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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 469 records · Page 26
All sourcesNASA NTRSDOE OSTI
DOE OSTI2026

Evidence of nonlinear coupling in the edge harmonic oscillation sustaining quiescent high confinement in a tokamak plasma

In a tokamak plasma, we measure nonlinear coupling between harmonics comprising a saturated edge oscillation, as predicted by nonlinear magnetohydrodynamic simulations. The coherent structure formed by this coupling suppresses bursty edge-localized modes that cause energy and particle loss. We also measure nonlinear coupling of the edge harmonic oscillation to core-resonant magnetic tearing modes. When tearing modes are present, the edge oscillation harmonics decouple, and edge-localized modes return. In this article, we conclude that nonlinear interaction with tearing modes interrupts the formation of the edge harmonic oscillation.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2025

Intermodal microwave-to-optical transduction using silicon-on-sapphire optomechanical ring resonator

Optomechanical and electro-optomechanical systems have emerged as one of the most promising approaches for quantum microwave-to-optical transduction to interconnect distributed quantum modalities for scaling the quantum systems. These systems use suspended structures to increase mode overlap and mitigate loss to achieve high efficiency. However, the suspended design’s poor heat dissipation under strong drive limits the ultimate efficiency. Here, we demonstrate an unsuspended optomechanical ring resonator (OMR) based on the silicon-on-sapphire (SOS) platform for microwave-to-optical frequency conversion. The OMR achieves a triply resonant optical-to-optical conversion with an enhanced coupling rateG b = 3.6 gigahertz per square-root milliwatt at a peak conversion efficiency of 1.2% with 3.6-milliwatt microwave drive power and a microwave-to-optical conversion efficiency of 1.5 × 10 −5 at 10-milliwatt optical drive power. Our results show that the unsuspended SOS platform, which mitigates the thermal effect and is compatible with superconducting qubits, is a promising platform for optomechanical circuitry and quantum transduction.

Science & Technology - Other Topics↗
DOE OSTI2020

Multi-Axis Resonant Plate Shock Testing Evaluation and Test Specification Development

Resonant plate testing is a shock test method that is frequently used to simulate pyroshock events in the laboratory. Recently, it was discovered that if the unit under test is installed at an off-center location, a tri-axial accelerometer would record a shock response in three directions and the resulting shock response spectra implied that the test may have qualified the component in three directions simultaneously. The purpose of this research project was to evaluate this idea of multi-axis shock testing to determine if it was truly a multi-axis shock environment and if such a test could be used as an equivalent component qualification test. A study was conducted using generic, additively manufactured components tested on a resonant plate, along with an investigation of plate motion to evaluate the component response to off- center plate excitation. The data obtained here along with the analytical simulations performed indicate that off-center resonant plate tests are actually not three-axis shock tests, but rather single axis shocks at an arbitrary angle dictated by the location of the unit under test on the plate. This conclusion is supported by the fact that only one vectored shock input is provided to the component in a resonant plate test. Thus, the output response is a coupled response of the transverse plate vibration and the rotational motion of the component on the plate. Additionally, a multi-axis shock test defined by three single axis test environments always results in a significant component over-test in one direction.

