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At least 487 records · Page 27

4D Imaging of ZnO-Coated Nanoporous Al 2 O 3 Aerogels by Chemically Sensitive Ptychographic Tomography: Implications for Designer Catalysts

The 3D chemical structure (4D spectromicroscopy) of nanoporous Al 2 O 3 aerogels coated with ZnO by atomic layer deposition (ALD) was studied by multienergy scanning transmission X-ray microscopy. These materials are representative of a class of designer catalysts in which the nanoporous support is prepared separately from the active catalyst material, which is subsequently introduced by ALD, thereby allowing independent optimization of the morphology, chemistry, and spatial distribution of the support and catalyst. The samples studied were prepared by Ga ion and Xe plasma focused ion beam (FIB) milling as well as drop casting from water suspension. Zn L and Al K edge spectra of six samples with three different ZnO loadings were measured to investigate how loading and different sample preparation methods affect the 3D distribution of the ZnO and Al 2 O 3 . Scanning transmission X-ray microscopy (STXM) and ptychographic imaging at two energies each at the Zn L 3 and Al K edge were measured. The ptychography data were analyzed by using the SHARP reconstruction code to generate quantitative 2D chemical maps of the Al 2 O 3 and the ZnO. The STXM and ptychography maps were then measured at a sequence of tilt angles, covering up to 160° of rotation. The 3D structure of the ZnO and Al 2 O 3 was derived from the tilt series data by tomographic reconstruction using a compressed sensing algorithm. A twodimensional spatial resolution (half-period) of 6 nm, measured by Fourier ring correlation, and a 3D spatial resolution (half-period) of 9 nm, measured by Fourier shell correlation, were achieved when using the COSMIC beamline at the Advanced Light Source (ALS). The results show that for all of the ZnO loadings studied there is nonuniform coverage of the ZnO on the Al 2 O 3 aerogel framework. In addition, we found that both FIB methods create sample artifacts, although the distortion was less with Xe plasma than Ga ion FIB.

36 MATERIALS SCIENCE↗

Diffraction data from aerosolized Coliphage PR772 virus particles imaged with the Linac Coherent Light Source

Single Particle Imaging (SPI) with intense coherent X-ray pulses from X-ray free-electron lasers (XFELs) has the potential to produce molecular structures without the need for crystallization or freezing. Here we present a dataset of 285,944 diffraction patterns from aerosolized Coliphage PR772 virus particles injected into the femtosecond X-ray pulses of the Linac Coherent Light Source (LCLS). Additional exposures with background information are also deposited. The diffraction data were collected at the Atomic, Molecular and Optical Science Instrument (AMO) of the LCLS in 4 experimental beam times during a period of four years. The photon energy was either 1.2 or 1.7 keV and the pulse energy was between 2 and 4 mJ in a focal spot of about 1.3 μm x 1.7 μm full width at half maximum (FWHM). The X-ray laser pulses captured the particles in random orientations. The data offer insight into aerosolised virus particles in the gas phase, contain information relevant to improving experimental parameters, and provide a basis for developing algorithms for image analysis and reconstruction.

59 BASIC BIOLOGICAL SCIENCES↗

Cylinders and jets in crossflow: Wake formations as a result of varying geometric proximities

The combined flow physics of several canonical flow configurations is experimentally studied. Here, we analyze an array of jets issuing into a crossflow, then immediately navigating past an array of cylinders. This is achieved with a 2 × 3 triangular pattern of jets and symmetric cylinders at three jets to crossflow velocity ratios, enabling near-complete optical access of each jet, with velocities measured by time-resolved particle image velocimetry. Jet trajectories reveal that each configuration adheres to a power-law trend and that greater penetration is achieved by the downstream and confined jets compared to the more conventional upstream one. Recirculation regions of the upstream and downstream jets are nearly independent, with the confined jet encompassing regions of overlap with both. Turbulent statistics reveal the influence of geometric placement and velocity ratio on the time-averaged velocity, anisotropy, and Reynolds stresses incurred by each jet. Galilean decomposition utilizes a supplemental crossflow-only velocity field to delineate the influence of each jet's low- and high-pressure regions on the otherwise uniform stream. Proper orthogonal decomposition suggests that increased jet penetration decreases the number of modes required for truncation in the investigated spanwise plane. Vortex identification algorithms are applied to the reconstructed flow fields, reaffirming that with increasing velocity ratio, the jets generate vortices of their own in similar statistical formations as the cylinders. This investigation provides a foundation to aid future modeling efforts toward characterizing flow physics of importance in designing and passively controlling transverse jets with varying blockage proximities in a crossflow.

