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At least 487 records · Page 27

Shock-induced twinning/detwinning and spall failure in Cu–Ta nanolaminates at atomic scales

Here, this study provides new insights into the role of interfaces on the deformation and failure mechanisms in shock-loaded Cu–Ta–Cu trilayer system. The thickness of the Ta layer, piston velocities, and shock pulse durations were varied to explore the impact of impedance mismatch and loading conditions on spallation behavior and twin formation. It was found that the interfaces play a crucial role in the dynamic response of these multilayered systems since secondary reflection waves generated at the interfaces significantly affected the peak stress and pressure profiles, influencing void nucleation and failure modes. In the trilayer systems, failure predominantly occurred at interfaces and within the Ta layer, with void nucleation sites and twinning behavior being markedly different compared to single-crystal Cu and Ta. Increasing the Ta layer thickness modified the wave interactions, leading to different failure locations. Higher piston velocities were associated with increased spall strength by enhancing wave interactions and void formation, particularly at the interfaces and within the Ta layer, under specific configurations. Additionally, shorter shock pulse durations facilitated earlier initiation of the release fan, reducing twin formation and altering the failure dynamics by accelerating twin annihilation and pressure release.

36 MATERIALS SCIENCE↗

Analyzing the cosmic web environment in the vicinity of grand-design and flocculent spirals with local geometric index

We explore the environment of a combined set of 367 grand-design and 619 flocculent spiral galaxies. We introduce a novel estimator called the local geometric index to quantify the morphology of the local environment of these 986 spirals. The local geometric index allows us to classify the environment of galaxies into voids, sheets, filaments, and clusters. We find that grand-designs are mostly located in dense environments like clusters and filaments (∼ 78%), whereas the fraction of the flocculents lying in sparse environments like voids and sheets is significantly higher (> 10%) than that of the grand-designs. A p-value < 10 -3 from a Kolmogorov-Smirnov test indicates that our results are statistically significant at 99.9% confidence level. Further, we note that dense environments with large tidal flows are dominated by the grand-designs. On the other hand, low-density environments such as sheets and voids favor the growth of flocculents.

79 ASTRONOMY AND ASTROPHYSICS↗

Effects of baryonic feedback on the cosmic web

Here, we study the effect of baryons on the cosmic web—halos, filaments, walls, and voids. To do so, we apply a modified version of NEXUS, a cosmic web morphological analysis algorithm, to the IllustrisTNG simulations. We find that halos lose more than 10% of their mass due to baryons, mostly to filaments and a small portion to walls and voids. However, the mass transfer does not significantly shift the boundaries of structures, leaving the volume fractions of the cosmic structures largely unaffected. We quantify the effects of baryonic feedback on the power spectrum and the probability density function of the density field for individual cosmic structures. For the power spectrum, most suppression due to feedback can be accounted for by including M ≥ 10 12 M ⊙ /h halos, without considering other cosmic structures. However, when examining the probability density function of the density field, we find nearly 100% suppression of the emptiest regions and 10%-level effects (boost or suppression) in the remaining regions of filaments, walls, and voids. Our results indicate the importance of modeling the effects of baryons in the whole cosmic web, not just halos, for cosmological analysis beyond two-point statistics or field-based inferences.

79 ASTRONOMY AND ASTROPHYSICS↗

Cyclic phase transition of substrate-modulated two-dimensional dusty plasma driven by gyroscopic forces

Langevin dynamical simulations are performed to investigate the formation of clusters and voids of a two-dimensional periodic substrate (2DPS)-modulated two-dimensional dusty plasma (2DDP) driven by a gyroscopic force. It is discovered that, as the frequency of the gyroscopic force decreases gradually, the substrate-modulated 2DDP undergoes the cyclic transition between the ordered cluster and void phases. Between the observed ordered cluster and void phases, the studied 2DDP exhibits a more uniform arrangement of particles. The discovered cyclic transition is attributed to the symmetry of the time-averaged potential landscape induced by the 2DPS in the reference frame of the moving particle, as confirmed by superimposing the particle locations on the effective potential landscape under various conditions.

