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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 487 records · Page 27
All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

Crack‐Free Single‐Crystalline LiNiO 2 for High Energy Density All‐Solid‐State Batteries

Abstract Single‐crystalline layered oxide (LiNi 1‐ x ‐ y Mn x Co y O 2 ) cathodes have been found to exhibit exceptional electrochemical properties when coupled with various inorganic solid electrolytes (ISEs) in all‐solid‐state batteries (ASSBs). Their advantages stem from the robust morphological integrity with the absence of grain boundaries and the high electrochemical oxidative stability. Here, ASSBs featuring single‐crystalline LiNiO 2 (LNO) with the highest Ni content are reported, offering a high theoretical specific capacity of 275 mAh g ‐1 alongside a high average discharge voltage (3.7 V vs Li + /Li). Through a careful investigation, it is demonstrated that micron‐sized single‐crystalline LNO (µSC‐LNO) composite cathodes with a halide ISE exhibit a high initial discharge capacity of 205 mAh g ‐1 with an outstanding cycle performance over 200 cycles in room‐temperature ASSBs. The significance of engineering parameters is emphasized, such as particle size and specific density, in promoting a homogeneous and fast Li + transport within the composite cathodes. Furthermore, the formation of undesirable interphase between the halide ISE in the cathode and sulfide ISE separator is elucidated, which may be a critical factor impeding long‐term cyclability of ASSBs. This work provides insights into the design of composite cathodes for high‐energy‐density ASSBs.

Chemistry↗
DOE OSTI2024

Gate-Controlled Anyon Generation and Detection in Kitaev Spin Liquids

Reliable manipulation of non-Abelian Ising anyons supported by Kitaev spin liquids may enable intrinsically fault-tolerant quantum computation. Here, we introduce a standalone scheme for both generating and detecting individual Ising anyons using tunable gate voltages in a heterostructure containing a non-Abelian Kitaev spin liquid and a monolayer semiconductor. In this study, the key ingredients of our setup are a Kondo coupling to stabilize an Ising anyon in the spin liquid around each electron in the semiconductor, and a large charging energy to allow control over the electron numbers in distinct gate-defined regions of the semiconductor. In particular, a single Ising anyon can be generated at a disk-shaped region by gate tuning its electron number to one, while it can be interferometrically detected by measuring the electrical conductance of a ring-shaped region around it whose electron number is allowed to fluctuate between zero and one. We provide concrete experimental guidelines for implementing our proposal in promising candidate materials like α-RuCl 3 .

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2026

Site-decorated model for unconventional frustrated magnets: Ultranarrow phase crossover and two-dimensional spin reversal transition

Here, the site-decorated Ising model is introduced to advance the understanding and experimental realization of the recently discovered one-dimensional (1D) finite-temperature ultranarrow phase crossover in an external magnetic field, while mitigating the geometric complexities of traditional bond-decorated models. The unconventional frustration and physics are clarified by exactly mapping the 1D site-decorated Ising model in a magnetic field onto a zero-field bond-decorated 𝐽 1 −𝐽 2 Ising model with conventional geometrical frustration. Furthermore, although higher-dimensional Ising models in an external field remain unsolved exactly, an exact solution for a spin-reversal transition—driven by an exotic, hidden half-ice, half-fire state induced by site decoration—is derived. This transition, triggered by a slight variation in temperature or magnetic field—without changing its direction—even in the weak-field limit, offers a promising route toward energy-efficient applications such as data storage and processing. The results suggest that site decoration offers an avenue for materials and device design, particularly in systems such as mixed 𝑑−𝑓 compounds, optical lattices, and neural networks, calling for further studies with site-decorated Heisenberg models. In addition, the site-decorated model offers a rigorous test ground for artificial intelligence (AI) in science, as the analytic derivation of the present results was not only validated but also improved by a general-purpose large language model, inspiring the use of AI as scientific discoverer.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2024

DS-GL: Advancing Graph Learning via Harnessing the Power of Nature within Dynamic Systems

