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Investigations of Clouds and Aerosols on Mars, Venus and Titan

This final report was included as part of a new proposal. This new proposal was selected for funding on 9 Nov. 1999. For Titan our interest during the past few years was to explain the observed asymmetry in the albedo. We suggested earlier, from one-dimensional modeling studies, that vertical transport rates were comparable to particle fall speeds. Since heating of the upper atmosphere, which drives dynamical motions, is largely due to the aerosols, a nonlinear interaction between dynamics, radiative heating and particle microphysics is possible. We pursued this interaction in a two-dimensional model. We showed that the observed variations in the albedo between the two hemispheres and over an orbital cycle, could be due to dynamical motions suspending particles so that particle sizes and optical depths vary across the planet. In the Cassini time frame, future studies of this interaction between dynamics, radiation and microphysics may be worthwhile using, the strong modeling base that others, and we have developed. In our recently approved proposal, however, we plan to extend our modeling to hydrocarbon clouds that lie at lower levels. We know very little about such clouds, and numerical models for their properties are non-existent. These clouds may be observed by the Huygen's Probe, and by the Cassini orbiter, so predictions of their properties should help in the analysis of Cassini data. We have also developed a sophisticated model for the lower, condensational, clouds on Venus. In this model we explored the water vapor budget on Venus, and the properties of the clouds such as particle size distribution. During the past few years we have applied our model of the water ice clouds on Mars to new data sets from Pathfinder, and Mars Global Surveyor. We have compared our predictions of cloud properties with those seen by Pathfinder, and found reasonable agreement.

Toon, Owen B.↗

Investigations of Clouds and Aerosols on Mars, Venus and Titan

For Titan our interest during the past few years was to explain the observed asymmetry in the albedo. We suggested earlier, from one-dimensional modeling studies, that vertical transport rates were comparable to particle fall speeds. Since heating of the upper atmosphere, which drives dynamical motions, is largely due to the aerosols, a non- linear interaction between dynamics, radiative heating and particle microphysics is possible. We pursued this interaction in a two-dimensional model. We showed that the observed variations in the albedo between the two hemispheres and over an orbital cycle, could be due to dynamical motions suspending particles so that particle sizes and optical depths vary across the planet. In the Cassini time frame, future studies of this interaction between dynamics, radiation and microphysics may be worthwhile using the strong modeling base that others, and we have developed. In our recently approved proposal, however, we plan to extend our modeling to hydrocarbon clouds that lie at lower levels. We know very little about such clouds, and numerical models for their properties are non-existent. These clouds may be observed by the Huygen's Probe, and by the Cassini orbiter, so predictions of their properties should help in the analysis of Cassini data. We have also developed a sophisticated model for the lower, condensational, clouds on Venus. In this model we explored the water vapor budget on Venus, and the properties of the clouds such as particle size distribution. Most researchers have investigated the upper clouds on Venus, which are essentially a photochemical aerosol with a long lifetime. The lower clouds, however, are similar to stratus clouds on Earth. These clouds have short lifetimes, and are tightly coupled to the dynamics at the base of the Venus cloud deck. We believe that the holes in these clouds seen at near infrared wavelengths by Galileo are related to some interaction between dynamics and cloud physics. One goal of our recently approved proposed work is to better understand this interaction, and to better understand how these clouds may vary if the climate of Venus were to vary. During the past few years we have applied our model of the water ice clouds on Mars to new data sets from Pathfinder, and Mars Global Surveyor. We have compared our predictions of cloud properties with those seen by Pathfinder, and found reasonable agreement. More recently we have improved our model by including a radiative transfer algorithm and a boundary layer transport scheme . The goal of this work is to understand the thermal inversions seen in Mars Global Surveyor data. We find that the inversions are created by clouds radiatively cooling the atmospheric layers in which the clouds form. We have also initiated laboratory work on the physics of carbon dioxide particle formation. In our recently approved work we propose to use these laboratory data, and to extend our modeling to carbon dioxide clouds in the Martian atmosphere.

