in the high-¿ final triplet, generating excess path length via the geometric ¿¿ = - 1/2 ¿ (¿'2 + ¿'2) ¿¿ integral. Within the monoenergetic Balandin framework, ¿2¿2 with ¿ = - 1/2 ¿ ¿ ¿¿ dominates ¿2¿2 by over four million times; the full beam ¿¿ is a fur- ther factor of ~27 larger, driven by ¿¿ -induced chromatic amplitude growth. Phase-advance scans confirm that ¿¿ is insensitive to the apochromatic (¿ ˜ 0) condition. When combined with the geometric hourglass effect, this distor- tion poses a challenge to maximizing luminosity within the current lattice design.

Gamage, B. [Thomas Jefferson National Accelerator ↗

Advancements in HF-free bipolar pulsed electropolishing for next-generation superconducting cavities

Hydrofluoric acid (HF)-free bipolar pulsed electropolishing (BPEP) offers an environmentally sustainable alternative to conventional Buffered Chemical Polishing (BCP) and Electropolishing (EP) techniques for superconducting radiofrequency (SRF) cavities. Recent studies at Jefferson Lab have demonstrated that a single-cell 1.3 GHz niobium cavity processed using HF-free BPEP achieved an accelerating gradient Eacc of 35 MV/m with a quality factor Q0 of 1E10 at 2 K, following extensive research and optimization. This talk will highlight the challenges encountered in developing this technique, key insights gained from experimental studies, and ongoing efforts to enhance its capabilities. In particular, we will explore its potential for refining Nb3Sn-coated niobium cavities via vapor diffusion techniques and for electroplating Nb3Sn films onto various cavity substrates, contributing to the advancement of high-performance SRF systems.

Tian, Hui [Thomas Jefferson National Accelerator F↗

Topographic Characterization of Niobium Films on Copper for SRF Applications

Niobium films on copper substrates are being actively developed as a low-cost alternative to bulk niobium for superconducting radio-frequency (SRF) cavities, offering superior thermal conductivity, reduced material cost, and the potential for scalable cavity fabrication. The performance of such films can be limited by imperfect surfaces that reduce the peak achievable magnetic field. Nb films deposited under varied electron cyclotron resonance conditions were characterized via atomic force microscopy. The films exhibit a corrugated surface morphology which can be characterized by the depth of the corrugation, slope angle, and standard roughness parameters. The influence of this surface roughness on field limitations is examined within the framework of London theory. These measurements and models aid in understanding how ECR deposition conditions influence the nanometer-scale roughness of Nb films on Cu and its impact on high-field SRF cavity performance.

Redman, Brandi [Old Dominion Univ., Norfolk, VA (U↗

DAOS Benchmarks and Findings

We benchmark DAOS on a 127-node, 4,064-target pool using fio, IOR, IO500, and mdtest, comparing the DFS API against DFuse+POSIX. Single-client fio sweeps show larger block sizes and writes yield higher bandwidth, with similar random/sequential performance. Multi-node IOR (1–32 nodes, 6–48 tasks/node) shows bandwidth saturating around 32 tasks/node, with large transfer sizes hurting read throughput at high concurrency and write latency growing faster than read latency. An 8-node IO500 run shows DFS achieving ~5x higher bandwidth and ~190x higher IOPS than POSIX. We also detail operational issues: SCM target-filling under mdtest, intermittent NA_HOSTUNREACH errors, fio CPU-affinity failures, and a pool error storm resolved by recreation.

George, Rebecca [Thomas Jefferson National Acceler↗

Benchmarking DAOS Filesystem on Aurora

We benchmark the DAOS filesystem on Argonne's Aurora supercomputer (127 nodes, 4,064 targets) using fio, IOR, mdtest, and IO500 to characterize I/O and metadata performance across the DFS API and DFuse+POSIX. Single-client fio shows POSIX bandwidth saturating at 1–2 MiB I/O sizes, with write-heavy workloads outperforming reads. Multi-node IOR shows DFS bandwidth scaling well up to ~32 tasks/node, with write latency growing faster than read latency. An 8-node IO500 evaluation shows DFS achieving ~5x higher bandwidth and ~190x higher IOPS than POSIX. Results indicate DAOS is well-suited to read-heavy workloads like AI training data loading, given appropriately sized transfers and concurrency.

George, Rebecca [College of William and Mary, Will↗

Robotic Assembly of SRF Cavity Pair

Superconducting Radio Frequency (SRF) cavities for particle accelerators require tight tolerances, ultrahigh vacuum, and strict cleanliness during assembly. As in the semiconductor industry, defects such as particles and residues are deleterious to performance, possibly rendering a cavity unfit for use. This problem is addressed primarily through cleanroom assembly during sensitive steps and rigorous chemical processing to prevent and remove such defects. Human workers are often the largest source of contamination, even with proper gowning and practices. The semiconductor industry has long integrated robots in cleanroom operation, but this has not occurred for SRF cavity production; SRF cavities, unlike wafers, are complex shapes, require more hands-on mechanical assembly, and are low-volume production items. At Jefferson Laboratory, a co-operative robot (cobot) has been setup to overcome these problems. Cobots are safe for use alongside human workers and can integrate new tools such as a 3D camera part detection and gripper for item manipulation. Therefore, cobots represent a promising avenue for reducing particulate generated during a variety of assembly tasks. A mockup of a cavity pair and coupler was setup and the cobot programmed to automatically pick up the coupler and place on the mating cavity flange. Particle counting methods were setup to measure human vs cobot assembly particulate generation inside a cavity mockup. Other potential uses will be discussed for further improving SRF cavity assembly steps, where a cobot can replace or assist a human operator, and what potential gains are expected.

Duzik, Adam [Thomas Jefferson National Accelerator↗