With the rapid digitization of the world, an increasing number of real-world applications are turning to nonEuclidean data, modeled as graphs. Due to their intrinsic high complexity and irregularity, learning from graph data demands tremendous computational power. Recently, CMOS-compatible Ising machines, i.e., dynamic systems composed of CMOS components, have emerged as a new approach that harnesses the inherent power of natural annealing within dynamic systems to efficiently resolve binary optimization problems and have been adopted for traditional graph computation, such as max-cut. However, when performing complex Graph Learning (GL) tasks, Ising machines face significant hurdles: (i) they are inherently binary and thus ill-suited for real-valued problems; (ii) their expensive all-to-all coupling network that guarantees effective natural annealing poses daunting scalability concerns. To address these challenges, this paper proposes a nature-powered graph learning framework dubbed DS-GL, which is the first effort to transform the process of solving graph learning problems into the natural annealing process within a parameterized dynamic system embodied as a CMOS chip. To tackle the two major hurdles, DS-GL first augments the Ising machine architecture to modify the self-reaction term of its Hamiltonian function from linear to quadratic, effectively serving as an energy regulator. This adjustment maintains the system’s original physical interpretation while enabling it to process continuous, real-valued data. Second, to address the scaling issue, DS-GL further upgrades the real-valued dense Ising machine by decomposing it into a mesh-based multi-PE dynamic system that supports efficient distributed spatial-temporal co-annealing across different PEs through sparse interconnects. By exploiting the inherent sparsity and component structures in real-world graphs, DS-GL is able to map complex graph learning tasks onto the scalable dynamic system while maintaining high accuracy. Evaluations with three diverse GL applications across six real-world datasets, including traffic flow and COVID-19 prediction, show that DS-GL can deliver from 102× to 106× speedups and 500× energy reduction over Graph Neural Networks on GPUs, with 5% - 20% accuracy enhancement.

Song, Ruibing↗
DOE OSTI2026

Electrochemical testing of metals for petroleum wastewater monitoring

The purpose of this project was to determine the feasibility of ion-selective electrode (ISE) as compared to x-ray fluorescence (XRF) for determining the concentrations of metal ions in petroleum wastewater. ISEs for silver and cadmium were tested in a laboratory under increasingly realistic conditions, then deployed in the sewer wastewater monitoring complex to simulate a petroleum wastewater system. By verifying the ISE calibration after wastewater exposure and comparing its measurements to the XRF systems within the wastewater monitoring system, we determined that the ISE is more sensitive but less feasible for use in live wastewater monitoring due to fouling concerns.

Energy - Petroleum↗
NASA NTRS1977

International Sun-Earth Explorer - A three-spacecraft program

The International Sun-Earth Explorer (ISEE) is a three-spacecraft system developed by NASA and ESA to study the magnetospheric structure, paying attention to the quantitative mechanism of magnetospheric response to external perturbations, and the structure of its parts. In particular, the nature, structure, motion, and stability of magnetospheric boundaries will be studied, including bow shock, magnetopause, plasmapause, and neutral sheet. Spacecraft ISEE-A and ISEE-B will be launched into the same orbit (of apogee 23 earth radii) but separated by a small, controllable distance, and will make observations from within the magnetosphere. The ISEE-C spacecraft will be launched into a heliocentric orbit (234 earth radii upstream) and will make observations in the solar wind upstream of the earth.

Ogilvie, K. W.↗
NASA NTRS1980

Hectometer and kilometer solar observations

Three dimensional 'snapshots' of the large scale solar magnetic field topology as well as the solar wind electron density distribution from about 0.1 to 1 AU are obtained by tracking traveling solar radio bursts at the hectometer and kilometer wavelengths with instruments aboard the ISEE-3 satellite and the HELIOS-2 solar probe. Both instruments observe in the frequency range from 30 kHz to a 1 MHz and both are equipped with dipole antennas located in the vehicle spin plane. ISEE-3 also has a dipole along the spin axis and the signals from the two ISEE-3 antennas are combined to give the aximuth and elevation angles of the radio source. Triangulation between HELIOS-2 and ISEE-3 provides the additional observation necessary to determine uniquely the position of the radio source in space at each observing frequency.