Toon, Owen B.↗

COMMIT in 7-SEAS/BASELInE: Operation of and Observations from a Novel, Mobile Laboratory for Measuring In-Situ Properties of Aerosols and Gases

Trace gases and aerosols (particularly biomass-burning aerosols) have important implications for air quality and climate studies in Southeast Asia (SEA). This paper describes the purpose, operation, and datasets collected from NASA Goddard Space Flight Center's (NASA/GSFC) Chemical, Optical, and Microphysical Measurements of In-situ Troposphere (COMMIT) laboratory, a mobile platform designed to measure trace gases and optical/microphysical properties of naturally occurring and anthropogenic aerosols. More importantly, the laboratory houses a specialized humidification system to characterize hygroscopic growth/enhancement, a behavior that affects aerosol properties and cloud-aerosol interactions and is generally underrepresented in the current literature. A summary of the trace gas and optical/microphysical measurements is provided, along with additional detail and analysis of data collected from the hygroscopic system during the 2015 Seven South-East Asian Studies (7-SEAS) field campaign. The results suggest that data from the platform are reliable and will complement future studies of aerosols and air quality in SEA and other regions of interest.

aerosols↗

Aircraft-Measured Indirect Cloud Effects from Biomass Burning Smoke in the Arctic and Subarctic

The incidence of wildfires in the Arctic and subarctic is increasing; in boreal North America, for example, the burned area is expected to increase by 200-300% over the next 50-100 years, which previous studies suggest could have a large effect on cloud microphysics, lifetime, albedo, and precipitation. However, the interactions between smoke particles and clouds remain poorly quantified due to confounding meteorological influences and remote sensing limitations. Here, we use data from several aircraft campaigns in the Arctic and subarctic to explore cloud microphysics in liquid-phase clouds influenced by biomass burning. Median cloud droplet radii in smoky clouds were approx. 40- 60% smaller than in background clouds. Based on the relationship between cloud droplet number (N(liq)/ and various biomass burning tracers (BBt/ across the multi-campaign data set, we calculated the magnitude of subarctic and Arctic smoke aerosol-cloud interactions (ACIs, where ACI = (1/3) x dln(N(liq))/dln(BBt)) to be approx. 0.16 out of a maximum possible value of 0.33 that would be obtained if all aerosols were to nucleate cloud droplets. Interestingly, in a separate subarctic case study with low liquid water content (0.02 gm/cu m and very high aerosol concentrations (2000- 3000/ cu cm in the most polluted clouds, the estimated ACI value was only 0.05. In this case, competition for water vapor by the high concentration of cloud condensation nuclei (CCN) strongly limited the formation of droplets and reduced the cloud albedo effect, which highlights the importance of cloud feedbacks across scales. Using our calculated ACI values, we estimate that the smoke-driven cloud albedo effect may decrease local summertime short-wave radiative flux by between 2 and 4 W/sq m or more under some low and homogeneous cloud cover conditions in the subarctic, although the changes should be smaller in high surface albedo regions of the Arctic.We lastly explore evidence suggesting that numerous northern-latitude background Aitken particles can interact with combustion particles, perhaps impacting their properties as cloud condensation and ice nuclei.

cloud microphysics↗

Evaluating Subgrid-Scale Properties of Low Clouds over the Beaufort Sea in Arctic System Reanalysis using ARISE Airborne In Situ Observations

Arctic low clouds influence the evolution of the Arctic system through their effects on radiative fluxes, boundary layer mixing, stability, turbulence, humidity, and precipitation. Unfortunately, atmospheric models and retrospective analysis (reanalysis) products struggle to accurately simulate the occurrence and properties of low clouds in the Arctic. To better understand the magnitude and possible causes of this problem, we analyze the disagreements between the Arctic System Reanalysis version 2 (ASR) and data taken during the September 2014 Arctic Radiation-IceBridge Sea and Ice Experiment (ARISE) airborne campaign conducted over the Beaufort Sea. Previous analysis of grid scale-averaged meteorological variables revealed a lack of cloud water produced in ASR, related to warm/dry biases, a failure to produce sufficient cloud water in conditions that are observed to be favorable for large cloud water values, and sampling issues with the ARISE flight paths. However, ARISE collected meteorological observations at one second intervals, offering spatial data resolution comparable to the subgrid scale of ASR. Subgrid scale properties and processes must be parameterized in conventional atmospheric models and reanalyses such as ASR, and often rely on assumed distributions of meteorological variables about the grid box mean state. To enable an examination of the realism of ASR’s subgrid scale properties, we use high resolution data from ARISE determine the “subgrid scale” distributions of cloud water and thermodynamic variables in the real atmosphere. Preliminary results show that the subgrid scale distribution of thermodynamic variables about the grid scale mean resembles the triangular distribution assumed in many bulk microphysical parameterization schemes, but also with tails resembling Gaussian distributions. The main goal is to understand the partitioning of the total available atmospheric water into water vapor and cloud water. Models typically covert some percentage of total water in a grid box to cloud water based on the estimated amount of supersaturation from the assumed vapor distribution. The ARISE measurements can reveal the relationship between subgrid scale supersaturation and the partition between cloud water and water vapor.

