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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 469 records · Page 26
All sourcesNASA NTRSDOE OSTI
DOE OSTI2020

Single Shot Characterization of High Transformer Ratio Wakefields in Nonlinear Plasma Acceleration

We report that plasma wakefields can enable very high accelerating gradients for frontier high energy particle accelerators, in excess of 10 GeV/m. To overcome limits on single stage acceleration, specially shaped drive beams can be used in both linear and nonlinear plasma wakefield accelerators (PWFA), to increase the transformer ratio, implying that the drive beam deceleration is minimized relative to acceleration obtained in the wake. In this Letter, we report the results of a nonlinear PWFA, high transformer ratio experiment using high-charge, longitudinally asymmetric drive beams in a plasma cell. An emittance exchange process is used to generate variable drive current profiles, in conjunction with a long (multiple plasma wavelength) witness beam. The witness beam is energy modulated by the wakefield, yielding a response that contains detailed spectral information in a single-shot measurement. Using these methods, we generate a variety of beam profiles and characterize the wakefields, directly observing transformer ratios up to R=7.8. Lastly, a spectrally based reconstruction technique, validated by 3D particle-in-cell simulations, is introduced to obtain the drive beam current profile from the decelerating wake data.

43 PARTICLE ACCELERATORS↗
DOE OSTI2023

Symmetry Control of Unconventional Spin–Orbit Torques in IrO 2

Abstract Spin–orbit torques generated by a spin current are key to magnetic switching in spintronic applications. The polarization of the spin current dictates the direction of switching required for energy‐efficient devices. Conventionally, the polarizations of these spin currents are restricted to be along a certain direction due to the symmetry of the material allowing only for efficient in‐plane magnetic switching. Unconventional spin–orbit torques arising from novel spin current polarizations, however, have the potential to switch other magnetization orientations such as perpendicular magnetic anisotropy, which is desired for higher density spintronic‐based memory devices. Here, it is demonstrated that low crystalline symmetry is not required for unconventional spin–orbit torques and can be generated in a nonmagnetic high symmetry material, iridium dioxide (IrO 2 ), using epitaxial design. It is shown that by reducing the relative crystalline symmetry with respect to the growth direction large unconventional spin currents can be generated and hence spin–orbit torques. Furthermore, the spin polarizations detected in (001), (110), and (111) oriented IrO 2 thin films are compared to show which crystal symmetries restrict unconventional spin transport. Understanding and tuning unconventional spin transport generation in high symmetry materials can provide a new route towards energy‐efficient magnetic switching in spintronic devices.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2022

Amorphizing noble metal chalcogenide catalysts at the single-layer limit towards hydrogen production

Rational design of noble metal catalysts with the potential to leverage efficiency is vital for industrial applications. Such an ultimate atom-utilization efficiency can be achieved when all noble metal atoms exclusively contribute to catalysis. In this work, we demonstrate the fabrication of a wafer-size amorphous PtSex film on a SiO 2 substate via a low-temperature amorphization strategy, which offers single-atom-layer Pt catalysts with high atom-utilization efficiency (~26 wt%). This amorphous PtSex (1.2 < x < 1.3) behaves as a fully activated surface, accessible to catalytic reactions, and features a nearly 100% current density relative to a pure Pt surface and reliable production of sustained high-flux hydrogen over a 2 inch wafer as a proof-of-concept. Furthermore, an electrolyser is demonstrated to generate a high current density of 1,000 mA cm –2 . Such an amorphization strategy is potentially extendable to other noble metals, including the Pd, Ir, Os, Rh and Ru elements, demonstrating the universality of single-atom-layer catalysts.

