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At least 487 records · Page 27

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NASA NTRS2001

Microwave Remote Sensing and the Cold Land Processes Field Experiment

The Cold Land Processes Field Experiment (CLPX) has been designed to advance our understanding of the terrestrial cryosphere. Developing a more complete understanding of fluxes, storage, and transformations of water and energy in cold land areas is a critical focus of the NASA Earth Science Enterprise Research Strategy, the NASA Global Water and Energy Cycle (GWEC) Initiative, the Global Energy and Water Cycle Experiment (GEWEX), and the GEWEX Americas Prediction Project (GAPP). The movement of water and energy through cold regions in turn plays a large role in ecological activity and biogeochemical cycles. Quantitative understanding of cold land processes over large areas will require synergistic advancements in 1) understanding how cold land processes, most comprehensively understood at local or hillslope scales, extend to larger scales, 2) improved representation of cold land processes in coupled and uncoupled land-surface models, and 3) a breakthrough in large-scale observation of hydrologic properties, including snow characteristics, soil moisture, the extent of frozen soils, and the transition between frozen and thawed soil conditions. The CLPX Plan has been developed through the efforts of over 60 interested scientists that have participated in the NASA Cold Land Processes Working Group (CLPWG). This group is charged with the task of assessing, planning and implementing the required background science, technology, and application infrastructure to support successful land surface hydrology remote sensing space missions. A major product of the experiment will be a comprehensive, legacy data set that will energize many aspects of cold land processes research. The CLPX will focus on developing the quantitative understanding, models, and measurements necessary to extend our local-scale understanding of water fluxes, storage, and transformations to regional and global scales. The experiment will particularly emphasize developing a strong synergism between process-oriented understanding, land surface models and microwave remote sensing. The experimental design is a multi-sensor, multi-scale (1-ha to 160,000 km ^ {2}) approach to providing the comprehensive data set necessary to address several experiment objectives. A description focusing on the microwave remote sensing components (ground, airborne, and spaceborne) of the experiment will be presented.

Kim, Edward J.↗

DOE OSTI2020

Subcloud and Cloud-Base Latent Heat Fluxes during Shallow Cumulus Convection

Doppler and Raman lidar observations of vertical velocity and water vapor mixing ratio are used to probe the physics and statistics of subcloud and cloud-base latent heat fluxes during cumulus convection at the ARM Southern Great Plains (SGP) site in Oklahoma, United States. The statistical results show that latent heat fluxes increase with height from the surface up to ~0.8 Z i (where Z i is the convective boundary layer depth) and then decrease to ~0 at Z i . Peak fluxes aloft exceeding 500 W m −2 are associated with periods of increased cumulus cloud cover and stronger jumps in the mean humidity profile. These entrainment fluxes are much larger than the surface fluxes, indicating substantial drying over the 0–0.8 Z i layer accompanied by moistening aloft as the CBL deepens over the diurnal cycle. We also show that the boundary layer humidity budget is approximately closed by computing the flux divergence across the 0–0.8 Z i layer. Composite subcloud velocity and water vapor anomalies show that clouds are linked to coherent updraft and moisture plumes. The moisture anomaly is Gaussian, most pronounced above 0.8 Z i and systematically wider than the velocity anomaly, which has a narrow central updraft flanked by downdrafts. This size and shape disparity results in downdrafts characterized by a high water vapor mixing ratio and thus a broad joint probability density function (JPDF) of velocity and mixing ratio in the upper CBL. We also show that cloud-base latent heat fluxes can be both positive and negative and that the instantaneous positive fluxes can be very large (~10 000 W m −2 ). However, since cloud fraction tends to be small, the net impact of these fluxes remains modest.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS1993

Simulated retrieval of land surface parameters using multichannel satellite microwave radiometry