42 ENGINEERING↗
DOE OSTI2024

Introduction to Special Issue on the Early History of Nuclear Fusion

This introductory paper to the special issue of Fusion Science and Technology commemorates early research on fusion conducted at Los Alamos (the singular entity denoted Los Alamos Laboratory/Los Alamos Scientific Laboratory/Los Alamos National Laboratory at different times is designated “Los Alamos” in this paper) in support of the eventual H-bomb program. We survey the historical origins of the thermonuclear program, what was known of fusion reactions at the outbreak of the war, and the remarkable breakthroughs involving particularly the prospect of deuterium-tritium (DT) reactions conducted during the war, and we summarize the papers in this volume. Much of the nuclear fusion technical history presented herein has not been previously reported. Papers describe aspects of fusion science during these days, on shock hydrodynamics and on electron-radiation coupling, and on nuclear physics including the discoveries of resonances in both the DT cross section and in the lithium tritium-breeding cross section. Three papers follow our colleague Mark Paris’s finding Arthur Ruhlig’s 1938 paper on the first observation of DT fusion: one on how it influenced subsequent Manhattan Project research, another on a modern calculation of that historic experiment, and a third that has repeated the experiment using modern experimental capabilities. Other papers discuss how the first H-bomb test, Ivy Mike, led to the discovery of the new elements einsteinium and fermium and how the DT fusion processes played a key role in our universe’s development after the Big Bang. We also present a paper that analyzes the pioneering Cambridge University 1934 experiment by Marcus Oliphant, Paul Harteck, and Ernest Rutherford where deuterium-deuterium fusion was first observed and that describes how Ernest Lawrence missed identifying fusion in 1933. Finally, we present a summary of early concepts for controlled fusion energy that grew out of wartime discussions at Los Alamos. The papers show how J. Robert Oppenheimer played a leading technical role in the early developments of the H-bomb, before his later opposition—our first paper in this issue addresses the U.S. Department of Energy’s 2022 vacation of the earlier 1954 decision to revoke his security clearance.

45 MILITARY TECHNOLOGY, WEAPONRY, AND NATIONAL DEF↗
DOE OSTI2024

Trapping light in air with membrane metasurfaces for vibrational strong coupling

Optical metasurfaces can manipulate electromagnetic waves in unprecedented ways at ultra-thin engineered interfaces. Specifically, in the mid-infrared (mid-IR) region, metasurfaces have enabled numerous biochemical sensing, spectroscopy, and vibrational strong coupling (VSC) applications via enhanced light-matter interactions in resonant cavities. However, mid-IR metasurfaces are usually fabricated on solid supporting substrates, which degrade resonance quality factors (Q) and hinder efficient sample access to the near-field electromagnetic hotspots. Besides, typical IR-transparent substrate materials with low refractive indices, such as CaF 2 , NaCl, KBr, and ZnSe, are usually either water-soluble, expensive, or not compatible with low-cost mass manufacturing processes. Here, we present novel free-standing Si-membrane mid-IR metasurfaces with strong light-trapping capabilities in accessible air voids. We employ the Brillouin zone folding technique to excite tunable, high-Q quasi-bound states in the continuum (qBIC) resonances with our highest measured Q-factor of 722. Leveraging the strong field localizations in accessible air cavities, we demonstrate VSC with multiple quantities of PMMA molecules and the qBIC modes at various detuning frequencies. Our new approach of fabricating mid-IR metasurfaces into semiconductor membranes enables scalable manufacturing of mid-IR photonic devices and provides exciting opportunities for quantum-coherent light-matter interactions, biochemical sensing, and polaritonic chemistry. The authors introduce a mid-IR metasurface fabricated by decorating a free-standing Si-membrane with air holes. The enhanced light-matter interactions in such air cavities enable vibrational strong coupling and advanced biochemical sensing.

infrared spectroscopy↗
DOE OSTI2021

Properties of isoscalar giant multipole resonances in medium-heavy closed-shell nuclei: A semimicroscopic description

The semimicroscopic particle-hole dispersive optical model (PHDOM) is implemented to describe main properties of Isoscalar Giant Multipole Resonances (up to L=3) in medium-heavy closed-shell nuclei. Here, the main properties are characterized by the strength distribution, transition density, partial and total probabilities of direct one-nucleon decay. Calculation results obtained for the 208 Pb nucleus are compared with available experimental data.