Stone, R. G.↗
NASA NTRS1983

Energetic ions upstream of the earth's bow shock during an energetic storm particle event

Simultaneous observations of low-energy protons and alpha particles from ISEE 3 far upstream and from ISEE 1 close to the earth's bow shock during the passage of an interplanetary shock wave with its associated energetic storm particles are presented. Intensities, spectra, and anisotropies of the energetic storm particles are modified due to the interaction of these particles with the earth's bow shock. An intensity spike observed at ISEE 1 during the passage of the interplanetary shock is interpreted as being due to postacceleration of energetic storm particles at the bow shock by the first-order Fermi mechanism. The spikes observed at ISEE 1 after the passage of the interplanetary shock are most probably due to reflection of the energetic storm particles at the bow shock.

Scholer, M.↗
NASA NTRS1984

Magnetic field draping against the dayside magnetopause

Interplanetary magnetic fields observed upstream of Earth's magnetosphere at ISEE 3 form input for a gasdynamic model of magnetic field draping in the dayside magnetosheath. Model results near the magnetopause are compared with appropriately lagged observations at ISEE 1. In 16 to 24 cases, the angle between the transverse component of the model and observed fields is less than 20 deg. The agreement is surprisingly good in view of the uncertainty introduced by the large distances between ISEE 1 and ISEE 3. The results indicate that magnetohydrodynamic and energy transfer processes at the magnetopause do not cause large distortions of the magnetosheath magnetic field. In addition, a comparison between observed and model field magnitudes indicates that immediately outside the magnetopause the observed field behaves like the model field at a distance of approx. 0.5 R sub E from the magnetopause, outside the region where magnetohydrodynamic effects make the gasdynamic model inapplicable. Patterns of model magnetic field orientation at the magnetopause are presented for practical application.

Crooker, N. U.↗
NASA NTRS1984

Drift mirror mode waves in the distant (about 200 earth radii) magnetosheath

The physical mechanisms which produced large magnetic field magnitude changes beyond 60 earth radii during ISEE-3 passage are discussed in relation to interplanetary conditions. The ISEE-3 data were taken close to the time that IMP-8 data signaled an interplanetary shock and the crossing of the terrestrial magnetosheath. The ISEE detected decreases (10-50 percent) in field magnitude that the IMP did not. The electron temperature and density and magnetic field data made by the ISEE indicated the presence of drift mirror mode waves. The instabilities would have been triggered in the magnetosheath plasma by arrival of the driver gas of the solar wind detected by the IMP-8. The waves were especially prominent due to the relative quiescence of the usually turbulent magnetosheath when the shock arrived.

Tsurutani, B. T.↗
NASA NTRS1985

Electric fields in the plasma sheet and plasma sheet boundary layer

Results obtained by Forbes et al. (1981) on the basis of time delay measurements between ISEE 1 and ISEE 2 imply that the plasma flow and the boundary contracting velocity were nearly the same, whereas the expanding boundary velocity was not accompanied by any significant plasma sheet plasma motion. In the present study, this observation is discussed in conjunction with electric field data. The study is based on electric field data from the spherical double probe experiment on ISEE 1. Electric field data from GEOS 2 are used to some extent to monitor the electric fields near the geostationary orbit during the considered eve nts. Electric field data during CDAW 6 events are discussed, taking into account positions of ISEE 1/ISEE 2 and GEOS 2; March 22, 0600-1300 UT; and March 22, UT; and March 31, 1400-2400 UT.