36 MATERIALS SCIENCE↗
DOE OSTI2026

Testing of a 15 kA Superconducting Transformer

Here, the manufacturing of superconducting magnets for High Energy Physics (HEP) and Fusion Energy Sciences (FES) applications requires high-current conductors to generate stronger magnetic fields without increasing the inductance of the magnet. Increased inductance is undesirable due to the associated AC losses, which reduce the temperature margin; and the quench protection also becomes complicated. Testing high-current conductors with a direct current (DC) room temperature power supply is unfeasible for two primary reasons: 1) the limited capacity to supply large currents, and 2) the significant heat load losses at the current leads. A superconducting transformer offers a solution to both challenges. A 50-kA superconducting transformer is planned for manufacturing and commissioning at Brookhaven National Laboratory as part of its user facility upgrade. This transformer will facilitate the testing of superconducting cables, conductors, joints, and insert coils under high magnetic field conditions (10 T) and with currents up to 50-kA. To evaluate the manufacturing process and validate the theoretical models, the magnet division has developed and tested a 15-kA prototype transformer. A control loop has been implemented to ensure precise current delivery to the sample. This paper presents the coil design, manufacturing, and experimental results from the cold tests.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2019

Design of Fieldable Head Space Manifold

A system has been designed and built to meet the expected requirements for sampling large UF 6 cylinders in the field and to provide similar purification and analyses to those currently performed for 1S and 2S samples at Oak Ridge National Laboratory (ORNL). The system was designed to be modular, allowing flexibility to perform under a variety of conditions. At a minimum, a large cylinder can be accessed to collect head space samples. These samples can additionally be processed in the field to generate 10 cc purified samples that should be similar to ones currently generated at ORNL from sampling of smaller cylinders. Variable inlet mass spectrometer operation can be performed at the time of purification or at a different location on a purified sample. This design should allow collection, processing and analysis of one extracted sample per day based on similar operations using the ORNL manifold. Reduced operations can be performed at a slightly faster rate although movement between cylinders does require time to evacuate and dry the connection adequately for accessing the UF 6 head space.

42 ENGINEERING↗
DOE OSTI2022

First Measurement Of Charged-current 1 Muon 2 Proton 0 Pion Single Differential Cross-sections On Argon-40 At 0.8 Gev Average Neutrino Energy With The MicroBooNE Detector

Constraining systematic uncertainties that arise from neutrino-nucleon cross-section modeling is critical for upcoming neutrino oscillation experiments. Neutrino interactions that lead to the ejection of 2 particles from the target nucleus, leaving the nucleus with 2 holes, are one cross-section of interest. These instances, known as 2-particle 2-hole (2p2h) states, can be produced either by neutrino interaction modes or from the influence of nuclear physics on the neutrino interaction. While there are many theoretical models that attempt to describe the nature of 2p2h states, very few experimental measurements of this process exist, making it difficult to benchmark theoretical calculations. Furthermore, no high statistic cross-section measurements of 2p2h states exist on $^{40}$Ar, the target nucleus of many current and next generation neutrino oscillation experiments. This analysis aims to address this issue by providing the first high-statistic single differential cross-section me asurements of 2p2h states. Using data collected from the first 3 years of running of the MicroBooNE experiment, we select $\nu_\mu$ charged-current interaction events that produce a single muon, 2 protons, and no pions in the final state (CC1$\mu$2p0$\pi$). The single differential cross-section is then extracted as a function of a variety of physics variables and compared to theoretical predictions from several event generator model sets.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2023

Robust Adaptive Control for Large-scale Inverter-based Resources with Partial and Complete Loss of Inverters

This article proposes an approach to address the current and the aggregated active power control challenge for large-scale inverter-based resources subjected to partially or completely loss of inverters and grid voltage variations. To address this problem, a distributed active power mechanism is proposed which generates desired inverters current. Then an adaptive mechanism distributes the voltage control input automatically between inverters in response to the partial or complete loss of inverters. An L2-gain-based controller is designed for each inverter to track the desired current and rejects the grid voltage disturbance. Here, simulation results show a significant robust tracking for collective active power and current.

