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At least 451 records · Page 25

Radiocarbon Fingerprinting Black Carbon Source History in the Himalayas

Abstract Black carbon (BC) is considered as an important contributor to the Himalayan glaciers melt in the past few decades. However, the long‐term source apportionment of BC remains unclear. Here we present the first radiocarbon ( 14 C)‐based annual variation of BC source apportionment in an ice core spanning the period of 1959–2012 drilled from the Southeastern Tibetan Plateau, a receptor site of South Asia outflow. We find fossil fuel combustion is a major contribution (73% ± 5%), yet the biomass burning fraction ( ƒ biomass ) has grown from 24% ± 4% to 30% ± 4% since 1990. Intriguingly, we further find the ƒ biomass demonstrating a robust correlation with South Asian wildfires linked to climate oscillations. Thus, for mitigating BC impacts on Himalayan glaciers, South Asia's transition from fossil fuels to clean energy is a more efficient and urgent strategy than reducing residential biomass burning.

Wang, Mo [State Key Laboratory of Tibetan Plateau ↗

Remotely Sensed High‐Resolution Soil Moisture and Evapotranspiration: Bridging the Gap Between Science and Society

This paper reviews the current state of high‐resolution remotely sensed soil moisture (SM) and evapotranspiration (ET) products and modeling, and the coupling relationship between SM and ET. SM downscaling approaches for satellite passive microwave products leverage advances in artificial intelligence and high‐resolution remote sensing using visible, near‐infrared, thermal‐infrared, and synthetic aperture radar sensors. Remotely sensed ET continues to advance in spatiotemporal resolutions from MODIS to ECOSTRESS to Hydrosat and beyond. These advances enable a new understanding of bio‐geo‐physical controls and coupled feedback mechanisms between SM and ET reflecting the land cover and land use at field scale (3–30 m, daily). Still, the state‐of‐the‐science products have their challenges and limitations, which we detail across data, retrieval algorithms, and applications. We describe the roles of these data in advancing 10 application areas: drought assessment, food security, precision agriculture, soil salinization, wildfire modeling, dust monitoring, flood forecasting, urban water, energy, and ecosystem management, ecohydrology, and biodiversity conservation. We discuss that future scientific advancement should focus on developing open‐access, high‐resolution (3–30 m), sub‐daily SM and ET products, enabling the evaluation of hydrological processes at finer scales and revolutionizing the societal applications in data‐limited regions of the world, especially the Global South for socio‐economic development.

54 ENVIRONMENTAL SCIENCES↗

Recent Accelerated Decadal Shift in Winter North American Temperature Patterns Under Pacific‐Atlantic Decadal Variability

Global warming and internal climate variability have changed winter temperature extreme regimes in North America, affecting droughts and wildfires in the western United States. However, how internal climate variability influences North American winter temperature extreme patterns remains poorly understood. Here, we demonstrate that the recent winter North American surface air temperature (SAT) exhibits an accelerated decadal alternation between Warm West-Cold East (WWCE) and Cold West-Warm East (CWWE) dipoles because their variations show shorter decadal periods during 1990–2022 than during 1950–1989 and are regulated by the Pacific Decadal Oscillation (PDO) variability. While the winter WWCE dipole mainly linked to North Pacific blocking events exhibited a smaller mean amplitude during 1990–2022 than 1950–1989 due to the weakened positive PDO phase during 1990–2022 under the positive phase of the Atlantic Multidecadal Oscillation (AMO), the winter CWWE showed a larger mean amplitude during 1990–2022 due to the stronger negative PDO phase than during 1950–1989. Our results further suggest that the recent rapid decadal shift of North American winter temperatures is primarily attributed to the PDO variability likely due to anthropogenic warming under the positive AMO.

Atlantic Multidecadal Oscillation↗

Semi‐Volatile Organic Partitioning Improves Simulation of Biomass Burning Aerosol Mixing State Evolution

Biomass burning aerosols significantly contribute to atmospheric composition and radiative forcing, with black carbon (BC) mixing states critically influencing optical properties and climate impacts. Recent field observations reveal a systematic three‐phase evolution in BC coating thickness during plume aging: rapid initial growth, quasi‐equilibrium, and gradual coating loss. Current models misrepresent this evolution due to oversimplified treatment of organic aerosol volatility. Here we demonstrate that incorporating semi‐volatile organic partitioning through the MATRIX‐VBS model fundamentally improves simulation accuracy compared to traditional non‐volatile approaches. Evaluation against four field campaigns spanning fresh to aged plumes shows MATRIX‐VBS successfully captures the observed three‐phase pattern, and global application reveals universal three‐phase evolution with substantial regional variations. These advances address critical gaps in aerosol mixing state representation and provide essential improvements for climate model predictions in wildfire‐affected regions.

