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At least 487 records · Page 27

Adiabatic cooling of planar motion in a Penning-trap ion crystal to sub-millikelvin temperatures

Two-dimensional planar ion crystals in a Penning trap are a platform for quantum information science experiments. However, the low-frequency planar modes of these crystals are not efficiently cooled by laser cooling, which can limit the utility of the drumhead modes for quantum information processing. Recently, it has been shown that nonlinear mode coupling can enhance the cooling of the low-frequency planar modes. Here, in this study, we demonstrate in numerical simulations that this coupling can be dynamically tuned by adiabatically changing the rotation frequency of the ion crystal during experiments. Furthermore, we show that this technique can, in addition, produce lower temperatures for the low-frequency planar modes via an adiabatic cooling process. This result allows cooling of the planar modes to sub-millikelvin temperatures, resulting in improved spectral resolution of the drumhead modes at experimentally relevant rotation frequencies, which is crucial for quantum information processing applications.

Johnson, Wes [Univ. of Colorado, Boulder, CO (Unit↗

Simulating strongly correlated molecules with a superconducting quantum processor

Many of the biggest challenges in expanding the nation’s access to clean and low-cost energy resources are fundamentally chemistry or materials challenges. An important case is the development of new catalysts for the up-conversion of cheap and readily available materials such as methane or water into materials suitable for use as a fuel such as methanol or oxygen. To understand and exploit such processes, computer simulations of chemical reactions provide a natural complement to experimental studies. Unfortunately, most catalytic reactions involve so-called “strongly correlated” molecules which are notoriously difficult to study with simulation algorithms that can be executed on existing (classical) computers. The recent growth in quantum information science offers an alternative potential route for simulating these difficult systems. As a result, an increasing number of computational chemists are becoming interested in quantum computing. At the same time, quantum information scientists have identified chemistry simulation as a possible first demonstration of a quantum computer providing an improvement over a classical computer. The objective of this project is to accurately simulate strongly correlated molecules on a quantum processor. To meet the high challenges of this objective, new hybrid quantum/classical algorithms will be co-designed with advanced quantum gate developments and computed on customized quantum hardware. Some of the developed techniques will be transferable to study other molecular systems, while the project as a whole will help define better strategies for advancing the quantum simulation of matter more generally.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Influence of substituents on the vectorial difference static dipole upon excitation in synthetic bacteriochlorins

Organic dye aggregates have been shown to exhibit exciton delocalization in natural and synthetic systems. Such dye aggregates show promise in the emerging area of quantum information science (QIS). We believe that the difference static dipole (Δd) is an essential dye parameter in the development of molecular QIS systems. However, a foundational understanding of the structural factors influencing Δd remains elusive. Bacteriochlorins play a vital role in photosynthesis due to their exceptional photophysical properties. Therefore, bacteriochlorins are particularly suitable dyes for the construction of aggregate systems for QIS. Synthetic bacteriochlorins further offer stability and tunability via chemical modifications. Here, the influence of substituents on the Δd of monomeric (non-aggregated) dyes was investigated via density functional theory (DFT) and time-dependent (TD-)DFT in a set of 5-methoxybacteriochlorins progressively substituted with ethynyl, phenyl, and phenylethynyl substituents at the 3,13- and 3,13,15-positions of the macrocycle. Symmetrically substituted 5-methoxybacteriochlorins were shown to have the largest Δd. The increase in Δd in the series of dyes was largely due to changes in orientation of the static dipole upon excitation rather than large changes in magnitude. In addition, the transition dipole (μ) and the angle between Δd and μ (ζ) were calculated. Three 5-methoxybacteriochlorins with high predicted Δd and μ were synthesized and characterized spectroscopically. The trend in Δd values empirically determined using the solvatochromic Stokes shift method was comparable with the DFT calculations.

36 MATERIALS SCIENCE↗

Quantum Control of Spins in Diamond for Nanoscale Magnetic Sensing and Imaging

Our research activities during the grant period focused on the challenges of highly accurate and precise magnetometry and magnetic imaging using quantum spins inside diamond. Our work has resulted in 6 papers published in peer-reviewed journals, with two more currently under consideration by referees. We showed that through the use of novel phase estimation algorithms inspired by quantum information science we can carry out accurate and high dynamic range DC magnetometry as well as lock-in detection of oscillating (AC) magnetic fields. We investigated the geometric phase as a route to higher precision quantum information and magnetic sensing applications, and probed the experimental limits to the fidelity of such geometric phase gates. We also demonstrated that there is a spin dependent signal in the charge state flipping of the NV defect center in diamond, which could potentialy be useful for higher fidelity spin readout at room temperature. Some of these projects have now led to further investigation in our lab on multi-photon spectroscopy (manuscript in preparation), and plasmonic guiding of light in metal nanowires (manuscript available on arxiv). In addition, several invited talks were given by the PI, and conference presentations were given by the graduate students and postdocs.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Enabling Communities in the Use and Application of NASA's Earth Science Data and Information Products: Interactive Webinars that Work