Pedersen, A.↗
NASA NTRS1985

Magnetic field draping against the dayside magnetopause

Interplanetary magnetic fields observed upstream of earth's magnetosphere at ISEE 3 form input for a gasdynamic model of magnetic field draping in the dayside magnetosheath. Model results near the magnetopause are compared with appropriately lagged observations at ISEE 1. In 16 to 24 cases, the angle between the transverse component of the model and observed fields is less than 20 deg. The agreement is surprisingly good in view of the uncertainty introduced by the large distances between ISEE 1 and ISEE 3. The results indicate that magnetohydrodynamic and energy transfer processes at the magnetopause do not cause large distortions of the magnetosheath magnetic field. In addition, a comparison between observed and model field magnitudes indicates that immediately outside the magnetopause the observed field behaves like the model field at a distance of approx. 0.5 R sub E from the magnetopause, outside the region where magnetohydrodynamic effects make the gasdynamic model inapplicable. Patterns of model magnetic field orientation at the magnetopause are presented for practical application.

Crooker, N. U.↗
NASA NTRS1986

On the use of a sunward libration-point-orbiting spacecraft as an interplanetary magnetic field monitor for magnetospheric studies

In order to test the accuracy of using magnetometer data from a spacecraft orbiting the sunward libration point to determine the orientation of the interplanetary magnetic field (IMF), the angle between the IMF at ISEE 3, when it was positioned around the libration point, and at ISEE 1, orbiting the earth, has been calculated for a data set of 1-hour periods covering four months. For each period, a 10-minute average of ISEE 1 data is compared with 10-minute averages of ISEE 3 data at successively lagged intervals. It is concluded that the IMF orientation at a libration-point-orbiting spacecraft, lagged by the time required for the solar wind to convect to the earth, is a convenient predictor of IMF orientation near the earth, to within about 20-degree accuracy.

Kelly, T. J.↗
NASA NTRS1988

Implications of large flow velocity signatures in nearly isotropic ion distributions

ISEE-1 energetic ion distributions are compared with previously published lower-energy ISEE-1 H(+) and He(2+) distributions in the quiet-time plasma sheet at about 15 earth radii and within about 1 earth radius of the expected neutral sheet position. Although moment calculations performed over the nearly isotropic H(+) and He(2+) plasma distributions yield low bulk velocities of less than 14 km/s, the spectral shapes of these signatures are indicative of high flow speeds. It is suggested that H(+) and H(2+) ions of solar wind origin were accelerated through an electrostatic potential of about 2.4 kV prior to the ISEE-1 observations in the plasma sheet on a closed magnetospheric field line, and that a second plasma sheet population existed at this ISEE-1 position in the geomagnetic field.

Williams, D. J.↗
NASA NTRS1990

Magnetic field line draping in the plasma depletion layer

Simultaneous IMP 8 solar wind and ISEE 1/2 observations for a northern dawn ISEE 1/2 magnetopause crossing on November 6, 1977. During this crossing, ISEE 1/2 observed quasi-periodic pulses of magnetosheathlike plasma on northward magnetic field lines. The ISEE 1/2 observations were originally interpreted as evidence for strong diffusion of magnetosheath plasma across the magnetopause and the Kelvin-Helmholtz instability at the inner edge of the low-latitude boundary layer. An alternate explanation, in terms of magnetic field merging and flux transfer events, has also been advocated. In this paper, a third interpretation is proposed in terms of quasi-periodic magnetopause motion which causes the satellites to repeatedly exit the magnetosphere and observe draped northward magnetosheath magnetic field lines in the plasma depletion layer.