Jason Brant Dodson↗

Aerosol Properties Derived from Airborne Sky Radiance and Direct Beam Measurements in Recent NASA and DoE Field Campaigns

The AERONET (AErosol RObotic NETwork) ground-based suite of sunphotometers provides measurements of spectral aerosol optical depth (AOD), precipitable water and spectral sky radiance, which can be inverted to retrieve aerosol microphysical properties that are critical to assessments of aerosol-climate interactions. Because of data quality criteria and sampling constraints, there are significant limitations to the temporal and spatial coverage of AERONET data and their representativeness for global aerosol conditions.The 4STAR (Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research) instrument, jointly developed by NASA Ames and PNNL (Pacific Northwest National Laboratory) with NASA Goddard collaboration, combines airborne sun tracking and AERONET-like sky scanning with spectroscopic detection. Being an airborne instrument, 4STAR has the potential to fill gaps in the AERONET data set. The 4STAR instrument operated successfully in the SEAC4RS (Studies of Emissions and Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys) experiment in Aug./Sep. 2013 aboard the NASA DC-8 and in the DoE (Department of Energy)-sponsored TCAP (Two Column Aerosol Project, July 2012 & Feb. 2013) experiment aboard the DoE G-1 aircraft. 4STAR provided direct beam measurements of hyperspectral AOD, columnar trace gas retrievals (H2O, O3, NO2), and the first ever airborne hyperspectral sky radiance scans, which can be inverted to yield the same products as AERONET ground-based observations. In this presentation, we provide an overview of the new 4STAR capabilities, with an emphasis on 26 high-quality sky radiance measurements carried out by 4STAR in SEAC4RS. We compare collocated 4STAR and AERONET sky radiances, as well as their retrievals of aerosol microphysical properties for a subset of the available case studies. We summarize the particle property and air-mass characterization studies made possible by the combined 4STAR direct beam and sky radiance observations.