The vast active archives of NASA's Earth science data reflect the agency's ongoing commitment to producing the highest quality data, services and tools intended for a myriad of science and application uses worldwide. These data span the whole of Earth science domains, and most have direct uses in societal applications. As many internet-based tools mature they enable NASA to increase the availability to and, most importantly, the uses of these disparate data types. This poster/paper highlights one particularly effective tool the NASA Earth Science Data and Information System (ESDIS) Project is utilizing to increase our user communities' understanding of these data, services and tools and their varied uses. Webinars, or video-based, on-line, interactive discussions and presentations have become a staple for exchanging information via the internet. The NASA ESDIS Project is using this platform to create a rich, highly-available, source of cutting-edge insights into the uses of Earth science data and applications. As evidence, we present a representative sample of the webinar offerings created by ESDIS beginning in 2013.

Lindsay, Francis E.↗

Snowmass Computational Frontier: Topical Group Report on Quantum Computing

Quantum computing will play a pivotal role in the High Energy Physics (HEP) science program over the early parts of the 21$^{st}$ Century, both as a major expansion of our capabilities across the Computational Frontier, and in synthesis with quantum sensing and quantum networks. This report outlines how Quantum Information Science (QIS) and HEP are deeply intertwined endeavors that benefit enormously from a strong engagement together. Quantum computers do not represent a detour for HEP, rather they are set to become an integral part of our discovery toolkit. Problems ranging from simulating quantum field theories, to fully leveraging the most sensitive sensor suites for new particle searches, and even data analysis will run into limiting bottlenecks if constrained to our current computing paradigms. Easy access to quantum computers is needed to build a deeper understanding of these opportunities. In turn, HEP brings crucial expertise to the national quantum ecosystem in quantum domain knowledge, superconducting technology, cryogenic and fast microelectronics, and massive-scale project management. The role of quantum technologies across the entire economy is expected to grow rapidly over the next decade, so it is important to establish the role of HEP in the efforts surrounding QIS. Fully delivering on the promise of quantum technologies in the HEP science program requires robust support. It is important to both invest in the co-design opportunities afforded by the broader quantum computing ecosystem and leverage HEP strengths with the goal of designing quantum computers tailored to HEP science.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Approach to Managing MeaSURES Data at the GSFC Earth Science Data and Information Services Center (GES DISC)

A major need stated by the NASA Earth science research strategy is to develop long-term, consistent, and calibrated data and products that are valid across multiple missions and satellite sensors. (NASA Solicitation for Making Earth System data records for Use in Research Environments (MEaSUREs) 2006-2010) Selected projects create long term records of a given parameter, called Earth Science Data Records (ESDRs), based on mature algorithms that bring together continuous multi-sensor data. ESDRs, associated algorithms, vetted by the appropriate community, are archived at a NASA affiliated data center for archive, stewardship, and distribution. See http://measures-projects.gsfc.nasa.gov/ for more details. This presentation describes the NASA GSFC Earth Science Data and Information Services Center (GES DISC) approach to managing the MEaSUREs ESDR datasets assigned to GES DISC. (Energy/water cycle related and atmospheric composition ESDRs) GES DISC will utilize its experience to integrate existing and proven reusable data management components to accommodate the new ESDRs. Components include a data archive system (S4PA), a data discovery and access system (Mirador), and various web services for data access. In addition, if determined to be useful to the user community, the Giovanni data exploration tool will be made available to ESDRs. The GES DISC data integration methodology to be used for the MEaSUREs datasets is presented. The goals of this presentation are to share an approach to ESDR integration, and initiate discussions amongst the data centers, data managers and data providers for the purpose of gaining efficiencies in data management for MEaSUREs projects.

Vollmer, Bruce↗

Ultralow-light-level all-optical transistor in rubidium vapor

An all-optical transistor (AOT) is a device in which one light beam can efficiently manipulate another. It is the foundational component of an all-optical communication network. An AOT that can operate at ultralow light levels is especially attractive for its potential application in the quantum information field. Here, we demonstrate an AOT driven by a weak light beam with an energy density of 2.5 × 10{sup −5} photons/(λ{sup 2}/2π) (corresponding to 6 yJ/(λ{sup 2}/2π) and about 800 total photons) using the double-Λ four-wave mixing process in hot rubidium vapor. This makes it a promising candidate for ultralow-light-level optical communication and quantum information science.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Unitary circuit synthesis for tomography of generalized coherent states