Gao, Chloe Yuchao [Fudan Univ., Shanghai (China); ↗

Forest fire threatens global carbon sinks and population centres under rising atmospheric water demand

Levels of fire activity and severity that are unprecedented in the instrumental record have recently been observed in forested regions around the world. Using a large sample of daily fire events and hourly climate data, here we show that fire activity in all global forest biomes responds strongly and predictably to exceedance of thresholds in atmospheric water demand, as measured by maximum daily vapour pressure deficit. The climatology of vapour pressure deficit can therefore be reliably used to predict forest fire risk under projected future climates. We find that climate change is projected to lead to widespread increases in risk, with at least 30 additional days above critical thresholds for fire activity in forest biomes on every continent by 2100 under rising emissions scenarios. Escalating forest fire risk threatens catastrophic carbon losses in the Amazon and major population health impacts from wildfire smoke in south Asia and east Africa.

54 ENVIRONMENTAL SCIENCES↗

Hot season gets hotter due to rainfall delay over tropical land in a warming climate

Tropical land generally experiences the hottest period (spring) in a year just before the onset of wet season. Previous studies suggested that in a warming climate, the wet season would come later, but its origin is debated and its impact on temperature remains unknown. Here, we find that the warming of hot season would be amplified under global warming, and refer to it as “hot-season-gets-hotter” phenomenon. The amplified hot season warming is closely tied to the amplified warming of hot temperature percentiles. The hot-season-gets-hotter phenomenon is mainly due to the rainfall delay and most evident in the Amazon, where spring is warming by almost 1?K more than the annual mean and the 99th percentile temperatures are warming ~30% more than the mean by the end of 21st century in a high emission scenario. Comparing experiments with and without land-atmosphere coupling, it is further found that the rainfall delay is initially driven by the enhanced effective atmospheric heat capacity and then substantially amplified by positive soil moisture-atmosphere feedback. In the satellite period, observations consistently show that the hot-season-gets-hotter phenomenon has already emerged along with the rainfall delay in the Amazon. Intensified hot and dry spring climate can enhance risks of drought, heatwaves and wildfires, threatening the Amazon forest and habitats in the tropics.

54 ENVIRONMENTAL SCIENCES↗

Knitting while Australia burns

A global biodiversity hotspot, Australia has reached a tipping point from which many of its forests may never recover. Record-breaking heat, drought and windy conditions have burned at least 10 million hectares. Halfway through the season, fires have persisted for months with no end in sight. Here, the continent faces an exponential rise in future wildfire risk as the climate warms and dries.

54 ENVIRONMENTAL SCIENCES↗

Spatial variability in Arctic–boreal fire regimes influenced by environmental and human factors

Abstract Wildfire activity in Arctic and boreal regions is rapidly increasing, with severe consequences for climate and human health. Regional long-term variations in fire frequency and intensity characterize fire regimes. The spatial variability in Arctic–boreal fire regimes and their environmental and anthropogenic drivers, however, remain poorly understood. Here we present a fire tracking system to map the sub-daily evolution of all circumpolar Arctic–boreal fires between 2012 and 2023 using 375 m Visible Infrared Imaging Radiometer Suite active fire detections and the resulting dataset of the ignition time, location, size, duration, spread and intensity of individual fires. We use this dataset to classify the Arctic–boreal biomes into seven distinct ‘pyroregions’ with unique climatic and geographic environments. We find that these pyroregions exhibit varying responses to environmental drivers, with boreal North America, eastern Siberia and northern tundra regions showing the highest sensitivity to climate and lightning density. In addition, anthropogenic factors play an important role in influencing fire number and size, interacting with other factors. Understanding the spatial variability of fire regimes and its interconnected drivers in the Arctic–boreal domain is important for improving future predictions of fire activity and identifying areas at risk for extreme events.

Geology↗

The critical role of soil moisture in compound hazards

Soil moisture regulates the exchange of energy, water, and carbon across land–vegetation–atmosphere interfaces. Extremes in soil moisture can amplify natural hazards through interactions with diverse Earth system processes. Despite its mechanistic importance, soil moisture remains underrepresented in hazard research and predictive frameworks. Here, in this study, we review our current understanding of the role of soil moisture in the evolution and onset of diverse compound hazards by synthesizing the latest findings from observational and modelling studies. We highlight key soil moisture mechanisms, including atmospheric feedbacks that amplify drought–heatwave–wildfire events, precipitation couplings that promote clustered storms, and threshold responses that drive vegetation die-offs, trigger landslides, and induce flooding. Persistent challenges in observational data, model representation and operational implementation have limited the integration of soil moisture into hazard early-warning systems. Addressing these gaps through advances in observations, data assimilation, and physics-based and data-driven modelling will enhance hazard prediction and preparedness in a rapidly changing world.

