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At least 469 records · Page 26
All sourcesNASA NTRSDOE OSTI
NASA NTRS1974

Ion-molecule reactions and vibrational deactivation of H2/+/ ions in mixtures of hydrogen and helium

Use of ion cyclotron resonance methods to measure the thermal energy rate constants for a number of ion-molecule reactions involving hydrogen and hydrogen-helium mixtures. Assuming that the distribution of initial vibrational states in the H2(+) ion is a near-Franck-Condon distribution, the occurrence of collisional deactivation of vibrationally excited H2(+) ions by He atoms is identified, and an approximate rate constant for the deactivation process and its dependence on vibrational energy are given.

Theard, L. P.↗
NASA NTRS1974

Plasmaspheric hiss intensity variations during magnetic storms

The storm time intensity variations of ELF electromagnetic emissions have been studied by using the Ogo 6 search coil magnetometer. Low-latitude signals exhibit a sharp low-frequency cutoff and are identified as plasmaspheric hiss. Such waves show pronounced intensification during the recovery phase of magnetic storms but remain close to background levels during the storm main phase. This behavior is consistent with cyclotron resonant generation within the plasmasphere as the latter expands into the intensified belt of outer zone electrons during the storm recovery.

Smith, E. J.↗
NASA NTRS1974

ICR study of nonreactive ion-molecule collision rate constants for Cl/-/ and Cr/CO/5/-/

Determination of experimental momentum transfer rate constants for systems of Cl(-) and Cr(CO)5(-) ions by means of an ion cyclotron resonance (ICR) line-broadening technique. It is found that in the pure polarization limit of small ion/large neutral collisions the Langevin ion mobility theory gives good agreement with experimental results. A comparison of isotropic and anisotropic neutral systems suggests that a correction for the anisotropic systems is necessary. Beyond the pure polarization limit the Langevin theory gives poor predictions for ion mobilities. The adjustable parameter, gamma, of the Mason-Schamp (12-6-4) potential function permits unique solution of the ion mobility for Cr(CO)5(-) in a wide range of neutral gases. The large values of gamma obtained for most of these systems imply, in terms of the Mason-Schamp theory, that the r to the minus 6th power contribution to the potential function is significant.

Dymerski, P. P.↗
NASA NTRS1974

Intensity variation of ELF hiss and chorus during isolated substorms

Electromagnetic ELF emissions (100-1000 Hz) observed on the polar-orbiting OGO-6 satellite within three hours of the dawn-dusk meridian consistently exhibit a predictable response to isolated substorm activity. Near dawn, the emissions intensify during the substorm and then subside following the magnetic activity; the waves are most intense at L greater than 4, exhibit considerable structure and have been primarily identified as chorus. At dusk the response is entirely different; the wave intensity falls to background levels during substorm activity but subsequently intensifies, usually reaching levels well in excess of that before the disturbance. The emissions near dusk extend to low L, are relatively featureless, and have been identified as plasmaspheric hiss. These features are interpreted in terms of changes in the drift orbits of outer-zone electrons which cyclotron resonate with ELF waves.

Thorne, R. M.↗
NASA NTRS1974

Midday Pc 1-2 pulsations observed at a subcleft location

A class of unstructured Pc 1-2 pulsation activity, as identified on Bar I (70.2 N) records taken during 1968-1972, is found to be present in midday hours on about half of the days in summer months. The events have some tendency to occur in the later part of the ring current recovery phase, especially at times of moderate AE when the cleft lines are just poleward of Bar I. The source lines of the Pc 1-2 are found to lie essentially outside the plasmapause. In terms of the proton cyclotron resonance instability the most likely source regions of the Bar I Pc 1-2 are the detached plasma regions convecting sunward on the dayside and the portion of the cleft plasma on the last closed field lines.

Heacock, R. R.↗
NASA NTRS1974

Reactions of ions in excited electronic states - Excited N2/+/ ion reacting with N2 to yield N3/+/ and N

Study of the mechanism of formation of the N3(+) ion from the bimolecular reaction of excited N2(+) ions in gaseous N2. Using ion cyclotron resonance spectroscopy, an attempt is made to inquire more deeply than hitherto into the origin of the N3(+) ions and to determine the rate constant for their formation and the limits on the lifetime of the reactant excited N2(+) ions.

Bowers, M. T.↗
NASA NTRS1975

Plasmaspheric hiss observations in the evening and afternoon quadrants

Data obtained with an Explorer-45 instrument for detecting the magnetic components of ELF signals propagating in the magnetosphere are examined, showing that the strongest, most persistent signals were plasmaspheric hiss from a few hundred to a few thousand Hertz. Broad-band signals of 25 milligamma were common. The most intense hiss was observed in the recovery phase of magnetic storms at the inner edge of the ring current. Its source appears to be the outer plasmasphere. Most of the hiss is attributed to generation of hiss through cyclotron resonance with energetic electrons. Ring current protons, forming a peak in the proton flux between 10 and 100 keV, may be a source of some of the hiss.