We present a method that outputs a sequence of simple unitary operations to prepare a given quantum state that is a generalized coherent state. Our method takes as inputs the expectation values of some relevant observables. Such expectations can be estimated by performing projective measurements on $\mathcal{O}$(M 3 log(M/δ)/ε 2 ) copies of the state, where M is the dimension of an associated Lie algebra, ε is a precision parameter, and 1 - δ is the required confidence level. The method can be implemented on a classical computer and runs in time $\mathcal{O}$(M 4 log(M/ε)). It provides $\mathcal{O}$(Mlog(M/ε)) simple unitaries that form the sequence. The overall complexity is then polynomial in M, being very efficient in cases where M is significantly smaller than the Hilbert space dimension, as for some fermion algebras. When the algebra of relevant observables is given by certain Pauli matrices, each simple unitary may be easily decomposed into two-qubit gates. We discuss applications to efficient quantum state tomography and classical simulations of quantum circuits. $\mathcal{O}$

97 MATHEMATICS AND COMPUTING↗

Correction to Norm-conserving pseudopotentials and basis sets to explore Lanthanide chemistry in complex environments

Correction was made to the funding and acknowledgment: Funding V.-A.G. was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division. R.R. and M.-T.N. were supported by the Laboratory Directed Research and Development Program at Pacific Northwest National Laboratory (PNNL) CheMSR Agile Investment. PNNL is operated by DE-AC05-76RLO01830. J.-B.L. and J.L. were supported by the National Natural Science Foundation of China (Nos. 21433005, 91645203, and 21590792). D.C.C. was supported by Research and Innovation at the University of Nevada, Reno. ACKNOWLEDGMENTS The research was performed using resources available through Research Computing at Pacific Northwest National Laboratory (PNNL), Tsinghua National Laboratory for Information Science and Technology and the Computational Chemistry Laboratory under Tsinghua Xuetang Talents Program, and University of Nevada, Reno High Performance Computing. J.- B.L. and J.L. acknowledge discussions with Dr. Yang-Gang Wang (Southern University of Science and Technology).

Lu, Jun-Bo↗

The Goddard Earth Sciences and Technology Center (GEST Center)

The following is a technical report of the progress made under Cooperative Agreement NCC5494, the Goddard Earth Sciences and Technology Center (GEST). The period covered by this report is October 1, 2001 through December 31, 2001. GEST is a consortium of scientists and engineers, led by the University of Maryland, Baltimore County (UMBC), to conduct scientific research in Earth and information sciences and related technologies in collaboration with the NASA Goddard Space Flight Center (GSFC). GEST was established through a cooperative agreement signed May 11, 2000, following a competitive procurement process initiated by GSFC.

Source record↗

Realization of optical bistability and multistability in Landau-quantized graphene

The solution of input-output curves in an optical ring cavity containing Landau-quantized graphene is theoretically investigated taking the advantage of density-matrix method. It is found that under the action of strong magnetic and infrared laser fields, one can efficiently reduce the threshold of the onset of optical bistability (OB) at resonance condition. At non-resonance condition, we observed that graphene metamaterial can support the possibility to obtain optical multistability (OM), which is more practical in all-optical switching or coding elements. We present an analytical approach to elucidate our simulations. Due to very high infrared optical nonlinearity of graphene stemming from very unique and unusual properties of quantized Landau levels near the Dirac point, such controllability on OB and OM may provide new technological possibilities in solid state quantum information science.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

The Carbon Storage Technical Viability Approach (CS TVA)

The Carbon Storage Technical Viability Approach (CS TVA) StoryMap provides an in-depth overview of the products created during the CS TVA research effort. In detail, the StoryMap addresses the CS TVA Matrix, Database Version 2.0, Database Catalog, Workflow, and Data Availability Result Database, discussing how each was developed and implemented. Information on how the matrix, database, and database catalog are interconnected, and their usage is also explained. The workflow section provides information on the CS TVA product development from the data-gathering stage to the final data availability results. A section on an expansion of the CS TVA workflow that utilizes Natural Language processing (NLP) section was included. Finally, the Data Availability Results Database is discussed. These results provide data science-informed insights into potential data gaps when assessing the viability of carbon storage in a given area or region.