Kristo, Paul J. (ORCID:0000000225605175)↗

3D imaging of magnetic domains in Nd 2 Fe 14 B using scanning hard X-ray nanotomography

Nanoscale structural and electronic heterogeneities are prevalent in condensed matter physics. Investigating these heterogeneities in 3D has become an important task for understanding material properties. To provide a tool to unravel the connection between nanoscale heterogeneity and macroscopic emergent properties in magnetic materials, scanning transmission X-ray microscopy (STXM) is combined with X-ray magnetic circular dichroism. A vector tomography algorithm has been developed to reconstruct the full 3D magnetic vector field without any prior noise assumptions or knowledge about the sample. Two tomographic scans around the vertical axis are acquired on single-crystalline Nd 2 Fe 14 B pillars tilted at two different angles, with 2D STXM projections recorded using a focused 120 nm X-ray beam with left and right circular polarization. Image alignment and iterative registration have been implemented based on the 2D STXM projections for the two tilts. Dichroic projections obtained from difference images are used for the tomographic reconstruction to obtain the 3D magnetization distribution at the nanoscale.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Static metrology of the meter-scale deformable heliostat

This paper describes a heliostat metrology system which is developed based on deflectometry, utilizing a static perforated panel instead of conventional dynamic monitor displays to provide incident rays. The developed method is named static screen deflectometry (SSD). This robust and scalable method is especially valuable for outdoor tests of large reflectors used in concentrating solar-thermal power (CSP) systems. The developed method has been successfully demonstrated on a 2.4 𝑚 × 3.3 𝑚 float glass deformable reflector bent to focus sunlight at 113 𝑚 distance throughout a day. From images obtained from a camera at 50𝑚 distance, the reflector surface was measured to an accuracy of less than 1 𝑚𝑟𝑎𝑑 rms slope error in the full test scope.

14 SOLAR ENERGY↗

Addressing uncertainty in genome-scale metabolic model reconstruction and analysis

The reconstruction and analysis of genome-scale metabolic models constitutes a powerful systems biology approach, with applications ranging from basic understanding of genotype-phenotype mapping to solving biomedical and environmental problems. However, the biological insight obtained from these models is limited by multiple heterogeneous sources of uncertainty, which are often difficult to quantify. Here we review the major sources of uncertainty and survey existing approaches developed for representing and addressing them. A unified formal characterization of these uncertainties through probabilistic approaches and ensemble modeling will facilitate convergence towards consistent reconstruction pipelines, improved data integration algorithms, and more accurate assessment of predictive capacity.

59 BASIC BIOLOGICAL SCIENCES↗

Reconstruction and Selection of Neutrino Interactions in MicroBooNE using Deep Convolutional Neural Networks

