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At least 469 records · Page 26

Thermodynamic investigation of the NaCl-KCl salt system from 25 to 950 °C

NaCl-KCl molten salt system has been proposed as a primary component of several promising heat transfer eutectics and fuel host for Generation IV molten salt reactors (MSR). In this work, several key thermodynamic parameters, including high temperature enthalpies, isobaric heat capacities (C p ) and molar enthalpies of mixing (ΔH mix ), of the NaCl -KCl system (NaCl, 75mol% NaCl – 25mol% KCl, 51mol% NaCl – 49mol% KCl, 25mol% NaCl – 75mol% KCl, and KCl) were measured by high temperature drop calorimetry (HTDC) utilizing laser sealed nickel and aluminum crucibles. Salts were checked for phase purity by X-ray diffraction (XRD), and water content by Karl Fischer coulometric titrimetry and thermogravimetric analysis (TGA). Thermo-mechanical analysis (TMA) utilizing custom-built boron nitride (BN) crucibles was employed to determine temperatures of phase transitions (solid $\rightarrow$ liquid) for the salts and plotted against the pseudobinary phase diagram for the NaCl-KCl system. Small deviations (3-10 %) were found among C p values obtained from HTDC, differential scanning calorimetry (DSC), and NIST, comparable to the average uncertainty based on two standard deviations of measured data that are ~6% for DSC and ~3% for HTDC. Additionally, the measured enthalpies and C p values of mixed NaCl-KCl salts (e.g., 51mol% NaCl – 49mol% KCl eutectic) were shown to behave as statistical mixtures of its pure endmembers, consistent with ΔH mix = ~ 0 kJ/mol at 800 °C, and a regular interaction parameter of Ω = 1.20 ± 0.76 kJ/mol. In conclusion, this study represents a step towards improved accuracy and precision in determinations of thermodynamic parameters of molten salts by using DSC, TMA, and HTDC, in completion of the Molten Salt Thermal Properties Database (MSTDB).

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Effects of magnetic fields on HPGe tracking detectors

Here, we present a study of magnetic fields effects on the position resolution and energy response of hyper-pure germanium detectors. Our results provide realistic estimates of the potential impact on the resolving power of tracking-arrays from (fringe) magnetic fields present when operating together with large spectrometers. By solving the equations of motion for the electron and holes in the presence of both electric and magnetic fields, we analyzed the drift trajectories of the charge carriers to determine the deviations in the positions at the end point of the trajectories, as well as changes in drift lengths affecting the energy resolution and peak shift due to trapping. Our results show that the major effect is in the deviation of the transverse (to the electric field direction) position and suggest that, if no corrective action is taken in the pulse-shape and tracking data analysis procedures, a field strength ≳ 0.1 T will start to impact the intrinsic position resolution of 2 mm (RMS). At fields above ~1 T, the degradation of the energy response becomes observable.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Anisotropic neutron response of trans-stilbene and impact on a handheld dual particle imager

Here this manuscript details measurements of the anisotropic light-output response of trans-stilbene, henceforth referred to as stilbene, along the three primary crystal planes and analyzes how this anisotropic response impacts neutron image reconstruction in a handheld dual particle imager (H2DPI). A prototype H2DPI composed of stilbene pillars (6 x 6 x 50 mm 3 ) coupled to silicon photomultipliers was built and is capable of imaging both fast neutrons and gamma rays from kilogram quantities of special nuclear material. Stilbene was chosen as the scintillating medium for the imager because of its pulse shape discrimination capability, time resolution and relatively high light output. A drawback to using stilbene, however, is the anisotropic response. A recoiling proton from a neutron elastic-scattering event in stilbene will yield different amounts of scintillation light depending on the direction of the recoiling proton with respect to the crystal lattice. This manuscript analyzes how this anisotropic response impacts neutron image reconstruction in 4π. The light output in the three primary crystal planes of stilbene were independently measured 6–7 times for proton recoil energies ranging from 0.5–5.0 MeV using a quasi-monoenergetic time-of-flight neutron source. The measured light-output data in the three crystal planes were fit with a semi-empirical function based on Birks’ formula. These fits were used to reconstruct the location of a 252 Cf source in front of the imager (0°, -0.8°), to the left of the imager (-90°, -0.8°) and directly above the imager (0°, 90°) to determine if it is necessary to apply the directionally-dependent response of stilbene to accurately reconstruct source locations. A bootstrapping technique was applied to the measured data sets to produce 1000 images composed of 2000 cone projections for each source location and each measured light-output curve. List-mode maximum likelihood expectation maximization was applied to each image; the highest pixel location and the full width at half maximum (FWHM) were then recorded. The average and standard deviations of these parameters were taken for each set of images. The maximum difference in the average azimuthal pixel location when varying between the appropriate and incorrect light-output curves for the source locations at (0°, -0.8°) and (-90°, -0.8°) were respectively found to be 1.85 ± 1.39° and 2.03 ± 1.78°. All other pixel locations and FWHMs were within a single standard deviation of uncertainty. Taken together, the anisotropic response of stilbene has negligible impact on the neutron image reconstruction capability of the H2DPI.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Search for new phenomena in three- or four-lepton events in pp collisions at $\sqrt{s}$ = 13 TeV with the ATLAS detector

