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At least 469 records · Page 26
All sourcesNASA NTRSDOE OSTI
NASA NTRS1996

Stratospheric Heterogeneous Chemistry and Microphysics: Model Development, Validation and Applications

The objectives of this project are to: define the chemical and physical processes leading to stratospheric ozone change that involve polar stratospheric clouds (PSCS) and the reactions occurring on the surfaces of PSC particles; study the formation processes, and the physical and chemical properties of PSCS, that are relevant to atmospheric chemistry and to the interpretation of field measurements taken during polar stratosphere missions; develop quantitative models describing PSC microphysics and heterogeneous chemical processes; assimilate laboratory and field data into these models; and calculate the extent of chemical processing on PSCs and the impact of specific microphysical processes on polar composition and ozone depletion. During the course of the project, a new coupled microphysics/physical-chemistry/ photochemistry model for stratospheric sulfate aerosols and nitric acid and ice PSCs was developed and applied to analyze data collected during NASA's Arctic Airborne Stratospheric Expedition-II (AASE-II) and other missions. In this model, detailed treatments of multicomponent sulfate aerosol physical chemistry, sulfate aerosol microphysics, polar stratospheric cloud microphysics, PSC ice surface chemistry, as well as homogeneous gas-phase chemistry were included for the first time. In recent studies focusing on AASE measurements, the PSC model was used to analyze specific measurements from an aircraft deployment of an aerosol impactor, FSSP, and NO(y) detector. The calculated results are in excellent agreement with observations for particle volumes as well as NO(y) concentrations, thus confirming the importance of supercooled sulfate/nitrate droplets in PSC formation. The same model has been applied to perform a statistical study of PSC properties in the Northern Hemisphere using several hundred high-latitude air parcel trajectories obtained from Goddard. The rates of ozone depletion along trajectories with different meteorological histories are presently being systematically evaluated to identify the principal relationships between ozone loss and aerosol state. Under this project, we formulated a detailed quantitative model that predicts the multicomponent composition of sulfate aerosols under stratospheric conditions, including sulfuric, nitric, hydrochloric, hydrofluoric and hydrobromic acids. This work defined for the first time the behavior of liquid ternary-system type-1b PSCS. The model also allows the compositions and reactivities of sulfate aerosols to be calculated over the entire range of environmental conditions encountered in the stratosphere (and has been incorporated into a trajectory/microphysics model-see above). Important conclusions that derived from this work over the last few years include the following: the HNO3 content of liquid-state aerosols dominate PSCs below about 195 K; the freezing of nitric acid ice from sulfate aerosol solutions is likely to occur within a few degrees K of the water vapor frost point; the uptake and reactions of HCl in liquid aerosols is a critical component of PSC heterogeneous chemistry. In a related application of this work, the inefficiency of chlorine injection into the stratosphere during major volcanic eruptions was explained on the basis of nucleation of sulfuric acid aerosols in rising volcanic plumes leading to the formation of supercooled water droplets on these aerosols, which efficiently scavenges HCl via precipitation.

Turco, Richard P.↗
NASA NTRS2009

Presolar Organic Globules in Tagish Lake Meteorite, and other Astromaterials

Presolar grains were identified in meteorite residues 20 years ago based on their exotic isotopic compositions. Their study has provide new insights into stellar evolution and the first view of the original building blocks of the solar system. Organic matter in meteorites and IDPs is highly enriched in D/H and N-15/N-14 at micrometer scales, possibly due to presolar organic grains. These anomalies are ascribed to the partial preservation of presolar cold molecular cloud material. Identifying the carriers of these anomalies and elucidating their physical and chemical properties may give new views of interstellar chemistry and better understanding of the original components of the protosolar disk. However, identifying the carriers has been hampered by their small size and the inability to chemically isolate them. Thanks to immediate careful collection of Tagish Lake meteorite specimen, as well as major advances in nano-scale analytical techniques and advanced sample preparation, we were able to show that in the Tagish Lake meteorite, the principle carriers of these isotopic anomalies are sub-micrometer, hollow organic globules. The organic globules likely formed by photochemical processing of organic ices in a cold molecular cloud or the outermost regions of the protosolar disk. Organic globules with similar physical, chemical, and isotopic properties are also recently found from Bells CM2 carbonaceous chondrite, in IDPs and in the comet Wild-2 samples returned by Stardust. These results support the view that microscopic organic grains were widespread constituents of the protoplanetary disk. Their exotic isotopic compositions trace their origins to the outermost portions of the protosolar disk or a presolar cold molecular cloud.

