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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 469 records · Page 26
All sourcesNASA NTRSDOE OSTI
DOE OSTI2015

Extracting source parameters from beam monitors on a chopper spectrometer

The intensity distributions of beam monitors in direct-geometry time-of-flight neutron spectrometers provide important information about the instrument resolution. For short-pulse spallation neutron sources in particular, the asymmetry of the source pulse may be extracted and compared to Monte Carlo source simulations. An explicit formula using a Gaussian-convolved Ikeda-Carpenter distribution is given and compared to data from the ARCS instrument at the Spallation Neutron Source.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2017

SNS Proton Beam Window Disposal

In order to support the disposal of the proton beam window assembly of the Spallation Neutron Source beamline to the target station, waste classification analyses are performed. The window has a limited life-time due to radiation-induced material damage. Here, analyses include calculation of the radionuclide inventory and shielding analyses for the transport package/container to ensure that the container is compliant with the transportation and waste management regulations. In order to automate this procedure and minimize manual work a script in Perl language was written.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
DOE OSTI2013

IBIS: An inverse geometry Brillouin inelastic neutron spectrometer for the SNS

The high power target station at the Spallation Neutron Source (SNS) currently has about 20 completed neutron scattering instruments. With a broad coverage of the momentum transfer (Q)-energy (E) space, these instruments serve an extensive user community. In an effort to further expand the scientific capabilities of the SNS instrument suites, we propose a low background, inverse geometry Brillouin inelastic spectrometer for the SNS which will expand the Q-E coverage of the current instrument suite and facilitate the study of inelastic and quasi-elastic scatterings at low Q values. The possible location for the proposed instrument is either beamline 8 which views the decoupled water moderator, or beamline 14A, which views a cold, coupled super critical hydrogen moderator. The instrument parameters, optimizations, and performances at these two beamline locations are discussed.

43 PARTICLE ACCELERATORS↗
DOE OSTI2014

FRIB cryogenic distribution system

The Michigan State University Facility for Rare Isotope Beams (MSU-FRIB) helium distribution system has been revised to include bayonet/warm valve type disconnects between each cryomodule and the transfer line distribution system, similar to the Thomas Jefferson National Accelerator Facility (JLab) and the Spallation Neutron Source (SNS) cryogenic distribution systems. The heat loads at various temperature levels and some of the features in the design of the distribution system are outlined. The present status, the plans for fabrication, and the procurement approach for the helium distribution system are also included.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2014

Very low electron temperature in warm dense matter formed by focused picosecond soft x-ray laser pulses

We investigated the optical emission from the ablating surfaces induced by the irradiations of soft x-ray laser (SXRL) pulses with the aim of estimation of the maximum electron temperature. No emission signal in the spectral range of 400–800 nm could be observed despite the formation of damage structures on the target surfaces. Hence, we estimated an upper limit for the electron temperature of 0.4–0.7 eV for the process duration of 100–1000 ps. Our results imply that the ablation and/or surface modification by the SXRL is not accompanied by plasma formation but is induced by thermo-mechanical pressure, which is so called a spallative ablation. This spallative ablation process occurs in the low electron temperature region of a non-equilibrium state of warm dense matter.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2019

Requirements and sensitivity analysis for temporally- and spatially-resolved thermometry using neutron resonance spectroscopy

Neutron resonance spectroscopy (NRS) has been used extensively to make temperature measurements that are accurate, absolute, and nonperturbative within the interior of material samples under extreme conditions applied quasistatically. Yet NRS has seldom been used in dynamic experiments. There is a compelling incentive to do so because of the significant shortcomings of alternative techniques. An important barrier to adopting dynamic NRS thermometry is the difficulty in fielding it with conventional spallation neutron sources. To enable time-dependent and spatially resolved temperature measurements in dynamic environments, more compact neutron sources that can be used at user facilities in conjunction with other diagnostic probes (such as x-ray light sources) are required. Such sources may be available using ultrafast high-intensity optical lasers. We evaluate such possibilities by determining the sensitivities of the temperature estimate on neutron-beam and diagnostic parameters. Based on that evaluation, requirements are set on a pulsed neutron-source and diagnostics to make a meaningful dynamic temperature measurement. Dynamic thermometry measurements are examined in this context when driven by two alternative fast-neutron sources: the Los Alamos Neutron Scattering Center (LANSCE) proton accelerator driving isotropic spallation neutrons as a baseline and a laser-plasma ion accelerator driving a neutron beam from deuterium breakup. Strategies to close the gap between the required and demonstrated performance of laser-based fast-neutron sources are presented. A short-pulse high-intensity laser with state-of-the-art pulse contrast and an energy of a few hundred Joules would drive a compact neutron source suitable for NRS thermometry that could transform the dynamic study of materials.

