Ultra-high Q Whispering-gallery Microactivites for Narrow-linewidth Lasers and Optoelectronic Oscillators
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Recent Progress in Laboratory Astrophysics and Astrochemistry Achieved with the COSmIC Facility
We describe the characteristics and the capabilities of the laboratory facility, COSmIC, that was developed at NASA Ames to generate, process and analyze interstellar, circumstellar and planetary analogs in the laboratory. COSmIC stands for "Cosmic Simulation Chamber" and is dedicated to the study of neutral and ionized molecules and nanoparticles under the low temperature and high vacuum conditions that are required to simulate various space environments such as diffuse interstellar clouds, circumstellar outflows and planetary atmospheres. COSmIC integrates a variety of state-of-the-art instruments that allow recreating simulated space conditions to generate, process and monitor cosmic analogs in the laboratory. The COSmIC experimental setup is composed of a Pulsed Discharge Nozzle (PDN) expansion, that generates a plasma in the stream of a free supersonic jet expansion, coupled to high-sensitivity, complementary in situ diagnostics: cavity ring down spectroscopy (CRDS) and laser induced fluorescence (LIF) systems for photonic detection, and Reflectron Time-Of-Flight Mass Spectrometer (ReTOF-MS) for mass detection. Recent results obtained using COSmIC will be highlighted. In particular, the progress that has been achieved in the domain of the diffuse interstellar bands (DIBs) and in monitoring, in the laboratory, the formation of circumstellar dust grains and planetary atmosphere aerosols from their gas-phase molecular precursors. Plans for future laboratory experiments on interstellar and planetary molecules and grains will also be addressed, as well as the implications of the studies underway for astronomical observations and past and future space mission data analysis.
Salama, Farid↗
Neutron Skin Measurement of 208Pb and 48Ca Using Parity Violating Electron Scattering
Parity-violating electron scattering experiments (PVES) provides a clean probe of neutron densities that is model independent and free from strong interaction uncertainties in interpretation. The PREX-2 and CREX experiments were run in 2019 and 2020 at Jefferson laboratory measured the nucleon skin thickness, the difference between the r.m.s. neutron radius Rn and the r.m.s. proton radius Rp, of 208Pb and 48Ca via parity violating electroweak asymmetry in the elastic scattering of longitudinally polarized electrons. PREX-2 experiment was performed with 950 MeV electrons scattered at a 5¿ angle with Q2 = 0.00616 ± 0.00004 (GeV/c)2, while CREX used 2182 MeV electrons at the same angle with Q2 = 0.0297 ± 0.0002 (GeV/c)2. For PREX-2 the measured asymmetry was AP V = 550 ± 16 (stat.) ± (syst.) ppb, which corresponds to Rskin = 0.278 ± 0.078 (exp.) ± 0.012 (theo.) fm. The CREX asymmetry was AP V = 2668 ± 106 (stat.) ± 40 (syst.) ppb, which corresponds to Rskin = 0.121 ± 0.026 (exp.) ±0.024 (model) fm. One of the crucial systematic uncertainty that PREX-2 and CREX were sensitive to was the non-parity violating asymmetries that resulted from the helicity correlated false asymmetries in the polarized electron beam. There was a lot of work put towards understanding and suppressing the asymmetries arising from these effects. The parity violating asymmetry measurement required a very precise determination of the electron beam polarization. To accurately determine the beam polarization, a Compton polarimeter was used during both PREX-2 and CREX. A careful alignment of the laser to the Fabry-Perot cavity, data analysis and systematic control was employed to get a precise beam polarization result for the experiments. The PREX-2 measurement has broad implications for increasing our knowledge about neutron star structure and the equation of state of nuclear matter. The combined PREX and CREX results will have implications for future energy density functional calculations and the theory of nuclear structure.
Premathilake, Sachinthani↗
Beam Profile Measurements Utilizing an Amplitude Modulated Pulsed Fiber Laser at PIP2IT
Fermilab is undertaking the development of a new 800 MeV superconducting RF linac to replace its present normal conducting 400 MeV linac. The PIP-II linac consists of a warm front-end generating 2 mA of 2.1 MeV H⁻ followed immediately by a series of superconducting RF cryomodules to 800 MeV. To limit the potential damage to the superconducting RF cavities, PIP-II will utilize laser-based monitors to obtain beam profiles via photoionization. This paper will present the results of transverse and longitudinal beam profile measurements using a prototype profile monitor that was tested with 2.1 MeV H⁻ beam at the PIP-II Injector Test (PIP2IT) accelerator. This prototype profile monitor utilizes a high repetition rate fiber laser and fiber optic transport into the PIP2IT enclosure. In addition, results will be shown of narrow-band electron detection from amplitude modulated laser pulses.
