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At least 469 records · Page 26

Effects of fast and thermal neutron irradiation on Ga-polar and N-polar GaN diodes

Studies of the radiation tolerance and electrical behavior of gallium nitride (GaN) based devices are important for the next generation of high-power and high-voltage electronics that may be subjected to harsh environments such as nuclear reactor and fusion facilities, particle accelerators, and post-denotation environments. Here, in this work, we study the behavior of Ga-polar and N-polar GaN Schottky diodes before and after exposure to fast and thermal + fast neutrons. Temperature-dependent current–voltage (I–V) and circular transmission line method (CTLM) measurements were used to study the electrical characteristics. A strong reduction in reverse leakage current and an increase in differential resistance in forward bias were observed after neutron irradiation. Thermionic emission (TE), Frenkel–Poole (FP) emission, and Fowler–Nordheim (FN) tunneling models were used to explain the forward and reverse I–V characteristics pre- and post-irradiation. The study confirms that Ga-polar and N-polar GaN Schottky diodes exhibit different electrical responses to fast and thermal neutron irradiations. The reverse bias characteristics of N-polar diodes are less affected after the fast neutron irradiation compared to Ga-polar diodes, while in the forward bias region, the electrical behavior after fast and thermal neutron irradiations is similar in Ga-polar and N-polar diodes. The results indicate that the role of orientation should be considered in the design of GaN-based radiation-tolerant electronics.

42 ENGINEERING↗

Transmission electron microscopy with in-situ ion irradiation: Facilities and community

Whilst there is a clear scientific and technological need for the technical capabilities of transmission electron microscopes with in-situ ion irradiation, it also requires a collaborative community of international researchers to support such facilities in successfully meeting this demand. Instruments of this type serve to provide fundamental understanding of the mechanisms which drive changes in materials important to nuclear fission and fusion energy, the semiconductor industry, quantum information systems, space travel, astronomy, geology and many more applications. As these areas continue to evolve and the instrumentation possibilities expand, the capacity of in-situ ion irradiation facilities must also develop hand-in-hand with the user community to deliver an ever-greater diversity of high-fidelity extreme-environment experimentation. Future directions for the field, such as miniaturization from MEMS/microfluidic devices and advanced controls with ML-based analysis, continuously emerge to advance both the hardware and software which support the coupling of TEMs with ion beams. This review sets out to provide up-to-date insights into the community and advancement of current, and development of future, facilities which have the potential to further unlock access to the nanoscale exploration of coupled extreme environments crucial to many of the important science and engineering challenges we face today.

In-situ irradiation↗

Microstructure and fracture toughness characterization of three 9Cr ODS EUROFER steels with different thermo-mechanical treatments

Ferritic martensitic ODS steels are one of the candidate structural materials for future Gen-IV nuclear fission and fusion reactors. Here, the dependence of fracture toughness on microstructure was investigated by comparing three 9Cr ODS EUROFER steels manufactured through different thermo-mechanical processing routes. Quasi-static fracture toughness testing was performed with sub-sized C(T) specimens and microstructural characterization was carried out using scanning electron microscopy, electron backscatter diffraction, and transmission electron microscopy. It was found that at lower test temperatures (-100 – 22 °C), the fracture toughness was primarily controlled by crack initiation at sub-micron particles and by production of secondary cracks during fracture. At higher temperatures (above 100 °C), fracture toughness was predominantly controlled by the matrix ductility and the grain boundary strength with a relatively ductile coarse-grained alloy demonstrating higher fracture toughness compared to high-strength fine-grained alloys. These results and discussion show that variations in thermomechanical treatments can produce significant differences in microstructure and fracture toughness behavior of ferritic martensitic ODS steels.

36 MATERIALS SCIENCE↗

Cryogenically enhanced quasi-optical resonator for megawatt pulsed millimeter-wave sources

We report the design, cryogenic optimization, and performance modeling of a compact quasi-optical ring resonator intended to compress microwaves pulses at 170 and 250 GHz to the megawatt level. By combining ultra-low-loss CVD diamond and gold-doped silicon wafers with high-RRR copper mirrors, the calculated unloaded quality factor exceeds 4.3 × 10 5 at 20 K and yields simulated gains up to $\mathscr{G}$ = 4.1 × 10 3 . Coupling the resonator with a laser-driven semiconductor switch described by an extended Vogel model shows that 1 MW, nanosecond pulses can be generated from only 445 W of microwave drive power while dissipating 272 W into the cryostat. A practical cooling architecture using two Gifford–McMahon stages (20 and 80 K) is proposed, demonstrating that high-repetition-rate (10–20 kHz) operation is feasible with commercially available cryocoolers. The results outline a clear path toward cost-effective, table-top sources for extreme-ultraviolet lithography, dynamic nuclear polarization, and fusion systems.

