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At least 487 records · Page 27

Laser Ablation Plasmas and Spectroscopy for Nuclear Applications

The development of measurement methodologies to detect and monitor nuclear-relevant materials remains a consistent and significant interest across the nuclear energy, nonproliferation, safeguards, and forensics communities. Optical spectroscopy of laser-produced plasmas is becoming an increasingly popular diagnostic technique to measure radiological and nuclear materials in the field without sample preparation, where current capabilities encompass the standoff, isotopically resolved and phase-identifiable (e.g., UO and UO[Formula: see text]) detection of elements across the periodic table. These methods rely on the process of laser ablation (LA), where a high-powered pulsed laser is used to excite a sample (solid, liquid, or gas) into a luminous microplasma that rapidly undergoes de-excitation through the emission of electromagnetic radiation, which serves as a spectroscopic fingerprint for that sample. This review focuses on LA plasmas and spectroscopy for nuclear applications, covering topics from the wide-area environmental sampling and atmospheric sensing of radionuclides to recent implementations of multivariate machine learning methods that work to enable the real-time analysis of spectrochemical measurements with an emphasis on fundamental research and development activities over the past two decades. Background on the physical breakdown mechanisms and interactions of matter with nanosecond and ultrafast laser pulses that lead to the generation of laser-produced microplasmas is provided, followed by a description of the transient spatiotemporal plasma conditions that control the behavior of spectroscopic signatures recorded by analytical methods in atomic and molecular spectroscopy. High-temperature chemical and thermodynamic processes governing reactive LA plasmas are also examined alongside investigations into the condensation pathways of the plasma, which are believed to serve as chemical surrogates for fallout particles formed in nuclear fireballs. Laser-supported absorption waves and laser-induced shockwaves that accompany LA plasmas are also discussed, which could provide insights into atmospheric ionization phenomena from strong shocks following nuclear detonations. Furthermore, the standoff detection of trace radioactive aerosols and fission gases is reviewed in the context of monitoring atmospheric radiation plumes and off-gas streams of molten salt reactors. Finally, concluding remarks will present future outlooks on the role of LA plasma spectroscopy in the nuclear community.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

On the role of a supernova in the formation of the solar system

Four possible scenarios relating the proto-solar cloud to the 'last-minute' supernova presumed responsible for the isotopic anomalies in Allende and other meteorites are considered. The probability that a chance supernova occurred close enough to an already-collapsing proto-solar cloud to inject sufficient matter is extremely small, even if the sun formed in a region of enhanced supernova activity such as Orion OB1. The ambient level of Al-26 inside a molecular cloud in Orion is also apparently too low to account for the meteorite data, unless the supernova ejecta accumulates at the edges of the cloud and star formation occurs there preferentially. Two modes of supernova-induced star formation are discussed. In one, the supernova shock collapses a preexisting cloud; in the other, stars form within the snowplow shell of the supernova. Canis Major R1 and Monoceros R1 are possible present-day examples of such star formation regions.

Herbst, W.↗

Space commerce in a global economy: Comparison of US and Australian approaches

The United States and Australia are among the 20 or more nations of the world having industries currently engaging in some form of space commerce. As a matter of national policy, the United States has encouraged private investment and involvement in space activities since 1984, when the Congress declared it in the best interest of the Nation that NASA '...seek and encourage to the maximum extent possible, the fullest commercial use of space.' Australia's space policy, announced in 1986, has the objective of encouraging greater involvement by industry in space research and development, and the development of commercial space activities. This paper discusses the underlying policies, current status, and prospects for the future of commercial space business activities in the two countries.

Stone, Barbara A.↗

The Gamma-ray Large Area Space Telescope and Gamma-Ray Bursts

The Gamma-ray Large Area Telescope (GLAST) is a satellite-based observatory to study the high energy gamma-ray sky. The main instrument on GLAST, the Large Area Telescope (LAT) is a pair-conversion telescope that will survey the sky from 20 MeV to greater than 300 GeV. With the GLAST launch in 2007, the LAT will open a new and important window on a wide variety of high energy phenomena, including supermassive black holes and active galactic nuclei, gamma-ray bursts, supernova remnants and cosmic ray acceleration and dark matter. A second instrument, the GLAST Burst Monitor (GBM), greatly enhances GLAST s capability to study GRB by providing important spectral and timing information in the 10 keV to 30 MeV range. We describe how the instruments, spacecraft and ground system work together to provide observations of gamma-ray bursts from 8 keV - 300 GeV and to provide rapid notification of bursts to the wider gamma-ray burst community.