Nakamura-Messenger, K.↗
NASA NTRS1982

Physical properties of Saturn's rings

Spaceborne astronomy data on Saturn's rings is summarized. The main rings are composed primarily of ice, possibly of low density and including small amounts of reddish material; particle radii are primarily centimeter-to-several meters, but significant amounts of micron-sized dust exists in certain regions including regions of resonance-induced collisions. The particle surface albedo and size distribution varies globally and locally. Evidence suggests several embedded moonlets of 10 km radius within Encke's division. The cause of the abrupt regional boundaries and associated differences in particle properties, especially the cause of the very abrupt and qualitatively similar inner A and B ring boundaries; the gap-ringlet structure and broad plateau features observed in the C and Cassini regions; the F and G rings (assuming that Enceladus is responsible for the E ring); and the cause of spokes and the SED are not understood.

Cuzzi, J. N.↗
NASA NTRS2012

Presolar Organic Globules in Astromaterials

Presolar grains were identified in meteorite residues 20 years ago based on their exotic isotopic compositions [1]. Their study has provide new insights into stellar evolution and the first view of the original building blocks of the solar system. Organic matter in meteorites and IDPs is highly enriched in D/H and N-15/N-14 at micron scales, possibly due to presolar organic grains [2-4]. These anomalies are ascribed to the partial preservation of presolar cold molecular cloud material. Identifying the carriers of these anomalies and elucidating their physical and chemical properties may give new views of interstellar chemistry and better understanding of the original components of the protosolar disk. However, identifying the carriers has been hampered by their small size and the inability to chemically isolate them. Thanks to major advances in nano-scale analytical techniques and advanced sample preparation, we were able to show that in the Tagish Lake meteorite, the principle carriers of these isotopic anomalies are sub-microns, hollow organic globules [5]. The organic globules likely formed by photochemical processing of organic ices in a cold molecular cloud or the outermost regions of the protosolar disk [5]. Organic globules with similar physical, chemical, and isotopic properties are also recently found from Bells CM2 carbonaceous chondrite, in IDPs [6] and in the comet Wild-2 samples returned by Stardust [7]. These results support the view that microscopic organic grains were widespread constituents of the protoplanetary disk. Their exotic isotopic compositions trace their origins to the outermost portions of the protosolar disk or a presolar cold molecular cloud.

Nakamura-Messenger, K.↗
NASA NTRS1993

Sensitivity of Asian and African climate to variations in seasonal insolation, glacial ice cover, sea surface temperature, and Asian orography

A general circulation model was used to investigate the sensitivity of Asian and African climate to prescribed changes in boundary conditions with the objective of identifying the relative importance of individual high-latitude glacial boundary conditions on seasonal climate and providing a physical basis for interpreting the paleoclimate record. The circulation model is described and results are presented. Insolation forcing increased summer Asian monsoon winds, while increased high-latitude ice cover strengthened winter Asian trade winds causing decreased precipitation. These factors had little effect on African climate. Cooler North Atlantic sea surface temperatures enhanced winter trade winds over North Africa, southern Asian climate was relatively unaffected. Reducing Asian orography enhanced Asian winter circulation while decreasing the summer monsoon. These model results suggest that African and southern Asian climate respond differently to separate elements of high-latitude climate variability.

