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At least 451 records · Page 25

High Flux Isotope Reactor Low-Enriched Uranium High Density Silicide Fuel Preliminary Design Update: System Transient Analysis

As a part of conversion efforts from highly enriched uranium (HEU) to low-enriched uranium (LEU) fuel under direction of the National Nuclear Security Administration of the U.S. Department of Energy, multiple proposed designs of the High Flux Isotope Reactor (HFIR) have been created and assessed regarding reactor physics performance metrics, including designs utilizing uranium silicide dispersion fuel (U3Si2-Al). This report updates the previous analyses that evaluated the nuclear safety performance of LEU fuel designs with respect to selected accident events from the HFIR Safety Analysis Report (SAR). Both the Low Density (LD) and High Density (HD) Optimized designs’ reactivity initiated accident fuel performance improved relative to the HEU fuel, attributed to greater 238 U negative Doppler feedback. However, the thermal margins for primary coolant system accidents were reduced with some acceptance criteria unable to be met. The need to resolve reduced thermal margin, open modeling items, and unresolved assumptions was identified.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Risk Informed Timelines (RIT) v.1.0

Risk Informed Timelines (RIT) is a more modern and holistic method for understanding how access delay timelines are developed and utilized in physical security system evaluations. The software utilizes Bayesian methods to combine subject matter expert judgement and small performance test datasets in a consistent and defensible way. It allows a more holistic view of delay performance that provides distributions of task times and task success probabilities to account for tasks that, if failed, would result in failure of the attack. The RIT methodology is meant to enable security risk managers to begin the transition into more comprehensive delay timeline analysis. Sandia National Laboratories is a multimission laboratory managed and operated by National Technology & Engineering Solutions of Sandia, LLC, a wholly owned subsidiary of Honeywell International Inc., for the U.S. Department of Energy’s National Nuclear Security Administration under contract DE-NA0003525. SAND2021-8294 O

Noel, ToddG.↗

FY21 NNSA-IAEC Science Area V, Environmental ISR, Waste Management and Subsurface Science (Final Report)

The FY21 NNSA NA-22 Final Report represents the progress achieved over the past year (FY21) by the research team for Topic Area 3, Waste Management & Subsurface Science (WM3), and Topic Area 7, Radiation and Thermal Effects on Bituminous Rocks (WM7). WM3 and WM7 are part of Science Area V (Subsurface Science and Waste Management) in the NNSA-IAEC Science and Technology Working Group. The project was initiated four years ago (2017) with an MOU agreement between the U.S. National Nuclear Security Administration (NNSA) and the Israel Atomic Energy Commission (IAEC) to evaluate the feasibility of geological subsurface disposal of radioactive waste in Israel. The core WM3 and WM7 teams are comprised of scientists and engineers from Los Alamos National Laboratory, the Geologic Survey of Israel (GSI), and the Nuclear Research Center - Negev (NRCN), with a close collaboration to the teams from Sandia National Laboratory (SNL) and Lawrence Livermore Laboratory (LLNL)

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Multi-fidelity equations of state and transport coefficient datasets for pulsed-power applications

Reliably simulating experiments relevant to the National Nuclear Security Administration (NNSA) requires a detailed description of material properties across a wide range of conditions. Such properties include the equations of state, charged-particle transport coefficients, and optical properties like the opacity. Together, these properties make up the material models used in radiation-magnetohydrodynamic simulations of nuclear fusion experiments. Many of these models do not incorporate uncertainties in the data used to produce them. It is unknown whether these uncertainties significantly impact the interpretation of simulation results and diagnostics. The purpose of this work is to quantify how such uncertainties impact simulations of pulsed-power experiments. We accomplished this task by first assessing discrepancies between approaches used to generate the data. This included bringing together members of the high-energy-density community spanning the three NNSA laboratories and multiple universities. Then, using these data, we developed a general framework that systematically incorporates physical uncertainties within the material models suitable for uncertainty quantification analyses. The framework utilizes machine learning, Bayesian inference, and incorporates multi-fidelity datasets. We demonstrated the framework by quantifying the impact that material model uncertainties have on simulations of pulsed-power experiments underway on Z at Sandia National Laboratories. As a result of this work, we discovered that modest uncertainties in material models (roughly 20%) correspond to significant uncertainties in the outputs from simulations. Our framework has enabled rapid construction of material models through an automated procedure and allows for the generation of material models of interest to the NNSA.