McEnery, Julie↗

Gamma-400 Science Objectives Built on the Current HE Gamma-Ray and CR Results

The main scientific interest of the Russian Gamma-400 team: Observe gamma-rays above approximately 50 GeV with excellent energy and angular resolution with the goals of: (1) Studying the fine spectral structure of the isotropic high-energy gamma-radiation, (2) Attempting to identify the many still-unidentified Fermi-LAT gamma-ray sources. Gamma-400 will likely be the only space-based gamma-ray observatory operating at the end of the decade. In our proposed Gamma-400-LE version, it will substantially improve upon the capabilities of Fermi LAT and AGILE in both LE and HE energy range. Measuring gamma-rays from approx 20 MeV to approx 1 TeV for at least 7 years, Gamma-400-LE will address the topics of dark matter, cosmic ray origin and propagation, neutron stars, flaring pulsars, black holes, AGNs, GRBs, and actively participate in multiwavelength campaigns.

Moiseev, Alexander↗

MeV Emission from Pulsar Wind Nebulae: Understanding Extreme Particle Acceleration in Highly Relativistic Outflows

The Earth is constantly bombarded from outer space by energetic particles. Where and how these "cosmic rays" are produced is poorly understood, with various particle types and energies likely originating from different sources. Particularly mysterious is the source of high-energy e+/- produced in our Galaxy, especially those responsible for both the high fraction of e+ in the GeV cosmic ray lepton spectrum and the e+/- and observed excess of microwaves and gamma-rays detected towards the Galactic center and bulge. While these particles could be evidence for exotic forms of dark matter, they might also be produced by "normal" astrophysical sources such as pulsars the strongly magnetized, rapidly rotating neutron stars whose rotational energy powers an ultra-relativistic outflow (commonly referred to as a "pulsar wind") whose interaction with the surrounding medium creates a pulsar wind nebula .While the detection of TeV emission from numerous PWNe strongly suggest they contain e+/- with PeV or higher energies, how and to what energies these particles are produced is unknown, let alone their dependence on the properties of the pulsar, pulsar wind, and surrounding medium. A major reason for this uncertainty is the lack of information concerning their MeV properties, since the synchrotron emission from the highest energy e+/- peaks in this waveband. Only by combining the MeV spectrum of PWNe measured by proposed missions with that obtained at lower (primarily radio and X-ray) and higher (TeV) photon energies by current and hopefully future facilities is it possible to measure the full spectrum of e+/- in these sources. The resultant insights into the underlying acceleration mechanism would significantly impact many areas of astrophysics from indirect searches for dark matter to the origin of cosmic rays to the physics of relativistic outflows observed from active galactic nuclei, gamma-ray bursts, and some gravitational wave events.

Gelfand, Joseph D.↗

Aerosol Physics for the Lunar Environment: Equations for Lunar Dust Control and Mitigation Technologies

Sticky and jagged dust was ubiquitous during the Apollo missions, causing soiling and abrasion problems with seals, coatings and equipment, in addition to eye irritation and breathing discomfort in the cabin. The Artemis Program of NASA aims to place astronauts on the lunar surface by 2024 and establish a sustainable presence in the following decade. Returning to the Moon requires controlling and mitigating the dust which will be inevitably brought inside the cabins. The state-of-the-science for effective collection of aerosols is based on dynamics of airborne particulate matter under terrestrial conditions. However, the governing physics does not apply to extra-vehicular activity in the hard-vacuum lunar condition. For example, the substantial difference in gravity will dictate particle transport both outside and inside the cabin. In this study, we revisited the aerosol physical phenomena that are assumed in the design of Earth-based aerosol instruments and extend the applicability to different scenarios in lunar missions. As shown, long-term lunar habitats, transfer vehicles to lunar orbital platforms, and low pressure cabin atmospheres have different aerosol dynamics. In all cases, the impact of dust control strategies using gravitational, electrical, and thermal techniques for various mitigation and monitoring hardware is explored. The guidelines provided through this study will show how terrestrial aerosol equipment can translate to lunar dust applications.