Parady, B. K.↗
NASA NTRS1975

Hydromagnetic waves and cosmic-ray diffusion theory

Pitch-angle (and energy) diffusion of cosmic rays in hydromagnetic wave fields is considered. The treatment remains strictly within the quasi-linear approximation. It is shown that the popular assumption of an isotropic power spectrum tensor of magnetic fluctuations requires in this case equal forms and magnitudes of Alfven and magnetosonic wave spectra - a situation which is generally unlikely. The relative contributions to the pitch-angle diffusion coefficient from the cyclotron resonances and Landau resonance due to the different types of waves are evaluated for a typical situation in the solar wind. Since the Landau resonance in this approximation also does not lead to particle reflections, a proper consideration of the nonlinear particle orbits is indeed necessary to overcome the well-known difficulties of quasi-linear scattering theory for cosmic rays near 90 deg pitch angle.

Lee, M. A.↗
NASA NTRS1975

Mid-latitude VLF emissions observed in the topside ionosphere

Narrow-band VLF emissions observed on different days by Alouette-2 are described. It is found that narrow-band VLF hiss (3.5-7.0 kHz) occurs at midlatitudes (at 54 to 64 deg) in the topside ionosphere during both the geomagnetically disturbed and quiet periods, although the hiss region moves towards the auroral zone during the disturbed period. It is likely that the midlatitude hiss at around 5 kHz is the origin of the narrow-band hiss (5 plus or minus 1 kHz) often observed at ground stations at low latitudes, since no VLF emissions above 2 kHz appear in the auroral zone. The midlatitude VLF hiss observed in the topside ionosphere may be generated by the transverse (electron cyclotron) resonance instability in the magnetosphere.

Ondoh, T.↗
NASA NTRS1975

Hydromagnetic waves and cosmic ray diffusion theory

Pitch angle diffusion of cosmic rays in hydromagnetic wave fields is considered strictly within the quasilinear approximation. It is shown that the popular assumption of an isotropic power spectrum tensor of magnetic fluctuations requires in this case equal forms and magnitudes of Alfven and magnetosonic wave spectra - a situation which is generally unlikely. The relative contributions to the pitch angle diffusion coefficient from the cyclotron resonances and Landau resonance due to the different types of waves are evaluated for a typical situation in the solar wind. Since in this approximation also the Landau resonance does not lead to particle reflections a proper consideration of the nonlinear particle orbits is indeed necessary to overcome the well known difficulties of quasilinear scattering theory for cosmic rays near 90 degrees pitch angle.

Lee, M. A.↗
NASA NTRS1976

Measurement and significance of the equilibrium reaction C-13/+/ + /C-12/O yields C-12/+/ + /C-13/O for alteration of the C-13/C-12 ratio in interstellar molecules

Laboratory measurements using the ion-cyclotron resonance technique yield a rate constant of 2 by 10 to the -10th power cu cm/sec at 300 K for the isotope exchange C-13(+) + (C-12)O yields C-12(+) + (C-13)O. According to the usual ideas about ion-molecule reactions, this rate constant should also be appropriate at temperatures not exceeding about 100 K. Then the observed C-13/C-12 ratio obtained from radio observation of interstellar molecules may be either larger or smaller than the actual value in the interstellar medium by factors of 2 or so. If the ratio is altered from the actual interstellar value, it will not be the same in all molecules, and CO will tend to have the highest value. The chief astronomical uncertainty for the occurrence of this isotope fractionation is the abundance of 'unobservable' molecules which can react rapidly with C(+): e.g., O2, H2O, CO2, and CH4. If their abundance is greater than about one-tenth that of CO, the isotope fractionation will be inhibited.

Watson, W. D.↗
NASA NTRS1976

On the reaction of N/+/ ions with O2

The reaction of atomic nitrogen ions with molecular oxygen is a major loss mechanism for N(+) ions in the ionosphere and is a source of NO(+) ions and atomic nitrogen at certain altitudes. Ion cyclotron resonance methods are used to measure the product distribution of thermal energy N(+) ions reacting with O2. Three product channels are identified with the following fractional distributions: O2(+) + N, 0.65 plus or minus 0.04; NO(+) + O, 0.31 plus or minus 0.04; O(+) + NO, 0.04 plus or minus 0.02.