43 PARTICLE ACCELERATORS↗
Coupling, Q-Factor, and Integration Aspects of Microsphere Applications
With suggested applications varying from microlaser and cavity QED through optical locking of diode lasers to modulators and sensors, high-Q silica microspheres with whispering-gallery (WG) modes so far remain the subject of tabletop feasibility demonstrations. Despite the uniquely high quality-factor and submillimeter dimensions suitable for tight packaging, this novel type of high-finesse cavity still has to be adapted to fiber- and integrated-optic hardware. In the visible and near infrared-band experiments (633-850nm) measuring the ringdown time tau of free oscillations, Q = (0.6 to 0.8 ) x 10(exp 10) has been obtained in silica spheres of diameter -800 microns (corresponding tau = 3 to 4 microseconds). It was proved that under normal laboratory conditions, quality-factor is subject to deterioration within several-minute scale down to (2 ... 3 ) x 10(exp 9). The responsible mechanism was identified as adsorption of a monolayer of atmospheric water, so that preservation of the ultimate Q requires manipulation in dry environment, or fast packaging into sealed devices. Larger Q can be expected closer to minimum of attenuation in fused silica alpha = 0.2 dB/km; Q greater than or equal to 1 x 10(exp 11) at lambda=1.55 microns, with corresponding energy storage time tau approx. 0.1ms. Experiments are currently underway to determine whether this high Q can be realized experimentally. The evident difficulty is that OH-related optical absorption has its peaks located near the reported minimum of attenuation in silica. We can also mention here that some of proposed fiber materials, yet not ready for fiber drawing, have been predicted to have smaller attenuation than fused silica and may be suitable for microsphere fabrication (sodium-magnesium silicate glass, alpha = 0.06dB/km). WG modes possess very small radiative loss (it does not prevent Q-10(exp 20) and more) and therefore are electromagnetically isolated and cannot be excited by free-space beams. If no modification (such as grating) is made on the sphere surface, the coupling has to he provided by an appropriate near-field device. A systematic theoretical approach has been recently developed to quantify the performance of near-field couplers for WG modes. Efficient coupling can be obtained upon fulfillment of two main conditions: (1) mode matching and (2) sufficient coupling strength to provide the buildup of a WG mode with a given intrinsic loss. In other words, the wave in the coupler has to be phase-matched and sufficiently overlapped with the WG mode to provide enough buildup in the cavity. If the coupling efficiency is characterized by the fractional depth K(sup 2) of the resonance dip in intensity transmittance observed upon varying the frequency of the exciting wave in the coupler.
Ilchenko, V. S.↗
Review of the frequency stabilization of TEA CO2 laser oscillators
Most applications of TEA CO2 lasers in heterodyne radar systems require that the transmitter has a high degree of frequency stability. This ensures good Doppler resolution and maximizes receiver sensitivity. However, the environment within the device is far from benign with fast acoustic and electrical transients being present. Consequently the phenomena which govern the frequency stability of pulsed lasers are quite different from those operative in their CW counterparts. This review concentrates on the mechanisms of chirping within the output pulse; pulse to pulse frequency drift may be eliminated by frequency measurement and correction on successive pulses. It emerges that good stability hinges on correct cavity design. The energy-dependent laser-induced frequency sweep falls dramatically as mode diameter is increased. Thus, it is necessary to construct resonators with good selectivity for single mode operation while having a large spot size.
Willetts, David V.↗
Free electron lasers for transmission of energy in space
A one-dimensional resonant-particle model of a free electron laser (FEL) is used to calculate laser gain and conversion efficiency of electron energy to photon energy. The optical beam profile for a resonant optical cavity is included in the model as an axial variation of laser intensity. The electron beam profile is matched to the optical beam profile and modeled as an axial variation of current density. Effective energy spread due to beam emittance is included. Accelerators appropriate for a space-based FEL oscillator are reviewed. Constraints on the concentric optical resonator and on systems required for space operation are described. An example is given of a space-based FEL that would produce 1.7 MW of average output power at 0.5 micrometer wavelength with over 50% conversion efficiency of electrical energy to laser energy. It would utilize a 10 m-long amplifier centered in a 200 m-long optical cavity. A 3-amp, 65 meV electrostatic accelerator would provide the electron beam and recover the beam after it passes through the amplifier. Three to five shuttle flights would be needed to place the laser in orbit.