36 MATERIALS SCIENCE↗

The Dual-Axis Radiographic Hydrodynamic Test Facility Capability eXpansion (DCX) Strategy

This document details the strategy proposed to meet the National Nuclear Security Administration (NNSA) requirement for the Dual-Axis Radiographic Hydrodynamic Test (DARHT) Facility Sustainment and Modernization projects identified in multiple NNSA Stockpile Stewardship and Management Plan (SSMP) reports to Congress [NNSA, 2020; 2021; 2022; 2023; 2024]. DARHT has become indispensable for the certification of the primaries of U.S. nuclear weapons since the current U.S. moratorium halted underground nuclear testing more than 30 years ago. However, aging facilities, evolving technology, and other issues are limiting or threatening the capability of DARHT to meet NNSA’s expanding mission needs now and into the future. This DARHT Capability eXpansion (DCX) strategy was developed to address NNSA needs by extending DARHT’s reliability and resilience, increasing the quality and quantity of DARHT data, and enabling hydrodynamic measurements in complex environments. The strategy can be implemented through integration of line-item projects, acquisition of major items of equipment, and other actions coordinated with the execution of the SSMP. This strategy document is intended for U.S. Government officials, particularly authorizers, appropriators, and program leaders. It may also be furnished to DARHT users, customers, collaborators, stakeholders, and visitors as needed

45 MILITARY TECHNOLOGY, WEAPONRY, AND NATIONAL DEF↗

Validation of the Public Radiation Exposure Calculation for the Incident at the National Institute of Standards and Technology Center for Neutron Research on February 3, 2021

The Department of Energy/National Nuclear Security Administration Consequence Management Program was contacted by the Health Physics Chief of the National Institute of Standards and Technology Center for Neutron Research (NCNR) to review public radiation exposure calculations for an event that occurred on its Gaithersburg, Maryland, campus on February 3, 2021. Subject matter experts from the Nuclear Emergency Support Team (NEST) assets, specifically the Consequence Management Home Team (CMHT) and the National Atmospheric Release Advisory Center (NARAC), were selected to provide support. CMHT used three separate modeling codes to validate the results the scientists at NCNR calculated using the HotSpot model. The analyses were performed using NARAC’s in-house Lagrangian dispersion codes known as LODI and Aeolus, as well as the Turbo FRMAC software from Sandia National Laboratories. The team used parameters provided by the NCNR scientists regarding the site, applicable observable meteorological data, and environmental survey and sampling data to estimate public exposure. Each model estimated public dose at much less than 0.5 mrem. CMHT concurs with the NCNR public radiation exposure calculations which state that members of the public at the 400-meter boundary would have received a radiological dose of less than 0.5 mrem.

61 RADIATION PROTECTION AND DOSIMETRY↗

Smart Packaging for Critical Energy Shipment (SPaCES)

Recent technical advances have brought forth revolutionary Smart Packaging (SP) technology. SP incorporates multiple electronics, chemical, and mechanical sensing technologies into packaging materials, and utilizes them to monitor and display package content status. SP can also employ embedded micro actuators to react to undesirable package conditions such as moisture/temperature anomalies or harmful chemical reactions and neutralize it. When further integrated with wireless sensing and secure networking, SP provides wholistic system-wide remote situation awareness capability for real-time crisis management. Finally, we also see that SP can be further integrated with 3D printing technology to offer form-factor customization and application specific solutions suitable for DOE (Department of Energy) NNSA’s (National Nuclear Security Administration) R/N (radiological/nuclear) material shipment and management needs; this has the potential to improve safety, security, and overall operation process quality. This report surveys SP technology as the state of the art (SOTA) and analyzes how it can integrate with cybersecurity and 3D printing to address NNSA’s critical R/N material shipment and storage requirements. This report further presents our FY23/24 investigation plan describing project background, goal, motivation, proposed work, and statement of work and cost.

47 OTHER INSTRUMENTATION↗

Panel Session 34: US DOE Featured Site: Savannah River Operations Office: 70 Years of Service