Panisset, Constant [Ecole Polytechnique Federale L↗

The LIBRA Experiment: Investigating Robust Tritium Accountancy in Molten FLiBe Exposed to a D-T Fusion Neutron Spectrum

The Liquid Immersion Blanket: Robust Accountancy (LIBRA) experiment will be a first-of-a-kind experiment to explore and develop the liquid immersion blanket (LIB) concept. The LIB is a radically simple molten–LiF-BeF2 (FLiBe)–salt tritium breeding blanket for deuterium-tritium (D-T)–fueled fusion power plants (FPPs) achieving a high tritium breeding ratio (TBR) in neutronics models. However, tritium breeding in FLiBe is inherently difficult to study experimentally. As a result, the coupled issues of FLiBe radiochemistry and tritium (T) transport are poorly understood. LIBRA approaches this challenge by simulating an FPP blanket environment using a D-T neutron generator and ≈ 1000 kg of FLiBe. LIBRA will investigate T breeding, containment, and extraction, coupled with FLiBe redox control and radiochemistry. The primary goal of LIBRA is to demonstrate robust T accountancy in blanket prototypical conditions. Here, T accountancy encompasses accurate predictions of T breeding in the FLiBe; detection and measurement of all T bred in LIBRA; and speciation of the T extracted from the FLiBe. Initial neutronics simulations of LIBRA indicate that a global TBR of ~ 1 is possible, where the TBR is defined as the number of tritons bred and extracted from FLiBe relative to the number of neutrons produced by D-T fusion reactions in the neutron generator. In this paper, we present the LIBRA concept and its scientific goals in the context of T breeding experiments. We also consider the potential impact of the LIB on the future fusion power industry, motivating further development of FLiBe-based T breeding research activities such as LIBRA.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Request for Information: Access to Quantum Systems

Quantum science and technology is a focal point of research at Lawrence Livermore National Laboratory (LLNL). Quantum-coherent devices offer the potential for unprecedented precision in sensing and the ability to directly simulate complex quantum phenomena that have no known efficient classical algorithms. Thus, development and implementation of quantum technologies is expected to have a significant impact on our ability to address some of the most complex national security problems. LLNL maintains projects involving a broad spectrum of Quantum Information Science (QIS) research activities including investigating sources of decoherence, the 3DQ microscope, studies into quantum interconnects, 3-D printed ion traps, fusion energy and nuclear physics simulations, modeling for data-starved environments, and quantum sensing, including accelerometry and timing.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Demonstrating Advanced Sensors for In-Situ Monitoring Towards Qualification of Nuclear Relevant Components

The U.S. Department of Energy’s Office of Nuclear Energy Advanced Materials and Manufacturing Technologies (AMMT) program is pursuing qualification of laser powder bed fusion (LPBF) components for nuclear applications. A major focus of this effort is the use of in situ process monitoring and machine learning–based tools to establish real-time quality assurance. The primary objective of this report is to identify and evaluate the most relevant in situ sensor systems for LPBF, and to document the deployment of these systems across platforms critical to the AMMT program. This work demonstrates how in situ monitoring can detect process anomalies, track geometry-dependent flaws, and identify limiting combinations of processing parameters—particularly those related to energy density and complex geometries (e.g., overhanging structures). To support this goal, a diverse suite of sensor modalities was evaluated across LPBF platforms, including visible and near-infrared (NIR) imaging, fringe projection profilometry, long-wavelength infrared (LWIR) thermography, and high-speed photodiode/pyrometry systems. These sensor streams were integrated with Peregrine, a machine-agnostic software platform that, among other capabilities, can generate real-time process anomaly classification. This report documents sensor deployments on multiple AMMT flagship platforms, including the Concept Laser M2 and Renishaw AM400/AM250 systems. Calibration builds with complex, flaw-prone geometries such as unsupported overhangs, stepped features, and thin walls, were used to evaluate how well Peregrine and its associated sensors could detect process anomalies and other instabilities under varied energy densities. It will be shown how Peregrine reliably identifies common process anomalies such as recoater streaking, superelevation, etc., and can be used in post-build analysis for anomaly spatial distributions throughout the build height to better understand the impact of geometry and processing parameter choice on the build. This work demonstrates measurable progress toward the vision that components can be born-qualified by establishing a real-time monitoring framework, identifying limiting process conditions, and laying the foundation for sensor fusion–enabled prediction pipelines that are scalable across platforms and applicable to nuclear-relevant components.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Primary yields of protons measured using CR-39 in laser-induced deuteron–deuteron fusion reactions