A search with minimal model dependence for physics beyond the Standard Model in events featuring three or four charged leptons (3ℓ and 4ℓ, ℓ = e,μ) is presented. The analysis aims to be sensitive to a wide range of potential new-physics theories simultaneously. This analysis uses data from pp collisions delivered by the Large Hadron Collider at a centre-of-mass energy of $\sqrt{s}$ = 13 TeV and recorded with the ATLAS detector, corresponding to the full Run 2 dataset of 139 fb -1 . The 3ℓ and 4ℓ phase space is divided into 22 event categories according to the number of leptons in the event, the missing transverse momentum, the invariant mass of the leptons, and the presence of leptons originating from a Z-boson candidate. These event categories are analysed independently for the presence of deviations from the Standard Model. No statistically significant deviations from the Standard Model predictions are observed. Upper limits for all signal regions are reported in terms of the visible cross-section.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Search for new heavy resonances decaying to WW, WZ, ZZ, WH, or ZH boson pairs in the all-jets final state in proton-proton collisions at √s = 13 TeV

A search for new heavy resonances decaying to WW, WZ, ZZ, WH, or ZH boson pairs in the all-jets final state is presented. The analysis is based on proton-proton collision data recorded by the CMS detector in 2016–2018 at a centre-of-mass energy of 13 TeV at the CERN LHC, corresponding to an integrated luminosity of 138 fb –1 . The search is sensitive to resonances with masses between 1.3 and 6 TeV, decaying to bosons that are highly Lorentz-boosted such that each of the bosons forms a single large-radius jet. Machine learning techniques are employed to identify such jets. No significant excess over the estimated standard model background is observed. A maximum local significance of 3.6 standard deviations, corresponding to a global significance of 2.3 standard deviations, is observed at masses of 2.1 and 2.9 TeV. In a heavy vector triplet model, spin-1 Z' and W' resonances with masses below 4.8 TeV are excluded at the 95% confidence level (CL). These limits are the most stringent to date. In a bulk graviton model, spin-2 gravitons and spin-0 radions with masses below 1.4 and 2.7 TeV, respectively, are excluded at 95% CL. Production of heavy resonances through vector boson fusion is constrained with upper cross section limits at 95% CL as low as 0.1 fb.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Evidence for four-top quark production in proton-proton collisions at s = 13 TeV

The production of four top quarks ($\mathrm{t\bar{t}t\bar{t}}$) is studied with LHC proton-proton collision data samples collected by the CMS experiment at a center-of-mass energy of 13 TeV, and corresponding to integrated luminosities of up to 138 fb$^{-1}$. Events that have no leptons (all-hadronic), one lepton, or two opposite-sign leptons (where lepton refers only to prompt electrons or prompt muons) are considered. This is the first $\mathrm{t\bar{t}t\bar{t}}$ measurement that includes the all-hadronic final state. The observed significance of the $\mathrm{t\bar{t}t\bar{t}}$ signal in these final states of 3.9 standard deviations (1.5 expected) provides evidence for $\mathrm{t\bar{t}t\bar{t}}$ production, with a measured cross section of 36 $^{+12}_{-11}$ fb. Combined with earlier CMS results in other final states, the signal significance is 4.0 standard deviations (3.2 expected). The combination returns an observed cross section of 17 $\pm$ 4 (stat) $\pm$ 3 (syst) fb, which is consistent with the standard model prediction.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Observation of four top quark production in proton-proton collisions at s = 13 TeV

