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At least 469 records · Page 26
All sourcesNASA NTRSDOE OSTI
NASA NTRS1984

Latitudinal and altitudinal variation of size distribution of stratospheric aerosols inferred from SAGE aerosol extinction coefficient measurements at two wavelengths

A method of retrieving aerosol size distribution from the measured extinction of solar radiation at wavelengths of 0.45 microns and 1.0 microns has recently been proposed. This method is utilized to obtain latitudinal and altitudinal variations of size distributions of stratospheric aerosols from the Stratospheric Aerosol and Gas Experiment data for March 1979. Small particles are found in the lower stratosphere of the tropical region, and large particles are found at higher altitudes and latitudes in both hemispheres. Results of this study are consistent with the suggestion that the upper troposphere in tropical regions is a source of condensation nuclei in the stratosphere, and they become mature as they move to higher altitudes and latitude.

Yue, G. K.↗
NASA NTRS1984

Implications of the stratospheric water vapor distribution as determined from the Nimbus 7 LIMS experiment

The LIMS experiment on Nimbus 7 has provided new results on the stratospheric water vapor distribution. The data show (1) a latitudinal gradient with mixing ratios that increase by a factor of 2 from equator to + or - 60 degrees at 50 mb, (2) most of the time there is a fairly uniform mixing ratio of 5 ppmv at high latitudes, but more variation exists during winter, (3) a well-developed hygropause at low to midlatitudes of the lower stratosphere, (4) a source region of water vapor in the upper stratospehere to lower mesosphere that is consistent with methane oxidation chemistry, at least within the uncertainties of the data, (5) an apparent zonal mean H2O distribution that is consistent with the circulation proposed by Brewer in 1949, and (6) a zonal mean distribution in the lower stratosphere that is consistent with the idea of quasi-isentropic transport by eddies in the meridional direction. Limits to the use of the data in the refinement of our understanding of the stratospheric water vapor budget are noted.

Remsberg, E. E.↗
NASA NTRS1985

Behavior of zonal mean aerosol extinction ratio and its relationship with zonal mean temperature during the winter 1978-1979 stratospheric warming

The behavior of the zonal mean aerosol extinction ratio in the lower stratosphere near 75 deg N and its relationship with the zonal mean temperature during the January-February 1979 stratospheric sudden warming have been investigated based on the satellite sensor SAM II (Stratospheric Aerosol Measurement) and auxiliary meteorological measurements. The results indicate that distinct changes in the zonal mean aerosol extinction ratio occurred during this stratospheric sudden warming. It is also found that horizontal eddy transport due to planetary waves may have played a significant role in determining the distribution of the zonal mean aerosol extinction ratio.

Wang, P.-H.↗
NASA NTRS1985

Accurate stratospheric particle size distributions from a flat plate collection surface

Flat plate particle collections have revealed the presence of a remarkable variety of both terrestrial and extraterrestrial material in the stratosphere. It is found that the ratio of terrestrial to extraterrestrial material and the nature of the material collected may vary significantly over short time scales. These fluctuations may be related to massive injections of volcanic ash, emissions from solid fuel rockets, or variations in the micrometeoroid flux. The variations in particle number density can be of great importance to the earth's atmospheric radiation balance, and, therefore, its climate. With the objective to assess the number density of solid particles in the stratosphere, an examination has been conducted of all particles exceeding 1 micron in average diameter for a representative suite of particles obtained from a single flat plate collection surface. Attention is given to solid particle size distributions in the stratosphere, and the origin of important stratospheric particle types.

Zolensky, M. E.↗
NASA NTRS1985

Tentative identification of the 780/cm nu-4 band Q branch of chlorine nitrate in high-resolution solar absorption spectra of the stratosphere

According to models of the photochemistry of the stratosphere, chlorine nitrate (ClONO2) is an important temporary reservoir of stratospheric chlorine. At night, ClO is believed to combine in a three-body reaction with NO2 to form chlorine nitrate. During daylight, chlorine nitrate is destroyed by photolysis to form free chlorine and NO3. Infrared spectroscopy has the potential to provide a technique for conducting important quantitative measurements of stratospheric chlorine nitrate. The present paper reports a detailed study of spectra in the 780/cm region. This study has led to the tentative identification of the nu-4 band Q branch of ClONO2 as a significant contributor to the observed stratospheric absorption near 780.21 per cm.