Li, Chuxuan [University of California, Los Angeles↗

A high resolution, gridded product for vapor pressure deficit using Daymet

Vapor pressure deficit (VPD) is a critical variable in assessing drought conditions and evaluating plant water stress. Gridded products of global and regional VPD are not freely available from satellite remote sensing, model reanalysis, or ground observation datasets. We present two versions of the first gridded VPD product for the Continental US and parts of Northern Mexico and Southern Canada (CONUS+) at a 1 km spatial resolution and daily time step. We derived VPD from Daymet maximum daily temperature and average daily vapor pressure and scale the estimates based on (1) climate determined by the Köppen-Geiger classifications and (2) land cover determined by the International Geosphere-Biosphere Programme. Ground-based VPD data from 253 AmeriFlux sites representing different climate and land cover classifications were used to improve the Daymet-derived VPD estimates for every pixel in the CONUS+ grid to produce the final datasets. We evaluated the Daymet-derived VPD against independent observations and reanalysis data. The CONUS+ VPD datasets will aid in investigating disturbances including drought and wildfire, and informing land management strategies.

54 ENVIRONMENTAL SCIENCES↗

Unified 0.25-degree gridded infrastructure-critical extreme weather for the United States from 1979 to 2100

Extreme weather events can severely disrupt critical infrastructure, triggering cascading effects on power, transportation, and essential services. However, standard weather and climate datasets often lack specialized variables necessary for hazard assessments. We present a unified dataset of infrastructure-critical weather and climate variables across the United States at 0.25° resolution, covering daily or sub-daily intervals from 1979 to 2100. The dataset includes temperature, dew point, wind gusts, precipitation partitioned by rain, snow, and freezing rain or ice pellets, lightning, and wildfire metrics. Historical conditions (1979-2023) are synthesized from observations and reanalysis products, while future projections are derived from 14 CMIP6 global climate models (historical, SSP245, and SSP585 experiments). Physically based and data-driven methods are used to estimate variables not directly provided by existing models. By integrating these variables into a single unified dataset, we enable consistent, high-resolution assessments of weather-related infrastructure risks across past and future periods, supporting wide-ranging applications in energy, transportation, water resources, emergency management, and beyond.

Climate and Earth system modelling↗

Predicting wind-driven spatial deposition through simulated color images using deep autoencoders

Abstract For centuries, scientists have observed nature to understand the laws that govern the physical world. The traditional process of turning observations into physical understanding is slow. Imperfect models are constructed and tested to explain relationships in data. Powerful new algorithms can enable computers to learn physics by observing images and videos. Inspired by this idea, instead of training machine learning models using physical quantities, we used images, that is, pixel information. For this work, and as a proof of concept, the physics of interest are wind-driven spatial patterns. These phenomena include features in Aeolian dunes and volcanic ash deposition, wildfire smoke, and air pollution plumes. We use computer model simulations of spatial deposition patterns to approximate images from a hypothetical imaging device whose outputs are red, green, and blue (RGB) color images with channel values ranging from 0 to 255. In this paper, we explore deep convolutional neural network-based autoencoders to exploit relationships in wind-driven spatial patterns, which commonly occur in geosciences, and reduce their dimensionality. Reducing the data dimension size with an encoder enables training deep, fully connected neural network models linking geographic and meteorological scalar input quantities to the encoded space. Once this is achieved, full spatial patterns are reconstructed using the decoder. We demonstrate this approach on images of spatial deposition from a pollution source, where the encoder compresses the dimensionality to 0.02% of the original size, and the full predictive model performance on test data achieves a normalized root mean squared error of 8%, a figure of merit in space of 94% and a precision-recall area under the curve of 0.93.

54 ENVIRONMENTAL SCIENCES↗

Evaluating the efficacy and equity of environmental stopgap measures

Contemporary environmental policy is rife with measures that do not fully resolve a problem, but instead are proposed to “buy time” for the development and future implementation of more durable solutions. In this perspective, we define such measures as “stopgap measures,” and examine examples from wildfire risk management, hydrochlorofluorocarbon regulation, and Colorado River water management. We introduce an analytical framework to assess stopgaps, and apply this framework to solar geoengineering, a controversial stopgap for climate action. Studying stopgaps as a novel category of policy and management measures can help us understand the why stopgaps emerge, and weigh the equity and efficacy of stopgaps against other policy proposals