DoE↗

GPM Mission Overview and U.S. Science Status

The Global Precipitation Measurement (GPM) Mission is an international satellite mission to unify and advance precipitation measurements from a constellation of research and operational sensors to provide "next-generation" precipitation products [1-2]. Water is fundamental to life on Earth. Knowing where and how much rain and snow falls globally is vital to understanding how weather and climate impact both our environment and Earth's water and energy cycles, including effects on agriculture, fresh water availability, and responses to natural disasters. Since rainfall and snowfall vary greatly from place to place and over time, satellites can provide more uniform observations of rain and snow around the globe than ground instruments, especially in areas where surface measurements are difficult. Relative to current global rainfall products, GPM data products will be characterized by: (l) more accurate instantaneous precipitation measurements (especially for light rain and cold-season solid precipitation), (2) more frequent sampling by an expanded constellation of domestic and international microwave radiometers including operational humidity sounders, (3) intercalibrated microwave brightness temperatures from constellation radiometers within a unified framework, and (4) physical-based precipitation retrievals from constellation radiometers using a common a priori cloud/hydrometeor database derived from GPM Core sensor measurements. The cornerstone of the GPM mission is the deployment of a Core Observatory in a unique 65 non-Sun-synchronous orbit to serve as a physics observatory and a reference standard to unify precipitation measurements by a constellation of dedicated and operational passive microwave sensors. The design of the GPM Core Observatory is an advancement of the Tropical Rainfall Measuring Mission (TRMM)'s highly successful rain-sensing package. The Core Observatory will carry a Ku/Ka-band Dual-frequency Precipitation Radar (DPR) and a multichannel (l0-183 GHz) GPM Microwave Radiometer (GMI). Since light rain and falling snow account for a significant fraction of precipitation occurrence in middle and high latitudes, the GPM instruments extend the capabilities of the TRMM sensors to detect falling snow, measure light rain, and provide, for the first time, quantitative estimates of microphysical properties of precipitation particles. The combined use of DPR and GMI measurements will place greater constraints on possible solutions to radiometer retrievals to improve the accuracy and consistency of precipitation retrievals from all constellation radiometers. The GMI uses 13 different microwave channels to observe energy from the different types of precipitation through clouds for estimating everything from heavy to light rain and for detecting falling snow. As the satellite passes over Earth, the GMI constantly scans a region 885 kilometers across. The Ball Aerospace and Technology Corporation built the GMI under contract with NASA Goddard Space Flight Center. The DPR provides three-dimensional information about precipitation particles derived from reflected energy by these particles at different heights within the cloud system. The two frequencies of the DPR also allow the radar to infer the sizes of precipitation particles and offer insights into a storm's physical characteristics. The Ka-band frequen~y scans across a region of 125 kilometers and is nested within the wider scan of the Ku-band frequency of 245 kilometers. The Japan Aerospace and Exploration Agency (JAXA) and Japan's National Institute of Information and Communications Technology (NICT) built the DPR. The Core Observatory satellite will fly at an altitude of 253 miles (407 kilometers) in a non-Sun-synchronous orbit that covers the Earth from 65 S to 65 N - from about the Antarctic Circle to the Arctic Circle. The GPM Core Observatory is being developed and tested at NASA Goddard Space Flight Center. Once complete, a Japanese H-lIA rocket will carry thPM Core Observatory into orbit from Tanegashima Island, Japan in 2014. The GPM constellation is envisioned to comprise 8 or more microwave sensors provided by partners, including both conical imagers and cross-track sounders. GPM is currently a partnership between NASA and the Japan Aerospace Exploration Agency (JAXA). Additional partnerships are under development to include microwave radiometers on the French-Indian Megha-Tropiques satellite and U.S. Defense Meteorological Satellite Program (DMSP) satellites, as well as humidity sounders or precipitation sensors on operational satellites such as the National Polar-orbiting Operational Environmental Satellite System (NPOESS) Preparatory Project (NPP), NOAA-NASA Joint Polar Satellite System (JPSS) satellites, European MetOp satellites, and DMSP follow-on sensors. In addition, data from Chinese and Russian microwave radiometers may be available through international cooperation under the auspices of the Committee on Earth Observation Satellites (CEOS) and Group on Earth Observations (GEO). GPM's next-generation global precipitation data will lead to scientific advances and societal benefits in the following areas: (1) Improved knowledge of the Earth's water cycle and its link to climate change (2) New insights into precipitation microphysics, storm structures and large-scale atmospheric processes (3) Better understanding of climate sensitivity and feedback processes (4) Extended capabilities in monitoring and predicting hurricanes and other extreme weather events (5) Improved forecasting capabilities for natural hazards, including floods, droughts and landslides. (6) Enhanced numerical prediction skills for weather and climate (7) Better agricultural crop forecasting and monitoring of freshwater resources. An overview of the GPM mission concept and science activities in the United States, together with an update on international collaborations in radiometer intercalibration and ground validation, will be presented.

Hou, Arthur Y.↗

The 27-28 October 1986 FIRE IFO cirrus case study - Spectral properties of cirrus clouds in the 8-12 micron window

Lidar and radiometric observations are employed for detecting the presence of cirrus and describing their radiative properties. The study focuses on observations of the radiative properties of cirrus clouds within the 8-12 micron spectral region. The instrumentation that achieved the spectral radiance observations used in this study is described. Results are presented for October 28, 1986 FIRE case study day in terms of brightness temperature differences, cirrus effective emissivities, and the gross microphysical characteristics of the observed clouds. The HIS and lidar observations were combined to derive the spectral effective beam emissivity of the cirrus clouds. Fifty percent of clouds on this day displayed a spectral variation of effective beam emissivity from 2-10 percent. These differences, in conjunction with large differences in the HIS observed brightness temperatures, indicate that cirrus clouds cannot be considered gray in the 8-12 micron region. Also, the derived spectral transmittance of the cloud is used to infer the effective radii of the particle size distribution.

Ackerman, Steven A.↗

Use of Aerosol Observations From Aircraft in Satellite Remote Sensing and Modelling Comparisons