The current global change research emphasis on understanding water and energy fluxes at the land-atmosphere interface provided renewed interest in using passive microwave satellite data for land studies. Radiative transfer models of microwave emission and scattering in the soil-vegetation-atmosphere column, though still in the process of development, can be used to estimate the accuracies with which land surface parameters can be derived from satellite data. These parameters include surface soil moisture, surface temperature, vegetation water content, and atmospheric water content. A microwave radiative transfer model is used to develop linear and nonlinear versions of a multichannel retrieval algorithm to simulate retrievals of the surface and atmospheric parameters. These simulations include the effect of additive noise, and examine the effects of nonlinearities in the radiative transfer models. However, effects of spatial heterogeneity are not considered. Satellite data to which the retrieval algorithms may be applied include the SSMR and SSM/I, and in future will include the Multifrequency Imaging Microwave Radiometer (MIMR) to be launched as part of the Earth Observing System (EOS). The Scanning Multichannel Microwave Radiometer (SMMR) on the Nimbus-7 satellite provided data from 1978 to 1987 at five microwave frequencies between 6.6 and 37 GHz. The series of Special Sensor Microwave/Imager (SSM/I) instruments launched on the DMSP satellites provide data from 1987 to the present at four frequencies between 19.35 and 8.5 GHz. Spatial resolutions of the data range from approximately 12 to 120 km depending on the frequency. Examples using data from these sensors are shown to indicate the results of applying retrieval algorithms based on model simulations to real data.

Njoku, Eni G.↗

NASA NTRS1999

Impact of Assimilating GOES-Derived Land Surface Variables into the PSU/NCAR MM5

Land surface processes are known to have a profound impact on the overlying atmosphere over a wide range of spatial and temporal scales. Many atmospheric numerical models include special parameterizations to improve the specification and partitioning of surface fluxes which are critical to the accurate prediction of warm season boundary layer behavior, organized mesoscale circulations, and convective precipitation. However, the added degrees of freedom resulting from the inclusion of vegetation and soil schemes require the specification of additional surface parameters such as vegetative resistances, green vegetation fraction, leaf area index, soil physical and hydraulic characteristics, and the vertical distribution of soil moisture. As satellite data have become more readily available in recent years, many investigations have attempted to use these new measurements to infer missing components of the surface energy budget. Sensitivity studies have shown land-skin temperature (LST) tendencies during the mid-morning hours are strongly sensitive to the surface moisture availability (a function of soil wetness and vegetation) and less sensitive to other parameters such as surface roughness. Based upon results from these and other studies, developed a simple technique that dynamically assimilates Geostationary Operational Environmental Satellite (GOES) derived land-surface products into the surface energy budget of a mesoscale model. The purpose of this paper is to demonstrate that assimilating the GOES satellite data has the potential to improve the representation of land surface characteristics within the model without prior knowledge of the land surface characteristics. The assimilation technique is presented in Section 2 and the numerical experiments are detailed in Section 3. Preliminary results and conclusions are presented in Sections 4 and 5, respectively.

Lapenta, William M.↗

NASA NTRS2014

Sensitivity of CO2 Simulation in a GCM to the Convective Transport Algorithms

Convection plays an important role in the transport of heat, moisture and trace gases. In this study, we simulated CO2 concentrations with an atmospheric general circulation model (GCM). Three different convective transport algorithms were used. One is a modified Arakawa-Shubert scheme that was native to the GCM; two others used in two off-line chemical transport models (CTMs) were added to the GCM here for comparison purposes. Advanced CO2 surfaced fluxes were used for the simulations. The results were compared to a large quantity of CO2 observation data. We find that the simulation results are sensitive to the convective transport algorithms. Overall, the three simulations are quite realistic and similar to each other in the remote marine regions, but are significantly different in some land regions with strong fluxes such as Amazon and Siberia during the convection seasons. Large biases against CO2 measurements are found in these regions in the control run, which uses the original GCM. The simulation with the simple diffusive algorithm is better. The difference of the two simulations is related to the very different convective transport speed.

Convection↗

NASA NTRS2012

Projections of Declining Surface-Water Availability for the Southwestern United States

Global warming driven by rising greenhouse-gas concentrations is expected to cause wet regions of the tropics and mid to high latitudes to get wetter and subtropical dry regions to get drier and expand polewards. Over southwest North America, models project a steady drop in precipitation minus evapotranspiration, P -- E, the net flux of water at the land surface, leading to, for example, a decline in Colorado River flow. This would cause widespread and important social and ecological consequences. Here, using new simulations from the Coupled Model Intercomparison Project Five, to be assessed in Intergovernmental Panel on Climate Change Assessment Report Five, we extend previous work by examining changes in P, E, runoff and soil moisture by season and for three different water resource regions. Focusing on the near future, 2021-2040, the new simulations project declines in surface-water availability across the southwest that translate into reduced soil moisture and runoff in California and Nevada, the Colorado River headwaters and Texas.