The deuteron and deuteron (DD) fusion reactions is the most crucial reaction in the nuclear astrophysics and inertial confinement fusion, which is responsible for synthesizing chemical elements, and for powering the stellar evolution. The plasma environment generated by the high-intensity laser used in a DD fusion reaction is similar to the early stage of the Big Bang. Therefore, it is important to study laser-induced DD fusion reactions. Recently, we experimentally investigated such reactions using eight laser beams with the third harmonic impact on a deuterated polyethylene target at the ShenGuang-II Upgrade facility. In this work, we focused on the application of range-filter spectrometers assembled from a 70 μm aluminum filter and two CR-39 nuclear track detectors to measure the yields of primary DD protons. Based on the track diameter calibration results of 3 MeV protons used to diagnose the tracks on the range- filter spectrometers, we measured a primary DD proton yield of approximately (8:52 ± 1:7) × 10 6 , consistent with the yields from similar laser facilities worldwide, indicating that range-filter spectrometry is an effective way to measure primary DD protons. Furthermore, using other accurate detectors may help to measure the rare events of D 3 He protons.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Proton damage in (Y,Lu,Gd) 3 (Al,Ga) 5 O 12 :Ce mixed garnet scintillators

Scintillators are vital components for nuclear instrumentation and its applications, including plasma diagnostics and imaging. As yields in controlled fusion experiments increase, the radiation tolerance of scintillator candidates for use in instrumentation is of particular importance. High radiation exposure can damage scintillating materials and alter the optical properties. The effects of radiation damage in Ce-doped mixed garnet ceramics over the compositional range (Y,Gd,Lu) 3 (Al,Ga) 5 O 12 are investigated using optical techniques. The samples were exposed to 200 keV protons to an accumulated fluence of 10 16 protons per square centimeter, then characterized using diffuse reflectance spectroscopy (DRS). DRS with visible light can assess the radiation tolerance of opaque poly-crystalline samples, which can be easily sintered from powders and thus offer distinct advantages in characterization compared to single crystals. Qualitative trends in induced absorption are presented as a function of composition, and the ideal cerium dopant concentration for Y 2 LuAl 5 O 12 is determined to be 0.60–0.75 mol.%.

47 OTHER INSTRUMENTATION↗

Physics Flash Fall 2020

The Fall 2020 edition of Physics Flash includes article briefs on: Patrick Younk, Fusing concepts, technology to past performance of nuclear explosives; LANL inertial confinement fusion programs aims to develop burning plasma for weapons science; Lab's high energy nuclear physics explored at international conference; and, Novel study reveals new details on the impact of thermal interfaces in dynamic compression experiments.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Quantifying resonance behavior in the fusion of O 17 with C 12 at above-barrier energies

Recent measurement of the fusion excitation function for 17 O + 12 C reported the significant suppression of the fusion cross section at E c.m. ≈ 14 MeV. This suppression was hypothesized to signal the existence of a 16 O + n + 12 C molecular configuration. Using the active-target detector MuSIC@Indiana provided an effective means of reexamining the fusion excitation function for 17 O + 12 C.The accuracy of this thick-target measurement is strengthened through comparison with the thin-target measurement of the excitation function for 17 F + 12 C. Furthermore, the result provides important information about the dependence of the average fusion cross section for the oxygen isotopic chain on neutron excess.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Developing Capabilities in Physical and Computational Sciences

The Physical and Computational Sciences Directorate (PCSD) performs fundamental research in support of the science missions of Offices of Basic Energy Sciences (BES), Advanced Scientific Computing Research (ASCR), High Energy Physics (HEP), Nuclear Physics (NP), and Fusion Energy Sciences (FES), and others within the domains of the chemical, materials, computational sciences, mathematics, and physics. This LDRD project aims to provide funding to develop/demonstrate research capabilities for proposals and publications to support these science missions. Staff will propose small research tasks/projects to be performed under this overall project.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Laser Powder Bed Fusion Manufactured Alloys 625 and 282 and Properties Relevant to Advanced Nuclear Components