47 OTHER INSTRUMENTATION↗
DOE OSTI2018

Next-generation diamond cell and applications to single-crystal neutron diffraction

In this paper, a diamond cell optimized for single-crystal neutron diffraction is described. It is adapted for work at several of the single-crystal diffractometers of the Spallation Neutron Source and the High Flux Isotope Reactor at the Oak Ridge National Laboratory (ORNL). A simple spring design improves portability across the facilities and affords load maintenance from offline pressurization and during temperature cycling. Compared to earlier prototypes, pressure stability of polycrystalline diamond (Versimax®) has been increased through double-conical designs and ease of use has been improved through changes to seat and piston setups. These anvils allow ~30%-40% taller samples than possible with comparable single-crystal anvils. Hydrostaticity and the important absence of shear pressure gradients have been established with the use of glycerin as a pressure medium. Large single-crystal synthetic diamonds have also been used for the first time with such a clamp-diamond anvil cell for pressures close to 20 GPa. The cell is made from a copper beryllium alloy and sized to fit into ORNL’s magnets for future ultra-low temperature and high-field studies. Finally, we show examples from the Spallation Neutron Source’s SNAP and CORELLI beamlines and the High Flux Isotope Reactor’s HB-3A and IMAGINE beamlines.

36 MATERIALS SCIENCE↗
DOE OSTI2021

3D-printed B 4 C collimation for neutron pressure cells

A design for an incident-beam collimator for the Paris–Edinburgh pressure cell is described here. This design can be fabricated from reaction-bonded B 4 C but also through fast turnaround, inexpensive 3D-printing. 3D-printing thereby also offers the opportunity of composite collimators whereby the tip closest to the sample can exhibit even better neutronic characteristics. Here, we characterize four such collimators: one from reaction-bonded B 4 C, one 3D-printed and fully infiltrated with cyanoacrylate, a glue, one with a glue-free tip, and one with a tip made from enriched 10 B 4 C. The collimators are evaluated on the Spallation Neutrons and Pressure Diffractometer of the Spallation Neutron Source and the Wide-Angle Neutron Diffractometer at the High Flux Isotope Reactor, both at Oak Ridge National Laboratory. This work clearly shows that 3D-printed collimators perform well and also that composite collimators improve performance even further. Beyond use in the Paris–Edinburgh cell, these findings also open new avenues for collimator designs as clearly more complex shapes are possible through 3D printing. An example of such is shown here with a collimator made for single-crystal samples measured inside a diamond anvil cell. These developments are expected to be highly advantageous for future experimentation in high pressure and other extreme environments and even for the design and deployment of new neutron scattering instruments.

47 OTHER INSTRUMENTATION↗
DOE OSTI2021

H- ion source research and development at the Oak Ridge National Laboratory

The U.S. Spallation Neutron Source (SNS) is a state-of-the-art neutron scattering facility delivering the world's most intense pulsed neutron beams to a wide array of instruments which are used to conduct investigations in many fields of science and engineering. Neutrons are produced by spallation of liquid Hg due to bombardment of short (~1µs), intense (~35 A) pulses of protons delivered at 60 Hz from a storage ring which is fed by a high-intensity, 1 GeV H- LINAC. This facility has operated almost continuously since 2006, with ion source performance increasing over those years, and currently providing 50-60 mA of H- ions with a duty-factor of 6% for maintenance-free runs of ~120 days with near 100% availability. Ion source research and development at ORNL has played a key role in enabling and supporting these achievements: this report provides some historical highlights of this effort, describes our current ion source testing facilities, discusses the goals of the program and finally provides a snapshot of some of our ongoing R&D activities. In particular, we have recently simplified and improved the reliability of the plasma ignition gun for the external antenna ion source which is discussed in detail.

Welton, Robert F.↗
DOE OSTI2021

Methods for neutron diffraction studies on hydride superconductors and other metal hydrides

High-pressure neutron diffraction is an extremely useful technique in the quest for making and understanding novel hydride superconductors. Neutron diffraction can be used to directly determine elemental stoichiometries and atomic positions of many light elements such as hydrogen or deuterium, even in the presence of heavy elements such as rare-earth metals. In this work, we report on the current status and ongoing developments on high-pressure neutron diffraction for hydride superconductors and other metal hydrides with a special focus on current advancements at the Spallation Neutrons and Pressure (SNAP) beamline of the Spallation Neutron Source at Oak Ridge National Laboratory. For broader context, an overview of high-pressure neutron diffractometers and pressure cells is included together with insight into critical sample considerations. There, attention is given to the requirements for powdered hydride samples and the need for deuterium rather than hydrogen. Additionally, the advantages of angular access and data representation as possible at SNAP are described. We demonstrate the current capability for high-pressure neutron diffraction on two different samples created via hydrogen gas loading, specifically pure deuterium and nickel-deuteride. The deuterium example highlights the usefulness of adding sample materials that facilitate the formation of a good powder while the nickel-deuteride example demonstrates that atomic deuterium positions and stoichiometry can be directly determined. Both examples highlight the importance of large scattering apertures. These enable investigation of the data resolved by scattering angle that is needed to identify parasitic peaks and background features. Finally, future directions beyond current high-pressure neutron powder diffraction are also discussed.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2024