Seager, Richard↗

NASA NTRS2019

NCA-LDAS: Overview and Analysis of Hydrologic Trends for the National Climate Assessment

Terrestrial hydrologic trends over the conterminous United States are estimated for 1980–2015 using the National Climate Assessment Land Data Assimilation System (NCA-LDAS) reanalysis. NCA-LDAS employs the uncoupled Noah version 3.3 land surface model at 0.125° 3 0.125° forced with NLDAS-2 meteorology, rescaled Climate Prediction Center precipitation, and assimilated satellite-based soil moisture, snow depth, and irrigation products. Mean annual trends are reported using the nonparametric Mann–Kendall test at p < 0.1 significance. Results illustrate the interrelationship between regional gradients in forcing trends and trends in other land energy and water stores and fluxes. Mean precipitation trends range from +3 to +9 mm/yr in the upper Great Plains and Northeast to -1 to -9 mm/yr in the West and South, net radiation flux trends range from +0.05 to +0.20 W/sq. m yr in the East to -0.05 to -0.20 W/sq. m yr in the West, and U.S.-wide temperature trends average about +0.03K/yr. Trends in soil moisture, snow cover, latent and sensible heat fluxes, and runoff are consistent with forcings, contributing to increasing evaporative fraction trends from west to east. Evaluation of NCA-LDAS trends compared to independent data indicates mixed results. The RMSE of U.S.-wide trends in number of snow cover days improved from 3.13 to 2.89 days/yr while trend detection increased 11%. Trends in latent heat flux were hardly affected, with RMSE decreasing only from 0.17 to 0.16 W/sq. m yr, while trend detection increased 2%. NCA-LDAS runoff trends degraded significantly from 2.6 to 16.1 mm/yr while trend detection was unaffected. Analysis also indicated that NCA-LDAS exhibits relatively more skill in low precipitation station density areas, suggesting there are limits to the effectiveness of satellite data assimilation in densely gauged regions. Overall, NCA-LDAS demonstrates capability for quantifying physically consistent, U.S. hydrologic climate trends over the satellite era.

Michael F. Jasinski↗

DOE OSTI2025

Experimental Soil Warming Impacts Soil Moisture and Plant Water Stress and Thereby Ecosystem Carbon Dynamics

Experimental soil heating experiments have found a consistent increase in soil-surface CO 2 emissions ( F s ), but inconsistent soil organic carbon (SOC) responses. Interpretation of heating effects is complicated by spatial heterogeneity and soil moisture, nitrogen availability, and microbial and plant responses. Here we applied a mechanistic ecosystem model to interpret heating impacts on a California forest subjected to 1 m deep, 4°C heating. The model accurately simulated control-plot CO 2 fluxes, SOC stocks, fine root biomass, soil moisture, and soil temperature, and the observed increases in F s and decreases in fine root biomass. We show that a complex suite of interactions can lead to a consistent increase in F s (~17%) over the 5-year study period, with very small changes in SOC stocks (<1%). Modeled increases in leaf water stress from soil drying reduced GPP and NPP. The resulting reduction in leaf and fine root allocation increased fine root litter inputs to the soil and reduced root exudation. Soil heating led to about a 50% larger increase in root autotrophic respiration than in heterotrophic respiration, with the heating effect on both these fluxes decreasing over the simulation period. Increased heterotrophic respiration led to increased soil N availability and plant N uptake. These heating responses are mechanistically linked, of magnitudes that can affect ecosystem dynamics, and long-term observations of them are rarely made. Therefore, we conclude that a coupled observational and mechanistic modeling framework is needed to interpret manipulation experiments, and to improve projections of climate change impacts on terrestrial ecosystem carbon dynamics.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS2019

NCA-LDAS: Overview and Analysis of Hydrologic Trends for the National Climate Assessment