54 ENVIRONMENTAL SCIENCES↗

Synthesis of the land carbon fluxes of the Amazon region between 2010 and 2020

The Amazon is the largest continuous tropical forest in the world and plays a key role in the global carbon cycle. Human-induced disturbances and climate change have impacted the Amazon carbon balance. Here we conduct a comprehensive synthesis of existing state-of-the-art estimates of the contemporary land carbon fluxes in the Amazon using a set of bottom-up methods (i.e., dynamic vegetation models and bookkeeping models) and a top-down inversion (atmospheric inversion model) over the Brazilian Amazon and the whole Biogeographical Amazon domain. Over the whole biogeographical Amazon region bottom-up methodologies suggest a small average carbon sink over 2010-2020, in contrast to a small carbon source simulated by top-down inversion (2010-2018). However, these estimates are not significantly different from one another when accounting for their large individual uncertainties, highlighting remaining knowledge gaps, and the urgent need to reduce such uncertainties. Nevertheless, both methodologies agreed that the Brazilian Amazon has been a net carbon source during recent climate extremes and that the south-eastern Amazon was a net land carbon source over the whole study period (2010-2020). Overall, our results point to increasing human-induced disturbances (deforestation and forest degradation by wildfires) and reduction in the old-growth forest sink during drought.

54 ENVIRONMENTAL SCIENCES↗

Future increases in Amazonia water stress from CO 2 physiology and deforestation

Several different drivers are contributing to climate change within the Amazon basin, including forcing from greenhouse gases and aerosols, plant physiology responses to rising CO 2 , and deforestation. Attribution among these drivers has not been quantified for Shared Socioeconomic Pathway (SSP) climate simulations. Here we identify the contribution of CO 2 physiology and deforestation to future hydroclimate change in the Amazon basin by combining information from four experiments and eight different Earth system models in Coupled Model Intercomparison Project Phase 6. Together, forcing from CO 2 physiology and deforestation account for about 44% of the projected annual precipitation decline, 48% of surface relative humidity decline and 11% of warming over the Amazon basin by 2100 for SSP3-7.0. Further, other Coupled Model Intercomparison Project Phase 6 SSP simulations have similar contributions from the two drivers. Insight from our attribution analysis can aid in identifying research priorities aimed at reducing uncertainty in future projections of water availability, carbon dynamics and wildfire risk.

54 ENVIRONMENTAL SCIENCES↗

Sunlight can turn smoldering pine wood smoke into a glass

Wildfires inject biomass burning organic aerosols (BBOA) into the atmosphere. During their lifetimes of weeks to months, they are exposed to ultraviolet (UV) irradiation. Viscosity and phase behaviour are essential properties for understanding their chemical and climate impacts. Here, we quantify changes in viscosity and phase behavior after UV exposure. After an atmospheric equivalent of 8.7 days of boundary layer UV exposure, BBOA develop a highly viscous (glassy) outer phase with a viscosity at least five orders of magnitude higher than unaged BBOA, which persists up to at least 58% relative humidity. High-resolution mass spectrometry indicates that UV-aging increases oxidation and molecular weight. Using our viscosity results, we predict that UV-aged BBOA are frequently glassy above ~2.5 km and can have viscosities up to eight orders of magnitude higher than unaged particles in some atmospheric regions, which may influence lifetimes of pollutants and brown carbon, and impact stratospheric ozone chemistry.

Golay, Zoe↗

Spherical tarball particles form through rapid chemical and physical changes of organic matter in biomass-burning smoke

Significance Wildfires emit large amounts of biomass-burning (BB) aerosol particles and contribute to regional and global climate. Moreover, BB emissions are expected to increase in coming decades as a result of climate change. Tarballs, spherical organic BB particles, are estimated to contribute up to ∼30% of the BB aerosol mass. However, uncertainty still exists as to how tarballs form and how they influence climate. Our observations show that tarballs form through a combination of chemical and physical changes of primary organic aerosols within the first hours following emission. The finding of tarball formation will improve assessments of BB particle evolution and of BB impacts on regional and global climate.

09 BIOMASS FUELS↗

The contribution of black carbon to global ice nucleating particle concentrations relevant to mixed-phase clouds

Significance The Earth’s climate is affected by the radiative properties of clouds. In clouds containing both supercooled water droplets and ice particles (mixed-phase clouds), cloud lifetime and albedo are affected by the presence of ice nucleating particles (INP). After decades of research, the importance of black carbon (BC) as an INP remains unresolved. In this work, we determined the contribution of BC to INP concentrations ([INP]) from real-world wildfires and prescribed burns. We found that BC does not contribute significantly to [INP] in near-field biomass burning plumes. These results were applied as parameterizations to global climate model output. Combined with previous work on diesel-engine exhaust, we find that BC does not contribute significantly to global [INP] relevant to mixed-phase clouds.

54 ENVIRONMENTAL SCIENCES↗