In this document, we describe a new reconstruction workflow developed for the MicroBooNE experiment. It features the use of Deep Convolutional Neural Networks trained to recognize key structures within the data sufficient for the 3D reconstruction of neutrino interactions within the detector. As a test of the reconstruction utility, the products of the reconstruction workflow are used to select inclusive charged-current (CC) $\nu_e$ and $\nu_\mu$ interactions in both simulated and real MicroBooNE data. In simulation, our $\nu_e$ and $\nu_\mu$ selections achieve an efficiency of 57% and 68\%, respectively, with a purity of 91% and 96%, respectively. We find that these selections are competitive with the inclusive selections used for the most recent MicroBooNE LEE searches. In particular, the CC-$\nu_e$ inclusive selection efficiency improves by over 20% while also improving sample purity. As a first step in quantifying potential bias, the data and Monte Carlo expectati ons are compared for both selections using the MicroBooNE open data. Within statistical and systematic uncertainties, both the electron and muon CC-inclusive event samples agree. A comparison of the real data events chosen by our work and another reconstruction framework shows that the two analyses each identify a sizeable fraction of events the other does not. This suggests that future analyses integrating the strengths of each could lead to combined gains. This work demonstrates, for the first time on real LArTPC data, state-of-the-art neutrino interaction reconstruction centered around deep learning algorithms.

43 PARTICLE ACCELERATORS↗

Novel experimental probes of QCD in SIDIS and e + e - annihilation (Final Technical Report)

The research addressed with this award seeks to advance our understanding of the structure and dynamics underlying the properties of visible matter. In our current understanding the nucleons (protons and neutrons) are not fundamental but are comprised of quarks and gluons, which are collectively called partons. A static quark picture fails to explain the properties of the nucleons, such as their mass and intrinsic spin, which are thought to emerge dynamically from the quark-gluon interactions via the strong force. In this work, novel observables employing correlations of particles produced in the scattering of high energy electrons off protons at the CLAS12 experiment at Jefferson Lab were analyzed to probe quark-gluon interactions. The ultimate goal of this line of inquiry is to be able to describe the properties of protons and neutrons from first principles, similar to how studying the hydrogen atom has led to the formulation of the theory of Quantum Electrodynamics. Because quarks cannot be observed directly but only as part of more complex composite particles, a smaller, complimentary part of this work was the analysis of particle production in electron-positron annihilation at the Belle II experiment to understand the production of particles from initial quarks. This takes advantage of the fact that in e + e - annihilation the initial quark dynamics is known, unlike in the scattering of nucleons. Several new applications using Machine Learning algorithms for event tagging and reconstruction to support this program were developed as part of this award. In addition, we had a significant role in the development of the physics program for the future Electron-Ion Collider, which is a new collider to be build in the US within the next decade.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Molecular phylogenetic trees - On the validity of the Goodman-Moore augmentation algorithm

A response is made to the reply of Nei and Tateno (1979) to the letter of Holmquist (1978) supporting the validity of the augmentation algorithm of Moore (1977) in reconstructions of nucleotide substitutions by means of the maximum parsimony principle. It is argued that the overestimation of the augmented numbers of nucleotide substitutions (augmented distances) found by Tateno and Nei (1978) is due to an unrepresentative data sample and that it is only necessary that evolution be stochastically uniform in different regions of the phylogenetic network for the augmentation method to be useful. The importance of the average value of the true distance over all links is explained, and the relative variances of the true and augmented distances are calculated to be almost identical. The effects of topological changes in the phylogenetic tree on the augmented distance and the question of the correctness of ancestral sequences inferred by the method of parsimony are also clarified.

Holmquist, R.↗

The OMV Data Compression System Science Data Compression Workshop

The Video Compression Unit (VCU), Video Reconstruction Unit (VRU), theory and algorithms for implementation of Orbital Maneuvering Vehicle (OMV) source coding, docking mode, channel coding, error containment, and video tape preprocessed space imagery are presented in viewgraph format.

Lewis, Garton H., Jr.↗

Experimental Control of Thermocapillary Convection in a Liquid Bridge

We demonstrate the stabilization of an isolated unstable periodic orbit in a liquid bridge convection experiment. A model independent, nonlinear control algorithm uses temperature measurements near the liquid interface to compute control perturbations which are applied by a thermoelectric element. The algorithm employs a time series reconstruction of a nonlinear control surface in a high dimensional phase space to alter the system dynamics.