190 ≤ A ≤ 219↗
DOE OSTI2020

Coupling between plasmonic and photonic crystal modes in suspended three-dimensional meta-films

A complementary metal oxide semiconductor (CMOS) compatible fabrication method for creating three-dimensional (3D) meta-films is presented. In contrast to metasurfaces, meta-films possess structural variation throughout the thickness of the film and can possess a sub-wavelength scale structure in all three dimensions. Here we use this approach to create 2D arrays of cubic silicon nitride unit cells with plasmonic inclusions of elliptical metallic disks in horizontal and vertical orientations with lateral array-dimensions on the order of millimeters. Fourier transform infrared (FTIR) spectroscopy is used to measure the infrared transmission of meta-films with either horizontally or vertically oriented ellipses with varying eccentricity. Shape effects due to the ellipse eccentricity, as well as localized surface plasmon resonance (LSPR) effects due to the effective plasmonic wavelength are observed in the scattering response. The structures were modeled using rigorous coupled wave analysis (RCWA), finite difference time domain (Lumerical), and frequency domain finite element (COMSOL). The silicon nitride support structure possesses a complex in-plane photonic crystal slab band structure due to the periodicity of the unit cells. We show that adjustments to the physical dimensions of the ellipses can be used to control the coupling to this band structure. The horizontally oriented ellipses show narrow, distinct plasmonic resonances while the vertically oriented ellipses possess broader resonances, with lower overall transmission amplitude for a given ellipse geometry. We attribute this difference in resonance behavior to retardation effects. The ability to couple photonic slab modes with plasmonic inclusions enables a richer space of optical functionality for design of metamaterial-inspired optical components.

42 ENGINEERING↗
DOE OSTI2020

Penetration Through Slots in Cylindrical Cavities Operating at Fundamental Cavity Modes

In this article, we examine the coupling into an electrically short azimuthal slot on a cylindrical cavity operating at fundamental cavity modal frequencies. We first develop a matched bound formulation through which we can gather information for maximum achievable levels of interior cavity fields. Actual field levels are below this matched bound; therefore, we also develop an unmatched formulation for frequencies below the slot resonance to achieve a better insight on the physics of this coupling. Good agreement is observed between the unmatched formulation, full-wave simulations, and experimental data, providing a validation of our analytical models. We then extend the unmatched formulation to treat an array of slots, found again in good agreement with full-wave simulations. These analytical models can be used to investigate ways to mitigate electromagnetic interference and electromagnetic compatibility effects within cavities.

42 ENGINEERING↗
DOE OSTI2022

Magnetoelastic properties of multiferroic hexagonal ErMnO 3

Here, the strength and dynamics of magnetoelastic coupling through the paramagnetic (PM) – antiferromagnetic (AFM) – ferrimagnetic (FIM) transitions in multiferroic hexagonal ErMnO 3 have been investigated by Resonant Ultrasound Spectroscopy. Elastic stiffening by up to 2% below the PM – AFM transition at 80 K arises from biquadratic coupling between strain and the magnetic order parameter with relaxation times longer than ~10 -6 s for the response of spins to changes in strain. In contrast with YMnO 3 , the PM – AFM transition in ErMnO 3 is accompanied by a peak in acoustic loss immediately below the Néel point which is interpreted in terms of strain relaxation accompanying ordering of spins of Er 3+ at 4b sites. Changes in the magnetic ordering scheme at the AFM – FIM transition near 3 K are accompanied by elastic softening of ~0.03 %. During poling of the low temperature ferrimagnetic structure round magnetic hysteresis loops, small changes in elastic stiffness which arise due to the contribution of piezomagnetic and/or piezoelectric moduli are detected. Contributions of piezoelectric moduli to acoustic resonance frequencies also permit changes in the configuration of ferroelectric domains to be detected in response both to cycling through this transition and to application of a magnetic field. A peak in acoustic loss in the vicinity of 250 K is attributed to strain-mediated pinning/freezing of some aspect of the domain microstructure with an activation energy of ~0.25–0.3 eV. A return to the original elastic properties on heating to temperatures above ~250 K is interpreted in terms of backswitching of domains to the configuration they had at the start. These observations confirm the existence of subtle variations in magnetoelastic coupling behaviour relating to both the magnetic order parameters and magnetic domain structures.