Rinsland, C. P.↗
NASA NTRS1985

Trends in upper stratospheric temperatures as observed by rocketsondes (1965-1983)

Recent interest in possible anthropogenically induced changes in stratospheric ozone has led to a number of modeling studies. These studies indicate that stratospheric temperature changes would be related to stratospheric ozone changes. Therefore, this study was motivated by a concern to find out whether or not any significant trend in upper stratospheric temperatures could be ascertained from available observational data. June monthly mean values for 40 to 45 km layer were calculated for all Western Hemisphere rocketsonde stations for which data was available. Mean temperatures for each June were then used to calculate linear least squares regression coefficients with latitude of the stations as the independent variable. The resulting coefficients were used to calculate area-weighted mean temperatures for 25 deg N to 55 deg N. A two-to-three degree temperature drop in the early 1970s is indicated. It was noted, however, that this temperature decline coincides with a change in the principal observing system from the Arcasconde system to the Datasonde system. In order to study this temperature decrease more closely, similar mean temperatures were calculated for the 25 to 30 km layer using both rocketsondes and support radiosondes.

Johnson, K. W.↗
NASA NTRS1985

Discrimination of a major stratospheric warming event in February-March 1984 from earlier minor warmings

As part of its responsibility for stratospheric monitoring, the Climate Analysis Center derives time trends of various dynamic parameters from NMC stratospheric analyses. Selected figures from this stratospheric monitoring data base are published in Climate Diagnostics Bulletin in March and October, after each hemispheric winter. During the Northern Hemisphere winter of December 1983-February 1984 several warming events may be seen in the plot of 60 deg. N zonal mean temperatures for 10 mb. Minor warmings may be noted in early December, late December, mid January and early February. A major warming with the 60 deg. N zonal mean temperatures reaching -40C is observed in late February, associated with a circulation reversal. In all of the minor warming episodes, there is a polarward movement of the Aleutian anticyclone; however, at 10 mb the North Pole remains in the cyclonic circulation of the stratospheric vortex which is not displaced far from its usual position. In the case of the later February major warming, the 10 mb circulation pattern over the North Pole is anticyclonic, and the cyclonic circulation has moved to the south and east with a considerable elongation. Cross sections of heat transport and momentum transport are not dramatically different for the minor and major warming episodes.

Johnson, K. W.↗
NASA NTRS1985

Seasonal changes in the structure of the stratospheric circulation

The seasonal evolution of the stratospheric circulation in both hemispheres is studied using a coordinate independent diagnostic tied to the vortex, wherever it lies, rather than to latitude circles. Zonally averaged quantities are highly variable in the winter stratosphere, as the vortex moves on and off the pole, masking systematic changes in the structure of the vortex. The quantities shown here are the areas A(Q), where Ertel's potential vorticity is greater than a specified value Q, for various Q. In these calculations, Q is evaluated on the 850K isentropic surface which lies near 10 mb in the middle of the stratosphere. The advantage of using contours of Q (rather than contours of geopotential height, say) is that an area enclosed by such contours is approximately constant for quasi nondivergent, adiabatic, inviscid motion. Changes in area will occur if any of the above restrictions on the motion are invalid, and also if scales of motions are generated below those that can be adequately resolved. The evolution of area shows the systematic change in the average structure of the vortex. At a given time, the rate of change of Q with A(Q) gives a measure of the average gradient of Q. The gradient of Q is relevant for the propagation of large-scale disturbances into the stratosphere. Experience has also shown that winds tend to be strong (weak) when the gradient of Q is strong (weak).