24 POWER TRANSMISSION AND DISTRIBUTION↗
DOE OSTI2020

High resolution time- and angle-resolved photoemission spectroscopy with 11 eV laser pulses

Performing time- and angle-resolved photoemission (tr-ARPES) spectroscopy at high momenta necessitates extreme ultraviolet laser pulses, which are typically produced via high harmonic generation (HHG). Despite current advances, HHG-based setups still require large pulse energies (from hundreds of μ J to mJ) and their energy resolution is limited to tens of meV. Here, we present a novel 11 eV tr-ARPES setup that generates a flux of 5 × 10 10 photons/s and achieves an unprecedented energy resolution of 16 meV. It can be operated at high repetition rates (up to 250 kHz) while using input pulse energies down to 3 µ J. We demonstrate these unique capabilities by simultaneously capturing the energy and momentum resolved dynamics in two well-separated momentum space regions of a charge density wave material ErTe 3 . This novel setup provides the opportunity to study the non-equilibrium band structure of solids with exceptional energy and time resolutions at high repetition rates.

47 OTHER INSTRUMENTATION↗
DOE OSTI2020

Analysis of multi-electron, multi-step homogeneous catalysis by rotating disc electrode voltammetry: theory, application, and obstacles

Rotating disc electrode (RDE) voltammetry has been widely adopted for the study of heterogenized molecular electrocatalysts for multi-step fuel-forming reactions but this tool has never been comprehensively applied to their homogeneous analogues. Here, the utility and limitations of RDE techniques for mechanistic and kinetic analysis of homogeneous molecular catalysts that mediate multi-electron, multi-substrate redox transformations are explored. Using the ECEC' reaction mechanism as a case study, two theoretical models are derived based on the Nernst diffusion layer model and the Hale transformation. Current–potential curves generated by these computational strategies are compared under a variety of limiting conditions to identify conditions under which the more minimalist Nernst Diffusion Layer approach can be applied. Based on this theoretical treatment, strategies for extracting kinetic information from the plateau current and the foot of the catalytic wave are derived. RDEV is applied to a cobaloxime hydrogen evolution reaction (HER) catalyst under non-aqueous conditions in order to experimentally validate this theoretical framework and explore the feasibility of RDE as a tool for studying homogeneous catalysts. Importantly, analysis of the foot-of-the-wave via this theoretical framework provides rate constants for elementary reaction steps that agree with those extracted from stationary voltammetric methods, supporting the application of RDE to study homogeneous fuel-forming catalysts. Lastly, obstacles encountered during the kinetic analysis of cobaloxime, along with the voltammetric signatures used to diagnose this reactivity, are discussed with the goal of guiding groups working to improve RDE set-ups and help researchers avoid misinterpretation of RDE data.

08 HYDROGEN↗
DOE OSTI2024

Macroscopic trends of linear tearing stability in cylindrical current profiles

Abstract The likelihood of realising tokamak power-plants will be greatly improved by the discovery of high-gain equilibria that resist the formation of small islands and hence avoid the disruptive neoclassical tearing mode. We propose a series of studies to understand how simple tokamak design can leverage aspects of tearing onset physics to maximise passive resistance to island formation. Here we investigate the variation that current profiles can bring about in preventing tearing onset through the cylindrical linear tearing stability parameter Δ ′ . A database of 159148 realistic pilot-plant current profiles was generated with Monte Carlo sampling, and the distribution of Δ ′ values was linked with interpretable profile characteristics. In agreement with prior theoretical and experimental studies, Δ ′ was found to be strongly correlated with the existence and steepness of a local toroidal current well or hill, with the former destabilising and the latter stabilising. In the absence of these two cases, the remaining Δ ′ values were linearly bounded by the toroidal current gradient at the rational surface.