Carbon Storage↗

A Field Campaign to Study Lightning that Ignites the Bush

The impact of recent wildland fires in the United States and Australia have received much attention in the past several years. As a result, NASA has developed a new Earth Science program to better understand, predict, and manage this phenomenon, as well as a future suborbital mission to studying pyro-cumulonimbus clouds and their effects on the Earth system. In Australia, government and philanthropic stakeholders are supporting a series of field campaigns over the next few years to inform science requirements and advance technology for a future satellite mission to monitor Bushfires. Lightning flashes are a major source of wildland fires, but uncertainties remain about the physical characteristics of lightning and their parent thunderstorms responsible for igniting wildfires. It was long believed that most lightning-ignited wildfires are largely caused by positive flashes to the ground (CGs) and multi-stroke CGs, but a recent study looking at 26-years of NLDN data indicate otherwise. Perhaps this finding is due to statistical chance—there are more negative CGs that occur globally—or perhaps there is some unknown electrical property of the thundercloud from which the igniting flashes emanate. Regardless, new observing strategies are needed. Additionally, long continuing current CGs, which are more likely to ignite a fire, can elude detection by operational ground-based lightning location systems, making it difficult to efficiently identify potential wildland fires and manage them before they have adverse impacts. To address these science and operational gaps, NASA’s Lightning Mapping Array along with electric and magnetic field change meters will be deployed for the Australian Bushfire campaign to document the electrical structure and properties of thunderstorms and lightning that occur in a wildland fire susceptible region. Another aspect of the campaign will be the use of NASA’s airborne lightning observatory, which includes a spectrometer and high-speed imager, to document the radiometric attributes of these flashes coincident with the ground-based RF observations. These observations will be used to better understand the properties of lightning that ignite wildland fires as well as inform design of a lightning detection system for the future Bushfire Monitoring satellite mission.

lightning↗

Automation and hypermedia technology applications

This paper represents a progress report on HyLite (Hypermedia Library technology): a research and development activity to produce a versatile system as part of NASA's technology thrusts in automation, information sciences, and communications. HyLite can be used as a system or tool to facilitate the creation and maintenance of large distributed electronic libraries. The contents of such a library may be software components, hardware parts or designs, scientific data sets or databases, configuration management information, etc. Proliferation of computer use has made the diversity and quantity of information too large for any single user to sort, process, and utilize effectively. In response to this information deluge, we have created HyLite to enable the user to process relevant information into a more efficient organization for presentation, retrieval, and readability. To accomplish this end, we have incorporated various AI techniques into the HyLite hypermedia engine to facilitate parameters and properties of the system. The proposed techniques include intelligent searching tools for the libraries, intelligent retrievals, and navigational assistance based on user histories. HyLite itself is based on an earlier project, the Encyclopedia of Software Components (ESC) which used hypermedia to facilitate and encourage software reuse.

Jupin, Joseph H.↗

Optimizing for an arbitrary perfect entangler. II. Application

The difficulty of an optimization task in quantum information science depends on the proper mathematical expression of the physical target. In this paper we demonstrate the power of optimization functionals targeting an arbitrary perfect two-qubit entangler, which allow generation of a maximally entangled state from some initial product state. We show for two quantum information platforms of current interest, i.e., nitrogen vacancy centers in diamond and superconducting Josephson junctions, that an arbitrary perfect entangler can be reached faster and with higher fidelity than both specific two-qubit gates and local equivalence classes of two-qubit gates. Our results are obtained using two independent optimization approaches, underscoring the critical role of the optimization target.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Computing with Beowulf

Parallel computers built out of mass-market parts are cost-effectively performing data processing and simulation tasks. The Supercomputing (now known as "SC") series of conferences celebrated its 10th anniversary last November. While vendors have come and gone, the dominant paradigm for tackling big problems still is a shared-resource, commercial supercomputer. Growing numbers of users needing a cheaper or dedicated-access alternative are building their own supercomputers out of mass-market parts. Such machines are generally called Beowulf-class systems after the 11th century epic. This modern-day Beowulf story began in 1994 at NASA's Goddard Space Flight Center. A laboratory for the Earth and space sciences, computing managers there threw down a gauntlet to develop a $50,000 gigaFLOPS workstation for processing satellite data sets. Soon, Thomas Sterling and Don Becker were working on the Beowulf concept at the University Space Research Association (USRA)-run Center of Excellence in Space Data and Information Sciences (CESDIS). Beowulf clusters mix three primary ingredients: commodity personal computers or workstations, low-cost Ethernet networks, and the open-source Linux operating system. One of the larger Beowulfs is Goddard's Highly-parallel Integrated Virtual Environment, or HIVE for short.

Cohen, Jarrett↗

Tomography of the quantum state of photons entangled in high dimensions

Systems entangled in high dimensions have recently been proposed as important tools for various quantum information protocols, such as multibit quantum key distribution and loophole-free tests of nonlocality. It is therefore important to have precise knowledge of the nature of such entangled quantum states. We tomographically reconstruct the quantum state of the two photons produced by parametric downconversion that are entangled in a d-dimensional orbital angular momentum basis. We determine exactly the density matrix of the entangled two-qudit state with d ranging from 2 to 8. The recording of higher-dimensional states is limited only by the number of data points required and therefore the length of time needed to complete the measurements. We find all the measured states to have fidelities and linear entropies that satisfy the criteria required for a violation of the appropriate high-dimensional Bell inequality. Our results therefore precisely characterize the nature of the entanglement, thus establishing the suitability of such states for applications in quantum information science.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