36 MATERIALS SCIENCE↗
DOE OSTI2026

Combination of searches for heavy vector boson resonances in proton-proton collisions at $\sqrt{s}=13$ TeV

A combined statistical analysis of searches for heavy vector boson resonances decaying into pairs of W, Z, or Higgs bosons, as well as into quark pairs $\left(\mathrm{q}\overline{\mathrm{q}},\mathrm{b}\overline{\mathrm{b}},\mathrm{t}\overline{\mathrm{t}},\mathrm{t}\overline{\mathrm{b}}\right)$ or lepton pairs ℓ + ℓ – , ℓ$\bar{v}$, with ℓ = e, μ, τ, is presented. The results are based on proton-proton collision data at a center-of-mass energy of 13 TeV, corresponding to an integrated luminosity of 138 fb −1 , collected by the CMS experiment from 2016 to 2018. No significant deviation from the expectations of the standard model is observed. The results are interpreted in the simplified heavy vector triplet (HVT) framework, setting 95% confidence level upper limits on the production cross sections and on the coupling strengths of the HVT bosons to standard model particles. The results exclude HVT resonances with masses below 5.5 TeV in a weakly coupled scenario, below 4.8 TeV in a strongly coupled scenario, and up to 2.0 TeV in the case of production via vector boson fusion. The combination provides the most stringent constraints to date on new phenomena predicted by the HVT model.

beyond Standard Model↗
DOE OSTI2025

Cryogenic hybrid magnonic circuits based on spalled YIG thin films

Yttrium iron garnet (YIG) magnonics has garnered significant research interest because of the unique properties of magnons (quasiparticles of collective spin excitation) for signal processing. In particular, hybrid systems based on YIG magnonics show great promise for quantum information science due to their broad frequency tunability and strong compatibility with other platforms. However, their broad applications have been severely constrained by substantial microwave loss in the gadolinium gallium garnet (GGG) substrate at cryogenic temperatures. In this study, we demonstrate that YIG thin films can be spalled from YIG/GGG samples. Our approach is validated by measuring hybrid devices comprising superconducting resonators and spalled YIG films, which exhibit anti-crossing features that indicate strong coupling between magnons and microwave photons. Such new capability of separating YIG thin films from GGG substrates via spalling and the integrated superconductor-YIG devices represent a significant advancement for integrated magnonic devices, paving the way for advanced magnon-based coherent information processing.

36 MATERIALS SCIENCE↗
DOE OSTI2026

Mechanistic implications of excited high-spin states, spin–spin coupling, and differential [2Fe–2S] + cluster temperature relaxations in the electron-bifurcating NfnABC from Thermococcus sibiricus

Electron bifurcation (EB) is a mechanism of biological energy transduction in which multiple oxidation–reduction (redox) reactions are thermodynamically coupled within a single enzyme, enabling the enzyme to harness the excess free energy from an exergonic process to drive an endergonic process. Because of this unprecedented chemistry, there is interest to translate EB principles to artificial and bioengineered systems, but a hurdle is that knowledge pertaining to the fundamental design principles of EB enzymes remains scarce. Here, we investigated the fundamental physical and electronic properties of electron transfer sites in a spectroscopically uncharacterized member of the BfuABC family of EB enzymes, the NADH-dependent reduced-ferredoxin:NADP + oxidoreductase from Thermococcus sibiricus (Tsi NfnABC). Cryo-EM structures of Tsi NfnABC previously demonstrated that it contains twelve redox cofactors: two flavins (one FAD and one FMN), eight [4Fe–4S] clusters, and two [2Fe–2S] clusters. The FMN, one [4Fe–4S] cluster, and one [2Fe–2S] cluster comprise the bifurcating active site termed the electron-bifurcating flavobicluster (BF-FBC), which is found in all BfuABC family members. By using electron paramagnetic resonance spectroscopy, we identified spectral signatures originating from interactions between the FMN radical and [4Fe–4S] + cluster in the BF-FBC and observed temperature dependent behavior of the BF-FBC's [2Fe–2S] + cluster indicative of moderately slow spin–lattice relaxation. Additionally, we uncovered numerous spectral features corresponding to half-integer, S > ½ spin states of [4Fe–4S] + clusters, including one attributable to the consequences of lysine-ligation of a [4Fe–4S] cluster unique to NfnABC. We contextualize these findings to electron transfer theory and NfnABC's structure. Our insights further the understanding of how enzymes are designed to exert control over electron transfer to conduct thermodynamically challenging reactions.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗
DOE OSTI2025