Nima Afshar-Mohajer↗

Spacecraft Line-Of-Sight Jitter Mitigation and Management Lessons Learned and Engineering Best Practices

Predicting, managing, controlling, and testing spacecraft line-of-sight (LoS) jitter caused by micro-vibrations due to onboard internal disturbance sources is a formidable multidisciplinary engineering task. It is especially challenging for those missions hosting high-performance, vibration-sensitive optical sensor payloads with stringent pointing stability requirements. Both NASA and ESA are planning technically aggressive spaceflight missions that include ultra-high-performance optical payloads with delicate, highly vibration-sensitive scientific and observational instruments. The GN&C community of practice will need to leverage and build upon their collective experiences and lessons learned to better address future micro-vibration challenges. To identify lessons learned and best engineering practices the NASA Engineering & Safety Center (NESC) sponsored a two-day Spacecraft LoS Jitter Workshop in late 2019. The workshop’s goal was to provide a multidisciplinary forum to elicit deeper understanding of the issues related to solving the spacecraft LoS jitter/micro-vibration problem. A primary objective was to identify and share best practices, rules of thumb, and options for jitter-related activities. Representatives from NASA, JPL, ESA, along with NASA’s industrial partners, independent consultant subject matter experts, and members of academia participated in the workshop. This paper will describe the motivation for the NASA Spacecraft LoS Jitter Workshop and summarize the identified findings, observations, and recommendations.

Lessons Learned;↗

Deep Search for Decaying Dark Matter with XMM-Newton Blank-Sky Observations

Sterile neutrinos with masses in the keV range are well-motivated extensions to the Standard Model that could explain the observed neutrino masses while also making up the dark matter (DM) of the universe. If sterile neutrinos are DM then they may slowly decay into active neutrinos and photons, giving rise to the possibility of their detection through narrow spectral features in astrophysical x-ray data sets. Here, we perform the most sensitive search to date for this and other decaying DM scenarios across the mass range from 5 to 16 keV using archival XMM-Newton data. We reduce 547 Ms of data from both the MOS and PN instruments using observations taken across the full sky and then use this data to search for evidence of DM decay in the ambient halo of the Milky Way. We determine the instrumental and astrophysical baselines with data taken far away from the Galactic Center, and use Gaussian process modeling to capture additional continuum background contributions. No evidence is found for unassociated x-ray lines, leading us to produce the strongest constraints to date on decaying DM in this mass range.

79 ASTRONOMY AND ASTROPHYSICS↗

R&D for LAr + Xe + photosensitive dopants

LArTPCs are the technology of choice for current and future neutrino experiments, including those expected to make eagerly awaited measurements of accelerator neutrino oscillations in the coming decade. This technology provides a large active volume and sensitivity to GeV signals like accelerator neutrinos all the way down to 10s of MeV, covering part of the supernova neutrino spectrum.Expanding the reach of LArTPCs to below the 10 MeV range would substantially enhance the flagship analyses of experiments like DUNE, while potentially enabling the physics of solar neutrinos, dark matter searches, and neutrinoless double beta decay searches.We outline the R&D pathway for photosensitive dopants, whose introduction into the LAr active medium, has the potential to substantially increase ionization yields of LAr detectors and enable the detection of low energy signals in large LArTPCs. This R&D program will demonstrate the feasibility and impacts of introducing doped LAr into current and future neutrino detectors at the kTon scale including the Xenon + photosensitive doping strategy.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Personalized whole-brain neural mass models reveal combined Aβ and tau hyperexcitable influences in Alzheimer's disease.