Petrov, Valery↗

Beta in Streamers

Streamers are often described as regions of the corona in which the density is higher than in coronal holes because the plasma is trapped by closed loops of magnetic flux. In contrast, Magnetohydrodynamics (MHD) models of the global corona show that the plasma beta identically equal to 8(pi)p/B(exp 2) > 1 in streamers above approximately 1.2Rs heliocentric height (p=pressure, B=magnetic field strength). There are three recent contributions to this topic. The first is that heating near the cusp further drives Beta up and can result in release of new slow solar wind from the top of the streamer. The second is SOHO/UVCS observations, in combination with a potential field/source surface model of the magnetic field, show beta > 1 above 1.2Rs in a streamer observed near solar sunspot minimum. The third is a magnetic field reconstruction technique (using field deforming algorithms) which was applied both to an isolated active region (AR 7999) and to the Pneuman & Kopp global MHD model. In the active region, beta becomes larger than unity at approximately 1.2Rs. In the Pneuman & Kopp model, beta = 1.0 at the base of the streamer and rises with increasing height, becoming 15-20 at 1.6Rs and 35-55 at 1.7RS. The collective implication of these three results is that beta > 1 everywhere in streamers above approximately 1.2 Rs. Global simulations go on to show that the reason streamers do not simply explode under such high beta conditions is that they are held down by pressure from the sides due to the magnetic fields (and low beta) in adjacent coronal holes. The main role of the closed magnetic loops near the cusp is to keep the streamer from continuously leaking plasma, as otherwise happens in a magnetic pinch which is similar but has no closed loops. The purpose of this note is to summarize the results implying that beta > 1 is a general property of streamers above 1.2 Rs.

Suess, Steven T.↗

High-Resolution Gamma-Ray Imaging Measurements Using Externally Segmented Germanium Detectors

Fully two-dimensional gamma-ray imaging with simultaneous high-resolution spectroscopy has been demonstrated using an externally segmented germanium sensor. The system employs a single high-purity coaxial detector with its outer electrode segmented into 5 distinct charge collection regions and a lead coded aperture with a uniformly redundant array (URA) pattern. A series of one-dimensional responses was collected around 511 keV while the system was rotated in steps through 180 degrees. A non-negative, linear least-squares algorithm was then employed to reconstruct a 2-dimensional image. Corrections for multiple scattering in the detector, and the finite distance of source and detector are made in the reconstruction process.

spectroscopy gamma ray germanium sensor nucleosynt↗

Infrared Astronomical Satellite (IRAS) image reconstruction and restoration

IRAS sky mapping data is being reconstructed as images, and an entropy-based restoration algorithm is being applied in an attempt to improve spatial resolution in extended sources. Reconstruction requires interpolation of non-uniformly sampled data. Restoration is accomplished with an iterative algorithm which begins with an inverse filter solution and iterates on it with a weighted entropy-based spectral subtraction.

Gonsalves, R. A.↗

Optimal sensor placement for reconstructing wind pressure field around buildings using compressed sensing

Deciding how to optimally deploy sensors in a large, complex, and spatially extended structure is critical to ensure that the surface pressure field is accurately captured for subsequent analysis and design. In some cases, reconstruction of missing data is required in downstream tasks such as the development of digital twins. Here, this paper presents a data-driven sparse sensor selection algorithm, aiming to provide the most information contents for reconstructing aerodynamic characteristics of wind pressures over tall building structures parsimoniously. The algorithm first fits a set of basis functions to the training data, then applies a computationally efficient QR algorithm that ranks existing pressure sensors in order of importance based on the state reconstruction to this tailored basis. The findings of this study show that the proposed algorithm successfully re- constructs the aerodynamic characteristics of tall buildings from sparse measurement locations, generating stable and optimal solutions across a range of conditions. As a result, this study serves as a promising first step toward leveraging the success of data-driven and machine learning algorithms to supplement traditional genetic algorithms currently used in wind engineering.