Aerosol extensive and intensive properties vary throughout the world and remain one of the largest uncertainties in determining future climate both because of difficulties in their measurement and their modelled behaviors. Here we highlight the contributions of airborne sampling by the sunphotometer 4STAR (Spectrometers for Sky-Scanning Sun Tracking Atmospheric Research) from two different parts of the world; Korean peninsula and region during the KORUS-AQ experiment (KORean-US Air Quality in May-June 2016) and over the South East Atlantic during ORACLES (ObseRvations of CLouds above Aerosols and their intEractionS in August-September-October 2016, 2017, and 2018) field campaign. The high temporal and spatial resolution, afforded by airborne sampling during KORUS-AQ, are used to determine the variability of aerosol intensive and extensive properties, which is a metric than can be compared in between multiple different observations and models, even over varying surfaces and spanning multiple different aerosol emission sources. We show the consistency over spatial scales of the AOD (Aerosol Optical Depth), and the aerosol intensive properties (Angstrom exponent - AE, fine mode fraction - FMF) observed by 4STAR, GOCI (Geostationary Ocean Color Imager Yonsei aerosol retrieval v2), MERRA-2 reanalysis (Modern-Era Retrospective Analysis for Research and Applications, v2), and from airborne in situ aerosol optical measurements by LARGE (NASA Langley Aerosol Research Group Experiment). The majority of AODs due to fine mode aerosol is observed at altitudes lower than 2 km and is dependent on the prevailing meteorological conditions. AE and FMF are found to be more spatially variable than AOD during all of KORUS-AQ, even when accounting for potential sampling biases. This may indicate that microphysical processes like aerosol particle formation, growth, and coagulation impact the dominant aerosol size at shorter scales than their combined effect on the aerosol optical depth by the aerosol emission, transport, and removal. Averaging between measurements and model, the distance at which the correlation to itself is reduced by 15% is 65 km for AOD, and 22.7 km for AE. Vertically resolved measurement from an aircraft enable the direct measurements of aerosols overlying clouds. When aerosol overlie bright clouds, their radiative impact on the incident light can be either positive or negative. This difference in radiative impact promotes difficulties in remote sensing aerosol properties, which have shown biases in AOD retrievals when clouds are underneath. The AOD above clouds measured by 4STAR during ORACLES are used to build and improve upon the current Near-Real-Time MODACAERO algorithm for above cloud AOD from MODIS, into a continuity product for NASA EOS/SNPP/JPSS.

Aerosol↗

Intercomparison of Large-Eddy Simulations of Arctic Mixed-Phase Clouds: Importance of Ice Size Distribution Assumptions

Large-eddy simulations of mixed-phase Arctic clouds by 11 different models are analyzed with the goal of improving understanding and model representation of processes controlling the evolution of these clouds. In a case based on observations from the Indirect and Semi-Direct Aerosol Campaign (ISDAC), it is found that ice number concentration, Ni, exerts significant influence on the cloud structure. Increasing Ni leads to a substantial reduction in liquid water path (LWP), in agreement with earlier studies. In contrast to previous intercomparison studies, all models here use the same ice particle properties (i.e., mass-size, mass-fall speed, and mass-capacitance relationships) and a common radiation parameterization. The constrained setup exposes the importance of ice particle size distributions (PSDs) in influencing cloud evolution. A clear separation in LWP and IWP predicted by models with bin and bulk microphysical treatments is documented and attributed primarily to the assumed shape of ice PSD used in bulk schemes. Compared to the bin schemes that explicitly predict the PSD, schemes assuming exponential ice PSD underestimate ice growth by vapor deposition and overestimate mass-weighted fall speed leading to an underprediction of IWP by a factor of two in the considered case. Sensitivity tests indicate LWP and IWP are much closer to the bin model simulations when a modified shape factor which is similar to that predicted by bin model simulation is used in bulk scheme. These results demonstrate the importance of representation of ice PSD in determining the partitioning of liquid and ice and the longevity of mixed-phase clouds.

clouds↗

Observing Ice Phase Clouds and Precipitation with Millimeter- and Submillimeter-wave Radiometry during the IMPACTS field campaign: Algorithm Development for the Emerging Class of Microwave Radiometers