Neuronal dysfunction and cognitive deterioration in Alzheimer's disease (AD) are likely caused by multiple pathophysiological factors. However, mechanistic evidence in humans remains scarce, requiring improved non-invasive techniques and integrative models. We introduce personalized AD computational models built on whole-brain Wilson-Cowan oscillators and incorporating resting-state functional MRI, amyloid-β (Aβ) and tau-PET from 132 individuals in the AD spectrum to evaluate the direct impact of toxic protein deposition on neuronal activity. This subject-specific approach uncovers key patho-mechanistic interactions, including synergistic Aβ and tau effects on cognitive impairment and neuronal excitability increases with disease progression. The data-derived neuronal excitability values strongly predict clinically relevant AD plasma biomarker concentrations (p-tau217, p-tau231, p-tau181, GFAP) and grey matter atrophy obtained through voxel-based morphometry. Furthermore, reconstructed EEG proxy quantities show the hallmark AD electrophysiological alterations (theta band activity enhancement and alpha reductions) which occur with Aβ-positivity and after limbic tau involvement. Microglial activation influences on neuronal activity are less definitive, potentially due to neuroimaging limitations in mapping neuroprotective vs detrimental activation phenotypes. Mechanistic brain activity models can further clarify intricate neurodegenerative processes and accelerate preventive/treatment interventions.

60 APPLIED LIFE SCIENCES↗

Design and construction of a new detector to measure ultra-low radioactive-isotope contamination of argon

Large liquid argon detectors offer one of the best avenues for the detection of galactic weakly interacting massive particles (WIMPs) via their scattering on atomic nuclei. The liquid argon target allows exquisite discrimination between nuclear and electron recoil signals via pulse-shape discrimination of the scintillation signals. Atmospheric argon (AAr), however, has a naturally occurring radioactive isotope, 39Ar, a ß emitter of cosmogenic origin. For large detectors, the atmospheric 39Ar activity poses pile-up concerns. The use of argon extracted from underground wells, deprived of 39Ar, is key to the physics potential of these experiments. The DarkSide-20k dark matter search experiment will operate a dual-phase time projection chamber with 50 tonnes of radio-pure underground argon (UAr), that was shown to be depleted of 39Ar with respect to AAr by a factor larger than 1400. Assessing the 39Ar content of the UAr during extraction is crucial for the success of DarkSide-20k, as well as for future experiments of the Global Argon Dark Matter Collaboration (GADMC). This will be carried out by the DArT in ArDM experiment, a small chamber made with extremely radio-pure materials that will be placed at the centre of the ArDM detector, in the Canfranc Underground Laboratory (LSC) in Spain. The ArDM LAr volume acts as an active veto for background radioactivity, mostly ?-rays from the ArDM detector materials and the surrounding rock. This article describes the DArT in ArDM project, including the chamber design and construction, and reviews the background required to achieve the expected performance of the detector.

Noble liquid detectors, Dark Matter detectors, Cry↗

MeV Scale Physics in MicroBooNE

This thesis presents the reconstruction and measurement of low-energy electromagnetic activity with beam neutrino interactions within the MicroBooNE Liquid Argon Time Projection Chamber (LArTPC). LArTPCs have proven to be excellent detectors to measure neutrino interaction cross sections and are being used to perform precision measurements of neutrino oscillation parameters. The work presented in this thesis has demonstrated unprecedentedly low, sub-MeV energy thresholds that have increased sensitivity of LArTPCs to detect neutrino interactions from core collapse supernovae and Muon Decay at Rest (µDAR). In addition, such low thresholds have also increased measurement sensitivity for interactions from Beyond the Standard Model (BSM) candidates such as millicharged particles and nuclear and electron recoils from dark matter candidate particles. On the reconstruction side, this work has established an energy resolution of 6.3% for electromagnetic activity i the 0-5 MeV energy range within the MicroBooNE LArTPC. Additionally this work presents the quantitative analysis of the low-energy activity emanating from G-10 support ribs in MicroBooNE and discusses how such activity could be a problematic source of background for low-energy physics analyses in future neutrino detectors such as the Deep Underground Neutrino Experiment (DUNE).

