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At least 487 records · Page 27

Designing Phononic Crystals with Wide and Robust Band Gaps

Here, phononic crystals (PnCs) engineered to manipulate and control the propagation of mechanical waves have enabled the design of a range of novel devices, such as waveguides, frequency modulators, and acoustic cloaks, for which wide and robust phononic band gaps are highly preferable. While numerous PnCs have been designed in recent decades, to the best of our knowledge, PnCs that possess simultaneous wide and robust band gaps (to randomness and deformations) have not yet been reported. Here, we demonstrate that by combining the band-gap formation mechanisms of Bragg scattering and local resonances (the latter one is dominating), PnCs with wide and robust phononic band gaps can be established. The robustness of the phononic band gaps are then discussed from two aspects: robustness to geometric randomness (manufacture defects) and robustness to deformations (mechanical stimuli). Analytical formulations further predict the optimal design parameters, and an uncertainty analysis quantifies the randomness effect of each designing parameter. Moreover, we show that the deformation robustness originates from a local resonance-dominant mechanism together with the suppression of structural instability. Importantly, the proposed PnCs require only a small number of layers of elements (three unit cells) to obtain broad, robust, and strong attenuation bands, which offer great potential in designing flexible and deformable phononic devices.

36 MATERIALS SCIENCE↗

Superdiffusive heat conduction in semiconductor alloys. II. Truncated Lévy formalism for experimental analysis

Nearly all experimental observations of quasiballistic heat flow are interpreted using Fourier theory with modified thermal conductivity. Detailed Boltzmann transport equation (BTE) analysis, yet, reveals that the quasi-ballistic motion of thermal energy in semiconductor alloys is no longer Brownian but instead exhibits Lévy dynamics with fractal dimension α < 2 . In this work, we present a framework that enables full three-dimensional experimental analysis by retaining all essential physics of the quasiballistic BTE dynamics phenomenologically. A stochastic process with just two fitting parameters describes the transition from pure Lévy superdiffusion as short length and time scales to regular Fourier diffusion. The model provides accurate fits to time domain thermoreflectance raw experimental data over the full modulation frequency range without requiring any “effective” thermal parameters and without any a priori knowledge of microscopic phonon scattering mechanisms. Identified α values for InGaAs and SiGe match ab initio BTE predictions within a few percent. Our results provide experimental evidence of fractal Lévy heat conduction in semiconductor alloys. The formalism additionally indicates that the transient temperature inside the material differs significantly from Fourier theory and can lead to improved thermal characterization of nanoscale devices and material interfaces.

36 MATERIALS SCIENCE↗

Origin of the positive spin- 1 2 photoluminescence-detected magnetic resonance in π-conjugated materials and devices

The spin-1/2 single-modulation (SM) and double-modulation (DM) photoluminescence (PL) detected magnetic resonance (PLDMR) in poly(2-methoxy-5-(2'-ethyl)–hexoxy-1,4- phenylene vinylene) (MEH-PPV) films and poly(3-hexylthiophene) (P3HT) films is described, analyzed, and discussed. In particular, the models based on spin-dependent recombination of charge pairs (SDR) and triplet-polaron quenching (TPQ) are evaluated. By analyzing the dependence of the resonance amplitude on the microwave chopping (modulation) frequency using rate equations, it is demonstrated that the TPQ model can well explain the observed resonance behavior, while SDR model cannot reproduce the results of the observed DM-PLDMR. As a result, the observed spin-1/2 PLDMR is assigned to TPQ rather than SDR, even though the latter may also be present.

36 MATERIALS SCIENCE↗

Self-excited oscillation and synchronization of an on-fiber optomechanical cavity

Here, we study a fully on-fiber optomechanical cavity and characterize its performance as a sensor. The cavity is formed by patterning a suspended metallic mirror near the tip of an optical fiber and by introducing a static reflector inside the fiber. Optically induced self-excited oscillation (SEO) is observed above a threshold value of the injected laser power. The SEO phase can be synchronized by periodically modulating the optical power that is injected into the cavity. Noise properties of the system in the region of synchronization are explored. Furthermore, the spectrum is measured near different values of the modulation frequency, at which phase locking occurs. A universal behavior is revealed in the transition between the regions of phase locked and free running SEO.

42 ENGINEERING↗

Micromechanical origin of heat transfer to granular flow

Heat transfer across a granular flow is comprised of two resistances in series : near the wall and within the bulk particle bed, neither of which is well understood due to the lack of experimental probes to separate their respective contribution. Here, we use a frequency modulated photothermal technique to separately quantify the thermal resistances in the near-wall and the bulk bed regions of particles in flowing states. Compared to the stationary state, the flowing leads to a higher near-wall resistance and a lower thermal conductivity of bulk beds. As a result, coupled with discrete element method simulation, we show that the near-wall resistance can be explained by particle diffusion in granular flows.