36 MATERIALS SCIENCE↗

MACHINE LEARNING-ENABLED PREDICTION OF TRANSIENT INJECTION MAP IN AUTOMOTIVE INJECTORS WITH UNCERTAINTY QUANTIFICATION

Accurate prediction of injection profiles is a critical aspect of linking injector operation with engine performance and emissions. However, highly resolved injector simulations can take one to two weeks of wall-clock time, which is incompatible with engine design cycles with desired turnaround times of less than a day. Hence, it is important to reduce the time-to-solution of the internal flow simulations by several orders of magnitude to make it compatible with engine simulations. This work demonstrates a data-driven approach for tackling the computational overhead of injector simulations, whereby the transient injection profiles are emulated for a side-oriented, single-hole diesel injector using a Bayesian machine-learning framework. First, an interpretable Bayesian learning strategy was employed to understand the effect of design parameters on the total void fraction field. Then, autoencoders are utilized for efficient dimensionality reduction of the flowfields. Gaussian process models are finally used to predict the spatiotemporal void fraction field at the injector exit for unknown operating conditions. The Gaussian process models produce principled uncertainty estimates associated with the emulated flowfields, which provide the engine designer with valuable information of where the data-driven predictions can be trusted in the design space. The Bayesian flowfield predictions are compared with the corresponding predictions from a deep neural network, which has been transfer-learned from static needle simulations from a previous work by the authors. The emulation framework can predict the void fraction field at the exit of the orifice within a few seconds, thus achieving a speed-up factor of up to 38 x 10(6) over the traditional simulation-based approach of generating transient injection maps.

machine learning↗

Kinetic Monte Carlo simulations of aging in δ -Pu

We have developed a first-passage kinetic Monte Carlo approach for materials aging to investigate the sensitivity of void swelling to model parameters, including helium bubble density and size distribution. In addition to explicitly accounting for the spatial distribution of individual point defects, bubbles, and voids, our approach can simulate total doses equivalent to 100 years of natural aging on statistically representative volumes of materials. This technique enables us to study the effects on swelling and radiation damage evolution due to temperature and dose rate (as altered in artificially aged experiments), differences in effective interaction radii between vacancies and interstitials, and varying defect diffusion activation energies, while providing more detailed information than previous rate-equation based approaches. In conclusion, our results indicate that spatial effects that are not modeled in mean-field rate theories could play a significant role in void swelling initiation and growth for certain regimes of model parameters.

Actinides↗

Deformation and failure of the CrCoNi medium-entropy alloy subjected to extreme shock loading

The extraordinary work hardening ability and fracture toughness of the face-centered cubic (fcc) high-entropy alloys render them ideal candidates for many structural applications. Here, the deformation and failure mechanisms of an equiatomic CrCoNi medium-entropyalloy (MEA) were investigated by powerful laser-driven shock experiments. Multiscale characterization demonstrates that profuse planar defects including stacking faults, nanotwins, and hexagonal nanolamella were generated during shock compression, forming a three-dimensional network. During shock release, the MEA fractured by strong tensile deformation and numerous voids was observed in the vicinity of the fracture plane. High defect populations, nanorecrystallization, and amorphization were found adjacent to these areas of localized deformation. Molecular dynamics simulations corroborate the experimental results and suggest that deformation-induced defects formed before void nucleation govern the geometry of void growth and delay their coalescence. Our results indicate that the CrCoNi-based alloys are impact resistant, damage tolerant, and potentially suitable in applications under extreme conditions.

36 MATERIALS SCIENCE↗

Dual-Purpose Canister Filling Demonstration Project Progress Report

This report discusses the progress made at the Oak Ridge National Laboratory to support direct disposal of dual-purpose canisters (DPCs). Acceptable filler materials should demonstrate that the probability of criticality in DPCs during the disposal timeframe is below the probability threshold for inclusion in a repository performance assessment. This effort, which will ultimately result in a full-scale demonstration, includes computational fluid dynamics (CFD) modelling developed to gauge the filling process and to uncover any unforeseen issues. Filling simulations of the lower region (mouse holes) of a prototypic DPC show successfully simulate filling of the void space inside the canister and a smooth, even progression of the liquid level. Flow through a pipe that is similar to the drainpipe in a DPC is being investigated separately to gain valuable insight of the flow regime inside a pipe. Three physical experiments validating the computational filling model have been completed using surrogate liquids. One experiment using molten metal has been completed and the results demonstrate adequate filling of the canister void spaces. Although the scale experiment observed some void spaces related to shrinkage of the metal during cooling, the volume filled is expected to be sufficient to meet the purpose of moderator exclusion. Further experiments will scale up the geometry, moving towards a full-sized DPC demonstration, and provide a more rigorous investigation of candidate filler materials.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Capsule defects measurement [Slides]