Oneill, A.↗
NASA NTRS1985

Measurements of CCl3F, CCl2F2, CCl4, N2O and SF6 in the Northern Hemisphere stratosphere

An overview of the Department of Energy's High Altitude Sampling Program and some recent trace gas measurement results are presented. Analysis of whole air samples, collected in pressurized bottles, provides information on stratospheric inventories and distributions for CCl3F, CCl2F2, CCl4, N2O and SF6 in the Northern Hemisphere. Based on a linear regression analysis of the data the estimated mean Northern Hemisphere stratospheric concentration of each gas increased as follows: CCl3F changed from 54 to 142 p1/1 (4/74-11/83); CCl2F2 changed from 133 to 268 p1/1 (4/76-11/83); SF6 changed from 160 to 480 f1/1 (4/74-11/83); CC1, changed from 58 to 91 p1/1 (4/75-11/83); N2O changed from 246 to 261 n1/1 (4/76-11/83). The calculated mean Northern Hemisphere stratospheric concentrations of N2O, CCl3F, CCl2F2, and CCl4 after 1980 show larger than expected fluctuations with time. Recent volcanic activity may be a partial cause for these fluctuations through induced changes in stratospheric dynamical processes.

Leifer, R.↗
NASA NTRS1985

Transport processes in the stratosphere: Model simulations and comparisons with satellite observations

A three dimensional atmospheric model was used to study transport processes and to simulate the distribution of chemically active species in the stratosphere. The present results are part of a long term simulation of the seasonally varying structure of stratospheric trace constituents. The occurrence of a midwinter stratospheric warming and the associated transport of O3 and HNO3 during the simulation are described. Comparison of the simulated distributions of O3 and HNO3 are made with data from the Limb Infrared Monitor of the Stratosphere (LIMS) experiment. In addition, distributions of Ertel's potential vorticity on isentropic surfaces (IPV) are evaluated as a diagnostic for interpreting transport processes. Comparisons are made with IPV distributions inferred from LIMS temperature data.

Grose, W. L.↗
NASA NTRS1985

Ozone during sudden stratospheric warming: A three-dimensional simulation

Sudden warmings which are currently observed in the winter stratosphere are believed to be due to the upward propagation of planetary waves originating in the troposphere. Major warmings are characterized by local increases of the temperature in a deep layer beyond the stratopause, with values of the order of 50 K at 10 mbar appearing over a short period of time and leading to significant changes in the rate constant of several chemical reactions. During such events, the dynamical fields in the stratosphere are completely altered, so that dramatic changes in the transport of trace constituents are expected. Preliminary results of a 3-D model simulation of the ozone behavior during winter in connection with the appearance of stratospheric warmings are reported. The middle stratosphere (12 mbar or approximately 32 km) where the chemical lifetime of odd oxygen is quite long, and consequently, transport plays a major role is emphasized.

Rose, K.↗
NASA NTRS1985

Ion loss processes in the stratosphere

Small ions consisting of aggregates of a few molecules determine th stratospheric electrical parameters such as conductivity, mobility, etc. The small ion density is controlled by the ionizing mechanisms for the production of ions and electrons and the loss processes for these charged particles. Ion production in stratosphere is chiefly due to galactic cosmic rays, and the loss processes due to recombination and attachment. Free electrons do not exist at stratospheric heights. The primary positive ion O2+ and the electrons are converted into complex clusters of positive and negative ions. The equilibrium ion density is governed by the equation of continuity for the production and loss of these ions. In the generalized equation of continuity, the gain or loss of ions due to transport is neglected. When aerosols or particulates are not present in the atmosphere, ions are loss due to ion-ion recombination. In the presence of aerosols, small ions can also be lost by attachment to the aerosols, and thus aerosols are likely to cause perturbations in the stratosphere electrification. A simplified model approach is adopted to study the effect of aerosols on the equilibrium ion density. The results of the analysis for the equatorial station Thumba (8.5 deg N) are presented.

Prasad, B. S. N.↗
NASA NTRS1985

Balloon measurements of aerosol in the Antarctic stratosphere

Three balloon soundings of aerosol were conducted from Syowa Station, Antarctica in April, June and October 1983. Number concentration and the size distribution of aerosol particles with diameter greater than 0.3 microns were measured by using a light scattering aerosol particle counter. The influence of the eruption of Mt. El Chichon on the aerosol concentration in the stratosphere was observed on October 16. Very high aerosol concentration at stratospheric heights was obtained from the first successful aerosol sounding in winter Antarctic stratosphere. The result gives direct evidence of winter enhancement in the Antarctic stratosphere.