The observation of the production of four top quarks in proton-proton collisions is reported, based on a data sample collected by the CMS experiment at a center-of-mass energy of 13 TeV in 2016–2018 at the CERN LHC and corresponding to an integrated luminosity of 138 fb − 1 . Events with two same-sign, three, or four charged leptons (electrons and muons) and additional jets are analyzed. Compared to previous results in these channels, updated identification techniques for charged leptons and jets originating from the hadronization of b quarks, as well as a revised multivariate analysis strategy to distinguish the signal process from the main backgrounds, lead to an improved expected signal significance of 4.9 standard deviations above the background-only hypothesis. Four top quark production is observed with a significance of 5.6 standard deviations, and its cross section is measured to be 17.7 − 3.5 + 3.7 (stat) − 1.9 + 2.3 (syst) fb , in agreement with the available standard model predictions.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Search for pair production of boosted Higgs bosons via vector-boson fusion in the $b$$\overline{b}$$b$$\overline{b}$ final state using $pp$ collisions at $\sqrt{s}$ = 13 TeV with the ATLAS detector

A search for Higgs boson pair production via vector-boson fusion is performed in the Lorentz-boosted regime, where a Higgs boson candidate is reconstructed as a single large-radius jet, using 140 fb−1 of proton–proton collision data at $\sqrt{s}$ = 13 TeV recorded by the ATLAS detector at the Large Hadron Collider. Only Higgs boson decays into bottom quark pairs are considered. The search is particularly sensitive to the quartic coupling between two vector bosons and two Higgs bosons relative to its Standard Model prediction, K 2V . This study constrains K 2V to 0.55 < K 2V < 1.49 at the 95% confidence level. The value K 2V = 0 is excluded with a significance of 3.8 standard deviations with other Higgs boson couplings fixed to their Standard Model values. A search for new heavy spin-0 resonances that would mediate Higgs boson pair production via vector-boson fusion is carried out in the mass range of 1–5 TeV for the first time under several model and decay-width assumptions. No significant deviation from the Standard Model hypothesis is observed and exclusion limits at the 95% confidence level are derived.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Search for a standard model-like Higgs boson in the mass range between 70 and 110 GeV in the diphoton final state in proton-proton collisions at $\sqrt{s} = 13$ TeV

The results of a search for a standard model-like Higgs boson decaying into two photons in the mass range between 70 and 110 GeV are presented. The analysis uses the data set collected by the CMS experiment in proton-proton collisions at $\sqrt{s} = 13$ TeV corresponding to integrated luminosities of 36.3 fb -1 , 41.5 fb -1 and 54.4 fb -1 during the 2016, 2017, and 2018 LHC running periods, respectively. No significant excess over the background expectation is observed and 95% confidence level upper limits are set on the product of the cross section and branching fraction for decays of an additional Higgs boson into two photons. The maximum deviation with respect to the background is seen for a mass hypothesis of 95.4 GeV with a local (global) significance of 2.9 (1.3) standard deviations. The observed upper limit ranges from 15 to 73 fb.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Observation of VVZ production at $\sqrt{s}$ = 13 TeV with the ATLAS detector

A search for the production of three massive vector bosons, VVZ(V = W, Z) , in proton-proton collisions at $\sqrt{s}$ = 13 TeV is performed using data with an integrated luminosity of 140 fb -1 recorded by the ATLAS detector at the Large Hadron Collider. Events produced in the leptonic final states WWZ → ℓvℓvℓℓ (ℓ = e,μ), WZZ → ℓvℓℓℓℓ, ZZZ → ℓℓℓℓℓ, and the semileptonic final states WWZ → qq ℓvℓℓ and WZZ → ℓv qq ℓℓ, are analysed. The measured cross section for the pp → VVZ process is 660$^{+93}_{-90}$(stat.)$^{+80}_{-81}$(syst.) fb, and the observed (expected) significance is 6.4 (4.7) standard deviations, representing the observation of VVZ production. In addition, the measured cross section for the pp → WWZ process is 442 ± 94(stat.)$^{+60}_{-52}$(syst.) fb, and the observed (expected) significance is 4.4 (3.6) standard deviations, representing evidence of WWZ production. The measured cross sections are consistent with the Standard Model predictions. Constraints on physics beyond the Standard Model are also derived in the effective field theory framework by setting limits on Wilson coefficients for dimension-8 operators describing anomalous quartic gauge boson couplings.

Aad, G. (ORCID:0000000266654934)↗

Search for CP violation in events with top quarks and Z bosons at $\sqrt{s}$ = 13 and 13.6 TeV