Segall, S. B.↗
Single laser beam of spatial coherence from an array of GaAs lasers - Free-running mode
Spatially coherent radiation from a monolithic array of three GaAs lasers in a free-running mode is reported. The lasers, with their mirror faces antireflection coated, are operated in an external optical cavity built of spherical lenses and plane mirrors. The spatially coherent-beam formation makes use of the Fourier-transformation property of the internal lenses. Transverse mode control is accomplished by a spatial filter. The optical cavity is similar to that used for the phase-controlled mode of spatially coherent-beam formation; only the spatial filters are different. In the far field (when restored by an external lens), the intensities of the lasers in the array are concentrated in a single laser beam of spatial coherence, without any grating lobes. The far-field distribution of the laser array in the free-running mode differs significantly from the interference pattern of the phase-controlled mode. The modulation characteristics of the optical waveforms of the two modes are also quite different because modulation is related to the interaction of the spatial filter with the longitudinal modes of the laser array within the optical cavity. The modulation of the optical waveform of the free-running mode is nonperiodic, confirming that the fluctuations of the optical fields of the lasers are random.
Philipp-Rutz, E. M.↗
The causal relationship between melt pool geometry and energy absorption measured in real time during laser-based manufacturing
During laser powder bed fusion additive manufacturing, laser power absorption is governed by a pro -tean pool of molten metal that can present as a highly reflective surface, a deeply absorbing cavity, or some amalgamation thereof. These melt pool dynamics have been linked to defect creation, porosity, and surface finish quality. Although these are therefore critical for determining final part quality, their in-stantaneous influence on laser absorption have only been explored through simulation. To date, direct real-time observations have been elusive due to the locally extreme environment. In this work, we fo-cus a laser on Ti-6Al-4V powder and bare plate while quantifying the time-dependent, absolute energy absorption by monitoring omnidirectional backscattered laser intensity. We also simultaneously record the projective melt pool geometries with high-speed synchrotron x-ray imaging. We find that laser ab-sorption strongly reflects the stability of the vapor depression over a wide range of applied laser powers, oxygen content in the processing atmosphere, and with the presence of powder. During laser scanning of a powder bed surface, we find a significant absorption reduction after 400 mu s due to a dramatic change in the vapor depression aspect ratio-an event known to create porosity. Furthermore, as several industrial scan strate-gies necessitate thousands of these events during a build, their identification and control is of significant practical importance. Lastly, a normalized enthalpy model is demonstrated to be effective in quantifying the relationship between the laser absorption and cavity depth, even under transient conditions. In addi-tion to providing vital quantitative data for simulation calibration, the correlation of melt pool geometry with laser absorption during realistic processing conditions suggests the use of a total backscattered light detection system for real-time process control.
36 MATERIALS SCIENCE↗
Efficient second harmonic generation of picosecond laser pulses.
Efficient conversion to the second harmonic (SH) using KD2PO4 and CsH2AsO4 crystals inside a folded cavity of a high-power-dye mode-locked neodymium-glass laser is reported. For the first time, frequency-doubled picosecond light pulses have been obtained in CsH2AsO4 with peak powers of the order of 1 GW/sq cm at 0.531 micron for an effective pump power density of 4 GW/sq cm.
Rabson, T. A.↗
Longitudinal position dependence of dark line defect growth rate in high-power diode lasers at 790 nm
Using a nondestructive, in situ near-infrared defect imaging technique, we obtained time-resolved images of dark line defect (DLD) growth in the cavities of several high-power 790-nm diode lasers and calculated individual DLD growth rates. A clear longitudinal spatial dependence in the DLD growth rate was observed, in which the DLD growth rate was faster near the anti-reflective (AR) facet. Longitudinal spatial hole burning simulation results indicate that the total photon density increases toward the AR facet, while the carrier density decreases toward the AR facet. Here, these results suggest that photon absorption plays a key role in enhancing DLD growth beyond the contribution of the traditional carrier capture mechanism. Asymmetric DLD growth that was preferentially directed toward the high-reflectivity facet was also observed, providing further support for the role of photon absorption in the growth process. To account for these findings, we propose a photon-accelerated mechanism for the enhancement of DLD growth in which the slower carrier capture process in the traditional recombination-enhanced dislocation glide mechanism is replaced by a faster photon absorption process.