Recent high yield shots a NIF showed that capsule defects are limiting shot performance. Voids in the capsule are not well understood in how they degrade yield performance. Recent simulations show that voids can reduce compressibility without any diagnostic signatures but reduced yield. In extreme cases loss of compression is expected. Up to 10,000 voids might be necessary to measure the different effects. Experiments using capsules with engineered defects can help guide simulations and improve our understanding of the physics involved. The knowledge gained can be applied to other problems.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Zeus: Fast-Spectrum Critical Assemblies with a Pb-HEU Core Surrounded by a Copper Reflector

The Zeus experiments with lead (Pb) were a series of measurements performed at the National Criticality Experiments Research Center (NCERC) in collaboration with the Japan Atomic Energy Agency (JAEA). Personnel from the JAEA who assisted with the experiment were Masahiro Fukushima and Akito Oizumi. The measurements were performed by Joetta Goda, Geordie McKenzie, John Bounds, Jessie Walker, Travis Grove, Theresa Cutler, Rene Sanchez, and Jesson Hutchinson from Los Alamos National Laboratory (LANL). The purpose of these experiments was to validate Pb nuclear cross sections and Pb void reactivity worth using the Comet critical assembly machine. Plates of highly enriched uranium (HEU) and Pb were arranged in a cylindrical configuration with full copper (Cu) reflection. To study the Pb void reactivity worth, a varying number of cylindrical aluminum (Al) spacers with voids replaced Pb plates in different configurations. Four configurations, which used zero to eight Al spacers, were evaluated as benchmarks.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Effect of Hydrogen and Helium on Irradiation Damage Accumulation in Nickel

We report our results on the study of the effects of hydrogen and helium on irradiation damage accumulation in nickel, aiming to understand the TEM observations made by Edwards et al. regarding the Ni-coatings protecting the getter tube in a TPBAR. We hypothesized that differences in the fluxes of 3 H and/or He between the coatings might explain these microstructural variations. However, our simulation results show that during the initial stages of irradiation, the presence of H or He enhances void nucleation by stabilizing small vacancy clusters against thermal dissociation and does not enhance void growth. Nevertheless, we think that helium’s higher diffusivity, stronger binding with vacancy clusters, and ability to displace a nearby lattice atom—either to create a new vacancy or to enlarge an existing vacancy cluster—could result in a larger average vacancy cluster size. Therefore, it is likely that void growth will occur post-nucleation phase as more He accumulates at higher doses than those simulated in this study.

36 MATERIALS SCIENCE↗

Irradiated Microstructure of Zorita Materials

Reactor baffle plate materials were harvested from the decommissioned Zorita nuclear power reactor after 38 years of service and were characterized with transmission electron microscope. The samples were Type 304 stainless steels and had been irradiated to 0.05, 16.9, ad 48.6 dpa. Faulted dislocation loops, voids, and irradiation-induced precipitates were observed in this material. While dislocation loops were the dominant irradiation defects for all samples, small voids and precipitates were also observed at 16.9 and 48.6 dpa, but not at 0.05 dpa. The size of dislocation loops increased with irradiation dose and saturated below 16.9 dpa. The loop density continued to increase between 16.9 and 48.6 dpa. For voids, both the density and mean size were small, and the volume swelling was negligibly small even at 48.6 dpa. In addition, carbides or G-phase precipitates were detected at 16.9 and 48.6 dpa, and a complex dose dependence was observed. A range of irradiation hardening was estimated at each dose, and the resulting yield strengths were consistent with the previous tensile results measured from the Halden and BOR-60 specimens.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Micturition patterns of an unrestrained chimpanzee under entrained and free running conditions.