14 SOLAR ENERGY↗

Narrowband Emission in Compton/Thomson Sources Operating in the High-Field Regime

We present a novel and quite general analysis of the interaction of a high-field chirped laser pulse and a relativistic electron, in which exquisite control of the spectral brilliance of the upshifted Thomson-scattered photon is shown to be possible. Normally, when Thomson scattering occurs at high field strengths, there is ponderomotive line broadening in the scattered radiation. This effect makes the bandwidth too large for some applications, and reduces the spectral brilliance. In this paper we show that such broadening can be corrected and eliminated by suitable frequency modulation of the incident laser pulse. Further, we suggest a practical realization of this compensation idea in terms of a chirped-beam driven FEL oscillator configuration, and show that significant compensation can occur, even with the imperfect matching to be expected in these conditions.

43 PARTICLE ACCELERATORS↗

Landau-Zener-Stückelberg-Majorana Interferometry of a Single Hole

We perform Landau-Zener-Stückelberg-Majorana (LZSM) spectroscopy on a system with strong spin-orbit interaction (SOI), realized as a single hole confined in a gated double quantum dot. Analogous to electron systems, at a magnetic field B = 0 and high modulation frequencies, we observe photon-assisted tunneling between dots, which smoothly evolves into the typical LZSM funnel-shaped interference pattern as the frequency is decreased. In contrast to electrons, the SOI enables an additional, efficient spin-flip interdot tunneling channel, introducing a distinct interference pattern at finite B . Magnetotransport spectra at low-frequency LZSM driving show the two channels to be equally coherent. High-frequency LZSM driving reveals complex photon-assisted tunneling pathways, both spin conserving and spin flip, which form closed loops at critical magnetic fields. Finally, in one such loop, an arbitrary hole spin state is inverted, opening the way toward its all-electrical manipulation.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Anisotropic thermal transport in bulk hexagonal boron nitride

Hexagonal boron nitride (h-BN) has received great interest in recent years as a wide band-gap analog of graphene-derived systems along with its potential in a wide range of applications, for example, as the dielectric layer for graphene devices. However, the thermal transport properties of h-BN, which can be critical for device reliability and functionality, are little studied both experimentally and theoretically. The primary challenge in the experimental measurements of the anisotropic thermal conductivity of h-BN is that typically the sample size of h-BN single crystals is too small for conventional measurement techniques, as state-of-the-art technologies synthesize h-BN single crystals with lateral sizes only up to 2.5 mm and thicknesses up to 200 μm. Recently developed time-domain thermoreflectance (TDTR) techniques are suitable to measure the anisotropic thermal conductivity of such small samples, as it only requires a small area of 50 × 50 μm 2 for the measurements. Accurate atomistic modeling of thermal transport in bulk h-BN is also challenging due to the highly anisotropic layered structure. Here we conduct an integrated experimental and theoretical study on the anisotropic thermal conductivity of bulk h-BN single crystals over the temperature range of 100–500 K using TDTR measurements with multiple modulation frequencies and a full-scale numerical calculation of the phonon Boltzmann transport equation starting from first principles. Our experimental and numerical results compare favorably for both the in-plane and the through-plane thermal conductivities. We observe unusual temperature dependence and phonon-isotope scattering in the through-plane thermal conductivity of h-BN and elucidate their origins. Here, this article not only provides an important benchmark of the anisotropic thermal conductivity of h-BN, but also develops fundamental insight into the nature of phonon transport in this highly anisotropic layered material.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Simulating noncontact atomic force microscopy images

A scanning probe with an atomically sharp tip is used in atomic force microscopy. As the probe is rastered over the specimen of interest, changes in its vibration mode can be ascribed to changes in the interatomic forces between the specimen and the tip. Various modes for implementing atomic force measures exist. One of the most successful modes is frequency-modulation noncontact atomic force microscopy. Here we address the role of replicating accurate forces on the probe tip to simulate images within this mode. In this work, we examine several approaches. One involves the use of classical force fields based on interatomic potentials, where the potentials are often fit to experiment. Other approaches center on the use of forces generated from quantum-based calculations. We consider the development of a “virtual tip” approximation wherein the probe tip senses electrostatic forces generated by the specimen. This approach treats the specimen quantum mechanically, while the tip is treated as a classical object. We also consider the use of an embedding approximation to avoid direct computations of the specimen in the presence of the tip. In this method, the tip and specimen are treated quantum mechanically. However, the electronic structure of the specimen is computed in the absence of the probe tip. The electronic density of the specimen is then fixed and the electronic structure of the tip is then computed in the presence of the fixed density. As a general approach, we outline new methods for the full computation of quantum forces between the tip and specimen. We note that quantum-based forces are particularly important as they directly contain the chemical nature of the forces present without the use of any adjustable parameters. We illustrate recent algorithmic developments to computing quantum forces that can produce accurate simulations of atomic force microscopy images for large and complex molecular species. We also suggest new pathways to overcome current challenges in this rapidly evolving field.