Demenocal, Peter B.↗
NASA NTRS1986

Observations of cometary plasma wave phenomena

The ICE plasma wave investigation utilized very long electric antennas (100 m tip-to-tip) and a very high sensitivity magnetic search coil to obtain significant local information on plasma physics phenomena occurring in the distant pickup regions of Comet Giacobini-Zinner and Comet Halley; and information on the processes that developed in the coma and tail of Giacobini-Zinner. The ICE plasma wave measurements associated with both comet encounters are summarized, and high sensitivity ICE observations are related to corresponding measurements from the other Halley spacecraft.

Scarf, F. L.↗
NASA NTRS1990

Cirrus cloud model parameterizations: Incorporating realistic ice particle generation

Recent cirrus cloud modeling studies have involved the application of a time-dependent, two dimensional Eulerian model, with generalized cloud microphysical parameterizations drawn from experimental findings. For computing the ice versus vapor phase changes, the ice mass content is linked to the maintenance of a relative humidity with respect to ice (RHI) of 105 percent; ice growth occurs both with regard to the introduction of new particles and the growth of existing particles. In a simplified cloud model designed to investigate the basic role of various physical processes in the growth and maintenance of cirrus clouds, these parametric relations are justifiable. In comparison, the one dimensional cloud microphysical model recently applied to evaluating the nucleation and growth of ice crystals in cirrus clouds explicitly treated populations of haze and cloud droplets, and ice crystals. Although these two modeling approaches are clearly incompatible, the goal of the present numerical study is to develop a parametric treatment of new ice particle generation, on the basis of detailed microphysical model findings, for incorporation into improved cirrus growth models. For example, the relation between temperature and the relative humidity required to generate ice crystals from ammonium sulfate haze droplets, whose probability of freezing through the homogeneous nucleation mode are a combined function of time and droplet molality, volume, and temperature. As an example of this approach, the results of cloud microphysical simulations are presented showing the rather narrow domain in the temperature/humidity field where new ice crystals can be generated. The microphysical simulations point out the need for detailed CCN studies at cirrus altitudes and haze droplet measurements within cirrus clouds, but also suggest that a relatively simple treatment of ice particle generation, which includes cloud chemistry, can be incorporated into cirrus cloud growth.

Sassen, Kenneth↗
NASA NTRS2016

Analysis of the Warmest Arctic Winter, 2015-2016

December through February 2015-2016 defines the warmest winter season over the Arctic in the observational record. Positive 2m temperature anomalies were focused over regions of reduced sea ice cover in the Kara and Barents Seas and southwestern Alaska. A third region is found over the ice-covered central Arctic Ocean. The period is marked by a strong synoptic pattern which produced melting temperatures in close proximity to the North Pole in late December and anomalous high pressure near the Taymyr Peninsula. Atmospheric teleconnections from the Atlantic contributed to warming over Eurasian high-latitude land surfaces, and El Niño-related teleconnections explain warming over southwestern Alaska and British Columbia, while warm anomalies over the central Arctic are associated with physical processes including the presence of enhanced atmospheric water vapor and an increased downwelling longwave radiative flux. Preconditioning of sea ice conditions by warm temperatures affected the ensuing spring extent.

Barents and Kara Seas↗
NASA NTRS1987

Advances in terrestrial physics research at NASA/Goddard Space Flight Center

Some past, current, and future terrestrial physics research activities at NASA/Goddard Space Flight Center are described. The uses of satellites and sensors, such as Tiros, Landsat, Nimbus, and SMMR, for terrestrial physics research are discussed. The spaceborne data are applicable for monitoring and studying vegetation, snow, and ice dynamics; geological features; soil moisture; water resources; the geoid of the earth; and the earth's magnetic field. Consideration is given to improvements in remote sensing systems and data records and the Earth Observing System sensor concepts.