A young male chimpanzee was subjected to 30 days of isolation. Urine volumes and voiding times were recorded every hour beginning 14 days prior to isolation, ending 6 days after isolation, and approximately 2 months later for 10 days as a control. Observed during most periods of the experiment were (1) clear circadian micturition rhythms with the voiding peak occurring immediately after the subject awoke and (2) urine flow rhythms with the maximum volume voided in the morning hours. A 24-hour rhythm was seen when the subject was entrained to 12L:12D treatments and 24.8-hour rhythm when he was exposed to continuous light. A possible underlying 24-hour micturition rhythm was also seen during the continuous light period. Distorted rhythm curves indicating possible stress were obtained for the pre-isolation adaptation period and the initial period of isolation. As time passed, the curves were more like the controls, perhaps indicating a decrease in stress.

Hoshizaki, T.↗

Thermal properties of granulated materials.

Review of the thermophysical properties of granular materials or silicates believed to simulate the lunar surface layer. Emphasis is placed on thermal conductivity data and the effects of material and environmental variables on the thermal conductivity. There are three basic mechanisms of heat transfer in particulate materials: conduction by the gas contained in the void spaces between the particles; conduction within the solid particles and across the interparticle contacts; and thermal radiation within the particles, across the void spaces between particle surfaces, and between void spaces themselves. Gas and solid conduction, thermal radiation, and the interaction between conduction and radiation are considered.

Wechsler, A. E.↗

Diffusional creep and creep degradation in the dispersion-strengthened alloy TD-NiCr

Dispersoid-free regions were observed in TD-NiCr (Ni-20Cr-2ThO2) after slow strain rate testing in air from 1145 to 1590 K. Formation of the dispersoid-free regions appears to be the result of diffusional creep. The net effect of this creep is the degradation of TD-NiCr to a duplex microstructure. Degradation is further enhanced by the formation of voids and integranular oxidation in the thoria-free regions. These regions apparently provided sites for void formation and oxide growth since the strength and oxidation resistance of Ni-20Cr is much less than Ni-20Cr-2ThO2. This localized oxidation does not appear to reduce the static load bearing capacity of TD-NiCr since long stress rupture lives were observed even with heavily oxidized microstructures. But this oxidation does significantly reduce the ductility and impact resistance of the material. Dispersoid-free bands and voids were also observed for two other dispersion strengthened alloys, TD-NiCrAl and IN-853. Thus, it appears that diffusional creep is charactertistic of dispersion-strengthened alloys and can play a major role in the creep degradation of these materials.

Whittenberger, J. D.↗

Investigation of the plastic fracture of high strength steels

This investigation deals in detail with the three recognized stages of plastic fracture in high strength steels, namely, void initiation, void growth, and void coalescence. The particular steels under investigation include plates from both commercial purity and high purity heats of AISI 4340 and 18 Ni, 200 grade maraging steels. A scanning electron microscope equipped with an X-ray energy dispersive analyzer, together with observations made using light microscopy, revealed methods of improving the resistance of high strength steels to plastic fracture.

Cox, T. B.↗

Diffusional creep and creep-degradation in dispersion-strengthened Ni-Cr base alloys.

Dispersoid-free regions were observed in the dispersion-strengthened alloy TD-NiCr (Ni-20 Cr-2 ThO2) after slow strain rate testing (stress rupture, creep, and fatigue) in air from 1145 to 1590 K. Formation of the dispersoid-free regions appears to be the result of diffusional creep. The net effect of creep in TD-NiCr is the degradation of the alloy to a duplex microstructure. Creep degradation of TD-NiCr is further enhanced by the formation of voids and intergranular oxidation in the dispersoid-free bands. Void formation was observed after as little as 0.13% creep deformation at 1255 K. The dispersoid-free regions apparently provide sites for void formation and oxide growth since the strength and oxidation resistance of Ni-20 Cr-2 ThO2.

Whittenberger, J. D.↗

An investigation of the plastic fracture of high strength steels

Three generally recognized stages of plastic fracture in high strength steels are considered in detail. These stages consist of void initiation, void growth, and void coalescence. A brief review of the existing literature on plastic fracture is included along with an outline of the experimental approach used in the investigation.

Cox, T. B.↗