36 MATERIALS SCIENCE↗

Floquet engineering of polaritonic amplification in dispersive photonic time crystals

In this study, we investigate the dynamics of dispersive photonic time crystals (PTCs) and their potential applications for controlling light-matter interaction. Using the Lorentz-Drude as dispersive material model, we analyze the effects of periodic modulation of dispersion parameters through both theoretical and numerical analysis, revealing the emergence of hybrid bandgaps from the interaction of polaritonic branches with distinctive characteristics. Our study demonstrates that dispersive PTCs offer novel excitation channels and amplification possibilities, that require lower modulation frequencies compared to nondispersive systems thus alleviating experimental challenges for the realization of PTCs in the optical regime. These findings pave the way for advancements in polaritonic lasing and resonant Raman scattering.

Classical optics↗

A variable X-ray chopper system for phase-sensitive detection in synchrotron X-ray scanning tunneling microscopy

An ultra-high-vacuum compatible X-ray chopper system has been designed, constructed and integrated into the XTIP beamline at the Advanced Photon Source at Argonne National Laboratory. The XTIP beamline can operate at soft X-ray energies from 400 eV to 1900 eV while providing a focused beam down to about 10 µm × 10 µm into the synchrotron X-ray scanning tunneling microscopy (SX-STM) endstation instrument. The X-ray chopper is a critical component for separating topographic information from chemical information in SX-STM through phase-sensitive current detection. Depending on the experimental needs, the modulation frequency can be controlled from 100 Hz to 10 kHz. In addition, the chopper system is fully bakeable and can achieve a base pressure of 10 -10 mbar. Facilities for active water cooling have been designed, but passive cooling through copper braids has been shown to be sufficient at standard chopping frequencies. Using an Fe/Al 2 O 3 /CoAl(111) sample, the separation of the SX-STM current into a chemical component and a stable feedback signal is demonstrated.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

InSAR Time Series Analysis of L-Band Wide-Swath SAR Data Acquired by ALOS-2

We present that operating at L-band (24 cm wavelength) in wide-swath modes is one of the characteristics of the new and next generation satellite synthetic aperture radar (SAR) missions. After 3 years of operation, the Japan Aerospace Exploration Agency Advanced Land Observing Satellite-2 (ALOS-2) satellite has acquired a wealth of L-band wide-swath SAR data over many areas using its ScanSAR mode. We present interferometry SAR (InSAR) time series analysis results from ALOS-2 ScanSAR data. We analyze the possible error sources in the InSAR and correct them if possible. We present different time series analysis results including azimuth frequency modulation rate error, line of sight (LOS) ionospheric phase, azimuth shift caused by the ionosphere, and LOS displacement processed using both full-aperture and burst-by -burst workflows. The final InSAR LOS displacement time series result reveals both large-scale tectonic and small-scale anthropogenic deformation components. In conclusion, the results demonstrate the potential for measuring continental or even global-scale tectonic deformation and illustrate the promise of upcoming L-band wide-swath SAR missions, such as the NASA-ISRO SAR mission.

47 OTHER INSTRUMENTATION↗

Further developments of capillary absorption spectrometers using small hollow-waveguide fibers

Our objective is to enhance quantification of stable carbon and oxygen isotope ratios to better than 1‰ relative isotope precision for sample sizes < 1 pico-mole. A newer variant Capillary Absorption Spectrometer (CAS) is described using a proprietary linear-taper hollow waveguide in conjunction with wavelength and frequency modulation techniques of tunable laser absorption spectrometry. Previous work used circular capillaries with uniform 1 mm ID to measure 13C/12C ratios with ≥ 20 pico-mole samples to ≤ 10 ppm (1‰ precision against standards) [1]. While performing fairly well, it generated residual modal noise due to multipath propagation in the hollow-waveguides (HWGs). This system has been utilized with laser ablation-catalytic combustion techniques to analyze small resolution (~ 25 μm spot diameter) laser ablation events on solids. Using smaller ID capillary waveguides could improve detection limits and spatial resolutions. Reducing an IR compatible hollow waveguide’s inner diameter (ID) to < 300 μm, reduces modal noise significantly for mid-IR operation, but feedback noise with high gain semiconductor lasers can become problematic. A proprietary linear-taper small waveguide (mean ID = 0.35 mm, L = 1 m) was tested to understand whether modal noise and optical feedback effects could be simultaneously reduced. We see better mode filtering and, significant reductions of feedback noise under favorable coupling of a multi-spatial mode QC laser to the smaller ID of the linear-tapered HWG. We demonstrate that better modal coupling operation is consistent with Liouville’s theorem, where greater suppression of feedback from spurious scatter within the HWG occurs by injecting the laser into the smaller ID port. Our progress on developing lighter weight, potentially fieldable alternatives to Isotope Ratio Mass Spectrometers (IRMS) with a small volume (≤ 0.1 cm3) CAS system will be discussed and compared to other competitive systems.