Salomonson, Vincent V.↗
NASA NTRS1987

Effects of charged particles on the surfaces of the satellites of Uranus

Measurements of the ion and electron fluxes in the Uranian magnetosphere made by the low-energy charged-particle (LECP) instrument on the Voyager 2 spacecraft are used to discuss possible particle-induced modifications of the moons and rings of Uranus. The energy spectra of the orbit-integrated particle dosages expected on the major moons are derived from the LECP measurements of particle intensities and pitch-angle distributions. Laboratory-derived results on charged-particle-induced chemical and physical modifications of H2O, CH4, CO, and CO2 ions are used. The erosion rates of water ice and the darkening of organic ices on the surfaces of the moons are estimated from the orbit-integrated fluxes. Significant darkening of fresh organic ices to depths of the order of 1 micron is expected to occur for times as short as a few thousand years. Darkening at deeper depths will occur at increasingly longer times. The implications of these results for the interpretation of remote-sensing data are discussed.

Lanzerotti, L. J.↗
NASA NTRS1991

Homogeneous freezing nucleation of stratospheric solution droplets

The classical theory of homogeneous nucleation was used to calculate the freezing rate of sulfuric acid solution aerosols under stratospheric conditions. The freezing of stratospheric aerosols would be important for the nucleation of nitric acid trihydrate particles in the Arctic and Antarctic stratospheres. In addition, the rate of heterogeneous chemical reactions on stratospheric aerosols may be very sensitive to their state. The calculations indicate that homogeneous freezing nucleation of pure water ice in the stratospheric solution droplets would occur at temperatures below about 192 K. However, the physical properties of H2SO4 solution at such low temperatures are not well known, and it is possible that sulfuric acid aerosols will freeze out at temperatures ranging from about 180 to 195 K. It is also shown that the temperature at which the aerosols freeze is nearly independent of their size.

Jensen, Eric J.↗
NASA NTRS1993

Production and optical constraints of ice tholin from charged particle irradiation of (1:6) C2H6/H2O at 77 K

Fifty separate irradiations of a 6:1 mixture of H2O/C2H6 ice conducted over a 5-month period have yielded sufficient tholin for the determination of its physical constants in the 0.06 to 40 micron range. While the imaginary part of the refractive index k was obtained by transmission measurements on thin-film samples and Kramers-Kronig analysis (KKA), the real part of the refractive index was obtained by KKA and ellipsometry; these data may prove useful in cometary and outer solar system spectrometric interpretation.

Khare, B. N.↗
NASA NTRS2011

New Challenges of Cloud Remote Sensing from Space

Clouds are recognized as a major source of uncertainties in predicting climate change. Lack of observational constraints on cloud processes has hindered the development of more reliable climate and weather models. With the advanced NASA EOS and A-Train sensors, we now have better knowledge about vertical distribution, water content, and occurrence frequency of global cloudiness. New ice water content (IWC) measurements from CloudSat and MLS have led to several improvements in model physics and parameterization schemes. MISR and GPS high-resolution data start to reveal deep insights on cloud processes and dynamicS in the planetary boundary layer (PBL). However, Earth sciences are still facing urgent needs to measure cloud microphysical properties, interactions between clouds and aerosol/precipitation, and processes that are coupled in 3-D space but not adequately sampled by the A-Train curtains or by the 2-D imageries. Submillimeter- wave, multi-angle imaging, and GPS radio occultation have emerged as promising remote sensing techniques to meet the challenges and enable new sciences for mid-tropospheric and PBL clouds.