Engineering - Electronic and electrical engineerin↗
Calibration of diode laser spectra using a confocal etalon
The dual-beam diode laser spectrometer described by Jennings (1980) is adapted to use a 50-cm confocal etalon for frequency calibration. The collimated radiation from the laser is split at a wedged ZnSe window, and the reference beam is then focused at the midpoint of the etalon length. After the etalon, the reference beam is recollimated and continues its regular path to the monochromator and detectors. An aperture is placed before the etalon in order to limit the entrance beam diameter to approximately 5 mm. Both ends of the etalon are furnished with two-axis adjustments. Initial alignment is achieved using an He-Ne laser, and final optimization involves adjustment of the cavity length as well as the etalon pitch and yaw. The 50-cm confocal etalon produces fringes separated by 150 MHz (0.005/cm). With the aid of a CO2 laser, it is found to have fringe widths (FWHM) of 2 MHz. The confocal etalon makes it possible to improve the accuracy of relative frequency measurements in diode laser spectra and to check the spectral purity and stability of the laser during the recording of spectra.
Jennings, D. E.↗
Nanosecond semiconductor disk laser emitting at 496.5 nm
An optically pumped semiconductor disk laser based on a heterostructure containing ten CdS/ZnSe coupled quantum wells with type-II band offsets is studied. The structure was grown by metalorganic vapour phase epitaxy (MOVPE) on a GaAs substrate. The peak power of the semiconductor disk laser achieved at room temperature under longitudinal pumping by a repetitively pulsed N{sub 2} laser was 0.75 W at a wavelength of 496.5 nm, a pulse duration of 3 ns, and a pulse repetition rate of 100 Hz. The slope efficiency of the disk laser was 2.7 %. The total divergence angle at a cavity length of 1.1 mm varied from 5 mrad near the lasing threshold to 15 mrad at the maximum pump power. (lasers)
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
Seeded gas thrusters and related system components
A program involved with the construction and test of a number of laser heated thrusters is described. These thrusters, with a cavity approximately 23 cm long and 3.5 cm in i.d., are to be tested by NASA at a later date with a laser beam focused through the throat to heat hydrogen propellant containing an opacifier. The heated propellant exhausts through a supersonic nozzle with a 0.6 cm throat at 3000 C. Thrust stands and control systems were furnished with the thrusters. The report describes radio frequency plasma heated hot and cold flow simulation tests by the contractor.
Poole, J. W.↗
Pulse-by-pulse transient thermal deformation in crystal optics under high-repetition-rate FEL
Time-domain modeling of the thermal deformation of crystal optics can help define acceptable operational ranges across the pulse-energy repetition-rate phase space. In this paper, we have studied the transient thermal deformation of a water-cooled diamond crystal for a cavity-based X-ray free-electron laser (CBXFEL), either an X-ray free-electron laser oscillator (XFELO) or a regenerative amplifier X-ray free-electron laser (RAFEL), by numerical simulations including finite-element analysis and advanced data processing. Pulse-by-pulse transient thermal deformation of a 50 µm-thick diamond crystal has been performed with X-ray pulse repetition rates between 50 kHz and 1 MHz. Results for temperature and thermal deformation have been compared with the results of transient analysis using a continuous wave (CW) power loading. Temperature and thermal deformation results from pulse-by-pulse transient analysis vary with time about the results for the CW case for the same average power. The variation amplitude increases with pulse energy and decreases with repetition rate. When the repetition rate increases to infinity, both temperature and thermal deformation converge to the results for the CW case. Two critical time scales for the operation of crystal optics in a CBXFEL are (1) first-turn time, i.e. the time for the XFEL pulse to complete the first turn around the cavity so that the crystal sees the recirculated XFEL pulse, and (2) period-end time, i.e. the time that the next electron bunch arrives for the amplification, so that the crystal outcouples the amplified FEL power. For the same average power, simulation results show that the crystal thermal deformation seen by the XFEL beam decreases with repetition rate at the first-turn time of a 300 m-long cavity and increases with repetition rate at the period-end time. For the wavefront preservation requirement of the crystal optics, a pulse-energy versus repetition-rate phase space has been established. The upper bounds of the pulse energy at both first-turn and period-end times decreases with repetition rate, especially at the period-end time. The upper bound of the thermal deformation of the crystal at the period-end time for any repetition frequency can be estimated from the CW case. For a water-cooled diamond crystal of dimension 5 mm × 5 mm × 0.05 mm, the time to reach a quasi steady-state is about 50 ms for temperature and 50 µs for thermal deformation.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