Millimeter- and submillimeter-wave (mmWave, submm) radiometers provide significant information content on atmospheric water in liquid, ice, and vapor phases. Recent sensors, such as the Global Precipitation Measurement (GPM) or the Temporal Experiment for Storms and Tropical Systems Technology – Demonstration (TEMPEST-D), use mmWave bands to improve estimation of ice-phase precipitation, and future missions, such as the Atmosphere Observing System (AOS), will extend to submm to provide additional information on thinner ice clouds, linking clouds and precipitation and therefore elucidating the links between weather, climate, and the water cycle. To support the expanded use of mmWave/submm radiometry and exploit the available information content on condensed water mass, we demonstrate ice and liquid water path retrievals for NASA Goddard Space Flight Center's airborne radiometers the Conical Scanning Millimeter-wave Imaging Radiometer (CoSMIR) and the Configurable Scanning Submillimeter-wave Instrument/Radiometer (CoSSIR, formerly the Compact Scanning Submillimeter Imaging Radiometer). The analysis is based on data collected during the Investigation of Microphysics and Precipitation for Atlantic Coast-Threatening Storms (IMPACTS) field campaign. A simulation study compares and contrasts retrievals for CoSMIR and CoSSIR, with CoSSIR demonstrating higher skill in ice retrievals, particularly for thin clouds, and the CoSMIR frequencies performing better for liquid. Additionally, we look at dual-polarized radiances observed by CoSMIR during the first two IMPACTS deployments to understand the polarization signatures induced by oriented hydrometeors. Results will be presented in the context of upcoming missions and sensors including AOS and the Ice Cloud Imager (ICI). We will describe the objectives for the expected first flight of the newly upgraded CoSSIR during the final IMPACTS deployment, and we will share novel science investigations we plan to undertake with CoSSIR's new capabilities. Popular Summary: Ice in clouds and falling snow is an important component of weather, climate, and water resources. To better use a new class of sensors that provide information on atmospheric ice, we developed an approach to measure ice clouds and falling snow using airborne data taken during the Investigation of Microphysics and Precipitation for Atlantic Coast-Threatening Storms (IMPACTS), a field campaign to study winter storms. We look at the results for two similar instruments to understand how those differences affect these measurements of clouds and snow, and we further investigate the information the sensors can provide on properties of the clouds and snow.

Ian S Adams↗

Observing Ice Phase Clouds and Precipitation with Millimeter- and Submillimeter-wave Radiometry during the IMPACTS field campaign: Algorithm Development for the Emerging Class of Microwave Radiometers

Millimeter- and submillimeter-wave (mmWave, submm) radiometers provide significant information content on atmospheric water in liquid, ice, and vapor phases. Recent sensors, such as the Global Precipitation Measurement (GPM) or the Temporal Experiment for Storms and Tropical Systems Technology – Demonstration (TEMPEST-D), use mmWave bands to improve estimation of ice-phase precipitation, and future missions, such as the Atmosphere Observing System (AOS), will extend to submm to provide additional information on thinner ice clouds, linking clouds and precipitation and therefore elucidating the links between weather, climate, and the water cycle. To support the expanded use of mmWave/submm radiometry and exploit the available information content on condensed water mass, we demonstrate ice and liquid water path retrievals for NASA Goddard Space Flight Center's airborne radiometers the Conical Scanning Millimeter-wave Imaging Radiometer (CoSMIR) and the Configurable Scanning Submillimeter-wave Instrument/Radiometer (CoSSIR, formerly the Compact Scanning Submillimeter Imaging Radiometer). The analysis is based on data collected during the Investigation of Microphysics and Precipitation for Atlantic Coast-Threatening Storms (IMPACTS) field campaign. A simulation study compares and contrasts retrievals for CoSMIR and CoSSIR, with CoSSIR demonstrating higher skill in ice retrievals, particularly for thin clouds, and the CoSMIR frequencies performing better for liquid. Additionally, we look at dual-polarized radiances observed by CoSMIR during the first two IMPACTS deployments to understand the polarization signatures induced by oriented hydrometeors. Results will be presented in the context of upcoming missions and sensors including AOS and the Ice Cloud Imager (ICI). We will describe the objectives for the expected first flight of the newly upgraded CoSSIR during the final IMPACTS deployment, and we will share novel science investigations we plan to undertake with CoSSIR's new capabilities. Popular Summary: Ice in clouds and falling snow is an important component of weather, climate, and water resources. To better use a new class of sensors that provide information on atmospheric ice, we developed an approach to measure ice clouds and falling snow using airborne data taken during the Investigation of Microphysics and Precipitation for Atlantic Coast-Threatening Storms (IMPACTS), a field campaign to study winter storms. We look at the results for two similar instruments to understand how those differences affect these measurements of clouds and snow, and we further investigate the information the sensors can provide on properties of the clouds and snow.

Ian S Adams↗

The polarization lidar technique for cloud research - A review and current assessment

The development of the polarization lidar technique is reviewed, and the current capabilities and limitations of the technique for the cloud research are discussed. At present, polarization lidar is a key component of climate-research programs designed to characterize the properties of cirrus clouds and is an integral part of multiple remote-sensor studies of mixed-phase cloud systems such as winter mountain storms, making it possible to discriminate between cloud phases and to identify some particle types and orientations. Recent theoretical approaches involving ice crystal ray-tracing and cloud microphysical-model simulations are expected to increase the utility of the polarization lidar technique.