Wu, Dong L.↗
NASA NTRS1985

Remote sensing of atmospheric and surface parameters from HIRS2/MSU on TIROS-N

At the Goddard Laboratory for Atmospheric Sciences (GLAS) a physically based satellite temperature sounding retrieval system was developed, involving the simultaneous analysis of sounding data, for determining atmospheric and surface conditions that are consistent with the observed radiances. In addition to determining accurate atmospheric temperature profiles even in the presence of clouds, the system provides global estimates of day and night sea or land surface temperatures, snow and ice cover, cloud amounts, cloudtop heights and temperatures, and albedo. The characteristics of the atmospheric and surface parameters derived from the GLAS Physical Retrieval System are reviewed, results for the FGGE year are presented and, whenever possible, compared with other measurements of the same fields. Some of the model-derived diagnostic fields available from the GLAS Analysis/Forecast System are also discussed. These fields may lead to more accurate determination of the source terms of the atmospheric heat and moisture budgets.

Susskind, J.↗
NASA NTRS1996

The Structural Properties of Vapor Deposited Water Ice and Astrophysical Implications

Films of vapor deposited water ice at low temperature (T<30 K) show a number of interesting structural changes during a gradual warmup. We would like to talk about the structure of the low temperature high density amorphous form of water ice, the process of crystallization, and some recent work on the morphological changes of water ice films at high temperature. The studies of the high density amorphous form are from in-situ electron microscopy as well as numerical simulations of molecular dynamics and have lead to new insights into the physical distinction between this high density amorphous form and the low density amorphous form. For the process of crystallization, we propose a model that describes the crystallization of water ice from the amorphous phase to cubic ice in terms of the nucleation of small domains in the ice. This model agrees well with the behavior of water ice in our electron microscopy studies and finds that pure water above the glass transition is a strong liquid. In more recent work, we have concentrated on temperatures above the crystallization temperature and we find interesting morphological changes related to the decrease in viscosity of the amorphous component in the cubic crystalline regime. Given enough time, we would like to put these results in an astrophysical context and discuss some observed features of the frost on interstellar grains and the bulk ice in comets.

Jenniskens, P.↗
NASA NTRS1987

Human Adaptation to Isolated and Confined Environments

A study was conducted over seven months in a winter Antarctic isolated and confined environment (ICE). Physiological and psychological data was collected several times a week. Information was collected on a monthly basis on behavior and the use of physical facilities. Adaptation and information indicated that there was a significant decrease in epinephrine and norepinephrine during the middle trimester of the winter. No vital changes were found for blood pressure. Self reports of hostility and anxiety show a linear increase. There were no significant changes in depression during ICE. The physiological and psychological data do not move in a synchronous fashion over time. The data also suggest that both ambient qualities of an ICE and discrete social environmental events, such as the arrival of the summer crew, have an impact on the outcome measures used. It may be most appropiate to develop a model for ICE's that incorporates not only global chronic stressors common to all ICE's but also the role of discrete environmental effects which can minimize or enhance the influence of more chronic stressors. Behavioral adjustment information highlight the importance of developing schedules which balance work and recreational activities.

Evans, Gary W.↗
NASA NTRS2004

Convective Instability in Ice I: Application to Callisto and Ganymede

Laboratory experiments measuring ice rheology suggest that it deforms under the influence of several nonNewtonian creep mechanisms, where the viscosity depends on both strain rate and temperature [Goldsby & Kohlstedt, 2001]. Whether or not a fluid with a purely temperature-dependent viscosity convects can be determined by comparing the Rayleigh number of the system to the critical Rayleigh number (Racr), which depends on rheological, thermal, and physical parameters of the fluid layer. However, in a nonNewtonian fluid where viscosity depends on the strain rate (i.e. velocity), convection can only occur if a temperature or velocity perturbation is issued to the system to lower the viscosity and permit fluid motions. Therefore, whether convection occurs in an ice I layer depends on initial conditions, in addition to rheological, thermal, and physical properties of the layer. We show new results for a scaling between the critical Rayleigh number and perturbation amplitude for grain boundary sliding rheology. This scaling can be used to determine the conditions required to initiate convection in the ice I shell of a generic icy satellite. We use this scaling to judge the convective instability of Ganymede and Callisto's ice shells in the absence of tidal dissipation.

Barr, A. C.↗