Huntress, W. T., Jr.↗
NASA NTRS1976

A statistical study of Pc 1 magnetic pulsations at synchronous orbit

The statistical properties of Pc 1 magnetic pulsations at synchronous orbit are examined by using measurements obtained with the UCLA flux-gate magnetometer on board ATS 1. In 1967, 121 intervals of Pc 1 activity occurred. These events typically had amplitudes of 1-7 gamma and periods of 2-5 sec. Most events lasted less than 30 min and occurred in the afternoon sector. Pc 1 waves were more probable during the main phase of a geomagnetic storm, within 1 hour of a substorm expansion. While they do not have the signature of IPDP (intervals of pulsations of diminishing periods) events at ATS, simultaneous ground records show the occurrence of rising frequency tones characteristic of IPDP events in seven out of ten cases. The wave frequency ranged principally from 0.1 to 0.2 of the local proton gyrofrequency, similar to observations of electron cyclotron waves. The observed Pc 1 activity is consistent with the generation by cyclotron resonance of 30-keV protons in a 30/cu cm plasma.

Bossen, M.↗
NASA NTRS1976

Mass spectrometry

Advances in mass spectrometry (MS) and its applications over the past decade are reviewed in depth, with annotated literature references. New instrumentation and techniques surveyed include: modulated-beam MS, chromatographic MS on-line computer techniques, digital computer-compatible quadrupole MS, selected ion monitoring (mass fragmentography), and computer-aided management of MS data and interpretation. Areas of application surveyed include: organic MS and electron impact MS, field ionization kinetics, appearance potentials, translational energy release, studies of metastable species, photoionization, calculations of molecular orbitals, chemical kinetics, field desorption MS, high pressure MS, ion cyclotron resonance, biochemistry, medical/clinical chemistry, pharmacology, and environmental chemistry and pollution studies.

Burlingame, A. L.↗
NASA NTRS1977

Calibration of marginal oscillator sensitivity for use in ICR spectrometry

A constant-reference load is utilized as Q-spoiler in calibrations of relative sensitivity variations of a marginal oscillator with frequency. Frequency-dependent effects troublesome in earlier Q-spoilers are compensated by employing a pure resistive calibration load with compensation for the small distributed capacitance of large resistors. The validity of the approach is demonstrated for a 2:1 mass ratio range, and validity for a mass ratio range greater than 10:1 is claimed. The circuit and technique were developed for use in ion cyclotron resonance (ICR) spectrometric practice.

Anicich, V. G.↗
NASA NTRS1977

Product distributions for some thermal energy charge transfer reactions of rare gas ions

Ion cyclotron resonance methods were used to measure the product distributions for thermal-energy charge-transfer reactions of He(+), Ne(+), and Ar(+) ions with N2, O2, CO, NO, CO2, and N2O. Except for the He(+)-N2 reaction, no molecular ions were formed by thermal-energy charge transfer from He(+) and Ne(+) with these target molecules. The propensity for dissociative ionization channels in these highly exothermic charge-transfer reactions at thermal energies contrasts with the propensity for formation of parent molecular ions observed in photoionization experiments and in high-energy charge-transfer processes. This difference is explained in terms of more stringent requirements for energy resonance and favorable Franck-Condon factors at thermal ion velocities.

Anicich, V. G.↗
NASA NTRS1978

Plasma waves in the polar cusp - Observations from Hawkeye 1

Based on data from the Hawkeye 1 spacecraft in the polar-cusp vicinity, the characteristics of plasma waves are studied. Four types of plasma waves are identified: (1) a band of ULF-ELF magnetic noise, (2) broadband electrostatic emissions with maximum intensities at 10-50 Hz, (3) electrostatic electron cyclotron waves near electron gyrofrequency, and (4) whistler mode auroral hiss emissions. Only ULF-ELF noise is a reliable index of the polar cusp region. Since ULF-ELF magnetic noise extends only to the local electron gyrofrequency, it is suggested that the noise consists of whistler-mode electromagnetic waves. Possible mechanisms for this noise include the whistler-mode cyclotron-resonance, Kelvin-Helmholtz, and drift-wave instabilities. It is felt that a current-driven electrostatic instability causes the broadband electrostatic noise.

Gurnett, D. A.↗
NASA NTRS1978

Adiabatic modulation of equatorial pitch angle anisotropy

Particle measurements from the geostationary ATS 6 satellite reveal striking equatorial pitch-angle anisotropies. A study of seven days of data shows a diurnal variation in anisotropy with the particle flux at a pitch angle of 40 deg greater than that at 90 deg during times of low magnetic-field intensity on the nightside and vice versa during times of high magnetic-field intensity on the dayside. Six representative anisotropy events are studied in finer detail. The 32- to 51-keV electron anisotropies increase and decrease with the total magnetic-field intensity. The proton and higher-energy electron anisotropies do not show as much variation. The particle anisotropies are studied in light of adiabatic and cyclotron resonance theory; the results indicate that adiabatic effects are the dominant modulation mechanism of particle pitch-angle distributions in the outer radiation belt

Kaye, S. M.↗