Additive manufacturing process parameter determination for a new Fe-C-Cu alloy
As a potential replacement for stainless steel alloys commonly used to print parts with laser powder bed fusion, a new Cu precipitation strengthened ferrous alloy, with composition Fe-0.2C-6Cu (wt%), was recently developed. This material is Co- and Ni-free, printable, has mechanical properties comparable to that of high strength stainless steels (approximately 1300 MPa UTS), and is cost-advantaged relative to existing low-alloy steels for additive manufacturing of parts with complex shapes. To gain traction for broader application, optimal laser powder bed fusion (LPBF) processing conditions to produce nearly defect-free parts without compromising mechanical strength are needed. Here, an optimal processing window based upon laser speeds that achieve minimal porosity was quantified via comparisons of measured melt pool penetration, scan speeds, printed material density and laser beam energy density on a commercial LPBF unit operating at 350 W, 80 μm hatch spacing, and 50 μm layer thickness based upon optimal parameters for 17-4PH. Furthermore, the window is 300 to 500 mm/s to achieve >99.8 % dense Fe-0.2C-6Cu (wt%) specimens. Other defects such as burning, spatter, and lack of fusion were also avoided in this window. The window was validated with in-situ synchrotron X-ray imaging that enabled visualization of the vapor cavity, melting, and solidification during a single laser track scan on a miniature powder bed sample. In addition, in-situ infrared imaging provided temperature fields, cooling rate and solidification range, and confirmed minimal printing defects and spatter within the processing window.
36 MATERIALS SCIENCE↗
Mode Selection for a Single-Frequency Fiber Laser
A superstructured fiber-grating-based mode selection filter for a single-frequency fiber laser eliminates all free-space components, and makes the laser truly all-fiber. A ring cavity provides for stable operations in both frequency and power. There is no alignment or realignment required. After the fibers and components are spliced together and packaged, there is no need for specially trained technicians for operation or maintenance. It can be integrated with other modules, such as telescope systems, without extra optical alignment due to the flexibility of the optical fiber. The filter features a narrow line width of 1 kHz and side mode suppression ratio of 65 dB. It provides a high-quality laser for lidar in terms of coherence length and signal-to-noise ratio, which is 20 dB higher than solid-state or microchip lasers. This concept is useful in material processing, medical equipment, biomedical instrumentation, and optical communications. The pulse-shaping fiber laser can be directly used in space, airborne, and satellite applications including lidar, remote sensing, illuminators, and phase-array antenna systems.
Liu, Jian↗
Dynamic motion trajectory control with nanoradian accuracy for multi-element X-ray optical systems via laser interferometry
The past decades have witnessed the development of new X-ray beam sources with brightness growing at a rate surpassing Moore’s law. Current and upcoming diffraction limited and fully coherent X-ray beam sources, including multi-bend achromat based synchrotron sources and high repetition rate X-ray free electron lasers, puts increasingly stringent requirements on stability and accuracy of X-ray optics systems. Parasitic motion errors at sub-micro radian scale in beam transport and beam conditioning optics can lead to significant loss of coherence and brightness delivered from source to experiment. To address this challenge, we incorporated optical metrology based on interferometric length and angle sensing and real-time correction as part of the X-ray optics motion control system. A prototype X-ray optics system was constructed following the optical layout of a tunable X-ray cavity. On-line interferometric metrology enabled dynamical feedback to a motion control system to track and compensate for motion errors. The system achieved sub-microradian scale performance, as multiple optical elements are synchronously and continuously adjusted. This first proof of principle measurement demonstrated both the potential and necessity of incorporating optical metrology as part of the motion control architecture for large scale X-ray optical systems such as monochromators, delay lines, and in particular, X-ray cavity systems to enable the next generation cavity-based X-ray free electron lasers.
47 OTHER INSTRUMENTATION↗