Sassen, Kenneth↗

Machine Learning Based Aerosol and Ocean Color Joint Retrieval Algorithm for Multiangle Polarimeters over Coastal Waters

NASA’s Plankton, Aerosol, Cloud, ocean Ecosystem (PACE) mission, recently launched in February 2024, carries two multiangle polarimeters (MAPs): the UMBC Hyper-Angular Rainbow Polarimeter (HARP2) and SRON Spectropolarimeter for Planetary Exploration One (SPEXone). Measurements from these MAPs will greatly advance ocean ecosystem and aerosol studies as their measurements contain rich information on microphysical properties of aerosols and hydrosols. The Multi-Angular Polarimetric Ocean coLor (MAPOL) joint retrieval algorithm has been developed to retrieve aerosol and ocean color information, which uses a vector radiative transfer (RT) model as the forward model. The RT model is computationally expensive, which makes processing a large amount of data challenging. FastMAPOL was developed to expedite retrieval using neural networks to replace the RT forward models. As a prototype study, FastMAPOL was initially limited to open ocean applications where the ocean Inherent Optical Properties (IOPs) were parameterized in terms of one parameter: chlorophyll-a concentration (Chla). In this study we further expand the FastMAPOL joint retrieval algorithm to incorporate NN based forward models for coastal waters, which use multi-parameter bio-optical models. In addition, aerosols are represented by six components, i.e., fine mode non absorbing insoluble (FNAI), brown carbon (BrC), black carbon (BC), fine mode non absorbing soluble (FNAS), sea salt (SS) and non-spherical dust (Dust). Sea salt and dust are coarse mode aerosols, while the other components are in the fine mode. The sizes and spectral refractive indices are fixed for each aerosol component, while their abundances are retrievable. The multi-parameter bio-optical model and aerosol components are chosen to represent the coastal marine environment. The retrieval algorithm is applied to synthetic measurements in three different configurations ofMAPs in the PACE mission: HARP2 observations only, SPEXone observations only and combined HARP2 and SPEXone observations. The retrieval results from synthetic measurements show that for aerosol retrieval the SPEXone-only configuration works equally well with the HAPR2-only configuration. On the other hand, for ocean color retrieval the SPEXone instrument provides better information due to its larger spectral coverage. For the surface parameters (wind speed), HARP2 measurements provide better information due to its wide field of view. Combined measurement configuration HARP2+SPEXone performed the best to retrieve all aerosol, ocean color and surface parameters. We also studied the impact of sun glint to aerosol and ocean color retrievals. The retrieval test revealed that wind speed and absorbing aerosol retrieval improves significantly when including measurements at glint geometries. Furthermore, the retrieval algorithm is equipped with modules for atmospheric correction and bidirectional reflectance distribution (BRDF) correction to obtain the remote sensing reflectance, which enables ocean biogeochemistry studies using the PACE polarimeter data.

PACE↗

Surface Emissivity Retrieved with Satellite Ultraspectral IR Measurements for Monitoring Global Change

Surface and atmospheric thermodynamic parameters retrieved with advanced ultraspectral remote sensors aboard Earth observing satellites are critical to general atmospheric and Earth science research, climate monitoring, and weather prediction. Ultraspectral resolution infrared radiance obtained from nadir observations provide atmospheric, surface, and cloud information. Presented here is the global surface IR emissivity retrieved from Infrared Atmospheric Sounding Interferometer (IASI) measurements under "clear-sky" conditions. Fast radiative transfer models, applied to the cloud-free (or clouded) atmosphere, are used for atmospheric profile and surface parameter (or cloud parameter) retrieval. The inversion scheme, dealing with cloudy as well as cloud-free radiances observed with ultraspectral infrared sounders, has been developed to simultaneously retrieve atmospheric thermodynamic and surface (or cloud microphysical) parameters. Rapidly produced surface emissivity is initially evaluated through quality control checks on the retrievals of other impacted atmospheric and surface parameters. Surface emissivity and surface skin temperature from the current and future operational satellites can and will reveal critical information on the Earth s ecosystem and land surface type properties, which can be utilized as part of long-term monitoring for the Earth s environment and global climate change.