The Savannah River Site celebrates its 70. anniversary on November 28, 2020. On this date in 1950, President Harry S. Truman requested the Dupont Company to design, build and operate what was then known as the Savannah River Plant in response to the Soviet Union's detonation of its first atomic weapon, which set the Cold War into motion. During the 1950's, six South Carolina towns were relocated for the construction of SRS and by 1953, the 310 square mile site was complete. Nearly 40,000 workers were employed t build five nuclear reactors and support facilities, two chemical separations plants, heavy water extraction plant, nuclear fuel and target fabrication facility tritium extraction facility and waste management facilities. SRS played a key role in winning the Cold War and for seven decades, SRS has been a leader within the DOE complex. Today, the site supports environmental stewardship and maintains the nation's nuclear deterrent while ensuring the safekeeping and disposal of domestic and international nuclear materials. The site continues to support the nation's nuclear defense as it explores new potential NNSA missions. SRS has a proud 70- year history and looks forward to a future of service as a national asset and strong community partner. The session was kicked off with a video message from Secretary of Energy, Dan Brouillette, who thanked employees past and current for their efforts. The video also provided an overview of the history and future of the Site. This panel provided an overview of the Savannah River Site's 70 years of service (history, challenges, opportunities, and future) presented by the SRS's Senior leadership and the local Aiken, South Carolina Mayor. Panelists with presentations: US DOE Secretary Dan Brouillette's Overview of DOE and SRS - A Legacy of 70 Years of Service (Amy Boyette); 70 Years of Service (Michael Budney); 70 Years of Service (Stuart MacVean); SRS Liquid Waste (Thomas Foster); National Nuclear Security Administration (Nicole Nelson-Jean)

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Dante

SAND2022-12905 O Dante is a physical security simulation package used in evaluating protective staffing and physical security elements against adversarial threats. Dante simulates force-on-force scenarios in a batch Monte Carlo process. Analysts use the included Scenario Editor to define the scenarios for their site and then execute and analyze the results using the Batch Manager tool. Dante provides insight into how well a security system performs against threats and lets analysts mine the results for key indicators of system performance. Sandia National Laboratories is a multimission laboratory managed and operated by National Technology & Engineering Solutions of Sandia, LLC, a wholly owned subsidiary of Honeywell International Inc., for the U.S. Department of Energy’s National Nuclear Security Administration under contract DE-NA0003525.

Hart, Brian↗

The Optics of Deterrence: How Science Assures the Nuclear Stockpile's Reliability In Lieu of Testing

When designing a product intended to perform a certain function and satisfy some set of criteria, the standard engineering method to assess its ability to perform is to test it. This nearly universal concept works consistently, assuring proper function and generally avoiding or mitigating the consequence of failure to within acceptable limits. What would happen if the product developers were told that they must continue to certify and validate the performance without testing it, that the landscape in which the product must serve its purpose is constantly evolving, and that the product in question is the United States’ nuclear weapons stockpile? This is the position the National Nuclear Security Administration (NNSA) finds itself in; the reliability of the stockpile must be verified without actually testing it to see if it works as intended.

43 PARTICLE ACCELERATORS↗

National Security Research Center 2021 Strategic Plan

The National Security Research Center (NSRC) is a dynamic organization staffed with an expert, highly trained experts. The NSRC opened its doors in June 2019, making it one of the newest large organizations at Los Alamos National Laboratory (LANL). It supports a broad range of researchers within the LANL Weapons Program, customers across other National Nuclear Security Administration (NNSA) labs and sites, and partners in the Department of Defense (DoD). The maintenance and growth of the NSRC necessitate strategy and foresight. The NSRC leadership has developed a series of strategic goals through discussions with NSRC staff, customers, LANL leadership, and similar research institutions around the country to guide the NSRC leadership in moving the Center forward over the next five years.

99 GENERAL AND MISCELLANEOUS↗

Preliminary Thermal-Hydraulic Analysis of the UTA–2 Subcritical Linear Accelerator–Driven System

The National Nuclear Security Administration’s mission includes establishing a reliable supply of 99 Mo without highly enriched uranium. Oak Ridge National Laboratory (ORNL) supports this objective through collaborative research and development with industrial partners. Niowave Inc., a current partner, is currently designing a subcritical linear accelerator-driven system (ADS) and preparing for the US Nuclear Regulatory Commission’s licensing process. Niowave’s system has the potential to efficiently supply medical radioisotopes. The technology includes a superconducting electron accelerator and a pile of both natural and low-enriched uranium (LEU) targets. The process fissions uranium and many valuable isotopes can then be extracted from the targets. Niowave is currently iterating through conceptual and detailed design processes for several system sizes. This report discusses UTA–2, which is at the demonstration stage. UTA–2 will validate numerical modeling results with experimental measurements before progressing to the detailed design of UTA–3, the commercial-sized ADS. The thermal-hydraulic behavior of the UTA–2 core design was numerically investigated using STAR-CCM+, as described in this report. STAR-CCM+, a state-of-the-art computational fluid dynamics (CFD) software that was commercially developed by Siemens, has an extensive user base and a set of validation studies. It is also compliant with the American Society of Mechanical Engineers’ Nuclear Quality Assurance 1 standard. Three cases are investigated in this report. Case 1 quantified the temperature field within the UTA–2 assembly and water tank using only conduction as the method of thermal energy transport. This simplified approach was overly conservative and yielded wetted cladding temperatures above the coolant saturation temperature. In this case, the maximum temperature of the wetted cladding surface of the highest power rod exceeded the saturation temperature of water by 63.8°C. Because of the overly conservative approach taken in Case 1 and its negative subcooled margin, buoyancy-driven natural circulation flow physics were implemented in Case 2. Adding coolant motion significantly distributed the thermal energy of the system through convective heat transfer. This relatively small amount of convective heat transfer significantly reduced system temperatures and increased the subcooled margin from –63.8 to 61.3°C. This margin confirmed that no boiling was expected during normal operation of UTA–2 at 230 W. Case 3 had no additional physics models but considered an overpower event during which the power of each LEU and natural uranium rod was at its respective peak values. This resulted in a study with the total assembly power equal to 176% of the nominal power of 230 W considered in Cases 1 and 2. The resulting natural circulation flows were slightly enhanced. The subcooled margin decreased slightly to 46.3°C, which is still a significant margin to local boiling of the water within the tank. This margin confirmed that no boiling was expected during an abnormal operation of UTA–2 at 406 W.