Terrestrial hydrologic trends over the conterminous United States are estimated for 1980-47 2015 using the National Climate Assessment-Land Data Assimilation System (NCA-LDAS) reanalysis. NCA-LDAS employs the uncoupled Noah Version 3.3 land surface model at 0.125 degreesx0.125 degrees forced with NLDAS-2 meteorology, rescaled Climate Prediction Center precipitation, and assimilated satellite-based soil moisture, snow depth and irrigation products. Mean annual trends are reported using the nonparametric Mann-Kendall test at p<0.1 significance. Results illustrate the interrelationship between regional gradients in forcing trends, and trends in other land energy and water stores and fluxes. Mean precipitation trends range from +3 to +9 mm/yr in the Upper Great Plains and Northeast to -1 to -9 in the West and South; net radiation flux trends range from +0.05 to +0.20 W/m(exp2)/yr in the East to -0.05 to -0.20 in the West; U.S.-wide temperature trends average about +0.03K/yr. Trends in soil moisture, snow cover, latent and sensible heat fluxes and runoff are consistent with forcings, contributing to increasing evaporative fraction trends from West to East. Evaluation of NCA-LDAS trends compared to independent data indicates mixed results. The RMSE of U.S.-wide trends in number of snow cover days improved from 3.13 to 2.89 days/yr while trend detection increased 11%; Trends in latent heat flux were hardly affected, RMSE decreasing only 0.17 to 0.16 W/m(exp 2)/yr, while trend detection increased 2%; NCA-LDAS runoff trends degraded significantly from 2.6 to 16.1 mm/yr while trend detection was unaffected. Analysis also indicated that NCA-LDAS exhibits relatively more skill in low precipitation station density areas, suggesting there are limits to the effectiveness of satellite data assimilation in densely gaged regions. Overall, NCA-LDAS demonstrates capability for quantifying physically consistent, U.S. hydrologic climate trends over the satellite era.

Snow depth↗

DOE OSTI2023

Hydrobiogeochemical Controls on the Delivery of Dissolved Organic Matter to Boreal Headwater Streams

Understanding controls on the delivery of dissolved organic matter (DOM) from terrestrial to aquatic systems is key for constraining carbon balances and fluxes in boreal headwater catchments. The largest export of DOM generally occurs during intense periods of water delivery to the landscape (e.g., rain events); however, the timing and magnitude of DOM is complicated by geomorphological, hydrometeorological, and biogeochemical variability. To better assess mechanisms controlling the delivery of DOM to boreal streams, DOM was investigated in two morphologically distinct catchments of an experimental forest watershed in western Newfoundland, one dominated by low relief wetlands and the other by steep hillslopes. The DOM was compared during two fall storms of similar magnitude but contrasting moisture conditions during the autumn transition. Variable concentrations and optical character highlighted antecedent conditions are important for the delivery of DOM to boreal streams. Concentration-discharge relationships with stream hydrograph separation analysis suggest preferential flowpaths through shallow mineral horizons as a key pathway for delivery of DOM in the hillslope dominated catchment compared to rapid input from near-stream wetlands in the low relief catchment. Loss of DOM via preferential pathways suggests an additional mechanism for surface soil carbon loss not directly informed by lateral flow and soil hydrology, which has important implications for our conceptualization and modeling of carbon fluxes in boreal systems. These results suggest watershed scale responses of DOM in boreal headwater catchments are complex, and better linkages between catchment scale hydrology and landscape hydrobiogeochemistry are required to constrain terrestrial to aquatic carbon fluxes in boreal landscapes.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2023

Thermodynamic and kinematic drivers of atmospheric boundary layer stability in the central Arctic during the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC)

Observations collected during the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) provide a detailed description of the impact of thermodynamic and kinematic forcings on atmospheric boundary layer (ABL) stability in the central Arctic. This study reveals that the Arctic ABL is stable and near-neutral with similar frequencies, and strong stability is the most persistent of all stability regimes. MOSAiC radiosonde observations, in conjunction with observations from additional measurement platforms, including a 10 m meteorological tower, ceilometer, microwave radiometer, and radiation station, provide insight into the relationships between atmospheric stability and various atmospheric thermodynamic and kinematic forcings of ABL turbulence and how these relationships differ by season. We found that stronger stability largely occurs in low-wind (i.e., wind speeds are slow), low-radiation (i.e., surface radiative fluxes are minimal) environments; a very shallow mixed ABL forms in low-wind, high-radiation environments; weak stability occurs in high-wind, moderate-radiation environments; and a near-neutral ABL forms in high-wind, high-radiation environments. Surface pressure (a proxy for synoptic staging) partially explains the observed wind speeds for different stability regimes. Cloud frequency and atmospheric moisture contribute to the observed surface radiation budget. Unique to summer, stronger stability may also form when moist air is advected from over the warmer open ocean to over the colder sea ice surface, which decouples the colder near-surface atmosphere from the advected layer, and is identifiable through observations of fog and atmospheric moisture.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2021