Gallium oxide (Ga 2 O 3 ) energy dependent scintillation response to fast neutrons and flash gamma-rays

Gallium oxide is a newly emerged ultrawide bandgap (4.9 eV) semiconductor that is suitable as a combined electronics and radiation detection platform. We have experimentally demonstrated fast neutron and gamma-ray scintillation from Czochralski-grown β-Ga 2 O 3 in a recent series (October 2023) of experiments at the unmoderated pulsed neutron spallation source located at the Los Alamos Neutron Science Center. Using the neutron time-of-flight (TOF) technique and a fast-gated intensified CCD camera, we observed energy-dependent neutron scintillation for neutron energies ranging from 1 to 400 MeV, including the 14.1 MeV neutron energy relevant to D–T fusion. Neutron flux is quantified and calibrated by cascading the scintillator after the fission chamber, enabling a detailed analysis of temporal and energy-dependent characteristics of the scintillation events. Further, a pronounced scintillation signal from the spallation gamma flash with a temporal full width of half maximum of ~4 ns is indicative of the material’s rapid response. Neutron energy dependent scintillation is observed using the TOF method at a 22.6-m distance from the neutron source. These results highlight the possibility of developing a Ga 2 O 3 based fusion neutron diagnostic platform integrated with both scintillation and electronics functions on the integrated chip scale.

47 OTHER INSTRUMENTATION↗
DOE OSTI2026

Analysis of Second Target Station Target Removal Dose Rates

The Second Target Station (STS) project at Oak Ridge National Laboratory’s spallation neutron source is a crucial initiative for maintaining U.S. leadership in neutron sciences. The STS aims to create the world’s brightest pulsed cold neutron source, enabling cutting-edge research across various scientific disciplines. To ensure safe and efficient maintenance operations, understanding the effects of shutdown dose rates from activated components within the STS target systems is essential. This study establishes a computational framework for calculating decay gamma sources and subsequent shutdown dose rates utilizing advanced methods to account for all activation channels, including high-energy interactions down to thermal neutron capture. This study describes a novel integration of multiple tools and provides an effective means of analyzing activation and shutdown dose rates at spallation neutron facilities. A custom-developed script automates the decay gamma source generation process, ensuring proper sampling during the variance reduction phase, which is critical for accurate predictions of shutdown dose rates.

Transmutation↗
DOE OSTI2012

Diffusive propagation of cosmic rays from supernova remnants in the Galaxy. I: spectrum and chemical composition

In this paper we investigate the effect of stochasticity in the spatial and temporal distribution of supernova remnants on the spectrum and chemical composition of cosmic rays observed at Earth. The calculations are carried out for different choices of the diffusion coefficient D(E) experienced by cosmic rays during propagation in the Galaxy. In particular, at high energies we assume that D(E)∝E{sup δ}, with δ = 1/3 and δ = 0.6 being the reference scenarios. The large scale distribution of supernova remnants in the Galaxy is modeled following the distribution of pulsars, with and without accounting for the spiral structure of the Galaxy. We find that the stochastic fluctuations induced by the spatial and temporal distribution of supernovae, together with the effect of spallation of nuclei, lead to mild but sensible violations of the simple, leaky-box-inspired rule that the spectrum observed at Earth is N(E)∝E{sup −α} with α = γ+δ, where γ is the slope of the cosmic ray injection spectrum at the sources. Spallation of nuclei, even with the small rates appropriate for He, may account for small differences in spectral slopes between different nuclei, possibly providing an explanation for the recent CREAM observations. For δ = 1/3 we find that the slope of the proton and helium spectra are ∼ 2.67 and ∼ 2.6 respectively (with fluctuations depending on the realization of source distribution) at energies around ∼ 1 TeV (to be compared with the measured values of 2.66±0.02 and 2.58±0.02). For δ = 0.6 the hardening of the He spectra is not observed. The stochastic effects discussed above cannot be found in ordinary propagation calculations, such as GALPROP, where these effects and the point like nature of the sources are not taken into account. We also comment on the effect of time dependence of the escape of cosmic rays from supernova remnants, and of a possible clustering of the sources in superbubbles. In a second paper we will discuss the implications of these different scenarios for the anisotropy of cosmic rays.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2018