07 ISOTOPE AND RADIATION SOURCES↗

A comparison of machine learning methods to classify radioactive elements using prompt-gamma-ray neutron activation data

The detection of illicit radiological materials is critical to establishing a robust second line of defence in nuclear security. Neutron-capture prompt-gamma activation analysis (PGAA) can be used to detect multiple radioactive materials across the entire Periodic Table. However, long detection times and a high rate of false positives pose a significant hindrance in the deployment of PGAA-based systems to identify the presence of illicit substances in nuclear forensics. In the present work, six different machine-learning algorithms were developed to classify radioactive elements based on the PGAA energy spectra. The model performance was evaluated using standard classification metrics and trend curves with an emphasis on comparing the effectiveness of algorithms that are best suited for classifying imbalanced datasets. We analyse the classification performance based on Precision, Recall, F1-score, Specificity, Confusion matrix, ROC-AUC curves, and Geometric Mean Score (GMS) measures. The tree-based algorithms (Decision Trees, Random Forest and AdaBoost) have consistently outperformed Support Vector Machine and K-Nearest Neighbours. Based on the results presented, AdaBoost is the preferred classifier to analyse data containing PGAA spectral information due to the high recall and minimal false negatives reported in the minority class.

97 MATHEMATICS AND COMPUTING↗

Proposal to use the DOE-STD-3009-2014 Methodology to Prepare the Documented Safety Analysis (DSA) for Research Reactor Nuclear Facilities

Sandia National Laboratories (SNL) personnel operate a low power research reactor (the Annular Core Research Reactor, or ACRR), and a zero-power critical experiment assembly referred to as CX. In accordance with 10 CFR 830, Subpart B, Appendix A, the acceptable methodology for developing a Documented Safety Analysis (DSA) for DOE nuclear reactors is the Nuclear Regulatory Commission’s (NRC’s) Regulatory Guide 1.70 (RG 1.70). RG 1.70 does not address certain areas required by 10 CFR 830 and expected by DOE (e.g., full facility hazard analysis).Thus, the current DSAs for SNL’s reactor nuclear facilities are based on RG 1.70, but also of necessity supplemented by DOE-STD-3009-94 methods. SNL personnel, in consultation with the National Nuclear Security Administration (NNSA) Sandia Field Office (SFO), have concluded that an alternate methodology is preferred to RG 1.70. The details of the proposal, and the reasons motivating its development, are discussed in the order described below. The proposed alternate methodology will be applicable to the ACRR and the CX (i.e., it will be applicable to nuclear facilities in which a reactor and/or a critical assembly will be operated).

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

FY22 Laboratory Directed Research and Development Annual Report

The Laboratory Directed Research and Development (LDRD) program yields foundational scientific research and development (R&D) essential to growing SRNL’s core competencies, in alignment with SRNL’s Strategic Plan to provide long-term benefits to the Department of Energy (DOE), the National Nuclear Security Administration (NNSA), and other customers and stakeholders. Five strategic goals are outlined in SRNL’s strategic plan: 1) Provide applied science and engineering for EM’s active clean-up sites and LM’s post closure management sites; 2) Provide science-based solutions for gaps identified in nonproliferation strategic vision and support the government in actives impacting national security; 3) Lead ST&E as the central technical authority for processing tritium loaded reservoirs and support production of plutonium pits; 4) Align science and energy security programs by focusing modern modeling, simulation, and data analytics tools on materials engineering and performance applications; 5) Build a workforce for the future.

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