42 ENGINEERING↗

Ensemble‐Based, Large‐Eddy Reconstruction of Wind Turbine Inflow in a Near‐Stationary Atmospheric Boundary Layer Through Generative Artificial Intelligence

ABSTRACT To validate the second‐by‐second dynamics of turbines in field experiments, it is necessary to accurately reconstruct the winds going into the turbine. Current time‐resolved inflow reconstruction techniques estimate wind behavior in unobserved regions using relatively simple spectral‐based models of the atmosphere. Here, we develop a technique for time‐resolved inflow reconstruction that is rooted in a large‐eddy simulation model of the atmosphere. Our “large‐eddy reconstruction” technique blends observations and atmospheric model information through a diffusion model machine learning algorithm, allowing us to generate probabilistic ensembles of reconstructions for a single 10‐min observational period. Our generated inflows can be used directly by aeroelastic codes or as inflow boundary conditions in a large‐eddy simulation. We verify the second‐by‐second reconstruction capability of our technique in three synthetic field campaigns, finding positive Pearson correlation coefficient values () between ground‐truth and reconstructed streamwise velocity, as well as smaller positive correlation coefficient values for unobserved fields (spanwise velocity, vertical velocity, and temperature). We validate our technique in three real‐world case studies by driving large‐eddy simulations with reconstructed inflows and comparing to independent inflow measurements. The reconstructions are visually similar to measurements, follow desired power spectra properties, and track second‐by‐second behavior ().

17 WIND ENERGY↗

Flux Cube Reconstruction from Slitless Spectroscopy

Slitless spectroscopy enables efficient, large-area surveys without target preselection, yet it faces challenges from source blending, higher noise, and lost spatial–spectral information. We present an advanced, nonparametric, data-driven algorithm that leverages multiple dispersion angles to reconstruct three-dimensional flux distributions, providing low-resolution integral field unit capabilities from slitless data. By treating each pixel as an independent element, our method naturally handles source confusion without requiring prior assumptions regarding redshifts, templates, or model libraries. We validate the algorithm using simulated Roman Space Telescope wide-field slitless spectroscopy images that are equivalent to what is expected from the High-Latitude Time-Domain Survey. First, we demonstrate that a host-galaxy model reconstructed from multiple dispersion angles can be used to accurately subtract host light from a transient, recovering a Type Ia supernova spectrum with minimal bias. Second, we showcase a high-fidelity flux-cube reconstruction of a complex galaxy, successfully measuring the redshift and recovering continuum, emission, and absorption features. This approach highlights the potential of multi-dispersion-angle slitless data to provide spatially resolved spectral information in a nonparametric way, which is traditionally accessible only with integral field spectroscopy, opening a new window into large, unbiased, and spatially resolved studies of galaxy evolution.

Griggio, M. [Space Telescope Science Institute, Ba↗

Slicing with deep learning models at ProtoDUNE-SP

DUNE is a cutting-edge experiment aiming to study neutrinos in detail, with a special focus on the flavor oscillation mechanism. The prototype of the DUNE Far Detector Single Phase TPC (ProtoDUNE-SP) was built and operated at CERN with a full set of reconstruction tools. To implement these reconstruction tools, Pandora, a multi-algorithm framework, has been developed. A large number of these algorithms, some of them being exploiting traditional clustering, detector physics and deep learning approaches, have been applied to images to gradually build up a picture out of singular events. One of such algorithms is the Pandora slicing algorithm which aims to partition the detector hits of an event in sets called slices. Each slice represents a single interaction in the detector and should identify all the hits related to the interacting particle and its subsequent decay products. We expect the order of tens of slices per event in ProtoDUNE-SP. In this paper we present a deep learning approach to the problem, designing a model able to outperform the state-of-the-art slicing algorithm which is currently implemented within Pandora. We assess the performance of our tool in terms of efficiency and accuracy, while exploiting hardware accelerating setups. The ultimate goal is to incorporate this deep learning approach in the Pandora reconstruction tool.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