Morita, Y.↗
NASA NTRS1985

A study on radiative damping of planetary waves utilizing stratospheric observations

Satellite ozone observations made by the Stratospheric Aerosol and Gas Experiment (SAGE) and corresponding meteorological temperature data are used to study the radiative damping processes associated with planetary waves during stratospheric warmings. Ramanathan's model has been adapted for the radiative heating and cooling calculations. The derived infrared damping coefficients, based on observed stratospheric ozone and temperature, are compared with the Newtonian cooling coefficients of Dickinson and Fels. It is also shown that the negative correlation between temperature and ozone solar heating in the upper stratosphere accelerates the damping rate due to infrared cooling alone, in agreement with the theoretical analysis and an earlier report based on observations. In addition, it is also found in this analysis that the phase relationship between ozone and solar heating waves is characterized by its behavior in three distinct layers. In the regions above about 2 mb and also below about 10 mb, the waves are closely in-phase. Between approximately 2 and 10 mb, they show a departure from the in-phase relationship which can be attributed to the so-called 'opacity effect'. This effect significantly determines the magnitude of radiative damping.

Ghazi, A.↗
NASA NTRS1986

Transient medium-scale wave activity in the summer stratosphere

Observations of medium-scale transient wave activity in the middle-latitude Southern Hemisphere summer stratosphere are interpreted using isentropic potential vorticity (IPV) distributions inferred from temperature data from the Nimbus-7 Limb Infrared Monitor of the Stratosphere (LIMS) instrument. Despite problems with errors in reference-level synoptic height information, the derived IPV distributions clearly exhibit dynamically coherent signatures of eddy mixing due to medium-scale disturbances in the lower-middle stratosphere during early January 1979. The IPV distributions are shown to be strongly correlated with those of a contemporaneous set of isentropic maps of quasi-conservative tracers such as ozone and nitric acid. The results suggest that IPV maps inferred from satellite temperature data provide a useful diagnostic for studies of large-scale dynamics and/or transport in the extratropical stratosphere. Furthermore, the comparatively high vertical resolution of the LIMS data has enabled the vertical attenuation of Southern Hemisphere wave activity to be diagnosed in greater detail than could be achieved from nadir-viewing satellite information.

Miles, T.↗
NASA NTRS1986

Polar stratospheric clouds inferred from satellite data

Anomalously high radiances from the ozone channel of the Limb Infrared Monitor of the Stratosphere (LIMS) sounding instrument have been observed in the Northern Hemisphere winter lower stratosphere. Such events, thought to be due to polar stratospheric clouds (PSCs), are examined further by computing relative humidities using Stratospheric Sounding Unit temperatures and water vapor measurements from the LIMS Map Archive Tape analyses. Regions identified as PSCs are found to correspond closely to regions of high humidity. While instances of saturation were found, the average humidity at the centers of 39 PSCs was calculated to be 58 percent. Possible reasons for this apparent discrepancy are discussed. Applying a similar approach to the Southern Hemisphere, in 1979, virtually no PSCs are found in the vortex after September 10 at 20 km. This result has important implications for a number of proposed explanations for the Antarctic ozone hole.

Austin, J.↗
NASA NTRS1986

Condensation of HNO3 and HCl in the winter polar stratospheres

Nitric acid and hydrochloric acid vapors may condense in the winter polar stratospheres. Nitric acid clouds, unlike water ice clouds, would form at the temperatures at which polar stratospheric clouds (PSCs) are observed and would have optical depths of the magnitude observed suggesting that HNO3 is a dominant component of PSCs. ClO, N2O5 and ClNO3 may react on cloud particle surfaces yielding additional HNO3, HCl, and HOCL. In the vicinity of PSCs these reactions could deplete the stratosphere of photochemically active NO(x) species. The sedimentation of PSCs may remove these materials from the stratosphere. The loss of vapor phase NO(x) might allow halogen-based chemistry to create the ozone hole.

Toon, Owen B.↗
NASA NTRS1986

On the relationship between the thermal structure of the stratosphere and the seasonal distribution of ozone

An attempt is made to put the phenomenon of Antarctic ozone hole in a global perspective by pointing out that there is a much larger and more persistent 'hole' over the tropics. The thermal structure of the Antarctic lower stratosphere in winter is more similar to the tropical lower stratosphere than the Arctic lower stratosphere in winter. The dynamical transport that is responsible for creating the two column ozone minima has similar relationships to the thermal structure in the lower stratosphere in the two regions.

Tung, Ka Kit↗