Bhat, Avinay↗

BENCAL Cruise Report

This report documents the scientific activities on board the South African Fisheries Research Ship (FRS) Africana during an ocean color calibration and validation cruise in the Benguela upwelling ecosystem (BEN-CAL), 4-17 October 2002. The cruise, denoted Afncana voyage 170, was staged in the southern Benguela between Cape Town and the Orange River within the region 14-18.5 deg E,29-34 deg S, with 15 scientists participat- ing from seven different international organizations. Uniquely in October 2002, four high-precision ocean color sensors were operational, and these included the Moderate Resolution Imaging Spectroradiometer (MODIS) instruments on the Aqua and Terra spacecraft, the Medium Resolution Imaging Spectrometer (MERIS), and the Sea-viewing Wide Field-of-view Sensor (SeaWiFS). SeaWiFS imagery was transmitted daily to the ship to assist in choosing the vessel's course and selecting stations for bio-optical deployments. There were four primary objectives of the cruise. The first was to conduct bio-optical measurements with above- and in-water optical instruments to vicariously calibrate the satellite sensors. The second was to interrelate diverse measurements of the apparent optical properties (AOPs) at satellite sensor wavelengths with inherent optical properties (IOPs) and bio-optically active constituents of seawater such as particles, pigments, and dissolved compounds. The third was to determine the interrelationships between optical properties, phytoplankton pigment composition, photosynthetic rates, and primary production, while the fourth objective was to collect samples for a second pigment round-robin intercalibration experiment. Weather conditions were generally very favorable, and a range of hyperspectral and fixed wavelength AOP instruments were deployed during daylight hours. Various IOP instruments were used to determine the absorption, attenuation, scattering, and backscattering properties of particulate matter and dissolved substances, while a Fast Repetition Rate Fluorometer (FRRF) was deployed to acquire data on phytoplankton photosynthetic activity. Hydrographic profiling was conducted routinely during the cruise, and seawater samples were collected for measurements of salinity, oxygen, inorganic nutrients, pigments, particulate organic carbon, suspended particulate material, and primary production. Location of stations and times of optical deployments were selected to coincide with satellite overpasses whenever possible, and to cover a large range in trophic conditions.

Hooker, Stanford B.↗

Uranium sorption to organic matter and long-term accumulation in a pristine alpine wetland

Understanding the controls on uranium (U) mobility in the environment is key to improve the management of sites contaminated by U mining activities. Previous research has shown that natural or engineered wetlands are particularly able to scavenge high amounts of U(VI) and U(IV) under noncrystalline forms. However, questions remain on the respective roles of sorption and reduction processes in the removal of U from running waters in wetlands, as well as on the long-term stability of U storage. Here, we performed a series of geochemical, isotopic ($δ$ 238 U, ( 234 U/ 238 U)), microscopic (SEM-EDXS, EPMA) and spectroscopic (µ-XRF, µ-XAS, XANES and EXAFS at the U L 3 and M 4 -edges and Fe K-edge) investigations to determine the modes of U accumulation and assess U mobility in a natural exceptionally U-enriched (up to 5000 µg/g) wetland on the shore of Lake Nègre (Mediterranean Alps, France). Uranium (VI) was largely dominant in the two studied soil cores, except a few samples containing as much as ~50 % U(IV). At the particle scale, U is associated to a variety of organic constituents of the soil matrix with a homogenous oxidation state. Bulk EXAFS spectroscopy at the U L 3 -edge shows that U is mostly mononuclear, with dominant monodentate binding to organic moieties (C neighbors at ~3.45 Å). An additional minor fraction of U under polymeric forms is inferred from wavelet (CCWT) analysis of the EXAFS data. These observations are reinforced by 1 M bicarbonate extractions that result in the dissolution of 82–96 % of total U, including putative polymeric species. At the wetland scale, similar or slightly fractionated isotopic ratios ($δ$ 238 U) between the wetland-feeding creek waters and the wetland soils are observed, supporting the idea that U(VI) sorption on organic matter is the primary U scavenging mechanism. Furthermore, it indicates that partial U(VI) reduction to U(IV) occurs as a second step, after sorption. Analysis of U decay chain disequilibria in the cores as a function of depth suggests that U accumulation in this wetland has lasted for several thousand years. In conclusion, we propose that the wetland acts as an active reactor where U has been massively accumulating for ~14500 years, especially as U(VI) forms associated to organic matter and is further partly exported to the lake through soil erosion.