Sibeck, D. G.↗
NASA NTRS1994

Statistical characteristics of bursty bulk flow events

Using a common methodology to analyze data from the Active Magnetospheric Particle Tracer Explorer/Ion Release Module (AMPTE/IRM) and International Sun-Earth Explorer 2 (ISEE 2) satellites we report on the statistical properties of bursty bulk flow events (BBFs) in the inner plasma sheet (IPS). A positive correlation between BBFs and the AE index suggests that BBFs are predominantly geomagnetically active time phenomena. Earthward BBFs are more frequent close to midnight and away from Earth, up to a distance of approximately 19 R(sub E). Tailward BBFs are very infrequent in the IRM data set and somewhat less infrequent in the ISEE 2 data set in the region of the satellites' spatial overlap, possibly due to the more active conditions prevailing during the ISEE 2 mission in that region. However, in both data sets the ratio of tailward to earthward BBFs increases with distance from Earth; more than 20% of all BBFs are anti-sunward tailward of X = -19 R(sub E) in the ISEE 2 data set. BBFs are responsible for 60-100% of the measured earthward transport of mass, energy and magnetic flux past the satellite in the regions of maximum occurrence rate, even though they last approximately 10-15% of the IPS observation time there. Thus BBFs represent the primary transport mechanism at those regions. The one-to-one correspondence between BBFs and substorm phase, as well as the relative contribution of BBFs to the total transport observed during substorms are questions that await further investigation based on multi instrument studies of individual events.

Angelopoulos, V.↗
NASA NTRS2000

Investigation of the Transport of Solar Ions Through the Earth's Magnetosphere

The objective of this study has been to infer, by statistical means, the most probable mode of entry of solar wind plasma into Earth's magnetotail, using a particular set of archived data from the Lockheed Plasma Composition Experiment on the International Sun-Earth Explorer One (ISEE-1) satellite, jointly sponsored by the National Aeronautics and Space Administration (NASA) and the European Space Agency (ESA) in the 1970's and 80's. Despite their considerable age, the Lockheed ISEE-1 data are still, at the time of this report, the only substantial ion composition data in the sub-keV to keV energy range available from the magnetotail beyond 9 R(sub E), because of various technical problems with ion mass spectrometers on later missions, and are therefore a unique source of information about the mixing of solar and terrestrial origin plasmas in the tail, within the ISEE-1 apogee of almost 23 R(sub E). The entire set of archived data used in this study, covering the 4.5 years of operation of the instrument and comprising not only tail measurements but also data from the inner magnetosphere as well as data from outside the magnetopause, is now available to the public via the WorldWideWeb at the address: http://cis.spasci.com/ISEE_ions The fundamental assumption of this and other studies of magnetosphere ion composition is that He++ and O+ ions are virtually certain "tags" of solar and terrestrial origins, respectively. This is an assumption with strong theoretical basis and it is corroborated by observational evidence, including the often substantial differences between the velocity distribution functions of those two species. The H+ ions can have a dual origin, in principle, but the close resemblance in the ISEE-1 data between the dynamics of H+ and He++ ions indicates a predominantly solar origin of the H+ ions in the tail, at least. By the same token, the usually minor He+ ions are probably almost entirely of terrestrial origin, because of their similarity to the O+ ions.

Lennartsson, O. W.↗
DOE OSTI2023

Noise dynamics of quantum annealers: estimating the effective noise using idle qubits

Quantum annealing is a type of analog computation that aims to use quantum mechanical fluctuations in search of optimal solutions of QUBO (quadratic unconstrained binary optimization) or, equivalently, Ising problems. Since NP-hard problems can in general be mapped to Ising and QUBO formulations, the quantum annealing paradigm has the potential to help solve various NP-hard problems. Current quantum annealers, such as those manufactured by D-Wave Systems, Inc. have various practical limitations including the size (number of qubits) of the problem that can be solved, the qubit connectivity, and error due to the environment or system calibration, which can reduce the quality of the solutions. Typically, for an arbitrary problem instance, the corresponding QUBO (or Ising) structure will not natively embed onto the available qubit architecture on the quantum chip. Thus, in these cases, a minor embedding of the problem structure onto the device is necessary. However, minor embeddings on these devices do not always make use of the full sparse chip hardware graph, and a large portion of the available qubits stay unused during quantum annealing. In this work, we embed a disjoint random QUBO on the unused parts of the chip alongside the QUBO to be solved, which acts as an indicator of the solution quality of the device over time. Using experiments on three different D-Wave quantum annealers, we demonstrate that (i) long term trends in solution quality exist on the D-Wave device, and (ii) the unused qubits can be used to measure the current level of noise of the quantum system.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