Kelly, James F.↗

Effect of the photon lifetime on the characteristics of 850-nm vertical-cavity surface-emitting lasers with fully doped distributed Bragg reflectors and an oxide current aperture

The effect of the photon lifetime in an optical microcavity on the characteristics of 850-nm vertical-cavity surface-emitting lasers (VCSELs) with fully doped distributed Bragg reflectors (DBRs) and an oxide current aperture is studied. The photon lifetime in the microcavity is controlled by varying the upper DBR reflectance. It is found that the speed of VCSELs with a current-aperture diameter of 10 μm is mainly limited by the self-heating effect, despite an increase in the relaxation-oscillation damping coefficient with increasing photon lifetime in the microcavity. At the same time, the higher level of internal optical loss in lasers with a current-aperture diameter of 1.5 μm leads to dominance of the effect of relaxation-oscillation damping independently of the radiation output loss. In the case of devices with a current-aperture diameter of 5.5 μm, both mechanisms limiting the speed operate, which allow an increase in the VCSEL effective modulation frequency from 21 to 24 GHz as the photon lifetime decreases from 3.7 to 0.8 ps.

36 MATERIALS SCIENCE↗

Vertical-Cavity Surface-Emitting 1.55-μm Lasers Fabricated by Fusion

The results of studies on fabrication of vertical-cavity surface-emitting 1.55-μm lasers by fusing AlGaAs/GaAs distributed-Bragg-reflector wafers and an active region based on thin In{sub 0.74}Ga{sub 0.26} As quantum wells grown by molecular-beam epitaxy are presented. Lasers with a current aperture diameter of 8 μm exhibit continuous lasing with a threshold current below 1.5 mA, an output optical power of 6 mW, and an efficiency of approximately 22%. Single-mode lasing with a side-mode suppression ratio of 40–45 dB is observed in the entire operating current range. The effective modulation frequency of these lasers is as high as 9 GHz and is limited by the low parasitic cutoff frequency and self-heating.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Evaluating the coherence and time-domain profile of quantum cascade laser frequency combs

Recently, much attention has been focused on the generation of optical frequency combs from quantum cascade lasers. We discuss how fast detectors can be used to demonstrate the mutual coherence of such combs, and present an inequality that can be used to quantitatively evaluate their performance. We discuss several technical issues related to shifted wave interference Fourier Transform spectroscopy (SWIFTS), and show how such measurements can be used to elucidate the time-domain properties of such combs, showing that they can possess signatures of both frequency-modulation and amplitude-modulation.

42 ENGINEERING↗

Broadband rapid-scanning phase-modulated Fourier transform electronic spectroscopy

We present a phase-modulated approach for ultrabroadband Fourier transform electronic spectroscopy. To overcome the bandwidth limitations and spatial chirp introduced by acousto-optic modulators (AOMs), pulses from a 1 µm laser are modulated using AOMs prior to continuum generation. This phase modulation is transferred to the continuum generated in a yttrium aluminum garnet crystal. Separately generated phase-modulated continua in two arms of a Mach-Zehnder interferometer interfere with the difference of their modulation frequencies, enabling physical under-sampling of the signal and the suppression of low-frequency noise. By interferometrically tracking the relative time delay of the continua, we perform continuous, rapid-scanning Fourier transform electronic spectroscopy with a high signal-to-noise ratio and spectral resolution. As proof of principle, we measure the linear absorption and fluorescence excitation spectra of a laser dye and various biological samples.

Javed, Ariba↗

Real-time single-element-detection structured illumination optical metrology for laser powder bed fusion

Laser powder bed fusion (LPBF) is a type of metal additive manufacturing which could benefit from improved process monitoring to improve quality control. We demonstrate, for the first time to our knowledge, the coaxial monitoring of melt track formation in steel powder with spatial frequency modulation imaging (SPIFI), an enhanced-resolution imaging technique which uses a photodiode to record one-dimensional images. Using a custom live-display software and a high-speed SPIFI geometry, we offset the SPIFI field of view from the fusing beam to monitor different regions of the LPBF melt pool and surrounding area. This demonstrates the potential of SPIFI to monitor spatial features within the melt pool in real-time with increased data efficiency.

Hunter, Scott (ORCID:0009000886150312)↗