63 RADIATION, THERMAL, AND OTHER ENVIRON. POLLUTAN↗

Disk-driven hydromagnetic winds as a key ingredient of active galactic nuclei unification schemes

Centrifugally driven winds from the surfaces of magnetized accretion disks have been recognized as an attractive mechanism of removing the angular momentum of the accreted matter and of producing the bipolar outflows and jets that are often associated with compact astronomical objects. As previously suggested in the context of young stellar objects, such winds have unique observational manifestations stemming from their highly stratified density and velocity structure and from their exposure to the strong continuum radiation field of the compact object. We have applied this scenario to active galactic nuclei (AGNs) and investigated the properties of hydromagnetic outflows that originate within approximately 10(M(sub 8)) pc of the central 10(exp 8)(M(sub 8)) solar mass black hole. On the basis of our results, we propose that hydromagnetic disk-driven winds may underlie the classification of broad-line and narrow-line AGNs (e.g., the Seyfert 1/Seyfert 2 dichotomy) as well as the apparent dearth of luminous Seyfert 2 galaxies. More generally, we demonstrate that such winds could strongly influence the spectral characteristics of Seyfert galaxies, QSOs, and BL Lac objects (BLOs). In our picture, the torus is identified with the outer regions of the wind where dust uplifted from the disk surfaces by gas-grain collisions is embedded in the outflow. Using an efficient radiative transfer code, we show that the infrared emission of Seyfert galaxies and QSOs can be attributed to the reprocessing of the UV/soft X-ray AGN continuum by the dust in the wind and the disk. We demonstrate that the radiation pressure force flattens the dust distribution in objects with comparatively high (but possibly sub-Eddington) bolometric luminosities, and we propose this as one likely reason for the apparent paucity of narrow-line objects among certain high-luminosity AGNs. Using the XSTAR photoionization code, we show that the inner regions of the wind could naturally account for the warm (greater than or approximately equal to 10(exp 5) K) and hot (greater than or approximately equal to 10(exp 6) K) gas components that have been inferred to exist on scales less than or approximately equal to 10(exp 2) pc in several Seyfert galaxies. We suggest that the partially ionized gas in the inner regions of the wind, rather than the dusty, neutral outflow that originates further out in the disk, could account for the bulk of the X-ray absorption in Seyferts observed at relatively small angles to their symmetry axes. Finally, we discuss the application of this model to the interpretation of the approximately 0.6 keV X-ray absorption feature reported in several BLOs.

Konigl, Arieh↗

The Sun to the Earth - and Beyond: A Decadal Research Strategy in Solar and Space Physics

The sun is the source of energy for life on earth and is the strongest modulator of the human physical environment. In fact, the Sun's influence extends throughout the solar system, both through photons, which provide heat, light, and ionization, and through the continuous outflow of a magnetized, supersonic ionized gas known as the solar wind. While the accomplishments of the past decade have answered important questions about the physics of the Sun, the interplanetary medium, and the space environments of Earth and other solar system bodies, they have also highlighted other questions, some of which are long-standing and fundamental. The Sun to the Earth--and Beyond organizes these questions in terms of five challenges that are expected to be the focus of scientific investigations in solar and space physics during the coming decade and beyond. While the accomplishments of the past decades have answered important questions about the physics of the Sun, the interplanetary medium, and the space environments of Earth and other solar system bodies, they have also highlighted other questions, some of which are long-standing and fundamental. This report organizes these questions in terms of five challenges that are expected to be the focus of scientific investigations in solar and space physics during the coming decade and beyond: Challenge 1: Understanding the structure and dynamics of the Sun's interior, the generation of solar magnetic fields, the origin of the solar cycle, the causes of solar activity, and the structure and dynamics of the corona. Challenge 2: Understanding heliospheric structure, the distribution of magnetic fields and matter throughout the solar system, and the interaction of the solar atmosphere with the local interstellar medium. Challenge 3: Understanding the space environments of Earth and other solar system bodies and their dynamical response to external and internal influences. Challenge 4: Understanding the basic physical principles manifest in processes observed in solar and space plasmas. Challenge 5: Developing a near-real-time predictive capability for understanding and quantifying the impact on human activities of dynamical processes at the Sun, in the interplanetary medium, and in Earth's magnetosphere and ionosphere. This report summarizes the state of knowledge about the total heliospheric system, poses key scientific questions for further research, and presents an integrated research strategy, with prioritized initiatives, for the next decade. The recommended strategy embraces both basic research programs and targeted basic research activities that will enhance knowledge and prediction of space weather effects on Earth. The report emphasizes the importance of understanding the Sun, the heliosphere, and planetary magnetospheres and ionospheres as astrophysical objects and as laboratories for the investigation of fundamental plasma physics phenomena.

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