Under the Advanced Materials and Manufacturing Technologies program, two Ni-based alloys fabricated by laser powder bed fusion (LPBF) have been evaluated: γ′-strengthened Haynes 282 and solution-strengthened Inconel 625. Large printing defects were observed in the LPBF 282 alloy fabricated using a Renishaw AM250 machine, likely due to particle spattering during printing. Annealing at 1,180°C for 1 h followed by 4 h at 800°C in a high density of 50 nm γ′-strengthening precipitates as well as partial recrystallization resulted in a bimodal grain distribution. Creep testing performed at 750°C revealed lower creep life and ductility for the LPBF 282 compared with wrought 282. X-ray computed tomography combined with optical and scanning electron microscopy microstructural characterization revealed crack formation during creep testing, initiated either from printing defects or from creep cavitation at grain boundaries. Printing defects were the likely reason for the lower creep performance of LPBF 282 and could be suppressed by optimizing the build configuration. Printing 625 on an EOS M290 machine using the recommended EOS parameters resulted in a very low defect density. Superior creep strength at 725°C was observed for the as-printed LPBF 625 along the build direction when compared with wrought 625. No defect larger than ~50 µm could be detected by X-ray computed tomography in the as-printed conditions and after creep testing for 1,000 h at 725°C and 150 MPa. Small, needle-like δ-phase precipitates were observed after creep testing for 100 h at 725°C and 200 MPa. The rapid formation of the γ phase is directly related to the initial Nb and Mo segregation in the LPBF 625 cell walls, and its effect on the alloy’s high-temperature performance will be evaluated. Solution annealing was carried out at 1,150°C for 1 h and led to full recrystallization of the alloy. A decrease in strength and increase in ductility were observed after solution annealing, and the alloy recrystallization resulted in isotropic tensile properties at room temperature, contrary to what was observed for the as-printed LPBF 625.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Inertial-confinement fusion-plasma-based cross-calibration of the deuterium-tritium γ-to-neutron branching ratio

The deuterium-tritium (D-T) γ -to-neutron branching ratio [ H 3 ( d , γ ) He 5 / H 3 ( d , n ) He 4 ] has been determined previously under inertial-confinement fusion (ICF) conditions and in beam-target based experiments. In the former case, neutron-induced backgrounds are mitigated compared to the latter due to the short pulse nature of ICF implosions and the use of gas Cherenkov γ -ray detectors. Furthermore, an added benefit of ICF based measurements is the ability to achieve lower center-of-mass energies as compared to accelerators. Previous ICF based experiments however report a large uncertainty in the D-T γ -to-neutron branching ratio of ≈ 48 % , which arises from the necessity of an absolute detector calibration and/or a cross-calibration against the D- He 3 γ -to-proton branching ratio. A more precise value for the branching ratio based on data taken at the OMEGA laser facility is reported here, which relies on a cross-calibration against the better known C 12 neutron inelastic scattering cross section. A D-T branching ratio value of ( 4.6 ± 0.6 ) × 10 - 5 is determined by this method.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Theoretical uncertainty quantification for heavy-ion fusion

Despite recent advances and focus on rigorous uncertainty quantification for microscopic models of quantum many-body systems, the uncertainty on the dynamics of those systems has been underexplored. To address this, we have used time-dependent Hartree-Fock to examine the model uncertainty for a collection of low-energy, heavy-ion fusion reactions. Fusion reactions at near-barrier energies represent a rich test-bed for the dynamics of quantum many-body systems owing to the complex interplay of collective excitation, transfer, and static effects that determine the fusion probability of a given system. The model uncertainty is sizable for many of the systems studied and the primary contribution arises from static properties that are ill-constrained, such as the neutron radius of neutron-rich nuclei. Furthermore, these large uncertainties motivate the use of information from reactions to better constrain existing models and to infer static properties from reaction data.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Particle-in-cell simulations of burning inertial confinement fusion capsule implosions

Anomalies observed in the neutron spectral shift of high-yield shots at the National Ignition Facility (NIF) suggest the presence of suprathermal ions [E. P. Hartouni et al., Nat. Phys. 19, 72 (2023)], implying that kinetic effects play a significant role in burning inertial confinement fusion (ICF) plasmas. Furthermore, recent measurements of reaction-in-flight (RIF) neutrons offer a direct probe of the stopping power in the burning fuel region of high-energy alpha particles and up-scattered fuel ions. We have developed the particle-in-cell code PICNIC, an exactly energy-conserving particle-in-cell Monte-Carlo collision (PIC-MCC) code to simulate the burn stage in ICF. We present results from 1D spherical simulations of NIF shot N210808, which was the first to exceed the Lawson criterion for laser fusion. We find that the suprathermal ions generated by large-angle Rutherford and nuclear elastic scattering (NES) with fusion alphas produce an alpha knock-on neutron (AKN) signal consistent with the extent and relative yield of the AKN spectrum identified in ignition experiments at the NIF. Furthermore, we also find that the inclusion of large-angle scattering physics does not explain the anomalously large spectral shift observed in the experiment.

High-energy-density plasmas↗