Raman Spectroscopy as an ortho-para diagnostic of liquid hydrogen moderators

The intense radiation environment of a neutron moderator provides a mechanism for significant up-conversion of parahydrogen to orthohydrogen inside the moderator, as well as intrinsically catalyzing relaxation of orthohydrogen to parahydrogen. It is plausible that the steady-state orthohydrogen fraction of a moderator in a radiation environment such as at the Spallation Neutron Source (SNS) or the European Spallation Source (ESS) is as high as 30 % without supplemental catalysis. Direct measurement of the orthohydrogen fraction in the liquid hydrogen flow itself is essential to predict and monitor moderator performance, especially for thick or flat moderator concepts such as the ones that have been proposed for the ESS and for upgrades to the SNS. Raman spectroscopy provides a well-known method for directly measuring the hydrogen make-up in an unambiguous way. We describe our tests of Raman spectroscopy for application to the measurement of the orthohydrogen fraction of the hydrogen moderators at SNS and at the ESS. As part of this work, we have additionally developed a sample holder that has been used to perform simultaneous Raman and neutron vibrational spectroscopy on the VISION spectrometer at SNS. We discuss our plans to incorporate such a system as a diagnostic for liquid hydrogen moderators at SNS and at the ESS.

Gillis, Robert Chad↗
DOE OSTI2022

Negative hydrogen ion sources for particle accelerators: Sustainability issues and recent improvements in long-term operations

High brightness, negative hydrogen ion sources are used extensively in scientific facilities operating worldwide. Negative hydrogen beams have become the preferred means of filling circular accelerators and storage rings as well as enabling efficient extraction from cyclotrons. Several well-known facilities now have considerable experience with operating a variety of sources such as RF-, filament-, magnetron- and Penning-type H- ion sources. These facilities include the US Spallation Neutron Source (SNS), Japan Proton Accelerator Research Complex (J-PARC), Rutherford Appleton Laboratory (RAL-ISIS), Los Alamos Neutron Science Center (LANSCE), Fermi National Accelerator Laboratory (FNAL), Brookhaven National Laboratory (BNL), numerous installations of D-Pace (licenced by TRIUMF) ion sources used mainly on cyclotrons and, most recently, the CERN-LINAC-1 injector. This report first summarizes the current performance of these ion sources in routine, daily operations with attention toward source service-periods and availability metrics. Sustainability issues encountered at each facility are also reported and categorized to identify areas of common concern and key issues. Recent ion source improvements to address these issues are also discussed as well as plans for meeting future facility upgrade requirements.

Welton, Robert F.↗
DOE OSTI2017

Data processing workflow for time of flight polarized neutrons inelastic measurements

We discuss the data processing workflow for polarized neutron scattering measurements performed at HYSPEC spectrometer at the Spallation Neutron Source, Oak Ridge National Laboratory. The effects of the focusing Heusler crystal polarizer and the wide-angle supermirror transmission polarization analyzer are added to the data processing flow of the non-polarized case. The implementation is done using the Mantid software package.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2017

Polarized neutron scattering on HYSPEC: the HYbrid SPECtrometer at SNS

Here, we describe some of the first polarized neutron scattering measurements performed at HYSPEC [1-4] spectrometer at the Spallation Neutron Source, Oak Ridge National Laboratory. Furthermore, we discuss details of the instrument setup and the experimental procedures in the mode with full polarization analysis. Examples of polarized neutron diffraction and polarized inelastic neutron data obtained on single crystal samples are presented.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2023

Recent H - ion source research and development at the Oak Ridge National Laboratory

The U.S. Spallation Neutron Source (SNS) is a state-of-the-art neutron scattering facility delivering the world's most intense pulsed neutron beams to a wide array of instruments which are used to conduct investigations in many fields of science and engineering. Neutrons are produced from spallation of liquid Hg by bombardment of short (~1 μs), intense (~35 A) pulses of protons delivered at 60 Hz by a storage ring which is fed by a high-intensity, ~1 GeV H - LINAC. This facility has operated almost continuously since 2006, with ion source performance increasing over those years, and currently providing 50–60 mA of H - ions with a duty-factor of 6% for maintenance-free runs of several months with near 100% availability. Ion source research and development at ORNL has played a key role in enabling and supporting this success: this report provides an update on some of the ongoing ion source research and development efforts which have been undertaken since the previous Negative Ion Beams and Sources (NIBS) conference in 2020. These include significant improvements to H - beam current by extraction from a larger source outlet aperture and improvements to the electron dumping system which should eliminate the gradual loss of electrode voltage over the course of a run which has occasionally impacted SNS operations. Improvement and simplification of the plasma ignition system for the external antenna ion source, a long-standing problem, was also realized. Lastly, RF coupling efficiency was measured for both the SNS internal and external antenna ion sources.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