Zhou, Daniel K.↗

Use of Collocated KWAJEX Satellite, Aircraft, and Ground Measurements for Understanding Ambiguities in TRMM Radiometer Rain Profile Algorithm

Coordinated ground, aircraft, and satellite observations are analyzed from the 1999 TRMM Kwajalein Atoll field experiment (KWAJEX) to better understand the relationships between cloud microphysical processes and microwave radiation intensities in the context of physical evaluation of the Level 2 TRMM radiometer rain profile algorithm and uncertainties with its assumed microphysics-radiation relationships. This talk focuses on the results of a multi-dataset analysis based on measurements from KWAJEX surface, air, and satellite platforms to test the hypothesis that uncertainties in the passive microwave radiometer algorithm (TMI 2a12 in the nomenclature of TRMM) are systematically coupled and correlated with the magnitudes of deviation of the assumed 3-dimensional microphysical properties from observed microphysical properties. Re-stated, this study focuses on identifying the weaknesses in the operational TRMM 2a12 radiometer algorithm based on observed microphysics and radiation data in terms of over-simplifications used in its theoretical microphysical underpinnings. The analysis makes use of a common transform coordinate system derived from the measuring capabilities of the aircraft radiometer used to survey the experimental study area, i.e., the 4-channel AMPR radiometer flown on the NASA DC-8 aircraft. Normalized emission and scattering indices derived from radiometer brightness temperatures at the four measuring frequencies enable a 2-dimensional coordinate system that facilities compositing of Kwajalein S-band ground radar reflectivities, ARMAR Ku-band aircraft radar reflectivities, TMI spacecraft radiometer brightness temperatures, PR Ku-band spacecraft radar reflectivities, bulk microphysical parameters derived from the aircraft-mounted cloud microphysics laser probes (including liquid/ice water contents, effective liquid/ice hydrometeor radii, and effective liquid/ice hydrometeor variances), and rainrates derived from any of the individual ground, aircraft, or satellite algorithms applied to the radar or radiometer measurements, or their combination. The results support the study's underlying hypothesis, particularly in context of ice phase processes, in that the cloud regions where the 2a12 algorithm's microphysical database most misrepresents the microphysical conditions as determined by the laser probes, are where retrieved surface rainrates are most erroneous relative to other reference rainrates as determined by ground and aircraft radar. In reaching these conclusions, TMI and PR brightness temperatures and reflectivities have been synthesized from the aircraft AMPR and ARMAR measurements with the analysis conducted in a composite framework to eliminate measurement noise associated with the case study approach and single element volumes obfuscated by heterogeneous beam filling effects. In diagnosing the performance of the 2a12 algorithm, weaknesses have been found in the cloud-radiation database used to provide microphysical guidance to the algorithm for upper cloud ice microphysics. It is also necessary to adjust a fractional convective rainfall factor within the algorithm somewhat arbitrarily to achieve satisfactory algorithm accuracy.

Smith, Eric A.↗

Physical processes in polar stratospheric ice clouds

The formulation and evolution of polar stratospheric ice clouds are simulated using a one-dimensional model of cloud microphysics. It is found that the optical thickness and particle size of ice clouds depend on the cooling rate of the air in which the cloud formed. It is necessary that there be an energy barrier to ice nucleation upon the preexisting aerosols in order to account for the cooling rate dependence of the cloud properties.

Toon, Owen B.↗

Aerosol Models for the CALIPSO Lidar Inversion Algorithms

We use measurements and models to develop aerosol models for use in the inversion algorithms for the Cloud Aerosol Lidar and Imager Pathfinder Spaceborne Observations (CALIPSO). Radiance measurements and inversions of the AErosol RObotic NETwork (AERONET1, 2) are used to group global atmospheric aerosols using optical and microphysical parameters. This study uses more than 105 records of radiance measurements, aerosol size distributions, and complex refractive indices to generate the optical properties of the aerosol at more 200 sites worldwide. These properties together with the radiance measurements are then classified using classical clustering methods to group the sites according to the type of aerosol with the greatest frequency of occurrence at each site. Six significant clusters are identified: desert dust, biomass burning, urban industrial pollution, rural background, marine, and dirty pollution. Three of these are used in the CALIPSO aerosol models to characterize desert dust, biomass burning, and polluted continental aerosols. The CALIPSO aerosol model also uses the coarse mode of desert dust and the fine mode of biomass burning to build a polluted dust model. For marine aerosol, the CALIPSO aerosol model uses measurements from the SEAS experiment 3. In addition to categorizing the aerosol types, the cluster analysis provides all the column optical and microphysical properties for each cluster.

Omar, Ali H.↗