Physics↗
DOE OSTI2023

Report on the Creation and Progress of the Hydrogen Regulatory Research Review Group

The current U.S. nuclear generation fleet is increasingly recognized by governmental, scientific, public policy, and industrial communities as having a strategic role in support of the ongoing national transition to a clean energy future. Federal incentives and actions are aligning to expand the role of nuclear power as a viable and more flexible contributor to the evolving national clean energy mix through programs and initiatives such as nuclear power loan guarantees; the Inflation Reduction Act’s (IRA) clean nuclear electrical, steam, and hydrogen incentives; the Infrastructure Investment and Jobs Act (IIJA, also referred to as the Bipartisan Infrastructure Act or BIL); and near term Department of Energy (DOE) funding opportunities related to nuclear based hydrogen hubs and nuclear integrated hydrogen demonstration projects. . Additionally, leveraging clean nuclear electricity and steam is being explored by industries desiring to transition away from carbon-intensive energy sources. Even with all these emerging enablers, notable barriers remain for the widespread adoption of these opportunities within the U.S. nuclear fleet, including the following: • Assurance of the markets for alternate products needed to support decision-making for large capital modification investments • Electric utility mindset and business history centered solely on producing electricity • Design change complexity and regulatory uncertainty associated with plant modifications needed to support alternate product streams The DOE Light Water Reactor Sustainability (LWRS) Flexible Plant Operations and Generation (FPOG) Pathway is developing options to help U.S. nuclear power plants (NPP) in all these areas to enable NPPs designed for steady baseload operation to integrate with intermittent wind and solar capacity to assure reliable clean energy for the nation. Current and near-term laboratory research is focusing on the technical, regulatory, safety, demonstration, and economic elements in support of improving nuclear plant flexibility through hybrid production of electricity and other non-electric products such as hydrogen and energy arbitrage.

42 ENGINEERING↗
DOE OSTI2022

Streaming readout for next generation electron scattering experiments

Current and future experiments at the high-intensity frontier are expected to produce an enormous amount of data that needs to be collected and stored for offline analysis. Thanks to the continuous progress in computing and networking technology, it is now possible to replace the standard ‘triggered’ data acquisition systems with a new, simplified and outperforming scheme. ‘Streaming readout’ (SRO) DAQ aims to replace the hardware-based trigger with a much more powerful and flexible software-based one, that considers the whole detector information for efficient real-time data tagging and selection. Considering the crucial role of DAQ in an experiment, validation with on-field tests is required to demonstrate SRO performance. In this paper, we report results of the on-beam validation of the Jefferson Lab SRO framework. In this work, we exposed different detectors (PbWO-based electromagnetic calorimeters and a plastic scintillator hodoscope) to the Hall-D electron-positron secondary beam and to the Hall-B production electron beam, with increasingly complex experimental conditions. By comparing the data collected with the SRO system against the traditional DAQ, we demonstrate that the SRO performs as expected. Furthermore, we provide evidence of its superiority in implementing sophisticated AI-supported algorithms for real-time data analysis and reconstruction.

47 OTHER INSTRUMENTATION↗
DOE OSTI2026

Transverse BBU Suppression with Feedback for Energy-Recovery Linacs

The Electron–Ion Collider (EIC) achieves its design luminosity by cooling the ion beam with a high-current electron beam generated in an energy-recovery linac (ERL). The baseline ERL lattice employs a BNL five-cell cavity that is frequency-scaled to 197 MHz, 591 MHz, and 1.773 GHz, raising concerns about multibunch beam-breakup (BBU) instabilities. Threshold currents for each frequency option are established with two independent BBU tracking codes, providing cross-validated operating margins that guide cavity selection. To further increase the current limit, we incorporate a digital transverse feedback (FB) system that targets the dominant higher-order modes (HOMs). Simulations show the FB raises the BBU threshold by roughly an order of magnitude: power-spectral-density analysis of the beam centroid at the linac exit confirms strong suppression of the aliased HOM peak, although some spectral growth appears at secondary frequencies. This combined study quantifies baseline BBU limits, demonstrates effective active mitigation, and charts a practical path toward robust, high-current operation of the EIC ERL.