Beehive haloscope for high-mass axion dark matter

We propose a new haloscope geometry that can arbitrarily increase the resonator volume for a given target axion mass. This geometry consists of closely packed, overlapping coaxial cavities operating as a single resonator. While the resonant frequency is still determined by the dimensions of the individual “cells,” the strong interactions between the cells encourage the entire “beehive” to oscillate in phase, a phenomenon expected of tightly coupled harmonic oscillators. This synchronization behavior allows the construction of a singly connected large volume resonator at high frequency by simply increasing the number of the cells. Using direct numerical simulations, we verify the existence of a global eigenmode that has a high (40%) form factor in a 169-element beehive resonator. The resonant frequency of the eigenmode is tunable by moving the center rods laterally in unison. The form factor is very tolerant to dimensional deviations and misalignment as a result of mode hybridization due to strong coupling. The beehive haloscope inherits many appealing properties from the conventional coaxial cavity: a high quality factor, compatibility with a solenoid magnet, and ease of fabrication, tuning, and coupling. We argue that this geometry is an excellent candidate for high-mass axion searches covering the post-inflationary parameter space (>5 GHz).

47 OTHER INSTRUMENTATION↗
DOE OSTI2022

Electronic structure of the frustrated diamond lattice magnet NiRh 2 O 4

We report the A -site spinel NiRh 2 O 4 is the only known realization of a spin-1 diamond lattice magnet and is predicted to host unconventional magnetic phenomena driven by frustrated nearest and next-nearest neighbor exchange as well as orbital degeneracy. Previous works found no sign of magnetic order but found a gapped dispersive magnetic excitation indicating a possible valence bond magnetic ground state. However, the presence of many competing low energy degrees of freedom and limited empirical microscopic constraints complicates further analysis. Here we carry out resonant inelastic x-ray scattering (RIXS), x-ray absorption spectroscopy (XAS), and inelastic neutron scattering (INS) to characterize the local electronic structure and lattice dynamics of NiRh 2 O 4 . The RIXS data can be partly described by a single-ion model for tetrahedrally coordinated Ni 2+ and indicates a tetragonal distortion Δt 2 = 70 meV that splits the t 2 orbitals into a high energy orbital singlet and lower energy orbital doublet. We identify features of the RIXS spectra that are consistent with a Rh-Ni two-site excitation indicating strong metal-metal hybridization mediated by oxygen in NiRh 2 O 4 . We also identify signatures of electron-phonon coupling through the appearance of phonon sidebands that dress crystal field excitations. These results establish the key energy scales relevant to the magnetism in NiRh 2 O 4 and further demonstrate that covalency and lattice dynamics play essential roles in controlling the magnetic ground states of A -site spinels.

36 MATERIALS SCIENCE↗
DOE OSTI2026

Er Al :Al 2 ⁢O 3 for telecom-band photonics: Electronic structure and optical properties

Er-doped Al 2 ⁢O 3 is a promising host for telecom-band integrated photonics. Here, in this study, we combine ab initio calculations with a symmetry-resolved analysis to elucidate substitutional Er on the Al site (Er Al ) in 𝛼−Al 2 ⁢O 3 . First-principles relaxations confirm the structural stability of Er Al . We then use the local trigonal crystal-field symmetry to classify the Er-derived impurity levels by irreducible representations and to derive polarization-resolved electric-dipole selection rules, explicitly identifying the symmetry-allowed 𝑓−𝑑 hybridization channels. Kubo-Greenwood absorption spectra computed from Kohn-Sham states quantitatively corroborate these symmetry predictions. Furthermore, we connect the calculated intra-4⁢𝑓 line strengths to Judd-Ofelt theory, clarifying the role of 4⁢𝑓−5⁢𝑑 admixture in enabling optical activity. Notably, we predict a characteristic absorption near 1.47 µ⁢m (telecom band), relevant for on-chip amplification and emission. To our knowledge, a symmetry-resolved first-principles treatment of Er:Al 2 ⁢O 3 with an explicit Judd-Ofelt interpretation has not been reported, providing a transferable framework for tailoring rare-earth dopants in wide-band-gap oxides for integrated photonics. Our results for the optical spectra are in good agreement with experimental data. The resulting symmetry-based selection rules translate directly to polarization-dependent coupling in Al 2 ⁢O 3 integrated photonic waveguides and resonators, enabling device-level design of TE/TM-mode interaction with Er emitters in the 1.5-µ⁢m telecom band.