A search for the violation of the charge-parity (CP) symmetry in the production of top quarks in association with Z bosons is presented, using events with at least three charged leptons and additional jets. The search is performed in a sample of proton-proton collision data collected by the CMS experiment at the CERN LHC in 2016–2018 at a center-of-mass energy of 13 TeV and in 2022 at 13.6 TeV, corresponding to a total integrated luminosity of 173 fb –1 . For the first time in this final state, observables that are odd under the CP transformation are employed. Also for the first time, physics-informed machine-learning techniques are used to construct these observables. While for standard model (SM) processes the distributions of these observables are predicted to be symmetric around zero, CP-violating modifications of the SM would introduce asymmetries. Two CP-odd operators $\mathcal{O}$$^{I}_{tW}$ and $\mathcal{O}$$^{I}_{tZ}$ in the SM effective field theory are considered that may modify the interactions between top quarks and electroweak bosons. The obtained results are consistent with the SM prediction within two standard deviations, and exclusion limits on the associated Wilson coefficients of –2.7 < $c$$^{I}_{tW}$ < 2.5 and –0.2 < $c$$^{I}_{tZ}$ < 2.0 and are set at 95 % confidence level. The largest discrepancy is observed in $c$$^{I}_{tZ}$ where data is consistent with positive values, with an observed local significance with respect to the SM hypothesis of 2.5 standard deviations, when only linear terms are considered.

CMS↗

Search for Higgs bosons produced in association with a high-energy photon via vector-boson fusion and decaying to a pair of b -quarks in the ATLAS detector

A search for Standard Model Higgs bosons produced in association with a high-energy photon and decaying to $b\bar{b}$ is performed using 133 fb −1 of $\sqrt{s}$ = 13 TeV pp collision data collected with the ATLAS detector at the Large Hadron Collider at CERN. The photon requirement reduces the multijet background, and the H → $b\bar{b}$ decay is the dominant decay mode. Event selection requirements target events produced by vector-boson fusion, the dominant production mode in this channel. Several improvements enhance the search sensitivity compared to previous measurements. These improvements include better background modelling and characterization, the use of a neural-network classifier, and an updated signal extraction strategy adopting a direct binned-likelihood fit to the classifier output. With these improvements, the Higgs boson signal strength is measured to be 0.2 ± 0.7 relative to the Standard Model prediction. This corresponds to an observed significance of 0.3 standard deviations, compared to an expectation of 1.5 standard deviations assuming the Standard Model.

ATLAS experiment↗

Search for the Higgs boson decay to a Z boson and a photon in pp collisions at $\sqrt{s}$ = 13 TeV and 13.6 TeV with the ATLAS detector

A search for the Higgs boson decay to a Z boson and a photon in the ℓℓγ (ℓ = 𝑒,𝜇) final state is performed using pp collisions at $\sqrt{s}$ = 13.6 TeV recorded with the ATLAS detector at the Large Hadron Collider during 2022–2024, corresponding to an integrated luminosity of 165 fb−1. The signal yield, normalised to the Standard Model prediction, is measured to be 𝜇 = 0.9$^{+0.7}_{−0.6}$, compatible with the expected value of 𝜇 = 1.0 ± 0.7. This corresponds to an observed (expected) signal significance of 1.4 (1.5) standard deviations under the background-only hypothesis. This result is combined with that of a similar search performed with 140 fb −1 of $\sqrt{s}$ = 13 TeV pp collisions to provide the best expected sensitivity to date to this rare decay, namely an observed (expected) signal strength of 𝜇 = 1.3$^{+0.6}_{−0.5}$ (𝜇 = 1.0$^{+0.6}_{−0.5}$), corresponding to an observed (expected) significance of 2.5 (1.9) standard deviations. The measurement is consistent with the Standard Model expectation.

Aad, G. (ORCID:0000000266654934)↗

Probing late-stage hadronic interactions at high baryon density via $K^{⁎0}$ production in the RHIC beam energy scan program

A precision measurement of the $K^{⁎0}$ meson yield is reported in Au+Au collisions at $\sqrt{s_{NN}}$ = 7.7, 11.5, 14.6, 19.6, and 27 GeV using the high-statistics data sample collected by the STAR experiment during the Beam Energy Scan II (BES-II) program at RHIC. The transeverse momentum (p T )-integrated yield ratios $\large{(}K^{⁎0} + \overline{K^{⁎0}}\large{)}/(K^+ + K^{-})$ in central collisions show a suppression relative to peripheral collisions at the (1.7–3.6) σ level, while a thermal model without final-stage rescattering overpredicts this ratio with a deviation of (6.9–8.2) σ. These results indicate a loss of the measured $K^{⁎0}$ signal in central collisions due to re-scattering of its hadronic decay products in the hadronic phase. The p T -integrated yield of charged kaons exhibits an approximate scaling with charged-particle multiplicity, independent of collision energy and system size. A similar trend is observed for the short-lived $K^{⁎0}$ resonance, although significant deviations emerge at lower energies. At BES energies, the $K^{⁎0}/K$ ratio shows stronger suppression than at the highest RHIC and LHC energies within a given multiplicity bin, particularly in central and mid-central collisions. This behavior is consistent with changes in the effective hadronic interaction cross section and is supported by transport model calculations, which indicate dominant meson–baryon interactions at lower energies and meson–meson interactions at higher energies.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Characterization of lift force and torque in prolate ellipsoid suspensions