Seismic Ambient Noise Analyses Reveal Changing Temperature and Water Signals to 10s of Meters Depth in the Critical Zone

The critical zone sustains terrestrial life, but we have few tools to explore it efficiently beyond the first few meters of the subsurface. Using analyses of high-frequency ambient seismic noise from densely spaced seismometers deployed in the forested Shale Hills subcatchment of the Susquehanna Shale Hills Critical Zone Observatory (SSHCZO), we show that temporal changes in seismic velocities at depths from ~1 m to tens of m can be detected. Furthermore, these changes are driven by variations at the land surface. The Moving-Window Cross-Spectral (MWCS) method was employed to measure seismic-velocity changes in coda waves at hourly resolution in 10 different frequency bands. We observed a diurnal signal, a seasonal signal, and a meteorological-event-based signal. These signals were compared to time-series measurements of precipitation, well water levels, soil moisture, soil temperature, air temperature, latent heat flux, and air pressure in the heavily instrumented catchment. Most of the velocity changes can be explained by variations in temperature that result in thermoelastic strains that propagate to depth. But some double minima in seismic velocity time-series observed after large rain events were attributed in part to the effects of water infiltration. These results show that high-frequency ambient noise data may in some locations be used to detect changes in the critical zone from ~1 to ~100 m or greater depth with hourly resolution. But interpretation of such data requires multiple environmental data sets to deconvolve the complex interrelationships among thermoelastic and hydrological effects in the subsurface critical zone.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS1991

A two-dimensional numerical investigation of the interaction between sea breezes and deep convection over the Florida peninsula

The Colorado State University Regional Atmospheric Modeling System is used to investigate the interaction between sea breezes and deep convection over the Florida peninsula, and it is shown that this model can simulate the broad features of the three characteristic types of convection systems classified by Blanchard and Lopez (1985). In sensitivity tests performed for a variety of wind and thermodynamic profiles and for different soil-moisture contents, it was found that increases in the low-level temperature and in moisture content speeded up the development of convection. It was found that the dry-soil simulation produced rapidly developing sea breezes that moved inland quickly, while the moist soil case produced a much more slowly developing sea breeze. The total rainfall over the peninsula for the dry-soil case was greater than for the moist soil; it is suggested that the enhanced surface heat fluxes for the dry soil case create stronger low-level convergence over the peninsula (than in the moist-soil case) to force the convection.

Nicholls, Melville E.↗

NASA NTRS2020

El Niño Related Tropical Land Surface Water and Energy Response in MERRA-2

Though El Niño events each have distinct evolutionary character they typically provide systematic large scale forcing for warming and increased drought frequency across the tropical continents. We assess this response in the MERRA-2 reanalysis and in a ten-member model AMIP ensemble. The lagged response (3-4 months) of mean tropical land temperature to El Niño warming in the Pacific Ocean is well represented. MERRA-2 reproduces the patterns of precipitation in the tropical regions, while the AMIP ensemble reproduces some regional responses better than others. Model skill is dependent on event forcing strength and temporal proximity to the peak of the sea surface warming. A composite approach centered on maximum Niño3.4 SSTs and lag relationships to energy fluxes and transports is used to identify mechanisms supporting tropical land warming. The composite necessarily moderates weather scale variability of the individual events, while retaining the systematic features across all events. We find that that reduced continental upward motions lead to reduced cloudiness and more shortwave radiation at the surface, as well as reduced precipitation. The increased shortwave heating at the land surface, along with reduced soil moisture leads to warmer surface temperature, more sensible heating and warming of the lower troposphere. While the composite provides a broad picture of the mechanisms governing the hydrologic response to El Niño forcing, the regional and temporal response in any given event can be quite variable. The 2015-16 El Niño, one of the strongest events, demonstrates some of the forced response noted in the composite, but with shifts in the evolution that depart from the composite, demonstrating the limitations of the composite and individuality of El Niño.