Accelerator Physics↗
DOE OSTI2019

Post-Irradiation Fracture Toughness Characterization of Generation II FeCrAl Alloys

Currently, the handbook on FeCrAl material properties contains only limited data regarding the fracture toughness properties of any FeCrAl alloy, let alone alloys currently under investigation within the Advanced Fuels Campaign (AFC) such as the Oak Ridge National Laboratory (ORNL) derived FeCrAl alloys. Unirradiated datasets developed both by ORNL and previously within literature using Charpy V-notch specimens to determine the ductile to brittle transition temperature (DBTT) showed key findings including (i) increasing Al and/or Cr content can raise the DBTT of FeCrAl alloys, (ii) DBTT values can typically reside at or above room temperature for FeCrAl alloys, and (iii) grain size and residual strain can have an effect on the fracture properties. These results suggest that the fracture toughness of FeCrAl alloys may be a factor in its deployment for nuclear power applications, but no studies have been completed prior regarding the DBTT or fracture toughness of FeCrAl alloys after neutron irradiation, especially for the leaner Cr content alloys currently under investigation as candidate alloys for light water reactor (LWR) cladding. Taken in isolation, embrittlement of a cladding alloy during service has no bearing on possible licensure. Hydriding of zirconium cladding alloys is well understood to result in significant embrittlement. Furthermore, mechanical failure of irradiated cladding containing fuel pellets occurs at far higher stresses than defueled cladding samples because the presence of the fuel toughens the fuel rod. Despite this absence of direct relevance to licensure, radiation embrittlement is a fundamental structure-property evolution that should be understood to guide further development of FeCrAl alloys. Licensure of FeCrAl incorporates far more complex system behaviors that will not be possible until larger quantities of fueled irradiated rodlets are available.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2023

High temperature and high beam current compatible targets and methods thereof for generating noble gas/radiohalogen generators for medical isotopes

A method of providing alpha particle emitters and materials suitable for use in generating the alpha particles for medical treatment is disclosed. Metal oxide targets, preferentially Bi 2 O 3 pellets and Bi 2 O 3 coatings on metallic or metal oxide substrates are formed. The targets placed in a heated vacuum chamber subjecting to irradiation using a 6 Li beam at an elevated temperature below the melting point of the target generate a radioactive gas, such as 211 Rn, the radioactive gas is carried by an inert gas which is delivered a carrier for, such as a carbon column or oil for delivery to a treatment facility. The radioactive gas such as 211 Rn generates 211 At, which has a useable half-life of at least about 14 hours, in turn releases alpha particles which are effective for use in medical procedures.

Sampathkumaran, Uma↗
DOE OSTI2025

Comparing Advanced Bipolar Membranes for High-Current Electrodialysis and Membrane Electrolysis

Advanced bipolar membranes (BPMs) with low water-dissociation overpotential (ηwd) may enable new electrochemical technologies for electrolysis, fuel cells, acid–base synthesis, brine remediation, lithium-battery recycling, and cement production. However, these advanced BPMs have only been demonstrated in BPM water electrolysis (BPMWE) configurations where the BPM is under static compression by the porous-transport layers. It is important to study these BPMs in applications like electrodialysis where large degrees of static compression are not possible. We present a BPM electrodialysis (BPMED) platform to measure water-dissociation overpotential (ηwd) and compare BPMWE and BPMED systems. We show advanced BPMs with half the ηwd compared to commercial BPMs for BPMED while maintaining ∼90% current efficiency from 0.05–0.5 A cm–2. The BPMED ηwd values are, however, about 0.2 V higher at 0.5 A cm–2 than those for BPMWE. Regardless, these results show that BPMs developed and optimized in BPMWE applications are well-suited for next-generation high-current-density BPMED technologies.

Vulpin, Olivia T↗
DOE OSTI2020

Physics of E × B discharges relevant to plasma propulsion and similar technologies

This paper provides perspectives on recent progress in understanding the physics of devices in which the external magnetic field is applied perpendicular to the discharge current. This configuration generates a strong electric field that acts to accelerate ions. The many applications of this set up include generation of thrust for spacecraft propulsion and separation of species in plasma mass separation devices. These “E × B” plasmas are subject to plasma–wall interaction effects and to various micro- and macroinstabilities. In many devices we also observe the emergence of anomalous transport. This perspective presents the current understanding of the physics of these phenomena and state-of-the-art computational results, identifies critical questions, and suggests directions for future research.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