Er-doped Al2O3↗
DOE OSTI2022

Structural Chirality of Polar Skyrmions Probed by Resonant Elastic X-Ray Scattering

An escalating challenge in condensed-matter research is the characterization of emergent orderparameter nanostructures such as ferroelectric and ferromagnetic skyrmions. Their small length scales coupled with complex, three-dimensional polarization or spin structures makes them demanding to trace out fully. Resonant elastic x-ray scattering (REXS) has emerged as a technique to study chirality in spin textures such as skyrmions and domain walls. It has, however, been used to a considerably lesser extent to study analogous features in ferroelectrics. Here, in this study, we present a framework for modeling REXS from an arbitrary arrangement of charge quadrupole moments, which can be applied to nanostructures in materials such as ferroelectrics. With this, we demonstrate how extended reciprocal space scans using REXS with circularly polarized x rays can probe the three-dimensional structure and chirality of polar skyrmions. Measurements, bolstered by quantitative scattering calculations, show that polar skyrmions of mixed chirality coexist, and that REXS allows valuation of relative fractions of right- and left-handed skyrmions. Our quantitative analysis of the structure and chirality of polar skyrmions highlights the capability of REXS for establishing complex topological structures toward future application exploits.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2021

Tuning Hybrid exciton–Photon Fano Resonances in Two-Dimensional Organic–Inorganic Perovskite Thin Films

As easy-to-grow quantum wells with narrow excitonic features at room temperature, two-dimensional (2D) Ruddleson–Popper perovskites are promising for realizing novel nanophotonic devices based on exciton–photon interactions. Here, we demonstrate a distinct hybrid exciton–photon Fano resonance in (C 4 H 9 NH 3 ) 2 PbI 4 thin films prepared via spin coating. Using a classical coupled-oscillator model and finite-difference time-domain simulations, we link the Fano interference to the coupling of the exciton with the Rayleigh-like scattering of the film microstructure. Combining colloidal plasmonic cavities with the 2D perovskite films, we demonstrate tuning of the Fano resonance. In combination with silver nanoparticles, the exciton–photon Fano interference couples to the in-plane plasmonic modes with indications of Rabi splitting. By creating a nanoparticle on mirror geometry, we address the out-of-plane excitonic component, reaching an intermediate coupling regime. Furthermore, these structures suggest possible photonic targets for biomolecular self-assembly applications.

2D perovskites↗
DOE OSTI2024

Bayesian optimization of Fisher Information in nonlinear multiresonant quantum photonics gyroscopes

Abstract We propose an on-chip gyroscope based on nonlinear multiresonant optics in a thin film χ (2) resonator that combines high sensitivity, compact form factor, and low power consumption simultaneously. We theoretically analyze a novel holistic metric – Fisher Information capacity of a multiresonant nonlinear photonic cavity – to fully characterize the sensitivity of our gyroscope under fundamental quantum noise conditions. Leveraging Bayesian optimization techniques, we directly maximize the nonlinear multiresonant Fisher Information. Our holistic optimization approach orchestrates a harmonious convergence of multiple physical phenomena – including noise squeezing, nonlinear wave mixing, nonlinear critical coupling, and noninertial signals – all encapsulated within a single sensor-resonator, thereby significantly augmenting sensitivity. We show that ∼ 470 × $\sim 470{\times}$ improvement is possible over the shot-noise limited linear gyroscope with the same footprint, intrinsic quality factors, and power budget.

42 ENGINEERING↗