Michael G Bosilovich↗

NASA NTRS1982

Delineation of cold-prone areas using nighttime SMS/GOES thermal data Effects of soils and water

Infrared digital data from geostationary satellites were used to demonstrate the usefulness of remotely sensed surface temperature data to delineate microscale and mesoscale climates. Nocturnal winter data (December-February) from 1976-77 to 1978-79 over Florida revealed noticeable contrasts in surface temperature patterns. Colder areas were associated with low soil moisture content in the upper layers of excessively drained and well drained sandy soils, whereas warmer areas were associated with bodies of water, wetlands, or poorly drained soils. An unexpected surface temperature pattern for one night where the north-central Florida climatic zone was colder than the north Florida climatic zone was found to be caused by differences in antecedent frontal rainfall. Differences in surface radiant energy fluxes over these two areas at 0200 EST 20 December 1977, based on average satellite-sensed surface temperatures, were compared with differences in soil heat fluxes that were computed from 1.5 m climatological temperatures and soil thermal properties by use of a simplified surface energy balance equation.

Chen, E.↗

NASA NTRS1991

The impact of greenhouse climate change on the energetics and hydrologic processes of mid-latitude transient eddies

Atmospheric transient eddies contribute significantly to mid-latitude energy and water vapor transports. Changes in the global climate, as induced by greenhouse enhancement, will likely alter transient eddy behavior. Unraveling all the feedbacks that occur in general circulation models (GCMs) can be difficult. The transient eddies are isolated from the feedbacks and are focused on the response of the eddies to zonal-mean climate changes that result from CO2-doubling. Using a primitive-equation spectral model, the impact of climate change on the life cycles of transient eddies is examined. Transient eddy behavior in experiments is compared with initial conditions that are given by the zonal-mean climates of the GCMs with current and doubled amounts of CO2. The smaller meridional temperature gradient in a doubled CO2 climate leads to a reduction in eddy kinetic energy, especially in the subtropics. The decrease in subtropical eddy energy is related to a substantial reduction in equatorward flux of eddy activity during the latter part of the life cycle. The reduction in equatorward energy flux alters the moisture cycle. Eddy meridional transport of water vapor is shifted slightly poleward and subtropical precipitation is reduced. The water vapor transport exhibits a relatively small change in magnitude, compared to changes in eddy energy, due to the compensating effect of higher specific humidity in the doubled-CO2 climate. An increase in high-latitude precipitation is related to the poleward shift in eddy water vapor flux. Surface evaporation amplifies climatic changes in water vapor transport and precipitation in the experiments.

Branscome, Lee E.↗

NASA NTRS1992

Relations between surface conductance and spectral vegetation indices at intermediate (100 m sq to 15 km sq) length scales

The relationship between surface conductance and spectral vegetation indices is investigated utilizing the FIFE data set, principally the surface flux station data and images from the TM instrument. It is found that the unstressed canopy conductance for a given site for a given day is near-linearly related to the incident PAR flux. Estimates of unstressed canopy conductance were acquired via a model inversion that separated the soil and vegetation contributions to evapotranspiration and made adjustments for the effects of vapor pressure deficit and soil moisture stress.

Sellers, Piers J.↗

DOE OSTI2026

Deep Convection‐Driven Downward Transport of Trace Gases and Aerosols From the Free Troposphere to the Boundary Layer

Deep convective clouds regulate Earth's energy and moisture budgets, yet their impact on the atmospheric boundary layer (BL) composition remains underexplored. Using long-term observations from three mid-latitude sites, we show that deep convection (DC) consistently enhances nighttime surface ozone and is often accompanied by modest increases in ultrafine particle concentrations. Within the BL, the condensational growth of these transported ultrafine particles may contribute up to 60% of total cloud condensation nuclei (CCN). Mass flux calculations suggest that short-lived convective cores (∼30 min) account for ∼2% of total vertical air mass transport relative to steady entrainment, increasing to ∼13% when the trailing stratiform regions are included. These results show that DC provides an episodic but efficient pathway linking the free troposphere and BL, influencing oxidant budgets, CCN variability, and climate forcing. Accurately representing this process in climate models may help reduce uncertainties in climate projections, under both preindustrial and present-day conditions.

54 ENVIRONMENTAL SCIENCES↗