The paper derives correlations for lift force and fluid torques acting on stationary prolate ellipsoid suspensions of aspect ratio (AR) 2.5, 5, and 10 subjected to uniform flow. Here, Particle Resolved Simulations (PRS) are conducted on a suspension of infinite extent in two directions for Reynolds number 10≤Re≤200 and solid fractions (φ) between 0.1≤φ≤0.3.The suspension-mean lift-to-drag ratio varies between 7% to 14% at Re=10 which increases to 14%~22% at Re=200. The torque-induced tip rotational acceleration can reach 38%~85% of drag-induced translational acceleration at Re=200. Single particle lift force and torque correlations of (Fröhlich et al., 2020) are modified and adapted to predict current angular-mean lift and torque data. The resulting lift correlation captures the PRS data within an average deviation below 7%. Torque exhibits a somewhat more complex dependency at AR=10 than the assumed sinθ ∙ cosθ variation but nevertheless the correlations predict angular-mean values with mean relative deviations of 16.6% at AR=10.

42 ENGINEERING↗

Real-Time Defect Correction in Large-Scale Polymer Additive Manufacturing via Thermal Imaging and Laser Profilometer

Defects can result in a failed part and are costly in terms of time and material. This cost is even greater in the context of large-scale additive manufacturing where the objects can be very large. As a result, a great deal of research has focused on defect identification and mitigation. To address defects during object construction, researchers at Oak Ridge National Laboratory’s Manufacturing Demonstration Facility investigated an in-situ control system comprised of two sensors: a thermal camera and laser profilometer. This control system adjusted material flow and build speed to mitigate three types of defects: low layer times, underfill, and overfill. Several test objects were constructed. The control system was found to adjust build parameters to handle low layer times of approximately 15 seconds and height deviations from -100% underfill (the absence of a layer) to 50% overfill. Within two layers, height deviations could be returned to within 10% of the expected layer height. Further, preliminary results suggest the system can compensate for uneven build surfaces.

Borish, Michael↗

Quantification of manganese for ChemCam Mars and laboratory spectra using a multivariate model

In this work, we report a new calibration model for manganese using the laser-induced breakdown spectroscopy instrument that is part of the ChemCam instrument suite onboard the NASA Curiosity rover. The model has been trained using an expanded set of 523 manganese-bearing rock, mineral, metal ore, and synthetic standards. The optimal calibration model uses the Partial Least Squares (PLS) and Least Absolute Shrinkage and Selection Operator (LASSO) multivariate techniques, with a novel “double blending” technique. We determined the detection limit for manganese is 82 ppm using a method blank procedure and is possibly as low as 27 ppm based on visual inspection of the spectra. Based on a representative test set consisting of measurements on 93 standards, the double blended multivariate model shows a Root Mean Squared Error of Prediction (RMSEP) accuracy of 1.39 wt% MnO for the full blended model. Employing a local RMSEP estimate where the model performance is evaluated based on nearby test samples, the accuracy is 0.03 wt% at the quantification limit (0.05 wt% MnO), 0.4 wt% accuracy at 1.0 wt% MnO, and 4.4 wt% accuracy at 100 wt% MnO. Precision is estimated using the standard deviation of the test set measurements, and is ±0.01 wt% MnO at the quantification limit, ±0.09 wt% MnO at 1.0 wt% MnO, and ± 2.1 wt% MnO at 100 wt% MnO (all 1 standard deviation). This new calibration is important for understanding the variation of manganese in the bedrock with the Curiosity rover on Mars, which provides insight into past redox conditions on Mars.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Observation of structure in the J/ψ-pair mass spectrum

Using proton-proton collision data at centre-of-mass energies of $\sqrt{s}$ = 7, 8 and 13 TeV recorded by the LHCb experiment at the Large Hadron Collider, corresponding to an integrated luminosity of 9 fb -1 , the invariant mass spectrum of J/ψ pairs is studied. A narrow structure around 6.9 GeV/c 2 matching the lineshape of a resonance and a broad structure just above twice the J/ψ mass are observed. The deviation of the data from nonresonant J/ψ-pair production is above five standard deviations in the mass region between 6.2 and 7.4 GeV/c 2 , covering predicted masses of states composed of four charm quarks. The mass and natural width of the narrow X(6900) structure are measured assuming a Breit-Wigner lineshape.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